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1. 发明申请

US20050181267A1 Membrane-electrode structure and method for producing the same 审中-公开
标题翻译：膜 - 电极结构及其制造方法
公开(公告)号：US20050181267A1
公开(公告)日：2005-08-18
申请号：US10505442
申请日：2003-10-28
申请人： Naoki Mitsuta , Hiroshi Shinkai , Masaaki Nanaumi
发明人： Naoki Mitsuta , Hiroshi Shinkai , Masaaki Nanaumi
IPC分类号： B05D5/12 , H01M2/08 , H01M4/86 , H01M8/00 , H01M8/02 , H01M8/10
CPC分类号： H01M8/1004 , H01M8/0284 , H01M2008/1095 , H01M2300/0082
摘要： The present invention provides a membrane-electrode structure having an adhesive support layer that does not peel off the solid polymer electrolyte membrane in a high-temperature high-humidity environment during the operation of a fuel cell, and a producing method thereof. The present invention also provides a polymer electrolyte fuel cell that uses the membrane-electrode structure, and an electric apparatus and a transport apparatus that use the polymer electrolyte fuel cell. The solid polymer electrolyte membrane 2 is sandwiched by catalyst layers 3 and 4 positioned in the inner circumferential side thereof, and one face is coated with the catalyst layers 3 and 4 and the adhesive support layer 9. The adhesive support layer 9 is formed of an adhesive that has fluorine atoms in the molecular structure. The adhesive has a tensile elongation at break of 150% or more after curing. Having porous diffusion layers 5 and 6 that coat the catalyst layers 3, 4 and the adhesive support layer 9, the adhesive support layer 9 is integrated with the diffusion layer 6 through adhesive permeating layers 10. Irregularity that has a maximum height Rmax of surface roughness within a range between 3 and 20 μm is formed on the area coated by the adhesive support layer 9 of the solid polymer electrolyte membrane 2, and the adhesive support layer 9 is bonded to the area where the irregularity has been formed by pressing under heating.
摘要翻译：本发明提供一种膜电极结构，其具有在燃料电池的运转中在高温高湿环境下不会剥离固体高分子电解质膜的粘合剂支撑层及其制造方法。本发明还提供一种使用该膜 - 电极结构的聚合物电解质型燃料电池，以及使用上述固体高分子型燃料电池的电气设备和输送装置。固体高分子电解质膜2被位于其内周侧的催化剂层3和4夹持，一面涂覆有催化剂层3和4以及粘合剂支撑层9。粘合剂支撑层9由分子结构中具有氟原子的粘合剂形成。粘合剂在固化后的拉伸断裂伸长率为150％以上。具有涂覆催化剂层3,4和粘合剂支撑层9的多孔扩散层5和6，粘合剂支撑层9通过粘合剂渗透层10与扩散层6一体化。在由固体聚合物电解质膜2的粘合剂支撑层9涂覆的区域上形成具有3-20μm范围内的表面粗糙度的最大高度R max max的不规则性，并且粘合剂支持体层9通过加热压制而结合到形成有凹凸的区域。

2. 发明授权

US07531265B2 Fuel cell 有权
标题翻译：燃料电池
公开(公告)号：US07531265B2
公开(公告)日：2009-05-12
申请号：US11061189
申请日：2005-02-17
申请人： Seiji Sugiura , Masaaki Nanaumi , Hiroshi Shinkai , Shuhei Goto
发明人： Seiji Sugiura , Masaaki Nanaumi , Hiroshi Shinkai , Shuhei Goto
IPC分类号： H01M8/02 , H01M8/10
CPC分类号： H01M4/926 , H01M8/0232 , H01M8/0234 , H01M8/0247 , H01M8/0258 , H01M8/0267 , H01M8/0271 , H01M8/0276 , H01M8/0297 , H01M8/1004
摘要： A fuel cell includes a membrane electrode assembly and first and second metal separators. The first metal separator has first outer protrusions provided outside an oxygen-containing gas flow field. The second metal separator has second outer protrusions provided outside a fuel gas flow field. The first and second protrusions sandwich outer edges of electrode catalyst layers.
摘要翻译：燃料电池包括膜电极组件和第一和第二金属分离器。第一金属隔板具有设置在含氧气体流场外的第一外部突起。第二金属分离器具有设置在燃料气体流场外部的第二外部突出部。第一和第二突起夹着电极催化剂层的外边缘。

