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1. 发明申请

US20080275279A1 Oxidative Halogenation of C1 Hydrocarbons to Halogenated C1 Hydrocarbons 审中-公开
标题翻译： C1碳氢化合物对卤代C1烃的氧化卤化
公开(公告)号：US20080275279A1
公开(公告)日：2008-11-06
申请号：US11912376
申请日：2006-04-25
申请人： Simon G. Podkolzin , Eric E. Stangland , Albert E. Schweizer , Mark E. Jones
发明人： Simon G. Podkolzin , Eric E. Stangland , Albert E. Schweizer , Mark E. Jones
IPC分类号： C07C1/02
CPC分类号： B01J27/08 , B01J23/10 , C07C17/154 , C07C17/158 , Y02P20/582 , C07C19/03
摘要： An oxidative halogenation process involving contacting methane, a C1 halogenated hydrocarbon, or a mixture thereof with a source of halogen and a source of oxygen, at a molar ratio of reactant hydrocarbon to source of halogen in a feed to the reactor greater than 23/1, and/or at a molar ratio of reactant hydrocarbon to source of oxygen in a feed to the reactor greater than about 46/1; in the presence of a rare earth halide or rare earth oxyhalide catalyst, to produce a halogenated C1 product having at least one more halogen as compared with the C1 reactant hydrocarbon, preferably, methyl chloride. The process can be advantageously conducted to total conversion of source of halogen and source of oxygen. The process can be advantageously conducted with essentially no halogen in the feed to the reactor, by employing a separate catalyst halogenation step in a pulse, swing or circulating bed mode. The production of methyl halide can be integrated into downstream processes for manufacture of valuable commodity chemicals.
摘要翻译：一种氧化卤化方法，包括使甲烷，C 1卤代烃或其混合物与卤素源和氧源以反应物烃与进料中卤素源的摩尔比接触大于23/1的反应物，和/或反应物烃与反应器进料中氧的来源的摩尔比大于约46/1; 在稀土卤化物或稀土卤氧化物催化剂的存在下，与C 1反应物烃相比产生具有至少一个以上卤素的卤代C 1 -C 1产物，优选氯甲烷。该方法可以有利地进行到卤素源和氧源的总转化。通过在脉冲，摆动或循环床模式中使用单独的催化剂卤化步骤，该方法可以有利地在反应器的进料中基本上不含卤素进行。甲基卤化物的生产可以整合到用于制造有价值的商品化学品的下游工艺中。

2. 发明授权

US09180430B2 Catalytic composition for production of olefins with decreased oxygenate byproducts 有权
标题翻译：用于生产具有降低的含氧化合物副产物的烯烃的催化组合物
公开(公告)号：US09180430B2
公开(公告)日：2015-11-10
申请号：US13634619
申请日：2011-02-25
申请人： Yu Liu , Andrzej M. Malek , Duncan Coffey , Eric E. Stangland , Albert E. Schweizer
发明人： Yu Liu , Andrzej M. Malek , Duncan Coffey , Eric E. Stangland , Albert E. Schweizer
IPC分类号： C07C1/22 , C07C1/24 , C07C1/00 , B01J21/04 , B01J21/12 , B01J23/10 , B01J37/00 , B01J37/04 , C10G3/00
CPC分类号： B01J21/04 , B01J21/12 , B01J23/10 , B01J37/0036 , B01J37/04 , C07C1/24 , C07C2523/10 , C10G3/44 , C10G3/49 , C10G3/54 , C10G2400/20 , C10G2400/22 , Y02P30/20 , C07C11/02
摘要： Catalytic composition for production of olefins and methods of using same to decrease production of oxygenate byproducts. The catalytic composition includes an admixture of an alumina dehydration catalyst and at least one additional metal oxide.
摘要翻译：用于生产烯烃的催化组合物及其使用方法以减少含氧化合物副产物的产生。催化剂组合物包括氧化铝脱水催化剂和至少一种另外的金属氧化物的混合物。

3. 发明申请

US20130012749A1 CATALYTIC COMPOSITION FOR PRODUCTION OF OLEFINS WITH DECREASED OXYGENATE BYPRODUCTS 有权
标题翻译：催化组合物用于生产具有减少氧化产物的烯烃
公开(公告)号：US20130012749A1
公开(公告)日：2013-01-10
申请号：US13634619
申请日：2011-02-25
申请人： Yu Liu , Andrzej M. Malek , Duncan Coffey , Eric E. Stangland , Albert E. Schweizer
发明人： Yu Liu , Andrzej M. Malek , Duncan Coffey , Eric E. Stangland , Albert E. Schweizer
IPC分类号： C07C1/22 , B01J8/00
CPC分类号： B01J21/04 , B01J21/12 , B01J23/10 , B01J37/0036 , B01J37/04 , C07C1/24 , C07C2523/10 , C10G3/44 , C10G3/49 , C10G3/54 , C10G2400/20 , C10G2400/22 , Y02P30/20 , C07C11/02
摘要： Catalytic composition for production of olefins and methods of using same to decrease production of oxygenate byproducts. The catalytic composition includes an admixture of an alumina dehydration catalyst and at least one additional metal oxide.
摘要翻译：用于生产烯烃的催化组合物及其使用方法以减少含氧化合物副产物的产生。催化剂组合物包括氧化铝脱水催化剂和至少一种另外的金属氧化物的混合物。

