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1. 发明授权

US6013114A Environmentally friendly diesel fuel 失效
标题翻译：环保柴油
公开(公告)号：US6013114A
公开(公告)日：2000-01-11
申请号：US13755
申请日：1998-01-27
申请人： Martin Hille , Frank Weinelt , Heinz Wittkus , Werner Reimann
发明人： Martin Hille , Frank Weinelt , Heinz Wittkus , Werner Reimann
IPC分类号： C10L1/08 , C10L1/02 , C10L1/18 , C10L1/19 , C10L10/12
CPC分类号： C10L1/026 , Y02E50/13
摘要： The present invention relates to environmentally friendly diesel fuel, containing natural, liquid triglycerides of natural or animal origin, such as rapeseed or soybean oil, and acetals of the formula (I) or (II) ##STR1## in which the substitutents have the meaning defined in the description. This diesel fuel is biodegradable and free of sulfur, nitrogen and aromatics.
摘要翻译：本发明涉及环境友好的柴油燃料，其含有天然或动物来源的天然，液体甘油三酯，例如油菜籽油或大豆油，以及式（I）或（II）的缩醛，其中取代基具有在描述。该柴油是可生物降解的，不含硫，氮和芳烃。

2. 发明授权

US08628591B2 Detergent additive-containing mineral oils having improved cold flow properties 有权
标题翻译：具有改善的冷流特性的含有洗涤剂添加剂的矿物油
公开(公告)号：US08628591B2
公开(公告)日：2014-01-14
申请号：US12665010
申请日：2008-06-17
申请人： Matthias Krull , Werner Reimann , Robert Janssen
发明人： Matthias Krull , Werner Reimann , Robert Janssen
IPC分类号： C10L1/18 , C10L1/22
CPC分类号： C10L1/143 , C10L1/1608 , C10L1/1641 , C10L1/1817 , C10L1/1981 , C10L1/2222 , C10L1/224 , C10L1/2383 , C10L10/14
摘要： The invention relates to the use of at least one oil-soluble compound B) which acts as a nucleating agent for paraffin crystallization and which is selected from substantially linear hydrocarbons with at least 22 C atoms, for improving the response of cold flow improvers for mineral oils C) in middle distillates that contain at least one ashless, nitrogenous detergent additive A), which is an oil-soluble, amphiphilic compound that comprises at least one alkyl or alkenyl group bound to a polar group, said alkyl or alkenyl group having 10 to 500 C atoms and the polar group having 2 or more nitrogen atoms.
摘要翻译：本发明涉及至少一种用作石蜡结晶的成核剂的油溶性化合物B）的用途，其选自具有至少22个C原子的基本上直链的烃，以改善用于矿物质的冷流改进剂的响应油C）在含有至少一种无灰，含氮洗涤剂添加剂A）的中间馏分中，其是包含与极性基团结合的至少一个烷基或烯基的油溶性两亲化合物，所述烷基或烯基具有10 至500个C原子和具有2个或更多个氮原子的极性基团。

3. 发明授权

US07872061B2 Preparation of additive mixtures for mineral oils and mineral oil distillates 有权
标题翻译：矿物油和矿物油馏分添加剂混合物的制备
公开(公告)号：US07872061B2
公开(公告)日：2011-01-18
申请号：US12247520
申请日：2008-10-08
申请人： Matthias Krull , Gerhard Bettermann , Curd-Werner Adams , Werner Reimann
发明人： Matthias Krull , Gerhard Bettermann , Curd-Werner Adams , Werner Reimann
IPC分类号： C08K3/00 , C08F210/02
CPC分类号： C08K3/00 , C10L1/146 , C10L1/1641 , C10L1/1955 , C10L1/1963 , C10L1/1966 , C10L1/1973 , C10L1/1981 , C10L1/1985
摘要： The present invention provides a continuous process for preparing additive mixtures for mineral oils and mineral oil distillates, comprising A) a cold flow improver for middle distillates, and at least one further component selected from B) and C): B) a further cold flow improver, C) an organic solvent, which comprises mixing cold flow improver and optionally solvent by means of a static mixer, the temperature of the additive mixture at the outlet of the static mixer being from 0° C. to 100° C.
摘要翻译：本发明提供了用于制备用于矿物油和矿物油馏出物的添加剂混合物的连续方法，其包括A）用于中间馏分的冷流改进剂和至少一种选自B）和C）的另外的组分：B）另外的冷流改进剂，C）有机溶剂，其包括通过静态混合器将冷流改进剂和任选溶剂混合，静态混合器出口处的添加剂混合物的温度为0℃至100℃

