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1. 发明申请

WO2009156436A3 PROCESS TO MAKE OLEFINS FROM ORGANICS 审中-公开
标题翻译：从有机物制备烯烃的方法
公开(公告)号：WO2009156436A3
公开(公告)日：2010-02-18
申请号：PCT/EP2009057890
申请日：2009-06-24
申请人： TOTAL PETROCHEMICALS RES FELUY , NESTERENKO NIKOLAI , VERMEIREN WALTER , GRASSO GIACOMO , VAN DONK SANDER , GARCIA WOLFGANG
发明人： NESTERENKO NIKOLAI , VERMEIREN WALTER , GRASSO GIACOMO , VAN DONK SANDER , GARCIA WOLFGANG
IPC分类号： C07C1/20 , B01J27/16 , B01J29/40 , B01J37/28 , C10G11/05
CPC分类号： C07C1/20 , B01J21/08 , B01J21/16 , B01J27/14 , B01J29/18 , B01J29/40 , B01J29/65 , B01J29/90 , B01J38/12 , B01J2229/16 , B01J2229/18 , B01J2229/36 , B01J2229/37 , C07C1/26 , C07C1/322 , C07C4/06 , C07C2529/40 , Y02P20/584 , Y02P30/42 , C07C11/02
摘要： The present invention relates to a process to make light olefins, in a combined XTO-OC process, from an oxygen-containing, halogenide-containing or sulphur-containing organic feedstock comprising : a0) providing a first portion and a second portion of said oxygen-containing, halogenide-containing or sulphur-containing organic feedstock, a) providing a catalyst comprising zeolitic molecular sieves containing at least 10 membered ring pore openings or larger in their microporous structure, b) providing an XTO reaction zone, an OC reaction zone and a catalyst regeneration zone, said catalyst circulating in the three zones, such that at least a portion of the regenerated catalyst is passed to the OC reaction zone, optionally at least a portion of the catalyst in the OC reaction zone is passed to the XTO reaction zone and at least a portion of the catalyst in the XTO reaction zone is passed to the regeneration zone; c) contacting the first portion of said oxygen-containing, halogenide- containing or sulphur-containing organic feedstock in the XTO reactor with the catalyst at conditions effective to convert at least a portion of the feedstock to form a XTO reactor effluent comprising light olefins and a heavy hydrocarbon fraction; d) separating said light olefins from said heavy hydrocarbon fraction; e) contacting said heavy hydrocarbon fraction and the second portion of said oxygen-containing, halogenide-containing or sulphur-containing organic feedstock in the OC reactor with the catalyst at conditions effective to convert at least a portion of said heavy hydrocarbon fraction and oxygen-containing, halogenide-containing or sulphur-containing organic feedstock to light olefins.
摘要翻译：本发明涉及一种在组合的XTO-OC方法中由含氧，含卤素或含硫有机原料制备轻质烯烃的方法，包括：a）提供所述氧气的第一部分和第二部分 a）提供包含在其微孔结构中含有至少10元环孔或更大孔沸石分子筛的催化剂，b）提供XTO反应区，OC反应区和催化剂再生区，所述催化剂在三个区域中循环，使得至少一部分再生催化剂通入OC反应区，任选地将OC反应区中的至少一部分催化剂通入XTO反应区域，并且XTO反应区中的至少一部分催化剂被传送到再生区; c）在有效地转化至少一部分原料以形成包含轻质烯烃的XTO反应器流出物的条件下，将XTO反应器中的含氧卤化物或含硫有机原料的第一部分与催化剂接触，重质烃馏分; d）从所述重质烃馏分中分离出所述轻质烯烃; e）在OC反应器中将所述重质烃部分和第二部分所述含氧卤化物或含硫有机原料与所述催化剂接触，所述条件有效地将至少一部分所述重质烃部分和氧 - 含卤素或含硫有机原料转化成轻质烯烃。

