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1. 发明专利

JP2011113703A Solid polymer fuel cell 有权
标题翻译：固体聚合物燃料电池
公开(公告)号：JP2011113703A
公开(公告)日：2011-06-09
申请号：JP2009267160
申请日：2009-11-25
申请人： Hitachi Ltd , 株式会社日立製作所
发明人： ONUMA ATSUHIKO , MORISHIMA SHIN , KAWAJI JUN
IPC分类号： H01M8/02 , H01M8/10
CPC分类号： Y02E60/523
摘要： PROBLEM TO BE SOLVED: To provide an inexpensive solid polymer electrolyte membrane having excellent mechanical characteristics and oxidation resistance, and to provide a solid polymer fuel cell high in output and high in durability (long life).
SOLUTION: The solid polymer fuel cell includes: a solid polymer electrolyte membrane/electrode conjugant obtained by joining solid polymer electrolyte membranes 24 and 25 and electrode catalyst layers 12 and 13 to be integrated; and gas diffusion layers 14 and 15 formed on both surfaces of the solid polymer electrolyte membrane/electrode conjugant. The gas diffusion layers 14 and 15 are formed so that entire surfaces of the electrode catalyst layers 12 and 13 are covered with the gas diffusion layers, and the periphery 40 of a projected image of each gas diffusion layer from the vertical direction is included in a surface of the solid polymer electrolyte membrane 24. The solid polymer electrolyte membrane has: the center 25 including at least a part where the electrode catalyst layers 12 and 13 are joined; and the peripheral section 24 in a range between the periphery 41 of the solid polymer electrolyte membrane and at least a position of the periphery 40 of each projected image of the gas diffusion layers 14 and 15. An ion exchange capacity of a polymer material at the peripheral section 24 is smaller than that of a polymer material at the center 25.
COPYRIGHT: (C)2011,JPO&INPIT
摘要翻译：要解决的问题：提供具有优异的机械特性和抗氧化性的廉价的固体聚合物电解质膜，并且提供高产出和高耐久性（长寿命）的固体聚合物燃料电池。固体聚合物燃料电池包括：通过将固体聚合物电解质膜24和25与电极催化剂层12和13接合而获得的固体聚合物电解质膜/电极共轭体，以一体化; 以及形成在固体高分子电解质膜/电极共轭体的两面的气体扩散层14,15。气体扩散层14和15形成为使得电极催化剂层12和13的整个表面被气体扩散层覆盖，并且每个气体扩散层的垂直方向的投影图像的周边40包括在该固体高分子电解质膜具有：至少包含电极催化剂层12,13的一部分的中心25; 以及周边部分24在固体聚合物电解质膜的周边41与气体扩散层14和15的每个投影图像的至少周边40的位置之间的范围内。在该处，聚合物材料的离子交换容量周边部分24小于中心部分25的聚合物材料。版权所有：（C）2011，JPO＆INPIT

2. 发明专利

JP2013196915A Solid polymer electrolyte for fuel cell 审中-公开
标题翻译：固体聚合物电解质燃料电池
公开(公告)号：JP2013196915A
公开(公告)日：2013-09-30
申请号：JP2012063005
申请日：2012-03-21
申请人： Hitachi Ltd , 株式会社日立製作所
发明人： ONUMA ATSUHIKO , TAKAMORI YOSHIYUKI , KAWAJI JUN
IPC分类号： H01M8/02 , C08G81/00 , H01B1/06 , H01M8/10
CPC分类号： C08J5/2256 , C08J2300/10 , C08J2387/00 , H01B1/122 , H01M8/1023 , H01M8/1025 , H01M8/1027 , H01M8/1032 , Y02E60/523
摘要： PROBLEM TO BE SOLVED: To provide a solid polymer electrolyte membrane for a direct methanol type fuel cell, high in ion conductivity and low in methanol permeability.SOLUTION: A solid polymer electrolyte for a direct methanol type fuel cell includes a block copolymer comprising a hydrophilic segment and a hydrophobic segment which contain an ion exchange group. The hydrophobic segment includes a structural unit represented by general formula (1), a number average molecular weight Mn of the hydrophobic segment is 2.0×10-1.0×10in terms of GPC, and a ratio between a number average molecular weight Mn of the hydrophilic segment and the number average molecular weight of the hydrophobic segment is 2.0-5.0.
摘要翻译：要解决的问题：提供用于直接甲醇型燃料电池的固体高分子电解质膜，离子传导性高，甲醇渗透性低。解决方案：用于直接甲醇型燃料电池的固体聚合物电解质包括含有亲水性的嵌段共聚物片段和含有离子交换基团的疏水片段。疏水性链段包括由通式（1）表示的结构单元，疏水性链段的数均分子量Mn为GPC为2.0×10-1.0×10，亲水性的数均分子量Mn 片段和疏水片段的数均分子量为2.0-5.0。

