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1. 发明授权

US6166143A Thermoplastic elastomer composition, hose comprising thermoplastic elastomer composition and process of production thereof 失效
标题翻译：热塑性弹性体组合物，软管包含热塑性弹性体组合物及其生产方法
公开(公告)号：US6166143A
公开(公告)日：2000-12-26
申请号：US101204
申请日：1998-07-02
申请人： Jiro Watanabe , Yuichi Hara , Daisuke Irii , Takashi Satoh , Gou Kawaguchi , Shigeru Yamauchi , Susumu Hatanaka , Noriaki Kuroda
发明人： Jiro Watanabe , Yuichi Hara , Daisuke Irii , Takashi Satoh , Gou Kawaguchi , Shigeru Yamauchi , Susumu Hatanaka , Noriaki Kuroda
IPC分类号： C08L23/02 , F16L11/08 , C08L37/00 , B32B1/08 , C08L51/06
CPC分类号： F16L11/08 , C08L23/02 , Y10T428/1386 , Y10T428/1393 , Y10T428/31855 , C08L2666/04 , C08L2666/24
摘要： A thermoplastic elastomer composition containing a component (A) (thermoplastic polyolefin resin), component (B) (epoxy-group-containing ethylene acrylic ester copolymer rubber), and component (C) (acid-modified polyolefin resin) comprising a continuous phase of the component (A) in which the component (B) is dispersed as a dispersed phase and is cross-linked by a peroxide; a thermoplastic elastomer composition comprising a continuous phase of a thermoplastic polyolefin resin (A) and a dispersed phase of an epoxy-group-containing ethylene-acrylic ester copolymer rubber component (B) and acrylonitrile butadiene rubber component (C), which is dynamically cross-linked; and a hose having an inner tube, at least one reinforcing layer, and an outer cover, wherein the inner tube and the outer cover contain a thermoplastic elastomer composition comprised of a thermoplastic resin in which is blended an at least partially cross-linked elastomer component, the reinforcing layer is a brass-plated wire, and the reinforcing layer and inner tube and the reinforcing layer and outer cover have between them a maleic-acid-modified polyolefin thermoplastic resin.
摘要翻译： PCT No.PCT / JP97 / 03987第 371日期：1998年7月2日 102（e）日期1998年7月2日PCT 1997年10月31日PCT公布。 WO98 / 20068 PCT出版物日期1998年5月14日一种含有组分（A）（热塑性聚烯烃树脂），组分（B）（含环氧基的乙烯丙烯酸酯共聚物橡胶）和组分（C）（酸改性聚烯烃树脂）的热塑性弹性体组合物，组分（A）的连续相，其中组分（B）作为分散相分散并通过过氧化物交联; 包含热塑性聚烯烃树脂（A）的连续相和含环氧基的乙烯 - 丙烯酸酯共聚物橡胶组分（B）和丙烯腈丁二烯橡胶组分（C）的分散相的热塑性弹性体组合物，其动态交联链接以及具有内管，至少一个加强层和外盖的软管，其中内管和外盖包含由热塑性树脂组成的热塑性弹性体组合物，其中将至少部分交联的弹性体组分加强层是镀黄铜丝，并且增强层和内管以及增强层和外盖之间具有马来酸改性的聚烯烃热塑性树脂。

