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1. 发明授权

US5164442A Rubber composition 失效
公开(公告)号：US5164442A
公开(公告)日：1992-11-17
申请号：US504364
申请日：1990-04-04
申请人： Kunio Itoh , Motoo Fukushima , Tsutomu Nakamura , Hiroyuki Ohata , Harukazu Okuda
发明人： Kunio Itoh , Motoo Fukushima , Tsutomu Nakamura , Hiroyuki Ohata , Harukazu Okuda
IPC分类号： C08F283/12 , C08K3/00 , C08K5/00 , C08K13/02 , C08L51/08 , C08L83/10
CPC分类号： C08L83/10 , C08F283/122 , C08K13/02 , C08L51/085
摘要： The polymeric ingredient of the inventive rubber composition is an acrylic polymer modified with a mercapto-containing organopolysiloxane as prepared by the emulsion polymerization of an acrylic monomer in an aqueous emulsion of the organopolysiloxane. Characteristically, the acrylic monomer is copolymerized with another monomer having an active halogen atom or an epoxy group. By virtue of this unique formulation of the rubbery polymer, the inventive rubber composition prepared by compounding the rubbery polymer with a reinforcing filler and a specified curing or crosslinking agent can be vulcanized to give a vulcanizate having excellent mechanical properties, heat resistance, oil resistance and cold resistance as a combination of the features of silicone rubbers and acrylic rubbers.

2. 发明授权

US5232997A Method for the preparation of an acrylic polymer modified with an organopolysiloxane 失效
标题翻译：制备用有机硅氧烷改性的丙烯酸聚合物的方法
公开(公告)号：US5232997A
公开(公告)日：1993-08-03
申请号：US670276
申请日：1991-03-15
申请人： Kunio Itoh , Motoo Fukushima , Toshio Ohba , Hiroyuki Ohata , Harukazu Okuda
发明人： Kunio Itoh , Motoo Fukushima , Toshio Ohba , Hiroyuki Ohata , Harukazu Okuda
IPC分类号： C08F230/08 , C08F290/06
CPC分类号： C08F230/08 , C08F290/068
摘要： An acrylic rubbery polymer having remarkably improved cold resistance can be prepared by modification with an organopolysiloxane by the emulsion copolymerization of a monomeric mixture of two acrylic monomers, of which one is, for example, an alkyl acrylate and the other is an acrylic compound having, in a molecule, at least one ethylenically unsaturated group other than acrylic group in an aqueous emulsion of an organopolysiloxane having a substantial amount of mercapto-substituted monovalent hydrocarbon groups bonded to the silicon atoms.
摘要翻译：具有显着改善的耐寒性的丙烯酸类橡胶状聚合物可以通过用两种丙烯酸类单体的单体混合物的乳液共聚物进行改性来制备，其中一种是例如丙烯酸烷基酯，另一种是丙烯酸类化合物，在具有大量巯基取代的单价烃基键合到硅原子的有机聚硅氧烷的水性乳液中，在分子中至少有一个除丙烯酸以外的烯属不饱和基团。

3. 发明授权

US4910278A Monomeric composition and polymer therefrom 失效
标题翻译：单体组成和聚合物
公开(公告)号：US4910278A
公开(公告)日：1990-03-20
申请号：US368513
申请日：1989-06-20
申请人： Kunio Itoh , Motoo Fukushima , Harukazu Okuda , Hiroyuki Ohata
发明人： Kunio Itoh , Motoo Fukushima , Harukazu Okuda , Hiroyuki Ohata
IPC分类号： C08F30/08 , C08F18/02 , C08F18/20 , C08F20/32 , C08F220/10 , C08F220/18 , C08F220/32 , C08F230/08 , C08F290/00 , C08F299/08 , C08G59/00 , C08G59/40 , C08L63/00
CPC分类号： C08F230/08
摘要： Rubber vulcanizates having excellent oil resistance, heat resistance and cold resistance can be obtained from a rubbery copolymer which is a polymerization product of an acrylic monomer mixture of which the essential components are an organosiloxy-containing acrylate compound such as acryloxymethyl pentamethyl disiloxane and 3-acryloxypropyl pentamethyl disiloxane and an epoxy group- or halogen-containing monomer such as allyl glycidyl ether, glycidyl methacrylate and vinyl chloroacetate, optionally, with addition of an acrylate ester monomer such as ethyl acrylate, n-butyl acrylate and 2-methoxyethyl acrylate.

