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31. 发明授权

US06733658B2 EU-1 zeolite catalyst and a process for the reduction of the pour point of feeds containing paraffins 失效
标题翻译： EU-1沸石催化剂和降低含有链烷烃的进料的倾点的方法
公开(公告)号：US06733658B2
公开(公告)日：2004-05-11
申请号：US09103528
申请日：1998-06-24
申请人： Eric Benazzi , Nathalie George-Marchal , Christophe Gueret , Patrick Briot , Alain Billon , Pierre Marion
发明人： Eric Benazzi , Nathalie George-Marchal , Christophe Gueret , Patrick Briot , Alain Billon , Pierre Marion
IPC分类号： C10G4716
CPC分类号： B01J29/7023 , B01J29/04 , B01J29/7446 , B01J29/7846 , B01J2229/16 , B01J2229/32 , B01J2229/37 , B01J2229/42 , C01B39/026 , C10G45/64 , C10G2300/1022 , C10G2300/1048 , C10G2300/1059 , C10G2300/1077 , C10G2300/301 , C10G2300/304 , C10G2300/4018
摘要： The invention concerns a process for improving the pour point of a feed comprising paraffins containing more than 10 carbon atoms, in which process the feed to be treated is brought into contact with a catalyst comprising an EU-1 zeolite and at least one hydro-dehydrogenating element, at a temperature which is in the range 170° C. to 500° C., a pressure in the range 1 to 250 bar and an hourly space velocity in the range 0.05 to 100 h−1, in the presence of hydrogen in a proportion of 50 to 2000 l/l of feed. The oils obtained have good pour points and high viscosity indices (VI). The process is also applicable to gas oils and other feeds requiring a reduction of pour point. The invention also concerns an EU-1 zeolite from which a portion of elements T (Al, Ga, Fe or B) have been removed and which has an Si/T atomic ratio of at least 10.
摘要翻译：本发明涉及一种改进含有多于10个碳原子的链烷烃的进料的倾点的方法，其中待处理的进料与包含EU-1沸石的催化剂和至少一种加氢脱氢的催化剂接触元素，温度范围为170℃至500℃，压力范围为1至250巴，小时空间速度为0.05至100小时-1，在存在氢气比例为50〜2000升/升饲料。所得油具有良好的倾点和高粘度指数（VI）。该方法也适用于需要降低倾点的瓦斯油和其他进料。本发明还涉及一部分元素T（Al，Ga，Fe或B）被去除并且其Si / T原子比至少为10的EU-1沸石。

32. 发明授权

US06527945B2 Catalyst comprising a phyllosilicate containing boron and/or silicon, and a hydrocracking process 失效
公开(公告)号：US06527945B2
公开(公告)日：2003-03-04
申请号：US09850078
申请日：2001-05-08
申请人： Eric Benazzi , Slavik Kasztelan , Nathalie George-Marchal
发明人： Eric Benazzi , Slavik Kasztelan , Nathalie George-Marchal
IPC分类号： C10G4702
CPC分类号： B01J21/16 , B01J23/85 , C10G47/20
摘要： The invention concerns a catalyst comprising at least one matrix, at least one dioctahedral 2:1 phyllosilicate which is optionally synthesised in a fluorine-containing medium and optionally bridged, at least one metal selected from elements from group VIB and/or group VIII of the periodic table, boron and/or silicon, optionally phosphorous, optionally at least one group VIIA element, and optionally at least one group VIIB element. The invention also concerns the use of the catalyst for hydrocracking hydrocarbon-containing feeds.

33. 发明授权

US06313363B1 Process for isomerizing aromatic compounds containing eight carbon atoms 有权
标题翻译：异构化含有8个碳原子的芳族化合物的方法
公开(公告)号：US06313363B1
公开(公告)日：2001-11-06
申请号：US09289655
申请日：1999-04-12
申请人： Jean-François Joly , Julia Magne-Drisch , Fabio Alario , Elisabeth Merlen , Eric Benazzi , Sylvie Lacombe
发明人： Jean-François Joly , Julia Magne-Drisch , Fabio Alario , Elisabeth Merlen , Eric Benazzi , Sylvie Lacombe
IPC分类号： C07C522
CPC分类号： B01J29/7023 , B01J29/068 , B01J29/18 , B01J29/22 , B01J29/74 , B01J29/7446 , B01J33/00 , B01J37/20 , B01J2229/26 , B01J2229/42 , C07C5/2702 , Y02P20/52 , Y02P20/582 , Y10S585/906 , C07C15/08
摘要： The present invention relates to a process for isomerizing aromatic compounds containing 8 carbon atoms, the catalysts containing at least one group VIII metal, comprising at least one sulfurization step and at least one passivation step using ammonia.
摘要翻译：本发明涉及使含有8个碳原子的芳族化合物异构化的方法，含有至少一种第Ⅷ族金属的催化剂，其包括至少一个硫化步骤和至少一个使用氨的钝化步骤。

