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1. 发明授权

US08471060B2 Process and reactor for the thermoneutral conversion of ethanol to acetic acid 有权
标题翻译：将乙醇热转化为乙酸的方法和反应器
公开(公告)号：US08471060B2
公开(公告)日：2013-06-25
申请号：US12624019
申请日：2009-11-23
申请人： Claus Hviid Christensen , Niels Christian Schiødt , Bodil Voss
发明人： Claus Hviid Christensen , Niels Christian Schiødt , Bodil Voss
IPC分类号： C07C51/00
CPC分类号： C07C45/38 , B01J8/04 , C07C51/235 , C07C47/06 , C07C53/08
摘要： A process and reactor for the production of acetic acid comprising the steps of: passing a feed stream containing ethanol and water together with a predetermined feed rate of an oxygen containing atmosphere in presence of one or more catalysts being active in simultaneous non-oxidative and oxidative conversion of ethanol to a product stream with acetic acid; recovering from the product stream a stream of acetic acid; optionally recovering reactive derivatives of acetic acid and recycling these to step (a).
摘要翻译：一种用于生产乙酸的方法和反应器，包括以下步骤：在一种或多种催化剂的存在下，使含有乙醇和水的进料流与预定的含氧气氛的进料速率一起通过同时进行的非氧化和氧化用乙酸将乙醇转化成产物流; 从产物流中回收乙酸流; 任选地回收乙酸的活性衍生物并将其再循环到步骤（a）。

2. 发明申请

US20100130776A1 PROCESS AND REACTOR FOR THE THERMONEUTRAL CONVERSION OF ETHANOL TO ACETIC ACID 有权
标题翻译：乙醇转化为乙酸的方法和反应物
公开(公告)号：US20100130776A1
公开(公告)日：2010-05-27
申请号：US12624019
申请日：2009-11-23
申请人： Claus Hviid Christensen , Niels Christian Schiødt , Bodil Voss
发明人： Claus Hviid Christensen , Niels Christian Schiødt , Bodil Voss
IPC分类号： C07C51/235 , B01J8/04
CPC分类号： C07C45/38 , B01J8/04 , C07C51/235 , C07C47/06 , C07C53/08
摘要： A process and reactor for the production of acetic acid comprising the steps of: passing a feed stream containing ethanol and water together with a predetermined feed rate of an oxygen containing atmosphere in presence of one or more catalysts being active in simultaneous non-oxidative and oxidative conversion of ethanol to a product stream with acetic acid; recovering from the product stream a stream of acetic acid; optionally recovering reactive derivatives of acetic acid and recycling these to step (a).
摘要翻译：一种用于生产乙酸的方法和反应器，包括以下步骤：在一种或多种催化剂的存在下，使含有乙醇和水的进料流与预定的含氧气氛的进料速率一起通过同时进行的非氧化和氧化用乙酸将乙醇转化成产物流; 从产物流中回收乙酸流; 任选地回收乙酸的活性衍生物并将其再循环到步骤（a）。

