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1. 发明申请

WO2008014964A3 MEMBRANE ELECTRODE ASSEMBLY AND FUEL CELLS WITH INCREASED POWER 审中-公开
标题翻译：带来了高性能的膜电极单元和燃料电池
公开(公告)号：WO2008014964A3
公开(公告)日：2008-05-08
申请号：PCT/EP2007006741
申请日：2007-07-31
申请人： BASF FUEL CELL GMBH , UENSAL OEMER , SCHMIDT THOMAS , WEBER MATHIAS
发明人： UENSAL OEMER , SCHMIDT THOMAS , WEBER MATHIAS
IPC分类号： H01M4/86 , B01D69/02 , H01M8/02 , H01M8/10
CPC分类号： H01M4/86 , B01D2325/24 , B01D2325/40 , H01M8/0289 , H01M8/1004 , H01M8/1007 , H01M8/1048 , H01M8/1051 , H01M8/1067 , H01M8/1072 , Y02P70/56 , Y10T29/49108 , Y10T29/49115
摘要： Membrane electrode assembly for fuel cells, comprising at least two electrochemically active electrodes, which are separated by at least one polymer electrolyte membrane, wherein the polymer electrolyte membrane has reinforcing elements which at least partially penetrate said polymer electrolyte membrane. The invention also relates to methods for producing a polymer electrolyte membrane of this type.
摘要翻译：用于燃料电池的膜电极单元，包括由至少一种聚合物电解质膜隔开的至少两个电化学活性电极，所述高分子电解质膜具有穿过聚合物电解质膜至少部分地为增强元件和方法生产这样的聚合物电解质膜的。

2. 发明申请

WO2005023914A3 PROTON-CONDUCTING POLYMER MEMBRANE COATED WITH A CATALYST LAYER, SAID POLYMER MEMBRANE COMPRISING PHOSPHONIC ACID POLYMERS, MEMBRANE/ELECTRODE UNIT AND THE USE THEREOF IN FUEL CELLS 审中-公开
标题翻译：与催化剂层包覆高分子膜含质子传导包含膦POLYMERS，膜电极单元及其使用在燃料电池中
公开(公告)号：WO2005023914A3
公开(公告)日：2005-06-02
申请号：PCT/EP2004009899
申请日：2004-09-04
申请人： PEMEAS GMBH , BELACK JOERG , KUNDLER ISABEL , SCHMIDT THOMAS , UENSAL OEMER , KIEFER JOACHIM , PADBERG CHRISTOPH , WEBER MATHIAS
发明人： BELACK JOERG , KUNDLER ISABEL , SCHMIDT THOMAS , UENSAL OEMER , KIEFER JOACHIM , PADBERG CHRISTOPH , WEBER MATHIAS
IPC分类号： B01D71/44 , C08F8/00 , C08J5/22 , C08J7/04 , C08J7/06 , H01M4/88 , H01M4/92 , H01M8/00 , H01M8/02 , H01M8/10
CPC分类号： C08J7/047 , C08J5/2231 , C08J5/2287 , C08J7/045 , C08J7/065 , C08J2379/06 , H01M4/881 , H01M4/8825 , H01M4/8896 , H01M4/92 , H01M4/926 , H01M8/1004 , H01M8/1023 , H01M8/1039 , H01M8/1067 , H01M8/1072 , H01M2300/0082 , Y02P70/56
摘要： The invention relates to a polymer membrane that is coated with a catalyst layer, said polymer membrane comprising phosphonic acid polymers. Said polymers are obtainable by polymerization of phosphonic acid monomers. The invention is characterized in that the catalyst layer comprises phosphonic acid ionomers, said ionomers being obtainable by polymerization of phosphonic acid monomers.
摘要翻译：本发明涉及涂覆有催化剂层的质子传导性聚合物膜的表面，所述聚合物膜膦包含大量的聚合物，其是由包含膦酸的单体的聚合获得，其特征在于，所述催化剂层膦包含大量的离聚物，其通过单体的聚合包含膦酸可获得，