4. 发明授权

US07713315B2 Mineral oils with improved conductivity and cold flowability 有权
标题翻译：具有改善导电性和冷流动性的矿物油
公开(公告)号：US07713315B2
公开(公告)日：2010-05-11
申请号：US11494841
申请日：2006-07-28
申请人： Matthias Krull , Werner Reimann
发明人： Matthias Krull , Werner Reimann
IPC分类号： C10L1/18 , C10L10/22
CPC分类号： C10L1/146 , C10L1/1981 , C10L1/236 , C10L1/2364 , C10L1/2366 , C10L1/2383 , C10L10/14
摘要： The invention provides mineral oil distillates having a water content of less than 150 ppm and a conductivity of at least 50 pS/m, which comprise from 0.1 to 200 ppm of at least one alkylphenol-aldehyde resin and from 0.1 to 200 ppm of at least one nitrogen-containing polymer.
摘要翻译：本发明提供了含水量小于150ppm，导电率至少为50pS / m的矿物油馏出物，其包含0.1至200ppm的至少一种烷基酚醛树脂和0.1至200ppm的至少一种含氮聚合物。

5. 发明申请

US20080016754A1 Additives for improving the cold properties of fuel oils 有权
标题翻译：用于改善燃油的冷特性的添加剂
公开(公告)号：US20080016754A1
公开(公告)日：2008-01-24
申请号：US11879431
申请日：2007-07-17
申请人： Bettina Siggelkow , Werner Reimann , Matthias Krull , Ulrike Neuhaus , Markus Kupetz , Andre Graf
发明人： Bettina Siggelkow , Werner Reimann , Matthias Krull , Ulrike Neuhaus , Markus Kupetz , Andre Graf
IPC分类号： C10L1/195 , C08F220/10 , C08L33/02
CPC分类号： C10L1/146 , C10L1/1641 , C10L1/165 , C10L1/1658 , C10L1/1966 , C10L1/1973 , C10L1/1981 , C10L1/1985 , C10L1/224 , C10L1/2364 , C10L10/14
摘要： The invention provides additive mixtures comprising A) at least one terpolymer of ethylene, propene and at least one ethylenically unsaturated ester, which i) contains from 6.0 to 12.0 mol % of structural units derived from at least one ethylenically unsaturated ester having a C1- to C3-alkyl radical, ii) contains from 0.5 to 4.0 methyl groups derived from propene per 100 aliphatic carbon atoms, iii) has fewer than 8.0 methyl groups stemming from chain ends per 100 CH2 groups, and B) from 0.5 to 20 parts by weight, based on A), of at least one further component which is effective as a cold additive for mineral oils and is selected from B1) copolymers of ethylene and ethylenically unsaturated compounds whose content of ethylenically unsaturated compounds is at least 2 mol % higher than the content of ethylenically unsaturated esters in the terpolymer defined under A), B2) comb polymers, and B3) mixtures of B1) and B2), and also their use as a cold additive for middle distillates.
摘要翻译：本发明提供添加剂混合物，其包含A）至少一种乙烯，丙烯和至少一种烯键式不饱和酯的三元共聚物，i）含有6.0-12.0mol％的至少一种具有C 1〜C 3 - 烷基，ii）含有每100个脂肪族碳原子衍生自丙烯的0.5〜4.0个甲基，iii）由链中衍生的少于8.0个甲基至少一种作为矿物油的冷添加剂有效的至少一种另外的组分，并且B）基于A）的0.5至20重量份，并且选自： B1）乙烯和烯键式不饱和化合物的共聚物，其烯键式不饱和化合物的含量比A），B2）梳状聚合物中定义的三元共聚物中烯属不饱和酯的含量高至少2摩尔％，和B3）B1）和 B2），以及它们作为冷添加剂的用途对于中间馏分。