3. 发明授权

US08440855B2 Process for the production of acetic acid ethylene and vinyl acetate monomer 有权
标题翻译：乙酸乙酸乙烯酯单体生产方法
公开(公告)号：US08440855B2
公开(公告)日：2013-05-14
申请号：US12963402
申请日：2010-12-08
申请人： Bodil Voss , Rachid Mabrouk , Claus Hviid Christensen
发明人： Bodil Voss , Rachid Mabrouk , Claus Hviid Christensen
IPC分类号： C07C67/04
CPC分类号： C07C67/055 , C07C1/24 , C07C67/05 , C07C2521/04 , C07C2523/06 , C07C2523/34 , C07C2523/745 , Y02P20/125 , C07C11/04 , C07C69/01 , C07C69/15
摘要： An integrated process for the production of acetic acid, ethylene and vinyl acetate monomer comprising the steps of: (a) evaporating at least part of an ethanol feed stock (b) producing in a first reaction zone a first product stream comprising acetic acid by oxidative or partly oxidative dehydrogenation of ethanol feed stock; (c) producing in a second reaction zone a second product stream comprising ethylene from an ethanol feed stock; (d) reacting in a third reaction zone an acetic acid reaction stream containing at least a portion of the acetic acid from the first reaction zone with an ethylene reaction stream containing at least a portion of the ethylene product from the second reaction zone and with oxygen to a third product stream comprising vinyl acetate monomer; (e) passing at least a portion of the third product stream to a distillation section and isolating at least a portion of the vinyl acetate monomer; (f) supplying at least part of reaction heat from the third reaction zone to provide heat for evaporating at least part of the ethanol feed stock in step (a); (g) supplying at least part of reaction heat from the first reaction zone to provide heat for producing the second product stream in the second reaction zone in step (c) and for distilling of the third product stream in the distillation section in step (e).
摘要翻译：一种用于生产乙酸，乙烯和乙酸乙烯酯单体的综合方法，包括以下步骤：（a）蒸发至少部分乙醇原料（b），在第一反应区产生包含乙酸的第一产物流，通过氧化或部分氧化脱氢乙醇饲料; （c）在第二反应区中产生包含来自乙醇原料的乙烯的第二产物流; （d）在第三反应区中使含有至少一部分来自第一反应区的乙酸的乙酸反应流与含有至少一部分来自第二反应区的乙烯产物和乙烯反应区的乙烯反应流反应，包含乙酸乙烯酯单体的第三产物流; （e）将第三产物流的至少一部分通入蒸馏段并分离至少一部分乙酸乙烯酯单体; （f）从第三反应区供应反应热的至少一部分以提供热量，用于在步骤（a）中蒸发至少部分乙醇原料; （g）从步骤（c）中提供来自第一反应区的反应热的至少一部分以提供热量以产生第二反应区中的第二产物流，并在步骤（e）中蒸馏蒸馏段中的第三产物流）。

4. 发明申请

US20110137074A1 PROCESS FOR THE PRODUCTION OF ACETIC ACID ETHYLENE AND VINYL ACETATE MONOMER 有权
标题翻译：乙酸乙烯酯和乙酸乙烯酯单体的生产方法
公开(公告)号：US20110137074A1
公开(公告)日：2011-06-09
申请号：US12963402
申请日：2010-12-08
申请人： Bodil Voss , Rachid Mabrouk , Claus Hviid Christensen
发明人： Bodil Voss , Rachid Mabrouk , Claus Hviid Christensen
IPC分类号： C07C67/54
CPC分类号： C07C67/055 , C07C1/24 , C07C67/05 , C07C2521/04 , C07C2523/06 , C07C2523/34 , C07C2523/745 , Y02P20/125 , C07C11/04 , C07C69/01 , C07C69/15
摘要： An integrated process for the production of acetic acid, ethylene and vinyl acetate monomer comprising the steps of: (a) evaporating at least part of an ethanol feed stock (b) producing in a first reaction zone a first product stream comprising acetic acid by oxidative or partly oxidative dehydrogenation of ethanol feed stock; (c) producing in a second reaction zone a second product stream comprising ethylene from an ethanol feed stock; (d) reacting in a third reaction zone an acetic acid reaction stream containing at least a portion of the acetic acid from the first reaction zone with an ethylene reaction stream containing at least a portion of the ethylene product from the second reaction zone and with oxygen to a third product stream comprising vinyl acetate monomer; (e) passing at least a portion of the third product stream to a distillation section and isolating at least a portion of the vinyl acetate monomer; (f) supplying at least part of reaction heat from the third reaction zone to provide heat for evaporating at least part of the ethanol feed stock in step (a); (g) supplying at least part of reaction heat from the first reaction zone to provide heat for producing the second product stream in the second reaction zone in step (c) and for distilling of the third product stream in the distillation section in step (e).
摘要翻译：一种用于生产乙酸，乙烯和乙酸乙烯酯单体的综合方法，包括以下步骤：（a）蒸发至少部分乙醇原料（b），在第一反应区产生包含乙酸的第一产物流，通过氧化或部分氧化脱氢乙醇饲料; （c）在第二反应区中产生包含来自乙醇原料的乙烯的第二产物流; （d）在第三反应区中使含有至少一部分来自第一反应区的乙酸的乙酸反应流与含有至少一部分来自第二反应区的乙烯产物和乙烯反应区的乙烯反应流反应，包含乙酸乙烯酯单体的第三产物流; （e）将第三产物流的至少一部分通入蒸馏段并分离至少一部分乙酸乙烯酯单体; （f）从第三反应区供应反应热的至少一部分以提供热量，用于在步骤（a）中蒸发至少部分乙醇原料; （g）从步骤（c）中提供来自第一反应区的反应热的至少一部分以提供热量以产生第二反应区中的第二产物流，并在步骤（e）中蒸馏蒸馏段中的第三产物流）。

