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1. 发明申请

US20100087693A1 Integrated Oxygenate Conversion and Product Cracking 审中-公开
标题翻译：综合氧化转化和产品开裂
公开(公告)号：US20100087693A1
公开(公告)日：2010-04-08
申请号：US12633253
申请日：2009-12-08
申请人： Tom N. Kalnes , Robert B. James, JR. , Daniel H. Wei , Bryan K. Glover
发明人： Tom N. Kalnes , Robert B. James, JR. , Daniel H. Wei , Bryan K. Glover
IPC分类号： C07C1/00
CPC分类号： C10G11/16 , C07C1/20 , C07C1/24 , C07C4/06 , C10G3/42 , C10G3/57 , C10G11/14 , C10G2300/4081 , C10G2400/20 , C07C11/02
摘要： Improved processing of an oxygenate-containing feedstock for increased production or yield of light olefins. Such processing involves oxygenate conversion to olefins and subsequent cracking of heavier olefins wherein at least a portion of the products from each of the reactors is elevated in pressure, using a common compressor, prior to being routed to a common product fractionation and recovery section. In one particular embodiment, the cracked product gas can be treated to remove acid gas therefrom. In another embodiment, the olefin cracking reactor is a moving bed reactor.
摘要翻译：改进含氧化合物原料的加工，以提高轻质烯烃的生产或产率。这种处理涉及含氧化合物转化为烯烃并随后开裂较重的烯烃，其中使用普通的压缩机将来自每个反应器的产物的至少一部分在压力下升高，然后被送至共同的产物分馏和回收段。在一个具体实施方案中，可以处理裂化产物气体以从其中除去酸性气体。在另一个实施方案中，烯烃裂解反应器是移动床反应器。

2. 发明申请

US20100048965A1 Integrated Oxygenate Conversion and Product Cracking 审中-公开
公开(公告)号：US20100048965A1
公开(公告)日：2010-02-25
申请号：US12610108
申请日：2009-10-30
申请人： Tom N. Kalnes , Robert B. James, JR. , Daniel H. Wei , Bryan K. Glover
发明人： Tom N. Kalnes , Robert B. James, JR. , Daniel H. Wei , Bryan K. Glover
IPC分类号： C07C1/00
CPC分类号： C07C1/20 , C07C1/24 , C07C4/06 , C10G3/42 , C10G3/57 , C10G11/18 , C10G2400/20 , Y02P30/42 , Y02P30/48 , C07C11/02
摘要： Improved processing of an oxygenate-containing feedstock for increased production or yield of light olefins. Such processing involves oxygenate conversion to olefins and subsequent cracking of heavier olefins wherein at least a portion of the products from each of the reactors is elevated in pressure, using a common compressor, prior to being routed to a common product fractionation and recovery section. In one particular embodiment, the cracked product gas can be treated to remove acid gas therefrom. In another embodiment, the olefin cracking reactor is a moving bed reactor.

3. 发明授权

US07663012B2 Conversion of dimethylether to propylene using moving bed technology 有权
标题翻译：使用移动床技术将二甲醚转化为丙烯
公开(公告)号：US07663012B2
公开(公告)日：2010-02-16
申请号：US12115788
申请日：2008-05-06
申请人： Tom N. Kalnes , Daniel H. Wei , Bryan K. Glover
发明人： Tom N. Kalnes , Daniel H. Wei , Bryan K. Glover
IPC分类号： C07C1/00
CPC分类号： C07C1/20 , C07C2529/40 , C07C2529/85 , Y02P20/52 , C07C11/06
摘要： The average cycle propylene selectivity of an oxygenate to propylene (OTP) process using one or more fixed beds of a dual-function oxygenate conversion catalyst is substantially enhanced by the use of moving bed reactor technology in the hydrocarbon synthesis portion of the OTP flow scheme in lieu of fixed bed technology coupled with the selection of a catalyst on-stream cycle time of 200 hours or less. Those provisions hold the build-up of coke deposits on the catalyst to a level which does not substantially degrade dual-function catalyst activity, oxygenate conversion and propylene selectivity, thereby enabling maintenance of propylene average cycle yield at essentially start-of-cycle levels. The propylene average cycle yield improvement enabled by the present invention over that achieved by the fixed bed system of the prior art using the same or a similar catalyst system is of the order of about 1.5 to 5.5 wt-% or more.
摘要翻译：使用一种或多种双功能含氧化合物转化催化剂固定床的含氧化合物对丙烯（OTP）方法的平均循环丙烯选择性通过在OTP流动方案的烃合成部分中使用移动床反应器技术而显着增强固定床技术的替代加上选择催化剂在线循环时间为200小时以下。这些规定将催化剂上的焦炭沉积物积聚到不会显着降低双重功能催化剂活性，含氧化合物转化率和丙烯选择性的水平，从而在基本上循环水平的初始阶段维持丙烯平均循环产率。通过使用相同或相似的催化剂体系的现有技术的固定床系统实现的本发明的丙烯平均循环产率提高约为1.5至5.5重量％或更多。

