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11. 发明申请

WO2008028343A1 一种烃类催化转化方法审中-公开
公开(公告)号：WO2008028343A1
公开(公告)日：2008-03-13
申请号：PCT/CN2006/002560
申请日：2006-09-28
申请人：中国石油化工股份有限公司 , 中国石油化工股份有限公司石油化工科学研究院 , 谢朝钢 , 朱根权 , 杨义华 , 罗一斌 , 龙军 , 舒兴田 , 张久顺
发明人：谢朝钢 , 朱根权 , 杨义华 , 罗一斌 , 龙军 , 舒兴田 , 张久顺
IPC分类号： C10G11/05 , B01J29/80 , B01J29/072 , B01J29/076 , B01J29/40
CPC分类号： B01J29/80 , B01J29/084 , B01J29/18 , B01J29/40 , B01J29/60 , B01J29/7057 , B01J29/7615 , B01J29/7815 , B01J37/0045 , B01J2229/18 , B01J2229/42 , C10G11/02 , C10G11/05 , C10G11/14 , C10G11/16 , C10G11/18 , C10G2300/1033 , C10G2300/104 , C10G2300/1044 , C10G2300/1055 , C10G2300/107 , C10G2300/1074 , C10G2300/1077 , C10G2300/4018 , C10G2300/4093 , C10G2300/807 , C10G2400/02 , C10G2400/04 , C10G2400/20
摘要： A process for catalytic converting a hydrocarbon feed includes the following steps: catalytic cracking the hydrocarbon feed in a reactor by contacting with a catalyst system, and fractionating the reaction product from the reactor to obtain low carbon olefins, gasoline, diesel, heavy oil and other low molecular saturated hydrocarbons. The catalyst system comprises 1-60wt% zeolite mixture, 5-99wt% refractory inorganic oxide and 0-70wt% clay, based on the total weight of the catalyst. The zeolite mixture includes 1-75wt% beta zeolite modified by phosphorus and transition metal M, 25-99wt% zeolite with MFI structure and 0-74wt% large pore size zeolite based on the total weight of the zeolite mixture. The anhydrous composition of the beta zeolite modified by phosphorus and transition metal M expressed as a weight percentage based on oxide is given by: (0-0.3) Na 2 O·(0.5-10) Al 2 O 3 ·(1.3-10) P 2 O 5 ·(0.7-15) M x O y ·(64-97) SiO 2 , wherein M is selected from the group consisting of Fe, Co, Ni, Cu, Mn, Zn and Sn, x represents the molecular number of M, and y represents the number needed for the oxidation state of M. The process for catalytic converting hydrocarbons of this invention can achieve enhanced ability of converting hydrocarbons, and increased yield of low carbon olefins, especially increased yield of propylene.

12. 发明申请

WO2006057954A3 USE OF A MONOLITH CATALYST TO PREPARE ETHYLBENZENE 审中-公开
标题翻译：用单一催化剂制备乙苯
公开(公告)号：WO2006057954A3
公开(公告)日：2006-12-14
申请号：PCT/US2005042122
申请日：2005-11-21
申请人： FINA TECHNOLOGY , KELLY KEVIN
发明人： KELLY KEVIN
IPC分类号： C07C2/66 , C07C2/70
CPC分类号： B01J35/04 , B01J19/2485 , B01J27/188 , B01J29/7057 , C07C2/66 , C07C2521/04 , C07C2521/08 , C07C2521/10 , C07C2523/10 , C07C2529/70 , Y02P20/582 , C07C15/073
摘要： Disclosed is an alkylation reactor for preparing ethylbenzene. The reactor comprises a monolith catalyst system that includes a monolith support impregnated orco-formed with a catalyst suitable to catalyze the alkylation of benzene with ethylene. The catalyst may be selected from, for example, zeolites such as beta zeolite and MCM-22 zeolite, and fixed super acids. Also disclosed is a method of preparing ethylbenzene by alkylating a mixture of benzene and ethylene in an alkylation reactor comprising a monolith catalyst system, to including a monolith support impregnated or co-formed with a suitable catalyst. In one embodiment the invention provides a convenient means of upgrading an existing reactor that has previously been used for conventional liquid phase alkylations such as those catalyzed by aluminum trichloride. The inventive alkylation method may be effectively and advantageously carried out under critical or near critical conditions, if desired.
摘要翻译：公开了一种用于制备乙苯的烷基化反应器。所述反应器包含整体式催化剂体系，所述整体式催化剂体系包括浸渍有或适于催化苯与乙烯的烷基化的催化剂的整体载体。催化剂可以选自例如沸石例如β沸石和MCM-22沸石，以及固定超酸。还公开了通过在包含整体式催化剂体系的烷基化反应器中将苯和乙烯的混合物烷基化来制备乙苯的方法，以包括浸渍或与合适的催化剂共成形的整料载体。在一个实施方案中，本发明提供了一种方便的方法来升级先前用于常规液相烷基化的现有反应器，例如由三氯化铝催化的那些。如果需要，本发明的烷基化方法可以在临界或接近临界条件下有效且有利地进行。