4. 发明授权

US06452058B1 Oxidative halogenation of C1 hydrocarbons to halogenated C1 hydrocarbons and integrated processes related thereto 有权
标题翻译：将C1碳氢化合物氧化成卤化C1烃及其相关的综合工艺
公开(公告)号：US06452058B1
公开(公告)日：2002-09-17
申请号：US09862058
申请日：2001-05-21
申请人： Albert E. Schweizer , Mark E. Jones , Daniel A. Hickman
发明人： Albert E. Schweizer , Mark E. Jones , Daniel A. Hickman
IPC分类号： C07C1715
CPC分类号： C07C17/156 , C07C1/26 , C07C17/10 , C07C17/154 , C07C17/158 , C07C21/06 , C07C29/124 , C07C2529/70 , Y02P20/125 , Y02P20/52 , Y02P30/42 , C07C11/02 , C07C19/075 , C07C19/03 , C07C31/04
摘要： An oxidative halogenation process involving contacting a reactant hydrocarbon selected from methane, a halogenated C1 hydrocarbon, or a mixture thereof with a source of halogen and, preferably, a source of oxygen in the presence of a rare earth halide or rare earth oxyhalide catalyst, so as to form a halogenated C1 hydrocarbon having a greater number of halogen substituents as compared with the reactant hydrocarbon. Preferably, the product is a monohalogenated methane, more preferably, methyl chloride. The oxidative halogenation process to form methyl halide can be integrated with downstream processes to produce valuable commodity chemicals, for example, methyl alcohol and/or dimethyl ether; light olefins, including ethylene, propylene, and butenes; higher hydrocarbons, including gasolines; vinyl halide monomer, and acetic acid. Hydrogen halide, which is a co-product of these downstream processes, can be recycled to the oxidative halogenation process.
摘要翻译：一种氧化卤化方法，包括在稀土卤化物或稀土氧化物催化剂的存在下使选自甲烷，卤代C1烃或其混合物的反应物烃与卤素源，优选氧源接触，因此以形成与反应物烃相比具有更多卤素取代基的卤代C1烃。优选地，产物是单卤代甲烷，更优选氯甲烷。形成甲基卤化物的氧化卤化方法可与下游方法结合，生产有价值的商品化学品，例如甲醇和/或二甲醚; 轻质烯烃，包括乙烯，丙烯和丁烯; 高级烃类，包括汽油; 乙烯基卤单体和乙酸。作为这些下游方法的共同产物的卤化氢可以再循环到氧化卤化过程中。

5. 发明授权

US06984763B2 Oxidative halogenation and optional dehydrogenation of c3+hydrocarbons 失效
标题翻译： c3 +烃的氧化卤化和任选脱氢
公开(公告)号：US06984763B2
公开(公告)日：2006-01-10
申请号：US10478265
申请日：2002-04-23
申请人： Albert E. Schweizer , Mark E. Jones , Daniel A. Hickman
发明人： Albert E. Schweizer , Mark E. Jones , Daniel A. Hickman
IPC分类号： C07C17/00
CPC分类号： C07C17/156 , B01J23/10 , B01J27/06 , B01J27/08 , B01J27/125 , C07C1/30 , C07C5/48 , C07C17/10 , C07C17/154 , C07C2527/06 , C07C2527/08 , Y02P20/52 , C07C11/02 , C07C19/01 , C07C21/067 , C07C11/06
摘要： An oxidative halogenation and optional dehydrogenation process involving contacting a reactant hydrocarbon having three or more carbon atoms, such as propane or propene, or a halogenated derivative thereof, with a source of halogen, and optionally, a source of oxygen in the presence of a rare earth halide or rare earth oxyhalide catalyst, so as to form a halogenated hydrocarbon product, such as allyl chloride, having three or more carbon atoms and having a greater number of halogen substituents as compared with the reactant hydrocarbon, and optionally, an olefinic co-product, such as propene. The less desired of the two products, that is, the halogenated hydrocarbon or the olefin as the case may be, can be recycled to the process to maximize the production of the desired product.
摘要翻译：氧化卤化和任选的脱氢方法，包括将具有三个或更多个碳原子的反应物烃如丙烷或丙烯或其卤化衍生物与卤素源和任选的氧源在罕见的存在下接触卤化物或稀土氧化物催化剂，以便与反应物烃相比形成具有三个或更多个碳原子并且具有更多数量的卤素取代基的卤代烃产物，如烯丙基氯，以及任选地，产品，如丙烯。根据情况，两种产物，即卤代烃或烯烃的需求不太可以被再循环到该方法中，以使所需产物的产生最大化。