34. 发明授权

US06245704B1 Catalyst with a base of modified MFI zeolite, and its use in the isomerization of a C8 aromatic cut 失效
标题翻译：具有改性MFI沸石基质的催化剂及其用于C8芳族化合物切割的异构化
公开(公告)号：US06245704B1
公开(公告)日：2001-06-12
申请号：US08187026
申请日：1994-01-27
申请人： Eric Benazzi , Jean-Francois Joly , Joao Miguel Da Silva , Maria Filipa Gomes Ribeiro
发明人： Eric Benazzi , Jean-Francois Joly , Joao Miguel Da Silva , Maria Filipa Gomes Ribeiro
IPC分类号： B01J2100
CPC分类号： B01J29/40 , B01J2229/16 , B01J2229/26 , B01J2229/42 , C07C5/2724 , C07C2523/42 , C07C2523/44 , C07C2529/74 , C10G2400/30 , C07C15/067
摘要： The invention is concerned with a catalyst comprising a matrix, a MFI type zeolite and at least one group VIII element, in which the crystals of the MFI type zeolite are desaluminated on their outer surface by at least one treatment with at least one solution of a fluorosilicate of a cation selected from the group formed by NH4+, alkylammoniums, K+, Na+, Li+, Ba2+, Mg2+, Cd2+, Cu+, Cu2+, Ca2+, Cs+, Fe2+, Co2+, Pb2+, Mn2+, Rb+, Ag+, Sr2+, Zn2+, Tl+ and H+, the global desalumination rate of said MFI zeolite thus treated being less than 5 atomic per cent.
摘要翻译：本发明涉及包含基质，MFI型沸石和至少一种VIII族元素的催化剂，其中MFI型沸石的晶体在其外表面上脱铝至少一种用至少一种溶液选自由NH4 +，烷基铵，K +，Na +，Li +，Ba2 +，Mg2 +，Cd2 +，Cu +，Cu2 +，Ca2 +，Cs +，Fe2 +，Co2 +，Pb2 +，Mn2 +，Rb +，Ag +，Sr2 +，Zn2 +形成的阳离子的阳离子的氟硅酸盐， Tl +和H +，如此处理的所述MFI沸石的全局脱盐速率小于5原子％。

35. 发明授权

US06235670B1 Catalyst comprising a phyllosilicate containing boron and/or silicon, and a hydrocracking process 失效
标题翻译：包含含有硼和/或硅的页硅酸盐以及加氢裂化方法的催化剂
公开(公告)号：US06235670B1
公开(公告)日：2001-05-22
申请号：US09310182
申请日：1999-05-12
申请人： Eric Benazzi , Slavik Kasztelan , Nathalie George-Marchal
发明人： Eric Benazzi , Slavik Kasztelan , Nathalie George-Marchal
IPC分类号： B01J2116
CPC分类号： B01J21/16 , B01J23/85 , C10G47/20
摘要： The invention concerns a catalyst comprising at least one matrix, at least one dioctahedral 2:1 phyllosilicate which is optionally synthesized in a fluorine-containing medium and optionally bridged, at least one metal selected from elements from group VIB and/or group VIII of the periodic table, boron and/or silicon, optionally phosphorous, optionally at least one group VIIA element, and optionally at least one group VIIB element. The invention also concerns the use of the catalyst for hydrocracking hydrocarbon-containing feeds.
摘要翻译：本发明涉及一种催化剂，其包含至少一种基质，至少一种二（双八面体）2：1页硅酸盐，其任选地在含氟介质中合成，并任选地桥接至少一种选自VIB族和/或第VIII族元素的金属周期表，硼和/或硅，任选的磷，任选的至少一个VIIA族元素和任选的至少一个VIIB族元素。本发明还涉及催化剂用于加氢裂化含烃原料的用途。

