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1. 发明授权

US5859113A Pigment dispersions containing hydroxylated AB-block polymer dispersant 失效
标题翻译：含有羟基化AB嵌段聚合物分散剂的颜料分散体
公开(公告)号：US5859113A
公开(公告)日：1999-01-12
申请号：US896588
申请日：1997-07-17
申请人： Patrick F. McIntyre , James G. King , Harry J. Spinelli , Henry G. Jakubauskas
发明人： Patrick F. McIntyre , James G. King , Harry J. Spinelli , Henry G. Jakubauskas
IPC分类号： C09D17/00 , C08F2/16 , C08F293/00 , C08L53/00 , C09D7/45 , C09D153/00
CPC分类号： C08L53/00 , C08F293/005 , C09D153/00 , C09D7/02 , Y10T428/31786 , Y10T428/31797 , Y10T428/31855 , Y10T428/31935
摘要： A pigment dispersion useful for forming coating compositions containing dispersed pigment, a carrier liquid and an AB-block polymer dispersant (binder);the AB block polymer has a number average molecular weight of about 5,000-20,000 and contains 20-80% by weight of a polymeric A segment and correspondingly 80-20% by weight of a polymeric B segment; whereinthe polymeric A segment of the block polymer is of polymerized glycidyl (meth)acrylate monomers reacted with an acid from the group of aromatic carboxylic acids or aliphatic carboxylic acids; andthe B segment is of polymerized alkyl (meth)acrylate monomers having 1-12 carbon atoms in the alkyl group, hydroxy alkyl (meth)acrylate monomers having about 1-4 carbon atoms in the alkyl group; andwherein the weight ratio of pigment to binder in the dispersion is about 1/100-200/100.
摘要翻译：用于形成含有分散颜料，载体液体和AB嵌段聚合物分散剂（粘合剂）的涂料组合物的颜料分散体; AB嵌段聚合物具有约5,000-20,000的数均分子量，并且包含20-80重量％的聚合物A链段和相应地80-20重量％的聚合物B链段; 其中所述嵌段聚合物的聚合物A链段是聚合的（甲基）丙烯酸缩水甘油酯单体与来自芳族羧酸或脂族羧酸的酸反应的单体; 并且B链段是在烷基中具有1-12个碳原子的（甲基）丙烯酸烷基酯单体，在烷基中具有约1-4个碳原子的（甲基）丙烯酸羟烷基酯单体; 并且其中颜料与粘合剂在分散体中的重量比为约+ E，fra 1/100 + EE - + E，fra 200/100 + EE。

2. 发明授权

US06306521B1 Pigment dispersions containing hydroxylated AB-block polymer dispersant 失效
标题翻译：含有羟基化AB嵌段聚合物分散剂的颜料分散体
公开(公告)号：US06306521B1
公开(公告)日：2001-10-23
申请号：US09699904
申请日：2000-10-30
申请人： Harry J. Spinelli , Henry L. Jakubauskas , Patrick F. McIntyre , James G. King
发明人： Harry J. Spinelli , Henry L. Jakubauskas , Patrick F. McIntyre , James G. King
IPC分类号： B32B2730
CPC分类号： C08L53/00 , C08F293/005 , C09D7/45 , C09D153/00 , Y10T428/31786 , Y10T428/31797 , Y10T428/31855 , Y10T428/31935 , C08L2666/02
摘要： A pigment dispersion useful for forming coating compositions containing dispersed pigment, a carrier liquid and an AB-block polymer dispersant (binder); the AB block polymer has a number average molecular weight of about 5,000-20,000 and contains 20-80% by weight of a polymeric A segment and correspondingly 80-20% by weight of a polymeric B segment; wherein the polymeric A segment of the block polymer is of polymerized glycidyl (meth)acrylate monomers reacted with an acid from the group of aromatic carboxylic acids or aliphatic carboxylic acids; and the B segment is of polymerized alkyl (meth)acrylate monomers having 1-12 carbon atoms in the alkyl group, hydroxy alkyl (meth)acrylate monomers having about 1-4 carbon atoms in the alkyl group; and wherein the weight ratio of pigment to binder in the dispersion is about 1/100-200/100.
摘要翻译：用于形成含有分散颜料，载体液和AB嵌段聚合物分散剂（粘合剂）的涂料组合物的颜料分散体; AB嵌段聚合物的数均分子量为约5,000-20,000，并含有20-80重量％聚合物A链段和相应地80-20重量％的聚合物B链段; 嵌段聚合物的聚合物A链段是聚合的（甲基）丙烯酸缩水甘油酯单体与来自芳族羧酸或脂族羧酸的酸反应的单体; 并且B段是在烷基中具有1-12个碳原子的（甲基）丙烯酸烷基酯单体，在烷基中具有约1-4个碳原子的（甲基）丙烯酸羟烷基酯单体; 并且其中颜料与粘合剂在分散体中的重量比为约1 / 100-200 / 100。

