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1. 发明授权

US06130266A Pre-expanded particles of propylene resin, process for preparing the same and flow-restricting device 失效
标题翻译：丙烯树脂的预发泡颗粒，其制备方法和流动限制装置
公开(公告)号：US06130266A
公开(公告)日：2000-10-10
申请号：US495329
申请日：2000-02-01
申请人： Tsuyoshi Mihayashi , Nobuhisa Ota , Naruhiko Akamatsu , Yutaka Yanagihara , Takeshi Satoh
发明人： Tsuyoshi Mihayashi , Nobuhisa Ota , Naruhiko Akamatsu , Yutaka Yanagihara , Takeshi Satoh
IPC分类号： C08J9/18 , C08L23/08 , C08L23/10 , C08J9/16 , C08J9/22
CPC分类号： C08J9/18 , C08L23/10 , C08J2203/06 , C08J2323/16 , C08L23/0876 , Y10S521/917
摘要： There is provided pre-expanded particles of a propylene resin having a high expansion ratio and excellent molding adhesion without using a volatile blowing agent or increasing an expansion pressure. The pre-expanded particles of a propylene resin are prepared by the process comprising dispersing resin particles comprising a propylene resin composition, which contains 100 parts by weight of (A) a random copolymer of ethylene and propylene having an ethylene content of 1.5 to 4.5% by weight and 0.001 to 10 parts by weight of (B) an alkali metal salt of a copolymer of ethylene and (meth)acrylic acid, into an aqueous dispersion medium in a pressure vessel to obtain a mixture, heating the mixture to an expansion temperature higher than a softening temperature of the resin particles, introducing an inorganic gas, and releasing the mixture into a lower atmosphere than the inner pressure of the pressure vessel; said mixture is expanded after a temperature of said mixture is maintained at a temperature region of not more than the expansion temperature to at least (the expansion temperature -1.degree. C.) for at least 30 minutes.
摘要翻译：在不使用挥发性发泡剂或增加膨胀压力的情况下，提供具有高膨胀率和优异的模制粘合性的丙烯树脂的预发泡颗粒。丙烯树脂的预发泡颗粒通过包括分散树脂颗粒的方法制备，所述树脂颗粒包含丙烯树脂组合物，其包含100重量份的（A）乙烯含量为1.5至4.5重量％的乙烯和丙烯的无规共聚物，和（B）乙烯与（甲基）丙烯酸的共聚物的碱金属盐0.001〜10重量份，在压力容器中的水分散介质中，得到混合物，将混合物加热至膨胀温度高于树脂颗粒的软化温度，引入无机气体，并将混合物释放到比压力容器的内部压力低的气氛中; 所述混合物在所述混合物的温度保持在不大于膨胀温度至少至（膨胀温度-1℃）的温度区域下膨胀至少30分钟。

2. 发明授权

US06273347B1 Pre-expanded particles of propylene resin, process for preparing the same and flow-restricting device 失效
标题翻译：丙烯树脂的预发泡颗粒，其制备方法和流动限制装置
公开(公告)号：US06273347B1
公开(公告)日：2001-08-14
申请号：US09642025
申请日：2000-08-21
申请人： Tsuyoshi Mihayashi , Nobuhisa Ota , Naruhiko Akamatsu , Yutaka Yanagihara , Takeshi Satoh
发明人： Tsuyoshi Mihayashi , Nobuhisa Ota , Naruhiko Akamatsu , Yutaka Yanagihara , Takeshi Satoh
IPC分类号： B05B130
CPC分类号： C08J9/18 , C08J2203/06 , C08J2323/16 , C08L23/0876 , C08L23/10 , Y10S521/917 , C08L2666/04
摘要： There is provided pre-expanded particles of a propylene resin having a high expansion ratio and excellent molding adhesion without using a volatile blowing agent or increasing an expansion pressure. The pre-expanded particles of a propylene resin are prepared by the process comprising dispersing resin particles comprising a propylene resin composition, which contains 100 parts by weight of (A) a random copolymer of ethylene and propylene having an ethylene content of 1.5 to 4.5% by weight and 0.001 to 10 parts by weight of (B) an alkali metal salt of a copolymer of ethylene and (meth)acrylic acid, into an aqueous dispersion medium in a pressure vessel to obtain a mixture, heating the mixture to an expansion temperature higher than a softening temperature of the resin particles, introducing an inorganic gas, and releasing the mixture into a lower atmosphere than the inner pressure of the pressure vessel; said mixture is expanded after a temperature of said mixture is maintained at a temperature region of not more than the expansion temperature to at least (the expansion temperature −1° C.) for at least 30 minutes.
摘要翻译：在不使用挥发性发泡剂或增加膨胀压力的情况下，提供具有高膨胀率和优异的模制粘合性的丙烯树脂的预发泡颗粒。丙烯树脂的预发泡颗粒通过包括分散树脂颗粒的方法制备，所述树脂颗粒包含丙烯树脂组合物，其包含100重量份的（A）乙烯含量为1.5至4.5重量％的乙烯和丙烯的无规共聚物，和（B）乙烯与（甲基）丙烯酸的共聚物的碱金属盐0.001〜10重量份，在压力容器中的水分散介质中，得到混合物，将混合物加热至膨胀温度高于树脂颗粒的软化温度，引入无机气体，并将混合物释放到比压力容器的内部压力低的气氛中; 所述混合物在所述混合物的温度保持在不大于膨胀温度至少至（膨胀温度-1℃）的温度区域下膨胀至少30分钟。