5. 发明申请

US20090313976A1 Method of Storing and Delivering Ammonia and the Use of Electromagnetic Radiation for Desorption of Ammonia from a Chemical Complex 有权
标题翻译：存储和提供氨的方法和使用电磁辐射从化学配合物中解吸氨
公开(公告)号：US20090313976A1
公开(公告)日：2009-12-24
申请号：US12279233
申请日：2002-02-27
申请人： Tue Johannessen , Rasmus Zink Sørensen , Claus Hviid Christensen , Ulrich Quaade , Jens Kehlet Nørskov , Henning Schmidt
发明人： Tue Johannessen , Rasmus Zink Sørensen , Claus Hviid Christensen , Ulrich Quaade , Jens Kehlet Nørskov , Henning Schmidt
IPC分类号： B01D53/90 , F17C9/02 , F17C11/00 , F01N3/20
CPC分类号： G09F19/22 , B01D53/90 , B01D53/9431 , B01D2251/2062 , B01D2259/80 , B01D2259/802 , B01D2259/804 , B01D2259/806 , B01J20/046 , B01J20/3433 , B01J20/3441 , C01C1/006 , F01N3/2066 , F01N2610/02 , F01N2610/06 , F01N2610/10 , F01N2610/1406 , G09F9/305 , G09F19/18 , Y02A50/2325 , Y02C20/10 , Y02T10/24
摘要： A method of storing and delivering ammonia and the use of electromagnetic radiation for desorption of ammonia from a chemical complex. Solid metal ammine complexes are applied for safe and high-density storage of ammonia to be released for use as reducing agent in selective catalytic reduction of NOx in exhaust gases. The compositional formula of the metal ammine complexes is M(NH3)nXz, where M2+ represents one or more metal ions capable of binding ammonia, X represents one or more anions, n is the coordination number (from 2 to 12), and z the valency of the metal ion (and thus the total number of compensating anion charges). Ammonia is released non-thermally by photon-activation using electromagnetic irradiation of the complex bond between ammonia coordinated to the metal ion
摘要翻译：一种储存和输送氨的方法，以及使用电磁辐射从化学络合物中解氨的方法。应用固体金属氨络合物用于安全和高密度地储存氨，以用作废气中选择性催化还原NOx的还原剂。金属络合物的组成式为M（NH 3）n X z，其中M 2 +表示一个或多个能结合氨的金属离子，X表示一个或多个阴离子，n为配位数（2至12），z为金属离子的化合价（因此补偿阴离子电荷的总数）。通过使用与金属离子配位的氨之间的复合键的电磁照射，通过光子激活而非热释放氨