13. 发明申请

WO2006128374A1 一种改性 β 沸石审中-公开
公开(公告)号：WO2006128374A1
公开(公告)日：2006-12-07
申请号：PCT/CN2006/001164
申请日：2006-05-31
申请人：中国石油化工股份有限公司 , 中国石油化工股份有限公司石油化工科学研究院 , 罗一斌 , 达志坚 , 欧阳颖 , 庄立 , 龙军 , 舒兴田 , 宗保宁
发明人：罗一斌 , 达志坚 , 欧阳颖 , 庄立 , 龙军 , 舒兴田 , 宗保宁
IPC分类号： B01J29/064 , B01J29/076 , C10G11/05 , C01B39/02
CPC分类号： C01B39/10 , B01J29/7057 , B01J29/7615 , B01J29/7815 , B01J29/85 , B01J2229/18 , C01B39/06 , C10G11/05
摘要： The present invention provides a modified zeolite beta, which is characterized that anhydrous formula of the modified zeolite beta is expressed as (0~0.3)Na 2 O·(0.5~10)Al 2 O 3 ·(1.3-10)P 2 O 5 ·(0.7~15)M x O y ·(70~97)SiO 2 by the weight percent of oxide, wherein said transition metal M is one or more selected from the group consisting of Fe, Co, Ni, Cu, Mn, Zn and Sn, x represents the atomicity of said transition metal, y represents a number used to satisfy the oxidation state of said transition metal M. The modified zeolite beta may be used as an active component of cracking catalysts or aids in the petroleum hydrocarbon catalytic cracking.

