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1. 发明授权

US06198015B1 Catalyst based on a molecular sieve and a process for selective hydroisomerisation of long linear and/or slightly branched paraffins using that catalyst 失效
标题翻译：基于分子筛的催化剂和使用该催化剂的长线性和/或稍微支化的链烷烃的选择性加氢异构化的方法
公开(公告)号：US06198015B1
公开(公告)日：2001-03-06
申请号：US09034350
申请日：1998-03-04
申请人： Christian Marcilly , Eric Benazzi , Nathalie George-Marchal
发明人： Christian Marcilly , Eric Benazzi , Nathalie George-Marchal
IPC分类号： C07C513
CPC分类号： C10G45/64 , B01J29/46
摘要： The invention concerns a process for selective hydroisomerization of compounds with an n-alkane chain containing more than 10 carbon atoms, in which the compound to be treated is brought into contact with a catalyst comprising at least one hydro-dehydrogenating element and at least one molecular sieve having a one- or two-dimensional pore network, the accessible pore openings of which are delimited by 10 oxygen atoms, and a distance termed the bridging distance between the pores of less then 0.70 nm, and the zeolite is such that a catalyst which undergoes a standard n-heptadecane isomerization test has, for a conversion of 95%, a selectivity of at least 70% for isomerized products, and the catalyst contains at least 5% by weight of at least one hydro-dehydrogenating element selected from the group formed by non noble GVIII metals, GVIB metals, and niobium, and the catalyst preferably contains phosphorous. The sieve is preferably a NU-10, NU-23, NU-87, EU-13 or Theta-1 zeolite.
摘要翻译：本发明涉及一种使含有多于10个碳原子的正烷烃链选择性加氢异构化的方法，其中待处理化合物与包含至少一个加氢脱氢元素的催化剂和至少一个分子具有一维或二维孔网的筛，其可及孔的开口由10个氧原子界定，并且称为孔之间的桥接距离小于0.70nm的距离，并且沸石使得催化剂进行标准的正十七烷异构化试验对于异构化产物具有至少70％的选择性为95％的转化率，并且催化剂含有至少5重量％的至少一种选自组中的加氢脱氢元件由非贵金属GVIII金属，GVIB金属和铌形成，并且催化剂优选含有磷。筛优选为NU-10，NU-23，NU-87，EU-13或Theta-1沸石。

2. 发明授权

US5954947A Process for mild hydrocracking of petroleum cuts using a catalyst containing at least two dealuminated Y zeolites 失效
标题翻译：使用含有至少两种脱铝Y沸石的催化剂轻度加氢裂化石油馏分的方法
公开(公告)号：US5954947A
公开(公告)日：1999-09-21
申请号：US955623
申请日：1997-10-22
申请人： Samuel Mignard , Nathalie George-Marchal , Eric Benazzi , Slavik Kasztelan
发明人： Samuel Mignard , Nathalie George-Marchal , Eric Benazzi , Slavik Kasztelan
IPC分类号： B01J29/16 , B01J29/08 , B01J29/40 , B01J29/80 , B01J37/20 , C10G47/16 , C10G47/18 , C10G47/20
CPC分类号： B01J29/80 , C10G47/16 , C10G47/20 , B01J2229/16 , B01J2229/26 , B01J2229/42 , B01J29/084 , B01J29/40
摘要： A mild hydroconversion process for petroleum cuts using a catalyst comprising at least one matrix, at least one Y zeolite with a lattice parameter which is in the range 24.15 .ANG. to 24.38 .ANG. (1 nm--10 .ANG.), at least one Y zeolite with a lattice parameter of more than 24.38 .ANG. and less than or equal to 24.51 .ANG., and at least one hydro-dehydrogenating element.
摘要翻译：用于使用包含至少一种基质，至少一种晶格参数的Y沸石的催化剂进行石油切割的温和加氢转化方法，所述Y沸石的范围为24.15至24.38（1nm-10），至少一个具有晶格参数大于24.38安培，小于或等于24.51安培，以及至少一个氢脱氢元件。

