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1. 发明授权

US08677762B2 Combined production of hydrocarbons and electrical power 有权
标题翻译：组合生产碳氢化合物和电力
公开(公告)号：US08677762B2
公开(公告)日：2014-03-25
申请号：US12674272
申请日：2008-08-13
申请人： Poul Erik Højlund Nielsen , Thomas Rostrup-Nielsen , Bodil Voss , Finn Joensen
发明人： Poul Erik Højlund Nielsen , Thomas Rostrup-Nielsen , Bodil Voss , Finn Joensen
IPC分类号： F02C6/18
CPC分类号： C07C29/1518 , C07C41/01 , C10G3/42 , C10G2300/1022 , C10G2400/02 , Y02E20/14 , Y02P30/20 , C07C31/04 , C07C43/043
摘要： A process for the preparation of hydrocarbon products and for the generation of power that includes the steps of (a) providing a synthesis gas having a hydrogen to carbon monoxide ratio of between 0.1 and 1; (b) contacting the synthesis gas with one or more catalysts which together catalyse a reaction of hydrogen and carbon monoxide to oxygenates comprising methanol and dimethyl ether with a dimethyl ether to methanol ratio of higher than 2 and a carbon dioxide content of above 20 mole %; (c) contacting the carbon dioxide containing oxygenate mixture at an inlet temperature of between 240° and 4000° C. with a catalyst being active in the conversion of oxygenate to higher hydrocarbons and a tail gas being rich in carbon dioxide; (d) combusting the carbon dioxide rich tail gas in a gas turbine combustion chamber to flue gas; and (e) expanding the flue gas stream through a gas turbine for the generation of power.
摘要翻译：一种用于制备烃产物和产生动力的方法，包括以下步骤：（a）提供氢与一氧化碳比为0.1至1的合成气; （b）使合成气与一种或多种催化剂接触，这些催化剂一起催化氢和一氧化碳与包含甲醇和二甲醚的含氧化合物的反应，甲醚与甲醇的比例高于2，二氧化碳含量高于20摩尔％ ; （c）在240℃和4000℃之间的入口温度下与含氧化合物混合物的接触与在含氧化合物转化为高级烃和富含二氧化碳的尾气中具有活性的催化剂接触; （d）将燃气轮机燃烧室中的富含二氧化碳的尾气燃烧成烟道气; 和（e）通过用于发电的燃气轮机扩大烟气流。

2. 发明授权

US08038906B2 Process for the preparation of synthesis gas from black liquor 有权
标题翻译：从黑液制备合成气的方法
公开(公告)号：US08038906B2
公开(公告)日：2011-10-18
申请号：US12431240
申请日：2009-04-28
申请人： Poul Erik Højlund Nielsen , Bodil Voss
发明人： Poul Erik Højlund Nielsen , Bodil Voss
IPC分类号： D21C11/00 , C10J3/46 , C01B3/24
CPC分类号： C01B3/36 , C01B3/32 , C01B3/50 , C01B3/52 , C01B2203/0415 , C01B2203/047 , C01B2203/0475 , C07C41/01 , D21C11/125 , C07C43/043
摘要： A process for the adjustment of the composition of a synthesis gas produced in a high temperature black liquor gasifier. The process includes the steps of (a) generating a gasifier effluent stream from black liquor in the gasifier by a blast and optionally an atomising stream; (b) optionally quenching the gasifier effluent stream with a gas stream to form a gas quenched effluent stream; (c) quenching the gasifier effluent of step (a) or the gas quenched effluent gas stream of step (b) with a water stream to form a raw synthesis gas; (d) further cooling and cleaning and separating the raw synthesis gas to form a purified unprocessed synthesis gas with an appropriate H2/CO ratio; (e) partly converting the purified synthesis gas to dimethyl ether in a synthesis section, producing at least a product stream of DME and a hydrogen rich purge stream of processed; (f) splitting and recycling individual or combinations of split streams of the processed or the unprocessed synthesis gas to step a and/or step (b); and recycling a by-product stream of CO2 being further generated in step (e) in part or completely to step (a) and/or step (b).
摘要翻译：用于调节在高温黑液气化器中生产的合成气的组成的方法。该方法包括以下步骤：（a）通过鼓风和任选的雾化流从气化器中的黑液生成气化器流出物流; （b）任选地用气流骤冷气化器流出物流以形成气体骤冷流出物流; （c）用水流淬火步骤（a）的气化器流出物或步骤（b）的气体骤冷流出物气流，以形成原始合成气; （d）进一步冷却和清洗并分离原始合成气以形成具有合适H 2 / CO比的纯化未加工合成气; （e）在合成部分中部分地将纯化的合成气转化为二甲醚，至少产生DME的产物流和加氢的富氢吹扫流; （f）将经处理或未经处理的合成气的分流或分离流分离和回收到步骤a和/或步骤（b）; 并且在步骤（e）中再次产生副产物二氧化碳流，部分或完全是步骤（a）和/或步骤（b）。

