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1. 发明授权

US06900279B2 Compositions containing copolymers of post-polymerization reacted (meth) acrylate monomers 失效
标题翻译：含有后聚合反应的（甲基）丙烯酸酯单体的共聚物的组合物
公开(公告)号：US06900279B2
公开(公告)日：2005-05-31
申请号：US10348367
申请日：2003-01-21
申请人： Simion Coca , Gregory J. McCollum , James B. O'Dwyer , Edward R. Coleridge , Steven V. Barancyk
发明人： Simion Coca , Gregory J. McCollum , James B. O'Dwyer , Edward R. Coleridge , Steven V. Barancyk
IPC分类号： B05D7/24 , B05D1/00 , B05D3/02 , B05D3/06 , B05D7/00 , B32B27/30 , C08F8/00 , C08F210/00 , C08F210/10 , C08F210/14 , C08F220/10 , C08F290/04 , C08G18/62 , C08G18/79 , C08G18/80 , C08K5/092 , C08L23/20 , C08L23/22 , C08L33/06 , C08L33/14 , C08L63/00 , C08L101/00 , C09D7/12 , C09D109/00 , C09D109/02 , C09D123/22 , C09D133/00 , C09D133/02 , C09D133/06 , C09D133/08 , C09D133/14 , C09D133/24 , C09D157/04 , C09D163/00 , C09D167/00 , C09D175/04 , C09D201/00 , C08F120/54 , C08F120/10
CPC分类号： B05D7/57 , B05D1/007 , B05D3/0209 , B05D3/067 , B05D7/53 , C08F8/00 , C08F210/10 , C08F220/10 , C08F290/046 , C08G18/6229 , C08G18/792 , C08G18/798 , C08G18/8025 , C08G18/807 , C08G18/8074 , C08G2150/20 , C08L33/068 , C09D123/22 , C09D133/062 , C09D133/08 , Y10T428/31504 , Y10T428/31511 , C08F220/00 , C08F220/12 , C08F210/00 , C08L2666/28 , C08L2666/02 , C08F214/18 , C08F2500/03 , C08F2500/02 , C08F212/00 , C08F222/00 , C08F2500/26 , C08L2666/04
摘要： A composition that includes a non-gelled copolymer that includes one or more residues of a first polymerizable ethylenically unsaturated monomer containing a pendant amide, ester or carboxylic acid group. The nearest neighboring monomer residues of the majority of the first monomer residues along the copolymer molecule do not contain pendant carbonyl functional groups. The amide, ester or carboxylic acid group of the residues of the first monomer are the post polymerization transesterification, transamidification or hydrolysis reaction product of a C1-C4 alkyl ester group in the unreacted first monomer with a compound selected from amine functional compounds and hydroxy functional compounds. The reacted copolymer is substantially free of cyclical structures resulting from the transesterification, transamidification or hydrolysis reaction. The compositions may be thermosetting compositions useful in multi-layer composite coatings.
摘要翻译：包含非凝胶共聚物的组合物，其包含含有侧酰胺，酯或羧酸基团的第一可聚合烯属不饱和单体的一个或多个残基。沿着共聚物分子的大部分第一单体残基的最邻近的单体残基不含有羰基官能团。第一单体的残基的酰胺，酯或羧酸基是C 1 -C 4烷基酯基的后聚合酯交换，转酰胺化或水解反应产物在未反应的第一单体中与选自胺官能化合物和羟基官能化合物的化合物反应。反应的共聚物基本上不含由酯交换，酰胺化或水解反应产生的循环结构。组合物可以是可用于多层复合涂层的热固性组合物。