36. 发明授权

US06231750B1 Hydrocracking catalyst comprising a beta zeolite and a group VB element 有权
标题翻译：包含β沸石和VB族元素的加氢裂化催化剂
公开(公告)号：US06231750B1
公开(公告)日：2001-05-15
申请号：US09344344
申请日：1999-06-25
申请人： Slavik Kasztelan , Eric Benazzi , Nathalie Marchal-George
发明人： Slavik Kasztelan , Eric Benazzi , Nathalie Marchal-George
IPC分类号： C10G4706
CPC分类号： C10G47/16 , B01J27/047 , B01J29/7815 , B01J2229/26 , B01J2229/42
摘要： The invention provides a hydrocracking catalyst comprising at least one mineral matrix, at least one beta zeolite, at least one group VB element or at least one mixed sulphide phase comprising sulphur, optionally at least one group VIB or group VIII element, optionally at least one element selected from the group formed by silicon, boron or phosphorous, and optionally at least one group VIIA element.
摘要翻译：本发明提供一种加氢裂化催化剂，其包含至少一种矿物基质，至少一种β沸石，至少一种VB族元素或至少一种含硫混合物，任选至少一种VIB族或VIII族元素的混合硫化物，任选至少一种元素选自由硅，硼或磷形成的基团，以及任选的至少一种VIIA族元素。

37. 发明授权

US06198015B1 Catalyst based on a molecular sieve and a process for selective hydroisomerisation of long linear and/or slightly branched paraffins using that catalyst 失效
标题翻译：基于分子筛的催化剂和使用该催化剂的长线性和/或稍微支化的链烷烃的选择性加氢异构化的方法
公开(公告)号：US06198015B1
公开(公告)日：2001-03-06
申请号：US09034350
申请日：1998-03-04
申请人： Christian Marcilly , Eric Benazzi , Nathalie George-Marchal
发明人： Christian Marcilly , Eric Benazzi , Nathalie George-Marchal
IPC分类号： C07C513
CPC分类号： C10G45/64 , B01J29/46
摘要： The invention concerns a process for selective hydroisomerization of compounds with an n-alkane chain containing more than 10 carbon atoms, in which the compound to be treated is brought into contact with a catalyst comprising at least one hydro-dehydrogenating element and at least one molecular sieve having a one- or two-dimensional pore network, the accessible pore openings of which are delimited by 10 oxygen atoms, and a distance termed the bridging distance between the pores of less then 0.70 nm, and the zeolite is such that a catalyst which undergoes a standard n-heptadecane isomerization test has, for a conversion of 95%, a selectivity of at least 70% for isomerized products, and the catalyst contains at least 5% by weight of at least one hydro-dehydrogenating element selected from the group formed by non noble GVIII metals, GVIB metals, and niobium, and the catalyst preferably contains phosphorous. The sieve is preferably a NU-10, NU-23, NU-87, EU-13 or Theta-1 zeolite.
摘要翻译：本发明涉及一种使含有多于10个碳原子的正烷烃链选择性加氢异构化的方法，其中待处理化合物与包含至少一个加氢脱氢元素的催化剂和至少一个分子具有一维或二维孔网的筛，其可及孔的开口由10个氧原子界定，并且称为孔之间的桥接距离小于0.70nm的距离，并且沸石使得催化剂进行标准的正十七烷异构化试验对于异构化产物具有至少70％的选择性为95％的转化率，并且催化剂含有至少5重量％的至少一种选自组中的加氢脱氢元件由非贵金属GVIII金属，GVIB金属和铌形成，并且催化剂优选含有磷。筛优选为NU-10，NU-23，NU-87，EU-13或Theta-1沸石。

