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1. 发明申请

WO2018183916A1 CATALYTIC SYNTHESIS OF SUPER LINEAR ALKENYL ARENES USING RHODIUM CATALYSTS 审中-公开
公开(公告)号：WO2018183916A1
公开(公告)日：2018-10-04
申请号：PCT/US2018/025501
申请日：2018-03-30
申请人： UNIVERSITY OF VIRGINIA PATENT FOUNDATION , SCHINSKI, William , GOLDMAN, Alan
发明人： SCHINSKI, William , GOLDMAN, Alan , GUNNOE, Thomas B. , WEBSTER-GARDINER, Michael S. , SCHWARTZ, Nichole
IPC分类号： B01J29/84 , C07C15/24
CPC分类号： C07C17/266 , B01J29/44 , B01J31/1805 , B01J31/1815 , B01J31/183 , B01J31/2226 , B01J31/2291 , B01J2231/32 , B01J2531/0244 , B01J2531/822 , C07C2/66 , C07C5/393 , C07C41/30 , C07C2531/22 , C07C15/46 , C07C15/44 , C07C25/02 , C07C43/215 , C07C15/24
摘要： Catalytic methods for synthesis of super linear alkenyl arenes and alkyl arenes are provided. The methods are capable of synthesizing super linear alkyl and alkenyl arenes from simple arene and olefin starting materials and with high selectivity for linear coupling. Methods are also provided for making a 2,6-dimethylnapthalene (DMN) or 2,6-methylethylnapthalene (MEN).

2. 发明申请

WO2017205041A1 HIGH CHARGE DENSITY METALLOPHOSPHATE MOLECULAR SIEVES 审中-公开
标题翻译：高电荷密度金属磷酸盐分子筛
公开(公告)号：WO2017205041A1
公开(公告)日：2017-11-30
申请号：PCT/US2017/031555
申请日：2017-05-08
申请人： UOP LLC
发明人： LEWIS, Gregory J. , MOSCOSO, Jaime G. , KNIGHT, Lisa M. , NICHOLAS, Christopher P. , SEO, Seungwan , LEE, Junghwan , HONG, Suk Bong
IPC分类号： B01J27/18 , B01J29/84 , B01J31/02 , C01B39/54 , C10G11/05 , C10G35/095
摘要： A new family of highly charged crystalline microporous metallophosphate molecular sieves has been synthesized. These metallophosphates are represented by the empirical formula of: Rp+rA+mM2+xEyPOz where A is an alkali metal cation, R is at least one quaternary organoammonium cation, M is a divalent metal such as zinc and E is a trivalent framework element such as aluminum or gallium. This family of high charge density metallophosphate materials are among the first metalloalumino(gallo)phosphate-type molecular sieves to be stabilized by combinations of alkali and quaternary organoammonium cations, enabling unique compositions. This family of high charge density metallophosphate molecular sieves has catalytic properties for carrying out various hydrocarbon conversion processes and separation properties for separating at least one component.
摘要翻译：已经合成了一族新的高电荷结晶微孔金属磷酸盐分子筛。这些金属磷酸盐由经验式表示：Rp + rA + mM2 + xEyPOz其中A是碱金属阳离子，R是至少一个季铵有机铵阳离子，M是二价金属如锌，E是三价骨架元素，例如如铝或镓。这种高电荷密度金属磷酸盐材料家族是第一个通过碱金属和季铵有机铵阳离子组合稳定的金属铝（磷酸）型磷酸盐型分子筛，从而形成独特的组合物。这类高电荷密度金属磷酸盐分子筛具有用于进行各种烃转化过程和用于分离至少一种组分的分离性质的催化性质。

