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1. 发明授权

US5609845A Catalytic production of hydrogen from hydrogen sulfide and carbon monoxide 失效
标题翻译：从硫化氢和一氧化碳催化生产氢气
公开(公告)号：US5609845A
公开(公告)日：1997-03-11
申请号：US385529
申请日：1995-02-08
申请人： Ronald J. Cimini , David O. Marler , Stephen J. McCarthy , Harry A. McVeigh , Gerald J. Teitman
发明人： Ronald J. Cimini , David O. Marler , Stephen J. McCarthy , Harry A. McVeigh , Gerald J. Teitman
IPC分类号： B01J23/881 , B01J23/882 , B01J23/888 , C01B3/06 , C01B17/04 , C01B17/50 , C01B17/74 , C01B32/50 , C01B3/02 , C01G1/04
CPC分类号： C01B31/20 , B01J23/881 , B01J23/882 , B01J23/888 , C01B17/0404 , C01B17/508 , C01B17/74 , C01B3/06 , Y02E60/36
摘要： There is provided a process for the catalytic production of hydrogen from the reaction of hydrogen sulfide and carbon monoxide with the elimination of the carbonyl sulfide and/or sulfur dioxide by-products. The carbonyl sulfide and the sulfur dioxide are combusted or reacted in one or more reaction steps with each other, oxygen and/or hydrogen sulfide to produce carbon dioxide, water, sulfur or sulfuric acid or a combination of these.
摘要翻译：提供了从硫化氢和一氧化碳的反应催化生成氢气以消除羰基硫化物和/或二氧化硫副产物的方法。羰基硫化物和二氧化硫在一个或多个反应步骤中彼此燃烧或反应，即氧气和/或硫化氢，以产生二氧化碳，水，硫或硫酸或它们的组合。

2. 发明授权

US5624964A Integration of steam reforming unit and cogeneration power plant 失效
标题翻译：蒸汽重整单元和热电联产电站的整合
公开(公告)号：US5624964A
公开(公告)日：1997-04-29
申请号：US471976
申请日：1995-06-06
申请人： Ronald J. Cimini , David O. Marler , Reuel Shinnar , Gerald J. Teitman
发明人： Ronald J. Cimini , David O. Marler , Reuel Shinnar , Gerald J. Teitman
IPC分类号： C01B3/44 , C07C27/06
CPC分类号： C01B3/44 , Y02E20/16 , Y02P20/584
摘要： A process for integration of a steam reforming unit and a cogeneration power plant in which said steam reforming unit comprises two communicating fluid beds; the first fluid bed comprising a reformer containing catalyst and which is used to react steam and light hydrocarbons at conditions sufficient to produce a mixture comprising synthesis gas hydrogen, carbon monoxide, and carbon dioxide, the second fluid bed comprising a combustor-regenerator which receives spent catalyst from the first fluid bed and which provides heat to heat the catalyst and balance the reaction endotherm, by combusting fuel gas in direct contact with the catalyst producing hot flue gas; said cogeneration power plant comprises a gas turbine equipped with an air compressor and a combustor; said integration which comprises drawing off a portion of compressed air from the power plant gas turbine air compressor leaving remainder compressed air; introducing the drawn off compressed air to the combustor-regenerator; mixing the hot flue gas from the combustor-regenerator with the remainder of the compressed air to produce a recombined gas stream and feeding this recombined gas stream to the combustor of the cogeneration gas turbine power plant.
摘要翻译：一种用于整合蒸汽重整单元和热电联产电厂的方法，其中所述蒸汽重整单元包括两个连通流体床; 所述第一流化床包括含有重整器的催化剂，其用于在足以产生包含合成气氢，一氧化碳和二氧化碳的混合物的条件下反应蒸汽和轻质烃，所述第二流化床包括燃烧器再生器催化剂，其提供热量以加热催化剂并平衡反应吸热，通过燃烧与产生热烟道气的催化剂直接接触的燃料气体; 所述热电联产电厂包括配备有空气压缩机和燃烧器的燃气轮机; 所述集成包括从发电厂燃气轮机空气压缩机中取出一部分压缩空气，留下剩余的压缩空气; 将抽出的压缩空气引入燃烧器 - 再生器; 将来自燃烧器 - 再生器的热烟气与剩余的压缩空气混合以产生重组气流，并将该重组气流送入热电联产燃气轮机发电厂的燃烧器。

