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1. 发明授权

US06908724B2 Fluorine-containing polymer having acid-reactive group and chemically amplifying type photoresist composition prepared from same 有权
标题翻译：具有酸反应性基团的含氟聚合物和由其制备的化学放大型光致抗蚀剂组合物
公开(公告)号：US06908724B2
公开(公告)日：2005-06-21
申请号：US10262893
申请日：2002-10-03
申请人： Takayuki Araki , Meiten Koh , Yoshito Tanaka , Takuji Ishikawa , Hirokazu Aoyama , Tetsuo Shimizu
发明人： Takayuki Araki , Meiten Koh , Yoshito Tanaka , Takuji Ishikawa , Hirokazu Aoyama , Tetsuo Shimizu
IPC分类号： G03F7/004 , G03F7/038 , G03F7/039 , G03F7/075
CPC分类号： G03F7/039 , G03F7/0045 , G03F7/0046 , G03F7/0382 , G03F7/0392 , G03F7/0395 , G03F7/0397 , G03F7/0758 , Y10S430/106 , Y10S430/108
摘要： There is provided a novel fluorine-containing polymer having an acid-reactive group which has a high transparency against energy rays (radioactive rays) in a vacuum ultraviolet region (157 nm), and further there are provided a material for fluorine-containing base polymer prepared from the polymer and suitable for a photoresist and a chemically amplifying type resist composition obtained therefrom.The polymer has a number average molecular weight of from 1,000 to 1,000,000 and represented by the formula: —(M1)—(M2)—(A)—, wherein M1 is a structural unit having an acid-labile or acid-degradable functional group, M2 is a structural unit of fluorine-containing acryl ester, A is a structural unit derived from other copolymerizable monomer, the percent by mole ratio M1/M2 is 1 to 99/99 to 1 and the polymer comprises from 1 to 99% by mole of the structural unit M1, from 1 to 99% by mole of the structural unit M2 and from 0 to 98% by mole of the structural unit A1. The material for fluorine-containing base polymer comprises a fluorine-containing polymer having an acid-reactive group such as the above-mentioned polymer and is suitable for a photoresist, and the chemically amplifying type resist composition is obtained from those polymer and material.
摘要翻译：提供了一种具有酸反应性基团的新型含氟聚合物，其具有对真空紫外区域（157nm）中的能量射线（放射线）的高透明性，并且还提供了含氟基础聚合物由聚合物制备并适用于由其获得的光致抗蚀剂和化学放大型抗蚀剂组合物。聚合物的数均分子量为1,000〜1,000,000，由下式表示： - （M1） - （M2） - （A） - ，其中M1是具有酸不稳定性或酸可降解官能团的结构单元 M2是含氟丙烯酸酯的结构单元，A是来自其它可共聚单体的结构单元，M1 / M2的摩尔比为1〜99/99〜1，聚合物的含量为1〜99％结构单元M1的摩尔数，结构单元M2的1〜99摩尔％和结构单元A1的0〜98摩尔％。含氟基础聚合物的材料包括具有酸反应性基团的含氟聚合物如上述聚合物，并且适用于光致抗蚀剂，化学放大型抗蚀剂组合物由那些聚合物和材料获得。

