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1. 发明申请

US20110105776A1 METHOD FOR ELECTROCHEMICAL PRODUCTION OF A CRYSTALLINE POROUS METAL ORGANIC SKELETON MATERIAL 有权
标题翻译：电铸多孔金属有机硅材料的电化学生产方法
公开(公告)号：US20110105776A1
公开(公告)日：2011-05-05
申请号：US12987548
申请日：2011-01-10
申请人： Ulrich Müller , Hermann Pütter , Michael Hesse , Markus Schubert , Helge Wessel , Jürgen Huff , Marcus Guzmann
发明人： Ulrich Müller , Hermann Pütter , Michael Hesse , Markus Schubert , Helge Wessel , Jürgen Huff , Marcus Guzmann
IPC分类号： C07F1/08 , C07F3/06 , C07F15/06 , C07C229/34 , C07F3/02 , C25B3/12
CPC分类号： C25B3/12 , B01D53/02 , B01D2253/204 , B01J20/226 , B01J20/28014 , B01J20/28042 , B01J31/1691 , B01J31/1805 , B01J31/1815 , B01J31/2239 , B01J31/226 , B01J2531/16 , B01J2531/26 , B01J2531/842 , C01B3/0015 , C01B21/0455 , C01B23/0057 , F17C11/005 , H01M8/04216 , Y02C10/08 , Y02E60/327 , Y02E60/328 , Y02P20/133 , Y02P70/56 , Y10S95/90 , Y10S502/526
摘要： A method of electrochemically preparing a crystalline, porous, metal-organic framework material comprising at least one at least bidentate organic compound coordinately bound to at least one metal ion, in a reaction medium comprising the at least one bidentate organic compound, wherein at least one metal ion is provided in the reaction medium by the oxidation of one anode comprising the corresponding metal.
摘要翻译：一种在包含至少一种二齿有机化合物的反应介质中电化学制备结晶多孔的金属 - 有机骨架材料的方法，其包含与至少一种金属离子配位结合的至少二齿有机化合物，其中至少一种金属离子通过包含相应金属的一个阳极的氧化在反应介质中提供。

2. 发明申请

US20090171107A1 PROCESS FOR PREPARING POROUS METAL ORGANIC FRAMEWORKS 有权
标题翻译：制备多孔金属有机框架的方法
公开(公告)号：US20090171107A1
公开(公告)日：2009-07-02
申请号：US12300902
申请日：2007-05-11
申请人： Hermann Pütter , Markus Schubert , Ingo Richter , Ulrich Müller , Natalia Trukhan
发明人： Hermann Pütter , Markus Schubert , Ingo Richter , Ulrich Müller , Natalia Trukhan
IPC分类号： C07F1/08
CPC分类号： C25B3/12
摘要： The present invention relates to a process for preparing a porous metal organic framework comprising at least two organic compounds coordinated to at least one metal ion, which comprises the steps (a) oxidation of at least one anode comprising the metal corresponding to at least one metal ion in a reaction medium in the presence of at least one first organic compound which is an optionally substituted monocyclic, bicyclic or polycyclic saturated or unsaturated hydrocarbon in which at least two ring carbons have been replaced by heteroatoms selected from the group consisting of N, O and S to form a reaction intermediate comprising the at least one metal ion and the first organic compound; and (b) reaction of the reaction intermediate at a prescribed temperature with at least one second organic compound which coordinates to the at least one metal ion, with the second organic compound being derived from a dicarboxylic, tricarboxylic or tetracarboxylic acid.
摘要翻译：本发明涉及一种制备多孔金属有机骨架的方法，所述多孔金属有机骨架包括与至少一种金属离子配位的至少两种有机化合物，其包括以下步骤：（a）至少一个阳极的氧化，所述至少一个阳极包含对应于至少一种金属在至少一种第一有机化合物存在下的反应介质中，所述第一有机化合物是任选取代的单环，双环或多环饱和或不饱和烃，其中至少两个环碳已经被选自N，O 和S形成包含所述至少一种金属离子和所述第一有机化合物的反应中间体; 和（b）将反应中间体在规定温度下与至少一种与至少一种金属离子配位的第二有机化合物反应，第二有机化合物衍生自二羧酸，三羧酸或四羧酸。