4. 发明申请

US20080242910A1 Conversion of Dimethylether to Propylene using Moving Bed Technology 有权
标题翻译：使用移动床技术将二甲醚转化成丙烯
公开(公告)号：US20080242910A1
公开(公告)日：2008-10-02
申请号：US12115788
申请日：2008-05-06
申请人： Tom N. Kalnes , Daniel H. Wei , Bryan K. Glover
发明人： Tom N. Kalnes , Daniel H. Wei , Bryan K. Glover
IPC分类号： C07C1/20
CPC分类号： C07C1/20 , C07C2529/40 , C07C2529/85 , Y02P20/52 , C07C11/06
摘要： The average cycle propylene selectivity of an oxygenate to propylene (OTP) process using one or more fixed beds of a dual-function oxygenate conversion catalyst is substantially enhanced by the use of moving bed reactor technology in the hydrocarbon synthesis portion of the OTP flow scheme in lieu of fixed bed technology coupled with the selection of a catalyst on-stream cycle time of 200 hours or less. Those provisions hold the build-up of coke deposits on the catalyst to a level which does not substantially degrade dual-function catalyst activity, oxygenate conversion and propylene selectivity, thereby enabling maintenance of propylene average cycle yield at essentially start-of-cycle levels. The propylene average cycle yield improvement enabled by the present invention over that achieved by the fixed bed system of the prior art using the same or a similar catalyst system is of the order of about 1.5 to 5.5 wt-% or more.
摘要翻译：使用一种或多种双功能含氧化合物转化催化剂固定床的含氧化合物对丙烯（OTP）方法的平均循环丙烯选择性通过在OTP流动方案的烃合成部分中使用移动床反应器技术而显着增强固定床技术的替代加上选择催化剂在线循环时间为200小时以下。这些规定将催化剂上的焦炭沉积物积聚到不会显着降低双重功能催化剂活性，含氧化合物转化率和丙烯选择性的水平，从而在基本上循环水平的初始阶段维持丙烯平均循环产率。通过使用相同或相似的催化剂体系的现有技术的固定床系统实现的本发明的丙烯平均循环产率提高约为1.5至5.5重量％或更多。

5. 发明申请

US20100021357A1 Integrated Oxygenate Conversion and Product Cracking 有权
公开(公告)号：US20100021357A1
公开(公告)日：2010-01-28
申请号：US12571841
申请日：2009-10-01
申请人： Tom N. Kalnes , Robert B. James, JR. , Daniel H. Wei , Bryan K. Glover
发明人： Tom N. Kalnes , Robert B. James, JR. , Daniel H. Wei , Bryan K. Glover
IPC分类号： B01J19/00
CPC分类号： C07C1/20 , C07C1/24 , C07C4/06 , C10G3/42 , C10G3/57 , C10G11/18 , C10G2400/20 , Y02P30/42 , Y02P30/48 , C07C11/02
摘要： Improved processing of an oxygenate-containing feedstock for increased production or yield of light olefins. Such processing involves oxygenate conversion to olefins and subsequent cracking of heavier olefins wherein at least a portion of the products from each of the reactors is elevated in pressure, using a common compressor, prior to being routed to a common product fractionation and recovery section. In one particular embodiment, the cracked product gas can be treated to remove acid gas therefrom. In another embodiment, the olefin cracking reactor is a moving bed reactor.