2. 发明申请

US20050287471A1 Novel fluorine-containing polymer having acid-reactive group and chemically amplifying type photoresist composition prepared from same 审中-公开
标题翻译：具有酸反应性基团的新型含氟聚合物和由其制备的化学放大型光致抗蚀剂组合物
公开(公告)号：US20050287471A1
公开(公告)日：2005-12-29
申请号：US11033954
申请日：2005-01-13
申请人： Takayuki Araki , Meiten Koh , Yoshito Tanaka , Takuji Ishikawa , Hirokazu Aoyama , Tetsuo Shimizu
发明人： Takayuki Araki , Meiten Koh , Yoshito Tanaka , Takuji Ishikawa , Hirokazu Aoyama , Tetsuo Shimizu
IPC分类号： G03F7/004 , G03F7/038 , G03F7/039 , G03F7/075 , G03C1/76
CPC分类号： G03F7/039 , G03F7/0045 , G03F7/0046 , G03F7/0382 , G03F7/0392 , G03F7/0395 , G03F7/0397 , G03F7/0758 , Y10S430/106 , Y10S430/108
摘要： There is provided a novel fluorine-containing polymer having an acid-reactive group which has a high transparency against energy rays (radioactive rays) in a vacuum ultraviolet region (157 nm), and further there are provided a material for fluorine-containing base polymer prepared from the polymer and suitable for a photoresist and a chemically amplifying type resist composition obtained therefrom. The polymer has a number average molecular weight of from 1,000 to 1,000,000 and represented by the formula: -(M1)-(M2)-(A)-, wherein M1 is a structural unit having an acid-labile or acid-degradable functional group, M2 is a structural unit of fluorine-containing acryl ester, A is a structural unit derived from other copolymerizable monomer, the percent by mole ratio M1/M2 is 1 to 99/99 to 1 and the polymer comprises from 1 to 99% by mole of the structural unit M1, from 1 to 99% by mole of the structural unit M2 and from 0 to 98% by mole of the structural unit A1. The material for fluorine-containing base polymer comprises a fluorine-containing polymer having an acid-reactive group such as the above-mentioned polymer and is suitable for a photoresist, and the chemically amplifying type resist composition is obtained from those polymer and material.
摘要翻译：提供了一种具有酸反应性基团的新型含氟聚合物，其具有对真空紫外区域（157nm）中的能量射线（放射线）的高透明性，并且还提供了含氟基础聚合物由聚合物制备并适用于由其获得的光致抗蚀剂和化学放大型抗蚀剂组合物。聚合物的数均分子量为1,000〜1,000,000，由下式表示： - （M1） - （M2） - （A） - ，其中M1是具有酸不稳定性或酸可降解官能团的结构单元 M2是含氟丙烯酸酯的结构单元，A是来自其它可共聚单体的结构单元，M1 / M2的摩尔比为1〜99/99〜1，聚合物的含量为1〜99％结构单元M1的摩尔数，结构单元M2的1〜99摩尔％和结构单元A1的0〜98摩尔％。含氟基础聚合物的材料包括具有酸反应性基团的含氟聚合物如上述聚合物，并且适用于光致抗蚀剂，化学放大型抗蚀剂组合物由那些聚合物和材料获得。

3. 发明授权

US07455934B1 Fluorocopolymer material with sulfonic acid functional groups as a solid polyelectrolyte for use in fuel cells 有权
标题翻译：具有磺酸官能团的含氟共聚物材料作为用于燃料电池的固体聚电解质
公开(公告)号：US07455934B1
公开(公告)日：2008-11-25
申请号：US09700185
申请日：1999-05-10
申请人： Takayuki Araki , Noritoshi Oka , Yoshito Tanaka , Takayuki Nakamura , Tetsuo Shimizu
发明人： Takayuki Araki , Noritoshi Oka , Yoshito Tanaka , Takayuki Nakamura , Tetsuo Shimizu
IPC分类号： H01M10/08
CPC分类号： H01S5/22 , C08J5/2237 , C08J2327/12 , G02B2006/12097 , G02B2006/12176 , H01B1/122 , H01M8/0289 , H01M8/1025 , H01M8/1039 , H01M8/1067 , H01S5/0655 , H01S5/20 , H01S5/2004 , H01S5/2213 , H01S5/2218 , H01S5/2227
摘要： The invention is a material for a solid polyelectrolyte, comprising a multi-segmented fluoropolymer that comprises a block copolymer and/or a graft copolymer, wherein the copolymer contains one or more blocks essentially consisting of segment A and one or more blocks essentially consisting of segment B, the segment A combines with the segment B, wherein the segment A has a molecular weight of 5,000 to 1,000.000, and the Segment A is a copolymer chain comprising (a) an ethylenicfluoromonomer containing sulfonic acid functional groups each represented by Formula (1) CX2═CX1—(O)n—Rf—SO2Y, wherein X and X1 may be the same or different and are each hydrogen or fluorine; Y is FI, Cl, or OY1 wherein y1 is hydrogen, alkali metal or C1-C5 alkyl; Rf is C1 to C40 divalent fluoroalkylene or C1 to C40 divalent fluoroalkylene having one or more ether bonds; and n is 0 or 1; and (b) at least one type of ethylenic fluoromonomer copolymerizable with the ethylenic fluoromonomer (a) and containing no sulfonic acid functional groups, the segment B is a fluoropolymer containing no sulfonic acid functional groups, has a molecular weight of 3,000 to 1,200,000, and has a crystalline melting point of 100° C. or higher or a glass transition point of 100° C. or higher, wherein the ratio of segment A:segment B in the segmented fluoropolymer is 5:9˜to 98:2 30:70 to 90:10 wt. %.
摘要翻译：本发明是用于固体聚电解质的材料，其包含多段含氟聚合物，其包含嵌段共聚物和/或接枝共聚物，其中所述共聚物含有一个或多个基本上由片段A组成的嵌段和一个或多个基本上由片段 B，段A与段B结合，其中段A的分子量为5,000〜1,000.000，段A为共聚物链，其包含（a）含有各自由式（1）表示的磺酸官能团的烯键式氟单体， CX 2 - - - - - - - - - - - - - - - - - - - - - - - - - - - - （O） SUP> 1可以相同或不同，分别为氢或氟; Y是FI，Cl或OY 1，其中y 1是氢，碱金属或C 1 -C 5 烷基; Rf是C 1至C 40二价氟代亚烷基或C 1至C 40二价氟代亚烷基，其具有一个或多个醚债券并且n为0或1; 和（b）至少一种可与烯属含氟单体（a）共聚并且不含磺酸官能团的烯属含氟单体，段B是不含磺酸官能团的含氟聚合物，分子量为3,000至1,200,000，具有100℃以上的结晶熔点或100℃以上的玻璃化转变温度，其中分段含氟聚合物中A段：B段的比例为5:9〜98:2 30:70 至90:10重量％。

