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1. 发明授权

US07307131B2 Fluorinated allyl ether polymer 有权
标题翻译：氟化烯丙基醚聚合物
公开(公告)号：US07307131B2
公开(公告)日：2007-12-11
申请号：US11043976
申请日：2005-01-28
申请人： Shigeru Morita , Hirotoshi Sakashita , Takayuki Araki , Tetsuo Shimizu
发明人： Shigeru Morita , Hirotoshi Sakashita , Takayuki Araki , Tetsuo Shimizu
IPC分类号： C08F18/20
CPC分类号： C08F16/24 , C08F290/062
摘要： A fluorine-containing allyl ether polymer having a number average molecular weight of 1,000 to 1,000,000 and consisting of chains of at least one repeating unit of the formula: wherein A is an organic group having 1 to 100 carbon atoms.
摘要翻译：一种数均分子量为1,000至1,000,000的含氟烯丙基醚聚合物，由至少一种下式重复单元的链组成：其中A为具有1至100个碳原子的有机基团。

2. 发明授权

US06930159B1 Fluorinated allyl ether polymer 有权
标题翻译：氟化烯丙基醚聚合物
公开(公告)号：US06930159B1
公开(公告)日：2005-08-16
申请号：US09936495
申请日：2000-03-10
申请人： Shigeru Morita , Hirotoshi Sakashita , Takayuki Araki , Tetsuo Shimizu
发明人： Shigeru Morita , Hirotoshi Sakashita , Takayuki Araki , Tetsuo Shimizu
IPC分类号： C08F16/24 , C08F290/06 , C08F120/22
CPC分类号： C08F16/24 , C08F290/062
摘要： A fluorine-containing allyl ether polymer having a number average molecular weight of 1,000 to 1,000,000 and consisting of chains of at least one repeating unit of the formula: wherein A is an organic group having 1 to 100 carbon atoms.
摘要翻译：一种数均分子量为1,000至1,000,000的含氟烯丙基醚聚合物，由至少一种下式重复单元的链组成：其中A为具有1至100个碳原子的有机基团。

3. 发明申请

US20050131145A1 Fluorinated allyl ether polymer 有权
公开(公告)号：US20050131145A1
公开(公告)日：2005-06-16
申请号：US11043976
申请日：2005-01-28
申请人： Shigeru Morita , Hirotoshi Sakashita , Takayuki Araki , Tetsuo Shimizu
发明人： Shigeru Morita , Hirotoshi Sakashita , Takayuki Araki , Tetsuo Shimizu
IPC分类号： C08F16/24 , C08F290/06 , C08L67/02
CPC分类号： C08F16/24 , C08F290/062
摘要： A fluorine-containing allyl ether polymer having a number average molecular weight of 1,000 to 1,000,000 and consisting of chains of at least one repeating unit of the formula: wherein A is an organic group having 1 to 100 carbon atoms.