2. 发明申请

WO2009156433A3 PROCESS TO MAKE OLEFINS FROM OXYGENATES 审中-公开
标题翻译：从氧化剂制备油脂的方法
公开(公告)号：WO2009156433A3
公开(公告)日：2010-02-18
申请号：PCT/EP2009057887
申请日：2009-06-24
申请人： TOTAL PETROCHEMICALS RES FELUY , NESTERENKO NIKOLAI , VERMEIREN WALTER , GRASSO GIACOMO , VAN DONK SANDER , GARCIA WOLFGANG
发明人： NESTERENKO NIKOLAI , VERMEIREN WALTER , GRASSO GIACOMO , VAN DONK SANDER , GARCIA WOLFGANG
IPC分类号： C07C1/20 , B01J29/40 , B01J37/28
CPC分类号： C07C1/22 , B01J21/08 , B01J21/16 , B01J27/14 , B01J29/18 , B01J29/40 , B01J29/65 , B01J29/90 , B01J37/10 , B01J38/12 , B01J2229/16 , B01J2229/186 , B01J2229/36 , C07C1/20 , C07C1/26 , C07C1/322 , C07C4/06 , C07C2529/40 , C10G3/44 , C10G3/49 , C10G3/62 , C10G9/00 , C10G55/04 , C10G2400/20 , Y02P20/584 , Y02P30/20 , Y02P30/42 , C07C11/02
摘要： The present invention relates to a process to make light olefins, in a combined XTO-OC process, from an oxygen-containing, halogenide-containing or sulphur-containing organic feedstock comprising : a) providing a catalyst comprising zeolitic molecular sieves containing 10 member and larger channels in their microporous structure, b) providing an XTO reaction zone, an OC reaction zone and a catalyst regeneration zone, said catalyst circulating in the three zones, such that at least a portion of the regenerated catalyst is passed to the OC reaction zone, at least a portion of the catalyst in the OC reaction zone is passed to the XTO reaction zone and at least a portion of the catalyst in the XTO reaction zone is passed to the regeneration zone; c) contacting said oxygen-containing, halogenide-containing or sulphur- containing organic feedstock in the XTO reactor with the catalyst at conditions effective to convert at least a portion of the feedstock to form a XTO reactor effluent comprising light olefins and a heavy hydrocarbon fraction; d) separating said light olefins from said heavy hydrocarbon fraction; e) contacting said heavy hydrocarbon fraction in the OC reactor with the catalyst at conditions effective to convert at least a portion of said heavy hydrocarbon fraction to light olefins.
摘要翻译：本发明涉及一种在组合的XTO-OC方法中由含氧的含卤素或含硫有机原料制备轻质烯烃的方法，包括：a）提供包含含有10个成员的沸石分子筛和在其微孔结构中较大的通道，b）提供XTO反应区，OC反应区和催化剂再生区，所述催化剂在三个区中循环，使得至少一部分再生催化剂通过OC反应区，将OC反应区中的至少一部分催化剂通入XTO反应区，并将XTO反应区中的至少一部分催化剂通入再生区; c）在有效地转化至少一部分原料以形成包含轻质烯烃和重质烃部分的XTO反应器流出物的条件下，将XTO反应器中的含氧，含卤素或含硫有机原料与催化剂接触 ; d）从所述重质烃馏分中分离出所述轻质烯烃; e）使OC反应器中的所述重质烃馏分与催化剂在有效将至少一部分所述重质烃馏分转化为轻质烯烃的条件下接触。

3. 发明申请

WO2009156435A3 PROCESS TO MAKE OLEFINS AND AROMATICS FROM ORGANICS 审中-公开
标题翻译：从有机物制备油脂和芳香油的工艺
公开(公告)号：WO2009156435A3
公开(公告)日：2010-02-18
申请号：PCT/EP2009057889
申请日：2009-06-24
申请人： TOTAL PETROCHEMICALS RES FELUY , NESTERENKO NIKOLAI , VERMEIREN WALTER , GRASSO GIACOMO , VAN DONK SANDER , GARCIA WOLFGANG
发明人： NESTERENKO NIKOLAI , VERMEIREN WALTER , GRASSO GIACOMO , VAN DONK SANDER , GARCIA WOLFGANG
IPC分类号： C07C1/20 , B01J29/40 , B01J37/28
CPC分类号： C07C1/20 , B01J21/08 , B01J21/16 , B01J27/14 , B01J29/18 , B01J29/40 , B01J29/65 , B01J29/90 , B01J38/12 , B01J2229/16 , B01J2229/18 , B01J2229/36 , B01J2229/37 , C07C1/26 , C07C1/322 , C07C2/864 , C07C4/06 , C07C2529/40 , Y02P20/584 , Y02P30/42 , C07C15/02 , C07C11/02
摘要： The present invention relates to a process to make light olefins and aromatics, in a combined XTO-OC process, from an oxygen-containing, halogenide-containing or sulphur-containing organic feedstock comprising : a0) providing a first portion and a second portion of said oxygen-containing, halogenide-containing or sulphur-containing organic feedstock, a) providing a catalyst comprising zeolitic molecular sieves containing at least 10 membered ring pore openings or larger in their microporous structure, b) providing an XTO reaction zone, an OC reaction zone and a catalyst regeneration zone, said catalyst circulating in the three zones, such that at least a portion of the regenerated catalyst is passed to the OC reaction zone, at least a portion of the catalyst in the OC reaction zone is passed to the XTO reaction zone and at least a portion of the catalyst in the XTO reaction zone is passed to the regeneration zone; c) contacting the first portion of said oxygen-containing, halogenide- containing or sulphur-containing organic feedstock in the XTO reactor with the catalyst at conditions effective to convert at least a portion of the feedstock to form a XTO reactor effluent comprising light olefins and a heavy hydrocarbon fraction; d) separating said light olefins from said heavy hydrocarbon fraction; e) contacting said heavy hydrocarbon fraction and the second portion of said oxygen-containing, halogenide-containing or sulphur-containing organic feedstock in the OC reactor with the catalyst at conditions effective to convert at least a portion of said heavy hydrocarbon fraction and oxygen-containing, halogenide-containing or sulphur-containing organic feedstock to light olefins and aromatics.
摘要翻译：本发明涉及一种在组合的XTO-OC方法中由含氧，含卤素或含硫有机原料制备轻质烯烃和芳族化合物的方法，包括：a0）提供第一部分和第二部分所述含氧，含卤素或含硫有机原料，a）提供包含在其微孔结构中含有至少10元环孔孔或更大的沸石分子筛的催化剂，b）提供XTO反应区，OC反应区域和催化剂再生区，所述催化剂在三个区域中循环，使得至少一部分再生催化剂通过OC反应区，OC反应区中的至少一部分催化剂通过XTO 反应区和XTO反应区中的至少一部分催化剂通入再生区; c）在有效地转化至少一部分原料以形成包含轻质烯烃的XTO反应器流出物的条件下，将XTO反应器中的含氧卤化物或含硫有机原料的第一部分与催化剂接触，重质烃馏分; d）从所述重质烃馏分中分离出所述轻质烯烃; e）在OC反应器中将所述重质烃部分和第二部分所述含氧卤化物或含硫有机原料与所述催化剂接触，所述条件有效地将至少一部分所述重质烃部分和氧 - 含有卤化物或含硫有机原料至轻质烯烃和芳族化合物。

