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1. 发明申请

US20050158577A1 Organic electroluminescent element and lumiscent device or display including the same 有权
标题翻译：有机电致发光元件和包含其的发光器件或显示器
公开(公告)号：US20050158577A1
公开(公告)日：2005-07-21
申请号：US10487584
申请日：2003-06-25
申请人： Tadashi Ishibashi , Mari Ichimura , Shinichiro Tamura , Naoyuki Ueda
发明人： Tadashi Ishibashi , Mari Ichimura , Shinichiro Tamura , Naoyuki Ueda
IPC分类号： H01L51/50 , C09K11/06 , H01L51/00 , H01L51/30 , H05B33/12
CPC分类号： H01L51/0054 , C09K11/06 , C09K2211/1003 , C09K2211/1007 , C09K2211/1011 , C09K2211/1014 , C09K2211/1029 , H01L51/0052 , H01L51/006 , H01L51/0081 , H01L51/5012 , H01L51/5048 , Y10S428/917
摘要： The present invention provides an organic electroluminescent element which is superior in luminance, reliability, and thermal stability and is capable of selectively emitting light with comparative long wavelengths such as red and good color purity and a light-emitting device or display device incorporated therewith. The organic electroluminescent element consists of a glass substrate (1), an anode (2), a hole transporting layer (10), an emitting layer (11), an electron transporting layer (12), and a cathode (3), which are sequentially laminated on top of the other. The emitting layer (11) is formed from a mixture composed of at least one species of the styryl compound represented by the general formula [I] below and a material with charge transporting capability. Y—CH═CH—X General formula [I](where X denotes an aryl group (such as phenyl group) which has a substituent group (such as cyano group and methyl group), and Y denotes a group having a skeleton of aminophenyl group or the like.)
摘要翻译：本发明提供了一种有优异的亮度，可靠性和热稳定性的有机电致发光元件，并且能够选择性地发射具有比较长的波长（例如红色和良好的色纯度）的光以及与其结合的发光器件或显示装置。有机电致发光元件由玻璃基板（1），阳极（2），空穴传输层（10），发光层（11），电子传输层（12）和阴极（3）组成，顺序层压在另一个之上。发光层（11）由由下述通式[I]表示的至少一种苯乙烯基化合物和具有电荷输送能力的材料构成的混合物形成。 <？in-line-formula description =“In-line Formulas”end =“lead”？> Y-CH-CH-X通用公式[I] <？in-line-formula description =“In-line Formulas”end =“尾”→（其中X表示具有取代基（例如氰基和甲基）的芳基（例如苯基），Y表示具有氨基苯基的骨架等的基团。

2. 发明授权

US06800382B2 Organic electroluminescent device 失效
标题翻译：有机电致发光器件
公开(公告)号：US06800382B2
公开(公告)日：2004-10-05
申请号：US10281583
申请日：2002-10-28
申请人： Tadashi Ishibashi , Mari Ichimura , Shinichiro Tamura
发明人： Tadashi Ishibashi , Mari Ichimura , Shinichiro Tamura
IPC分类号： H05B3314
CPC分类号： H01L51/0059 , H01L51/0052 , H01L51/006 , H01L51/0081 , H01L51/5012 , H01L51/5048 , H01L2251/308 , H01L2251/5315 , Y10S428/917
摘要： An organic electroluminescent device comprises an organic layer 5, 5a or 5b having a luminescent region and provided between an anode 2 and a cathode 3. The organic layer contains at least one distyryl compound represented by the following general formula (1). General formula (1): wherein R1 and R2 are, respectively, groups which may be the same or different and independently represent an aryl group of the following general formula (2). General formula (2) in which R4 to R8 may be the same or different and, respectively, represent a hydrogen atom, or at least one of them is a specified group such as a methoxy group, R3 represents a hydrogen atom or a specified group, and X represents a substituted or unsubstituted aryl group or hydrocarbon ring group.
摘要翻译：有机电致发光器件包括具有发光区域并且设置在阳极2和阴极3之间的有机层5,5a或5b。有机层含有至少一种由以下通式（1）表示的二苯乙烯基化合物。通式（ 1）：其中R 1和R 2分别是可以相同或不同并且独立地表示以下通式（2）的芳基的基团。其中R 4与R <8>可以相同或不同，分别表示氢原子，或者它们中的至少一个是指定的基团，例如甲氧基，R 3表示氢原子或指定的基团，X表示取代或未取代的芳基或烃环基。