3. 发明授权

US06596782B1 Hydrous polyolefin resin composition, preexpanded particles produced therefrom, process for producing the same, and expanded molding 有权
标题翻译：含水聚烯烃树脂组合物，由其制备的预剥离颗粒，其制备方法和膨胀成型
公开(公告)号：US06596782B1
公开(公告)日：2003-07-22
申请号：US09155544
申请日：1998-09-25
申请人： Kenji Mogami , Tsuyoshi Mihayashi , Kyoichi Nakamura , Naruhiko Akamatsu
发明人： Kenji Mogami , Tsuyoshi Mihayashi , Kyoichi Nakamura , Naruhiko Akamatsu
IPC分类号： C08J916
CPC分类号： C08J9/18 , B29C44/3461 , C08J9/0061 , C08J2203/10 , C08J2323/02
摘要： A water-containing polyolefin resin composition containing a polyolefin resin and a hydrophilic polymer and having a water content of 1 to 50% by weight which is suitable for use in preparation of polyolefin resin pre-expanded particles, and pre-expanded particles of a polyolefin resin prepared by pre-expanding the water-containing polyolefin resin composition the particles having a an apparent expansion ratio of 5 to 60, a closed cell ratio of 80 to 100% and an average cell diameter of 50 to 500 &mgr;m. The pre-expanded particles can be prepared without using a volatile blowing agent by dispersing resin particles made of a polyolefin resin composition containing a polyolefin resin and a hydrophilic polymer into an aqueous dispersion medium in a closed vessel to form a dispersion, heating to a temperature not lower than the softening point of the polyolefin resin to produce water-containing resin particles having a water content of 1 to 50% by weight, and releasing the aqueous dispersion from the closed vessel into a lower pressure than the inner pressure of the closed vessel, thereby expanding the water-containing resin particles. When the releasing of the dispersion from the vessel is conducted after raising the inner pressure to 25 to 75 kg/cm2G by introducing nitrogen gas, air or an inorganic gas including them as a main component into the vessel, pre-expanded particles providing foams having good physical properties and a high expansion ratio are obtained.
摘要翻译：含有聚烯烃树脂和亲水性聚合物的水含量聚烯烃树脂组合物，其水含量为1-50重量％，其适用于制备聚烯烃树脂预发泡颗粒和聚烯烃预发泡颗粒通过将含水聚烯烃树脂组合物的表观膨胀率为5〜60，闭孔率为80〜100％，平均泡孔直径为50〜500μm的颗粒预膨胀而制备的树脂。可以通过将含有聚烯烃树脂和亲水性聚合物的聚烯烃树脂组合物制成的树脂颗粒分散在密闭容器中的水性分散介质中而不使用挥发性发泡剂来制备预发泡颗粒，以形成分散体，加热到温度不低于聚烯烃树脂的软化点，以产生水含量为1至50重量％的含水树脂颗粒，并将水分散体从密闭容器中释放到比密封容器的内部压力低的压力从而使含水树脂颗粒膨胀。当通过将氮气，空气或其中包含它们的无机气体作为主要成分将内部压力升高到25至75kg / cm2G之后进行容器的分散时，预发泡颗粒提供具有获得良好的物理性能和高膨胀率。