3. 发明授权

US07879221B2 Process for preparing porous metal organic frameworks 有权
标题翻译：制备多孔金属有机骨架的方法
公开(公告)号：US07879221B2
公开(公告)日：2011-02-01
申请号：US12300902
申请日：2007-05-11
申请人： Hermann Pütter , Markus Schubert , Ingo Richter , Ulrich Müller , Natalia Trukhan
发明人： Hermann Pütter , Markus Schubert , Ingo Richter , Ulrich Müller , Natalia Trukhan
IPC分类号： C25B3/12 , C07F15/00 , C07F3/00
CPC分类号： C25B3/12
摘要： The present invention relates to a process for preparing a porous metal organic framework comprising at least two organic compounds coordinated to at least one metal ion, which comprises the steps (a) oxidation of at least one anode comprising the metal corresponding to at least one metal ion in a reaction medium in the presence of at least one first organic compound which is an optionally substituted monocyclic, bicyclic or polycyclic saturated or unsaturated hydrocarbon in which at least two ring carbons have been replaced by heteroatoms selected from the group consisting of N, O and S to form a reaction intermediate comprising the at least one metal ion and the first organic compound; and (b) reaction of the reaction intermediate at a prescribed temperature with at least one second organic compound which coordinates to the at least one metal ion, with the second organic compound being derived from a dicarboxylic, tricarboxylic or tetracarboxylic acid.
摘要翻译：本发明涉及一种制备多孔金属有机骨架的方法，所述多孔金属有机骨架包括与至少一种金属离子配位的至少两种有机化合物，其包括以下步骤：（a）至少一个阳极的氧化，所述至少一个阳极包含对应于至少一种金属在至少一种第一有机化合物存在下的反应介质中，所述第一有机化合物是任选取代的单环，双环或多环饱和或不饱和烃，其中至少两个环碳已经被选自N，O 和S形成包含所述至少一种金属离子和所述第一有机化合物的反应中间体; 和（b）将反应中间体在规定温度下与至少一种与至少一种金属离子配位的第二有机化合物反应，第二有机化合物衍生自二羧酸，三羧酸或四羧酸。

4. 发明授权

US07343747B2 Metal-organic framework materials for gaseous hydrocarbon storage 失效
标题翻译：用于气态碳氢化合物储存的金属 - 有机骨架材料
公开(公告)号：US07343747B2
公开(公告)日：2008-03-18
申请号：US11062861
申请日：2005-02-23
申请人： Ulrich Müller , Michael Hesse , Hermann Pütter , Omar M. Yaghi
发明人： Ulrich Müller , Michael Hesse , Hermann Pütter , Omar M. Yaghi
IPC分类号： F17C3/08 , B01D59/26 , B01D53/02
CPC分类号： F17C11/007 , Y10S502/50
摘要： The present invention relates to a method of storing a liquefied gas in a container containing a metal-organic framework material, the container filled with such a gas, a process for filling container and the use of the container to release the gas.
摘要翻译：本发明涉及一种将液化气体储存在容纳金属 - 有机骨架材料的容器中，装有这种气体的容器，用于填充容器的方法以及使用容器释放气体的方法。

5. 发明授权

US08057584B2 Pressurised gas container or storage means containing a gas pressurised container with filter means 有权
标题翻译：加压气体容器或包含具有过滤装置的气体加压容器的储存装置
公开(公告)号：US08057584B2
公开(公告)日：2011-11-15
申请号：US12299330
申请日：2007-04-26
申请人： Markus Schubert , Ulrich Müller , Michael Hesse , Kerstin Schierle-Arndt , Kai Oertel , Ian Faye , Thorsten Allgeier , Jan-Michael Graehn
发明人： Markus Schubert , Ulrich Müller , Michael Hesse , Kerstin Schierle-Arndt , Kai Oertel , Ian Faye , Thorsten Allgeier , Jan-Michael Graehn
IPC分类号： F17C11/00 , B01D53/02
CPC分类号： F17C11/005 , F17C11/007 , F17C2205/0341 , F17C2270/0168 , Y10S502/526
摘要： Hydrogen or methane gas pressure container having a minimum volume of 1 m3 a prescribed maximum filling pressure, has a filter through which oxygen, methane respectively, can flow during uptake. The filter has an adsorbent for adsorbing impurities selected from the group consisting of a higher hydrocarbon, ammonia, an odorous substance, hydrogen sulfide and a mixture of two or more of these substances. The pressure container and the filter comprise porous metal organic frameworks as adsorbent.
摘要翻译：具有规定的最大填充压力的最小体积为1m 3的氢气或甲烷气体压力容器具有分别在吸收期间氧气，甲烷可以通过其的过滤器。过滤器具有用于吸附选自高级烃，氨，恶臭物质，硫化氢和这些物质中的两种或更多种的混合物的杂质的吸附剂。压力容器和过滤器包括作为吸附剂的多孔金属有机骨架。