6. 发明申请

US20050155282A1 Demulsifiers for mixtures of middle distillates with fuel oils of vegetable or animal origin and water 失效
标题翻译：中间馏分与植物或动物来源的燃料油和水的混合物的破乳剂
公开(公告)号：US20050155282A1
公开(公告)日：2005-07-21
申请号：US11036693
申请日：2005-01-14
申请人： Bettina Siggelkow , Werner Reimann , Dirk Leinweber , Ulrike Neuhaus , Renate Braun
发明人： Bettina Siggelkow , Werner Reimann , Dirk Leinweber , Ulrike Neuhaus , Renate Braun
IPC分类号： C10L1/192 , C10L1/02 , C10L1/04 , C10L1/14 , C10L1/18 , C10L1/19 , C10L1/195 , C10L1/198 , C10L1/22 , C10L1/224 , C10L1/2387 , C10L1/28 , C10L5/00
CPC分类号： C10L1/146 , C10L1/143 , C10L1/1966 , C10L1/1973 , C10L1/1981 , C10L1/1985 , C10L1/2222 , C10L1/224 , C10L1/2364 , C10L1/2387 , C10L1/285
摘要： The invention provides fuel oils comprising a major proportion of a mixture of A) a middle distillate fuel oil and B) a biofuel oil, and also a minor proportion C) of an oil-soluble, crosslinked block copolymer composed of C2- to C4-alkylene oxides.
摘要翻译：本发明提供燃料油，其包含主要部分A）中间馏分燃料油和B）生物燃料油的混合物，以及较小比例的C）油溶性交联的嵌段共聚物，其由C 2 C 4 - 亚烷基氧基。

7. 发明授权

US06762253B2 Process for the preparation of ethylene copolymers, and their use as additives to mineral oil and mineral oil distillates 有权
标题翻译：制备乙烯共聚物的方法及其作为矿物油和矿物油馏出物添加剂的用途
公开(公告)号：US06762253B2
公开(公告)日：2004-07-13
申请号：US09956544
申请日：2001-09-18
申请人： Matthias Krull , Werner Reimann , Wilhelm Zoller , Heinz Dieter Bühnen , Gerhard Bettermann
发明人： Matthias Krull , Werner Reimann , Wilhelm Zoller , Heinz Dieter Bühnen , Gerhard Bettermann
IPC分类号： C08F200
CPC分类号： B01J3/042 , B01J19/2415 , B01J2219/00168 , B01J2219/00184 , B01J2219/00186 , C08F210/02 , C08F210/16 , C10L1/143 , C10L1/1608 , C10L1/1616 , C10L1/1641 , C10L1/195 , C10L1/1955 , C10L1/1963 , C10L1/1966 , C10L1/1973 , C10L1/1985 , C10L1/221 , C10L1/224 , C10L1/2364 , C08F2/00 , C08F218/08 , C08F218/10 , C08F210/14
摘要： The invention relates to a process for the preparation of terpolymers of ethylene and at least 2 further olefinically unsaturated compounds by polymerization in a tubular reactor fitted with at least one side branch, wherein the fresh monomer components, which are introduced into the tubular reactor via the reactor inlet (the primary stream) or via the side branch or side branches (secondary stream or secondary streams), in each of the streams contain ethylene and at most one further olefinically unsaturated compound.
摘要翻译：本发明涉及一种通过在装有至少一个侧枝的管式反应器中聚合制备乙烯和至少2种其它烯属不饱和化合物的三元共聚物的方法，其中新鲜单体组分通过反应器入口（主流）或经由侧分支或副分支（二级流或二级流）在每个流中含有乙烯和至多一种其它烯属不饱和化合物。