6. 发明授权

US5965475A Processes an catalyst for upgrading waxy, paraffinic feeds 失效
标题翻译：处理用于升级蜡质，石蜡饲料的催化剂
公开(公告)号：US5965475A
公开(公告)日：1999-10-12
申请号：US850358
申请日：1997-05-02
申请人： Robert Jay Wittenbrink , Russell J. Koveal , William J. Murphy , Ian A. Cody , Albert E. Schweizer
发明人： Robert Jay Wittenbrink , Russell J. Koveal , William J. Murphy , Ian A. Cody , Albert E. Schweizer
IPC分类号： B01J29/068 , B01J23/44 , B01J29/06 , C10G45/64 , B01J29/70 , B01J29/85
CPC分类号： B01J29/06 , C10G2400/10
摘要： An improved catalyst for the production of lube oil blending components, and lube oils, from waxy, paraffinic feeds, a process for producing such catalyst, and a process utilizing this catalyst in the production of lubes. The catalyst is a unitized mixed powder pellet catalyst constituted of a dehydrogenation component, or components, suitably a catalytically active Group VIB, VIIB, or VIII metal, or metals, an isomerization component, suitably an amorphous acidic solid support, and a small pore molecular sieve dewaxing component. The dewaxing component is characterized as a small pore molecular sieve wherein the pore windows are formed by 8 oxide atoms which form the limiting edge of the pore window, each of the oxide atoms constituting one of the four oxide atoms of a tetrahedrally coordinated cluster around a silicon or aluminum framework ion, or atom, each oxide ion is coordinated to two framework ions in these structures, and the pore size of the sieve ranges between about 6.3 .ANG. and 2.3 .ANG.. In preparation of the catalysts, the isomerization component, or the dewaxing component, or both, may provide the dehydrogenation function due to the presence of a catalytic metal, or metals, deposited thereon, in which case the components are powdered, the powders mixed together, compressed and formed into solids catalyst shapes comprised of these components. Alternatively, the dehydrogenation function can be added to preformed solids shapes made from powdered dewaxing and isomerization components.
摘要翻译：用于生产来自蜡质，石蜡原料的润滑油混合组分和润滑油的改进的催化剂，用于生产这种催化剂的方法，以及利用该催化剂生产润滑剂的方法。催化剂是由脱氢组分或适当的催化活性组VIB，VIIB或VIII金属或金属，异构化组分，合适地为无定形酸性固体载体和小孔分子的组分组成的混合粉末颗粒催化剂筛脱蜡组分。脱蜡组分的特征在于小孔分子筛，其中孔窗由形成孔窗的限制边缘的8个氧化物原子形成，每个氧化物原子构成四面体配位簇的四个氧化物原子之一硅或铝框架离子或原子，在这些结构中，每个氧化物离子与两个骨架离子配位，并且筛孔的孔径范围在约6.3安格姆和2.3安培之间。在催化剂的制备中，异构化组分或脱蜡组分或两者均可以提供脱氢功能，因为沉积在其上的催化金属或金属的存在，在这种情况下，组分被粉碎，粉末混合在一起，压缩并形成由这些组分组成的固体催化剂形状。或者，可以将脱氢功能加入由粉末状脱蜡和异构化组分制成的预制固体形状。

7. 发明授权

US4992402A Noble metal acidic zeolites for isomerization 失效
标题翻译：贵金属酸性沸石用于异构化
公开(公告)号：US4992402A
公开(公告)日：1991-02-12
申请号：US292783
申请日：1989-01-03
申请人： Albert E. Schweizer
发明人： Albert E. Schweizer
IPC分类号： B01J29/12 , B01J29/22 , C07C5/27 , C10G35/095
CPC分类号： C10G35/095 , B01J29/12 , B01J29/22 , C07C5/2724 , C07C5/2791
摘要： Disclosed is a method for preparing noble-metal containing zeolite materials suitable for isomerization reactions. The catalysts are prepared by contacting an zeolite selected from the acidic faujasite, LZ-210 type zeolites and mordenite with an effective amount of a noble metal compound selected from Pt(acetylacetonate).sub.2 or Pd(acetylacetonate).sub.2 then calcining at a temperature from about 250.degree. C. to 600.degree. for an effective amount of time.
摘要翻译：公开了一种制备适用于异构化反应的含贵金属的沸石材料的方法。催化剂通过使选自酸性八面沸石，LZ-210型沸石和丝光沸石的沸石与有效量的选自Pt（乙酰丙酮化物）2或Pd（乙酰丙酮化物）2的贵金属化合物接触而制备，然后在约 250℃至600℃有效量的时间。

