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1. 发明授权

US06464857B2 Crystalline phosphorus-containing molecular sieves 失效
公开(公告)号：US06464857B2
公开(公告)日：2002-10-15
申请号：US10087101
申请日：2002-02-28
申请人： Stephen J. Miller
发明人： Stephen J. Miller
IPC分类号： C10G4716
CPC分类号： C01B37/08 , B01D53/944 , B01J29/85 , B01J2229/36 , C01B37/002 , Y10S423/21 , Y10S423/30
摘要： Molecular sieves comprising (1) phosphorus oxide; (2) a first oxide comprising an oxide of silicon, germanium or mixtures thereof; and (3) a second oxide comprising an oxide of aluminum, boron or mixtures thereof, said molecular sieve having a mole ratio of the first oxide to the second oxide of greater than 1, containing at least about 10 weight percent phosphorus oxide in the crystal framework, and having pores greater than 5 Å in diameter are useful as catalysts in hydrocarbon conversion reactions.

2. 发明授权

US06344135B1 Hydrocracking process using a catalyst comprising an IM-5 zeolite and a catalyst comprising an IM-5 zeolite and a promoter element 失效
标题翻译：使用包含IM-5沸石的催化剂和包含IM-5沸石和促进剂元素的催化剂的加氢裂化方法
公开(公告)号：US06344135B1
公开(公告)日：2002-02-05
申请号：US09511490
申请日：2000-02-23
申请人： Eric Benazzi , Slavik Kasztelan
发明人： Eric Benazzi , Slavik Kasztelan
IPC分类号： C10G4716
CPC分类号： C10G47/20 , B01J29/78 , C10G47/16
摘要： The invention concerns a hydrocracking process using a catalyst comprising at least one matrix, an IM-5 zeolite, at least one metal selected from the group formed by metals from group VIB and group VIII of the periodic table, optionally at least one element selected from the group formed by phosphorous, boron and silicon, and optionally at least one group VIIA and/or at least one group VIIB and/or at least one group VB element (in particular niobium). The invention also concerns a catalyst containing at least one matrix, an IM-5 zeolite, at least one metal from groups VIII and/or VIB and at least one promoter element which is boron and/or silicon. The catalyst can also contain at least one group VIIA element and/or at least one group VIIB element and/or at least one group VB element.
摘要翻译：本发明涉及使用包含至少一种基质，IM-5沸石，至少一种选自元素周期表第VIB族和第VIII族金属形成的金属的金属的催化剂的加氢裂化方法，任选地至少一种选自由磷，硼和硅以及任选的至少一种VIIA族和/或至少一种VIIB族组合和/或至少一种VB族元素（特别是铌）形成的基团。本发明还涉及含有至少一种基质，IM-5沸石，至少一种来自VIII族和/或VIB族的金属和至少一种作为硼和/或硅的助催化剂元素的催化剂。催化剂还可含有至少一种VIIA族元素和/或至少一种VIIB族元素和/或至少一种VB族元素。

3. 发明授权

US06827843B2 Hydrocarbon conversion using molecular sieve SSZ-63 有权
公开(公告)号：US06827843B2
公开(公告)日：2004-12-07
申请号：US10329963
申请日：2002-12-26
申请人： Saleh Elomari
发明人： Saleh Elomari
IPC分类号： C10G4716
CPC分类号： B01J23/44 , B01J29/70 , B01J29/74 , B01J29/86 , B01J2229/183 , B01J2229/186 , C07C1/20 , C07C2/12 , C07C2/66 , C07C5/2737 , C10G11/05 , C10G35/095 , C10G45/64 , C10G47/16 , C10G69/12 , C10G69/123 , C10G69/126 , Y02P20/52 , Y10S585/943 , C07C15/08
摘要： The present invention relates to new crystalline molecular sieve SSZ-63 prepared using N-cyclodecyl-N-methyl-pyrrolidinium cation as a structure-directing agent, methods for synthesizing SSZ-63 and processes employing SSZ-63 in a catalyst.