4. 发明申请

WO2009156434A3 PROCESS TO MAKE OLEFINS FROM OXYGENATES 审中-公开
标题翻译：从氧化剂制备油脂的方法
公开(公告)号：WO2009156434A3
公开(公告)日：2010-02-18
申请号：PCT/EP2009057888
申请日：2009-06-24
申请人： TOTAL PETROCHEMICALS RES FELUY , NESTERENKO NIKOLAI , VERMEIREN WALTER , GRASSO GIACOMO , VAN DONK SANDER , GARCIA WOLFGANG
发明人： NESTERENKO NIKOLAI , VERMEIREN WALTER , GRASSO GIACOMO , VAN DONK SANDER , GARCIA WOLFGANG
IPC分类号： C07C1/20 , B01J27/16 , B01J29/40 , B01J37/28 , C10G11/05
CPC分类号： C07C1/20 , B01J21/08 , B01J21/16 , B01J27/14 , B01J29/18 , B01J29/40 , B01J29/65 , B01J29/90 , B01J38/02 , B01J38/12 , B01J2229/16 , B01J2229/18 , B01J2229/36 , B01J2229/37 , C07C1/26 , C07C1/322 , C07C4/06 , C07C2529/40 , Y02P20/584 , Y02P30/42 , C07C11/02
摘要： The present invention relates to a process to make light olefins, in a combined XTO-OC process, from an oxygen-containing, halogenide-containing or sulphur-containing organic feedstock comprising : a0) providing a first portion and a second portion of said oxygen-containing, halogenide-containing or sulphur-containing organic feedstock, a) providing a catalyst comprising zeolitic molecular sieves containing at least 10 membered ring pore openings or larger in their microporous structure, b) providing an XTO reaction zone, an OC reaction zone and a catalyst regeneration zone, said catalyst circulating in the three zones, such that at least a portion of the regenerated catalyst is passed to the OC reaction zone, at least a portion of the catalyst in the OC reaction zone is passed to the XTO reaction zone and at least a portion of the catalyst in the XTO reaction zone is passed to the regeneration zone;c) contacting the first portion of said oxygen-containing, halogenide- containing or sulphur-containing organic feedstock in the XTO reactor with the catalyst at conditions effective to convert at least a portion of the feedstock to form a XTO reactor effluent comprising light olefins and a heavy hydrocarbon fraction; d) separating said light olefins from said heavy hydrocarbon fraction; e) contacting said heavy hydrocarbon fraction and the second portion of said oxygen-containing, halogenide-containing or sulphur-containing organic feedstock in the OC reactor with the catalyst at conditions effective to convert at least a portion of said heavy hydrocarbon fraction and oxygen-containing, halogenide-containing or sulphur-containing organic feedstock to light olefins.
摘要翻译：本发明涉及一种在组合的XTO-OC方法中由含氧，含卤素或含硫有机原料制备轻质烯烃的方法，包括：a）提供所述氧气的第一部分和第二部分 a）提供包含在其微孔结构中含有至少10元环孔或更大孔沸石分子筛的催化剂，b）提供XTO反应区，OC反应区和催化剂再生区，所述催化剂在三个区域中循环，使得至少一部分再生催化剂通过OC反应区，OC反应区中的至少一部分催化剂通入XTO反应区并且将XTO反应区中的至少一部分催化剂通入再生区; c）使含氧化合物，含卤化物的或第一部分在XTO反应器中含有lphur的有机原料与催化剂在有效地转化至少一部分原料以形成包含轻质烯烃和重质烃馏分的XTO反应器流出物的条件下反应; d）从所述重质烃馏分中分离出所述轻质烯烃; e）在OC反应器中将所述重质烃部分和第二部分所述含氧卤化物或含硫有机原料与所述催化剂接触，所述条件有效地将至少一部分所述重质烃部分和氧 - 含卤素或含硫有机原料转化成轻质烯烃。