2. 发明授权

US07619040B2 Compositions containing copolymers of olefinic monomers 失效
标题翻译：含有烯属单体共聚物的组合物
公开(公告)号：US07619040B2
公开(公告)日：2009-11-17
申请号：US11116706
申请日：2005-04-28
申请人： Steven V. Barancyk , Simion Coca , Edward R. Coleridge , Gregory J. McCollum , James B. O'Dwyer
发明人： Steven V. Barancyk , Simion Coca , Edward R. Coleridge , Gregory J. McCollum , James B. O'Dwyer
IPC分类号： C08F8/32
CPC分类号： C08F8/00 , B05D1/007 , B05D3/0209 , B05D3/067 , B05D7/53 , B05D7/57 , C08F210/10 , C08F220/10 , C09D123/22 , C08F210/00 , C08F220/12 , C08L2666/28
摘要： A composition that includes a non-gelled copolymer that contains residues having structural units (I): where n is an integer from 1 to 10,000; R1 is linear or branched C1 to C4 alkyl; R2 is selected from the group consisting of methyl, linear, cyclic or branched C2 to C20 alkyl, alkenyl, aryl, alkaryl and aralkyl, and R3 is a group resulting from a post polymerization reaction selected from transesterification, transamidification and hydrolysis with a compound selected from hydroxy functional compounds and amine functional compounds. The composition may contain co-reactive functional groups and may be a thermosetting composition. A substrate may be coated with the thermosetting composition singly or as part of a multi-layer composite coating that includes a base coat layer and a substantially pigment free top coat layer.
摘要翻译：包含含有具有结构单元（I）的残基的非胶凝共聚物的组合物：其中n为1至10,000的整数; R1是直链或支链C1-C4烷基; R 2选自甲基，直链，环状或支链C 2至C 20烷基，烯基，芳基，烷芳基和芳烷基，并且R 3是由选择酯交换，转酰胺化和水解的后聚合反应得到的基团，由羟基官能化合物和胺官能化合物组成。组合物可以含有共反应性官能团并且可以是热固性组合物。基材可以单独地涂覆有热固性组合物，或者作为多层复合涂层的一部分，其包括底涂层和基本上不含颜料的顶涂层。

3. 发明授权

US07125931B2 Thermosetting compositions containing alternating copolymers of isobutylene type monomers 失效
公开(公告)号：US07125931B2
公开(公告)日：2006-10-24
申请号：US10887733
申请日：2004-07-09
申请人： Simion Coca , Edward R. Coleridge , Gregory J. McCollum , James B. O'Dwyer , James E. Poole , Victoria A. Trettel
发明人： Simion Coca , Edward R. Coleridge , Gregory J. McCollum , James B. O'Dwyer , James E. Poole , Victoria A. Trettel
IPC分类号： C08F8/00
CPC分类号： B05D7/57 , B05D1/007 , B05D3/0209 , B05D3/067 , B05D7/53 , C08F8/00 , C08F210/10 , C08F220/10 , C08F290/046 , C08G18/6229 , C08G18/792 , C08G18/798 , C08G18/8025 , C08G18/807 , C08G18/8074 , C08G2150/20 , C08L33/068 , C09D123/22 , C09D133/062 , C09D133/08 , Y10T428/31504 , Y10T428/31511 , C08F220/00 , C08F220/12 , C08F210/00 , C08L2666/28 , C08L2666/02 , C08F214/18 , C08F2500/03 , C08F2500/02 , C08F212/00 , C08F222/00 , C08F2500/26 , C08L2666/04
摘要： A thermosetting composition that includes an ungelled copolymer composition and a crosslinking agent. The ungelled copolymer composition includes a functional group-containing copolymer that includes segments of alternating residues derived from a donor monomer composition comprising an acceptor monomer composition. The donor monomer composition includes one or both of isobutylene and diisobutylene, and the acceptor monomer composition includes acrylic monomers and monomers containing functional groups. The ungelled copolymer composition is substantially free of transition metals and Lewis acids, and the copolymer is substantially free of maleate-type monomer residues and fumarate-type monomer residues. The crosslinking agent has at least two functional groups that are reactive with the functional groups of the copolymer. The thermosetting composition may be in liquid, powder, or dispersed form and may be applied by traditional or electrocoating methods.

4. 发明授权

US06992137B2 Alternating copolymers of isobutylene type monomers 失效
公开(公告)号：US06992137B2
公开(公告)日：2006-01-31
申请号：US10697413
申请日：2003-10-30
申请人： Simion Coca , Edward R. Coleridge , Gregory J. McCollum , James B. O'Dwyer , James E. Poole , Victoria A. Trettel
发明人： Simion Coca , Edward R. Coleridge , Gregory J. McCollum , James B. O'Dwyer , James E. Poole , Victoria A. Trettel
IPC分类号： C08F8/00
CPC分类号： C09D201/02 , C08F8/00 , C08F10/00 , C08F20/00
摘要： A copolymer composition that includes a copolymer comprised of at least 30 mol % of residues having the following alternating residues from a donor monomer and from an acceptor monomer. The copolymer contains at least 15 mol % of an isobutylene type donor monomer and at least 15 mol % of an acrylic monomer as an acceptor monomer. The copolymer is substantially free of maleate or fumarate monomer segments and the copolymer composition is substantially free of Lewis acids and transition metals. Also disclosed is a thermosetting composition that includes a reactant comprising functional groups, a crosslinking agent having at least two functional groups that are reactive with the functional groups first reactant, and a copolymer flow control agent that includes the copolymer composition as well as substrates coated with the thermosetting composition.