4. 发明授权

US5059648A Rubber composition 失效
标题翻译：橡胶组合物
公开(公告)号：US5059648A
公开(公告)日：1991-10-22
申请号：US427049
申请日：1989-10-25
申请人： Motoo Fukushima , Tsutomu Nakamura , Hiroyuki Ohata , Harukazu Okuda
发明人： Motoo Fukushima , Tsutomu Nakamura , Hiroyuki Ohata , Harukazu Okuda
IPC分类号： C08K5/05 , C08L21/00 , C08L83/10
CPC分类号： C08L21/00 , C08F265/04 , C08F283/124 , C08K5/05 , C08L23/16 , C08L83/10 , C08K3/04 , C08K3/36 , C08L2205/03 , C08L7/00 , C08L71/02
摘要： A rubber composition based on a rubbery polymer and a silica-based reinforcing filler can be imparted with a greatly improved workability in roll milling and molding as well as in the mechanical properties of the vulcanizates prepared therefrom when the rubber composition is admixed with an acetylene alcohol or an alkylene-oxide adduct of acetylene alcohol presumably by virtue of the improvement in the dispersibility of the reinforcing filler in the rubbery matrix. The improvement obtained by the addition of the acetylene alcohol compound is not limited to the dispersibility of silica fillers but also to the dispersibility of carbon black when the rubbery polymer is an organopolysiloxane-modified acrylic polymer.

5. 发明授权

US06680081B2 Conductive powder and making process 失效
标题翻译：导电粉和制作工艺
公开(公告)号：US06680081B2
公开(公告)日：2004-01-20
申请号：US10102846
申请日：2002-03-22
申请人： Motoo Fukushima , Kunio Itoh , Shigeru Mori , Masaki Kasashima , Yoshitaka Hamada , Mikio Aramata
发明人： Motoo Fukushima , Kunio Itoh , Shigeru Mori , Masaki Kasashima , Yoshitaka Hamada , Mikio Aramata
IPC分类号： C23C1832
CPC分类号： H01B1/22 , H05K3/323 , Y10T428/2991 , Y10T428/2993 , Y10T428/2995 , Y10T428/2996
摘要： A conductive powder having an organic silicon polymer layer on the surface of each particle and a metal layer enclosing the silicon polymer layer possesses a stronger bond between the particle base and the metal even at elevated temperature and exhibits a high and stable conductivity and heat resistance.
摘要翻译：在每个颗粒的表面上具有有机硅聚合物层的导电粉末和包围硅聚合物层的金属层即使在升高的温度下也具有更强的颗粒基体和金属之间的结合，并表现出高且稳定的导电性和耐热性。

6. 发明授权

US4952609A Acryl rubber foaming compositions and foamed acryl rubber 失效
标题翻译：丙烯酸橡胶发泡组合物和发泡丙烯酸橡胶
公开(公告)号：US4952609A
公开(公告)日：1990-08-28
申请号：US476595
申请日：1990-02-07
申请人： Motoo Fukushima , Masaharu Takahashi , Kunio Itoh
发明人： Motoo Fukushima , Masaharu Takahashi , Kunio Itoh
IPC分类号： C08J9/06 , C08J9/10
CPC分类号： C08J9/10 , C08J2333/04
摘要： Acryl rubber foaming compositions comprising (A) an acrylic polymer prepared by copolymerizing an acrylate or methacrylate with a monomer having at least two aliphatic unsaturated bonds per molecule, (B) a pyrolytic organic foaming agent, and (C) an organic peroxide can be molded, cured and foamed into acryl rubber foams having improved heat insulation, heat resistance, weatherability, crack resistance, and oil resistance without a need for sulfur vulcanizer.
摘要翻译：丙烯酸酯橡胶发泡组合物，其包含（A）通过使丙烯酸酯或甲基丙烯酸酯与每分子具有至少两个脂肪族不饱和键的单体（B）热解有机发泡剂和（C）有机过氧化物共聚而制备的丙烯酸类聚合物，固化并发泡成具有改善的隔热性，耐热性，耐候性，抗裂性和耐油性的丙烯酸橡胶泡沫，而不需要硫硫化剂。

7. 发明授权

US5041592A Organic silicon compounds, hydrolyzates thereof, and rubber plasticizers 失效
标题翻译：有机硅化合物，其水解产物和橡胶增塑剂
公开(公告)号：US5041592A
公开(公告)日：1991-08-20
申请号：US359696
申请日：1989-05-31
申请人： Motoo Fukushima , Jun Hatakeyama , Kunio Itoh
发明人： Motoo Fukushima , Jun Hatakeyama , Kunio Itoh
IPC分类号： C07F7/18 , C08G77/04 , C08K5/00 , C08K5/54 , C08K5/5415 , C08K5/5419 , C08L21/00
CPC分类号： C08K5/54 , C07F7/1836 , C08K5/5415
摘要： A novel organic silicon compound and hydrolyzate thereof are provided in which an alkoxysilane having an alkoxy radical attached to the silicon atom is attached to a polyester through an alkylene radical. They are useful as a plasticizer for rubber.
摘要翻译：提供了一种新的有机硅化合物及其水解产物，其中具有与硅原子连接的烷氧基的烷氧基硅烷通过亚烷基连接到聚酯上。它们可用作橡胶增塑剂。

