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1. 发明授权

US06346581B1 Modified cycloolefin addition polymer and curable resin composition containing the same 失效
标题翻译：改性环烯加成聚合物和含有它们的固化性树脂组合物
公开(公告)号：US06346581B1
公开(公告)日：2002-02-12
申请号：US09463077
申请日：2000-01-18
申请人： Yasuo Tsunogae , Masahiro Ichinose , Yasuhiro Wakizaka
发明人： Yasuo Tsunogae , Masahiro Ichinose , Yasuhiro Wakizaka
IPC分类号： C08F27700
CPC分类号： C08J5/18 , C08F8/00 , C08F8/02 , C08F2800/10 , C08F2800/20 , C08F2810/20 , C08J2345/00 , C08J2351/00 , C08F232/08 , C08F210/02
摘要： A curable resin composition comprising a modified cycloolefin addition polymer (A) obtained by introducing a functional group into a cycloolefin addition polymer containing a repeating unit (a) derived from a cycloolefin monomer having an organic group having at least 4 carbon atoms at its side chain at a rate of introduction of the functional group of 0.1 to 50 mol % based on the whole repeating unit of the cycloolefin addition polymer, and a hardening agent (B), and a modified cycloolefin addition polymer (A) obtained by introducing a functional group into a cycloolefin addition polymer containing a repeating unit (a) derived from a cycloolefin monomer having an organic group having at least 4 carbon atoms at its side chain at a rate of introduction of the functional group of 0.1 to 50 mol % based on the whole repeating unit of the cycloolefin addition polymer, and having a weight average molecular weight (Mw) of 1,000 to 1,000,000.
摘要翻译：一种可固化树脂组合物，其包含通过将官能团引入到其侧链上含有具有至少4个碳原子的有机基团的环烯烃单体的重复单元（a）的环烯加成聚合物而获得的改性环烯加成聚合物（A）基于环烯烃加成聚合物的全部重复单元，官能团的引入率为0.1〜50摩尔％，固化剂（B）和通过引入官能团而得到的改性环烯烃加成聚合物（A）成为含有重复单元（a）的环烯烃加成聚合物，该重复单元（a）衍生自具有在侧链上具有至少4个碳原子的有机基团的环烯烃单体，其官能团的引入速率为0.1〜50摩尔％，基于整体环烯烃加成聚合物的重复单元，重均分子量（Mw）为1,000〜1,000,000。

2. 发明授权

US06713154B1 Insulating material containing cycloolefin polymer 失效
标题翻译：含环烯烃聚合物的绝缘材料
公开(公告)号：US06713154B1
公开(公告)日：2004-03-30
申请号：US09445310
申请日：1999-12-06
申请人： Yasuo Tsunogae , Yasuhiro Wakizaka , Junji Kodemura , Tohru Hosaka
发明人： Yasuo Tsunogae , Yasuhiro Wakizaka , Junji Kodemura , Tohru Hosaka
IPC分类号： B32B310
CPC分类号： B32B15/085 , B32B27/32 , B32B27/325 , B32B2307/204 , B32B2307/206 , B32B2307/306 , B32B2307/7265 , B32B2457/08 , H01B3/44 , H05K1/032 , Y10T428/24273 , Y10T428/24322 , Y10T428/3175
摘要： An insulating material comprising a cycloolefin polymer, specifically, an interlayer insulating material for a high-density assembly board having interlayer-connecting via holes at most 200 &mgr;m in diameter, comprising a cycloolefin polymer containing at least 50 mol % of a repeating unit derived from a cycloolefin monomer; a dry film formed from a curable resin composition comprising a polymer having a number average molecular weight within a range of 1,000 to 1,000,000 as measured by gel permeation chromatography, and a hardener; and a resin-attached metal foil obtained by forming a film of a cycloolefin polymer on one side of a metal foil. Laminates, multi-layer laminates and build-up multi-layer laminates making use of these materials, and production processes thereof.
摘要翻译：一种包含环烯烃聚合物的绝缘材料，特别是用于高密度组装板的层间绝缘材料，其具有直径最大为200μm的夹层连接通孔，其包含含有至少50mol％重复单元的环烯烃聚合物环烯烃单体; 由通过凝胶渗透色谱法测定的数均分子量在1,000〜1,000,000范围内的聚合物的固化性树脂组合物形成的干膜和硬化剂; 以及通过在金属箔的一面上形成环烯烃聚合物膜而获得的树脂附着金属箔。使用这些材料的层压板，多层层压板和堆积多层层压板及其制造方法。