2. 发明授权

US06538066B2 Thermoplastic elastomer composition and process for producing the same and pneumatic tire and hose using the same 有权
标题翻译：热塑性弹性体组合物及其制造方法及使用其的充气轮胎和软管
公开(公告)号：US06538066B2
公开(公告)日：2003-03-25
申请号：US09800782
申请日：2001-03-08
申请人： Jiro Watanabe , Kazuto Yamakawa , Daisuke Kanenari , Noriaki Kuroda , Gou Kawaguchi , Yuichi Hara , Tetsuji Kawazura , Shigeru Yamauchi , Hideo Nemoto
发明人： Jiro Watanabe , Kazuto Yamakawa , Daisuke Kanenari , Noriaki Kuroda , Gou Kawaguchi , Yuichi Hara , Tetsuji Kawazura , Shigeru Yamauchi , Hideo Nemoto
IPC分类号： C08L4700
CPC分类号： C08L23/02 , B60C1/00 , B60C1/0008 , C08L23/283 , C08L77/00 , C08L2312/00 , Y10T152/10495 , C08L2666/04 , C08L2666/20
摘要： A thermoplastic elastomer composition dynamically vulcanized to a gelation rate of 50 to 95% which is superior in heat resistance and durability while maintaining flexibility and superior in air permeation preventive property which can be efficiently used as, for example, a pneumatic tire as an air permeation preventive layer.
摘要翻译：一种热塑性弹性体组合物，其动态硫化至50至95％的凝胶化速率，其耐热性和耐久性优异，同时保持柔软性和优异的防透气性，可有效地用作例如充气轮胎作为空气渗透预防层。

3. 发明授权

US06861470B2 Thermoplastic elastomer composition and process for producing the same and pneumatic tire and hose using the same 有权
标题翻译：热塑性弹性体组合物及其制造方法及使用其的充气轮胎和软管
公开(公告)号：US06861470B2
公开(公告)日：2005-03-01
申请号：US10347283
申请日：2003-01-21
申请人： Jiro Watanabe , Kazuto Yamakawa , Daisuke Kanenari , Noriaki Kuroda , Gou Kawaguchi , Yuichi Hara , Tetsuji Kawazura , Shigeru Yamauchi , Hideo Nemoto
发明人： Jiro Watanabe , Kazuto Yamakawa , Daisuke Kanenari , Noriaki Kuroda , Gou Kawaguchi , Yuichi Hara , Tetsuji Kawazura , Shigeru Yamauchi , Hideo Nemoto
IPC分类号： B60C1/00 , C08L23/02 , C08L23/28 , C08L77/00 , C98L77/00
CPC分类号： C08L23/02 , B60C1/00 , B60C1/0008 , C08L23/283 , C08L77/00 , C08L2312/00 , Y10T152/10495 , C08L2666/04 , C08L2666/20
摘要： A thermoplastic elastomer composition dynamically vulcanized to a gelation rate of 50 to 95% which is superior in heat resistance and durability while maintaining flexibility and superior in air permeation preventive property which can be efficiently used as, for example, a pneumatic tire as an air permeation preventive layer. The method includes mixing a composition (C) mixed under conditions of a ratio of melt viscosities of the rubber composition (A)/resin (B) of 0.8 to 1.2 and the formula (φA/φB)×(ηB/ηA)
摘要翻译：一种热塑性弹性体组合物，其动态硫化至50至95％的凝胶化速率，其耐热性和耐久性优异，同时保持柔软性和优异的防透气性，可有效地用作例如充气轮胎作为空气渗透预防层。该方法包括将橡胶组合物（A）/树脂（B）的熔融粘度比为0.8〜1.2，式（phiA / phiB）×（etaB / etaA））1.0的混合条件下混合的组合物（C）在橡胶组合物（D）/组合物（C）的熔体粘度比为0.8至1.2和式（phiD / phiC）x（etaC / etaD）<1.0的条件下，其中phiA：橡胶组合物的体积分数 A），phiB：树脂（B）的体积分数，etaA：橡胶组合物（A）的熔融粘度，etaB：树脂（B）的熔融粘度，phiC：组合物的体积分数（C），phiD：橡胶体积分数组成（D），etaC：组合物（C）的熔融粘度，etaD：橡胶组合物（D）的熔融粘度。

