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1. 发明授权

US06537943B1 Catalyst system composed of metallocenes comprising substituents containing fluorine 失效
标题翻译：由包含含氟取代基的茂金属组成的催化剂体系
公开(公告)号：US06537943B1
公开(公告)日：2003-03-25
申请号：US09673147
申请日：2000-10-11
申请人： Cornelia Fritze , Gerhard Erker , Johannes Ruwwe
发明人： Cornelia Fritze , Gerhard Erker , Johannes Ruwwe
IPC分类号： C08F416
CPC分类号： C08F10/00 , C08F4/65912 , C08F110/06 , Y10S526/943 , C08F4/65925
摘要： The invention relates to a catalyst system composed of metallocenes comprising substituents containing fluorine, a method for producing said system and its use for the polymerization of olefins.
摘要翻译：本发明涉及由包含氟的取代基的茂金属组成的催化剂体系，制备所述体系的方法及其用于烯烃聚合的用途。

2. 发明授权

US5807936A Transition metal compound 失效
标题翻译：过渡金属化合物
公开(公告)号：US5807936A
公开(公告)日：1998-09-15
申请号：US662040
申请日：1996-06-12
申请人： Cornelia Fritze , Hans-Friedrich Herrmann , Gerhard Erker , Johannes Ruwwe
发明人： Cornelia Fritze , Hans-Friedrich Herrmann , Gerhard Erker , Johannes Ruwwe
IPC分类号： B01J31/12 , C07F7/00 , C07F17/00 , C08F4/60 , C08F4/619 , C08F4/64 , C08F4/6592 , C08F10/00
CPC分类号： C07F17/00 , C08F10/00 , C08F4/619 , C08F4/61908 , Y10S526/943
摘要： The present invention relates to a transition metal compound of the formula I L.sub.n (X.sub.m A.sub.t R.sup.1.sub.q).sub.s MY.sub.r (I), where M is a metal atom of group IIIb, IVb, Vb or VIb of the Periodic Table of the Elements, L are identical or different and are each a .pi.-ligand or an electron donor, n is 1, 2, 3 or 4, Y are identical or different and are each a hydrogen atom, a halogen atom or an 1-dentate C.sub.1 -C.sub.40 -group, where l is 1, 2, 3 or 4, r is 0, 1, 2, 3, 4 or 5, and at least one of the radicals L bears at least one group X.sub.m A.sub.t R.sup.1.sub.q, where X are identical or different and are each a hetero atom or a C.sub.1 -C.sub.40 -group, m is 0 or 1, A is an atom of group IIIa, Va or VIa of the Periodic Table of the Elements, t is 1, R.sup.1 are identical or different and are each a C.sub.1 -C.sub.40 -group, q is 1, 2, 3, 4 or 5 and s is an integer from 1 to 20. The transition metal compound of the invention is suitable as a catalyst component for olefin polymerization.
摘要翻译：本发明涉及式In（XmAtR1q）sMYr（I）的过渡金属化合物，其中M是元素周期表IIIb族，IVb族，Vb或VIb族的金属原子，L相同或不同，各自为一个或多个电子给体，n为1,2,3或4，Y为相同或不同的，分别为氢原子，卤素原子或1-齿状的C1-C40-基团，其中l为 1,2,3或4，r为0,1,2,3,4或5，并且至少一个基团L具有至少一个基团XmAtR1q，其中X相同或不同，并且各自为杂原子或 C1-C40组，m为0或1，A为元素周期表IIIa，Va或VIa族的原子，t为1，R1相同或不同，为C1-C40-基团，q为1,2,3,4或5，s为1〜20的整数。本发明的过渡金属化合物适用于烯烃聚合的催化剂成分。

3. 发明授权

US07105690B2 Method for producing transition metal compounds and their use for the polymerization of olefins 失效
公开(公告)号：US07105690B2
公开(公告)日：2006-09-12
申请号：US10297054
申请日：2001-05-30
申请人： Jörg Schottek , Gerhard Erker , Klaus Kunz , Steve Döring
发明人： Jörg Schottek , Gerhard Erker , Klaus Kunz , Steve Döring
IPC分类号： C07F9/28 , C07F7/00 , B01J31/00 , C08F4/44
CPC分类号： C07F17/00 , C08F4/65912 , C08F10/00 , C08F110/02 , C08F210/16 , C08F232/00 , Y10S526/943 , C08F4/6592 , C08F210/14
摘要： The invention relates to a method for producing special transition metal compounds, to novel transition metal compounds and to their use for the polymerization of olefins.