3. 发明申请

US20110314834A1 COMBINED PRODUCTION OF HYDROCARBONS AND ELECTRICAL POWER 有权
标题翻译：联合生产碳氢化合物和电力
公开(公告)号：US20110314834A1
公开(公告)日：2011-12-29
申请号：US12674272
申请日：2008-08-13
申请人： Poul Erik Højlund Nielsen , Thomas Rostrup-Nielsen , Bodil Voss , Finn Joensen
发明人： Poul Erik Højlund Nielsen , Thomas Rostrup-Nielsen , Bodil Voss , Finn Joensen
IPC分类号： F02C6/18
CPC分类号： C07C29/1518 , C07C41/01 , C10G3/42 , C10G2300/1022 , C10G2400/02 , Y02E20/14 , Y02P30/20 , C07C31/04 , C07C43/043
摘要： A process for the preparation of hydrocarbon products and for the generation of power comprising the steps of (a) providing a synthesis gas having a hydrogen to carbon monoxide ratio of between 0.1 and 1; (b) contacting the synthesis gas with one or more catalysts which together catalyse a reaction of hydrogen and carbon monoxide to oxygenates comprising methanol and dimethyl ether with a dimethyl ether to methanol ratio of higher than 2 and a carbon dioxide content of above 20 mole %; (c) contacting the carbon dioxide containing oxygenate mixture at an inlet temperature of between 240 and 4000 C with a catalyst being active in the conversion of oxygenate to higher hydrocarbons and a tail gas being rich in carbon dioxide; (d) combusting the carbon dioxide rich tail gas, optionally admixed with fresh carbon monoxide rich synthesis gas in a gas turbine combustion chamber to flue gas; and (e) expanding the flue gas stream through a gas turbine for the generation of power.
摘要翻译：一种用于制备烃产物和产生动力的方法，包括以下步骤：（a）提供氢与一氧化碳比为0.1至1的合成气; （b）使合成气与一种或多种催化剂接触，这些催化剂一起催化氢和一氧化碳与包含甲醇和二甲醚的含氧化合物的反应，甲醚与甲醇的比例高于2，二氧化碳含量高于20摩尔％ ; （c）在240至4000℃的入口温度下使含二氧化碳混合物与含氧化合物转化为高级烃和富含二氧化碳的尾气有活性的催化剂接触; （d）燃烧富含二氧化碳的尾气，任选地与燃气轮机燃烧室中的新鲜的富含一氧化碳的合成气混合成烟道气; 和（e）通过用于发电的燃气轮机扩大烟气流。

