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1. 发明授权

US5296428A Catalyst comprising MCM-36 and a hydrogenation/dehydrogenation component 失效
标题翻译：包含MCM-36和氢化/脱氢组分的催化剂
公开(公告)号：US5296428A
公开(公告)日：1994-03-22
申请号：US929070
申请日：1992-08-12
申请人： Thomas F. Degnan , Kathleen M. Keville , Charles T. Kresge , David O. Marler , Brenda H. Rose , Wieslaw J. Roth , Kenneth G. Simons, deceased , Hye K. C. Timken , James C. Vartuli
发明人： Thomas F. Degnan , Kathleen M. Keville , Charles T. Kresge , David O. Marler , Brenda H. Rose , Wieslaw J. Roth , Kenneth G. Simons, deceased , Hye K. C. Timken , James C. Vartuli
IPC分类号： B01J21/16 , B01J29/04 , C01B33/36 , C01B39/02 , B01J21/06
CPC分类号： B01J29/049 , C01B39/026
摘要： There is provided a catalyst comprising MCM-36 and a hydrogenation/dehydrogenation component. A particular example of such a catalyst comprises MCM-36, nickel and tungsten.
摘要翻译：提供了包含MCM-36和氢化/脱氢组分的催化剂。这种催化剂的具体实例包括MCM-36，镍和钨。

2. 发明授权

US5294330A Hydrocracking process with a catalyst comprising MCM-36 失效
标题翻译：含有MCM-36催化剂的加氢裂化工艺
公开(公告)号：US5294330A
公开(公告)日：1994-03-15
申请号：US929065
申请日：1992-08-12
申请人： Thomas F. Degnan , Kathleen M. Keville , Charles T. Kresge , David O. Marler , Brenda H. Rose , Wieslaw J. Roth , Hye Kyung C. Timken
发明人： Thomas F. Degnan , Kathleen M. Keville , Charles T. Kresge , David O. Marler , Brenda H. Rose , Wieslaw J. Roth , Hye Kyung C. Timken
IPC分类号： C10G47/16 , C10G47/00 , C10G47/12 , C10G47/20
CPC分类号： C10G47/16
摘要： There is provided a hydrocracking process with a catalyst comprising MCM-36.
摘要翻译：提供了含有MCM-36的催化剂的加氢裂化方法。

3. 发明授权

US5183561A Demetallation of hydrocarbon feedstocks with a synthetic mesoporous crystalline material 失效
标题翻译：用合成介孔结晶材料对烃原料进行脱金属化
公开(公告)号：US5183561A
公开(公告)日：1993-02-02
申请号：US734992
申请日：1991-07-24
申请人： Charles T. Kresge , Michael E. Leonowicz , Wieslaw J. Roth , James C. Vartuli , Kathleen M. Keville , Stuart S. Shih , Thomas F. Degnan , Francis G. Dwyer , Michael E. Landis
发明人： Charles T. Kresge , Michael E. Leonowicz , Wieslaw J. Roth , James C. Vartuli , Kathleen M. Keville , Stuart S. Shih , Thomas F. Degnan , Francis G. Dwyer , Michael E. Landis
IPC分类号： B01J29/06 , B01D53/86 , B01J20/02 , B01J29/03 , B01J29/04 , B01J29/40 , B01J29/70 , B01J29/82 , B01J29/83 , B01J29/85 , B01J37/00 , C01B37/00 , C01B37/02 , C01B37/08 , C01B39/00 , C10G11/05 , C10G45/08 , C10G45/12 , C10G47/16
CPC分类号： C10G45/12 , B01D53/8628 , B01J20/02 , B01J20/041 , B01J20/06 , B01J20/08 , B01J20/103 , B01J20/12 , B01J29/041 , B01J29/044 , B01J29/045 , B01J29/40 , B01J29/70 , B01J29/82 , B01J29/83 , B01J29/85 , C01B37/00 , C01B37/02 , C01B37/08 , C01B39/00 , C10G11/05 , C10G47/16 , B01J2229/26 , B01J2229/32 , B01J2229/34 , B01J2229/36 , B01J2229/40 , B01J2229/42 , B01J37/0009
摘要： There is provided a process for demetallizing hydrocarbon feedstocks, such as resids or shale oil. The process uses a catalyst comprising at least one hydrogenation metal, such as nickel and molybdenum, and an ultra-large pore oxide material. This ultra-large pore oxide material may have uniformly large pores, e.g., having a size of about 40 Angstroms in diameter.
摘要翻译：提供了一种使烃原料脱金属的方法，例如残油或页岩油。该方法使用包含至少一种氢化金属如镍和钼的催化剂和超大孔隙氧化物材料。这种超大孔隙氧化物材料可以具有均匀的大孔，例如具有约40埃直径的尺寸。