3. 发明授权

US06730736B1 Alicyclyc structure-containing resin composition 有权
标题翻译：含有脂环结构的树脂组合物
公开(公告)号：US06730736B1
公开(公告)日：2004-05-04
申请号：US09647573
申请日：2000-10-02
申请人： Shojiro Kaita , Takashi Iga , Yasuhiro Wakizaka , Yasuo Tsunogae
发明人： Shojiro Kaita , Takashi Iga , Yasuhiro Wakizaka , Yasuo Tsunogae
IPC分类号： C08F25500
CPC分类号： C08F8/00 , C08L45/00 , C08F32/00 , C08L2666/02
摘要： An alicyclic structure-containing resin composition comprising an alicyclic structure-containing resin (A) having a polar group in a proportion of 3 to 50 mol % based on the whole repeating unit in the resin, and a soft polymer (B), a varnish containing the resin composition, a sheet formed of the resin composition, and an insulating film formed of the resin composition.
摘要翻译：含有脂环式结构的树脂组合物，其含有相对于树脂中的全部重复单元为3〜50摩尔％的极性基团的脂环式结构的树脂（A）和软质聚合物（B），清漆含有树脂组合物，由树脂组合物形成的片材和由树脂组合物形成的绝缘膜。

4. 发明授权

US07238405B2 Insulating material containing cycloolefin polymer 失效
标题翻译：含环烯烃聚合物的绝缘材料
公开(公告)号：US07238405B2
公开(公告)日：2007-07-03
申请号：US10772181
申请日：2004-02-04
申请人： Yasuo Tsunogae , Yasuhiro Wakizaka , Junji Kodemura , Tohru Hosaka
发明人： Yasuo Tsunogae , Yasuhiro Wakizaka , Junji Kodemura , Tohru Hosaka
IPC分类号： B32B27/00 , C08F8/00
CPC分类号： B32B15/085 , B32B27/32 , B32B27/325 , B32B2307/204 , B32B2307/206 , B32B2307/306 , B32B2307/7265 , B32B2457/08 , H01B3/44 , H05K1/032 , Y10T428/24273 , Y10T428/24322 , Y10T428/3175
摘要： An insulating material comprising a cycloolefin polymer, specifically, an interlayer insulating material for a high-density assembly board having interlayer-connecting via holes at most 200 μm in diameter, comprising a cycloolefin polymer containing at least 50 mol % of a repeating unit derived from a cycloolefin monomer; a dry film formed from a curable resin composition comprising a polymer having a number average molecular weight within a range of 1,000 to 1,000,000 as measured by gel permeation chromatography, and a hardener; and a resin-attached metal foil obtained by forming a film of a cycloolefin polymer on one side of a metal foil. Laminates, multi-layer laminates and build-up multi-layer laminates making use of these materials, and production processes thereof.
摘要翻译：一种包含环烯烃聚合物的绝缘材料，特别是用于高密度组装板的层间绝缘材料，其具有直径最大为200μm的夹层连接通孔，其包含含有至少50mol％重复单元的环烯烃聚合物环烯烃单体; 由通过凝胶渗透色谱法测定的数均分子量在1,000〜1,000,000范围内的聚合物的固化性树脂组合物形成的干膜和硬化剂; 以及通过在金属箔的一面上形成环烯烃聚合物膜而获得的树脂附着金属箔。使用这些材料的层压板，多层层压板和堆积多层层压板及其制造方法。