3. 发明专利

JP2013157227A Direct alcohol type fuel cell 审中-公开
标题翻译：直接酒精型燃料电池
公开(公告)号：JP2013157227A
公开(公告)日：2013-08-15
申请号：JP2012017482
申请日：2012-01-31
申请人： Hitachi Ltd , 株式会社日立製作所
发明人： KAWAJI JUN , SUZUKI SHUICHI , MIZUKAMI TAKAAKI , ANDO SHINSUKE , ONUMA ATSUHIKO
IPC分类号： H01M8/02 , H01M8/10
CPC分类号： Y02E60/522
摘要： PROBLEM TO BE SOLVED: To provide a direct alcohol type fuel cell with a long life by preventing deterioration and breakage of an electrolyte membrane at an electrode outer periphery accompanied with continuous power generation.SOLUTION: A direct alcohol type fuel cell comprises: a pair of anode and cathod provided on both faces of a solid polymer electrolyte membrane; a non-ion conductive frame body provided on a surface of the solid polymer electrolyte membrane and covering peripheries of the anode and the cathode; and a conductive plate opposed to the anode and the cathode and having a reaction gas passage. The anode, the cathode and the frame body are arranged to have a first region, in which an end of the cathode is positioned on an outer side than an inner peripheral edge of the frame body provided on the anode side, and a second region, in which the end of the cathode and the end of the anode are at the same position or the end of the cathode is positioned on an inner side than the end of the anode. The end of the cathode adjacent to a manifold for supplying fuel provided on the solid polymer membrane and the conductive plate serves as the first region.
摘要翻译：要解决的问题：通过防止伴随连续发电的电极外周处的电解质膜的劣化和断裂来提供具有长寿命的直链醇型燃料电池。解决方案：直链醇型燃料电池包括：一对设置在固体聚合物电解质膜的两面上的阳极和阴极; 设置在固体聚合物电解质膜的表面上并覆盖阳极和阴极的周边的非离子导电性框架体; 和与阳极和阴极相对的并具有反应气体通道的导电板。阳极，阴极和框架体被布置成具有第一区域，其中阴极的端部位于设置在阳极侧的框架体的内周边缘的外侧上，第二区域，其中阴极的端部和阳极的端部处于相同的位置或阴极的端部位于比阳极的端部更靠内侧。靠近用于供给设置在固体聚合物膜上的燃料的歧管的阴极的端部和导电板用作第一区域。

4. 发明专利

JP2011113799A Membrane electrode assembly and fuel cell using the same 有权
标题翻译：膜电极组件和使用它的燃料电池
公开(公告)号：JP2011113799A
公开(公告)日：2011-06-09
申请号：JP2009268893
申请日：2009-11-26
申请人： Hitachi Ltd , 株式会社日立製作所
发明人： KAWAJI JUN , MORISHIMA SHIN , SUZUKI SHUICHI , TAKAMORI YOSHIYUKI , ONUMA ATSUHIKO
IPC分类号： H01M4/96 , H01M4/88 , H01M8/02 , H01M8/10
CPC分类号： H01M4/881 , H01M4/8652 , H01M4/8663 , H01M4/8828 , H01M4/926 , H01M8/1007 , Y02P70/56
摘要： PROBLEM TO BE SOLVED: To provide a membrane electrode assembly for a fuel cell that prevents entry of a binder resin into micropores of catalyst carrying carbon, thereby improving the effective utilization factor and the material diffusibility of a catalyst metal, and to provide a method of manufacturing the same.
SOLUTION: The membrane electrode assembly includes an anode, a cathode and a solid polymer electrolyte membrane, and has a configuration in which the solid polymer electrolyte membrane is sandwiched between the anode and the cathode. Carbon structures, formed of a plurality of carbon primary particles carrying catalyst particles, are contained in the anode and the cathode. Particulate media, having solid polymer electrolyte on the surfaces, are contained between the adjacent carbon structures.
COPYRIGHT: (C)2011,JPO&INPIT
摘要翻译：解决的问题：提供一种用于燃料电池的膜电极组件，其防止粘合剂树脂进入催化剂载体碳的微孔中，从而提高催化剂金属的有效利用率和材料扩散性，并提供其制造方法。解决方案：膜电极组件包括阳极，阴极和固体聚合物电解质膜，并且具有将固体聚合物电解质膜夹在阳极和阴极之间的构造。由负载催化剂颗粒的多个碳一次颗粒形成的碳结构包含在阳极和阴极中。在表面上具有固体聚合物电解质的颗粒介质包含在相邻的碳结构之间。版权所有（C）2011，JPO＆INPIT