4. 发明授权

US09255227B2 Process for the synthesis of hydrocarbon constituents of gasoline 有权
标题翻译：合成汽油烃成分的方法
公开(公告)号：US09255227B2
公开(公告)日：2016-02-09
申请号：US12518616
申请日：2007-11-20
申请人： Finn Joensen , Poul Erik Højlund Nielsen , Niels Christian Schiødt , Ton V. W. Janssens , Bodil Voss
发明人： Finn Joensen , Poul Erik Højlund Nielsen , Niels Christian Schiødt , Ton V. W. Janssens , Bodil Voss
IPC分类号： C07C1/20 , C10G3/00
CPC分类号： C10G3/49 , C10G2300/1011 , C10G2300/1022 , C10G2300/805 , C10G2400/02 , C10G2400/20 , Y02P30/20
摘要： Process for the synthesis of hydrocarbon constituents of gasoline comprising catalytic conversion in a gasoline synthesis step of an oxygenate-containing feed comprising methanol and/or dimethyl ether and a mixture of at least on a total oxygenate basis 0.05 wt % C3+ higher alcohols and/or their oxygenate equivalents to hydrocarbon constituents of gasoline.
摘要翻译：在包含甲醇和/或二甲醚的含氧化合物进料的汽油合成步骤和至少在总含氧化合物基础上的混合物，基于0.05重量％的C3 +高级醇和/或它们的含氧化合物等同于汽油的烃成分。

5. 发明申请

US20110137074A1 PROCESS FOR THE PRODUCTION OF ACETIC ACID ETHYLENE AND VINYL ACETATE MONOMER 有权
标题翻译：乙酸乙烯酯和乙酸乙烯酯单体的生产方法
公开(公告)号：US20110137074A1
公开(公告)日：2011-06-09
申请号：US12963402
申请日：2010-12-08
申请人： Bodil Voss , Rachid Mabrouk , Claus Hviid Christensen
发明人： Bodil Voss , Rachid Mabrouk , Claus Hviid Christensen
IPC分类号： C07C67/54
CPC分类号： C07C67/055 , C07C1/24 , C07C67/05 , C07C2521/04 , C07C2523/06 , C07C2523/34 , C07C2523/745 , Y02P20/125 , C07C11/04 , C07C69/01 , C07C69/15
摘要： An integrated process for the production of acetic acid, ethylene and vinyl acetate monomer comprising the steps of: (a) evaporating at least part of an ethanol feed stock (b) producing in a first reaction zone a first product stream comprising acetic acid by oxidative or partly oxidative dehydrogenation of ethanol feed stock; (c) producing in a second reaction zone a second product stream comprising ethylene from an ethanol feed stock; (d) reacting in a third reaction zone an acetic acid reaction stream containing at least a portion of the acetic acid from the first reaction zone with an ethylene reaction stream containing at least a portion of the ethylene product from the second reaction zone and with oxygen to a third product stream comprising vinyl acetate monomer; (e) passing at least a portion of the third product stream to a distillation section and isolating at least a portion of the vinyl acetate monomer; (f) supplying at least part of reaction heat from the third reaction zone to provide heat for evaporating at least part of the ethanol feed stock in step (a); (g) supplying at least part of reaction heat from the first reaction zone to provide heat for producing the second product stream in the second reaction zone in step (c) and for distilling of the third product stream in the distillation section in step (e).
摘要翻译：一种用于生产乙酸，乙烯和乙酸乙烯酯单体的综合方法，包括以下步骤：（a）蒸发至少部分乙醇原料（b），在第一反应区产生包含乙酸的第一产物流，通过氧化或部分氧化脱氢乙醇饲料; （c）在第二反应区中产生包含来自乙醇原料的乙烯的第二产物流; （d）在第三反应区中使含有至少一部分来自第一反应区的乙酸的乙酸反应流与含有至少一部分来自第二反应区的乙烯产物和乙烯反应区的乙烯反应流反应，包含乙酸乙烯酯单体的第三产物流; （e）将第三产物流的至少一部分通入蒸馏段并分离至少一部分乙酸乙烯酯单体; （f）从第三反应区供应反应热的至少一部分以提供热量，用于在步骤（a）中蒸发至少部分乙醇原料; （g）从步骤（c）中提供来自第一反应区的反应热的至少一部分以提供热量以产生第二反应区中的第二产物流，并在步骤（e）中蒸馏蒸馏段中的第三产物流）。