4. 发明申请

US20060008652A1 Curable fluorine-containing polymer, curable resin composition prepared from same and antireflection film 有权
公开(公告)号：US20060008652A1
公开(公告)日：2006-01-12
申请号：US11226355
申请日：2005-09-15
申请人： Takayuki Araki , Mihoko Ohashi , Yoshito Tanaka , Tetsuo Shimizu
发明人： Takayuki Araki , Mihoko Ohashi , Yoshito Tanaka , Tetsuo Shimizu
IPC分类号： B05D3/02 , B32B27/00 , C08F114/18 , C08F118/00
CPC分类号： C09D127/12 , C08F8/00 , C08F8/14 , C08F16/32 , C08F214/18 , C08F290/04 , Y10T428/3154 , C08F14/18
摘要： There are provided a curable fluorine-containing polymer which can realize a high hardness by photo-curing while maintaining a low refractive index, an antireflection film possessing improved scratch resistance and abrasion resistance while maintaining a reflection reducing effect, and an antireflection-treated article provided with such an antireflection film. The curable fluorine-containing polymer has a number average molecular weight of from 500 to 1,000,000 and is represented by the formula (1): AM (1) in which the structural unit M is a structural unit derived from a fluorine-containing ethylenic monomer and represented by the formula (M): wherein X1 and X2 are the same or different and each is H or F; X3 is H, F, CH3 or CF3; X4 and X5 are the same or different and each is H, F or CF3; Rf is an organic group in which 1 to 3 of Y1 (Y1 is a monovalent organic group having 2 to 10 carbon atoms and an ethylenic carbon-carbon double bond at its end) are bonded to a fluorine-containing alkyl group having 1 to 40 carbon atoms or a fluorine-containing alkyl group having 2 to 100 carbon atoms and ether bond; a is 0 or an integer of from 1 to 3; b and c are the same or different and each is 0 or 1, the structural unit A is a structural unit derived from a monomer copolymerizable with the fluorine-containing ethylenic monomer represented by the formula (M), and the structural unit M and the structural unit A are contained in amounts of from 0.1 to 100% by mole and from 0 to 99.9% by mole, respectively.