4. 发明授权

US07455934B1 Fluorocopolymer material with sulfonic acid functional groups as a solid polyelectrolyte for use in fuel cells 有权
标题翻译：具有磺酸官能团的含氟共聚物材料作为用于燃料电池的固体聚电解质
公开(公告)号：US07455934B1
公开(公告)日：2008-11-25
申请号：US09700185
申请日：1999-05-10
申请人： Takayuki Araki , Noritoshi Oka , Yoshito Tanaka , Takayuki Nakamura , Tetsuo Shimizu
发明人： Takayuki Araki , Noritoshi Oka , Yoshito Tanaka , Takayuki Nakamura , Tetsuo Shimizu
IPC分类号： H01M10/08
CPC分类号： H01S5/22 , C08J5/2237 , C08J2327/12 , G02B2006/12097 , G02B2006/12176 , H01B1/122 , H01M8/0289 , H01M8/1025 , H01M8/1039 , H01M8/1067 , H01S5/0655 , H01S5/20 , H01S5/2004 , H01S5/2213 , H01S5/2218 , H01S5/2227
摘要： The invention is a material for a solid polyelectrolyte, comprising a multi-segmented fluoropolymer that comprises a block copolymer and/or a graft copolymer, wherein the copolymer contains one or more blocks essentially consisting of segment A and one or more blocks essentially consisting of segment B, the segment A combines with the segment B, wherein the segment A has a molecular weight of 5,000 to 1,000.000, and the Segment A is a copolymer chain comprising (a) an ethylenicfluoromonomer containing sulfonic acid functional groups each represented by Formula (1) CX2═CX1—(O)n—Rf—SO2Y, wherein X and X1 may be the same or different and are each hydrogen or fluorine; Y is FI, Cl, or OY1 wherein y1 is hydrogen, alkali metal or C1-C5 alkyl; Rf is C1 to C40 divalent fluoroalkylene or C1 to C40 divalent fluoroalkylene having one or more ether bonds; and n is 0 or 1; and (b) at least one type of ethylenic fluoromonomer copolymerizable with the ethylenic fluoromonomer (a) and containing no sulfonic acid functional groups, the segment B is a fluoropolymer containing no sulfonic acid functional groups, has a molecular weight of 3,000 to 1,200,000, and has a crystalline melting point of 100° C. or higher or a glass transition point of 100° C. or higher, wherein the ratio of segment A:segment B in the segmented fluoropolymer is 5:9˜to 98:2 30:70 to 90:10 wt. %.
摘要翻译：本发明是用于固体聚电解质的材料，其包含多段含氟聚合物，其包含嵌段共聚物和/或接枝共聚物，其中所述共聚物含有一个或多个基本上由片段A组成的嵌段和一个或多个基本上由片段 B，段A与段B结合，其中段A的分子量为5,000〜1,000.000，段A为共聚物链，其包含（a）含有各自由式（1）表示的磺酸官能团的烯键式氟单体， CX 2 - - - - - - - - - - - - - - - - - - - - - - - - - - - - （O） SUP> 1可以相同或不同，分别为氢或氟; Y是FI，Cl或OY 1，其中y 1是氢，碱金属或C 1 -C 5 烷基; Rf是C 1至C 40二价氟代亚烷基或C 1至C 40二价氟代亚烷基，其具有一个或多个醚债券并且n为0或1; 和（b）至少一种可与烯属含氟单体（a）共聚并且不含磺酸官能团的烯属含氟单体，段B是不含磺酸官能团的含氟聚合物，分子量为3,000至1,200,000，具有100℃以上的结晶熔点或100℃以上的玻璃化转变温度，其中分段含氟聚合物中A段：B段的比例为5:9〜98:2 30:70 至90:10重量％。

5. 发明授权

US5986150A Fluorine-containing olefin, fluorine-containing polymer and thermoplastic resin composition prepared by using said polymer 失效
标题翻译：含氟烯烃，含氟聚合物和通过使用所述聚合物制备的热塑性树脂组合物
公开(公告)号：US5986150A
公开(公告)日：1999-11-16
申请号：US856594
申请日：1997-05-15
申请人： Takayuki Araki , Tetsuo Shimizu , Takafumi Yamato , Masahiro Kumegawa , Yoshihisa Yamamoto
发明人： Takayuki Araki , Tetsuo Shimizu , Takafumi Yamato , Masahiro Kumegawa , Yoshihisa Yamamoto
IPC分类号： C07C33/42 , C07C43/178 , C07C57/52 , C07C69/708 , C07D303/24 , C08F14/18 , C08F214/18 , C08F216/14 , C08F220/22 , C08L27/12 , C08L67/00 , C08L67/02 , C08L69/00 , C08L77/00 , C07C41/00 , C07D303/08
CPC分类号： C08L27/12 , C07C33/423 , C07C43/178 , C07C57/52 , C07C69/708 , C07D303/24 , C08F14/185 , C08F214/184 , C08L67/00 , C08L67/02 , C08L69/00 , C08L2205/02 , C08L77/00
摘要： To provide a fluorine-containing olefin represented, for example, by CH.sub.2 .dbd.CFCF.sub.2 --R.sub.f.sup.6 --(CH.sub.2).sub.k --X.sup.2 [wherein, X.sup.2 is ##STR1## R.sub.f.sup.6 is a fluorine-substituted fluorine-containing alkyl group having 1 to 40 carbon atoms or --OR.sub.f.sup.7 --(Rf.sup.7 is a fluorine-substituted fluorine-containing alkyl group having 1 to 40 carbon atoms or a fluorine-substituted fluorine-containing ether group having 3 to 50 carbon atoms), k is 0 or an integer of 1 to 6]; a fluorine-containing polymer with functional group which is prepared by polymerizing the above-mentioned olefin, has good affinity with various heat-resisting thermoplastic resins and is capable of forming homogeneous dispersion with the thermoplastic resin; and a thermoplastic resin composition comprising the above-mentioned fluorine-containing polymer with functional group and an aromatic polyester or the like as the heat-resisting thermoplastic resin.
摘要翻译：提供例如通过CH 2 = CFCF 2 -R f 6 - （CH 2）k -X 2表示的含氟烯烃[其中，X 2是Rf 6是具有1〜40个碳原子的氟取代的含氟烷基或-OR f7 - （Rf7为碳原子数为1〜40的氟取代的含氟烷基或碳原子数为3〜50的氟取代的含氟醚基），k为0或1〜6的整数]。通过聚合上述烯烃制备的具有官能团的含氟聚合物与各种耐热性热塑性树脂具有良好的亲和性，并且能够与热塑性树脂形成均匀的分散体; 以及包含上述具有官能团的含氟聚合物和芳族聚酯等作为耐热性热塑性树脂的热塑性树脂组合物。