14. 发明申请

WO2004033395A2 CRITICAL PHASE ALKYLATION PROCESS 审中-公开
标题翻译：临界相烷基化过程
公开(公告)号：WO2004033395A2
公开(公告)日：2004-04-22
申请号：PCT/US0330401
申请日：2003-09-25
申请人： FINA TECHNOLOGY
发明人： KELLY KEVIN P , BUTLER JAMES R
IPC分类号： C07C2/66 , C07C6/12 , C07C
CPC分类号： B01J29/90 , B01J29/7057 , B01J38/14 , C07C2/66 , C07C6/126 , C07C2529/08 , C07C2529/70 , Y02P20/584 , C07C15/073
摘要： A process for the production of ethylbenzene by the ethylation of benzene in the critical phase over a molecular sieve aromatic alkylation catalyst comprising cerium-promoted zeolite beta. An aromatic feedstock having a benzene content of at least 90 wt.% is supplied into a reaction zone and into contact with the cerium-promoted zeolite beta having a silica/alumina mole ratio within the range of 50-150 and a cerium-aluminum ratio of 0.5-1.5. Ethylene is supplied to the alkylation reaction zone in an amount to provide a benzene/ethylene mole ratio of 1-15. The reaction zone is operated at temperature and pressure conditions in which benzene is in the super critical phase to cause ethylation of the benzene in the presence of the cerium zeolite beta alkylation catalyst. An alkylation product is produced containing ethylbenzene as a primary product with the attendant production of heavier alkylated by-products of no more than 60 wt.% of the ethylbenzene. The critical phase alkylation reaction may be followed by the transalkylation of a polyalkylated aromatic component.
摘要翻译：通过在包含铈促进的沸石β的分子筛芳族烷基化催化剂上在临界相中苯的乙基化生产乙苯的方法。将苯含量至少为90重量％的芳族原料供入反应区并与二氧化硅/氧化铝摩尔比在50-150范围内的铈促进沸石β接触，并将铈铝比为0.5-1.5。将乙烯以提供1-15的苯/乙烯摩尔比的量供应到烷基化反应区。反应区在温度和压力条件下操作，其中苯处于超临界相中，以在铈沸石β烷基化催化剂存在下引起苯的乙基化。生产含有乙苯作为主要产品的烷基化产物，伴随地生产不超过60重量％乙苯的重质烷基化副产物。关键相烷基化反应之后可以是多烷基化芳族化合物的烷基转移。

15. 发明申请

WO03022430A2 HYDROTHERMALLY STABLE METAL PROMOTED ZEOLITE BETA FOR NOx REDUCTION 审中-公开
标题翻译：水热稳定的金属促进沸石BETA减少NOx
公开(公告)号：WO03022430A2
公开(公告)日：2003-03-20
申请号：PCT/US0226308
申请日：2002-08-16
申请人： ENGELHARD CORP
发明人： TRAN PASCALINE H , LIU XINSHENG , CHEN JAMES M
IPC分类号： B01D53/94 , B01D53/56 , B01D53/86 , B01J23/52 , B01J29/072 , B01J29/70 , B01J29/76 , B01J35/00 , B01J29/14
CPC分类号： B01J29/7615 , B01D53/8628 , B01J29/072 , B01J29/7057 , B01J35/002 , B01J2229/18 , B01J2229/24
摘要： The present invention is directed to an iron-promoted zeolite beta catalyst useful in the selective catalytic reduction nitrogen oxides with ammonia in which the iron-promoted zeolite beta is treated so as to provide increased amounts of the iron promoter in the form of Fe(OH). The stabilized zeolite is formed by cation exchange of an iron salt into a zeolite beta which has a reduced sodium content such as by exchanging a sodium beta with ammonium or hydrogen cations. A zeolite beta having a reduced carbon content and a Si/Al ratio of no more than 10 also increases the Fe(OH) content of the iron-promoted catalyst. The iron-promoted catalyst which has the iron in the form of Fe(OH) is characterized by a peak at 3680 +/- 5 cm in the IR spectra.
摘要翻译：本发明涉及用于选择性催化还原氮氧化物与氨的铁促进沸石β催化剂，其中铁促进沸石β被处理以提供更多量的Fe（OH））。通过将铁盐阳离子交换成具有降低的钠含量的沸石β，例如通过用铵或氢阳离子交换钠β来形成稳定的沸石。具有降低的碳含量和不超过10的Si / Al比的沸石β也增加了铁促进的催化剂的Fe（OH）含量。具有Fe（OH）形式的铁的铁促进的催化剂的特征在于在IR光谱中在3680 +/- 5cm-1处具有峰。