3. 发明申请

WO2015187311A1 CRYSTALLINE POROUS SILICOALUMINOPHOSPHATES AND METAL-SUBSTITUTED SILICOALUMINOPHOSPHATES WITH A HIERARCHICAL PORE STRUCTURE COMPRISING MICROPORES AND MESOPORES, METHODS FOR MAKING THE SAME, AND PROCESSES FOR CONVERTING OXYGENATES TO OLEFINS VIA REACTIONS CATALYZED BY THE SAME 审中-公开
标题翻译：晶体多孔硅烷基磷酸酯和金属取代的硅烷基磷酸酯具有包含微孔和多孔体的分层孔结构，其制备方法，以及通过其催化反应将氧化物转化为烯烃的方法
公开(公告)号：WO2015187311A1
公开(公告)日：2015-12-10
申请号：PCT/US2015/030313
申请日：2015-05-12
申请人： UOP LLC
发明人： YUHAS, Benjamin, Daniel
IPC分类号： B01J29/85 , B01J29/84 , B01J35/10 , B01J37/02 , B01J37/03 , B01J37/10 , C07C1/20 , C07C4/06 , C07C11/04 , C07C11/06
CPC分类号： B01J29/85 , B01J29/84 , B01J35/002 , B01J37/031 , B01J37/036 , B01J37/04 , B01J37/08 , B01J37/10 , C01B39/54 , C07C1/20 , C07C2529/06 , C07C2529/85 , Y02P20/52 , Y02P30/42 , C07C11/04 , C07C11/06
摘要： Crystalline porous silicoaluminophosphates and metal-substituted silicoaluminophosphates with a hierarchical pore structure comprising micropores and mesopores, methods for making the same, and methods for converting an oxygenate to an olefin via reactions catalyzed by the same are provided. In an embodiment, crystalline porous silicoaluminophosphates with a hierarchical pore structure have mesopores with a minimum dimension of 25 to 475 that constitute at least 7% of the total pore volume.
摘要翻译：提供了具有包含微孔和中孔的等级孔结构的结晶多孔硅铝磷酸盐和金属取代的硅铝磷酸盐，其制备方法以及通过其催化的反应将含氧化合物转化为烯烃的方法。在一个实施方案中，具有分级孔结构的结晶多孔硅铝磷酸盐具有构成总孔体积的至少7％的最小尺寸为25至475的介孔。

4. 发明申请

WO2015154827A1 METHOD FOR PRODUCING METAL EXCHANGED METALLO-ALUMINOPHOSPHATES BY SOLID-STATE ION EXCHANGE AT LOW TEMPERATURES 审中-公开
标题翻译：在低温下通过固体离子交换生产金属交换的金属铝 - 磷酸酯的方法
公开(公告)号：WO2015154827A1
公开(公告)日：2015-10-15
申请号：PCT/EP2014/072143
申请日：2014-10-15
申请人： HALDOR TOPSØE A/S
发明人： JANSSENS, Ton V. W. , VENNESTRØM, Peter N. R.
IPC分类号： B01J37/02 , B01J37/08 , B01J37/16 , B01D53/94 , B01J29/84 , B01J29/85 , B01J37/00 , B01J37/04 , B01J38/08
CPC分类号： B01J29/85 , B01D53/9418 , B01D2251/2062 , B01D2251/208 , B01D2255/20761 , B01D2255/50 , B01J29/084 , B01J29/84 , B01J37/0018 , B01J37/0036 , B01J37/0238 , B01J37/04 , B01J37/08 , B01J37/30 , B01J38/08 , B01J2229/183 , B01J2229/186 , B01J2229/38 , B01J2229/40 , C01B39/54 , F01N3/208 , F01N2370/02 , F01N2570/14 , F01N2610/02 , F01N2610/03 , F01N2610/10 , Y02P20/584
摘要： Method for the preparation of a metal exchanged crystalline microporous metalloaluminophosphate or mixtures containing metal exchanged microporous metalloaluminophosphates materials comprising the steps of providing a dry mixture containing a) one or more metalloaluminophosphates starting materials that exhibit ion exchange capacity, and b) one or more metal compounds; heating the mixture in a gaseous atmosphere containing ammonia to a temperature and for a time sufficient to initiate and perform a solid state ion exchange of ions of the metal compound and ions of the crystalline microporous material; and obtaining the metal-exchanged microporous metalloaluminophosphate material or mixtures containing the metal-exchanged microporous metalloaluminophosphate material.
摘要翻译：一种用于制备金属交换的结晶微孔金属铝磷酸盐或含有金属交换的微孔金属铝磷酸盐材料的混合物的方法，包括以下步骤：提供干混合物，该混合物含有a）一种或多种显示离子交换能力的金属铝磷酸盐原料，和b）一种或多种金属化合物 ; 将混合物在含有氨的气态气氛中加热至足以引发并进行结晶微孔材料的金属化合物和离子的离子的固态离子交换的温度和时间; 并获得金属交换的微孔金属铝磷酸盐物质或含有金属交换的微孔金属铝磷酸盐物质的混合物。