6. 发明申请

US20110060174A1 CATALYST, A PROCESS FOR SELECTIVE HYDROGENATION OF ACETYLENE TO ETHYLENE AND A METHOD FOR THE MANUFACTURE OF THE CATALYST 审中-公开
标题翻译：催化剂，乙烯选择性氢化成乙烯的方法和制备催化剂的方法
公开(公告)号：US20110060174A1
公开(公告)日：2011-03-10
申请号：US12811801
申请日：2009-01-07
申请人： Felix Studt , Jens Kehlet Nørskov , Claus Hviid Christensen , Rasmus Zink Sørensen , Frank Abild-Pedersen , Thomas Bligaard
发明人： Felix Studt , Jens Kehlet Nørskov , Claus Hviid Christensen , Rasmus Zink Sørensen , Frank Abild-Pedersen , Thomas Bligaard
IPC分类号： B01J23/825 , C07C5/09
CPC分类号： B01J23/825 , B01J23/005 , B01J23/22 , B01J23/31 , B01J23/80 , B01J37/0201 , C07C5/09 , C07C7/167 , C07C2521/04 , C07C2521/06 , C07C2521/08 , C07C2521/10 , C07C2523/80 , C07C2523/825 , C07C2527/232 , C10G45/36 , Y02P20/52 , C07C11/04
摘要： Provided is a catalyst including a mixture of metal A selected from Fe, Co and Ni, and metal B selected from Zn and Ga, and a support material, where the two metals are present in an intermetallic composition; A method for the manufacture of the catalyst; and the use of the catalyst for the selective hydrogenation of acetylene to ethylene in a gas mixture including acetylenic impurities and hydrogen, and one or more of ethylene and carbon monoxide. The catalyst has a high selectivity and is based an easily available metal compounds.
摘要翻译：提供了包含选自Fe，Co和Ni的金属A和选自Zn和Ga的金属B的混合物的催化剂和其中两种金属存在于金属间组合物中的载体材料; 催化剂的制造方法; 以及催化剂用于在包括炔属杂质和氢气以及一种或多种乙烯和一氧化碳的气体混合物中乙炔选择性氢化成乙烯的用途。催化剂具有高选择性，并且是易于获得的金属化合物。

7. 发明授权

US07790776B2 Process and catalyst for hydrogenation of carbon oxides 有权
标题翻译：用于碳氧化物氢化的方法和催化剂
公开(公告)号：US07790776B2
公开(公告)日：2010-09-07
申请号：US12065166
申请日：2006-08-28
申请人： Claus Hviid Christensen , Martin Andersson , Arkady Kustov , Tue Johannesen , Thomas Bligaard , Kasper E. Larsen , Jens K. Nørskov , Jens Sehested
发明人： Claus Hviid Christensen , Martin Andersson , Arkady Kustov , Tue Johannesen , Thomas Bligaard , Kasper E. Larsen , Jens K. Nørskov , Jens Sehested
IPC分类号： C07C27/00
CPC分类号： B01J23/75 , B01J21/005 , B01J23/745 , B01J23/755 , B01J23/78 , B01J37/0201 , C07C1/044 , C07C2523/75 , C07C2523/755 , H01M8/0668 , C07C9/04
摘要： A process for hydrogenation of carbon oxides comprising contacting a gas mixture containing carbon oxides and of hydrogen with a catalyst comprising bimetallic iron-nickel or iron-cobalt alloys as the active catalytic material supported on a carrier of an oxide. The carrier is preferably formed to have a surface area greater than 20 m2/g.
摘要翻译：一种用于碳氧化物氢化的方法，包括使含有碳氧化物和氢气的气体混合物与包含双金属铁镍或铁 - 钴合金的催化剂作为负载在氧化物载体上的活性催化材料接触。载体优选形成为具有大于20m 2 / g的表面积。

8. 发明授权

US07285696B2 Process for catalytic alkylation of monocyclic aromatic compounds and composition for use therein 有权
标题翻译：单环芳族化合物的催化烷基化方法及其用途的组合物
公开(公告)号：US07285696B2
公开(公告)日：2007-10-23
申请号：US10840644
申请日：2004-05-07
申请人： Iver Schmidt , Claus Hviid Christensen , Christina Christensen , Kim Johannsen
发明人： Iver Schmidt , Claus Hviid Christensen , Christina Christensen , Kim Johannsen
IPC分类号： C07C2/68
CPC分类号： C07C2/66 , B01J29/40 , B01J35/10 , B01J35/1042 , B01J35/1057 , B01J35/1061 , B01J35/109 , B01J37/0018 , B01J37/082 , B01J2229/40 , B01J2229/42 , B01J2229/60 , C07C2/864 , C07C2529/40 , C07C15/073 , C07C15/02
摘要： A process for the catalytic alkylation of monocyclic aromatic compounds in a hydrocarbon process stream comprising contacting the monocyclic aromatic compound-containing hydrocarbon process stream with an alkylation agent under alkylation conditions with a mesoporous zeotype catalyst having an intracrystalline, non-crystallographic mesopore system and a mesopore volume of the zeotype crystals above 0.25 ml/g.
摘要翻译：在烃工艺流中催化烷基化单环芳族化合物的方法，包括在烷基化条件下使含单体芳族化合物的烃工艺流与烷基化试剂与具有结晶非结晶介孔体系和中孔的介孔沸石型催化剂接触沸石晶体的体积高于0.25ml / g。