16. 发明申请

WO2016167698A1 CATALYSED BAEYER-VILLIGER OXIDATION OF CYCLIC KETONES 审中-公开
标题翻译：催化剂BAEYER-VILLIGER氧化循环克隆
公开(公告)号：WO2016167698A1
公开(公告)日：2016-10-20
申请号：PCT/SE2016/000009
申请日：2016-03-04
申请人： PERSTORP AB
发明人： PAJALIC, Oleg , LUNDMARK, Stefan
IPC分类号： C07D313/02 , B01J29/00 , C01B15/01 , C07B41/12
CPC分类号： C07D313/02 , B01J23/06 , B01J23/14 , B01J27/0573 , B01J29/061 , B01J29/7057
摘要： Disclosed is a catalysed Baeyer-Villiger oxidation of cyclic ketones yielding corresponding lactones. Hydrogen peroxide is used as oxidant and said oxidation is catalysed by a catalytically active amount of at least one catalyst comprising Sn, Se and/or Zn loaded in an amount of 0.1-1 mmol/g, calculated as elemental substance, on a carrier material. An azeotropic solvent, such as a non-polar solvent is optionally used.
摘要翻译：公开了催化的Baeyer-Villiger氧化产生相应内酯的环酮。过氧化氢用作氧化剂，所述氧化通过催化活性量的至少一种催化剂催化，所述催化剂包含以载体材料计的元素为0.1-1mmol / g的量的Sn，Se和/或Zn 。任选使用共沸溶剂，例如非极性溶剂。

17. 发明申请

WO2015193461A3 CRYSTALLINE MICROPOROUS MATERIAL MEDIATED CONVERSION OF C1-3 OXYGENATE COMPOUNDS TO C4- OXYGENATE COMPOUNDS 审中-公开
标题翻译： C 3-氧化物化合物向C4-氧化物化合物的晶体微结构材料介导的转化
公开(公告)号：WO2015193461A3
公开(公告)日：2016-08-11
申请号：PCT/EP2015063774
申请日：2015-06-18
申请人： HALDOR TOPSØE AS
发明人： SHUNMUGAVEL SARAVANAMURUGAN , SADABA ZUBIRI IRANTZU , TAARNING ESBEN , HOLM MARTIN SPANGSBERG
IPC分类号： C07H1/00 , B01J29/85 , B01J29/89 , C07H3/02
CPC分类号： C07H1/00 , A23L27/34 , A23L33/10 , A23V2002/00 , B01J29/041 , B01J29/405 , B01J29/7049 , B01J29/7057 , B01J29/89 , B01J37/0018 , B01J37/0201 , B01J37/04 , B01J37/10 , B01J2229/186 , B01J2229/37 , C01B37/005 , C01B39/026 , C01B39/085 , C01B39/40 , C01B39/46 , C07C51/16 , C07C67/08 , C07D307/36 , C07H3/02
摘要： A process for the preparation of C4 oxygenate compounds such as threose, erythrose or erythrulose starting from a composition comprising C1-3 oxygenate compounds such as formaldehyde, glycolaldehyde, glyoxal, pyruvaldehyde or acetol, wherein the process is carried out in the presence of a crystalline microporous materia! having a ring pore structure selected from an eight-membered ring pore structure or a ten-membered ring pore structure.
摘要翻译：一种从包含C1-3含氧化合物如甲醛，乙二醇醛，乙二醛，丙酮醛或丙酮醇的组合物开始制备C4含氧化合物如苏糖，赤藓糖或赤藓酮酸的方法，其中该方法在结晶微孔材料！具有选自八元环孔结构或十元环孔结构的环孔结构。

18. 发明申请

WO2016005391A1 ALKYLATION PROCESS USING A CATALYST COMPRISING CERIUM RICH RARE EARTH CONTAINING ZEOLITES AND A HYDROGENATION METAL 审中-公开
标题翻译：使用包含含稀土元素的含有沸石和氢化金属的催化剂的烷基化方法
公开(公告)号：WO2016005391A1
公开(公告)日：2016-01-14
申请号：PCT/EP2015/065481
申请日：2015-07-07
申请人： ALBEMARLE EUROPE SPRL
发明人： VAN BROEKHOVEN, Emanuel Hermanus , VAN LOEVEZIJN, Arnold , BAKKER, Richard Hendrik Marc
IPC分类号： C10G29/20 , B01J29/08 , C07C2/58 , B01J35/02 , B01J38/56 , B01J38/58 , B01J29/12 , B01J29/70 , B01J29/90
CPC分类号： B01J29/068 , B01J29/085 , B01J29/12 , B01J29/7057 , B01J29/7415 , C07C2/58 , C07C2529/068 , C10G29/205 , C10G2300/70 , C10G2400/02
摘要： An improved alkylation process utilizing a solid-acid catalyst comprising a cerium rich rare earth containing zeolite and a hydrogenation metal is disclosed.
摘要翻译：公开了利用包含富含铈的稀土类沸石和氢化金属的固体酸催化剂的改进的烷基化方法。