8. 发明授权

US06593426B2 Copolymer blends and their use as additives for improving the cold flow properties of middle distillates 失效
标题翻译：共聚物共混物及其用作改善中间馏分冷流特性的添加剂
公开(公告)号：US06593426B2
公开(公告)日：2003-07-15
申请号：US09808481
申请日：2001-03-14
申请人： Matthias Krull , Thomas Volkmer , Werner Reimann
发明人： Matthias Krull , Thomas Volkmer , Werner Reimann
IPC分类号： C08L118
CPC分类号： C10L1/195 , C10L1/146 , C10L1/1963 , C10L1/1966 , C10L1/1973 , C10L1/2364
摘要： The invention relates to additives for improving the cold flow properties of middle distillates, containing from 10 to 95% by weight of copolymers A), from 5 to 90% by weight of copolymers B) and, if required, from 0 to 70% by weight of copolymers C), which correspond to the following formulae: A) copolymers of lower olefins and vinyl esters, B) copolymers comprising B1) from 40 to 60 mol % of bivalent structural units of the formula where X is O or N—R4 and in which a and b are 0 or 1 and a +b=1, and B2) from 60 to 40 mol % of bivalent structural units of the formula —H2C—CR11R5— B2 and, if required, B3) from 0 to 20 mol % of bivalent structural units which are derived from polyolefins, the polyolefins being derivable from monoolefins having 3 to 5 carbon atoms, and in which a) R4 is an alkyl or alkenyl radical having 10 to 40 carbon atoms or an alkoxyalkyl radical having 1 to 100 alkoxy units and 1 to 30 carbon atoms in the alkyl radical, and b) R5 is a radical of the formula OCOR12 or COOR12, in which R12 is C1-to C3-alkyl, and c) the number of carbon atoms of the polyolefin molecules on which the structural units B3) are based is from 35 to 350, and d) R11 is hydrogen or methyl, and, if required, C) a further copolymer differing from A) and B) and comprising ethylene and one or more vinyl esters or acrylates, which by itself is effective as a cold flow improver for middle distillates.
摘要翻译：本发明涉及用于改善中间馏分的冷流动性的添加剂，其含有10至95重量％的共聚物A），5至90重量％的共聚物B），如果需要，0至70重量％共聚物C）的重量，其对应于下式：A）低级烯烃和乙烯基酯的共聚物，B）包含B1至40摩尔％的下式的二价结构单元的共聚物，其中X为O或N-R 4，其中a和b分别为0或1，a + b = 1，B 2）为60至40摩尔％的二价结构单元，如果需要，B3）0至20摩尔％的二价结构单元衍生聚烯烃可以衍生自具有3至5个碳原子的单烯烃，并且其中a）R4是具有10至40个碳原子的烷基或烯基或具有1至100个烷氧基单元和1至30个碳原子的烷氧基烷基在烷基中，和b）R 5是式OCOR 12或COOR 12的基团，其中R 1 2是C1-C3烷基，c）结构单元B3）所基于的聚烯烃分子的碳原子数为35〜350，d）R 11为氢或甲基，如果需要， C）与A）和B）不同的另外的共聚物，并且包含乙烯和一种或多种乙烯基酯或丙烯酸酯，其本身作为中间馏分的冷流改进剂是有效的。