3. 发明申请

WO2005081351A3 HIGH-PERFORMANCE MEMBRANE ELECTRODE UNIT AND THE USE THEREOF IN FUEL CELLS 审中-公开
标题翻译：高性能膜电极单元及其使用燃料电池
公开(公告)号：WO2005081351A3
公开(公告)日：2006-07-20
申请号：PCT/EP2005001761
申请日：2005-02-20
申请人： PEMEAS GMBH , SCHMIDT THOMAS , UENSAL OEMER , WEBER MATHIAS , KUNDLER ISABEL , CALUNDANN GORDON , BAURMEISTER JOCHEN
发明人： SCHMIDT THOMAS , UENSAL OEMER , WEBER MATHIAS , KUNDLER ISABEL , CALUNDANN GORDON , BAURMEISTER JOCHEN
IPC分类号： H01M8/10 , H01M4/86 , H01M4/88 , H01M4/90 , H01M4/92 , H01M8/02
CPC分类号： H01M4/921 , H01M4/8605 , H01M4/881 , H01M4/8814 , H01M4/8832 , H01M4/8835 , H01M4/886 , H01M4/8882 , H01M4/8896 , H01M4/90 , H01M4/926 , H01M8/1004 , H01M8/1027 , H01M8/103 , H01M8/1032 , H01M8/1034 , H01M8/1044 , H01M8/1048 , H01M8/1072 , H01M8/1081 , Y02P70/56
摘要： The invention relates to a membrane electrode unit comprising a polymer membrane doped with a mineral acid, and two electrodes, said unit being characterised in that the polymer membrane comprises at least one polymer containing at least one nitrogen atom, and at least one electrode comprises a catalyst formed from at least one precious metal and at least one base metal according to the electrochemical series.
摘要翻译：本发明涉及包括与无机酸聚合物膜与两个电极的掺杂的膜电极组件，其特征在于，具有至少一个氮原子的聚合物膜和至少一个电极包括至少一种聚合物具有的催化剂由至少一种贵金属和至少一种的根据电化学系列中形成较少的贵金属。

4. 发明申请

WO2004034498A3 PROTON-CONDUCTING POLYMER MEMBRANE THAT CONTAINS POLYAZOLES AND IS COATED WITH A CATALYST LAYER, AND APPLICATION THEREOF IN FUEL CELLS 审中-公开
标题翻译：与催化剂涂上一层高分子膜含质子传导性的聚唑及其使用燃料电池
公开(公告)号：WO2004034498A3
公开(公告)日：2005-05-12
申请号：PCT/EP0310903
申请日：2003-10-02
申请人： PEMEAS GMBH , BAURMEISTER JOCHEN , KUNDLER ISABEL , PADBERG CHRISTOPH , UENSAL OEMER , KEIFER JOACHIM , CALUNDANN GORDON , BENICEWICZ BRIAN , WEBER MATHIAS
发明人： BAURMEISTER JOCHEN , KUNDLER ISABEL , PADBERG CHRISTOPH , UENSAL OEMER , KEIFER JOACHIM , CALUNDANN GORDON , BENICEWICZ BRIAN , WEBER MATHIAS
IPC分类号： B01D71/62 , C08G73/18 , C08J5/22 , H01M4/86 , H01M4/92 , H01M8/10 , B01D67/00
CPC分类号： C08J5/2256 , B01D71/62 , C08G73/18 , C08J2379/06 , H01M4/8605 , H01M4/92 , H01M8/1004 , H01M8/1027 , H01M8/103 , H01M8/1067 , H01M8/1072 , H01M8/109 , Y02P70/56
摘要： The invention relates to a proton-conducting polymer membrane that contains polyazoles, is coated with a catalyst layer, and is obtained by a method comprising the steps of A) producing a mixture containing polyphosphoric acid, at least one polyazole (polymer A), and/or at least one or several compounds that are suitable for forming polyazoles under the influence of heat according to step B), B) heating the mixture obtained in step A) to temperatures of up to 400 DEG C under inert gas, C) applying a layer to a support by using the mixture according to step A) and/or B), D) treating the membrane formed in step C) until said membrane is self-supporting, and E) applying at least one coating containing a catalyst to the membrane formed in step C) and/or step D).
摘要翻译：本发明涉及涂布在催化剂层的质子传导含有由包括A的制备的混合物中的步骤），其包含多磷酸，至少一个聚唑（聚合物A）在根据加热步骤的应用和/或至少一种或多种化合物的方法得到的聚唑的聚合物膜 B）是适合用于形成聚唑，B）加热该混合物得到根据在惰性气体下在步骤a）至温度高达400℃，C）根据步骤a），并使用该混合物施加层/或B）上的载体，D）治疗将至少一个涂层包括在所述形成步骤C）和/或在步骤d）的膜的催化剂）中形成的步骤C中的膜，直到它是自支撑的，E）。