5. 发明授权

US06838139B2 Heat-resistant material and coating material for OA equipments having flexibility 有权
标题翻译：具有柔性的OA设备的耐热材料和涂料
公开(公告)号：US06838139B2
公开(公告)日：2005-01-04
申请号：US10241490
申请日：2002-09-12
申请人： Takayuki Araki , Yoshito Tanaka , Masahiro Kumegawa , Norihito Otsuki , Masami Kato , Tetsuo Shimizu
发明人： Takayuki Araki , Yoshito Tanaka , Masahiro Kumegawa , Norihito Otsuki , Masami Kato , Tetsuo Shimizu
IPC分类号： C08F214/26 , C08F293/00 , C08L53/00 , C09D153/00 , G03G15/20 , B32B27/00
CPC分类号： C08F214/262 , C08F293/00 , C08L53/00 , C09D153/00 , G03G15/2057 , Y10T428/1352
摘要： It is possible to provide the heat resistant material and coating material for OA equipment which comprise a fluorine-containing multi-segment polymer having heat resistance, abrasion resistance, non-sticking property against toner and oil resistance in addition to flexibility and are used particularly on surfaces of fuser roll and belt. Those materials comprise a fluorine-containing multi-segment polymer having an elastomeric fluorine-containing polymer chain segment A and a non-elastomeric fluorine-containing polymer chain segment B, and the elastomeric fluorine-containing polymer chain segment A comprises not less than 90% by mole of perhaloolefin unit as a recurring unit and imparts flexibility to the whole polymer.
摘要翻译：可以提供包含含氟多层聚合物的OA设备的耐热材料和涂层材料，其具有耐热性，耐磨性，对调色剂的不粘附性和耐油性以及柔性，并且特别用于定影辊和皮带的表面。这些材料包括具有弹性体含氟聚合物链段A和非弹性含氟聚合物链段B的含氟多段聚合物，弹性体含氟聚合物链段A包含不少于90％的全卤代烯烃单元作为重复单元，并赋予整个聚合物柔性。

6. 发明授权

US06737164B2 Composite materials for cookware 失效
标题翻译：炊具复合材料
公开(公告)号：US06737164B2
公开(公告)日：2004-05-18
申请号：US09380499
申请日：1999-09-03
申请人： Takayuki Araki , Yoshito Tanaka , Masahiro Kumegawa , Noritoshi Oka , Hisato Sanemasa , Tetsuo Shimizu
发明人： Takayuki Araki , Yoshito Tanaka , Masahiro Kumegawa , Noritoshi Oka , Hisato Sanemasa , Tetsuo Shimizu
IPC分类号： B32B2708
CPC分类号： A47J36/02 , C08F214/20 , C08F216/04 , C08F220/00 , C09D127/12 , C09D127/18 , Y10T428/3154 , Y10T428/31544
摘要： Composite materials for cooking apparatuses which are produced by applying, to a substrate, a material comprising a fluorine-containing polymer having an excellent adhesive property to the substrate without necessitating complicated steps and are excellent in heat resistance, non-sticking property, stain-proofing property, water- and oil-repelling property, stain-removing property, chemical resistance, rust-preventing property, antibacterial property, resistance to energy ray and abrasion resistance. The composite materials for cooking apparatuses are produced by applying, to the substrate, the material comprising a fluorine-containing ethylenic polymer having functional group which is prepared by copolymerizing (a) 0.05 to 30% by mole of at least one of fluorine-containing ethylenic monomers having at least one functional group selected from the group consisting of hydroxyl, carboxyl, a carboxylic salt group, a carboxylic ester group and epoxy, and (b) 70 to 99.95% by mole of at least one of fluorine-containing ethylenic monomers having no functional group mentioned above.
摘要翻译：用于烹饪设备的复合材料是通过向衬底施加包含具有优异粘合性的含氟聚合物的材料而制成的，而不需要复杂的步骤，并且具有优异的耐热性，不粘附性，防污染性性能，防油和排斥性能，去污性，耐化学腐蚀性，防锈性，抗菌性，耐光能和耐磨性。用于烹饪设备的复合材料是通过向基材施加含有具有官能团的含氟乙烯性聚合物的材料制造的，所述官能团通过使（a）0.05〜30摩尔％的含氟乙烯性聚合物中的至少一种具有选自羟基，羧基，羧酸盐基，羧酸酯基和环氧基中的至少一种官能团的单体，和（b）70〜99.95摩尔％的至少一种含氟乙烯性单体，没有上述功能组。