3. 发明授权

US06235960B1 Process for improving the pour point, and a catalyst based on at least one MTT, Ton or Fer zeolite 有权
标题翻译：改善倾点的方法，以及基于至少一种MTT，Ton或Fer沸石的催化剂
公开(公告)号：US06235960B1
公开(公告)日：2001-05-22
申请号：US09310181
申请日：1999-05-12
申请人： Eric Benazzi , Slavik Kasztelan , Nathalie George-Marchal
发明人： Eric Benazzi , Slavik Kasztelan , Nathalie George-Marchal
IPC分类号： C07C513
CPC分类号： C10G45/64 , B01J29/67 , B01J29/7284 , B01J29/7292 , B01J29/7484 , B01J29/7492 , B01J29/7884 , B01J29/7892 , B01J35/1061 , B01J35/1085 , B01J2229/26 , B01J2229/42
摘要： A process for improving the pour point of a feed comprising paraffins containing more than 10 carbon atoms, in which the feed to be treated is brought into contact with a catalyst comprising at least one zeolite with structure type MTT, TON or FER or any possible combination of these three, at least one hydro-dehydrogenating element selected from elements from group VIB and group VIII of the periodic table, at least one deposited promoter element (boron, silicon, phosphorous), optionally at least one group VIIA element, optionally at least one group VIIB element, at a temperature in the range 170° C. to 500° C., a pressure in the range 1 to 250 bars and at an hourly space velocity in the range 0.05 to 100 h−1, in the presence of hydrogen in an amount of 50 to 2000 l/l of feed. The oils obtained have good pour points and high viscosity indices (VI). The process is also applicable to gas oils, and other feeds requiring a reduction in pour point. The invention also relates to a catalyst containing silicon and to its use for converting hydrocarbon-containing feeds.
摘要翻译：一种用于改进含有多于10个碳原子的链烷烃的进料的倾点的方法，其中待处理的进料与包含至少一种结构类型为MTT，TON或FER的沸石或任何可能的组合的催化剂接触这些三种中的至少一种选自元素周期表第VIB族和第VIII族元素的至少一种加氢脱氢元素，至少一种沉积的促进元素（硼，硅，磷），任选至少一种VIIA族元素，任选至少一组VIIB元素，在170℃至500℃的温度范围内，压力范围为1至250巴，时间空间速度为0.05至100小时-1，在存在量为50至2000升/升的进料的氢。所得油具有良好的倾点和高粘度指数（VI）。该方法也适用于需要降低倾点的瓦斯油和其它进料。本发明还涉及含硅的催化剂及其用于转化含烃物料的用途。

4. 发明授权

US6106698A Catalyst comprising a zeolite selected from the group formed by NU-85, NU-86 and NU-87 zeolites and its use for hydroconverting hydrocarbon-containing petroleum feeds 失效
标题翻译：包含选自由NU-85，NU-86和NU-87沸石形成的基团的沸石及其用于加氢转化含烃石油原料的催化剂
公开(公告)号：US6106698A
公开(公告)日：2000-08-22
申请号：US257932
申请日：1999-02-26
申请人： Eric Benazzi , Nathalie George-Marchal , Slavik Kasztelan
发明人： Eric Benazzi , Nathalie George-Marchal , Slavik Kasztelan
IPC分类号： B01J29/72 , B01J29/06 , B01J29/78 , C10G45/12 , C10G47/00 , C10G47/16 , C10G47/20
CPC分类号： C10G47/20 , B01J29/78 , B01J2229/26 , B01J2229/42
摘要： The invention provides a hydrocracking catalyst comprising at least one matrix, a zeolite selected from the group formed by NU-85, NU-86 and NU-87 zeolites, at least one metal selected from the group formed by metals from group VIB and VIII of the periodic table, at least one element selected from the group formed by boron and silicon, optionally phosphorous, optionally at least one group VIIA element, and optionally at least one group VIIB element. The invention also relates to the use of the catalyst for hydrocracking hydrocarbon feeds.
摘要翻译：本发明提供一种加氢裂化催化剂，其包括至少一种基质，选自由NU-85，NU-86和NU-87沸石形成的基团的沸石，至少一种选自由VIB和VIII族的金属形成的金属周期表，选自由硼和硅形成的组中的至少一种元素，任选的磷，任选的至少一种VIIA族元素和任选的至少一种VIIB族元素。本发明还涉及催化剂用于加氢裂化烃进料的用途。