6. 发明授权

US07405337B2 Conversion of oxygenate to propylene with selective hydrogen treatment of heavy olefin recycle stream 有权
标题翻译：通过选择性氢处理重质烯烃循环流将含氧化合物转化为丙烯
公开(公告)号：US07405337B2
公开(公告)日：2008-07-29
申请号：US10946605
申请日：2004-09-21
申请人： Tom N. Kalnes , Daniel H. Wei , Bryan K. Glover
发明人： Tom N. Kalnes , Daniel H. Wei , Bryan K. Glover
IPC分类号： C07C1/00
CPC分类号： C07C11/06 , C07C1/20 , C07C2529/40 , C07C2529/80 , C07C2529/85 , Y02P20/52 , Y02P20/582 , Y02P20/584
摘要： The average cycle propylene selectivity of an oxygenate to propylene (OTP) process using one or more fixed or moving beds of a dual-function oxygenate conversion catalyst with recycle of one or more C4+ olefin-rich fractions is substantially enhanced by the use of selective hydrotreating technology on these C4+ olefin-rich recycle streams to substantially eliminate detrimental coke precursors such as dienes and acetylenic hydrocarbons. This hydrotreating step helps hold the build-up of detrimental coke deposits on the catalyst to a level which does not substantially degrade dual-function catalyst activity, oxygenate conversion and propylene selectivity, thereby enabling a substantial improvement in propylene average cycle yield. The propylene average cycle yield improvement enabled by the present invention over that achieved by the prior art using the same or a similar catalyst system but without the use of the hydrotreating step on the C4+ olefin-rich recycle stream is of the order of about 1.5 to 5.5 wt-% or more.
摘要翻译：使用一种或多种双功能含氧化合物转化催化剂的固定或移动床与一种或多种富含C 4 O 5烯烃的级分的再循环，使含氧化合物与丙烯（OTP）方法的平均循环丙烯选择性通过使用选择性加氢处理技术在这些富含C 4 O 3的富烯烃循环物流上基本上消除了有害的焦炭前体如二烯和炔烃。该加氢处理步骤有助于将催化剂上的有害焦炭沉积物的积聚保持在基本上不降低双功能催化剂活性，含氧化合物转化率和丙烯选择性的水平，从而可以显着提高丙烯平均循环产率。本发明的丙烯平均循环产率提高超过现有技术使用相同或类似的催化剂体系实现的丙烯平均循环产率的改进，但不使用富含C 4 O 5的富烯烃循环的加氢处理步骤流量约为1.5〜5.5重量％以上。

7. 发明授权

US07371916B1 Conversion of an alcoholic oxygenate to propylene using moving bed technology and an etherification step 有权
标题翻译：使用移动床技术将醇类含氧化合物转化为丙烯和醚化步骤
公开(公告)号：US07371916B1
公开(公告)日：2008-05-13
申请号：US10943833
申请日：2004-09-16
申请人： Tom N. Kalnes , Daniel H. Wei , Bryan K. Glover
发明人： Tom N. Kalnes , Daniel H. Wei , Bryan K. Glover
IPC分类号： C07C1/00
CPC分类号： C07C11/06 , C07C1/20 , C07C2529/40 , C07C2529/85 , Y02P20/52 , Y02P20/584
摘要： The average propylene selectivity per on-stream cycle of an alcoholic oxygenate to propylene (OTP) process using one or more fixed beds of a dual-function oxygenate conversion catalyst is substantially enhanced by the use of a feed pretreatment step involving a catalytic etherification reaction, by switching to moving bed reactor technology in the olefin synthesis portion of the OTP flow scheme in lieu of fixed bed technology and by the selection of a catalyst on-stream cycle time of 300 hours or less. These provisions hold the build-up of coke deposits on the dual-function catalyst to a level which does not substantially degrade catalyst activity, oxygenate conversion and propylene selectivity, thereby enabling maintenance of propylene average cycle yield at essentially start-of-cycle levels. The propylene average cycle yield improvement enabled by the present invention over that achieved by the fixed bed system of the prior art using the same or a similar dual-function catalyst system is of the order of about 1.5 to 5.5 wt-% or more.
摘要翻译：通过使用包含催化醚化反应的进料预处理步骤，使用一种或多种双功能含氧化合物转化催化剂的固定床的酒精含氧化合物对丙烯（OTP）方法的每个流动循环的平均丙烯选择性大大提高，通过在OTP流动方案的烯烃合成部分中切换到移动床反应器技术来代替固定床技术，并且通过选择300小时以下的催化剂流动循环时间。这些规定将双功能催化剂上的焦炭沉积物积聚到基本上不会降低催化剂活性，含氧化合物转化率和丙烯选择性的水平，从而使得在基本上循环水平上维持丙烯平均循环产率。通过使用相同或相似的双功能催化剂体系的现有技术的固定床系统实现的本发明丙烯平均循环产率改进为约1.5至5.5重量％或更多。