5. 发明专利

JP2010108908A Fuel cell 有权
标题翻译：燃料电池
公开(公告)号：JP2010108908A
公开(公告)日：2010-05-13
申请号：JP2009154520
申请日：2009-06-30
申请人： Hitachi Ltd , 株式会社日立製作所
发明人： KAWAJI JUN , MORISHIMA SHIN , SUZUKI SHUICHI , TAKAMORI YOSHIYUKI , ONUMA ATSUHIKO , MOGI AKIRA
IPC分类号： H01M8/02 , H01M4/86 , H01M8/10
CPC分类号： Y02E60/523 , Y02P70/56
摘要： PROBLEM TO BE SOLVED: To provide a structure of a membrane-electrode assembly suppressing deterioration and breakage of an electrolyte membrane in the outer peripheral region of an electrode by suppressing the generation of hydrogen peroxide at an electrode end part in a fuel cell and the diffusion of hydrogen peroxide to the outer peripheral region of the electrode, to provide its constituent material, its manufacturing method, and to provide a fuel cell using the membrane-electrode assembly. SOLUTION: The fuel cell is configured such that at least one of an anode and a cathode is embedded in a solid polymer electrolyte membrane, and the thickness of an electrolyte in the periphery of the electrode is larger than the sum of the thickness of the electrode between electrodes, the thickness of the anode and the thickness of the cathode. COPYRIGHT: (C)2010,JPO&INPIT
摘要翻译：要解决的问题：通过抑制在燃料电池的电极端部产生过氧化氢，提供抑制电极外周区域中的电解质膜的劣化和断裂的膜 - 电极组件的结构以及过氧化氢扩散到电极的外周区域，提供其构成材料及其制造方法，并提供使用该膜 - 电极组件的燃料电池。解决方案：燃料电池被构造为使得阳极和阴极中的至少一个嵌入固体聚合物电解质膜中，并且电极周围的电解质的厚度大于厚度的总和的电极之间的电极，阳极的厚度和阴极的厚度。版权所有（C）2010，JPO＆INPIT

6. 发明专利

JP2012059406A Membrane electrode assembly 审中-公开
标题翻译：膜电极组件
公开(公告)号：JP2012059406A
公开(公告)日：2012-03-22
申请号：JP2010199047
申请日：2010-09-06
申请人： Hitachi Ltd , 株式会社日立製作所
发明人： ASANO NAOKI , UESHIMA KOICHI , ONUMA ATSUHIKO , MORISHIMA SHIN
IPC分类号： H01M8/02 , C08J5/22 , H01M8/10
CPC分类号： Y02E60/521
摘要： PROBLEM TO BE SOLVED: To provide a membrane electrode assembly which has excellent long-period durability and output characteristics.SOLUTION: The membrane electrode assembly includes a catalyst layer and a hydrocarbon electrolyte membrane. The hydrocarbon electrolyte membrane has a hydrophilic part, a hydrophobic part, and a crosslinked structure, and the hydrophilic part has a specific structure having a proton acid group selected from the group consisting of a sulfonate group (-SOH) and a phosphate group (-POH).
摘要翻译：要解决的问题：提供一种具有优异的长周期耐久性和输出特性的膜电极组件。解决方案：膜电极组件包括催化剂层和烃电解质膜。烃电解质膜具有亲水部分，疏水部分和交联结构，亲水部分具有选自磺酸酯基（-SO 3 H）和磷酸基（-PO 3 2 ）。版权所有（C）2012，JPO＆INPIT