4. 发明授权

US5750752A Transition metal compound 失效
标题翻译：过渡金属化合物
公开(公告)号：US5750752A
公开(公告)日：1998-05-12
申请号：US668790
申请日：1996-06-21
申请人： Michael Riedel , Frank Kuber , Michael Aulbach , Gerhard Erker , Martin Konemann
发明人： Michael Riedel , Frank Kuber , Michael Aulbach , Gerhard Erker , Martin Konemann
IPC分类号： C07F17/00 , C08F4/60 , C08F4/602 , C08F4/6192 , C08F4/622 , C08F4/642 , C08F4/74 , C08F10/00 , B01J31/00
CPC分类号： C07F17/00 , C08F10/00 , C08F4/6192 , Y10S526/943
摘要： The present invention relates to a stereorigid transition metal compound having as ligands a cyclopentadienyl group and a substituted or unsubstituted heteroatom which are connected to one another via a monocyclic or polycyclic ring system, with the cyclopentadienyl group being fused onto the monocyclic or polycyclic ring system. The transition metal compound of the invention is suitable as a catalyst component for olefin polymerization.
摘要翻译：本发明涉及一种具有环戊二烯基配位体和取代或未取代的杂原子的立体刚性过渡金属化合物，它们通过单环或多环系统相互连接，环戊二烯基被稠合在单环或多环系统上。本发明的过渡金属化合物适合用作烯烃聚合的催化剂组分。

5. 发明授权

US06861384B2 Process for preparation of a salt-like chemical compound and its use in catalyst systems for preparing polyolefins 失效
标题翻译：盐类化合物的制备方法及其在制备聚烯烃的催化剂体系中的应用
公开(公告)号：US06861384B2
公开(公告)日：2005-03-01
申请号：US10659163
申请日：2003-09-10
申请人： Jörg Schottek , Gerhard Erker , Gerald Kehr
发明人： Jörg Schottek , Gerhard Erker , Gerald Kehr
IPC分类号： C07F5/02 , C08F4/603 , C08F4/626 , C08F4/6392 , C08F4/659 , C08F4/6592 , C08F10/00 , C08F110/02 , C08F110/06 , C08F4/64 , C07F5/05
CPC分类号： C08F10/00 , C07F5/027 , C08F4/65912 , C08F4/65916 , C08F4/65922 , C08F110/02 , C08F110/06 , Y10S526/943 , C08F4/61908 , C08F4/65908 , C08F4/603 , C08F2500/15
摘要： A process for preparing salt-like compounds of the formula (1), (C6R115)3MR2 (I) where R1 are identical or different and are each a hydrogen atom, a halogen atom, C1-C20-alkyl, C6-C14-aryl, C1-C10-alkoxy, C2-C10-alkenyl, C7-C20-arylalkyl, C7-C20-alkylaryl, C6-C10-aryloxy, C1-C10-haloalkyl, C6-C10-haloaryl, C2-C10-alkynyl or C3-C20-alkylsilyl, M is an element of main group III of the Periodic Table of the Elements, and R2 is a substituted or unsubstituted heterocycle, and the use of such compounds in catalyst systems for preparing polyolefins.
摘要翻译：制备式（1）的盐类化合物的方法，其中R 1相同或不同，各自为氢原子，卤素原子，C 1 -C 20烷基，C 6 -C 14 - 芳基，C 1 -C 10 - 烷氧基，C 2 -C 10 - 烯基，C 7 -C 20 - 芳烷基，C 7 -C 20烷基芳基，C 6 -C 10 - 芳氧基，C 1 -C 10卤代烷基，C 6 -C 10 - 卤代芳基，C 2 -C 10 - 炔基或C 3 -C 20烷基甲硅烷基， M是元素周期表的主要组III的元素，R 2是取代或未取代的杂环，以及这些化合物在催化剂体系中用于制备聚烯烃的用途。

6. 发明授权

US06486277B1 Zwitterionic transition metal compound which contains boron 失效
标题翻译：含有硼的两性离子过渡金属化合物
公开(公告)号：US06486277B1
公开(公告)日：2002-11-26
申请号：US09622205
申请日：2000-08-14
申请人： Gerhard Erker , Gerald Kehr , Jörg Schottek , Roland Kratzer
发明人： Gerhard Erker , Gerald Kehr , Jörg Schottek , Roland Kratzer
IPC分类号： C08F464
CPC分类号： C08F10/00 , C07F17/00 , C08F4/65908 , C08F4/65912 , C08F4/65916 , C08F4/65927 , Y10S526/943 , C08F4/65925
摘要： A boron-containing zwitterionic neutral transition metal compound which can advantageously be used for the polymerization of olefins is described. Here, the use of aluminoxanes, such as methylaluminoxane (MAO), as a cocatalyst can be dispensed with and a high catalyst activity and a good polymer morphology can nevertheless be achieved.
摘要翻译：描述了可有利地用于烯烃聚合的含硼两性离子中性过渡金属化合物。这里，可以省去使用铝氧烷如甲基铝氧烷（MAO）作为助催化剂，并且仍能实现高催化剂活性和良好的聚合物形态。