3. 发明授权

US06790974B2 Bis(aminostyryl) naphthalene compound, synthesis intermediate thereof, and process for production thereof 有权
标题翻译：双（氨基苯乙烯基）萘化合物，其合成中间体及其制备方法
公开(公告)号：US06790974B2
公开(公告)日：2004-09-14
申请号：US10389787
申请日：2003-03-17
申请人： Mari Ichimura , Tadashi Ishibashi , Shinichiro Tamura
发明人： Mari Ichimura , Tadashi Ishibashi , Shinichiro Tamura
IPC分类号： C07C940
CPC分类号： H01L51/006 , C07C211/50 , C07C211/54 , C07C211/58 , C07C211/60 , C07C217/88 , C07C217/92 , C07C255/58 , C07C2601/14 , C07C2602/28 , C07F9/4025 , C07F9/5456 , G03G5/0614 , G03G5/0672 , H01L51/5048 , Y10T428/31678
摘要： A bis(aminostyryl)naphthalene compound represented by the general formula [I] or the like below. General Formula [I] (where R2 and R3 each denotes an unsubstituted aryl group; R1 and R4 each denotes an aryl group having a specific substituent such as methoxy group; and R5 and R6 each denotes a cyano group or the like.) A process for producing a bis(aminostyryl)naphthalene compound represented by the general formula [I] by condensation of, for example, 4-(N,N-diarylamino)benzaldehyde with diphosphonic ester or diphosphonium. The bis(aminostyryl)naphthalene compound emits intense yellow or red light. The process permits efficient production of the bis(aminostyryl)naphthalene compound.
摘要翻译：通式[I]等表示的双（氨基苯乙烯基）萘化合物等。通式[I]（其中R 2和R 3各自表示未取代的芳基; R 1， 4>表示具有特定取代基的芳基，例如甲氧基; R 5和R 6各自表示氰基等。）一种制备由下式表示的双（氨基苯乙烯基）萘化合物的方法：通式[I]通过例如4-（N，N-二芳基氨基）苯甲醛与二膦酸酯或二鏻的缩合。双（氨基苯乙烯基）萘化合物发射强烈的黄色或红色光。该方法允许有效生产双（氨基苯乙烯基）萘化合物。

4. 发明授权

US06765108B2 Bis (aminostyryl) naphthalene compound, synthesis intermediate thereof, and process for production thereof 有权
标题翻译：双（氨基苯乙烯基）萘化合物，其合成中间体及其制备方法
公开(公告)号：US06765108B2
公开(公告)日：2004-07-20
申请号：US10390381
申请日：2003-03-17
申请人： Mari Ichimura , Tadashi Ishibashi , Shinichiro Tamura
发明人： Mari Ichimura , Tadashi Ishibashi , Shinichiro Tamura
IPC分类号： C07C25550
CPC分类号： H01L51/006 , C07C211/50 , C07C211/54 , C07C211/58 , C07C211/60 , C07C217/88 , C07C217/92 , C07C255/58 , C07C2601/14 , C07C2602/28 , C07F9/4025 , C07F9/5456 , G03G5/0614 , G03G5/0672 , H01L51/5048 , Y10T428/31678
摘要： A bis(aminostyryl)naphthalene compound represented by the general formula [I] or the like below. General formula [I] (where R2 and R3 each denotes an unsubstituted aryl group; R1 and R4 each denotes an aryl group having a specific substituent such as methoxy group; and R5 and R6 each denotes a cyano group or the like.) A process for producing a bis(aminostyryl)naphthalene compound represented by the general formula [I] by condensation of, for example, 4-(N,N-diarylamino)benzaldehyde with diphosphonic ester or diphosphonium. The bis(aminostyryl)naphthalene compound emits intense yellow or red light. The process permits efficient production of the bis(aminostyryl)naphthalene compound.
摘要翻译：由下述通式[I]表示的双（氨基苯乙烯基）萘化合物等。通式[I]（其中R 2和R 3各自表示未取代的芳基; R 1和R 4各自表示具有特定取代基的芳基，例如甲氧基; R 5 >和R 6各自表示氰基等。）由通式[I]表示的双（氨基苯乙烯基）萘化合物通过例如4-（N，N-二芳基氨基）苯甲醛与二膦酸酯或二磷酸盐。双（氨基苯乙烯基）萘化合物发出强烈的黄色或红色光。该方法允许有效生产双（氨基苯乙烯基）萘化合物。