5. 发明授权

US06492443B1 Norbornene polymer composition 有权
标题翻译：降冰片烯聚合物组成
公开(公告)号：US06492443B1
公开(公告)日：2002-12-10
申请号：US09269964
申请日：1999-04-07
申请人： Junji Kodemura , Yasuo Tsunogae , Yasuhiro Wakizaka
发明人： Junji Kodemura , Yasuo Tsunogae , Yasuhiro Wakizaka
IPC分类号： C08K515
CPC分类号： C08L63/00 , C08G61/04 , C08L65/00 , C08L79/08 , H05K1/032 , C08L2666/22 , C08L2666/08 , C08L2666/16
摘要： A norbornene resin composition comprising 100 parts by weight of a thermoplastic norbornene polymer and 1 to 150 parts by weight of a thermosetting resin.
摘要翻译：一种降冰片烯树脂组合物，其包含100重量份的热塑性降冰片烯聚合物和1至150重量份的热固性树脂。

6. 发明申请

US20140005338A1 POLYMERIZABLE COMPOSITION, RESIN SHAPED ARTICLE, AND LAMINATE 审中-公开
标题翻译：可聚合组合物，树脂形状和层压材料
公开(公告)号：US20140005338A1
公开(公告)日：2014-01-02
申请号：US14003504
申请日：2012-03-08
申请人： Akihiko Yoshiwara , Yasuo Tsunogae
发明人： Akihiko Yoshiwara , Yasuo Tsunogae
IPC分类号： C08F232/08
CPC分类号： C08F232/08 , C08G61/08 , C08G2261/3325 , C08G2261/418
摘要： A polymerizable composition which contains a cycloolefin monomer and a ruthenium carbene complex which is expressed by the following general formula (I): (in which general formula (I), R1 and R2 respectively independently represent a hydrogen atom, halogen atom, or cyclic or chain C1 to C20 hydrocarbon group which may contain a halogen atom, oxygen atom, nitrogen atom, sulfur atom, phosphorus atom, or silicon atom; X1 and X2 respectively independently represent an anionic ligand; L1 and L2 respectively independently represent a neutral electron donor ligand; L2 is a group with a higher three-dimensionally bulk than L1, where L1 and L2 are at cis positions with each other; R1 and R2 may bond with each other to form an aliphatic ring or aromatic ring which may contain a hetero atom; and R1, R2, X1, X2, L1, and L2 may bond with each other in any combination to form a multidentate chelating ligand).
摘要翻译：含有由以下通式（I）表示的环烯烃单体和钌卡宾络合物的可聚合组合物（其中通式（I），R 1和R 2分别独立地表示氢原子，卤素原子或环状或可以含有卤素原子，氧原子，氮原子，硫原子，磷原子或硅原子的C1〜C20烃链; X1和X2分别独立地表示阴离子配体; L1和L2分别独立地表示中性给电子体配体 ; L2是具有比L1更高的三维体积的基团，其中L1和L2彼此是顺式位置; R1和R2可以彼此键合以形成可以含有杂原子的脂族环或芳香环; 并且R1，R2，X1，X2，L1和L2可以以任何组合彼此键合形成多齿螯合配体）。

7. 发明申请

US20090221750A1 Thermoplastic Resin, Method for Producing Same and Molding Material 审中-公开
标题翻译：热塑性树脂，其制造方法和成型材料
公开(公告)号：US20090221750A1
公开(公告)日：2009-09-03
申请号：US11886727
申请日：2006-03-20
申请人： Yasuo Tsunogae , Shigetaka Hayano , Atsushi Ishiguro
发明人： Yasuo Tsunogae , Shigetaka Hayano , Atsushi Ishiguro
IPC分类号： C08L51/06 , C08L53/00
CPC分类号： C08G81/021 , C08G61/06 , C08G61/08
摘要： A thermoplastic resin comprising a block copolymer or a graft copolymer possessing (A) a crystalline hydrogenated norbornene ring-opening polymer unit and (B) a non-crystalline polymer unit having a glass transition temperature of 40 to 300° C.; A method for producing thermoplastic resin comprising hydrogenating a block copolymer or a graft copolymer possessing a norbornene ring-opening polymer unit (C) and a polymer unit (D) which is converted into the above-mentioned non-crystalline polymer unit (B) after hydrogenation, in the presence of a hydrogenation catalyst; and a molding material comprising the thermoplastic resin are provided. The thermoplastic resin of the present invention excels in transparency, heat resistance, and mechanical strength.
摘要翻译：包含具有（A）结晶氢化降冰片烯开环聚合物单元的嵌段共聚物或接枝共聚物的热塑性树脂和（B）玻璃化转变温度为40〜300℃的非结晶性聚合物单元。一种制备热塑性树脂的方法，包括将具有降冰片烯开环聚合物单元（C）的嵌段共聚物或接枝共聚物和聚合物单元（D）氢化，所述聚合物单元（D）经过转化成上述非晶态聚合物单元（B）在氢化催化剂的存在下进行氢化; 并且提供包含热塑性树脂的成型材料。本发明的热塑性树脂的透明性，耐热性和机械强度优异。