5. 发明申请

WO2022129539A1 PROCESS 审中-公开
公开(公告)号：WO2022129539A1
公开(公告)日：2022-06-23
申请号：PCT/EP2021/086514
申请日：2021-12-17
申请人： UNIVERSITETET I OSLO
发明人： OLSBYE, Unni , XIE, Jingxiu
IPC分类号： C07C1/04 , C07C1/06 , C07C1/20 , C07C11/04 , C07C11/06 , C07C11/08 , C07C11/10 , B01J29/84
摘要： The invention provides a process for preparing olefins from a mixed gaseous feed stream, wherein said mixed gaseous feed stream comprises three or more components selected from the group consisting of carbon dioxide, carbon monoxide, hydrogen, methanol and dimethyl ether, said process comprising contacting the mixed gaseous feed stream with a catalyst of formula (I): Μ(ΙΙ)χΑl11-χΡO4 (I), wherein M(II) is a divalent metal ion; and x = 0.002 to 0.5

6. 发明申请

WO2011010007A2 PROCEDE DE PREPARATION D'UN SOLIDE CRISTALLISE DE TYPE STRUCTURAL LTA EN MILIEU LIQUIDE IONIQUE 审中-公开
标题翻译：在离子液体介质中制备LTA结构型结晶固体的过程
公开(公告)号：WO2011010007A2
公开(公告)日：2011-01-27
申请号：PCT/FR2010/000464
申请日：2010-06-23
申请人： IFP ENERGIES NOUVELLES , FAYAD, Elie , BATS, Nicolas , MARTENS, Johan , KIRSCHHOCK, Christine , REBOURS, Bernadette , QUOINEAUD, Anne-Agathe
发明人： FAYAD, Elie , BATS, Nicolas , MARTENS, Johan , KIRSCHHOCK, Christine , REBOURS, Bernadette , QUOINEAUD, Anne-Agathe
IPC分类号： C01B37/04 , C01B39/14 , B01J29/83 , B01J29/84 , B01J29/82
CPC分类号： B01J29/83 , B01J29/84 , C01B37/04 , C01B39/14
摘要： On décrit un procédé de préparation d'un solide métallophosphate cristallisé de type structural LTA comprenant au moins les étapes suivantes : i) le mélange, en présence d'au moins un liquide ionique constitué d'un sel de 1-benzyl-3- méthylimidazolium, d'au moins une source d'anions phosphates, d'au moins une source d'au moins un élément trivalent G, d'au moins une source d'anions fluorures et éventuellement d'au moins une source d'un élément tétravalent, ii) le traitement ionothermal jusqu'à ce que ledit solide de type structural LTA se forme.
摘要翻译：
我们正在描述一个程序。为了制备结晶固体结晶磷酸，结构类型的LTA至少包括以下阶段：i）在至少一种离子液体存在下，所述混合物由以下物质构成： 1-苄基-3-甲基咪唑鎓的盐，至少一种磷酸根阴离子源，至少一种三价G的至少一种来源，至少一种氟化物阴离子的来源和可能至少有一个永久性故障的来源，（ii）离子热处理长达一年; 什么说结构固体LTA形式。