5. 发明申请

WO2006015806A3 MEMBRANE-ELECTRODE UNIT AND FUEL ELEMENTS WITH INCREASED SERVICE LIFE 审中-公开
标题翻译：延长了寿命的膜电极单元和燃料电池
公开(公告)号：WO2006015806A3
公开(公告)日：2006-08-17
申请号：PCT/EP2005008487
申请日：2005-08-05
申请人： PEMEAS GMBH , PAWLIK JUERGEN , UENSAL OEMER , SCHMIDT THOMAS , PADBERG CHRISTOPH , HOPPES GLEN
发明人： PAWLIK JUERGEN , UENSAL OEMER , SCHMIDT THOMAS , PADBERG CHRISTOPH , HOPPES GLEN
IPC分类号： H01M8/02 , H01M8/10
CPC分类号： H01M8/0271 , H01M4/8605 , H01M8/1007 , H01M8/1027 , H01M8/103 , H01M8/1048
摘要： The invention relates to a membrane-electrode unit comprising a) two electrochemically active electrodes (1, 3) divided by a polymer electrolytic membrane (5), wherein the surfaces of said polymer electrolytic membrane (5) are in contact with the electrodes (1, 3) in such a way that the first electrode (1) partially or entirely covers the front side of the polymer electrolytic membrane (5) and the second electrode (3) partially or entirely covers the rear side thereof, b) a sealing material (7, 9) is applied to the front and rear sides of the polymer electrolytic membrane (5), wherein the polymer electrolytic membrane (5) is provided with one or several recesses (11) and the sealing material (7) applied to the front side of the polymer electrolytic membrane (5) is in contact with the sealing material (9) applied to the rear side thereof. A method for producing said membrane-electrode unit and fuel cells provided therewith are also disclosed.
摘要翻译：本发明涉及一种包含膜电极组件的）两个电化学活性电极（1,3），它们由聚合物电解质膜（5），分离，其中，所述高分子电解质膜（5）以这样的方式表面与电极（1,3）相接触，使得第一电极（1）的聚合物电解质膜（5）和第二电极的前侧（3）高分子电解质膜的背面侧（5）的每个部分或完全覆盖，b）中的密封材料（7,9）上的前部和高分子电解质膜（5）的背面，其中，所述高分子电解质膜（5）和一个或多个凹槽（11），密封材料（7）是在所述高分子电解质膜（5）的与所述高分子电解质膜（5）的背面侧的密封材料（9）的前侧接触。此外，本发明涉及用于制备膜 - 电极组件和具有这种膜电极组件的燃料电池