8. 发明申请

US20090124769A1 Process for producing cycloolefin addition polymer, catalyst for addition polymerization of cycloolefin, and transition metal compound 有权
标题翻译：环烯加成聚合物的制造方法，环烯烃的加成聚合用催化剂和过渡金属化合物
公开(公告)号：US20090124769A1
公开(公告)日：2009-05-14
申请号：US12073704
申请日：2008-03-07
申请人： Kei Nishii , Sigetaka Hayano , Yasuo Tsunogae
发明人： Kei Nishii , Sigetaka Hayano , Yasuo Tsunogae
IPC分类号： C08F4/42 , C07F17/00 , C08F4/52
CPC分类号： C07F7/28 , C08F4/65912 , C08F4/6592 , C08F210/02 , Y10S526/943 , C08F232/00
摘要： A process for producing a cycloolefin addition polymer comprising addition-polymerizing a cycloolefin in the presence of a catalyst comprising a combination of a specific transition metal compound of Group 4 of the Periodic Table, with an organoaluminum oxy compound, and/or a compound capable of reacting with the Group 4 transition metal compound to form an ion pair. The specific group 4 transition metal compound preferably has a structure such that the group 4 transition metal is bonded to a cyclopentadienyl ring in an η1 mode. The above-mentioned catalyst exhibits high activity for both of addition homopolymerization of a cycloolefin and addition copolymerization of a cycloolefin with an α-olefin.
摘要翻译：一种制备环烯加成聚合物的方法，包括在包含周期表第4族的特定过渡金属化合物与有机铝氧化合物的组合的催化剂存在下，将环烯加成聚合，和/或能够与第4族过渡金属化合物反应形成离子对。特别的第4族过渡金属化合物优选具有使第4族过渡金属以eta1模式键合到环戊二烯基环上的结构。上述催化剂对于环烯烃的加成均聚和环烯烃与α-烯烃的加成共聚均显示出高活性。

9. 发明授权

US09045617B2 Ring-opening polymer of cyclopentene and method of production of same 有权
标题翻译：环戊烯的开环聚合物及其生产方法
公开(公告)号：US09045617B2
公开(公告)日：2015-06-02
申请号：US13521262
申请日：2011-01-14
申请人： Yasuo Tsunogae , Yoshihisa Takeyama
发明人： Yasuo Tsunogae , Yoshihisa Takeyama
IPC分类号： C08F232/04 , C08K3/04 , C08K3/36 , C08F4/78 , C08L7/00
CPC分类号： C08K3/04 , C08G2261/3321 , C08G2261/418 , C08K3/36 , C08L65/00
摘要： There is provided a ring-opening polymer of cyclopentene wherein a cis ratio of the cyclopentene-derived structural units is 30% or more, a weight average molecular weight (Mw) is 100,000 to 1,000,000, and a functional group containing a structure represented by the general formula (1) or (2) is included at an end of the polymer chain. —Y—H (1) (in the above general formula (1), Y represents an oxygen atom or a sulfur atom.) —NH-Q (2) (in the above general formula (2), Q represents a hydrogen atom or a hydrocarbon group or a silyl group which may have a substituent group.)
摘要翻译：提供环戊烯的开环聚合物，其中环戊烯衍生的结构单元的顺式比例为30％以上，重均分子量（Mw）为100,000〜1,000,000，以及含有由通式（1）或（2）包括在聚合物链的末端。 -Y-H（1）（在上述通式（1）中，Y表示氧原子或硫原子。）-NH-Q（2）（在上述通式（2）中，Q表示氢原子或可以具有取代基的烃基或甲硅烷基。）