7. 发明专利

JP2011216380A Solid polymer electrolyte fuel cell 审中-公开
标题翻译：固体聚合物电解质燃料电池
公开(公告)号：JP2011216380A
公开(公告)日：2011-10-27
申请号：JP2010084761
申请日：2010-04-01
申请人： Hitachi Ltd , 株式会社日立製作所
发明人： ONUMA ATSUHIKO , MORISHIMA SHIN
IPC分类号： H01M8/02 , H01M4/86 , H01M8/10
CPC分类号： Y02E60/521
摘要： PROBLEM TO BE SOLVED: To provide a solid polymer electrolyte fuel cell using a hydrocarbonaceous polymer as an inexpensive raw material having improved mechanical characteristics and oxidation resistance for a polymer electrolyte membrane, and having combined reduced cost, high output and high durability (long life) by minimizing the effects of peroxide or peroxide radicals even when produced along with power generation.SOLUTION: The solid polymer electrolyte fuel cell includes a membrane-electrode assembly having the polymer electrolyte membrane and electrode catalyst layers arranged on both sides of the polymer electrolyte membrane and integrally joined thereto, and gas diffusion layers provided on both sides of the membrane-electrode assembly in contact with the electrode catalyst layers. The electrode catalyst layers each consist of a membrane-shaped electrode catalyst part where power-generation electrode reaction takes place, and a ring-shaped peroxide decomposing part containing a peroxide decomposing catalyst and formed on the outer periphery of the electrode catalyst part. The main surface of the electrode catalyst layer is larger than that of the gas diffusion layer, and the whole main surface on one side of the electrode catalyst layer is joined to the polymer electrode membrane.
摘要翻译：要解决的问题：为了提供一种使用含烃聚合物作为廉价原料的固体聚合物电解质燃料电池，其对于聚合物电解质膜具有改进的机械特性和抗氧化性，并且具有组合的降低成本，高产出和高耐久性（长寿命）通过最小化过氧化物或过氧化物自由基的作用，即使当与发电一起产生时也是如此。解决方案：固体聚合物电解质燃料电池包括具有聚合物电解质膜和布置在聚合物电解质膜两侧的电极催化剂层的膜 - 电极组件，和与电极催化剂层接触的设置在膜 - 电极组件两侧的气体扩散层。电极催化剂层各自由发生发电电极反应的膜状电极催化剂部分和形成在电极催化剂部分的外周上的含有过氧化物分解催化剂的环状过氧化物分解部构成。电极催化剂层的主表面大于气体扩散层的主表面，电极催化剂层一侧的整个主表面与聚合物电极膜接合。

8. 发明专利

JP2010189503A Block copolymer, solid polymer electrolyte for fuel cell using the same, solid polymer electrolyte membrane for fuel cell, membrane electrode assembly, and fuel cell 有权
标题翻译：用于燃料电池的固体聚合物电解质，用于燃料电池，膜电极组件和燃料电池的固体聚合物电解质膜
公开(公告)号：JP2010189503A
公开(公告)日：2010-09-02
申请号：JP2009033771
申请日：2009-02-17
申请人： Hitachi Ltd , 株式会社日立製作所
发明人： ONUMA ATSUHIKO , MORISHIMA SHIN , ASANO NAOKI
IPC分类号： C08G81/00 , C08G61/00 , H01B1/06 , H01M8/02 , H01M8/10
CPC分类号： C08J5/2256 , C08G65/4056 , C08G75/0227 , C08G75/0245 , C08G75/04 , C08G75/23 , C08J2371/12 , C08J2381/06 , C08L2205/05 , H01M8/1025 , H01M8/1027 , H01M8/1032
摘要： PROBLEM TO BE SOLVED: To provide a solid polymer electrolyte for fuel cells which is inexpensive, is excellent in mechanical properties, has oxidation resistance, is high ionic conductivity, and hardly swells. SOLUTION: The solid polymer electrolyte for fuel cells is composed of a block copolymer containing a hydrophilic segment and a hydrophobic segment, wherein the hydrophilic segment has a structural unit expressed by chemical formula (1). COPYRIGHT: (C)2010,JPO&INPIT
摘要翻译：要解决的问题：为了提供廉价的燃料电池用固体聚合物电解质，机械性能优异，具有抗氧化性，离子电导率高，几乎不溶胀。解决方案：用于燃料电池的固体聚合物电解质由含有亲水链段和疏水链段的嵌段共聚物组成，其中亲水链段具有由化学式（1）表示的结构单元。版权所有（C）2010，JPO＆INPIT