3. 发明授权

US06187854B1 Pigment dispersions containing hydroxylated AB-block polymer dispersant 失效
公开(公告)号：US06187854B1
公开(公告)日：2001-02-13
申请号：US09136265
申请日：1998-08-19
申请人： Harry J. Spinelli , Henry L. Jakubauskas , Patrick F. McIntyre , James G. King
发明人： Harry J. Spinelli , Henry L. Jakubauskas , Patrick F. McIntyre , James G. King
IPC分类号： C08L5300
CPC分类号： C08L53/00 , C08F293/005 , C09D7/45 , C09D153/00 , Y10T428/31786 , Y10T428/31797 , Y10T428/31855 , Y10T428/31935 , C08L2666/02
摘要： A pigment dispersion useful for forming coating compositions containing dispersed pigment, a carrier liquid and an AB-block polymer dispersant (binder); the AB block polymer has a number average molecular weight of about 5,000-20,000 and contains 20-80% by weight of a polymeric A segment and correspondingly 80-20% by weight of a polymeric B segment; wherein the polymeric A segment of the block polymer is of polymerized glycidyl (meth)acrylate monomers reacted with an acid from the group of aromatic carboxylic acids or aliphatic carboxylic acids; and the B segment is of polymerized alkyl (meth)acrylate monomers having 1-12 carbon atoms in the alkyl group, hydroxy alkyl (meth)acrylate monomers having about 1-4 carbon atoms in the alkyl group; and wherein the weight ratio of pigment to binder in the dispersion is about 1/100-200/100.

4. 发明授权

US06204319B1 Aqueous coating compositions 失效
标题翻译：水性涂料组合物
公开(公告)号：US06204319B1
公开(公告)日：2001-03-20
申请号：US09183458
申请日：1998-10-30
申请人： Eric Charles Houze , Patrick F. McIntyre , Harry J. Spinelli , Ayumu Yokoyama
发明人： Eric Charles Houze , Patrick F. McIntyre , Harry J. Spinelli , Ayumu Yokoyama
IPC分类号： C08K300
CPC分类号： C09D17/001 , C01P2006/22 , C08J3/212 , C08J2353/00 , C09C1/56 , C09D5/027 , C09D17/005
摘要： An aqueous coating composition containing: (a) an aqueous carrier medium: (b) a pigment having a pH below 7.0; (c) an AB block copolymer pigment dispersant resin of (1) an A block of a hydrophobic polymer having amine groups; and (2) a B block of a hydrophilic polymer having hydroxyl groups and carboxyl groups; the AB block copolymer has a number average molecular weight of 5,000-20,000 and contains 20-80% by weight of a polymeric A segment and correspondingly 80-20% by weight of a polymeric B segment; wherein the pigment and the dispersant are present in a pigment to dispersant weight ratio of 0.1/1-20/1; (d) a film forming polymeric binder containing carboxyl groups and (e) a crosslinking agent which on curing of the coating composition will react with the carboxyl and hydroxyl groups of the AB block copolymer and the carboxyl groups of the film forming polymeric binder. Pigment dispersions of the AB block copolymer and process for forming the dispersions also are part of this invention.
摘要翻译：一种水性涂料组合物，其包含：（a）水性载体介质：（b）pH低于7.0的颜料;（c）（1）具有胺基的疏水性聚合物的A嵌段的AB嵌段共聚物颜料分散剂树脂; 和（2）具有羟基和羧基的亲水性聚合物的B嵌段; AB嵌段共聚物的数均分子量为5,000-20,000，并且包含20-80重量％的聚合物A链段，并且相应地为80-20 聚合物B链段的重量％;其中颜料和分散剂以颜料与分散剂的重量比为0.1 / 1-20 / 1存在;（d）含羧基的成膜聚合物粘合剂和（e）交联涂料组合物的固化剂将与AB嵌段共聚物的羧基和羟基以及成膜聚合物粘合剂的羧基反应。AB嵌段共聚物的分散体和形成分散体的方法也是其中的一部分发明。