7. 发明授权

US5710297A Metallocenes, and their use as catalysts 失效
标题翻译：金属茂及其作为催化剂的用途
公开(公告)号：US5710297A
公开(公告)日：1998-01-20
申请号：US712681
申请日：1996-09-13
申请人： Thomas Weller , Michael Aulbach , Frank Kuber , Gerhard Erker , Christian Psiorz , Bernd Bachmann , Frank Osan
发明人： Thomas Weller , Michael Aulbach , Frank Kuber , Gerhard Erker , Christian Psiorz , Bernd Bachmann , Frank Osan
IPC分类号： B01J31/06 , B01J31/22 , C07C13/15 , C07F5/00 , C07F5/06 , C07F7/00 , C07F7/02 , C07F9/00 , C07F17/00 , C08F4/42 , C08F4/60 , C08F4/619 , C08F4/6192 , C08F4/642 , C08F4/659 , C08F4/6592 , C08F10/00 , C08F110/02 , C08F110/06 , C08F210/16 , C08F210/18 , B01J31/00 , C07F7/28
CPC分类号： C08F10/00 , C07F17/00 , C08F110/02 , C08F110/06 , C08F210/16 , C08F210/18 , C08F4/61912 , C08F4/61927 , C08F4/65912 , C08F4/65927 , Y10S526/943
摘要： The present invention relates to a stereorigid metallocene compound containing, as ligands, at least two substituted or unsubstituted cyclopentadienyl groups which are bonded to one another via a monocyclic or polycyclic ring system, where at least one cyclopentadienyl group is fused to the monocyclic or polycyclic ring system, and to a process for the preparation of a cycloolefin copolymer. The cycloolefin copolymers obtained in this way have high tear strengths and are suitable for the production of extrusion parts and injection moldings.
摘要翻译：本发明涉及一种立体刚性茂金属化合物，其含有通过单环或多环系统彼此键合的至少两个取代或未取代的环戊二烯基作为配体，其中至少一个环戊二烯基与单环或多环稠合系统，以及制备环烯烃共聚物的方法。以这种方式获得的环烯烃共聚物具有很高的撕裂强度，适用于生产挤出部件和注射成型品。

8. 再颁专利

USRE40121E1 Transition metal compound 有权
标题翻译：过渡金属化合物
公开(公告)号：USRE40121E1
公开(公告)日：2008-02-26
申请号：US09851643
申请日：2001-05-08
申请人： Gerhard Erker , Bodo Temme , Michael Aulbach , Bernd Bachmann , Frank Küber
发明人： Gerhard Erker , Bodo Temme , Michael Aulbach , Bernd Bachmann , Frank Küber
IPC分类号： C07F7/08 , C07F17/00 , B01J31/00
CPC分类号： C08F10/00 , C07F17/00 , C08F4/61908 , C08F4/61912 , C08F4/61922 , C08F4/65916 , C08F4/65922 , C08F110/02 , C08F110/06 , C08F210/02 , C08F210/16 , C08F4/65908 , C08F2500/03 , C08F2500/17 , C08F2500/15 , C08F2500/12 , C08F2500/16 , C08F232/00 , C08F2500/25 , C08F210/14
摘要： The present invention relates to zwitterionic neutral transition metal compounds. The compounds are suitable as catalyst components for the polymerization of olefins.
摘要翻译：本发明涉及两性离子中性过渡金属化合物。该化合物适用于烯烃聚合的催化剂组分。