3. 发明申请

US20050186464A1 Fuel cell 有权
标题翻译：燃料电池
公开(公告)号：US20050186464A1
公开(公告)日：2005-08-25
申请号：US11061189
申请日：2005-02-17
申请人： Seiji Sugiura , Masaaki Nanaumi , Hiroshi Shinkai , Shuhei Goto
发明人： Seiji Sugiura , Masaaki Nanaumi , Hiroshi Shinkai , Shuhei Goto
IPC分类号： H01M2/08 , H01M2/18 , H01M4/86 , H01M4/92 , H01M8/02 , H01M8/04 , H01M8/10
CPC分类号： H01M4/926 , H01M8/0232 , H01M8/0234 , H01M8/0247 , H01M8/0258 , H01M8/0267 , H01M8/0271 , H01M8/0276 , H01M8/0297 , H01M8/1004
摘要： A fuel cell includes a membrane electrode assembly and first and second metal separators. The first metal separator has first outer protrusions provided outside an oxygen-containing gas flow field. The second metal separator has second outer protrusions provided outside a fuel gas flow field. The first and second protrusions sandwich outer edges of electrode catalyst layers.
摘要翻译：燃料电池包括膜电极组件和第一和第二金属分离器。第一金属隔板具有设置在含氧气体流场外的第一外部突起。第二金属分离器具有设置在燃料气体流场外部的第二外部突出部。第一和第二突起夹着电极催化剂层的外边缘。

4. 发明授权

US07306876B2 Method for producing membrane-electrode structure and polymer electrolyte fuel cell 有权
标题翻译：膜 - 电极结构和聚合物电解质燃料电池的制造方法
公开(公告)号：US07306876B2
公开(公告)日：2007-12-11
申请号：US10721505
申请日：2003-11-26
申请人： Masaki Tani , Hiroshi Shinkai , Katsuhiko Kohyama , Ichiro Tanaka , Yuichiro Hama , Junichi Yano
发明人： Masaki Tani , Hiroshi Shinkai , Katsuhiko Kohyama , Ichiro Tanaka , Yuichiro Hama , Junichi Yano
IPC分类号： H01M4/00 , H01M4/88 , B05D5/12
CPC分类号： H01M4/926 , H01M4/8605 , H01M4/8814 , H01M4/8882 , H01M4/8896 , H01M4/921 , H01M8/0234 , H01M8/1004 , Y02P70/56
摘要： A membrane-electrode structure having an electrode catalyst layer adhered to a diffusion electrode, wherein the structure is manufactured by applying a catalyst paste onto a sheet substrate, and then dried to form a plurality of electrode catalyst layers. The electrode catalyst layers are thermally transferred onto each side of a polymer electrolyte membrane to form a laminated body. A first slurry is applied on a carbon substrate layer, and dried to form a water-repellent layer, and then, a second slurry is applied on the water-repellent layer, and dried to form a hydrophilic layer to form a diffusion electrode. The diffusion electrode is then laminated on the electrode catalyst layer through the hydrophilic layer, and then pressed under heating to integrate the laminated body and the diffusion electrode.
摘要翻译：一种具有粘附到扩散电极的电极催化剂层的膜 - 电极结构，其中通过将催化剂浆料涂布在片状基材上，然后干燥以形成多个电极催化剂层来制造该结构。将电极催化剂层热转印到聚合物电解质膜的每一侧上以形成层压体。将第一浆料涂布在碳基材层上，干燥形成防水层，然后将第二浆料涂覆在防水层上，干燥形成亲水层，形成扩散电极。然后通过亲水层将扩散电极层叠在电极催化剂层上，然后在加热下加压以使层叠体和扩散电极结合。