5. 发明授权

US5085698A Aqueous pigmented inks for ink jet printers 失效
标题翻译：用于喷墨打印机的水性着色油墨
公开(公告)号：US5085698A
公开(公告)日：1992-02-04
申请号：US508145
申请日：1990-04-11
申请人： Sheau-Hwa Ma , Howard Matrick , Arthur C. Shor , Harry J. Spinelli
发明人： Sheau-Hwa Ma , Howard Matrick , Arthur C. Shor , Harry J. Spinelli
IPC分类号： C09D11/00 , C09D11/10
CPC分类号： C09B67/0008 , C09D11/326
摘要： A pigmented ink for ink jet printers which comprises an aqueous carrier medium, and pigment particles dispersed in an AB or BAB block copolymer having a hydrophilic segment and a segment that links to the pigment. The A block and the B block(s) have molecular weights of at least 300. These inks give images having good print quality, water and smear resistance, lightfastness, and storage stability.
摘要翻译：一种用于喷墨打印机的着色油墨，其包含水性载体介质和分散在具有亲水链段和连接于颜料的链段的AB或BAB嵌段共聚物中的颜料颗粒。 A块和B嵌段的分子量至少为300.这些油墨给出了具有良好印刷质量，耐水和耐沾污性，耐光性和储存稳定性的图像。

6. 发明授权

US5057576A Acrylic block copolymer with crosslinkable silicon substituent 失效
标题翻译：具有可交联硅取代基的丙烯酸嵌段共聚物
公开(公告)号：US5057576A
公开(公告)日：1991-10-15
申请号：US414416
申请日：1989-09-29
申请人： Harry J. Spinelli
发明人： Harry J. Spinelli
IPC分类号： C08F230/08 , C08F293/00 , C08F297/00 , C08G77/42 , C08G77/442
CPC分类号： C08F293/00 , C08F230/08
摘要： Hybrid star polymers with acrylic arms and crosslinked polysiloxane cores can be made by a polycondensation of substituent alkoxysilyl groups contained in acrylic ester groups of acrylic block copolymers to form the cores.

7. 发明授权

US4695607A Group transfer processes for acrylic star polymers 失效
标题翻译：丙烯酸类星形聚合物的组转移方法
公开(公告)号：US4695607A
公开(公告)日：1987-09-22
申请号：US771684
申请日：1985-09-03
申请人： Harry J. Spinelli
发明人： Harry J. Spinelli
IPC分类号： C08F290/04 , C08F293/00 , C08F295/00 , C08F297/00
CPC分类号： C08F290/046 , Y10T428/31855
摘要： Large acrylic star polymers, are made by group transfer polymerization techniques by arm-first, core-first, or arm-core-arm approaches.
摘要翻译：大型丙烯酸星形聚合物，通过臂转，聚焦，或者臂 - 臂 - 手臂方式通过组转移聚合技术制成。