6. 发明申请

US20120091064A1 PROCESS FOR PREPARING POROUS METAL-ORGANIC FRAMEWORK MATERIALS 有权
标题翻译：制备多孔金属有机框架材料的方法
公开(公告)号：US20120091064A1
公开(公告)日：2012-04-19
申请号：US13336396
申请日：2011-12-23
申请人： Markus SCHUBERT , Ulrich Müller , Michael Hesse , Uwe Diehlmann
发明人： Markus SCHUBERT , Ulrich Müller , Michael Hesse , Uwe Diehlmann
IPC分类号： B01J20/28 , B01D53/02 , B01D15/00 , C07F1/08
CPC分类号： C07C51/418 , C07C63/307
摘要： The present invention relates to a method for producing a porous metal-organic framework material comprising the stepreacting a reaction mixture in the liquid phase of at least one copper compound having at least one at least bidentate, organic compound which can bind by coordination to the copper in the presence of a nonaqueous solvent, the at least one at least bidentate, organic compound being derived from a polycarboxylic acid having at least three carboxyl groups, and the reaction proceeding at atmospheric pressure above 80° C.
摘要翻译：本发明涉及多孔金属 - 有机骨架材料的制造方法，该方法包括使具有至少一种至少二齿的有机化合物的至少一种铜化合物的液相中的反应混合物反应，该有机化合物可通过配位与铜在非水溶剂的存在下，所述至少一种至少二齿的有机化合物衍生自具有至少三个羧基的多元羧酸，并且所述反应在大气压下高于80℃进行。

7. 发明授权

US08518264B2 Method of using a metal organic frameworks based on aluminum fumarate 有权
标题翻译：使用富马酸铝的金属有机骨架的方法
公开(公告)号：US08518264B2
公开(公告)日：2013-08-27
申请号：US13347212
申请日：2012-01-10
申请人： Christoph Kiener , Ulrich Müller , Markus Schubert
发明人： Christoph Kiener , Ulrich Müller , Markus Schubert
IPC分类号： B01D15/00
CPC分类号： B01J20/0211 , B01J20/226 , B01J20/28042 , B01J20/28066 , B01J20/3085 , B01J31/1691 , B01J31/2239 , B01J2231/48 , B01J2231/72 , B01J2531/31 , C01B3/001 , C01B3/508 , C07C51/418 , Y02C10/08 , Y02E60/324 , Y10T428/249953 , C07C63/38 , C07C57/15 , C07C63/26
摘要： A method comprising (i) providing a metal organic framework formed by AlIII ions to which fumarate ions are coordinated to produce a porous framework structure, (ii) bringing a substance into contact with the metal organic framework such that the substance is uptaken by the porous metal organic framework to provide storage of or controlled release of, the substance.
摘要翻译：一种方法，包括（i）提供由AlIII离子形成的金属有机骨架，其中富马酸根离子被配位以产生多孔骨架结构，（ii）使物质与金属有机骨架接触，使得物质被多孔金属有机骨架提供物质的储存或控制释放。

8. 发明授权

US08501150B2 Metal oxides from metal-organic framework materials 失效
标题翻译：金属 - 有机骨架材料的金属氧化物
公开(公告)号：US08501150B2
公开(公告)日：2013-08-06
申请号：US12297298
申请日：2007-04-12
申请人： Markus Schubert , Ulrich Müller , Natalia Trukhan
发明人： Markus Schubert , Ulrich Müller , Natalia Trukhan
IPC分类号： C01F7/02 , C01B13/14
CPC分类号： B01J20/0211 , B01J20/041 , B01J20/06 , B01J20/08 , B01J20/28042 , B01J20/28057 , C01F5/02 , C01F7/30 , C01G1/02 , C01G9/02 , C01G23/047 , C01G25/00 , C01G25/02 , C01P2002/72 , C01P2004/03 , C01P2006/12 , C01P2006/13 , C07C51/418 , Y10T428/2982 , C07C63/38 , C07C63/26 , C07C57/15
摘要： The present invention relates to a method for producing a metal oxide by heating a porous metal-organic framework material, the framework material comprising at least one at least bidentate organic compound bound to at least one metal ion by coordination, and the metal ion being selected from the metals comprising groups 2 to 4 and 13 of the Periodic Table of the Elements, above the complete decomposition temperature of the framework material, and also to metal oxides obtainable by this method, and to the use thereof.
摘要翻译：本发明涉及通过加热多孔金属 - 有机骨架材料来生产金属氧化物的方法，所述骨架材料包含至少一种至少二齿有机化合物，其通过配位与至少一种金属离子结合，并且选择金属离子包括元素周期表第2至4和13族的金属，高于骨架材料的完全分解温度，以及可通过该方法获得的金属氧化物及其用途。