3. 发明授权

US5639931A Process for producing low aromatic diesel fuel with high cetane index 失效
标题翻译：具有高十六烷指数的低芳烃柴油的生产工艺
公开(公告)号：US5639931A
公开(公告)日：1997-06-17
申请号：US459062
申请日：1995-06-02
申请人： Stuart D. Hellring , Albin Huss, Jr. , Michael E. Landis , David O. Marler , Gerald J. Teitman , Hye Kyung C. Timken , Jeffrey C. Trewella
发明人： Stuart D. Hellring , Albin Huss, Jr. , Michael E. Landis , David O. Marler , Gerald J. Teitman , Hye Kyung C. Timken , Jeffrey C. Trewella
IPC分类号： B01J29/04 , C01B39/12 , C01B39/48 , C07B61/00 , C07C2/58 , C07C5/27 , C07C9/12 , C07C9/18 , C10G11/05
CPC分类号： B01J29/04 , C01B39/12 , C01B39/48 , C07C2/58 , C07C2529/70
摘要： At least one olefin and at least one isoparaffin are converted to a diesel fuel blending component by contacting the olefin and the isoparaffin with a catalyst selected from MCM-22, MCM-36, MCM-49, and MCM-56 to provide a product containing a diesel fuel.
摘要翻译：通过使烯烃和异链烷烃与选自MCM-22，MCM-36，MCM-49和MCM-56的催化剂接触，将至少一种烯烃和至少一种异链烷烃转化为柴油燃料调和组分，以提供含一种柴油。

4. 发明授权

US5780703A Process for producing low aromatic diesel fuel with high cetane index 失效
标题翻译：具有高十六烷指数的低芳烃柴油的生产工艺
公开(公告)号：US5780703A
公开(公告)日：1998-07-14
申请号：US513107
申请日：1995-08-09
申请人： Clarence D. Chang , Stuart D. Hellring , David O. Marler , Jose G. Santiesteban , James C. Vartuli
发明人： Clarence D. Chang , Stuart D. Hellring , David O. Marler , Jose G. Santiesteban , James C. Vartuli
IPC分类号： B01J23/30 , B01J23/882 , B01J23/888 , B01J37/03 , C07C2/58 , C07C5/27 , C10G50/00 , C10G35/04
CPC分类号： C10G50/00 , B01J23/30 , B01J23/882 , B01J23/888 , C07C2/58 , C07C5/2772 , B01J37/03 , C07C2521/06 , C07C2523/30
摘要： A process for converting at least one olefin and at least one isoparaffin to a diesel fuel blending component comprising the steps of contacting the olefin and the isoparaffin with a catalyst comprising an acidic solid comprising a Group IVB metal oxide modified with an oxyanion of a Group VIB metal to provide a diesel fuel. Process conditions can be varied to favor the formation of gasoline, distillate, lube range products or mixtures thereof.
摘要翻译：一种将至少一种烯烃和至少一种异链烷烃转化为柴油燃料共混组分的方法，包括以下步骤：使烯烃和异链烷烃与包含酸性固体的催化剂接触，所述酸性固体包含用VIB族氧基反应改性的IVB族金属氧化物金属提供柴油。工艺条件可以变化以有利于形成汽油，馏出物，润滑剂产品或其混合物。