5. 发明申请

US20050008920A1 Membrane electrode assembly for polymer electrolyte fuel cell 审中-公开
标题翻译：用于聚合物电解质燃料电池的膜电极组件
公开(公告)号：US20050008920A1
公开(公告)日：2005-01-13
申请号：US10844583
申请日：2004-05-13
申请人： Katsuhiko Kohyama , Hiroshi Shinkai , Masaki Tani
发明人： Katsuhiko Kohyama , Hiroshi Shinkai , Masaki Tani
IPC分类号： H01M8/02 , H01M2/00 , H01M2/02 , H01M4/86 , H01M8/04 , H01M8/10 , H01M8/12
CPC分类号： H01M4/8605 , H01M4/8657 , H01M8/1004
摘要： A membrane electrode assembly for a polymer electrolyte fuel cell has, as basic components, a polymer electrolyte membrane, a pair of electrode layers which sandwich the polymer electrolyte membrane, and a pair of gas-diffusion layers disposed outside the respective electrode layers. Electric medium layers are respectively provided between the electrode layer and the gas-diffusion layer at one side and between the electric layer and the gas-diffusion layer at the other side. Each of the electric medium layers is constituted of a plurality of carbon whiskers, a plurality of carbon particles and a binder including an electrolyte material. A content GW of the carbon whiskers in each of the electric medium layers is set at 10 wt %≦GW≦25 wt %. Thus, the membrane electrode assembly for the polymer electrolyte fuel cell can keep a high power generating performance by reducing the contact resistance between the gas-diffusion layers and the electrode layers.
摘要翻译：固体高分子型燃料电池用的膜电极组件作为基本成分，具有高分子电解质膜，夹着聚合物电解质膜的一对电极层和配置在各电极层的外侧的一对气体扩散层。电介质层分别设置在电极层和气体扩散层之间的一侧以及电层和另一侧的气体扩散层之间。每个电介质层由多个碳晶须，多个碳颗粒和包含电解质材料的粘合剂构成。每个电介质层中的碳晶须的含量GW被设定为10重量％<= GW <= 25重量％。因此，通过降低气体扩散层和电极层之间的接触电阻，用于聚合物电解质燃料电池的膜电极组件可以保持高发电性能。

6. 发明授权

US4829082A Pharmaceutical compositions for the treatment of skin diseases 失效
标题翻译：用于治疗皮肤疾病的药物组合物
公开(公告)号：US4829082A
公开(公告)日：1989-05-09
申请号：US902299
申请日：1986-08-29
申请人： Hiroshi Shinkai , Takao Kishiye
发明人： Hiroshi Shinkai , Takao Kishiye
IPC分类号： C07D311/72 , A61K31/352 , A61K31/355 , A61P17/00
CPC分类号： A61K31/355 , Y10S514/928
摘要： This invention relates to pharmaceutical compositions for the treatment of skin diseases which comprises as an active ingredient vitamin A esters of .alpha.-tocopherol.