19. 发明申请

WO2015193461A2 CRYSTALLINE MICROPOROUS MATERIAL MEDIATED CONVERSION OF C1-3 OXYGENATE COMPOUNDS TO C4- OXYGENATE COMPOUNDS 审中-公开
标题翻译： C 3-氧化物化合物向C4-氧化物化合物的晶体微结构材料介导的转化
公开(公告)号：WO2015193461A2
公开(公告)日：2015-12-23
申请号：PCT/EP2015/063774
申请日：2015-06-18
申请人： HALDOR TOPSØE A/S
发明人： SHUNMUGAVEL, Saravanamurugan , SADABA ZUBIRI, Irantzu , TAARNING, Esben , HOLM, Martin, Spangsberg
CPC分类号： C07H1/00 , A23L27/34 , A23L33/10 , A23V2002/00 , B01J29/041 , B01J29/405 , B01J29/7049 , B01J29/7057 , B01J29/89 , B01J37/0018 , B01J37/0201 , B01J37/04 , B01J37/10 , B01J2229/186 , B01J2229/37 , C01B37/005 , C01B39/026 , C01B39/085 , C01B39/40 , C01B39/46 , C07C51/16 , C07C67/08 , C07D307/36 , C07H3/02
摘要： A process for the preparation of C 4 oxygenate compounds from a composition comprising C 1-3 oxygenate compounds, wherein the process is carried out in the presence of a crystalline microporous material comprising a small or medium-pore structure.
摘要翻译：一种由包含C 1-3含氧化合物的组合物制备C 4含氧化合物的方法，其中该方法在包含小孔或中孔结构的结晶微孔材料存在下进行。

20. 发明申请

WO2015072813A1 글리세린 탈수반응용 촉매, 이의 제조 방법 및 아크롤레인의 제조 방법 审中-公开
标题翻译：甘氨酸脱水催化剂，其制备方法及其制备方法
公开(公告)号：WO2015072813A1
公开(公告)日：2015-05-21
申请号：PCT/KR2014/011079
申请日：2014-11-18
申请人： 주식회사 엘지화학
发明人： 김지연 , 최준선 , 천주영 , 조왕래
IPC分类号： B01J29/072 , C07C29/76 , C07C47/22
CPC分类号： B01J29/46 , B01J27/053 , B01J27/055 , B01J29/072 , B01J29/40 , B01J29/405 , B01J29/42 , B01J29/7007 , B01J29/7057 , B01J29/7215 , B01J29/7615 , B01J35/0006 , B01J37/0036 , B01J37/04 , B01J2229/20 , C07C45/52 , C07C47/22
摘要： 본 발명은 글리세린 탈수반응용 촉매, 이의 제조 방법 및 아크롤레인의 제조 방법에 관한 것이다. 상기 글리세린 탈수반응용 촉매는 글리세린의 전환율이 높고, 부산물의 생성을 최소화하여 아크롤레인의 선택도를 개선할 수 있고, 반응 동안 촉매 활성을 높게 유지할 수 있다.
摘要翻译：本发明涉及一种甘油脱水用催化剂及其制备方法，以及丙烯醛的制备方法。用于甘油脱水的催化剂具有高甘油转化率，可以使副产物的产生最小化，从而提高丙烯醛的选择性，并且可以在反应期间保持高的催化活性。

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