8. 发明授权

US5314960A Silicone-containing polymers, oxygen permeable hydrophilic contact lenses and methods for making these lenses and treating patients with visual impairment 失效
标题翻译：含硅聚合物，透氧亲水性隐形眼镜和制造这些镜片的方法以及治疗视力障碍的患者
公开(公告)号：US5314960A
公开(公告)日：1994-05-24
申请号：US773714
申请日：1991-10-09
申请人： Harry J. Spinelli , Waifong L. Anton , Leonard Seidner , Henry D. Coleman , Mohammed I. Ali , Lester Weintraub , Paul White
发明人： Harry J. Spinelli , Waifong L. Anton , Leonard Seidner , Henry D. Coleman , Mohammed I. Ali , Lester Weintraub , Paul White
IPC分类号： C08F287/00 , C08F290/04 , C08F293/00 , G02B1/04 , C08F271/02 , C08F275/00
CPC分类号： G02B1/043 , C08F287/00 , C08F290/04 , C08F293/00
摘要： The present invention relates to novel copolymers and contact lenses made from these copolymers comprising preformed silicone-containing acrylic star polymers, graft copolymers and macromonomers, preparation of these contact lenses and a therapeutic method for treating patients with visual impairment.Described is a composition comprising at least about 10% by weight of a preformed silicone-containing acrylic copolymer and no more than about 90% by weight of a matrix formed from the random polymerization of a mixture of monomers. The mixture of monomers comprises at least one hydrophilic monomer and optionally, monomers selected from the group consisting of silicone acrylates, esters of alpha, beta-unsaturated acids and crosslinking monomers. The preformed silicone-containing acrylic copolymer is preferably copolymerized throughout the matrix. The final compositions are hydrated to a final water content of at least about 10% by weight.
摘要翻译：本发明涉及由这些共聚物制成的新型共聚物和隐形眼镜，包括预先形成的含硅酮的丙烯酸类星形聚合物，接枝共聚物和大分子单体，这些隐形眼镜的制备以及用于治疗视力障碍的患者的治疗方法。描述了包含至少约10重量％的预成型含硅氧烷的丙烯酸共聚物和不超过约90重量％的由单体混合物的无规聚合形成的基体的组合物。单体混合物包含至少一种亲水性单体和任选的选自硅氧烷丙烯酸酯，α，β-不饱和酸的酯和交联单体的单体。预制的含有机硅的丙烯酸共聚物优选在整个基质中共聚。将最终组合物水合至至少约10重量％的最终含水量。

9. 发明授权

US5019628A Silicone containing acrylic star polymers 失效
标题翻译：含有丙烯酸的聚合物有机硅
公开(公告)号：US5019628A
公开(公告)日：1991-05-28
申请号：US507277
申请日：1990-04-10
申请人： Harry J. Spinelli
发明人： Harry J. Spinelli
IPC分类号： C08F220/28 , C08F20/10 , C08F20/32 , C08F22/32 , C08F22/36 , C08F30/08 , C08F220/32 , C08F220/42 , C08F222/40 , C08F230/08 , C08F290/00 , C08F290/14 , C08F299/08 , G02B1/04 , G02C7/04
CPC分类号： C08F299/08 , C08F290/148 , G02B1/043 , Y10S525/901 , Y10S525/91 , Y10S528/901
摘要： Acrylic star polymers containing polysiloxanylalkyl ester groups in their arms and terminal organo groups containing a polymerizable carbon-carbon double bond are useful for improving polymer compositions for contact lenses.

10. 发明授权

US4847328A Hybrid acrylic star polymers 失效
标题翻译：混合丙烯酸星形聚合物
公开(公告)号：US4847328A
公开(公告)日：1989-07-11
申请号：US31931
申请日：1987-03-30
申请人： Clyde S. Hutchins , Harry J. Spinelli
发明人： Clyde S. Hutchins , Harry J. Spinelli
IPC分类号： C08G18/62 , C08G59/40 , C08G85/00
CPC分类号： C08G18/6245 , C08G59/40 , C08G85/00 , Y10S424/16
摘要： Hybrid star polymers with functional acrylic arms and crosslinked cores.
摘要翻译：具有功能性丙烯酸臂和交联芯的混合星形聚合物。

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