5. 发明授权

US06677422B2 Method of making alternating copolymers of isobutylene type monomers 失效
标题翻译：制备异丁烯型单体的交替共聚物的方法
公开(公告)号：US06677422B2
公开(公告)日：2004-01-13
申请号：US10077559
申请日：2002-02-15
申请人： Simion Coca , Edward R. Coleridge , Gregory J. McCollum , James B. O'Dwyer , James E. Poole , Victoria A. Trettel
发明人： Simion Coca , Edward R. Coleridge , Gregory J. McCollum , James B. O'Dwyer , James E. Poole , Victoria A. Trettel
IPC分类号： C08F1000
CPC分类号： C08F220/12
摘要： A method of making a copolymer composition containing a copolymer, which includes the steps of (a) providing a donor monomer composition that includes an isobutylene type monomer; (b) mixing the donor monomer composition with an ethylenically unsaturated monomer composition that includes one or more ethylenically unsaturated acceptor monomers, and is substantially free of maleate type monomers and fumarate type monomers, and (c) polymerizing the mixture resulting from step (b) in the presence of a free radical polymerization initiator. The polymerization is carried out in the substantial absence of Lewis acids and/or transition metals. The isobutylene type monomer is present at a molar excess of at least 10 mol % based on the molar concentration of monomers in the ethylenically unsaturated monomer composition. The ethylenically unsaturated acceptor monomers are present in an amount of at least 15 mol % of the total monomer composition.
摘要翻译：一种制备含有共聚物的共聚物组合物的方法，其包括以下步骤：（a）提供包含异丁烯型单体的供体单体组合物; （b）将供体单体组合物与包含一种或多种烯键式不饱和受体单体的烯属不饱和单体组合物混合，并且基本上不含马来酸盐型单体和富马酸盐型单体，和（c）将由步骤（b）得到的混合物聚合，在自由基聚合引发剂存在下进行。基本上不存在路易斯酸和/或过渡金属进行聚合。基于烯属不饱和单体组合物中单体的摩尔浓度，异丁烯型单体的摩尔过量为至少10摩尔％。烯属不饱和受体单体的存在量为总单体组合物的至少15摩尔％。

6. 发明授权

US07132476B2 Thermosetting compositions containing alternating copolymers of isobutylene type monomers 失效
公开(公告)号：US07132476B2
公开(公告)日：2006-11-07
申请号：US10887682
申请日：2004-07-09
申请人： Simion Coca , Edward R. Coleridge , Gregory J. McCollum , James B. O'Dwyer , James E. Poole , Victoria A. Trettel
发明人： Simion Coca , Edward R. Coleridge , Gregory J. McCollum , James B. O'Dwyer , James E. Poole , Victoria A. Trettel
IPC分类号： C08F8/00
CPC分类号： B05D7/57 , B05D1/007 , B05D3/0209 , B05D3/067 , B05D7/53 , C08F8/00 , C08F210/10 , C08F220/10 , C08F290/046 , C08G18/6229 , C08G18/792 , C08G18/798 , C08G18/8025 , C08G18/807 , C08G18/8074 , C08G2150/20 , C08L33/068 , C09D123/22 , C09D133/062 , C09D133/08 , Y10T428/31504 , Y10T428/31511 , C08F220/00 , C08F220/12 , C08F210/00 , C08L2666/28 , C08L2666/02 , C08F214/18 , C08F2500/03 , C08F2500/02 , C08F212/00 , C08F222/00 , C08F2500/26 , C08L2666/04
摘要： A thermosetting composition that includes an ungelled copolymer composition and a crosslinking agent. The ungelled copolymer composition includes a functional group-containing copolymer that includes segments of alternating residues derived from a donor monomer composition comprising an acceptor monomer composition. The donor monomer composition includes one or both of isobutylene and diisobutylene, and the acceptor monomer composition includes acrylic monomers and monomers containing functional groups. The ungelled copolymer composition is substantially free of transition metals and Lewis acids, and the copolymer is substantially free of maleate-type monomer residues and fumarate-type monomer residues. The crosslinking agent has at least two functional groups that are reactive with the functional groups of the copolymer. The thermosetting composition may be in liquid, powder, or dispersed form and may be applied by traditional or electrocoating methods.