4. 发明授权

US5156828A Method for manufacturing synthetic mesoporous crystalline material 失效
标题翻译：制造合成介孔结晶材料的方法
公开(公告)号：US5156828A
公开(公告)日：1992-10-20
申请号：US732516
申请日：1991-07-18
申请人： Thomas F. Degnan , Ivy D. Johnson , Kathleen M. Keville
发明人： Thomas F. Degnan , Ivy D. Johnson , Kathleen M. Keville
IPC分类号： B01J29/04 , B01J29/70 , C01B37/00 , C01B37/02 , C01B39/00
CPC分类号： C01B37/02 , B01J29/04 , B01J29/70 , C01B37/00 , C01B39/00 , B01J2229/26 , B01J2229/36 , B01J2229/42
摘要： This invention relates to a method for synthesizing an ultra-large pore crystalline material and the use of such crystalline material as a sorbent and in catalytic conversion of organic and inorganic compounds. The synthesis method includes hydrothermally treating the as-synthesized crystalline material in the presence or absence of a binder. In a preferred embodiment, the crystalline material contains organic directing agent and is composited in an alumina binder. The crystalline material exhibits unusually large sorption capacity demonstrated by its benzene adsorption capacity of greater than about 15 grams benzene/100 grams at 50 torr and 25.degree. C., a hexagonal electron diffraction pattern that can be indexed with a d.sub.100 value greater than about 18 Angstrom Units and a hexagonal arrangement of uniformly sized pores with a maximum perpendicular cross section of at least about 13 Angstrom units.
摘要翻译：本发明涉及一种用于合成超大孔结晶材料的方法以及这种结晶材料作为吸附剂的用途以及催化转化有机和无机化合物。合成方法包括在存在或不存在粘合剂的情况下水解处理合成的结晶材料。在优选的实施方案中，结晶材料含有有机导向剂并且在氧化铝粘合剂中复合。结晶物质表现出非常大的吸附能力，其吸附能力在50托和25℃时苯吸附能力大于约15克/ 100克，六方形电子衍射图可用d100值大于约18 埃单位和具有至少约13埃单位的最大垂直截面的均匀尺寸孔的六边形排列。

5. 发明授权

US5536894A MCM-56 as sorbent and catalyst component 失效
标题翻译： MCM-56作为吸附剂和催化剂组分
公开(公告)号：US5536894A
公开(公告)日：1996-07-16
申请号：US266082
申请日：1994-06-27
申请人： Thomas F. Degnan , Anthony S. Fung , Terry E. Helton , Stephen L. Lawton , Daria N. Lissy , Wieslaw J. Roth
发明人： Thomas F. Degnan , Anthony S. Fung , Terry E. Helton , Stephen L. Lawton , Daria N. Lissy , Wieslaw J. Roth
IPC分类号： B01J20/18 , B01J29/03 , B01J29/06 , B01J29/40 , B01J29/70 , C01B33/38 , C01B35/00 , C01B39/00 , C01B39/02 , C01B39/48 , C07C2/66 , C07C15/02 , C10G35/06 , C10G35/095 , C07C2/56 , C07C4/02 , C07C7/12
CPC分类号： B01J29/70 , B01J37/0009 , C01B33/38 , B01J2229/42
摘要： This invention relates to use of synthetic layered material MCM-56 as a sorbent and as a catalyst component in catalytic conversion of organic compounds. Examples of sorbent use include rapid sorption of hydrocarbons and separating at least one hydrocarbon component from a mixture of hydrocarbon components having differential sorption characteristics with respect to MCM-56. Examples of catalytic use include acid catalyzed reactions, such as cracking, aromatic compound alkylation, and isoalkane alkylation.
摘要翻译：本发明涉及合成层状材料MCM-56作为吸附剂和作为有机化合物催化转化的催化剂组分的用途。吸附剂使用的实例包括快速吸附烃并从相对于MCM-56的差异吸附特性的烃组分的混合物中分离至少一种烃组分。催化用途的实例包括酸催化反应，例如裂解，芳族化合物烷基化和异烷烃烷基化。