4. 发明授权

US06326409B1 In-mold foaming article of polypropylene resin composition 有权
标题翻译：聚丙烯树脂组合物的模内发泡制品
公开(公告)号：US06326409B1
公开(公告)日：2001-12-04
申请号：US09694264
申请日：2000-10-24
申请人： Tsuyoshi Mihayashi , Yutaka Yanagihara , Takayuki Goda
发明人： Tsuyoshi Mihayashi , Yutaka Yanagihara , Takayuki Goda
IPC分类号： C08J922
CPC分类号： C08J9/228 , C08J9/0061 , C08J9/18 , C08J2323/10 , C08L23/0876 , C08L23/10 , C08L2203/14 , C08L2666/04
摘要： The object of the present invention is to provide an in-mold foaming article of a propylene resin composition having improved productivity and stable quality in internal molding, and simultaneously a compressive strength and a tensile strength thereof at high density range are improved at the same time. The in-mold foaming article is obtained by using a pre-foamed particle having a density of 90 to 300 g/L and an open cell ratio of at most 12%, wherein the pre-foamed particle comprises a resin composition having (A) 100 parts by weight of a polypropylene resin and (B) 0.01 to 20 parts by weight of a hydrophilic polymer as a base material resin, and water as a foaming agent, the pre-foamed particle having at least two endothermic peaks in a DSC curve obtained in differential scanning calorimetry.
摘要翻译：本发明的目的是提供一种在内部成型中具有提高的生产率和稳定质量的丙烯树脂组合物的模内发泡制品，并同时提高在高密度范围内的抗压强度和抗拉强度。通过使用密度为90〜300g / L，开孔率为12％以下的预发泡粒子得到模内发泡体，其中，所述预发泡粒子包含具有（A）成分的树脂组合物， 100重量份的聚丙烯树脂和（B）0.01〜20重量份作为基材树脂的亲水性聚合物，作为发泡剂的水，预发泡颗粒在DSC曲线中具有至少两个吸热峰以差示扫描量热法获得。

5. 发明授权

US08057875B2 Resin composition for tubes and tube 有权
标题翻译：用于管和管的树脂组合物
公开(公告)号：US08057875B2
公开(公告)日：2011-11-15
申请号：US11720511
申请日：2005-12-01
申请人： Kenji Noda , Tsuyoshi Mihayashi , Kazumasa Ohara
发明人： Kenji Noda , Tsuyoshi Mihayashi , Kazumasa Ohara
IPC分类号： B29D22/00 , B29D23/00 , B32B1/08
CPC分类号： C08L53/02 , C08L31/00 , C08L53/00 , C08L53/005 , C08L53/025 , C08L75/06 , C08L2205/03 , Y10T428/1352 , Y10T428/139 , Y10T428/1393 , Y10T428/1397 , C08L2666/14 , C08L2666/02
摘要： The present invention has its object to provide a resin composition for tubes excellent in balance among wear resistance, flexibility, gas permeation resistance and low resilience (pliability). The object is accomplished by a resin composition for tubes which comprises an isobutylene block copolymer (A) constituted of a polymer block (a) derived from isobutylene as a main constituent and a polymer block (b) derived from a monomer component other than isobutylene as a main constituent, and a thermoplastic polyurethane resin (B).
摘要翻译：本发明的目的是提供一种耐磨性，柔软性，耐气体渗透性和低弹性（柔韧性）之间的平衡优异的管用树脂组合物。该目的是通过包含由异丁烯作为主要成分的聚合物嵌段（a）和异丁烯以外的单体成分得到的聚合物嵌段（b）构成的异丁烯系嵌段共聚物（A）主要成分和热塑性聚氨酯树脂（B）。