5. 发明申请

WO2011073226A2 DEBOTTLENECKING OF A STEAM CRACKER UNIT TO ENHANCE PROPYLENE PRODUCTION 审中-公开
标题翻译：蒸汽破碎机单元的加固以增强丙烯生产
公开(公告)号：WO2011073226A2
公开(公告)日：2011-06-23
申请号：PCT/EP2010069694
申请日：2010-12-15
申请人： TOTAL PETROCHEMICALS RES FELUY , VERMEIREN WALTER , BOUVART FRANCOIS , CELIE INEKE , GARCIA WOLFGANG
发明人： VERMEIREN WALTER , BOUVART FRANCOIS , CELIE INEKE , GARCIA WOLFGANG
IPC分类号： C10G9/00 , C10G51/04 , C10G69/06
CPC分类号： C10G51/04 , C10G9/002 , C10G69/06 , C10G2300/807 , C10G2400/20 , C10G2400/26
摘要： The present invention is a method for debottlenecking an existing steam cracker unit of which the operation is modified from high severity to low severity operation, having a cracking zone and a fractionation zone, said fractionation zone comprising a gasoline stripper, a de-methaniser (I), a de-ethaniser (I), a de-propaniser (I) and a de-butaniser (I), said de-propaniser (I) receiving product from the bottom of the de-ethaniser (I) and optionally product from the bottom of the gasoline stripper (I), wherein said debottlenecking method comprises the steps of : a) adding a selective hydrogenation unit (II), b) adding a cracking reactor (II) comprising a catalyst selective towards light olefins in the outlet, c) adding a re-run column and a de-propaniser (II), d) sending a part or all of the bottoms stream of the gasoline stripper (I) to the selective hydrogenation unit (II) and subsequently to the cracking reactor (II) at conditions effective to produce an outlet with an olefin content of lower molecular weight than that of the inlet, e) sending a part of the bottoms stream of the de-ethaniser (I) to the de-propaniser (II), such as, not to overload the de-propaniser (I), f) optionally sending a part or all of the overhead raw C4 fraction of the de-butaniser (I) to the selective hydrogenation unit (II), g) sending the cracking reactor (II) outlet to the re-run column to produce a C6+ bottom stream and a C1-C5 overhead, sending said overhead to the de-propaniser (II) to produce a C1-C3 overhead and a C4+ bottom stream recycled in whole or in part to the selective hydrogenation unit (II), optionally withdrawing a part of said C4+ bottom stream.
摘要翻译：本发明是一种用于对现有蒸汽裂化装置进行脱瓶的方法，该装置的操作由高严重度到低严重性操作改变，具有裂化区和分馏区，所述分馏区包含汽提汽提塔，脱甲烷反应器），脱乙烷化酶（I），去propaniser（I）和脱丁烷（I），脱唾液酸酶（I）从脱乙烷（I）的底部接收产物，汽油汽提器（I）的底部，其中所述消除瓶颈方法包括以下步骤：a）加入选择性氢化单元（II），b）在出口中加入包含对轻质烯烃选择性的催化剂的裂化反应器（II） c）加入再运行的塔和去推进剂（II），d）将汽提汽提塔（I）的一部分或全部底部物流送入选择性加氢装置（II），随后将其送入裂解反应器 II）在有效产生具有烯烃含量的出口的条件下分子量低于入口的分子量，e）将去乙烷化器（I）的一部分底部物流送至去岐化器（II），例如不使去岐化剂（I）过载， f）任选将脱丁烷（I）的塔顶馏分C4馏分的一部分或全部送入选择氢化单元（II），g）将裂解反应器（II）出口送至再运行塔，以产生 C6 +底部流和C1-C5塔顶馏出物，将所述开销送到脱丙烷（II）以产生C1-C3塔顶馏出物，以及将全部或部分再循环至选择性加氢装置（II）的C4 +底部物流，任选地退出所述C4 +底部流的一部分。

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