6. 发明授权

US5001295A Process for preparing dialkylnaphthalene 失效
标题翻译：制备二烷基萘的方法
公开(公告)号：US5001295A
公开(公告)日：1991-03-19
申请号：US494203
申请日：1990-03-15
申请人： Philip J. Angevine , Thomas F. Degnan , David O. Marler
发明人： Philip J. Angevine , Thomas F. Degnan , David O. Marler
IPC分类号： B01J29/04 , C07C2/12
CPC分类号： C07C2/12 , B01J29/04 , C07C2529/70
摘要： A catalytic process is provided for the preparation of dialkylnaphthalenes by alkylating a 2-alkylnaphthalene with an alkylating agent having an aliphatic group of from one to five carbon atoms, such as methanol. The catalyst comprises a synthetic zeolite characterized by an X-ray diffraction pattern including interplanar d-spacings at 12.36.+-.0.4, 11.03.+-.0.2, 8.83.+-.0.14, 6.18.+-.0.12, 6.00.+-.0.10, 4.06.+-.0.07, 3.91.+-.0.07 and 3.42.+-.0.06 Angstroms.
摘要翻译：提供了通过用具有1至5个碳原子的脂族基团如甲醇的烷基化烷基化2-烷基萘来制备二烷基萘的催化方法。该催化剂包括合成沸石，其特征在于X射线衍射图包括在12.36 +/- 0.4,11.03 +/- 0.2,8.83±0.14,6.18±0.12,6.00±0.10， 4.06 +/- 0.07,3.91 +/- 0.07和3.42 +/- 0.06埃。

7. 发明授权

US4895638A Catalytic cracking process 失效
标题翻译：催化裂化过程
公开(公告)号：US4895638A
公开(公告)日：1990-01-23
申请号：US339284
申请日：1989-04-17
申请人： Brent A. Aufdembrink , Thomas F. Degnan , Charles T. Kresge
发明人： Brent A. Aufdembrink , Thomas F. Degnan , Charles T. Kresge
IPC分类号： C10G11/04 , C10G11/05
CPC分类号： C10G11/04 , C10G11/05
摘要： A process for the catalytic cracking of heavy petroleum fractions into lower hydrocarbons, such as fuel products. The process comprises contacting the petroleum fractions at an elevated temperature with a cracking catalyst comprising (a) a layered metal oxide of the titanometallate type intercalated with an interspathic polymeric chalcogenide, e.g., polymeric silica and, optionally (b) a porous crystalline silicate component such as a large pore zeolite material.
摘要翻译：将重质石油馏分催化裂化成低级烃，如燃料产品的方法。该方法包括在升高的温度下使石油馏分与裂解催化剂接触，所述裂化催化剂包含（a）层状金属氧化物，金属螯合物层状金属氧化物，其插入有间位聚合硫属化物，例如聚合二氧化硅，和任选地（b）多孔结晶硅酸盐组分，作为大孔沸石材料。

8. 发明授权

US5358628A Production of high viscosity index lubricants 失效
标题翻译：生产高粘度指数润滑剂
公开(公告)号：US5358628A
公开(公告)日：1994-10-25
申请号：US898615
申请日：1992-06-15
申请人： Minas R. Apelian , Charles L. Baker, Jr. , Thomas F. Degnan , David O. Marler , Dominick N. Mazzone , Dennis E. Walsh
发明人： Minas R. Apelian , Charles L. Baker, Jr. , Thomas F. Degnan , David O. Marler , Dominick N. Mazzone , Dennis E. Walsh
IPC分类号： B01J29/18 , B01J29/70 , B01J29/74 , C10G45/64 , C10G49/12 , C10G65/12 , C10G69/02
CPC分类号： B01J29/7415 , B01J29/18 , B01J29/7007 , C10G65/12 , B01J2229/36 , B01J2229/37 , C10G2400/10
摘要： Petroleum wax feeds are converted to high Viscosity Index lubricants by a two-step hydrocracking-hydroisomerization process in which the wax feed is initially subjected to hydrocracking under mild conditions with a conversion to non-lube range products of no more than about 30 weight percent of the feed. The hydrocracking is carried out at a hydrogen pressure of at least 1000 psig using an amorphous catalyst which preferentially removes the aromatic components present in the initial feed. The hydrocracked effluent is then subjected to hydroisomerization in a second step using a low acidity dicarboxylic acid-treated zeolite Beta or mordenite catalyst which effects a preferential isomerization on the paraffin components to less waxy, high V.I. isoparaffins. The second stage may be operated at high pressure by cascading the first stage product into the second stage or at a lower pressure, typically from 200 to 1000 psig. The second stage catalyst is preferably a noble metal containing zeolite Beta catalyst which is treated with oxalic acid to give a low Alpha Value, typically below 10. The second stage is carried out at relatively low temperature, typically from 600.degree. to 650.degree. F. with a 650.degree. F.+ conversion in the range of 10 to 20 weight percent of the second stage feed but with high selectivity for isomerization of the paraffins. A final dewaxing step to target pour point may be used with relatively low loss, typically no more than 15 weight percent, during this dewaxing. The final products typically have V.I. values in excess of 130 and usually in the range of 140 to 155 and are characterized by exceptional stability.
摘要翻译：石油蜡进料通过两步加氢裂化加氢异构化方法转化为高粘度指数润滑剂，其中蜡进料最初在温和条件下进行加氢裂化，转化为非润滑范围产物的不超过约30重量％饲料。加氢裂化在至少1000psig的氢气压力下进行，使用优选除去初始进料中存在的芳族组分的无定形催化剂。然后使用低酸度二羧酸处理的沸石β-或丝光沸石催化剂，将加氢裂化的流出物在第二步骤中进行加氢异构化，其对石蜡组分进行优先异构化，以降低蜡，高V.I。异链烷烃第二阶段可以通过将第一阶段产品级联到第二阶段或通常为200至1000psig的较低压力下在高压下操作。第二阶段催化剂优选是含贵金属的沸石β催化剂，其用草酸处理以得到低α值，通常低于10。第二阶段在相对较低的温度下进行，通常为600至650°F。 +转化率在第二阶段进料的10至20重量％的范围内，但对于链烷烃的异构化具有高选择性。在该脱蜡过程中，目标倾点的最终脱蜡步骤可以使用相当低的损失，通常不超过15重量％。最终产品通常有V.I. 值超过130，通常在140至155的范围内，并且具有出色的稳定性。