7. 发明申请

WO2010085708A2 CATALYTIC DEHYDRATION OF ALCOHOLS USING PHASE PURE, CALCINED SINGLE AND MULTI-SITE HETEROGENEOUS CATALYSTS 审中-公开
标题翻译：用纯相煅烧单相和多相多相催化剂对醇进行催化脱水
公开(公告)号：WO2010085708A2
公开(公告)日：2010-07-29
申请号：PCT/US2010/021882
申请日：2010-01-22
申请人： SIGNA CHEMISTRY, INC. , LEFENFELD, Michael , RAJA, Robert , PATERSON, Alexander, James , POTTER, Matthew, Edward
发明人： LEFENFELD, Michael , RAJA, Robert , PATERSON, Alexander, James , POTTER, Matthew, Edward
IPC分类号： B01J29/84 , B01J29/85 , C01B37/06 , C01B37/08 , C07C1/24 , B01J37/08
CPC分类号： B01J29/84 , B01J29/85 , B01J35/1057 , C01B37/065 , C01B37/08 , C01B39/54 , C07C1/24 , C07C2529/84 , C07C2529/85 , Y02P20/52 , C07C11/04 , C07C11/09 , C07C11/06 , C07C15/46
摘要： The disclosure describes a new class of isomorphously metal- substituted aluminophosphate materials with high phase purity that are capable of performing selective Brönsted acid catalyzed chemical transformations, such as transforming alcohols to olefins, with high conversions and selectivities using mild conditions. Isomorphous substitutions of functional metal ions for both the aluminum ions and the phosphorous ions were successful in various AlPO structures, along with multiple metal substitutions into a single aluminum site and/or a phosphorous site. This invention can be used towards the catalytic conversion of hydroxylated compounds of linear and/or branched moiety with the possibility of being substituted to their respective hydrocarbon products, preferably light olefins containing 2 to 10 carbon atoms, among other chemistries.
摘要翻译：本公开描述了一类具有高相纯度的新型同型金属取代的铝磷酸盐材料，其能够进行选择性布朗斯特酸催化的化学转化，例如将醇转化成烯烃，具有高转化率和使用温和条件的选择性。铝离子和磷离子的功能金属离子的同晶型取代在各种AlPO结构中是成功的，以及多个金属取代成单个铝位点和/或磷位置。本发明可以用于直链和/或支链部分的羟基化化合物的催化转化，其中可能被取代成其各自的烃产物，优选其它化学物质中含有2至10个碳原子的轻烯烃。

8. 发明申请

WO2005039761A3 MOLECULAR SIEVE CATALYST COMPOSITION, ITS MAKING AND USE IN CONVERSION PROCESSES 审中-公开
标题翻译：分子筛催化剂组合物，其在转化过程中的制备和使用
公开(公告)号：WO2005039761A3
公开(公告)日：2007-02-01
申请号：PCT/US2004026547
申请日：2004-08-16
申请人： EXXONMOBIL CHEM PATENTS INC , CHANG YUN-FENG , VAUGHN STEPHEN N , CLEM KENNETH R , MARTENS LUC R M , HU WEIGUO
发明人： CHANG YUN-FENG , VAUGHN STEPHEN N , CLEM KENNETH R , MARTENS LUC R M , HU WEIGUO
IPC分类号： B01J37/00 , B01J29/06 , B01J29/84 , B01J29/85 , B01J35/00 , C07C1/20 , C10G3/00
CPC分类号： B01J37/0045 , B01J29/06 , B01J29/84 , B01J29/85 , B01J35/002 , B01J37/0009 , C07C1/20 , C07C2521/04 , C07C2521/06 , C07C2521/16 , C07C2529/85 , Y02P30/20 , Y02P30/42 , Y10S502/504 , C07C11/02
摘要： This invention provides methods of making molecular sieve catalyst particles, molecular sieve slurries that can be used in such methods, molecular sieve catalyst compositions and their use in catalytic hydrocarbon conversion processes. In one of its aspects, the invention provides a method of making molecular sieve catalyst particles, the method comprising the steps of: a) providing a solution or suspension of an aluminum-containing inorganic oxide precursor in a liquid medium; b) combining the solution or suspension of aluminum-containing inorganic oxide precursor with a molecular sieve, and optionally other formulating agents, to form a catalyst formulation slurry; c) aging the catalyst formulation slurry to generate in said slurry a percentage, or increase in said slurry the existing percentage, of aluminum atoms of the aluminum-containing precursor in the form of oligomers having a sharp 27 Al NMR peak at 62-63 ppm; and d) forming molecular sieve catalyst particles from the catalyst formulation slurry. The catalyst compositions obtained by the methods of the present invention have improved attrition resistance, and are particularly useful in hydrocarbon conversion processes.
摘要翻译：本发明提供制备分子筛催化剂颗粒，可用于这些方法的分子筛浆料，分子筛催化剂组合物及其在催化烃转化方法中的应用的方法。在其一个方面，本发明提供了制备分子筛催化剂颗粒的方法，该方法包括以下步骤：a）提供含铝无机氧化物前体在液体介质中的溶液或悬浮液; b）将含铝的无机氧化物前体的溶液或悬浮液与分子筛和任选的其它配制剂组合以形成催化剂配方浆料; c）使所述催化剂配方浆料老化以在所述浆料中产生一种百分比，或增加所述浆料中含铝前体的铝原子的现有百分比，其具有尖锐的Al 2 O 3 在62-63ppm的NMR峰; 和d）从催化剂配方浆料形成分子筛催化剂颗粒。通过本发明的方法获得的催化剂组合物具有改善的耐磨耗性，并且在烃转化方法中特别有用。