9. 发明授权

US09889403B2 Solid ammonia storage and delivery material 有权
公开(公告)号：US09889403B2
公开(公告)日：2018-02-13
申请号：US13777175
申请日：2013-02-26
申请人： Claus Hviid Christensen , Tue Johannessen , Ulrich Quaade , Jens Kehlet Nørskov , Rasmus Zink Sørensen
发明人： Claus Hviid Christensen , Tue Johannessen , Ulrich Quaade , Jens Kehlet Nørskov , Rasmus Zink Sørensen
IPC分类号： B01D53/94 , B01D53/56 , B01D53/90 , B01J20/04 , B01J20/30 , C01C1/00 , C01F5/00 , C01G3/14 , C01G9/00 , C01G45/00 , C01G49/00 , C01G51/12 , C01G53/12 , F01N3/20 , B01J20/28
CPC分类号： B01D53/565 , B01D53/90 , B01D53/9431 , B01J20/046 , B01J20/28011 , B01J20/3035 , C01C1/006 , C01F5/00 , C01G3/14 , C01G9/00 , C01G45/00 , C01G49/00 , C01G51/12 , C01G53/12 , C01P2006/10 , F01N3/2066 , F01N2610/02 , F01N2610/06 , F01N2610/10 , F17C11/00 , Y02T10/24
摘要： Disclosed is a method for the selective catalytic reduction of NOx in waste/exhaust gas by using ammonia provides by heating one or more salts of formula Ma(NH3)nXz, wherein M represents one or more cations selected from alkaline earth metals and transition metals, X represents one or more anions, a represents the number of cations per salt molecule, z represents the number of anions per salt molecule, and n is a number of from 2 to 12, the one or more salts having been compressed to a bulk density above 70% of the skeleton density before use thereof.

10. 发明申请

US20100024403A1 High Density Storage of Ammonia 有权
标题翻译：氨的高密度储存
公开(公告)号：US20100024403A1
公开(公告)日：2010-02-04
申请号：US12577921
申请日：2009-10-13
申请人： Tue Johannessen , Claus Hviid Christensen , Jens Kehlet Norskov , Ulrich Quaade , Rasmus Zink Sorensen
发明人： Tue Johannessen , Claus Hviid Christensen , Jens Kehlet Norskov , Ulrich Quaade , Rasmus Zink Sorensen
IPC分类号： B01D53/56 , F17C11/00 , F17C13/00
CPC分类号： C01G3/14 , B01D53/56 , B01D53/79 , B01D53/8625 , B01D53/90 , B01D53/9409 , B01J20/046 , B01J20/28011 , B01J20/28014 , B01J20/2803 , B01J20/28042 , B01J20/3042 , C01C1/006 , C01F11/24 , F01N2610/02 , F01N2610/06 , F17C11/00 , Y02E60/364
摘要： A solid ammonia storage and delivery material comprising an ammonia absorbing/desorbing solid material, said storage and delivery material having been compacted to a density above 50% of the theoretic skeleton density provides a solid ammonia storage material which is easy to produce and handle and has a very high density of stored ammonia which is readily released under controlled conditions even though the porosity of the material is very low, and which storage material is safe for storage and transport of ammonia without special safety measures.
摘要翻译：包含氨吸收/解吸固体材料的固体氨储存和输送材料，所述储存和输送材料已压实至理论骨架密度的50％以上的密度，提供了易于生产和处理的固体氨储存材料，并具有尽管材料的孔隙率非常低，但在受控条件下容易释放的非常高密度的储存氨，并且哪些储存材料在没有特别的安全措施的情况下可以安全地存储和运输氨。

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