9. 发明授权

US5013422A Catalytic hydrocracking process 失效
标题翻译：催化加氢裂化工艺
公开(公告)号：US5013422A
公开(公告)日：1991-05-07
申请号：US479790
申请日：1990-02-14
申请人： Robert P. L. Absil , Thomas F. Degnan , Scott Han , David O. Marler , Richard F. Socha , Michael R. Stapleton
发明人： Robert P. L. Absil , Thomas F. Degnan , Scott Han , David O. Marler , Richard F. Socha , Michael R. Stapleton
IPC分类号： B01J29/04 , B01J29/14 , B01J29/16 , B01J29/70 , B01J29/74 , B01J29/80 , C07C2/12 , C10G47/16 , C10G65/10 , C10G65/12
CPC分类号： B01J29/7038 , B01J29/04 , B01J29/146 , B01J29/166 , B01J29/7088 , B01J29/7415 , B01J29/7815 , B01J29/7876 , B01J29/80 , B01J29/86 , C07C2/12 , C10G47/16 , C10G65/10 , C10G65/12 , B01J2229/16 , B01J2229/26 , B01J2229/42 , C07C2529/70
摘要： A hydrocracking process is provided comprising contacting a hydrocarbon stream under hydrocracking conditions and in the presence of hydrogen with a catalyst composition which comprises a synthetic porous crystalline zeolite having a particular X-ray diffraction pattern. An embodiment of the invention provides a process for reducing the pour point of a waxy component-containing hydrocarbon oil by hydrocracking and dewaxing. Another embodiment of the invention provides a dual-stage hydrocracking process to produce premium gasoline and distillate boiling range products.
摘要翻译：提供加氢裂化方法，包括在加氢裂化条件下和氢存在下使烃流与包含具有特定X射线衍射图的合成多孔结晶沸石的催化剂组合物接触。本发明的一个实施方案提供了通过加氢裂化和脱蜡来降低含蜡组分的烃油的倾点的方法。本发明的另一个实施方案提供了一种双级加氢裂化方法，用于生产高级汽油和馏出物沸点产物。

10. 发明授权

US4982040A Process for the catalytic disproportionation of methylnaphthalenes 失效
标题翻译：甲基萘催化歧化过程
公开(公告)号：US4982040A
公开(公告)日：1991-01-01
申请号：US454481
申请日：1989-12-21
申请人： Philip J. Angevine , Thomas F. Degnan , David O. Marler
发明人： Philip J. Angevine , Thomas F. Degnan , David O. Marler
IPC分类号： B01J29/86 , B01J29/04 , B01J29/70 , C07B61/00 , C07C2/12 , C07C6/12 , C07C15/24
CPC分类号： C07C6/123 , B01J29/04 , C07C2/12 , C07C2529/06 , C07C2529/70
摘要： A methylnaphthalene such as 2-methylnaphthalene undergoes catalytic disproportionation to naphthalene and a mixture of dimethylnaphthalene isomers, preferably containing substantial quantities of 2,6-dimethylnaphthalene, employing catalyst comprising zeolite characterized by an X-ray diffraction pattern including interplanar d-spacings at 12.36.+-.0.4, 11.03.+-.0.2, 8.83.+-.0.14, 6.18.+-.0.12, 6.00.+-.0.10, 4.06.+-.0.07, 3.91.+-.0.07 and 3.42.+-.0.06 Angstroms.
摘要翻译：使用包含沸石的催化剂，其特征在于X射线衍射图包括12.36+的平面d间距，甲基萘如2-甲基萘经历催化歧化萘和二甲基萘异构体的混合物，优选含有大量的2,6-二甲基萘， /-0.4,11.03 +/- 0.2,8.83±0.14 6.18 +/- 0.12,6.00 +/- 0.10,4.06 +/- 0.07,3.91 +/- 0.07和3.42 +/- 0.06埃。

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