9. 发明申请

WO0205952A3 ATTRITION RESISTANT CATALYST FOR LIGHT OLEFIN PRODUCTION 审中-公开
标题翻译：耐光催化剂用于轻质烯烃生产
公开(公告)号：WO0205952A3
公开(公告)日：2002-06-06
申请号：PCT/US0121958
申请日：2001-07-12
申请人： UOP LLC , BARGER PAUL T , MARKER TERRY L , KARCH JOHN A
发明人： BARGER PAUL T , MARKER TERRY L , KARCH JOHN A
IPC分类号： B01J29/85 , C07C1/20 , B01J29/84
CPC分类号： B01J29/85 , B01J2229/26 , B01J2229/42 , C07C1/20 , C07C2521/04 , C07C2521/06 , C07C2521/08 , C07C2521/12 , C07C2527/167 , C07C2529/84 , Y02P30/42 , C07C11/02
摘要： Catalyst compositions that are effective for the conversion of methanol to light olefins (e.g. ethylene) are disclosed. The catalysts comprise a crystalline metalloaluminophosphate molecular sieve (e.g. SAPO-34) and a matrix material comprising an inorganic oxide binder and a filler, preferably a clay (e.g. kaolin). It has been discovered that by maintaining the content of the molecular sieve at 40 % or less by weight, the overall catalyst attrition resistance is markedly improved.
摘要翻译：公开了有效将甲醇转化成轻质烯烃（例如乙烯）的催化剂组合物。催化剂包含结晶金属铝磷酸盐分子筛（例如SAPO-34）和包含无机氧化物粘合剂和填料（优选粘土（例如高岭土））的基质材料。已经发现，通过将分子筛的含量保持在按重量计40％或更少，整体催化剂耐磨性得到显着改善。

10. 发明申请

WO01036329A1 MOLECULAR SIEVES 审中-公开
标题翻译：分子筛
公开(公告)号：WO01036329A1
公开(公告)日：2001-05-25
申请号：PCT/US2000/030346
申请日：2000-11-03
IPC分类号： B01J29/84 , B01J29/85 , C01B37/06 , C01B37/08
CPC分类号： B01J29/85 , B01J29/84 , C01B37/06 , C01B37/065 , C01B37/08 , Y10S423/30
摘要： The present invention provides a method for the synthesis of MeAPO molecular sieves which includes the following steps: providing a source of alumina, a source of phosphorus, water, and a template suitable for forming a MeAPO molecular sieves; providing a source of metal (Me) including metal particles, the metal particles measuring, in their largest dimension, equal to or less than five nanometers; providing a water soluble organic solvent capable of solubilizing the source of metal; forming a synthesis mixture from the source of alumina, the source of phosphorus, the water, the template, the source of metal, and the solvent; and forming a MeAPO molecular sieve from the synthesis mixture.
摘要翻译：本发明提供了一种合成MeAPO分子筛的方法，其包括以下步骤：提供氧化铝源，磷源，水和适于形成MeAPO分子筛的模板; 提供包括金属颗粒的金属（Me）源，金属颗粒在其最大尺寸上测量等于或小于5纳米; 提供能溶解金属源的水溶性有机溶剂; 从氧化铝源，磷源，水，模板，金属源和溶剂形成合成混合物; 并从合成混合物中形成MeAPO分子筛。

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