4. 发明授权

US06359071B1 Thermoplastic elastomer composition, process for producing the same, and pneumatic tire and hose made with the same 有权
标题翻译：热塑性弹性体组合物及其制造方法，以及由其制成的充气轮胎和软管
公开(公告)号：US06359071B1
公开(公告)日：2002-03-19
申请号：US09380588
申请日：1999-12-07
申请人： Jiro Watanabe , Kazuto Yamakawa , Daisuke Kanenari , Noriaki Kuroda , Gou Kawaguchi , Yuichi Hara , Tetsuji Kawazura , Shigeru Yamauchi , Hideo Nemoto
发明人： Jiro Watanabe , Kazuto Yamakawa , Daisuke Kanenari , Noriaki Kuroda , Gou Kawaguchi , Yuichi Hara , Tetsuji Kawazura , Shigeru Yamauchi , Hideo Nemoto
IPC分类号： C08L7700
CPC分类号： C08L23/02 , B60C1/00 , B60C1/0008 , C08L23/283 , C08L77/00 , C08L2312/00 , Y10T152/10495 , C08L2666/04 , C08L2666/20
摘要： A thermoplastic elastomer composition dynamically vulcanized to a gelation rate of 50 to 95% which is superior in heat resistance and durability while maintaining flexibility and superior in air permeation preventive property which can be efficiently used as, for example, a pneumatic tire as an air permeation preventive layer. In particular, a thermoplastic elastomer composition having a reduced particle size of the domain rubber is produced by a material having a high rubber ratio by mixing a composition (C) mixed under conditions of a ratio of melt viscosities of the rubber composition (A)/resin (B) of 0.8 to 1.2 and the formula (&phgr;A/&phgr;B)×(&eegr;B/&eegr;A)
摘要翻译：一种热塑性弹性体组合物，其动态硫化至50至95％的凝胶化速率，其耐热性和耐久性优异，同时保持柔软性和优异的防透气性，可有效地用作例如充气轮胎作为空气渗透预防层。特别地，通过混合在橡胶组合物（A）/（A）的熔体粘度的比例的条件下混合的组合物（C），通过使用具有高橡胶比的材料来制造具有减小的领域橡胶粒径的热塑性弹性体组合物，在橡胶组合物（D）/组合物（C）的熔融粘度比为0.8〜1.2的条件下，树脂（B）为0.8〜1.2，式（phiA / phiB）x（etaB / etaA）公式（phiD / phiC）x（etaC / etaD）<1.0，其中phiA：橡胶组合物（A）的体积分数，phiB：树脂（B）的体积分数，etaA：橡胶组合物（A）的熔融粘度，etaB：树脂（B）的熔融粘度，phiC：组合物（C）的体积分数，phiD：橡胶组合物的体积分数（D），etaC：组合物（C）的熔融粘度，etaD：橡胶组合物（D）的熔融粘度。