6. 发明授权

US07998124B2 Catheter tube and catheter comprising the tube 有权
标题翻译：导管和导管包括管
公开(公告)号：US07998124B2
公开(公告)日：2011-08-16
申请号：US12302736
申请日：2007-05-31
申请人： Kazumasa Ohara , Tsuyoshi Mihayashi
发明人： Kazumasa Ohara , Tsuyoshi Mihayashi
IPC分类号： A61M25/00
CPC分类号： C08L53/02 , A61L29/049 , C08F297/00 , C08L53/00 , C08L53/025 , C08L75/08 , C08L75/04 , C08L2666/02 , C08L2666/14
摘要： The present invention relates to provide a catheter tube having excellent insertability into the body, excellent operability and an excellent anti-thrombogenic property, and also provide a catheter having the tube. For the purpose, a catheter tube of the present invention comprises a mixture of an isobutylene block copolymer and a thermoplastic polyurethane resin, wherein the isobutylene block copolymer is composed of a polymer block mainly comprising isobutylene and a polymer block mainly comprising a monomeric component other than isobutylene; and a catheter using the tube.
摘要翻译：本发明涉及提供一种具有优异的插入性的导管，优异的可操作性和优异的抗血栓形成性，并且还提供具有该管的导管。为此，本发明的导管包含异丁烯嵌段共聚物和热塑性聚氨酯树脂的混合物，其中异丁烯嵌段共聚物由主要包含异丁烯的聚合物嵌段和主要包含除异丁烯以外的单体组分的聚合物嵌段组成异丁烯和使用该管的导管。

7. 发明授权

US08377352B2 Medical catheter tubes and process for production thereof 有权
标题翻译：医用导管及其生产方法
公开(公告)号：US08377352B2
公开(公告)日：2013-02-19
申请号：US13064493
申请日：2011-03-29
申请人： Satoshi Inamoto , Fumihiko Nakao , Mitsuharu Korogi , Tsuyoshi Mihayashi
发明人： Satoshi Inamoto , Fumihiko Nakao , Mitsuharu Korogi , Tsuyoshi Mihayashi
IPC分类号： B29C47/00
CPC分类号： A61M25/0009 , A61L29/041 , B29C47/0004 , B29C47/0026 , B29C47/0057 , B29C47/02 , B29C47/20 , B29C47/54 , B29C67/04 , B29K2027/18 , B29L2023/005 , B29L2031/7542 , C08L27/18
摘要： A medical catheter tube containing a tetrafluoroethylene polymer, which has a wall thickness of 0.1 mm or below and exhibits a tensile strength (S1) at 1.0 mm displacement of 5.0 N/mm or above; and a process for the production of medical catheter tubes, characterized by molding a composition both a tetrafluoroethylene polymer and a lubricant having high affinity for the polymer by paste extrusion. The invention provides thin-wall medical catheter tubes excellent in elongation resistance, kink resistance and internal cavity lubricity.
摘要翻译：一种含有四氟乙烯聚合物的医疗导管，其具有0.1mm或更小的壁厚，并且在1.0mm位移处的拉伸强度（S1）为5.0N / mm以上; 以及用于生产医用导管的方法，其特征在于通过糊料挤出成型具有对聚合物具有高亲和力的四氟乙烯聚合物和润滑剂的组合物。本发明提供了耐伸长性，扭结性和内腔润滑性优异的薄壁医用导管。

8. 发明申请

US20090234329A1 Medical Catheter Tubes and Process for Production Thereof 审中-公开
标题翻译：医疗导管及其生产工艺
公开(公告)号：US20090234329A1
公开(公告)日：2009-09-17
申请号：US12089708
申请日：2006-10-17
申请人： Satoshi Inamoto , Fumihiko Nakao , Mitsuharu Korogi , Tsuyoshi Mihayashi
发明人： Satoshi Inamoto , Fumihiko Nakao , Mitsuharu Korogi , Tsuyoshi Mihayashi
IPC分类号： A61M25/00 , B29D23/00
CPC分类号： A61M25/0009 , A61L29/041 , B29C48/0018 , B29C48/022 , B29C48/10 , B29C48/15 , B29C48/30 , B29C48/32 , B29C48/475 , B29C67/04 , B29K2027/18 , B29L2023/005 , B29L2031/7542 , C08L27/18
摘要： A medical catheter tube containing a tetrafluoroethylene polymer, which has a wall thickness of 0.1 mm or below and exhibits a tensile strength (S1) at 1.0 mm displacement of 5.0 N/mm or above; and a process for the production of medical catheter tubes, characterized by molding a composition both a tetrafluoroethylene polymer and a lubricant having high affinity for the polymer by paste extrusion. The invention provides thin-wall medical catheter tubes excellent in elongation resistance, kink resistance and internal cavity lubricity.
摘要翻译：一种含有四氟乙烯聚合物的医疗导管，其具有0.1mm或更小的壁厚，并且在1.0mm位移处的拉伸强度（S1）为5.0N / mm以上; 以及用于生产医用导管的方法，其特征在于通过糊料挤出成型具有对聚合物具有高亲和力的四氟乙烯聚合物和润滑剂的组合物。本发明提供了耐伸长性，扭结性和内腔润滑性优异的薄壁医用导管。