5. 发明授权

US5989410A Process for improving the pour point of paraffin feedstocks with a catalyst containing an IM-5 zeolite base 有权
标题翻译：用含有IM-5沸石基质的催化剂改进石蜡原料倾点的方法
公开(公告)号：US5989410A
公开(公告)日：1999-11-23
申请号：US172757
申请日：1998-10-15
申请人： Eric Benazzi , Nathalie George-Marchal , Christophe Gueret , Patrick Briot , Alain Billon , Pierre Marion
发明人： Eric Benazzi , Nathalie George-Marchal , Christophe Gueret , Patrick Briot , Alain Billon , Pierre Marion
IPC分类号： B01J29/72 , B01J29/44 , B01J29/74 , C01B39/08 , C08L91/06 , C09K3/00 , C10G35/06 , C10G45/04 , C10G45/20 , C10G45/64 , C10G35/085 , C10G35/095 , C10G47/12
CPC分类号： C10G45/64 , B01J29/74 , B01J2229/16 , B01J2229/26 , B01J2229/42
摘要： The invention relates to a process for improving the pour point of a feedstock that comprises paraffins of more than 10 carbon atoms, in which the feedstock that is to be treated is brought into contact with a catalyst that comprises the IM-5 zeolite and at least one hydro-dehydrogenating element, at a temperature of between 170 and 500.degree. C., a pressure of between 1 and 250 bar, and an hourly volume velocity of between 0.05 and 100 h.sup.-1, in the presence of hydrogen at a ratio of 50 to 2000 l/l of feedstock. The oils that are obtained have good pour points and high viscosity indices (VI). The process can also be applied to gas-oils and other feedstocks whose pour points need to be lowered.
摘要翻译：本发明涉及一种改进原料倾点的方法，该方法包括超过10个碳原子的链烷烃，其中待处理的原料与包含IM-5沸石的催化剂接触，并且至少一个加氢脱氢元件，在170-500℃的温度下，压力为1-250巴，小时体积速度为0.05-100小时-1，在氢存在下，比例为 50至2000升/原料。获得的油具有良好的倾点和高粘度指数（VI）。该方法也可应用于需要降低其倾点的瓦斯油和其他原料。

6. 发明授权

US5932088A Process for improving the pour point of paraffinic feeds using a catalyst based on NU-86 zeolite 失效
标题翻译：使用基于NU-86沸石的催化剂改进石蜡原料的倾点的方法
公开(公告)号：US5932088A
公开(公告)日：1999-08-03
申请号：US977739
申请日：1997-11-25
申请人： Eric Benazzi , Nathalie George-Marchal
发明人： Eric Benazzi , Nathalie George-Marchal
IPC分类号： B01J29/70 , C10G45/64 , C10G47/18 , C10M101/02 , C10M177/00 , C10N30/02 , C10N40/25 , C10G45/62
CPC分类号： C10G45/64
摘要： The invention concerns a process for improving the pour point of a feed comprising paraffins containing more than 10 carbon atoms, in which process the feed to be treated is brought into contact with a catalyst comprising NU-86 zeolite, preferably dealuminated, and at least one hydro-dehydrogenating element, at a temperature which is in the range 170.degree. C. to 500.degree. C., a pressure in the range 1 to 250 bar and an hourly space velocity in the range 0.05 to 100 h.sup.-1, in the presence of hydrogen in a proportion of 50 to 2000 l/l of feed. The product from heavy feeds is fractionated to produce at least one cut including at least one middle distillate with a reduced pour point, and a residue including oil bases with a reduced pour point and a high viscosity index.
摘要翻译：本发明涉及一种改进含有多于10个碳原子的链烷烃的进料的倾点的方法，其中待处理的进料与包含NU-86沸石，优选脱铝的催化剂和至少一种加氢脱氢元件，温度范围为170〜500℃，压力范围为1〜250巴，小时空速为0.05〜100小时-1，存在时的氢气比例为50至2000升/升的进料。将来自重质进料的产物分馏以产生至少一个包含至少一个具有降低的倾点的中间馏分的馏分，以及包含具有降低的倾点和高粘度指数的油基的残余物。