8. 发明授权

US4876344A Novel organosilicon compounds 失效
标题翻译：新型有机硅化合物
公开(公告)号：US4876344A
公开(公告)日：1989-10-24
申请号：US277632
申请日：1988-11-29
申请人： Kunio Itoh , Motoo Fukushima , Tsutomu Nakamura
发明人： Kunio Itoh , Motoo Fukushima , Tsutomu Nakamura
IPC分类号： C07D251/38 , C07F7/18 , C08G59/40 , C08K5/548
CPC分类号： C07F7/1816 , C07D251/38 , C08K5/548
摘要： Organosilicon compounds of the following formula, or hydrolyzates thereof, ##STR1## ps in which Rhu 1 l and Rhu 2 l are independently a hydrogen atom or an alkyl group having from 1 to 8 carbon atoms, m is an integer of from 1 to 8, and n is an integer of from 1 to 3. The compound is useful as a vulcanizing agent particularly for vulcanizable elastomer compositions comprising inorganic fillers.
摘要翻译：下式的有机硅化合物或其水解产物，其中R 1和L 2独立地为氢原子或具有1至8个碳原子的烷基，m为1至8的整数，n为1〜3的整数。该化合物特别用于含有无机填料的可硫化弹性体组合物，可用作硫化剂。

9. 发明授权

US4761452A Oil-resistant rubber composition 失效
标题翻译：耐油橡胶组合物
公开(公告)号：US4761452A
公开(公告)日：1988-08-02
申请号：US883535
申请日：1986-07-09
申请人： Kunio Itoh , Motoo Fukushima , Tsutomu Nakamura
发明人： Kunio Itoh , Motoo Fukushima , Tsutomu Nakamura
IPC分类号： C08L23/00 , C08K3/00 , C08L23/16 , C08L33/00 , C08L33/04 , C08L33/08 , C08L43/04
CPC分类号： C08L43/04 , C08L23/16 , C08L2312/08
摘要： A rubber composition capable of giving a highly oil-resistant vulcanizate with an organic peroxide as the vulcanizing agent is proposed. The composition is a blend of an EPM or EPDM rubber and an acrylic rubber loaded with a reinforcing filler, of which the latter rubber is a copolymer having at least two vinylsilyl groups in a molecule as the pendant groups introduced by the copolymerization of one or more acrylic monomers with a vinylsilyl-containing organosilicon compound having an aliphatically unsaturated group copolymerizable with the acrylic monomers in a molecule, such as CH.sub.2 .dbd.CH--CO--O--CH.sub.2 CH.sub.2 CH.sub.2 --Si-- and CH.sub.2 .dbd.CH--C.sub.6 H.sub.4 --Si--. The covulcanizate has the high mechanical strengths of the EPM or EPDM rubber and the high oil resistance of the acrylic rubber in combination.
摘要翻译：提出了能够以有机过氧化物作为硫化剂赋予高耐油硫化橡胶的橡胶组合物。该组合物是EPM或EPDM橡胶和装载有增强填料的丙烯酸橡胶的共混物，其中后者橡胶是在分子中具有至少两个乙烯基甲硅烷基的共聚物，作为通过一个或多个丙烯酸类单体与具有乙烯基甲硅烷基的有机硅化合物在分子中具有可与丙烯酸单体共聚的脂族不饱和基团，例如CH 2 = CH-CO-O-CH 2 CH 2 CH 2 -Si-和CH 2 = CH-C 6 H 4 -Si。共硫化橡胶具有EPM或EPDM橡胶的高机械强度和丙烯酸橡胶的高耐油性组合。

10. 发明授权

US06485831B1 Conductive powder and making process 失效
标题翻译：导电粉和制作工艺
公开(公告)号：US06485831B1
公开(公告)日：2002-11-26
申请号：US09570696
申请日：2000-05-12
申请人： Motoo Fukushima , Kunio Itoh , Shigeru Mori , Masaki Kasahima , Yoshitaka Hamada , Mikio Aramata
发明人： Motoo Fukushima , Kunio Itoh , Shigeru Mori , Masaki Kasahima , Yoshitaka Hamada , Mikio Aramata
IPC分类号： B32B1800
CPC分类号： H01B1/22 , H05K3/323 , Y10T428/2991 , Y10T428/2993 , Y10T428/2995 , Y10T428/2996
摘要： A conductive powder having an organic silicon polymer layer on the surface of each particle and a metal layer enclosing the silicon polymer layer possesses a stronger bond between the particle base and the metal even at elevated temperature and exhibits a high and stable conductivity and heat resistance.
摘要翻译：在每个颗粒的表面上具有有机硅聚合物层的导电粉末和包围硅聚合物层的金属层即使在升高的温度下也具有更强的颗粒基体和金属之间的结合，并表现出高且稳定的导电性和耐热性。

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