5. 发明申请

US20050103417A1 Thermoplastic elastomer composition and process for producing the same and pneumatic tire and hose using the same 有权
标题翻译：热塑性弹性体组合物及其制造方法及使用其的充气轮胎和软管
公开(公告)号：US20050103417A1
公开(公告)日：2005-05-19
申请号：US11008962
申请日：2004-12-13
申请人： Jiro Watanabe , Yuichi Hara , Shigeru Yamauchi , Hideo Nemoto
发明人： Jiro Watanabe , Yuichi Hara , Shigeru Yamauchi , Hideo Nemoto
IPC分类号： B60C1/00 , C08L23/02 , C08L23/28 , C08L77/00 , B60C5/12 , B60C5/14
CPC分类号： C08L23/02 , B60C1/00 , B60C1/0008 , C08L23/283 , C08L77/00 , C08L2312/00 , Y10T152/10495 , C08L2666/04 , C08L2666/20
摘要： A thermoplastic elastomer composition dynamically vulcanized to a gelation rate of 50 to 95% which is superior in heat resistance and durability while maintaining flexibility and superior in air permeation preventive property which can be efficiently used as, for example, a pneumatic tire as an air permeation preventive layer. In particular, a thermoplastic elastomer composition having a reduced particle size of the domain rubber is produced by a material having a high rubber ratio by mixing a composition (C) mixed under conditions of a ratio of melt viscosities of the rubber composition (A)/resin (B) of 0.8 to 1.2 and the formula (φA/φB)×(ηB/ηA)
摘要翻译：一种热塑性弹性体组合物，其动态硫化至50至95％的凝胶化速率，其耐热性和耐久性优异，同时保持柔软性和优异的防透气性，可有效地用作例如充气轮胎作为空气渗透预防层。特别地，通过混合在橡胶组合物（A）/（A）的熔体粘度的比例的条件下混合的组合物（C），通过使用具有高橡胶比的材料来制造具有减小的领域橡胶粒径的热塑性弹性体组合物，树脂（B）为0.8〜1.2，通式（i> i i i i i <<<<<<<<<<<<<<<<<<<<<<<<<<< 橡胶组合物（D）/组合物（C）的熔体粘度比为0.8〜1.2和式（phi / D / C / C）的条件下， /SUB>）x(eta_C/eta_D)1.0，其中橡胶组合物（A）的体积分数，phi B：树脂（B）的体积分数，ηA：橡胶组合物（A）的熔融粘度，乙烯B：树脂的熔融粘度（B），化合物（C）的体积分数，橡胶组合物（D）的体积分数，ηC ：组合物（C）的熔融粘度，η的熔体粘度：r的熔体粘度 ubber组成（D）。另外，具有作为分散相的弹性体组合物（A）和热塑性树脂组合物（B）作为基质并具有由至少两种热塑性树脂的共混物组成的热塑性树脂组合物的热塑性弹性体组合物。

6. 发明授权

US07275574B2 Thermoplastic elastomer composition and process for producing the same and pneumatic tire and hose using the same 有权
标题翻译：热塑性弹性体组合物及其制造方法及使用其的充气轮胎和软管
公开(公告)号：US07275574B2
公开(公告)日：2007-10-02
申请号：US11008962
申请日：2004-12-13
申请人： Jiro Watanabe , Yuichi Hara , Shigeru Yamauchi , Hideo Nemoto
发明人： Jiro Watanabe , Yuichi Hara , Shigeru Yamauchi , Hideo Nemoto
IPC分类号： B60C5/00 , C08L77/00
CPC分类号： C08L23/02 , B60C1/00 , B60C1/0008 , C08L23/283 , C08L77/00 , C08L2312/00 , Y10T152/10495 , C08L2666/04 , C08L2666/20
摘要： Thermoplastic elastomer composition dynamically vulcanized with a 50 to 95% gelation rate has superior heat resistance, durability, and air permeation prevention, is flexible and usable as a pneumatic tire air permeation preventive layer. A composition having reduced domain rubber particle size is produced from a high rubber ratio material by mixing composition (C) under melt viscosities ratio of rubber composition (A)/resin (B) of 0.8 to 1.2 and formula (φA/φB)×(ηB/ηA)
摘要翻译：以50〜95％凝胶化速度动态硫化的热塑性弹性体组合物具有优异的耐热性，耐久性和防透气性，是柔性的，可用作充气轮胎防气层。通过在橡胶组合物（A）/树脂（B）的熔融粘度比为0.8〜1.2和式（phi A）之间混合组合物（C），由高橡胶比材料制造具有减小的畴橡胶粒径的组合物， /SUB>/phi_B)x(eta_B/eta_A)1.0在橡胶组合物（D）/组合物的熔体粘度比下（C）为0.8至1.2和式（i> i i i SUB SUB SUB SUB SUB SUB SUB SUB SUB SUB SUB SUB SUB SUB SUB SUB SUB SUB SUB >）<1.0，其中phiA，i i i i i i>>>>>>>>>>>>>>>>>>>>>> rubber rubber rubber 组合物（A）和树脂（B），组合物（C）和橡胶组合物（D）分别为乙烯，乙烯和/ >和η'分别是橡胶组合物（A），树脂（B），组合物（C）和橡胶组合物（D）的熔体粘度。热塑性弹性体组合物可以具有弹性体组合物（A）分散相和热塑性树脂组合物（B）基质。