9. 发明专利

JP2010116503A Production method of block copolymer using reactive oligomer 审中-公开
标题翻译：使用反应性低聚物制备嵌段共聚物的方法
公开(公告)号：JP2010116503A
公开(公告)日：2010-05-27
申请号：JP2008291437
申请日：2008-11-13
申请人： Hitachi Ltd , 株式会社日立製作所
发明人： FUKUCHI IWAO , ASANO NAOKI , TAKEDA SHINJI , ONUMA ATSUHIKO , MORISHIMA SHIN
IPC分类号： C08G75/23 , H01B1/06 , H01M8/02 , H01M8/10
CPC分类号： Y02P70/56
摘要： PROBLEM TO BE SOLVED: To efficiently provide a block copolymer comprising a hydrophilic aromatic polymer compound having a protonic acid group and a hydrophobic aromatic polymer compound having no protonic acid group. SOLUTION: The block copolymer is produced through steps of: (a) preparing a first aromatic polymer compound having a perfluorobiphenyl group at a molecular end and having a protonic acid group; (b) preparing a second aromatic polymer compound having a reactive group at a molecular end that can react with the perfluorobiphenyl group described in (a) and having no protonic acid group; and (c) preparing a copolymer comprising the first aromatic polymer compound and the second aromatic polymer compound bonded to each other. COPYRIGHT: (C)2010,JPO&INPIT
摘要翻译：要解决的问题：有效提供包含具有质子酸基团的亲水性芳香族高分子化合物和不具有质子酸基团的疏水性芳香族高分子化合物的嵌段共聚物。解决方案：通过以下步骤制备嵌段共聚物：（a）制备在分子末端具有全氟联苯基并具有质子酸基团的第一芳族聚合物化合物; （b）制备在分子端具有反应性基团的第二芳族聚合物化合物，其可以与（a）中所述的全氟联苯基反应并且不具有质子酸基团; 和（c）制备包含彼此键合的第一芳族聚合物化合物和第二芳族聚合物化合物的共聚物。版权所有（C）2010，JPO＆INPIT

10. 发明专利

JP2007329015A Polymer electrolyte membrane, membrane electrode assembly, and fuel cell using it 有权
标题翻译：聚合物电解质膜，膜电极组件和燃料电池
公开(公告)号：JP2007329015A
公开(公告)日：2007-12-20
申请号：JP2006159202
申请日：2006-06-08
申请人： Hitachi Ltd , 株式会社日立製作所
发明人： ONUMA ATSUHIKO , HONBOU HIDETOSHI , KOBAYASHI TOSHIYUKI
IPC分类号： H01M8/02 , H01B1/06 , H01M8/10
CPC分类号： H01M8/1011 , H01M8/1027 , H01M8/1032 , H01M8/1053 , H01M8/106 , H01M2300/0094 , Y02E60/523
摘要： PROBLEM TO BE SOLVED: To provide an electrolyte membrane and a membrane electrode assembly which are low in cost and have a long life since deterioration caused by peroxides generated in an air pole electrode catalyst layer is slow. SOLUTION: The electrolyte membrane has a first electrolyte layer having ion conductivity, a second electrolyte layer which has the ion conductivity, and which is thicker, or larger in the ion-exchange equivalent, or larger in the number average molecular weight than that the first electrolyte membrane has when methanol is brought into contact with the surface, and a porous layer into which an ion conductive electrolyte formed between the first electrode layer and the second electrode layer is impregnated. COPYRIGHT: (C)2008,JPO&INPIT
摘要翻译：解决的问题：提供一种成本低且寿命长的电解质膜和膜电极组件，因为在空气极电极催化剂层中产生的过氧化物引起的劣化是缓慢的。解决方案：电解质膜具有离子传导性的第一电解质层，具有离子传导性的第二电解质层，离子交换当量更大或更大，数均分子量大于数均分子量第一电解质膜在甲醇与表面接触时具有多孔层，并且在第一电极层和第二电极层之间形成有离子导电电解质的多孔层被浸渍。版权所有（C）2008，JPO＆INPIT

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