9. 发明授权

US5990254A Metallocenes as catalysts in the preparation of cycloolefin copolymers 失效
标题翻译：金属茂作为制备环烯烃共聚物的催化剂
公开(公告)号：US5990254A
公开(公告)日：1999-11-23
申请号：US780179
申请日：1996-12-26
申请人： Thomas Weller , Michael Aulbach , Frank Kuber , Gerhard Erker , Christian Psiorz , Bernd Bachmann , Frank Osan
发明人： Thomas Weller , Michael Aulbach , Frank Kuber , Gerhard Erker , Christian Psiorz , Bernd Bachmann , Frank Osan
IPC分类号： B01J31/06 , B01J31/22 , C07C13/15 , C07F5/00 , C07F5/06 , C07F7/00 , C07F7/02 , C07F9/00 , C07F17/00 , C08F4/42 , C08F4/60 , C08F4/619 , C08F4/6192 , C08F4/642 , C08F4/659 , C08F4/6592 , C08F10/00 , C08F110/02 , C08F110/06 , C08F210/16 , C08F210/18 , C08F232/04
CPC分类号： C08F10/00 , C07F17/00 , C08F110/02 , C08F110/06 , C08F210/16 , C08F210/18 , C08F4/61912 , C08F4/61927 , C08F4/65912 , C08F4/65927 , Y10S526/943
摘要： The present invention relates to a stereorigid metallocene compound containing, as ligands, at least two substituted or unsubstituted cyclopentadienyl groups which are bonded to one another via a monocyclic or polycyclic ring system, where at least one cyclopentadienyl group is fused to the monocyclic or polycyclic ring system, and to a process for the preparation of a cycloolefin copolymer. The cycloolefin copolymers obtained in this way have high tear strengths and are suitable for the production of extrusion parts and injection moldings.
摘要翻译：本发明涉及一种立体刚性茂金属化合物，其含有通过单环或多环系统彼此键合的至少两个取代或未取代的环戊二烯基作为配体，其中至少一个环戊二烯基与单环或多环稠合系统，以及制备环烯烃共聚物的方法。以这种方式获得的环烯烃共聚物具有很高的撕裂强度，适用于生产挤出部件和注射成型品。

10. 发明授权

US06218489B1 Polymerization process using a monocyclopentadienyl compound as a catalyst component 失效
标题翻译：使用单环戊二烯基化合物作为催化剂组分的聚合方法
公开(公告)号：US06218489B1
公开(公告)日：2001-04-17
申请号：US09238992
申请日：1999-01-28
申请人： Michael Riedel , Gerhard Erker , Lothar Duda
发明人： Michael Riedel , Gerhard Erker , Lothar Duda
IPC分类号： C08F444
CPC分类号： C07F17/00 , C08F4/61916 , C08F4/6192 , C08F10/00 , Y10S526/943
摘要： The present invention relates to a process to prepare an olefin using a transition metal compound of the formula I as a catalyst component where M1 is a metal of group IIIb, IVb or Vb of the Periodic Table of the Elements, R1, R2, R3 and R4 are identical or different and are each a hydrogen atom or a substituent, R5 are identical or different and are a substituent, Y are identical or different and are each a hydrogen atom, a C1-C40-hydrocarbon-containing group, an OH group, a halogen atom or an NR52 group, where R5 are identical or different and are each a halogen atom, a C1-C10-alkyl group or a C6-C10-aryl group, k is an integer which corresponds to the valence of the transition metal atom M1 minus two and if Y is a butadiene unit, k is 1, A is a bridge. R8 is a hydrogen atom, a halogen atom, a C1-C40-group, an —SiR53, —NR52, —Si(OR5)3, —Si(SR53 or —PR52 radical, where R5 are identical or different and are each a halogen atom, a C1-C10-alkyl group or a C6-C10-alkyl group or a C6-C10-aryl group, and X is an element of group Va or VIa of the Periodic Table of the Elements, where if X is an element of group Va, X bears a radical R9 which is a hydrogen atom, a halogen atom, a Cx-C40-group, an —SiR53, —NR52, —Si(OR5)3, —Si(SR5)3 or —PR52 radical, where R5 are identical or different and are each a halogen atom, a C1-C10-alkyl group or a C6-C10-aryl group.
摘要翻译：本发明涉及使用式I的过渡金属化合物作为催化剂组分制备烯烃的方法，其中M1是元素周期表IIIb，IVb或Vb族的金属，R1，R2，R3和R4 相同或不同，分别为氢原子或取代基，R5相同或不同，为取代基，Y相同或不同，为氢原子，含C1-C40烃基，OH基，卤素原子或NR52基团，其中R5相同或不同，并且各自为卤素原子，C1-C10烷基或C6-C10-芳基，k为对应于过渡金属化合价的整数原子M1减2，如果Y是丁二烯单元，则k是1，A是桥.R 8是氢原子，卤原子，C 1 -C 40基，-SiR 53，-NR 52，-Si（OR 5） 3，-Si（SR53或-PR52基团，其中R5相同或不同，各自为卤素原子，C1-C10烷基或C6-C10-烷基或C6-C10-芳基）并且X是元素周期表的Va或VIa族的元素，其中如果X是Va族的元素，X具有作为氢原子的基团R 9，卤素原子，C x -C 40 - 基团，-SiR 53，-NR 52，-Si（OR 5）3，-Si（SR 5）3或-PR 52基团，其中R 5相同或不同，各自为卤素原子，C1-C10-烷基或C6- C10-芳基。

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