7. 发明授权

US09604424B2 Method of manufacturing pneumatic tire 有权
公开(公告)号：US09604424B2
公开(公告)日：2017-03-28
申请号：US14367726
申请日：2012-08-08
申请人： Hideki Seto , Yuichi Hara , Hirokazu Shibata
发明人： Hideki Seto , Yuichi Hara , Hirokazu Shibata
IPC分类号： B29D30/06 , B29D30/30 , B26D3/00 , B26F3/08 , B26D1/00
CPC分类号： B29D30/3042 , B26D3/003 , B26D2001/0053 , B26D2001/0086 , B26F3/08 , B29D30/0681 , B29D2030/0682 , B60C2005/145 , B60C2005/147
摘要： The present technology provides a method of manufacturing a pneumatic tire. The method of manufacturing a pneumatic tire uses a laminated sheet having a predetermined length and an inner liner layer formed from the laminated sheet through a step of cure-molding the tire with end portions of the laminated sheet lap-spliced. In the method, when at least the sheet made of thermoplastic resin or a thermoplastic resin composition obtained by blending the thermoplastic resin and the elastomer is cut into the predetermined length, the cutting is performed by using an edge tool having a non-sharp edge under a temperature condition not lower than 60° C. and not higher than a melting point of the thermoplastic resin.

8. 发明申请

US20150225561A1 THERMOPLASTIC ELASTOMER COMPOSITION AND PROCESS TO PRODUCE SAME 审中-公开
标题翻译：热塑性弹性体组合物及其制备方法
公开(公告)号：US20150225561A1
公开(公告)日：2015-08-13
申请号：US14409012
申请日：2012-06-19
申请人： Yuichi Hara , Shun Sato , Edward John Blok , Maria D. Ellul , Anthony J. Dias , Randal Howard Kerstetter, III
发明人： Yuichi Hara , Shun Sato , Edward John Blok , Maria D. Ellul , Anthony J. Dias , Randal Howard Kerstetter, III
IPC分类号： C08L23/28
CPC分类号： C08L23/283 , C08K5/18 , C08L23/16 , C08L2201/08 , C08L2207/04 , C08L2312/00 , C08L77/00
摘要： Disclosed herein is a thermoplastic elastomer composition having improved uv and processability, comprising a post-vulcanized dynamically vulcanized alloy (DVA) and a low molecular weight aromatic amine stabilizer, wherein the DVA comprises an isobutylene elastomeric component dispersed as a domain in a continuous phase comprising at least one thermoplastic resin. A method to produce the thermoplastic elastomer composition is also disclosed.
摘要翻译：本文公开了具有改进的紫外线和加工性的热塑性弹性体组合物，其包含后硫化动态硫化合金（DVA）和低分子量芳族胺稳定剂，其中所述DVA包含分散在连续相中的结构域的异丁烯弹性体组分，至少一种热塑性树脂。还公开了一种制备热塑性弹性体组合物的方法。