5. 发明授权

US5475178A Supported heteropoly acid catalysts 失效
标题翻译：负载型杂多酸催化剂
公开(公告)号：US5475178A
公开(公告)日：1995-12-12
申请号：US292653
申请日：1994-08-18
申请人： Kenneth J. Del Rossi , Gregory A. Jablonski , Charles T. Kresge , Guenter H. Kuehl , David O. Marler , Gayatri S. Rav , Brenda H. Rose
发明人： Kenneth J. Del Rossi , Gregory A. Jablonski , Charles T. Kresge , Guenter H. Kuehl , David O. Marler , Gayatri S. Rav , Brenda H. Rose
IPC分类号： B01J27/188 , B01J29/03 , B01J29/04 , C07C2/62 , C07C2/64 , C07C2/68 , C07C5/22 , C07C15/107
CPC分类号： B01J29/0341 , B01J27/188 , B01J29/041 , B01J29/043 , C07C2/62 , B01J29/0308 , C07C2527/188 , Y02P20/588
摘要： There is provided a catalyst comprising a heteropoly acid, such as phosphotungstic acid, supported on a mesoporous crystalline material, such as M41S. A particular form of this M41S support is designated as MCM-41. There is also provided a method for preparing this catalyst by impregnating the heteropoly acid on the support. There is also provided a process for using this catalyst to catalyze acid catalyzed reactions, such as the isomerization of paraffins and the alkylation of aromatics.
摘要翻译：提供了一种催化剂，其包含负载在介孔结晶材料如M41S上的杂多酸如磷钨酸。该M41S支持的特定形式被指定为MCM-41。还提供了通过将杂多酸浸渍在载体上来制备该催化剂的方法。还提供了一种使用该催化剂催化酸催化反应的方法，例如链烷烃的异构化和芳族化合物的烷基化。

6. 发明授权

US5329059A Alkylaromatic disproportionation 失效
标题翻译：烷基芳族歧化
公开(公告)号：US5329059A
公开(公告)日：1994-07-12
申请号：US86256
申请日：1993-07-06
申请人： David O. Marler
发明人： David O. Marler
IPC分类号： B01J29/06 , C07B61/00 , C07C6/12 , C07C15/02 , C07C5/52
CPC分类号： C07C6/123
摘要： A process is provided for disproportionation of an alkylaromatic compound, alkyl being from 1 to about 6 carbon atoms, e.g., toluene and methylnaphthalene, comprising contacting said compound with catalyst comprising an active form of synthetic porous crystalline MCM-49.
摘要翻译：提供了用于歧化烷基芳族化合物，1至约6个碳原子的烷基，例如甲苯和甲基萘的方法，包括使所述化合物与包含活性形式的合成多孔结晶MCM-49的催化剂接触。