6. 发明专利

JP2011089123A Proton-conducting polymer membrane containing polyazole blend, and application thereof in fuel cell 审中-公开
标题翻译：含有聚酰胺混合物的导电聚合物膜及其在燃料电池中的应用
公开(公告)号：JP2011089123A
公开(公告)日：2011-05-06
申请号：JP2010258846
申请日：2010-11-19
申请人： Basf Fuel Cell Gmbh , ベーアーエスエフフューエルセルゲーエムベーハー
发明人： UENSAL OEMER , KIEFER JOACHIM , CALUNDANN GORDON , SANSONE MICHAEL , BENICEWICZ BRIAN , CHOE EUI WON
IPC分类号： C08J5/22 , B01D71/62 , C08G73/18 , C08L79/04 , C08L101/00 , H01B1/06 , H01B13/00 , H01M4/86 , H01M8/02 , H01M8/10
CPC分类号： C08J5/2275 , B01D71/62 , C08G73/18 , C08J2379/06 , H01M8/1023 , H01M8/1025 , H01M8/1027 , H01M8/103 , H01M8/1032 , H01M8/1034 , H01M8/1037 , H01M8/1039 , H01M8/1041 , H01M8/1048 , H01M8/1072 , H01M8/1081 , Y02P70/56
摘要： PROBLEM TO BE SOLVED: To provide a new polymer electrolyte membrane which can be used for a variety of purposes owing to its excellent chemical and thermal properties. SOLUTION: The proton-conducting polymer membrane containing polyazole is obtained by a method comprising the following steps: (A) preparation of a mixture comprising polyphosphoric acid, at least one polyazole (polymer A) and/or one or more compounds which are suitable for forming polyazoles under the action of heat according to step (B); (B) heating of the mixture obtainable according to step (A) under inert gas to temperatures of up to 400°C; (C) application of a layer using the mixture from step (A) and/or (B) to a support; and (D) treatment of the membrane formed in step (C) until it is self-supporting (wherein at least one further polymer (polymer B) which is not a polyazole is added to the composition obtainable according to step (A) and/or step (B) and the weight ratio of polyazole to polymer B is in the range from 0.1 to 50). COPYRIGHT: (C)2011,JPO&INPIT
摘要翻译：要解决的问题：提供一种由于其优异的化学和热性能而可用于各种目的的新的聚合物电解质膜。解决方案：含有聚唑的质子传导聚合物膜通过包括以下步骤的方法获得：（A）制备包含多磷酸，至少一种聚唑（聚合物A）和/或一种或多种化合物的混合物，适用于根据步骤（B）在热作用下形成多唑; （B）在惰性气体下将根据步骤（A）获得的混合物加热至高达400℃的温度; （C）使用来自步骤（A）和/或（B）的混合物将层施加到载体上; 和（D）处理在步骤（C）中形成的膜直到其自支撑（其中至少一种不是聚唑的另外的聚合物（聚合物B）加入到根据步骤（A）获得的组合物和/ 或步骤（B），并且聚唑与聚合物B的重量比在0.1至50的范围内）。版权所有（C）2011，JPO＆INPIT

7. 发明专利

JP2011252159A Proton-conducting membrane and use thereof 有权
标题翻译：导电膜及其使用
公开(公告)号：JP2011252159A
公开(公告)日：2011-12-15
申请号：JP2011166861
申请日：2011-07-29
申请人： Basf Fuel Cell Gmbh , ベーアーエスエフフューエルセルゲーエムベーハー
发明人： UENSAL OEMER , BREHL KILIAN , THIEMER EDMUND
IPC分类号： C08J5/22 , B01D67/00 , B01D71/62 , B01D71/64 , C08G73/18 , H01B1/06 , H01B13/00 , H01M8/02 , H01M8/10
CPC分类号： B01D67/0018 , B01D67/0011 , B01D67/0093 , B01D71/62 , B01D2323/08 , B01D2323/30 , B01D2325/26 , C08G73/18 , C08J5/2256 , C08J2379/06 , H01M8/1004 , H01M8/1027 , H01M8/103 , H01M8/1044 , H01M8/1048 , H01M8/1081 , H01M8/1086 , H01M2300/0082 , Y02E60/521 , Y02P70/56
摘要： PROBLEM TO BE SOLVED: To provide a novel proton-conducting polymer membrane which exhibits advantages of the polymer membrane based on polyazole, has increased specific conductivity particularly at the operating temperature exceeding 100°C and exhibits a remarkably lower overvoltage particularly at a cathode.SOLUTION: The proton-conducting polymer membrane is obtained by a method comprising: a step (A) of dissolving a polyazole polymer in organic phosphoric anhydride to form a solution and/or a dispersion; a step (B) of heating the solution, which is obtained at the step (A), to 400°C in an inert gas; a step (C) of forming a membrane on a support by using the solution obtained at the step (B); and a step (D) of treating the membrane, which is formed at the step (C), as far as the membrane has self-supporting properties. The proton-conducting polymer membrane is particularly suitable as a polymer electrolyte membrane (PEM) for producing a membrane electrode unit for PEM fuel cells.
摘要翻译：要解决的问题为了提供一种基于聚唑的聚合物膜的优点的新颖的导电聚合物膜，特别是在超过100℃的操作温度下具有特别高的比电导率，特别是在阴极。导电聚合物膜是通过以下方法获得的，所述方法包括：将聚唑聚合物溶解在有机磷酸酐中以形成溶液和/或分散体的步骤（A）; 将在步骤（A）中获得的溶液在惰性气体中加热至400℃的步骤（B）; 通过使用在步骤（B）获得的溶液在支持体上形成膜的步骤（C）; 以及在步骤（C）中形成的膜的步骤（D），只要膜具有自支撑性即可。质子传导性聚合物膜特别适用于制造用于PEM燃料电池的膜电极单元的聚合物电解质膜（PEM）。版权所有（C）2012，JPO＆INPIT