8. 发明授权

US06605749B2 Synthesis of molecular sieve catalysts 有权
公开(公告)号：US06605749B2
公开(公告)日：2003-08-12
申请号：US10342601
申请日：2003-01-15
申请人： Stephen N. Vaughn , Luc R. M. Martens , Keith H. Kuechler , Albert E. Schweizer
发明人： Stephen N. Vaughn , Luc R. M. Martens , Keith H. Kuechler , Albert E. Schweizer
IPC分类号： C07C100
CPC分类号： B01J29/005 , B01J29/85 , B01J2229/26 , B01J2229/42 , C10G3/45 , C10G3/49 , C10G2300/4081 , C10G2300/708 , C10G2400/20 , Y02P30/20 , Y02P30/42 , Y10S423/30 , Y10S502/514
摘要： Disclosed is a molecular sieve catalyst which contains molecular sieve-containing attrition particles and virgin molecular sieve, the attrition particles having been recycled from a catalyst manufacture process or from a reaction system. The catalyst can be used in a variety of catalytic reaction processes. A desired process is making olefins from an oxygenate feedstock. The recovery and use of the attrition particles in the catalyst is beneficial in minimizing waste, thereby reducing problems relating to both environmental and economic constraints.

9. 发明授权

US06541415B2 Synthesis of molecular sieve catalysts 有权
公开(公告)号：US06541415B2
公开(公告)日：2003-04-01
申请号：US09894158
申请日：2001-06-27
申请人： Stephen N. Vaughn , Luc R. M. Martens , Keith H. Kuechler , Albert E. Schweizer
发明人： Stephen N. Vaughn , Luc R. M. Martens , Keith H. Kuechler , Albert E. Schweizer
IPC分类号： B01J27182
CPC分类号： B01J29/005 , B01J29/85 , B01J2229/26 , B01J2229/42 , C10G3/45 , C10G3/49 , C10G2300/4081 , C10G2300/708 , C10G2400/20 , Y02P30/20 , Y02P30/42 , Y10S423/30 , Y10S502/514
摘要： Disclosed is a molecular sieve catalyst which contains molecular sieve-containing attrition particles and virgin molecular sieve, the attrition particles having been recycled from a catalyst manufacture process or from a reaction system. The catalyst can be used in a variety of catalytic reaction processes. A desired process is making olefins from an oxygenate feedstock. The recovery and use of the attrition particles in the catalyst is beneficial in minimizing waste, thereby reducing problems relating to both environmental and economic constraints.

10. 发明授权

US06482313B1 FCC process incorporating crystalline microporous oxide catalysts having increased Lewis acidity 有权
标题翻译： FCC方法结合具有增加的路易斯酸度的结晶微孔氧化物催化剂
公开(公告)号：US06482313B1
公开(公告)日：2002-11-19
申请号：US09653135
申请日：2000-08-31
申请人： William L. Schuette , Albert E. Schweizer
发明人： William L. Schuette , Albert E. Schweizer
IPC分类号： C10G1104
CPC分类号： B01J29/08 , B01J37/0238 , C10G11/05 , C10G11/18
摘要： A catalyst component, a catalyst, and a process for making the component and catalyst are disclosed herein. Also disclosed herein is a fluid catalytic cracking process for converting petroleum feedstocks to lower boiling products wherein the feedstock is contacted with the catalyst. The catalyst component is a crystalline microporous oxide catalyst to which a compound for promoting dehydrogenation and increasing Lewis acidity is effectively added. This catalyst component can be included in an inorganic oxide matrix material and used as a catalyst. Preferably, the compound for promoting dehydrogenation and increasing Lewis acidity is effectively added to a non-framework portion of the crystalline microporous oxide.
摘要翻译：本文公开了催化剂组分，催化剂和制备组分和催化剂的方法。本文还公开了用于将石油原料转化为较低沸点产物的流化催化裂化方法，其中原料与催化剂接触。催化剂组分是一种结晶微孔氧化物催化剂，其中有效地添加了用于促进脱氢和增加路易斯酸度的化合物。该催化剂组分可以包括在无机氧化物基质材料中并用作催化剂。优选地，用于促进脱氢和增加路易斯酸度的化合物被有效地加入结晶微孔氧化物的非骨架部分。

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