7. 发明授权

US06784248B2 Thermosetting compositions containing alternating copolymers of isobutylene type monomers 失效
标题翻译：含有异丁烯型单体交替共聚物的热固性组合物
公开(公告)号：US06784248B2
公开(公告)日：2004-08-31
申请号：US10077645
申请日：2002-02-15
申请人： Simion Coca , Edward R. Coleridge , Gregory J. McCollum , James B. O'Dwyer , James E. Poole , Victoria A. Trettel
发明人： Simion Coca , Edward R. Coleridge , Gregory J. McCollum , James B. O'Dwyer , James E. Poole , Victoria A. Trettel
IPC分类号： C08F832
CPC分类号： B05D7/57 , B05D1/007 , B05D3/0209 , B05D3/067 , B05D7/53 , C08F8/00 , C08F210/10 , C08F220/10 , C08F290/046 , C08G18/6229 , C08G18/792 , C08G18/798 , C08G18/8025 , C08G18/807 , C08G18/8074 , C08G2150/20 , C08L33/068 , C09D123/22 , C09D133/062 , C09D133/08 , Y10T428/31504 , Y10T428/31511 , C08F220/00 , C08F220/12 , C08F210/00 , C08L2666/28 , C08L2666/02 , C08F214/18 , C08F2500/03 , C08F2500/02 , C08F212/00 , C08F222/00 , C08F2500/26 , C08L2666/04
摘要： A thermosetting composition that includes an ungelled copolymer composition and a crosslinking agent. The ungelled copolymer composition includes a functional group-containing copolymer that includes segments of alternating residues derived from a donor monomer composition comprising an acceptor monomer composition. The donor monomer composition includes one or both of isobutylene and diisobutylene, and the acceptor monomer composition includes acrylic monomers and monomers containing functional groups. The ungelled copolymer composition is substantially free of transition metals and Lewis acids, and the copolymer is substantially free of maleate-type monomer residues and fumarate-type monomer residues. The crosslinking agent has at least two functional groups that are reactive with the functional groups of the copolymer. The thermosetting composition may be in liquid, powder, or dispersed form and may be applied by traditional or electrocoating methods.
摘要翻译：包含未凝胶化共聚物组合物和交联剂的热固性组合物。非凝胶共聚物组合物包括含官能团的共聚物，其包含衍生自包含受体单体组合物的供体单体组合物的交替残基的片段。供体单体组合物包括异丁烯和二异丁烯中的一种或两种，并且受体单体组合物包括丙烯酸单体和含有官能团的单体。未凝胶化的共聚物组合物基本上不含过渡金属和路易斯酸，共聚物基本上不含马来酸盐型单体残基和富马酸盐型单体残基。交联剂具有与共聚物的官能团反应的至少两个官能团。热固性组合物可以是液体，粉末或分散形式，并且可以通过传统或电泳方法施加。