5. 发明授权

US07402344B2 Organic electroluminescent devices and aminostyrylnaphthalene compounds 有权
标题翻译：有机电致发光器件和氨基苯乙烯基萘化合物
公开(公告)号：US07402344B2
公开(公告)日：2008-07-22
申请号：US10807984
申请日：2004-03-24
申请人： Mari Ichimura , Tadashi Ishibashi , Shinichiro Tamura
发明人： Mari Ichimura , Tadashi Ishibashi , Shinichiro Tamura
IPC分类号： H01L51/50 , C07C211/00
CPC分类号： H01L51/0052 , C07C255/58 , C07C255/59 , C07F9/4056 , C07F9/5456 , C09K11/06 , C09K2211/1011 , C09K2211/1014 , H01L51/0059 , H01L51/006 , H01L51/0081 , H01L51/5012 , H01L51/5048 , H01L2251/308 , H05B33/14 , Y10S428/917
摘要： An organic electroluminescent device includes an anode, a cathode, and an organic layer having a light-emitting area and arranged between the anode and the cathode. The organic layer contains in at least a part thereof at least one aminostyrylnaphthalene compound represented by the following formula [I], [II] or [III]: wherein R1, R2, R11, R12, R23 and R24 are each a phenyl or naphthyl group, R3, R4, R13, R14, R25 and R26 are each an electron attracting group such as a cyano group, and R5, R15 and R27 are each a substituent group such as an alkyl group.
摘要翻译：有机电致发光器件包括阳极，阴极和具有发光区域并且布置在阳极和阴极之间的有机层。有机层的至少一部分含有至少一种由下式[I]，[II]或[III]表示的氨基苯乙烯基萘化合物：其中R 1，R 2， R 11，R 11，R 12，R 23和R 24各自为苯基或萘基， R 3，R 4，R 13，R 14，R 25和R 15，和 R 26各自为吸电子基团，例如氰基，R 5，R 15和R 27， >各自为取代基，例如烷基。

6. 发明授权

US07255935B2 Organic electroluminescent element and luminescent apparatus employing the same 失效
标题翻译：有机电致发光元件和采用其的发光装置
公开(公告)号：US07255935B2
公开(公告)日：2007-08-14
申请号：US10009021
申请日：2001-04-09
申请人： Tadashi Ishibashi , Mari Ichimura , Naoyuki Ueda , Shinichiro Tamura
发明人： Tadashi Ishibashi , Mari Ichimura , Naoyuki Ueda , Shinichiro Tamura
IPC分类号： H01J1/62
CPC分类号： H01L51/5012 , C07C211/54 , C07C211/58 , C07C217/92 , C07C255/58 , H01L27/32 , H01L51/0052 , H01L51/0059 , H01L51/006 , H01L51/0081 , H01L51/5048 , H01L2251/308 , Y10S428/917
摘要： This invention provides an organic electroluminescent element which emits red light with high color purity, high luminance, and high reliability, owing to the compound used therein which has high fluorescence yields and good thermal stability. The organic electroluminescent element which is made up of a glass substrate (1), an ITO transparent electrode (2), a hole transfer layer (6), an electron transfer layer (7), and a metal electrode (3) (which are laminated in the order mentioned), with the hole transfer layer (6) and/or the electron transfer layer (7) being formed of a mixture containing at least one species of the aminostyryl compound represented by the following general formula [I], and a hole blocking layer (30) is interposed between the hole transfer layer (6) and the electron transfer layer (7). Y1—CH═CH—X1—CH═CH—Y2General formula [I] [where, in the general formula [I] above, X1 denotes any aryl group such as a phenyl group having a substituent groups such as a nitro group, and Y1 and Y2 each is a group having an aminophenyl group in the skeleton.]
摘要翻译：本发明提供了由于其中使用的具有高荧光产率和良好的热稳定性的化合物而发出具有高纯度，高亮度和高可靠性的红光的有机电致发光元件。由玻璃基板（1），ITO透明电极（2），空穴转移层（6），电子转移层（7）和金属电极（3）构成的有机电致发光元件以所述顺序层叠），空穴转移层（6）和/或电子转移层（7）由含有至少一种由以下通式[I]表示的氨基苯乙烯基化合物的混合物形成，以及在空穴转移层（6）和电子转移层（7）之间插入空穴阻挡层（30）。 <？in-line-formula description =“In-line Formulas”end =“lead”？> Y -CH-CH-X 1 -CH-CH- 通式[I] <？in-line-formula description =“In-line Formulas”end =“tail”？> [其中，在上述通式[I]中，X < SUP> 1表示任何芳基，例如具有硝基等取代基的苯基，Y 1和Y 2各自为基团在骨架中具有氨基苯基。]