9. 发明申请

US20110180955A1 Medical catheter tubes and process for production thereof 有权
标题翻译：医用导管及其生产方法
公开(公告)号：US20110180955A1
公开(公告)日：2011-07-28
申请号：US13064493
申请日：2011-03-29
申请人： Satoshi Inamoto , Fumihiko Nakao , Mitsuharu Korogi , Tsuyoshi Mihayashi
发明人： Satoshi Inamoto , Fumihiko Nakao , Mitsuharu Korogi , Tsuyoshi Mihayashi
IPC分类号： B29C47/00
CPC分类号： A61M25/0009 , A61L29/041 , B29C47/0004 , B29C47/0026 , B29C47/0057 , B29C47/02 , B29C47/20 , B29C47/54 , B29C67/04 , B29K2027/18 , B29L2023/005 , B29L2031/7542 , C08L27/18
摘要： A medical catheter tube containing a tetrafluoroethylene polymer, which has a wall thickness of 0.1 mm or below and exhibits a tensile strength (S1) at 1.0 mm displacement of 5.0 N/mm or above; and a process for the production of medical catheter tubes, characterized by molding a composition both a tetrafluoroethylene polymer and a lubricant having high affinity for the polymer by paste extrusion. The invention provides thin-wall medical catheter tubes excellent in elongation resistance, kink resistance and internal cavity lubricity.
摘要翻译：一种含有四氟乙烯聚合物的医疗导管，其具有0.1mm或更小的壁厚，并具有5.0N / mm以上的1.0mm位移的拉伸强度（S1）; 以及用于生产医用导管的方法，其特征在于通过糊料挤出成型具有对聚合物具有高亲和力的四氟乙烯聚合物和润滑剂的组合物。本发明提供了耐伸长性，扭结性和内腔润滑性优异的薄壁医用导管。

10. 发明申请

US20090187162A1 Catheter Tube and Catheter Comprising the Tube 有权
标题翻译：导管和导管包括管
公开(公告)号：US20090187162A1
公开(公告)日：2009-07-23
申请号：US12302736
申请日：2007-05-31
申请人： Kazumasa Ohara , Tsuyoshi Mihayashi
发明人： Kazumasa Ohara , Tsuyoshi Mihayashi
IPC分类号： A61M25/00
CPC分类号： C08L53/02 , A61L29/049 , C08F297/00 , C08L53/00 , C08L53/025 , C08L75/08 , C08L75/04 , C08L2666/02 , C08L2666/14
摘要： The present invention relates to provide a catheter tube having excellent insertability into the body, excellent operability and an excellent anti-thrombogenic property, and also provide a catheter having the tube. For the purpose, a catheter tube of the present invention comprises a mixture of an isobutylene block copolymer and a thermoplastic polyurethane resin, wherein the isobutylene block copolymer is composed of a polymer block mainly comprising isobutylene and a polymer block mainly comprising a monomeric component other than isobutylene; and a catheter using the tube.
摘要翻译：本发明涉及提供一种具有优异的插入性的导管，优异的可操作性和优异的抗血栓形成性，并且还提供具有该管的导管。为此，本发明的导管包含异丁烯嵌段共聚物和热塑性聚氨酯树脂的混合物，其中异丁烯嵌段共聚物由主要包含异丁烯的聚合物嵌段和主要包含除异丁烯以外的单体组分的聚合物嵌段组成异丁烯和使用该管的导管。

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