10. 发明申请

US20090275719A1 Film Comprising Norbornene Compound Addition Polymer 有权
标题翻译：包含降冰片烯化合物加成聚合物的薄膜
公开(公告)号：US20090275719A1
公开(公告)日：2009-11-05
申请号：US12223324
申请日：2007-01-26
申请人： Atsushi Ishiguro , Yoshihisa Takeyama , Yasuo Tsunogae
发明人： Atsushi Ishiguro , Yoshihisa Takeyama , Yasuo Tsunogae
IPC分类号： C08F32/04
CPC分类号： C08J5/18 , B32B27/08 , B32B27/18 , B32B27/20 , B32B27/22 , B32B27/306 , B32B27/32 , B32B27/325 , B32B27/34 , B32B2255/10 , B32B2255/20 , B32B2307/202 , B32B2307/308 , B32B2307/40 , B32B2307/412 , B32B2307/714 , B32B2307/7242 , B32B2307/7265 , B32B2307/734 , B32B2457/202 , C08F232/08 , C08J2345/00 , Y10T428/10 , Y10T428/31938
摘要： [Problems] To provide a film comprising a norbornene (NB) compound addition polymer that is excellent in chemical resistance, optical properties and the like, has a high Tg, a low water absorption ratio and a low linear expansion coefficient, and is soluble in an ordinary solvent.[Means for Solving Problems] A film comprising a NB compound addition polymer essentially consisting of repeating units derived from NB compound monomers, wherein the addition polymer has a specific Mw and has a sum of the units (A1) and (A2) of 70% by mol or more based on the total units, wherein the molar number of each unit satisfies the following equations: 70/30≦[{(A1)+(A2)}/(B)]≦100 and 10/90≦(A1)/(A2)≦98/2, or the addition polymer has a specific Mw and Mn and essentially consists of the units (A1) and (B), wherein the molar number of each unit satisfies the following equation: 70/30≦[(A1)/(B)]≦98/2: (A1) a unit derived from a NB compound monomer (a1) consisting of carbon atoms and hydrogen atoms with all the carbon atoms being involved in constitution of a condensed ring skeleton; (A2) a unit derived from a monomer having a structure wherein a part of hydrogen atoms of the monomer (a1) is substituted with only a hydrocarbon group having 2 or less carbon atoms; and (B) a unit derived from a monomer having a structure wherein a part of hydrogen atoms of the monomer (a1) is substituted with only a functional group having 2 or less carbon atoms, or with only a functional group having 2 or less carbon atoms and a hydrocarbon group having 2 or less carbon atoms.
摘要翻译： [问题]为了提供具有耐化学性，光学特性等优异的降冰片烯（NB）化合物加成聚合物的膜，具有高Tg，低吸水率和低线膨胀系数，并且可溶于普通溶剂。解决问题的手段一种包含NB化合物加成聚合物的膜，其基本上由衍生自NB化合物单体的重复单元组成，其中加成聚合物具有特定的Mw，单元（A1）和（A2）之和为70％其中每个单位的摩尔数满足以下等式：70/30 <= [{（A1）+（A2）} /（B）] <= 100和10/90 < =（A1）/（A2）<= 98/2，或加成聚合物具有特定的Mw和Mn，并且基本上由单元（A1）和（B）组成，其中每个单元的摩尔数满足以下等式： 70/30 <= [（A1）/（B）] <= 98/2：（A1）衍生自由碳原子和氢原子构成的NB化合物单体（a1）的单元，其全部碳原子参与构成的稠环骨架; （A2）来自具有单体（a1）的一部分氢原子仅被碳原子数2以下的烃基取代的单体的单元，和（B）单体衍生自单体的单体，其中单体（a1）的一部分氢原子仅被碳原子数2以下的官能团取代，或者仅具有碳原子数为2以下的官能团原子和碳原子数为2以下的烃基。

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