6. 发明申请

US20100036186A1 PROCESS FOR THE SYNTHESIS OF HYDROCARBON CONSTITUENTS OF GASOLINE 有权
标题翻译：汽油组合物合成方法
公开(公告)号：US20100036186A1
公开(公告)日：2010-02-11
申请号：US12518616
申请日：2007-11-20
申请人： Finn Joensen , Poul Erik Hojlund Nielsen , Niels Christian Schiodt , Ton V.W. Janssens , Bodil Voss
发明人： Finn Joensen , Poul Erik Hojlund Nielsen , Niels Christian Schiodt , Ton V.W. Janssens , Bodil Voss
IPC分类号： C07C1/20
CPC分类号： C10G3/49 , C10G2300/1011 , C10G2300/1022 , C10G2300/805 , C10G2400/02 , C10G2400/20 , Y02P30/20
摘要： Process for the synthesis of hydrocarbon constituents of gasoline comprising catalytic conversion in a gasoline synthesis step of an oxygenate-containing feed comprising methanol and/or dimethyl ether and a mixture of at least on a total oxygenate basis 0.05 wt % C3+ higher alcohols and/or their oxygenate equivalents to hydrocarbon constituents of gasoline.
摘要翻译：在包含甲醇和/或二甲醚的含氧化合物进料的汽油合成步骤和至少在总含氧化合物基础上的混合物，基于0.05重量％的C3 +高级醇和/或它们的含氧化合物等同于汽油的烃成分。

7. 发明授权

US08471060B2 Process and reactor for the thermoneutral conversion of ethanol to acetic acid 有权
标题翻译：将乙醇热转化为乙酸的方法和反应器
公开(公告)号：US08471060B2
公开(公告)日：2013-06-25
申请号：US12624019
申请日：2009-11-23
申请人： Claus Hviid Christensen , Niels Christian Schiødt , Bodil Voss
发明人： Claus Hviid Christensen , Niels Christian Schiødt , Bodil Voss
IPC分类号： C07C51/00
CPC分类号： C07C45/38 , B01J8/04 , C07C51/235 , C07C47/06 , C07C53/08
摘要： A process and reactor for the production of acetic acid comprising the steps of: passing a feed stream containing ethanol and water together with a predetermined feed rate of an oxygen containing atmosphere in presence of one or more catalysts being active in simultaneous non-oxidative and oxidative conversion of ethanol to a product stream with acetic acid; recovering from the product stream a stream of acetic acid; optionally recovering reactive derivatives of acetic acid and recycling these to step (a).
摘要翻译：一种用于生产乙酸的方法和反应器，包括以下步骤：在一种或多种催化剂的存在下，使含有乙醇和水的进料流与预定的含氧气氛的进料速率一起通过同时进行的非氧化和氧化用乙酸将乙醇转化成产物流; 从产物流中回收乙酸流; 任选地回收乙酸的活性衍生物并将其再循环到步骤（a）。

8. 发明授权

US6059995A Process and preparation of hydrogen-rich gas 失效
标题翻译：富氢气体的处理和制备
公开(公告)号：US6059995A
公开(公告)日：2000-05-09
申请号：US233116
申请日：1999-01-19
申请人： Haldor F. A. Topsoe , Ib Dybkj.ae butted.r , Poul Erik Nielsen , Bodil Voss
发明人： Haldor F. A. Topsoe , Ib Dybkj.ae butted.r , Poul Erik Nielsen , Bodil Voss
IPC分类号： B01J19/00 , B01J23/38 , C01B3/02 , C01B3/32 , C01C1/04 , C07C273/04 , C07C1/02 , C01B31/18 , C01B31/20
CPC分类号： C01B3/025 , C01B3/323 , C01B3/326 , C01B2203/1064 , C01B2203/1076 , Y02P20/142 , Y02P20/52
摘要： A process for the production of hydrogen rich gas from a feedstock containing dimethyl ether and/or methanol by steam reforming dimethyl ether in presence of a reforming catalyst to a product gas being rich in hydrogen, wherein necessary heat for the endothermic steam reforming reactions is supplied through oxidation of part of the hydrogen contained in the steam reformed feedstock process in heat conducting relationship with the steam reforming reactions.
摘要翻译：在重整催化剂存在下，通过蒸汽重整二甲醚在含有二甲醚和/或甲醇的原料中生产富氢气体的方法，其中富含氢气的产物气体被供应，其中供给吸热蒸汽重整反应所需的热量通过蒸汽重整原料过程中包含的部分氢气与蒸汽重整反应导热的关系。