7. 发明授权

US5173278A Denitrification of flue gas from catalytic cracking 失效
标题翻译：烟气从催化裂化中脱氮
公开(公告)号：US5173278A
公开(公告)日：1992-12-22
申请号：US669821
申请日：1991-03-15
申请人： David O. Marler , Ajit V. Sapre , David S. Shihabi , Richard F. Socha , Scott A. Stevenson
发明人： David O. Marler , Ajit V. Sapre , David S. Shihabi , Richard F. Socha , Scott A. Stevenson
IPC分类号： B01D53/86 , C10G11/18
CPC分类号： B01D53/8625 , B01D53/8621 , C10G11/182 , B01D2257/408 , Y02P30/446
摘要： A flue gas that contains small amounts of both HCN and NO.sub.x, produced, for example, by catalyst regeneration in the fluid catalytic cracking of a petroleum gas oil, is readily denitrified by the catalyzed reaction that proceeds approximately according to:HCN+NO.fwdarw.N.sub.2 (gas)+CO+CO.sub.2 +H.sub.2 OIf the molar ratio of HCN to NO in the flue gas is about 1.0, e.g. in the range of about 0.8 to 1.2, effective denitrification is achieved without first changing the composition of the flue gas by contacting it with catalyst under conversion conditions including elevated temperature. If the molar ratio of HCN to NO exceeds 1.2, the ratio may be adjusted to about 1.0 to 1.1 by thermal or catalytic oxidation in the presence of oxygen gas, followed by catalytic denitrification. If the molar ratio is less than about 0.8, the effective molar ratio is adjusted to about 1.0 to 1.1 by adding NH.sub.3 gas, followed by denitirification. In all three instances an excessive content of carbon monoxide in the flue gas may be corrected by passing the denitrified flue gas to a CO-boiler.Catalysts for the denitrification reaction are described and exemplified by crystalline zeolites of the ZSM-5 type, and by vanadium oxide supported on titania.
摘要翻译：含有少量HCN和NOx的烟道气，例如通过在石油瓦斯油的流化催化裂化中的催化剂再生产生的烟气，可以通过大致按以下方式进行的催化反应脱氮：HCN + NO-> N2（气体）+ CO + CO2 + H2O如果烟气中HCN与NO的摩尔比为约1.0，在约0.8至1.2的范围内，无需首先在包括升高的温度的转化条件下将催化剂与催化剂接触，而不改变烟道气的组成，实现有效的脱氮。如果HCN与NO的摩尔比超过1.2，则在氧气存在下通过热或催化氧化将该比例调节至约1.0至1.1，然后进行催化反硝化。如果摩尔比小于约0.8，则通过加入NH 3气体将有效摩尔比调节至约1.0-1.1，然后进行脱硝。在所有三种情况下，可以通过将反硝化烟道气通过CO锅炉来校正烟道气中过量的一氧化碳。用于脱氮反应的催化剂通过ZSM-5型的结晶沸石和负载在二氧化钛上的氧化钒来描述和例示。

8. 发明授权

US5108969A Low acidity catalyst for conversion of paraffins to olefins and/or aromatics 失效
标题翻译：用于将烷烃转化为烯烃和/或芳族化合物的低酸度催化剂
公开(公告)号：US5108969A
公开(公告)日：1992-04-28
申请号：US571470
申请日：1990-08-22
申请人： Kenneth J. Del Rossi , Ralph M. Dessau , Albin Huss, Jr. , Garry W. Kirker , David O. Marler , Randall D. Partridge
发明人： Kenneth J. Del Rossi , Ralph M. Dessau , Albin Huss, Jr. , Garry W. Kirker , David O. Marler , Randall D. Partridge
IPC分类号： B01J29/04 , C07C2/12 , C07C5/41
CPC分类号： C07C5/41 , B01J29/04 , C07C2/12 , C07C2529/04 , C07C2529/70
摘要： A low acidity Group VIII metal-containing zeolite MCM-22 catalyst, said zeolite exhibiting an Alpha value of not greater than about 150, is provided for conversion of aliphatic C.sub.2 to C.sub.12 hydrocarbon(s) to olefin(s) and/or aromatic(s).
摘要翻译：提供了低含量的含VIII族金属的沸石MCM-22催化剂，所述沸石表现出不大于约150的α值，用于将脂族C2转化为C12烃到烯烃和/或芳族（ s）。

9. 发明授权

US5073655A Method for preparing diarylalkanes 失效
标题翻译：二芳基烷烃的制备方法
公开(公告)号：US5073655A
公开(公告)日：1991-12-17
申请号：US559242
申请日：1990-07-27
申请人： Philip J. Angevine , Ivy D. Johnson , David O. Marler , John P. McWilliams
发明人： Philip J. Angevine , Ivy D. Johnson , David O. Marler , John P. McWilliams
IPC分类号： B01J29/04 , C07C2/12
CPC分类号： B01J29/04 , C07C2/12 , C07C2529/70
摘要： Diarylalkanes are prepared by alkylating an aromatic hydrocarbon with an aromatic alkylation agent in the presence of a synthetic porous crystalline material catalyst composition. The aromatic hydrocarbon can be, for example, benzene, toluene, naphthalene, etc. The aromatic alkylating agent can be an aromatic compound with a hydroxy group, such as phenol, or benzyl alcohol, or an aromatic halide, aldehyde, ether, or an aromatic olefin such as styrene.
摘要翻译：二芳基烷烃通过在合成的多孔结晶材料催化剂组合物的存在下用芳族烷基化剂烷基化芳族烃来制备。芳族烃可以是例如苯，甲苯，萘等。芳族烷基化剂可以是具有羟基的芳香族化合物，例如苯酚或苄醇，或芳族卤化物，醛，醚或芳族烯烃如苯乙烯。