6. 发明授权

US5869574A Thermoplastic resin composition 失效
公开(公告)号：US5869574A
公开(公告)日：1999-02-09
申请号：US838063
申请日：1997-04-17
申请人： Tetsuo Shimizu , Yoshihisa Yamamoto , Seitaro Yamaguchi , Nobuhiko Tsuda , Noriyasu Yamane , Takafumi Yamato , Masahiro Kumegawa , Takayuki Araki
发明人： Tetsuo Shimizu , Yoshihisa Yamamoto , Seitaro Yamaguchi , Nobuhiko Tsuda , Noriyasu Yamane , Takafumi Yamato , Masahiro Kumegawa , Takayuki Araki
IPC分类号： C08G59/30 , C08G59/32 , C08G61/12 , C08L27/12 , C08L27/16 , C08L67/00 , C08L67/02 , C08L67/03 , C08L69/00 , C08L71/10 , C08L77/00 , C08L77/02 , C08L77/06 , C08L81/04 , C08L101/00
CPC分类号： C08L77/06 , C08G59/30 , C08G59/3254 , C08G61/12 , C08L101/00 , C08L27/12 , C08L27/16 , C08L67/00 , C08L67/02 , C08L67/03 , C08L69/00 , C08L77/00 , C08L77/02 , C08L81/04 , C08L2201/00
摘要： A thermoplastic resin composition comprising a blend obtainable by blending 0.1 to 99% by weight of (a) a fluorine-containing polymer having a number-average molecular weight of 2000 to 1000000 and having hydroxy group or epoxy group at least at one of end portions of a main chain and side chain of the polymer, and 1 to 99.9% by weight of (b) a heat resisting thermoplastic resin having a crystalline melting point or glass transition temperature of not less than 150.degree. C. The present invention can provide a composition comprising various heat resisting thermoplastic resins and a fluorine-containing polymer having a functional group which is capable of developing an affinity with said resins and forming a uniform dispersion.

7. 发明授权

US5767198A Thermoplastic resin composition 失效
标题翻译：热塑性树脂组合物
公开(公告)号：US5767198A
公开(公告)日：1998-06-16
申请号：US564243
申请日：1995-12-20
申请人： Tetsuo Shimizu , Takayuki Araki , Takafumi Yamato , Yoshihisa Yamamoto
发明人： Tetsuo Shimizu , Takayuki Araki , Takafumi Yamato , Yoshihisa Yamamoto
IPC分类号： C08L27/12 , C08L27/18 , C08L67/00 , C08L67/02 , C08L67/04 , C08L67/03
CPC分类号： C08L27/12 , C08L27/18 , C08L67/00 , C08L67/02 , C08L67/04
摘要： To provide a thermoplastic resin composition which comprises a fluorine-containing polymer having a molecular weight of 5.times.10.sup.2 to 5.times.10.sup.5 and 2.times.10.sup.2 to 1.times.10.sup.5 methylol groups per 1.times.10.sup.6 carbon atoms at its molecular chain ends and a liquid crystal polyester or in addition a perfluoro type resin having less than 2.times.10.sup.2 methylol groups mentioned above, and has improved shrinkage from mold dimensions and dimensional stability represented by a coefficient of linear expansion with maintaining excellent characteristics of the fluorine-containing resin, such as thermal resistance, chemical resistance, weather resistance, surface properties (non-stickiness, excellent friction property), antisoil property and dielectric property.
摘要翻译： PCT No.PCT / JP95 / 00833 Sec。 371 1995年12月20日第 102（e）1995年12月20日日期PCT提交1995年4月26日PCT公布。 WO95 / 29956 PCT公开号日期：1995年11月9日提供一种热塑性树脂组合物，其包含分子链末端分子量为5×10 2〜5×10 5的含氟聚合物和1×10 6个碳原子的2×102〜1×10 5个羟甲基，以及液晶聚酯，具有上述小于2×102羟甲基的全氟型树脂，并且通过保持含氟树脂的优异特性，例如耐热性，耐化学性，耐候性，由模具尺寸和线性膨胀系数表示的尺寸稳定性提高了收缩率，表面性（不粘性，优异的摩擦性），防垢性和介电性。