38. 发明授权

US6136180A Catalyst comprising a NU-88 zeolite, a group VB element and its use for hydroconverting hydrocarbon-containing petroleum feeds 失效
标题翻译：包含NU-88沸石，VB族元素及其用于加氢转化含烃石油原料的催化剂
公开(公告)号：US6136180A
公开(公告)日：2000-10-24
申请号：US253011
申请日：1999-02-19
申请人： Eric Benazzi , Nathalie Marchal-George , Fabrice Diehl , Slavik Kasztelan
发明人： Eric Benazzi , Nathalie Marchal-George , Fabrice Diehl , Slavik Kasztelan
IPC分类号： B01J29/04 , B01J29/06 , B01J29/78 , C01B39/48 , C10G47/16 , C10G47/20 , C01G11/04
CPC分类号： C10G47/20 , B01J29/04 , B01J29/78 , C01B39/48 , B01J2229/26 , B01J2229/42
摘要： The invention provides a hydrocracking catalyst comprising at least one NU-88 zeolite, at least one group VB metal, preferably niobium, at least one amorphous or low crystallinity matrix, optionally at least one metal selected from the group formed by group VIB and VIII metals, optionally at least one element selected from the group formed by phosphorous, boron and silicon, and optionally at least one group VIIA element. The invention also relates to the use of the catalyst for hydrocracking hydrocarbon-containing feeds.
摘要翻译：本发明提供一种加氢裂化催化剂，其包括至少一种NU-88沸石，至少一种VB族金属，优选铌，至少一种无定形或低结晶度基体，任选至少一种选自由VIB族和VIII族金属形成的基团的金属，任选的至少一种选自由磷，硼和硅形成的基团，以及任选的至少一种VIIA族元素。本发明还涉及催化剂用于加氢裂化含烃原料的用途。

39. 发明授权

US6123831A Catalyst comprising a zeolite selected from the group formed by zeolites NU-85, NU-86 and NU-87, an element from group VB and its use in the hydroconversion of hydrocarbon petroleum charges 失效
标题翻译：包含选自由沸石NU-85，NU-86和NU-87形成的沸石的沸石，来自VB组的元素及其在烃石油加氢转化中的用途
公开(公告)号：US6123831A
公开(公告)日：2000-09-26
申请号：US320269
申请日：1999-05-27
申请人： Eric Benazzi , Nathalie Marchal-George , Fabrice Diehl , Slavik Kasztelan
发明人： Eric Benazzi , Nathalie Marchal-George , Fabrice Diehl , Slavik Kasztelan
IPC分类号： B01J29/076 , B01J29/58 , B01J29/78 , C10G47/20 , C10G47/00
CPC分类号： C10G47/20 , B01J29/78
摘要： The invention concerns a hydrocracking catalyst comprising at least one amorphous or poorly crystallised matrix of oxide type, at least one element from group VB, preferably niobium, at least one zeolite selected from the group formed by zeolites NU-85, NU-86 and NU-87, and at least one element selected among boron and silicon, optionally P, optionally at least one element selected from the elements from group VIB and group VIII, and/or optionally at least one element from group VIIA. The invention also concerns the use of that catalyst in the hydrocracking of hydrocarbon charges.
摘要翻译：本发明涉及一种加氢裂化催化剂，其包含至少一种氧化物类型的无定形或不完全结晶的基质，来自VB族的元素，优选铌的至少一种元素，选自由沸石NU-85，NU-86和NU形成的基团中的至少一种沸石 -87，以及选自硼和硅中的至少一种元素，任选地P，任选地至少一种选自VIB族和VIII族元素的元素和/或任选的至少一种来自VIIA族的元素。本发明还涉及该催化剂在烃装料加氢裂化中的用途。

40. 发明授权

US06117307A Catalyst comprising a NU-88 zeolite and its use for hydroconverting hydrocarbon-containing petroleum feeds 失效
标题翻译：包含NU-88沸石的催化剂及其用于加氢转化含烃石油原料的用途
公开(公告)号：US06117307A
公开(公告)日：2000-09-12
申请号：US253012
申请日：1999-02-19
申请人： Eric Benazzi , Nathalie George-Marchal , Slavik Kasztelan
发明人： Eric Benazzi , Nathalie George-Marchal , Slavik Kasztelan
IPC分类号： B01J29/04 , B01J29/06 , B01J29/72 , B01J29/76 , B01J29/78 , C01B39/48 , C10G47/16
CPC分类号： C10G47/16 , B01J29/04 , B01J29/76 , C01B39/48
摘要： An NU-88 zeolite and a hydrocracking catalyst comprising at least one matrix, a NU-88 zeolite, at least one group VIB or VII metal, a phosphorous, boron or silicon promoter, optionally at least one group VIIA element, and optionally at least one group VIIB element, and also the use of the catalyst for hydrocracking hydrocarbon feeds.
摘要翻译： NU-88沸石和加氢裂化催化剂，其包含至少一种基体，NU-88沸石，至少一种VIB或VII族金属，磷，硼或硅促进剂，任选至少一种VIIA族元素，以及任选地至少一组VIIB元素，以及催化剂用于加氢裂化烃进料的用途。

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