9. 发明授权

US08440855B2 Process for the production of acetic acid ethylene and vinyl acetate monomer 有权
标题翻译：乙酸乙酸乙烯酯单体生产方法
公开(公告)号：US08440855B2
公开(公告)日：2013-05-14
申请号：US12963402
申请日：2010-12-08
申请人： Bodil Voss , Rachid Mabrouk , Claus Hviid Christensen
发明人： Bodil Voss , Rachid Mabrouk , Claus Hviid Christensen
IPC分类号： C07C67/04
CPC分类号： C07C67/055 , C07C1/24 , C07C67/05 , C07C2521/04 , C07C2523/06 , C07C2523/34 , C07C2523/745 , Y02P20/125 , C07C11/04 , C07C69/01 , C07C69/15
摘要： An integrated process for the production of acetic acid, ethylene and vinyl acetate monomer comprising the steps of: (a) evaporating at least part of an ethanol feed stock (b) producing in a first reaction zone a first product stream comprising acetic acid by oxidative or partly oxidative dehydrogenation of ethanol feed stock; (c) producing in a second reaction zone a second product stream comprising ethylene from an ethanol feed stock; (d) reacting in a third reaction zone an acetic acid reaction stream containing at least a portion of the acetic acid from the first reaction zone with an ethylene reaction stream containing at least a portion of the ethylene product from the second reaction zone and with oxygen to a third product stream comprising vinyl acetate monomer; (e) passing at least a portion of the third product stream to a distillation section and isolating at least a portion of the vinyl acetate monomer; (f) supplying at least part of reaction heat from the third reaction zone to provide heat for evaporating at least part of the ethanol feed stock in step (a); (g) supplying at least part of reaction heat from the first reaction zone to provide heat for producing the second product stream in the second reaction zone in step (c) and for distilling of the third product stream in the distillation section in step (e).
摘要翻译：一种用于生产乙酸，乙烯和乙酸乙烯酯单体的综合方法，包括以下步骤：（a）蒸发至少部分乙醇原料（b），在第一反应区产生包含乙酸的第一产物流，通过氧化或部分氧化脱氢乙醇饲料; （c）在第二反应区中产生包含来自乙醇原料的乙烯的第二产物流; （d）在第三反应区中使含有至少一部分来自第一反应区的乙酸的乙酸反应流与含有至少一部分来自第二反应区的乙烯产物和乙烯反应区的乙烯反应流反应，包含乙酸乙烯酯单体的第三产物流; （e）将第三产物流的至少一部分通入蒸馏段并分离至少一部分乙酸乙烯酯单体; （f）从第三反应区供应反应热的至少一部分以提供热量，用于在步骤（a）中蒸发至少部分乙醇原料; （g）从步骤（c）中提供来自第一反应区的反应热的至少一部分以提供热量以产生第二反应区中的第二产物流，并在步骤（e）中蒸馏蒸馏段中的第三产物流）。

10. 发明授权

US5908963A Preparation of fuel grade dimethyl ether 失效
标题翻译：燃料级二甲醚的制备
公开(公告)号：US5908963A
公开(公告)日：1999-06-01
申请号：US894066
申请日：1997-12-12
申请人： Bodil Voss , Finn Joensen , John Bogild Hansen
发明人： Bodil Voss , Finn Joensen , John Bogild Hansen
IPC分类号： C07C41/09 , C07C41/01 , C07C41/42 , C07C43/04 , C10L1/02 , C07C41/00 , C07C27/00
CPC分类号： C07C41/01
摘要： A process for the preparation of dimethyl ether. The process prepares fuel grade dimethyl ether from a hydrogen and carbon oxides synthesis gas.
摘要翻译： PCT No.PCT / DK96 / 00047 Sec。 371日期1997年12月12日 102（e）日期1997年12月12日PCT 1996年1月29日PCT PCT。公开号WO96 / 23755 日期1996年8月8日制备二甲醚的方法。该方法由氢和碳氧化物合成气制备燃料级二甲醚。

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