9. 发明申请

US20130144010A1 METHOD FOR PRODUCING THERMOPLASTIC RESIN COMPOSITIONS 有权
标题翻译：生产热塑性树脂组合物的方法
公开(公告)号：US20130144010A1
公开(公告)日：2013-06-06
申请号：US13816861
申请日：2011-05-19
申请人： Koichi Kawaguchi , Yuichi Hara
发明人： Koichi Kawaguchi , Yuichi Hara
IPC分类号： C08L29/02 , C08L21/00 , C08L77/00
CPC分类号： C08L29/02 , B60C1/0008 , C08J3/203 , C08J5/18 , C08J2377/02 , C08J2377/06 , C08J2423/26 , C08L21/00 , C08L23/0861 , C08L23/0884 , C08L23/26 , C08L51/06 , C08L77/00 , C08L77/02 , C08L77/06 , F16L9/12 , F16L11/04 , F16L11/085 , F16L2011/047
摘要： Provided is a method for producing thermoplastic resin compositions, the method comprising the step of melt-blending (A) a thermoplastic elastomer composition, obtained by dispersing (ii) an acid anhydride-modified or epoxy-modified rubber in (i) an ethylene-vinyl alcohol copolymer, with (B-1) a resin composition comprising at least one resin selected from (i) unmodified polyamide resins and modified polyamide resins or (B-2) a thermoplastic elastomer composition obtained by dispersing (ii) an acid anhydride-modified or epoxy-modified rubber in (i) at least one resin selected from unmodified polyamide resins and modified polyamide resins. Said thermoplastic elastomer composition has excellent gas barrier properties and the decrease in gas barrier properties associated with fatigue has been reduced.
摘要翻译：提供一种热塑性树脂组合物的制造方法，其特征在于，包括使（A）通过将（ⅱ）酸酐改性或环氧改性橡胶分散在（ⅰ）乙烯 - 乙烯醇共聚物，（B-1）含有选自（i）未改性的聚酰胺树脂和改性聚酰胺树脂中的至少一种树脂的树脂组合物或（B-2）通过将（ii）酸酐 - （i）选自未改性的聚酰胺树脂和改性聚酰胺树脂中的至少一种树脂的改性或环氧改性橡胶。所述热塑性弹性体组合物具有优异的气体阻隔性能，并且与疲劳相关的气体阻隔性能的降低已经降低。

10. 发明申请

US20120136100A1 THERMOPLASTIC ELASTOMER COMPOSITION 有权
标题翻译：热塑性弹性体组合物
公开(公告)号：US20120136100A1
公开(公告)日：2012-05-31
申请号：US13368539
申请日：2012-02-08
申请人： Yuichi Hara , Naoyuki Morooka
发明人： Yuichi Hara , Naoyuki Morooka
IPC分类号： C08K5/435 , C08L77/02
CPC分类号： B60C1/0008 , C08K5/0016 , C08K5/435 , C08L23/28 , C08L23/283 , C08L77/02 , C08L77/06 , C08L77/10 , C08L2207/04 , C08L2312/00 , C08L2666/20
摘要： Provided is a thermoplastic elastomer composition, which includes a halogenated isoolefin/para-alkylstyrene copolymer rubber dispersed in a polyamide resin in order to improve the fatigue durability of a polyamide resin, while maintaining high flowability of the polyamide. A thermoplastic elastomer composition comprising a continuous phase composed of a modified polyamide resin (A) and a dispersed phase composed of a halogenated isoolefin/para-alkylstyrene copolymer rubber (B) is provided. The modified polyamide resin (A) is a resin obtained by melt-kneading 100 parts by weight of a polyamide resin (C) with not less than 0.05 part by weight and less than 3 parts by weight a compound (D), such as a monofunctional epoxy compound, capable of binding to a terminal amino group of the polyamide resin at a temperature not lower than the melting point of the polyamide resin (C). The composition can be used as an inner liner of a pneumatic tire.
摘要翻译：提供一种热塑性弹性体组合物，其包含分散在聚酰胺树脂中的卤化异烯烃/对烷基苯乙烯共聚物橡胶，以提高聚酰胺树脂的疲劳耐久性，同时保持聚酰胺的高流动性。提供了包含由改性聚酰胺树脂（A）构成的连续相和由卤代异烯烃/对烷基苯乙烯共聚物橡胶（B）组成的分散相的热塑性弹性体组合物。改性聚酰胺树脂（A）是通过将100重量份的聚酰胺树脂（C）以0.05重量份以上且小于3重量份的化合物（D），如能够在不低于聚酰胺树脂（C）的熔点的温度下与聚酰胺树脂的末端氨基结合的单官能环氧化合物。组合物可以用作充气轮胎的内衬。

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