8. 发明授权

US07087679B2 Thermoplastic resin composition 失效
标题翻译：热塑性树脂组合物
公开(公告)号：US07087679B2
公开(公告)日：2006-08-08
申请号：US10334066
申请日：2002-12-31
申请人： Tetsuo Shimizu , Yoshihisa Yamamoto , Seitaro Yamaguchi , Nobuhiko Tsuda , Noriyasu Yamane , Takafumi Yamato , Masahiro Kumegawa , Takayuki Araki
发明人： Tetsuo Shimizu , Yoshihisa Yamamoto , Seitaro Yamaguchi , Nobuhiko Tsuda , Noriyasu Yamane , Takafumi Yamato , Masahiro Kumegawa , Takayuki Araki
IPC分类号： C08L27/02 , C08L67/02 , C08L69/00 , C08L71/00 , C08L79/00
CPC分类号： C08L77/06 , C08G59/30 , C08G59/3254 , C08G61/12 , C08L27/12 , C08L27/16 , C08L67/00 , C08L67/02 , C08L67/03 , C08L69/00 , C08L77/00 , C08L77/02 , C08L81/04 , C08L101/00 , C08L2201/00 , C08L2666/02 , C08L2666/04 , C08L27/00 , C08L2666/14
摘要： A thermoplastic resin composition comprising a blend obtainable by blending 0.1 to 99% by weight of (a) a fluorine-containing polymer having a number-average molecular weight of 2000 to 1000000 and having hydroxy group or epoxy group at least at one of end portions of a main chain and side chain of the polymer, and 1 to 99.9% by weight of (b) a heat resisting thermoplastic resin having a crystalline melting point or glass transition temperature of not less than 150° C. The present invention can provide a composition comprising various heat resisting thermoplastic resins and a fluorine-containing polymer having a functional group which is capable of developing an affinity with said resins and forming a uniform dispersion.
摘要翻译：一种热塑性树脂组合物，其包含通过将（a）数均分子量为2000〜1000000的含氟聚合物与至少一个末端部分具有羟基或环氧基的0.1〜99重量％的聚合物的主链和侧链，和1〜99.9重量％的（b）具有不低于150℃的结晶熔点或玻璃化转变温度的耐热性热塑性树脂。本发明可以提供一种包含各种耐热性热塑性树脂的组合物和具有能够与所述树脂形成亲和性并形成均匀分散体的官能团的含氟聚合物。