8. 发明授权

US07371915B1 Conversion of oxygenate to propylene using moving bed technology 失效
标题翻译：使用移动床技术将含氧化合物转化为丙烯
公开(公告)号：US07371915B1
公开(公告)日：2008-05-13
申请号：US10876394
申请日：2004-06-25
申请人： Tom N. Kalnes , Daniel H. Wei , Bryan K. Glover
发明人： Tom N. Kalnes , Daniel H. Wei , Bryan K. Glover
IPC分类号： C07C1/00
CPC分类号： C07C1/20 , C07C2529/40 , C07C2529/85 , Y02P20/52 , Y02P20/584 , C07C11/06
摘要： The average cycle propylene selectivity of an oxygenate to propylene (OTP) process using one or more fixed beds of a dual-function oxygenate conversion catalyst is substantially enhanced by the use of moving bed reactor technology in the hydrocarbon synthesis portion of the OTP flow scheme in lieu of fixed bed technology coupled with the selection of a catalyst on-stream cycle time of 200 hours or less. Those provisions hold the build-up of coke deposits on the catalyst to a level which does not substantially degrade dual-function catalyst activity, oxygenate conversion and propylene selectivity, thereby enabling maintenance of propylene average cycle yield at essentially start-of-cycle levels. The propylene average cycle yield improvement enabled by the present invention over that achieved by the fixed bed system of the prior art using the same or a similar catalyst system is of the order of about 1.5 to 5.5 wt-% or more.
摘要翻译：使用一种或多种双功能含氧化合物转化催化剂固定床的含氧化合物对丙烯（OTP）方法的平均循环丙烯选择性通过在OTP流动方案的烃合成部分中使用移动床反应器技术而显着增强固定床技术的替代加上选择催化剂在线循环时间为200小时以下。这些规定将催化剂上的焦炭沉积物积聚到不会显着降低双重功能催化剂活性，含氧化合物转化率和丙烯选择性的水平，从而在基本上循环水平的初始阶段维持丙烯平均循环产率。通过使用相同或相似的催化剂体系的现有技术的固定床系统实现的本发明的丙烯平均循环产率提高约为1.5至5.5重量％或更多。

9. 发明授权

US08603399B2 Integrated oxygenate conversion and product cracking 有权
标题翻译：综合含氧化合物转化和产物开裂
公开(公告)号：US08603399B2
公开(公告)日：2013-12-10
申请号：US12571841
申请日：2009-10-01
申请人： Tom N. Kalnes , Robert B. James, Jr. , Daniel H. Wei , Bryan K. Glover
发明人： Tom N. Kalnes , Robert B. James, Jr. , Daniel H. Wei , Bryan K. Glover
IPC分类号： B01J8/18
CPC分类号： C07C1/20 , C07C1/24 , C07C4/06 , C10G3/42 , C10G3/57 , C10G11/18 , C10G2400/20 , Y02P30/42 , Y02P30/48 , C07C11/02
摘要： An improved processing system of an oxygenate-containing feedstock for increased production or yield of light olefins. Such processing involves oxygenate conversion to olefins and subsequent cracking of heavier olefins wherein at least a portion of the products from each of the reactors is elevated in pressure, using a common compressor, prior to being routed to a common product fractionation and recovery section. The system further comprises acid gas removal means to remove acid gases from the cracked product gas and that the olefin cracking reactor is a moving bed reactor.
摘要翻译：含氧化合物原料的改进处理系统，用于提高轻质烯烃的生产或产率。这种处理涉及含氧化合物转化为烯烃并随后开裂较重的烯烃，其中使用普通的压缩机将来自每个反应器的产物的至少一部分在压力下升高，然后被送至共同的产物分馏和回收段。该系统还包括从裂化产物气体除去酸性气体的酸性气体去除装置，并且烯烃裂解反应器是移动床反应器。

10. 发明授权

US07687671B2 Integrated oxygenate conversion and product cracking 有权
标题翻译：综合含氧化合物转化和产物开裂
公开(公告)号：US07687671B2
公开(公告)日：2010-03-30
申请号：US11293934
申请日：2005-12-05
申请人： Tom N. Kalnes , Robert B. James, Jr. , Daniel H. Wei , Bryan K. Glover
发明人： Tom N. Kalnes , Robert B. James, Jr. , Daniel H. Wei , Bryan K. Glover
IPC分类号： C07C1/00
CPC分类号： C07C1/20 , C07C1/24 , C07C4/06 , C10G3/42 , C10G3/57 , C10G11/18 , C10G2400/20 , Y02P30/42 , Y02P30/48 , C07C11/02
摘要： Improved processing of an oxygenate-containing feedstock for increased production or yield of light olefins. Such processing involves oxygenate conversion to olefins and subsequent cracking of heavier olefins wherein at least a portion of the products from each of the reactors is elevated in pressure, using a common compressor, prior to being routed to a common product fractionation and recovery section. In one particular embodiment, the cracked product gas can be treated to remove acid gas therefrom. In another embodiment, the olefin cracking reactor is a moving bed reactor.
摘要翻译：改进含氧化合物原料的加工，以提高轻质烯烃的生产或产率。这种处理涉及含氧化合物转化为烯烃并随后开裂较重的烯烃，其中使用普通的压缩机将来自每个反应器的产物的至少一部分在压力下升高，然后被送至共同的产物分馏和回收段。在一个具体实施方案中，可以处理裂化产物气体以从其中除去酸性气体。在另一个实施方案中，烯烃裂解反应器是移动床反应器。

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