7. 发明申请

US20100144993A1 CURABLE FLUORINE-CONTAINING POLYMER, CURABLE RESIN COMPOSITION PREPARED FROM SAME AND ANTIREFLECTION FILM 审中-公开
标题翻译：可固化的含氟聚合物，由其制备的可固化树脂组合物和抗反射膜
公开(公告)号：US20100144993A1
公开(公告)日：2010-06-10
申请号：US12684622
申请日：2010-01-08
申请人： Takayuki ARAKI , Mihoko Ohashi , Yoshito Tanaka , Tetsuo Shimizu
发明人： Takayuki ARAKI , Mihoko Ohashi , Yoshito Tanaka , Tetsuo Shimizu
IPC分类号： C08F220/22
CPC分类号： C09D127/12 , C08F8/00 , C08F8/14 , C08F16/32 , C08F214/18 , C08F290/04 , Y10T428/3154 , C08F14/18
摘要： A curable fluorine-containing polymer having a number average molecular weight of from 500 to 1,000,000 and is represented by the formula (1): -(A)-(M)- in which the structural unit M is a structural unit derived from a fluorine-containing ethylenic monomer and represented by the formula (M): [—(CX1X2—CX3)—]—(CX4CX5)a—(C═O)b(O)c—Rf, wherein X1 and X2 are the same or different and each is H or F; X3 is H, F, CH3 or CF3; X4 and X5 are the same or different and each is H, F or CF3; Rf is an organic group as defined herein; a is 0 or an integer of from 1 to 3; b and c are the same or different and each is 0 or 1, and the structural unit A is derived from a monomer copolymerizable with the fluorine-containing ethylenic monomer from which M is derived.
摘要翻译：数均分子量为500〜1,000,000的可固化的含氟聚合物，由式（1）表示： - （A） - （M） - 其中结构单元M是衍生自氟的结构单元由（M）表示：[ - （CX1X2-CX3） - ] - （CX4CX5）a-（C = O）b（O）c-Rf，其中X1和X2相同或不同并分别为H或F; X3是H，F，CH3或CF3; X4和X5相同或不同，分别为H，F或CF 3; Rf是本文定义的有机基团; a为0或1〜3的整数; b和c相同或不同，分别为0或1，结构单元A衍生自可与M衍生的含氟乙烯性单体共聚的单体。

8. 发明授权

US07670640B2 Curable fluorine-containing polymer, curable resin composition prepared from same and antireflection film 有权
标题翻译：可固化的含氟聚合物，由其制备的可固化树脂组合物和抗反射膜
公开(公告)号：US07670640B2
公开(公告)日：2010-03-02
申请号：US11226355
申请日：2005-09-15
申请人： Takayuki Araki , Mihoko Ohashi , Yoshito Tanaka , Tetsuo Shimizu
发明人： Takayuki Araki , Mihoko Ohashi , Yoshito Tanaka , Tetsuo Shimizu
IPC分类号： B05D5/06
CPC分类号： C09D127/12 , C08F8/00 , C08F8/14 , C08F16/32 , C08F214/18 , C08F290/04 , Y10T428/3154 , C08F14/18
摘要： There are provided a curable fluorine-containing polymer which can realize a high hardness by photo-curing while maintaining a low refractive index, an antireflection film possessing improved scratch resistance and abrasion resistance while maintaining a reflection reducing effect, and an antireflection-treated article provided with such an antireflection film. The curable fluorine-containing polymer has a number average molecular weight of from 500 to 1,000,000 and is represented by the formula (1): AM (1) in which the structural unit M is a structural unit derived from a fluorine-containing ethylenic monomer and represented by the formula (M): wherein X1 and X2 are the same or different and each is H or F; X3 is H, F, CH3 or CF3; X4 and X5 are the same or different and each is H, F or CF3; Rf is an organic group in which 1 to 3 of Y1 (Y1 is a monovalent organic group having 2 to 10 carbon atoms and an ethylenic carbon-carbon double bond at its end) are bonded to a fluorine-containing alkyl group having 1 to 40 carbon atoms or a fluorine-containing alkyl group having 2 to 100 carbon atoms and ether bond; a is 0 or an integer of from 1 to 3; b and c are the same or different and each is 0 or 1, the structural unit A is a structural unit derived from a monomer copolymerizable with the fluorine-containing ethylenic monomer represented by the formula (M), and the structural unit M and the structural unit A are contained in amounts of from 0.1 to 100% by mole and from 0 to 99.9% by mole, respectively.
摘要翻译：提供了一种可固化的含氟聚合物，其可以通过光固化同时保持低折射率实现高硬度，在保持反射降低效果的同时具有改善的耐擦伤性和耐磨性的抗反射膜，以及提供的抗反射处理制品具有这样的抗反射膜。可固化含氟聚合物的数均分子量为500〜1,000,000，由式（1）表示：AM（1）其中，结构单元M是来自含氟乙烯性单体的结构单元，由式（M）表示：其中X1和X2相同或不同，各自为H或F; X3是H，F，CH3或CF3; X4和X5相同或不同，分别为H，F或CF 3; Rf为1〜3的Y1（Y1为碳原子数为2〜10的一价有机基团，末端为烯属碳 - 碳双键）的1〜3的有机基团与1〜40的含氟烷基碳原子或碳原子数2〜100的含氟烷基和醚键; a为0或1〜3的整数; b和c相同或不同，分别为0或1，结构单元A是衍生自与式（M）表示的含氟乙烯性单体共聚的单体的结构单元，结构单元M和结构单元A的含量分别为0.1至100摩尔％和0至99.9摩尔％。