7. 发明授权

US5762902A Catalyst comprising a faujasite type zeolite and a ton type zeolite and a process for the hydroconversion of hydrocarbon petroleum feeds 失效
标题翻译：包含八面沸石型沸石和吨型沸石的催化剂以及烃石油原料的加氢转化方法
公开(公告)号：US5762902A
公开(公告)日：1998-06-09
申请号：US786646
申请日：1997-01-21
申请人： Eric Benazzi , Samuel Mignard , Nathalie George-Marchal , Slavik Kasztelan
发明人： Eric Benazzi , Samuel Mignard , Nathalie George-Marchal , Slavik Kasztelan
IPC分类号： B01J29/08 , B01J29/70 , B01J29/80 , C01B39/20 , C10G47/20 , C10G49/16 , C01B33/36 , B01J29/06
CPC分类号： C10G49/16 , B01J29/80 , B01J29/084 , B01J29/70 , Y10S423/21 , Y10S423/35
摘要： The invention concerns a composition comprising at least one matrix, at least one faujasite type zeolite and at least one TON type zeolite. The TON type zeolite can be Nu-10, THETA-1, KZ-2, or ISI-1. The catalyst also contains at least one hydrogenating element from groups VIII and VI. The catalyst is particularly for use for hydrocracking to maximize the yield of middle distillates (kerosine and gas oil).
摘要翻译：本发明涉及包含至少一种基质，至少一种八面沸石型沸石和至少一种TON型沸石的组合物。 TON型沸石可以是Nu-10，THETA-1，KZ-2或ISI-1。催化剂还含有至少一个来自VIII和VI族的氢化元素。催化剂特别用于加氢裂化以使中间馏分（煤油和瓦斯油）的产率最大化。

8. 发明授权

US06524470B1 Catalyst comprising beta zeolite and promoter element for hydrocracking 失效
标题翻译：包含β沸石和加氢裂化促进剂元素的催化剂
公开(公告)号：US06524470B1
公开(公告)日：2003-02-25
申请号：US09305290
申请日：1999-05-05
申请人： Slavik Kasztelan , Nathalie George-Marchal , Eric Benazzi
发明人： Slavik Kasztelan , Nathalie George-Marchal , Eric Benazzi
IPC分类号： B01J2976
CPC分类号： C10G47/20 , B01J29/7615 , B01J29/7815 , B01J2229/16 , B01J2229/26 , B01J2229/42 , C10G47/16
摘要： A catalyst comprising, in weight % with respect to the total catalyst weight 0.1% to 60% (expressed as the % by weight of oxide) of at least one hydro-dehydrogenating metal selected from the group formed by group VIB and VIII metals; 0.1% to 99% of at least one amorphous or low crystallinity porous matrix; 0.1% to 99.7% of beta zeolite; 0.1% to 20% (expressed as the % by weight of oxide) of at least one promoter element selected from the group formed by boron, silicon and phosphorous; 0 to 20% of at least one halogen; 0 to 20% (expressed as the % by weight of oxide) of at least one group VIIB element, the catalyst being especially useful for cracking hydrocarbon feeds.
摘要翻译：一种催化剂，其以相对于总催化剂重量％计含有选自由VIB族和VIII族金属形成的基团的至少一种加氢脱氢金属的0.1％至60％（以氧化物重量计） 0.1％至99％的至少一种无定形或低结晶度多孔基体; 0.1％至99.7％的β沸石; 至少一种选自硼，硅和磷形成的助催化剂元素的0.1％至20％（表示为氧化物的重量％）; 0至20％的至少一种卤素; 0至20％（表示为氧化物的重量％）的至少一种VIIB族元素，该催化剂特别适用于裂化烃进料。