4. 发明授权

US06733658B2 EU-1 zeolite catalyst and a process for the reduction of the pour point of feeds containing paraffins 失效
标题翻译： EU-1沸石催化剂和降低含有链烷烃的进料的倾点的方法
公开(公告)号：US06733658B2
公开(公告)日：2004-05-11
申请号：US09103528
申请日：1998-06-24
申请人： Eric Benazzi , Nathalie George-Marchal , Christophe Gueret , Patrick Briot , Alain Billon , Pierre Marion
发明人： Eric Benazzi , Nathalie George-Marchal , Christophe Gueret , Patrick Briot , Alain Billon , Pierre Marion
IPC分类号： C10G4716
CPC分类号： B01J29/7023 , B01J29/04 , B01J29/7446 , B01J29/7846 , B01J2229/16 , B01J2229/32 , B01J2229/37 , B01J2229/42 , C01B39/026 , C10G45/64 , C10G2300/1022 , C10G2300/1048 , C10G2300/1059 , C10G2300/1077 , C10G2300/301 , C10G2300/304 , C10G2300/4018
摘要： The invention concerns a process for improving the pour point of a feed comprising paraffins containing more than 10 carbon atoms, in which process the feed to be treated is brought into contact with a catalyst comprising an EU-1 zeolite and at least one hydro-dehydrogenating element, at a temperature which is in the range 170° C. to 500° C., a pressure in the range 1 to 250 bar and an hourly space velocity in the range 0.05 to 100 h−1, in the presence of hydrogen in a proportion of 50 to 2000 l/l of feed. The oils obtained have good pour points and high viscosity indices (VI). The process is also applicable to gas oils and other feeds requiring a reduction of pour point. The invention also concerns an EU-1 zeolite from which a portion of elements T (Al, Ga, Fe or B) have been removed and which has an Si/T atomic ratio of at least 10.
摘要翻译：本发明涉及一种改进含有多于10个碳原子的链烷烃的进料的倾点的方法，其中待处理的进料与包含EU-1沸石的催化剂和至少一种加氢脱氢的催化剂接触元素，温度范围为170℃至500℃，压力范围为1至250巴，小时空间速度为0.05至100小时-1，在存在氢气比例为50〜2000升/升饲料。所得油具有良好的倾点和高粘度指数（VI）。该方法也适用于需要降低倾点的瓦斯油和其他进料。本发明还涉及一部分元素T（Al，Ga，Fe或B）被去除并且其Si / T原子比至少为10的EU-1沸石。

5. 发明授权

US06719895B2 Catalyst comprising a zeolite Y globally non-dealuminated and containing boron and/or silicon 有权
标题翻译：催化剂包含全部非脱铝并含有硼和/或硅的沸石Y
公开(公告)号：US06719895B2
公开(公告)日：2004-04-13
申请号：US09965804
申请日：2001-10-01
申请人： Samuel Mignard , Nathalie George-Marchal , Slavik Kasztelan
发明人： Samuel Mignard , Nathalie George-Marchal , Slavik Kasztelan
IPC分类号： C10G4716
CPC分类号： C10G47/20 , B01J29/166
摘要： The present invention relates to a hydrocracking process including contacting a hydrocarbon feed with a catalyst which is carried out at a pressure of at least 2 MPa, a temperature of at least 230° C., using a quantity of hydrogen of at least 100 Nl hydrogen/l of feed and with an hourly space velocity of 0.1-10 h−1. The catalyst includes 0.1-99.7% by weight of at least one alumina matrix; 0.1-80% by weight of at least one globally non dealuminated Y zeolite with a lattice parameter of more than 2.438 nm, a global SiO2/Al2O3 mole ratio of less than 8, and a framework SiO2/Al2O3 mole ratio of less than 21 and more than the global SiO2/Al2O3 mole ratio; 0.1-30% by weight of at least one group VIII metal and/or 1-40% by weight of at least one group VIB metal (% oxide); 0.1-20% by weight of at least one promoter element selected from the group formed by boron and silicon (% oxide); 0-20% by weight of at least one group VIIA element; 0-20% by weight of phosphorous (% oxide); and 0.1-20% by weight of at least one group VIIB element.
摘要翻译：本发明涉及一种加氢裂化方法，包括使烃进料与催化剂接触，所述催化剂在至少2MPa的压力，至少230℃的温度下使用至少100N氢气的氢气进行 / l的饲料，每小时空速为0.1-10小时-1。催化剂包含0.1-99.7重量％的至少一个氧化铝基质; 0.1-80重量％的至少一种全部非脱铝Y沸石，其晶格参数大于2.438nm，全体SiO 2 / Al 2 O 3摩尔比小于8，并且SiO 2 / Al 2 O 3的骨架比小于21且大于全局SiO 2 / Al 2 O 3摩尔比; 0.1-30重量％的至少一种VIII族金属和/或1-40重量％至少一种VIB族金属（％氧化物）; 0.1-20％重量的选自硼和硅（氧化物％）的至少一种助催化剂元素; 0-20％重量的至少一种VIIA族元素 ; 0-20重量％的磷（％氧化物）; 和0.1-20重量％的至少一种VIIB族元素。

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