8. 发明申请

US20100160561A1 COPOLYMERS OF ALPHA-OLEFIN TYPE MONOMERS AND CURABLE FILM-FORMING COMPOSITIONS CONTAINING THEM 审中-公开
标题翻译： ALPHA-OLEFIN型单体的共聚物和含有它们的可固化成膜组合物
公开(公告)号：US20100160561A1
公开(公告)日：2010-06-24
申请号：US12343565
申请日：2008-12-24
申请人： Simion Coca , Edward R. Coleridge , Gregory J. McCollum , James B. O'Dwyer
发明人： Simion Coca , Edward R. Coleridge , Gregory J. McCollum , James B. O'Dwyer
IPC分类号： C08F220/06 , C08L75/00
CPC分类号： C08F210/14 , C08F210/10 , C08F4/34 , C08F220/12 , C08F220/26 , C08F2500/03 , C08F2500/02 , C08F2500/26
摘要： The present invention is directed to copolymers, which are polymerization products of: (i) a monomer having alpha-olefinic functionality; (ii) a monomer different from (i) having active hydrogen functionality; and (iii) a monomer different from (ii) having acrylic functionality. The molar ratio of the monomer (i) having alpha-olefinic functionality to the monomer (iii) having acrylic functionality is less than 1:1, and the conversion of the monomer (i) having alpha-olefinic functionality during polymerization is greater than 90%. When monomers having methacrylic functionality are used to prepare the copolymer, the molar ratio of the monomer (iii) having acrylic functionality to the monomers having methacrylic functionality is greater than 2:1. Also disclosed are curable film-forming compositions comprising the copolymers.
摘要翻译：本发明涉及共聚物，其是以下聚合产物：（i）具有α-烯属官能团的单体; （ii）不同于（i）具有活性氢官能团的单体; 和（iii）不同于具有丙烯酸官能度的（ii）的单体。具有α-烯属官能度的单体（i）与具有丙烯酸官能度的单体（iii）的摩尔比小于1:1，聚合过程中具有α-烯属官能度的单体（i）的转化率大于90 ％。当使用具有甲基丙烯酸官能度的单体制备共聚物时，具有丙烯酸官能度的单体（ⅲ）与具有甲基丙烯酸官能度的单体的摩尔比大于2:1。还公开了包含该共聚物的可固化成膜组合物。

9. 发明授权

US06686432B2 Alternating copolymers of isobutylene type monomers 失效
公开(公告)号：US06686432B2
公开(公告)日：2004-02-03
申请号：US10076984
申请日：2002-02-15
申请人： Simion Coca , Edward R. Coleridge , Gregory J. McCollum , James B. O'Dwyer , James E. Poole , Victoria A. Trettel
发明人： Simion Coca , Edward R. Coleridge , Gregory J. McCollum , James B. O'Dwyer , James E. Poole , Victoria A. Trettel
IPC分类号： C08F1000
CPC分类号： C09D201/02 , C08F8/00 , C08F10/00 , C08F20/00
摘要： A copolymer composition that includes a copolymer comprised of at least 30 mol % of residues having the following alternating residues from a donor monomer and from an acceptor monomer. The copolymer contains at least 15 mol % of an isobutylene type donor monomer and at least 15 mol % of an acrylic monomer as an acceptor monomer. The copolymer is substantially free of maleate or fumarate monomer segments and the copolymer composition is substantially free of Lewis acids and transition metals. Also disclosed is a thermosetting composition that includes a reactant comprising functional groups, a crosslinking agent having at least two functional groups that are reactive with the functional groups first reactant, and a copolymer flow control agent that includes the copolymer composition as well as substrates coated with the thermosetting composition.

10. 发明授权

US07332545B2 Fluoropolymers, methods for their production, and thermosetting compositions containing them 失效
标题翻译：含氟聚合物，它们的生产方法和含有它们的热固性组合物
公开(公告)号：US07332545B2
公开(公告)日：2008-02-19
申请号：US11239777
申请日：2005-09-30
申请人： Simion Coca , Edward R. Coleridge , James B. O'Dwyer , Brian E. Woodworth , Richard J. Winters
发明人： Simion Coca , Edward R. Coleridge , James B. O'Dwyer , Brian E. Woodworth , Richard J. Winters
IPC分类号： C08F114/18
CPC分类号： C08F214/18 , C08F8/12 , C08F214/28 , C08F2800/10 , C08F2800/20 , C09D123/22 , C08L2666/28 , C08F218/08
摘要： Fluoropolymers are disclosed. The fluoropolymers include (i) units derived from a fluoromonomer having the formula F2C═CXY, where X is CF3 and Y is either F or CF3, and (ii) units derived from at least one donor monomer. In the disclosed fluoropolymers, units (i) and (ii) are distributed along the fluoropolymer chain in a substantially alternating fashion. Also disclosed are thermosetting compositions containing such fluoropolymers, substrates coated with such compositions, methods for making such compositions, and methods for coating substrates with such compositions.
摘要翻译：公开了含氟聚合物。含氟聚合物包括（i）衍生自具有式F 2 C-CXY的含氟单体的单元，其中X是CF 3，Y是F或CF 3 和（ii）衍生自至少一种供体单体的单元。在所公开的含氟聚合物中，单元（i）和（ii）以基本交替的方式沿着含氟聚合物链分布。还公开了含有这样的含氟聚合物的热固性组合物，用这种组合物涂覆的基材，制备这种组合物的方法，以及用这种组合物涂覆基材的方法。

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