9. 发明申请

US20090312591A1 METHOD FOR PRODUCING PROPENE FROM PROPANE 审中-公开
标题翻译：从丙烷生产丙烯的方法
公开(公告)号：US20090312591A1
公开(公告)日：2009-12-17
申请号：US12294748
申请日：2007-03-13
申请人： Markus Schubert , Ulrich Müller , Christoph Kiener , Friedhalm Teich , Sven Crone , Falk Simon , Jörg Pastre
发明人： Markus Schubert , Ulrich Müller , Christoph Kiener , Friedhalm Teich , Sven Crone , Falk Simon , Jörg Pastre
IPC分类号： C07C5/327
CPC分类号： C07C5/333 , C07C7/12 , C07C7/13 , C07C11/06
摘要： The present invention relates to processes for preparing propene from propane, comprising the steps: A) a feed gas stream a comprising propane is provided; B) the feed gas stream a comprising propane, if appropriate steam and if appropriate and an oxygenous gas stream are fed into a dehydrogenation zone and propane is subjected to a dehydrogenation to propene to obtain a product gas stream b comprising propane, propene, methane, ethane, ethene, hydrogen, if appropriate carbon monoxide, carbon dioxide, steam and oxygen; C) the product gas stream b is cooled, if appropriate compressed and steam is removed by condensation to obtain a steam-depleted product gas stream c; D) the product gas stream c is contacted with a selective adsorbent which adsorbs propene selectively under the selected adsorption conditions to obtain a propene-laden adsorbent and a propene-depleted gas stream d2 comprising propane, methane, ethane, ethene and hydrogen, carbon monoxide and carbon dioxide; E) a propene-comprising gas stream e1 is released from the propane-laden adsorbent by pressure reduction and/or heating of the adsorbent.
摘要翻译：本发明涉及从丙烷制备丙烯的方法，包括以下步骤：A）提供包含丙烷的原料气流a; B）包含丙烷的进料气流a（如果合适的话，蒸汽和适当的话）和含氧气流被送入脱氢区，丙烷经脱氢至丙烯以获得包含丙烷，丙烯，甲烷，乙烷，乙烯，氢气，如果适用，一氧化碳，二氧化碳，蒸气和氧气; C）产物气流b被冷却，如果合适的话压缩并通过冷凝除去蒸汽，得到蒸汽消耗产物气流c; D）产物气流c与在选择的吸附条件下选择性吸附丙烯的选择性吸附剂接触以获得含有丙烯的吸附剂和包含丙烷，甲烷，乙烷，乙烯和氢气的一种贫含丙烯的气流d2，一氧化碳和二氧化碳; E）通过吸附剂的减压和/或加热将含丙烯气流e1从载有丙烷的吸附剂中释放。

10. 发明申请

US20090281341A1 METAL-ORGANIC ZIRCONIUM-BASED FRAMEWORK MATERIALS 审中-公开
标题翻译：金属有机基于ZIRCONIUM的框架材料
公开(公告)号：US20090281341A1
公开(公告)日：2009-11-12
申请号：US12297294
申请日：2007-04-17
申请人： Markus Schubert , Ulrich Müller , Stefan Marx
发明人： Markus Schubert , Ulrich Müller , Stefan Marx
IPC分类号： C07F7/00
CPC分类号： C07C51/412 , C07C29/70 , C07F7/003 , C07C63/28 , C07C63/14
摘要： The present invention relates to a porous metal-organic framework material comprising at least one at least bidentate organic compound which is bound to at least one metal ion by coordination, the at least one metal ion being zirconium, and the at least one at least bidentate organic compound being derived from a dicarboxylic, tricarboxylic or tetracarboxylic acid. In addition, the invention relates to methods for production thereof and also use thereof.
摘要翻译：多孔金属 - 有机骨架材料本发明涉及多孔金属 - 有机骨架材料，其包含至少一种至少二齿有机化合物，其通过配位与至少一种金属离子结合，所述至少一种金属离子是锆，以及所述至少一种至少二齿有机化合物衍生自二羧酸，三羧酸或四羧酸。此外，本发明涉及其生产方法及其用途。

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