7. 发明申请

US20050215811A1 Bis (aminostyryl) naphthalene compound, synthesis intermediate thereof, and process for production thereof 有权
标题翻译：双（氨基苯乙烯基）萘化合物，其合成中间体及其制备方法
公开(公告)号：US20050215811A1
公开(公告)日：2005-09-29
申请号：US11105082
申请日：2005-04-13
申请人： Mari Ichimura , Tadashi Ishibashi , Shinichiro Tamura
发明人： Mari Ichimura , Tadashi Ishibashi , Shinichiro Tamura
IPC分类号： C09K11/06 , C07C211/50 , C07C211/54 , C07C211/58 , C07C211/60 , C07C217/88 , C07C217/92 , C07C255/58 , C07F9/40 , C07F9/54 , G03G5/06 , H01L51/50 , C07C211/57
CPC分类号： H01L51/006 , C07C211/50 , C07C211/54 , C07C211/58 , C07C211/60 , C07C217/88 , C07C217/92 , C07C255/58 , C07C2601/14 , C07C2602/28 , C07F9/4025 , C07F9/5456 , G03G5/0614 , G03G5/0672 , H01L51/5048 , Y10T428/31678
摘要： A bis(aminostyryl)naphthalene compound represented by the general formula [I] or the like below. (where R2 and R3 each denotes an unsubstituted aryl group; R1 and R4 each denotes an aryl group having a specific substituent such as methoxy group; and R5 and R6 each denotes a cyano group or the like.) A process for producing a bis(aminostyryl)naphthalene compound represented by the general formula [I] by condensation of, for example, 4-(N,N-diarylamino)benzaldehyde with diphosphonic ester or diphosphonium. The bis(aminostyryl)naphthalene compound emits intense yellow or red light. The process permits efficient production of the bis(aminostyryl)naphthalene compound.
摘要翻译：由下述通式[I]表示的双（氨基苯乙烯基）萘化合物等。（其中R 2和R 3各自表示未取代的芳基; R 1和R 4各自表示具有特定取代基的芳基如甲氧基; R 5和R 6各自表示氰基等。）制备双（氨基苯乙烯基）由通式[I]表示的萘化合物通过例如4-（N，N-二芳基氨基）苯甲醛与二膦酸酯或二鏻的缩合。双（氨基苯乙烯基）萘化合物发出强烈的黄色或红色光。该方法允许有效生产双（氨基苯乙烯基）萘化合物。

8. 发明授权

US06897341B2 Bis(aminostyryl)naphthalene compound, synthesis intermediate thereof, and process for production thereof 有权
标题翻译：双（氨基苯乙烯基）萘化合物，其合成中间体及其制备方法
公开(公告)号：US06897341B2
公开(公告)日：2005-05-24
申请号：US10231419
申请日：2002-08-29
申请人： Mari Ichimura , Tadashi Ishibashi , Shinichiro Tamura
发明人： Mari Ichimura , Tadashi Ishibashi , Shinichiro Tamura
IPC分类号： C09K11/06 , C07C211/50 , C07C211/54 , C07C211/58 , C07C211/60 , C07C217/88 , C07C217/92 , C07C255/58 , C07F9/40 , C07F9/54 , G03G5/06 , H01L51/50
CPC分类号： H01L51/006 , C07C211/50 , C07C211/54 , C07C211/58 , C07C211/60 , C07C217/88 , C07C217/92 , C07C255/58 , C07C2601/14 , C07C2602/28 , C07F9/4025 , C07F9/5456 , G03G5/0614 , G03G5/0672 , H01L51/5048 , Y10T428/31678
摘要： A bis(aminostyryl)naphthalene compound represented by the general formula [I] or the like below. (where R2 and R3 each denotes an unsubstituted aryl group; R1 and R4 each denotes an aryl group having a specific substituent such as methoxy group; and R5 and R6 each denotes a cyano group or the like.) A process for producing a bis(aminostyryl)naphthalene compound represented by the general formula [I] by condensation of, for example, 4-(N,N-diarylamino)benzaldehyde with diphosphonic ester or diphosphonium.The bis(aminostyryl)naphthalene compound emits intense yellow or red light. The process permits efficient production of the bis(aminostyryl)naphthalene compound.
摘要翻译：由下述通式[I]表示的双（氨基苯乙烯基）萘化合物等。（其中R 2和R 3各自表示未取代的芳基; R 1和R 4各自表示具有特定取代基的芳基如甲氧基; R 5和R 6各自表示氰基等。）制备双（氨基苯乙烯基）由通式[I]表示的萘化合物通过例如4-（N，N-二芳基氨基）苯甲醛与二膦酸酯或二鏻的缩合。双（氨基苯乙烯基）萘化合物发出强烈的黄色或红色光。该方法允许有效生产双（氨基苯乙烯基）萘化合物。