10. 发明授权

US5063038A Zeolite synthesis using an alcohol or like molecule 失效
标题翻译：使用醇或类似分子的沸石合成
公开(公告)号：US5063038A
公开(公告)日：1991-11-05
申请号：US91612
申请日：1987-08-31
申请人： Garry W. Kirker , Donald J. Klocke , James C. Vartuli , Pochen Chu , David O. Marler , John P. McWilliams
发明人： Garry W. Kirker , Donald J. Klocke , James C. Vartuli , Pochen Chu , David O. Marler , John P. McWilliams
IPC分类号： B01J29/40 , B01J29/65 , B01J29/70 , C01B39/48 , C07C2/66 , C07C4/18
CPC分类号： C07C4/18 , B01J29/40 , B01J29/65 , B01J29/7046 , C01B39/48 , C07C2/66 , B01J2229/20 , B01J2229/26 , B01J2229/36 , B01J2229/42 , C07C2529/65 , C07C2529/70 , Y10S423/35 , Y10S423/36
摘要： There is provided a method for preparing a zeolite other than ZSM-5 from a reaction mixture comprising a mixed organic directing agent which is a combination of (a) an organic nitrogen containing compound such as an amine or a quaternary ammonium compound and (b) an alcohol and/or diol. Particular zeolites synthesized by this method include ZSM-22 and ZSM-23. The use of an alcohol or a diol may inhibit the coformation of ZSM-5. Especially when used to prepare ZSM-23, this method enables the preparation of more catalytically active ZSM-23 of reduced crystallite size and also enables the use of lower crystallization temperatures. Particular mixed organic directing agents for the preparation of ZSM-23 are combination of (a) pyrrolidine and (b) ethanol or ethylene glycol. Other factors which enhance the activity of ZSM-23 include the use of the following in the reaction mixtures for preparing ZSM-23: potassium ions; precipitated silica particles as sources of silica; and spray dried precipitated silica/alumina particles as sources of silica and alumina. The catalytic stability of alumina bound ZSM-23 catalysts is especially enhanced by steaming. Particular reactions which can be catalyzed by ZSM-23 made according to methods described herein include the dealkylation of ethylbenzene and the alkylation of benzene with ethylene.
摘要翻译：提供了一种从含有（a）有机氮化合物如胺或季铵化合物的组合的混合有机导向剂的反应混合物制备ZSM-5以外的沸石的方法，（b）醇和/或二醇。通过该方法合成的特定沸石包括ZSM-22和ZSM-23。使用醇或二醇可能会抑制ZSM-5的共形。特别是当用于制备ZSM-23时，该方法能够制备更小的微晶尺寸的更具催化活性的ZSM-23，并且还能够使用较低的结晶温度。用于制备ZSM-23的特殊混合有机导向剂是（a）吡咯烷和（b）乙醇或乙二醇的组合。提高ZSM-23活性的其他因素包括在制备ZSM-23：钾离子的反应混合物中使用以下物质：沉淀二氧化硅颗粒作为二氧化硅来源; 和喷雾干燥的沉淀二氧化硅/氧化铝颗粒作为二氧化硅和氧化铝的来源。氧化铝结合的ZSM-23催化剂的催化稳定性通过蒸汽特别提高。根据本文所述方法制备的可以由ZSM-23催化的特定反应包括乙苯的脱烷基化和苯与乙烯的烷基化。

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