9. 发明申请

US20060008652A1 Curable fluorine-containing polymer, curable resin composition prepared from same and antireflection film 有权
公开(公告)号：US20060008652A1
公开(公告)日：2006-01-12
申请号：US11226355
申请日：2005-09-15
申请人： Takayuki Araki , Mihoko Ohashi , Yoshito Tanaka , Tetsuo Shimizu
发明人： Takayuki Araki , Mihoko Ohashi , Yoshito Tanaka , Tetsuo Shimizu
IPC分类号： B05D3/02 , B32B27/00 , C08F114/18 , C08F118/00
CPC分类号： C09D127/12 , C08F8/00 , C08F8/14 , C08F16/32 , C08F214/18 , C08F290/04 , Y10T428/3154 , C08F14/18
摘要： There are provided a curable fluorine-containing polymer which can realize a high hardness by photo-curing while maintaining a low refractive index, an antireflection film possessing improved scratch resistance and abrasion resistance while maintaining a reflection reducing effect, and an antireflection-treated article provided with such an antireflection film. The curable fluorine-containing polymer has a number average molecular weight of from 500 to 1,000,000 and is represented by the formula (1): AM (1) in which the structural unit M is a structural unit derived from a fluorine-containing ethylenic monomer and represented by the formula (M): wherein X1 and X2 are the same or different and each is H or F; X3 is H, F, CH3 or CF3; X4 and X5 are the same or different and each is H, F or CF3; Rf is an organic group in which 1 to 3 of Y1 (Y1 is a monovalent organic group having 2 to 10 carbon atoms and an ethylenic carbon-carbon double bond at its end) are bonded to a fluorine-containing alkyl group having 1 to 40 carbon atoms or a fluorine-containing alkyl group having 2 to 100 carbon atoms and ether bond; a is 0 or an integer of from 1 to 3; b and c are the same or different and each is 0 or 1, the structural unit A is a structural unit derived from a monomer copolymerizable with the fluorine-containing ethylenic monomer represented by the formula (M), and the structural unit M and the structural unit A are contained in amounts of from 0.1 to 100% by mole and from 0 to 99.9% by mole, respectively.

10. 发明授权

US06908724B2 Fluorine-containing polymer having acid-reactive group and chemically amplifying type photoresist composition prepared from same 有权
标题翻译：具有酸反应性基团的含氟聚合物和由其制备的化学放大型光致抗蚀剂组合物
公开(公告)号：US06908724B2
公开(公告)日：2005-06-21
申请号：US10262893
申请日：2002-10-03
申请人： Takayuki Araki , Meiten Koh , Yoshito Tanaka , Takuji Ishikawa , Hirokazu Aoyama , Tetsuo Shimizu
发明人： Takayuki Araki , Meiten Koh , Yoshito Tanaka , Takuji Ishikawa , Hirokazu Aoyama , Tetsuo Shimizu
IPC分类号： G03F7/004 , G03F7/038 , G03F7/039 , G03F7/075
CPC分类号： G03F7/039 , G03F7/0045 , G03F7/0046 , G03F7/0382 , G03F7/0392 , G03F7/0395 , G03F7/0397 , G03F7/0758 , Y10S430/106 , Y10S430/108
摘要： There is provided a novel fluorine-containing polymer having an acid-reactive group which has a high transparency against energy rays (radioactive rays) in a vacuum ultraviolet region (157 nm), and further there are provided a material for fluorine-containing base polymer prepared from the polymer and suitable for a photoresist and a chemically amplifying type resist composition obtained therefrom.The polymer has a number average molecular weight of from 1,000 to 1,000,000 and represented by the formula: —(M1)—(M2)—(A)—, wherein M1 is a structural unit having an acid-labile or acid-degradable functional group, M2 is a structural unit of fluorine-containing acryl ester, A is a structural unit derived from other copolymerizable monomer, the percent by mole ratio M1/M2 is 1 to 99/99 to 1 and the polymer comprises from 1 to 99% by mole of the structural unit M1, from 1 to 99% by mole of the structural unit M2 and from 0 to 98% by mole of the structural unit A1. The material for fluorine-containing base polymer comprises a fluorine-containing polymer having an acid-reactive group such as the above-mentioned polymer and is suitable for a photoresist, and the chemically amplifying type resist composition is obtained from those polymer and material.
摘要翻译：提供了一种具有酸反应性基团的新型含氟聚合物，其具有对真空紫外区域（157nm）中的能量射线（放射线）的高透明性，并且还提供了含氟基础聚合物由聚合物制备并适用于由其获得的光致抗蚀剂和化学放大型抗蚀剂组合物。聚合物的数均分子量为1,000〜1,000,000，由下式表示： - （M1） - （M2） - （A） - ，其中M1是具有酸不稳定性或酸可降解官能团的结构单元 M2是含氟丙烯酸酯的结构单元，A是来自其它可共聚单体的结构单元，M1 / M2的摩尔比为1〜99/99〜1，聚合物的含量为1〜99％结构单元M1的摩尔数，结构单元M2的1〜99摩尔％和结构单元A1的0〜98摩尔％。含氟基础聚合物的材料包括具有酸反应性基团的含氟聚合物如上述聚合物，并且适用于光致抗蚀剂，化学放大型抗蚀剂组合物由那些聚合物和材料获得。

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