9. 发明授权

US06790975B2 Aminostyrylanthracene compound, synthetic intermediate thereof, and process for the production thereof 有权
标题翻译：氨基苯乙烯基蒽化合物，其合成中间体及其制备方法
公开(公告)号：US06790975B2
公开(公告)日：2004-09-14
申请号：US09980323
申请日：2002-03-19
申请人： Mari Ichimura , Tadashi Ishibashi , Shinichiro Tamura
发明人： Mari Ichimura , Tadashi Ishibashi , Shinichiro Tamura
IPC分类号： C07C25552
CPC分类号： C07C211/58 , C07C211/54 , C07C211/57 , C07C211/59 , C07C217/92 , C07C217/94 , C07C255/52 , C07C255/58 , C07C2602/10 , C07C2603/24 , C07F9/4056 , C07F9/5456 , H01L51/006
摘要： This invention is an aminostyrylanthracene compound represented by, for example, the following general formula [I]. This compound is produced by condensation from a corresponding aminobenzaldehyde and a phosphonic ester or phosphonium salt. [where, in the general formula [I] above, R2 represents an unsubstituted aryl group, R1 represents an aryl group which may have a variety of substituents, and R3 to R5 each represent a hydrogen atom, a cyano group, or a hydrocarbon group.]
摘要翻译：本发明是由例如以下通式[I]表示的氨基苯乙烯基蒽化合物。该化合物通过相应的氨基苯甲醛和膦酸酯或鏻盐的缩合产生[其中，在上述通式[I]中，R 2表示未取代的芳基，R 1表示可以具有各种取代基，R 3〜R 5各自表示氢原子，氰基或烃基。

10. 发明授权

US06774257B2 Bis (aminostyryl) naphthalene compound, synthesis intermediate thereof, and process for production thereof 有权
标题翻译：双（氨基苯乙烯基）萘化合物，其合成中间体及其制备方法
公开(公告)号：US06774257B2
公开(公告)日：2004-08-10
申请号：US10392435
申请日：2003-03-19
申请人： Mari Ichimura , Tadashi Ishibashi , Shinichiro Tamura
发明人： Mari Ichimura , Tadashi Ishibashi , Shinichiro Tamura
IPC分类号： C07C25550
CPC分类号： H01L51/006 , C07C211/50 , C07C211/54 , C07C211/58 , C07C211/60 , C07C217/88 , C07C217/92 , C07C255/58 , C07C2601/14 , C07C2602/28 , C07F9/4025 , C07F9/5456 , G03G5/0614 , G03G5/0672 , H01L51/5048 , Y10T428/31678
摘要： A bis(aminostyryl)naphthalene compound represented by the general formula [I] or the like below. General formula [I] (where R2 and R3 each denotes an unsubstituted aryl group; R1 and R4 each denotes an aryl group having a specific substituent such as methoxy group; and R5 and R6 each denotes a cyano group or the like.) A process for producing a bis(aminostyryl)naphthalene compound represented by the general formula [I] by condensation of, for example, 4-(N,N-diarylamino)benzaldehyde with diphosphonic ester or diphosphonium. The bis(aminostyryl)naphthalene compound emits intense yellow or red light. The process permits efficient production of the bis(aminostyryl)naphthalene compound.
摘要翻译：通式[I]等表示的双（氨基苯乙烯基）萘化合物等。通式[I]（其中R 2和R 3各自表示未取代的芳基; R 1和R 2' 4>表示具有特定取代基的芳基，例如甲氧基; R 5和R 6各自表示氰基等。）一种制备由下式表示的双（氨基苯乙烯基）萘化合物的方法：通式[I]通过例如4-（N，N-二芳基氨基）苯甲醛与二膦酸酯或二鏻的缩合。双（氨基苯乙烯基）萘化合物发射强烈的黄色或红色光。该方法允许有效生产双（氨基苯乙烯基）萘化合物。

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