8. 发明专利

JP2011138782A Forming method of proton conductive polymer membrane 审中-公开
标题翻译：原子导电聚合物膜的形成方法
公开(公告)号：JP2011138782A
公开(公告)日：2011-07-14
申请号：JP2011009959
申请日：2011-01-20
申请人： Basf Fuel Cell Gmbh , ビーエーエスエフフューエルセルゲゼルシャフトミットベシュレンクテルハフツング
发明人： KIEFER JOACHIM , UENSAL OEMER , CALUNDANN GORDON , CRIVELLO JAMES
IPC分类号： C08F2/44 , H01B13/00 , C08F228/02 , C08F230/02 , C08F291/00 , C08J5/22 , C08J7/18 , H01B1/06 , H01M8/02 , H01M8/04 , H01M8/10
CPC分类号： H01M8/1023 , C08J5/2231 , C08J2325/08 , H01M8/04197 , H01M8/1011 , H01M8/1025 , H01M8/1039 , H01M8/1044 , H01M8/106 , H01M8/1072 , H01M2300/0082 , Y02E60/523 , Y02P70/56
摘要： PROBLEM TO BE SOLVED: To provide a proton conductive electrolyte membrane with an intrinsic conductivity at 160°C of 0.001 S/cm or higher. SOLUTION: This forming method of the proton conductive electrolyte membrane of an intrinsic conductivity at 160°C of 0.001S/cm comprises a step (A) of dipping a polymer film in liquid containing a vinyl-content sulfonic acid and a vinyl-content phosphonic acid and impregnating the liquid in the film to be swollen, and a step (B) of polymerizing the vinyl-content sulfonic acid and the vinyl-content phosphonic acid existing in the film. However, the film for swelling is formed of polyazole, the liquid for swelling contains the vinyl-content phosphonic acid by 20 mass% or larger, a mass ratio of the vinyl-content phosphonic acid to the vinyl-content sulfonic acid in the liquid for swelling is 1:1 or larger, and the film after swelling contains the vinyl-content sulfonic acid by 10 mass%. COPYRIGHT: (C)2011,JPO&INPIT
摘要翻译：要解决的问题：提供在160℃下的固有电导率为0.001S / cm或更高的质子传导电解质膜。解决方案：160℃下固有电导率为0.001S / cm的质子传导电解质膜的形成方法包括将聚合物膜浸渍在含有乙烯基含量磺酸和乙烯基的液体的液体中的步骤（A） - 含有膦酸并浸渍在待溶胀的膜中的液体;以及聚合存在于膜中的乙烯基含量磺酸和乙烯基含量膦酸的步骤（B）。然而，用于溶胀的膜由聚唑形成，溶胀液含有乙烯基含量膦酸20质量％以上，乙烯基含量膦酸与乙烯基含量磺酸在液体中的质量比溶胀为1：1以上，溶胀后的膜含有10质量％的乙烯基含量的磺酸。版权所有（C）2011，JPO＆INPIT