9. 发明授权

US06350370B1 NU-85 zeolite catalyst and a process for improving the pour point of feeds containing paraffins 失效
标题翻译： NU-85沸石催化剂和改善含有链烷烃的进料的倾点的方法
公开(公告)号：US06350370B1
公开(公告)日：2002-02-26
申请号：US09635190
申请日：2000-08-09
申请人： Eric Benazzi , Nathalie George-Marchal , Christophe Gueret , Patrick Briot , Alain Billon , Pierre Marion
发明人： Eric Benazzi , Nathalie George-Marchal , Christophe Gueret , Patrick Briot , Alain Billon , Pierre Marion
IPC分类号： C10G4702
CPC分类号： C10G45/64 , B01J29/04 , C01B39/026
摘要： The present invention relates to a process for improving the pour point of a feed including paraffins containing more than 10 carbon atoms. Desirably, the feed to be treated is brought into contact with a catalyst based on NU-85 zeolite, at least partially in its acid form, and at least one hydro-dehydrogenating element, at a temperature which is in the range 170° C. to 500° C., a pressure in the range 1 to 250 bar and at an hourly space velocity in the range 0.05 to 100 h−1, in the presence of hydrogen in a proportion of 50 to 2000 l/l of feed.
摘要翻译：本发明涉及一种改善含有大于10个碳原子的链烷烃的进料的倾点的方法。理想地，待处理的进料与基于NU-85沸石的至少部分为其酸形式的催化剂和至少一种氢脱氢元件在170℃的温度下接触。在500至100℃的压力范围内，压力范围为1至250巴，时间空间范围为0.05至100小时-1，在氢气存在下，比例为50至2000升/升的进料。

10. 发明授权

US06171474B2 Zeolite Y catalyst containing silicon useful for hydrocracking 有权
标题翻译：含有可用于加氢裂化的硅的沸石Y催化剂
公开(公告)号：US06171474B2
公开(公告)日：2001-01-09
申请号：US09305288
申请日：1999-05-05
申请人： Slavik Kasztelan , Nathalie George-Marchal , Eric Benazzi
发明人： Slavik Kasztelan , Nathalie George-Marchal , Eric Benazzi
IPC分类号： C01G4700
CPC分类号： B01J29/08 , B01J2229/16 , B01J2229/22 , C10G47/20
摘要： Useful for example, for the hydrocracking of hydrocarbons is a catalyst comprising a matrix, at least one Y zeolite which is dealuminated and has a lattice parameter in the range 2.424 nm to 2.455 nm, a global SiO2/Al2O3 mole ratio is more than 8, the quantity of alkaline-earth metal cations or alkali metal cations and/or rare earth metal cations is such that the atomic ratio (n×Mn+)/Al is less than 0.8, the specific surface area, determined using the BET method, is more than 400 m2/g, and the water adsorption capacity is more than 6% by weight for P/P0 =0.2 at 25° C., said catalyst also comprising silicon deposited on the catalyst.
摘要翻译：对于例如烃的加氢裂解是有用的催化剂，它是一种催化剂，它包括一个基体，至少一个Y脱铝的Y沸石，其晶格参数在2.424 nm到2.455 nm之间，全球的SiO2 / Al2O3摩尔比大于8，碱土金属阳离子或碱金属阳离子和/或稀土金属阳离子的数量使得原子比（nxMn +）/ Al小于0.8，使用BET法测定的比表面积大于400 m2 / g，在25℃时P / P0 = 0.2，水吸附量大于6重量％，所述催化剂还含有沉积在催化剂上的硅。

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