9. 发明授权

US06461393B1 Mixtures of carboxylic acids, their derivatives and hydroxyl-containing polymers and their use for improving the lubricating effect of oils 失效
标题翻译：羧酸，其衍生物和含羟基聚合物的混合物及其用于改善油的润滑效果的用途
公开(公告)号：US06461393B1
公开(公告)日：2002-10-08
申请号：US09811306
申请日：2001-03-16
申请人： Matthias Krull , Werner Reimann
发明人： Matthias Krull , Werner Reimann
IPC分类号： C10L118
CPC分类号： C10L10/08 , C10L1/143 , C10L1/18
摘要： The invention relates to additives for improving lubricating properties of fuel oils, comprising A) 10-95% by weight of at least one oil-soluble amphiphile of the formulae 1 and/or 2 R1—X—R2 (2) B) 5-90% by weight of at least one copolymer which contains B1) from 5 to 80 mol % of structural units which are derived from olefinically unsaturated compounds, and B2) from 20 to 95 mol % of structural units which are derived from olefinically unsaturated compounds, B3) from 0 to 40 mol % of further structural units selected from the group consisting of (meth)acrylic acid, (meth)acrylates, vinyl esters, vinyl ethers and alkenes, and the copolymer has an average molar mass Mw of from 500 to 100,000 g/mol and an OH number of from 10 to 350 mg KOH/g.
摘要翻译：本发明涉及用于改善燃料油的润滑性能的添加剂，其包括A）10-95重量％的至少一种式1和/或2B的油溶性两亲物）5-90重量％的至少一种共聚物，含有B1-5摩尔％的衍生自烯属不饱和化合物的结构单元，B 2）20〜95摩尔％来自烯属不饱和化合物的结构单元，B3）0-40摩尔％的其它结构单元选自（甲基）丙烯酸，（甲基）丙烯酸酯，乙烯基酯，乙烯基醚和烯烃组成的组，所述共聚物的平均摩尔质量Mw为500〜100,000g / mol，OH数为10〜 350mg KOH / g。

10. 发明授权

US5718821A Copolymers of ethylenically unsaturated carboxylic acid esters with polyoxyalkylene ethers of lower, unsaturated alcohols as flow-improving agents for paraffin containing oils 失效
标题翻译：烯属不饱和羧酸酯与低级不饱和醇的聚氧化烯醚的共聚物作为含石蜡油的流动性改进剂
公开(公告)号：US5718821A
公开(公告)日：1998-02-17
申请号：US821284
申请日：1997-03-20
申请人： Matthias Krull , Sigmar-Peter von Halasz , Werner Reimann , Juliane Balzer , Horst Geiss
发明人： Matthias Krull , Sigmar-Peter von Halasz , Werner Reimann , Juliane Balzer , Horst Geiss
IPC分类号： C08F20/10 , C08F220/10 , C08F220/18 , C08F222/10 , C08F290/00 , C08F299/02 , C10L1/14 , C10L1/16 , C10L1/18 , C10L1/192 , C10L1/196 , C10L1/198 , C10L1/22 , C10M145/14 , C10M145/38 , C10G73/00
CPC分类号： C10L1/192 , C08F220/18 , C10L1/143 , C10L1/146 , C10L1/1963 , C10L1/1966 , C10L1/1985 , C10M145/14 , C10M145/38 , C10L1/1616 , C10L1/2368 , C10M2209/084 , C10M2209/103 , C10M2209/104 , C10M2209/107 , C10M2209/109
摘要： The invention relates to novel copolymers of ethylenically unsaturated carboxylic acid esters with polyoxyalkylene ethers of lower, unsaturated alcohols, their preparation, their use as flow-improving agents for paraffin-containing oils, and oils which contain such copolymers. The invention also relates to the use of known copolymers of ethylenically unsaturated carboxylic acid esters with polyoxyalkylene ethers of allyl and/or methallyl alcohol as flow-improving agents for paraffin-containing oils.
摘要翻译：本发明涉及烯属不饱和羧酸酯与低级不饱和醇的聚氧化烯醚的新型共聚物，它们的制备，它们作为含链烷烃油的流动改进剂的用途，以及含有这些共聚物的油。本发明还涉及烯属不饱和羧酸酯与烯丙基和/或甲代烯丙醇的聚氧化烯醚的已知共聚物作为石蜡油的流动改进剂的用途。

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