9. 再颁专利

USRE41110E1 Heat-resistant material and coating material for OA equipments having flexibility 失效
标题翻译：具有柔性的OA设备的耐热材料和涂料
公开(公告)号：USRE41110E1
公开(公告)日：2010-02-09
申请号：US11512391
申请日：2006-08-30
申请人： Takayuki Araki , Yoshito Tanaka , Masahiro Kumegawa , Norihito Otsuki , Masami Kato , Tetsuo Shimizu
发明人： Takayuki Araki , Yoshito Tanaka , Masahiro Kumegawa , Norihito Otsuki , Masami Kato , Tetsuo Shimizu
IPC分类号： B32B27/00
CPC分类号： C08F214/262 , C08F293/00 , C08L53/00 , C09D153/00 , G03G15/2057 , Y10T428/1352
摘要： It is possible to provide the heat resistant material and coating material for OA equipment which comprise a fluorine-containing multi-segment polymer having heat resistance, abrasion resistance, non-sticking property against toner and oil resistance in addition to flexibility and are used particularly on surfaces of fuser roll and belt. Those materials comprise a fluorine-containing multi-segment polymer having an elastomeric fluorine-containing polymer chain segment A and a non-elastomeric fluorine-containing polymer chain segment B, and the elastomeric fluorine-containing polymer chain segment A comprises not less than 90% by mole of perhaloolefin unit as a recurring unit and imparts flexibility to the whole polymer.
摘要翻译：可以提供包含含氟多层聚合物的OA设备的耐热材料和涂层材料，其具有耐热性，耐磨性，对调色剂的不粘附性和耐油性以及柔性，并且特别用于定影辊和皮带的表面。这些材料包括具有弹性体含氟聚合物链段A和非弹性含氟聚合物链段B的含氟多段聚合物，弹性体含氟聚合物链段A包含不少于90％的全卤代烯烃单元作为重复单元，并赋予整个聚合物柔性。

10. 发明授权

US06207236B1 Coating composition, coating film, and method for producing coating film 有权
标题翻译：涂料组合物，涂膜及其制备方法
公开(公告)号：US06207236B1
公开(公告)日：2001-03-27
申请号：US09202592
申请日：1998-12-17
申请人： Takayuki Araki , Yoshito Tanaka , Masahiro Kumegawa , Noritoshi Oka , Tetsuo Shimizu
发明人： Takayuki Araki , Yoshito Tanaka , Masahiro Kumegawa , Noritoshi Oka , Tetsuo Shimizu
IPC分类号： B05D302
CPC分类号： C09D127/12 , C09D127/18 , C08L2666/54
摘要： To provide the water-repellent coating film having excellent transparency, abrasion resistance, weather resistance and water repellency, the method for producing the coating film, the multi-functional composite material provided with the coating film and the coating composition used therefor which has excellent dispersion stability. The coating composition comprises (A) the fluorine-containing ethylenic polymer prepared by copolymerizing a fluorine-containing ethylenic monomer having at least one functional group selected from hydroxyl, carboxyl, a carboxylic salt group, a carboxylic ester group and epoxy, (B-1) the metal oxide sol, and (C) the solvent.
摘要翻译：为了提供具有优异的透明性，耐磨性，耐候性和防水性的防水涂膜，涂膜的制备方法，设置有涂膜的多功能复合材料及其所用的涂料组合物具有优异的分散性稳定性。涂料组合物包含（A）通过共聚含有至少一个选自羟基，羧基，羧酸盐基，羧酸酯基和环氧基的官能团的含氟乙烯性单体制备的含氟乙烯性聚合物（B-1 ）金属氧化物溶胶，和（C）溶剂。

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