9. 发明专利

JP2011006690A Proton conductive polymer membrane 有权
标题翻译：原子导电聚合物膜
公开(公告)号：JP2011006690A
公开(公告)日：2011-01-13
申请号：JP2010177244
申请日：2010-08-06
申请人： Basf Fuel Cell Gmbh , ベーアーエスエフフューエルセルゲーエムベーハー
发明人： CALUNDANN GORDON , SANSONE MICHAEL J , UENSAL OEMER , KIEFER JOACHIM
IPC分类号： C08J5/22 , C08G73/08 , H01M8/02 , H01M8/10
CPC分类号： Y02E60/521
摘要： PROBLEM TO BE SOLVED: To provide a new polyazole-based proton conductive polymer membrane.SOLUTION: The polyazole-based proton conductive polymer membrane has superior chemical and thermal properties and, therefore, is useful, in particular, as a polymer electrolyte membrane (PEM) for producing a membrane-electrode unit for a PEM fuel cell.
摘要翻译：要解决的问题：提供一种新型的基于聚唑的质子传导性聚合物膜。解决方案：聚唑类质子传导性聚合物膜具有优异的化学和热性能，因此特别适用于聚合物电解质膜（PEM ），用于制造用于PEM燃料电池的膜电极单元。

10. 发明专利

JP2009293045A Proton-conducting polymer membrane comprising polymer with sulfonic acid group and use thereof in fuel cells 审中-公开
标题翻译：含有磺酸基的聚合物的导电聚合物膜和在燃料电池中的使用
公开(公告)号：JP2009293045A
公开(公告)日：2009-12-17
申请号：JP2009217782
申请日：2009-09-18
申请人： Basf Fuel Cell Gmbh , バスフ・ヒュエル・セル・ゲーエムベーハー
发明人： KIEFER JOACHIM , UENSAL OEMER , CALUNDANN GORDON
IPC分类号： C08G73/06 , C08J5/22 , B01D67/00 , B01D69/14 , B01D71/62 , B01D71/72 , C08F2/44 , C08F28/02 , C08F283/04 , C08G61/12 , C08G73/08 , C08G73/18 , C08G79/04 , H01B1/06 , H01B13/00 , H01M8/02 , H01M8/10
CPC分类号： B01D67/0006 , B01D69/141 , B01D71/62 , B01D71/72 , B01D2323/34 , B01D2325/24 , B01D2325/26 , C08G61/124 , C08G73/06 , C08G73/0616 , C08G73/0633 , C08G73/18 , C08G79/04 , C08J5/2256 , C08J2379/06 , H01M8/1004 , H01M8/1023 , H01M8/1027 , H01M8/103 , H01M8/1044 , H01M8/1072 , H01M2300/0082 , Y02P70/56
摘要： PROBLEM TO BE SOLVED: To provide a proton-conducting polymer membrane suitable for polymer electrolyte membranes and the like. SOLUTION: The proton-conducting polymer membrane comprises polymers containing sulfonic acid groups and has the conductivity of at least 0.001 S/cm. The membrane is obtainable by a method comprising the steps of: (A) mixing a vinyl-containing sulfonic acid with one or more aromatic polycarboxylic acids, their esters, their acid halides, and their acid anhydrides, and one or more of aromatic tetra-amino compounds, or mixing the vinyl-containing sulfonic acid with one or more aromatic and/or heteroaromatic diaminocarboxylic acids, their esters, their acid halides, or their acid anhydrides; (B) heating the mixture obtainable according to step (A) under inert gas to temperatures of up to 350°C, to form polyazole polymers; (C) applying a layer to a support, using the mixture according to step (A) and/or (B); and (D) polymerizing the vinyl-containing sulfonic acid present in the sheetlike structure obtainable according to step (C). COPYRIGHT: (C)2010,JPO&INPIT
摘要翻译：要解决的问题：提供适用于聚合物电解质膜等的质子传导聚合物膜。解决方案：质子传导性聚合物膜包含含有磺酸基的聚合物，其导电率至少为0.001S / cm。膜可以通过包括以下步骤的方法获得：（A）将含乙烯基的磺酸与一种或多种芳族多元羧酸，它们的酯，它们的酰卤和它们的酸酐混合，以及一种或多种芳族四或将含乙烯基的磺酸与一种或多种芳族和/或杂芳族二氨基羧酸，它们的酯，其酰基卤或其酸酐混合; （B）在惰性气体下将根据步骤（A）获得的混合物加热至高达350℃的温度，以形成聚唑聚合物; （C）使用根据步骤（A）和/或（B）的混合物将层施加到载体上; 和（D）使根据步骤（C）获得的片状结构中存在的含乙烯基磺酸聚合。版权所有（C）2010，JPO＆INPIT

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