7. 发明授权

US08236206B2 Electrode catalyst layer 有权
标题翻译：电极催化剂层
公开(公告)号：US08236206B2
公开(公告)日：2012-08-07
申请号：US12092316
申请日：2006-10-30
申请人： Satoshi Komatsu , Junji Kawai , Toshihiro Ohtsuki , Takanobu Yamamoto , Ryoichiro Takahashi , Kaoru Fukuda , Hiroshi Shinkai
发明人： Satoshi Komatsu , Junji Kawai , Toshihiro Ohtsuki , Takanobu Yamamoto , Ryoichiro Takahashi , Kaoru Fukuda , Hiroshi Shinkai
IPC分类号： H01B1/00
CPC分类号： C08G65/405 , C08G65/4006 , C08G65/4025 , C08G65/4037 , C08G65/4056 , C08G75/23 , C08L27/12 , C09D133/16 , H01M4/8605 , H01M4/8652 , H01M8/1004 , H01M2300/0082 , C08L2666/06
摘要： The present invention provides an electrode catalyst layer comprising catalyst particles, an ion exchange resin and a water repellent agent. The water repellent agent contains (A) a fluorine-containing copolymer having a structure unit derived from a polyfluoroalkyl-containing (meth)acrylate and/or (B) a fluorine-containing copolymer having a structural unit represented by derived from a fluorine-containing olefin monomer and a structure unit represented derived from a vinyl ether monomer. The electrode catalyst layer contains 0.1 to 20% by weight of the water repellant agent. The electrode catalyst layer exhibits excellent balance between water retention and drainage in an electrode, good power generation performance under any of low humidity and high humidity conditions, and also excellent durability in power generation.
摘要翻译：本发明提供了包含催化剂颗粒，离子交换树脂和防水剂的电极催化剂层。防水剂含有（A）具有衍生自含氟烷基的（甲基）丙烯酸酯的结构单元的含氟共聚物和/或（B）具有由含氟的烯烃单体和由乙烯基醚单体衍生的结构单元。电极催化剂层含有0.1〜20重量％的防水剂。电极催化剂层在电极的保水性和排水性之间表现出优异的平衡，在任何低湿度和高湿度条件下都具有良好的发电性能，并且还具有优异的发电耐久性。

8. 发明授权

US07566511B2 Solid polymer cell assembly 失效
标题翻译：固体聚合物电池组件
公开(公告)号：US07566511B2
公开(公告)日：2009-07-28
申请号：US10521059
申请日：2003-06-26
申请人： Yoshinori Wariishi , Naoyuki Enjoji , Yoichi Asano , Hiroshi Shinkai
发明人： Yoshinori Wariishi , Naoyuki Enjoji , Yoichi Asano , Hiroshi Shinkai
IPC分类号： H01M2/00 , H01M8/10
CPC分类号： H01M8/04089 , H01M8/04291 , H01M8/241 , H01M8/2484 , H01M8/249
摘要： A cell assembly (10) includes a first unit cell (12) and a second unit cell (14). The first unit cell (12) and the second unit cell (14) are juxtaposed such that electrode surfaces of the first unit cell (12) and electrode surfaces of the second unit cell (14) are aligned in parallel with each other. An oxygen-containing gas flow passage (32) includes a first oxygen-containing gas passage (38) in the first unit cell (12), an oxygen-containing gas connection passage (40) in a connection passage member (16), and a second oxygen-containing gas passage (42) in the second unit cell (14). The first oxygen-containing gas passage (38), the oxygen-containing gas connection passage (40), and the second oxygen-containing gas passage (42) are connected serially from the first unit cell (12) to the second unit cell (14).
摘要翻译：电池组件（10）包括第一单电池（12）和第二单电池（14）。第一单电池（12）和第二单电池（14）并置，使得第一单电池（12）的电极表面和第二单电池（14）的电极表面彼此平行排列。含氧气体流路（32）包括第一单元电池（12）中的第一含氧气体通路（38），连接通路部件（16）中的含氧气体连接通路（40），以及第二单元电池（14）中的第二含氧气体通道（42）。第一含氧气体通道（38），含氧气体连接通道（40）和第二含氧气体通道（42）从第一单元电池（12）串联连接到第二单元电池 14）。

9. 发明申请

US20090130526A1 ELECTRODE ELECTROLYTE FOR USE IN SOLID POLYMER FUEL CELL 有权
标题翻译：用于固体聚合物燃料电池的电极电解质
公开(公告)号：US20090130526A1
公开(公告)日：2009-05-21
申请号：US11995701
申请日：2006-06-30
申请人： Makoto Higami , Igor Rozhanskii , Yoshitaka Yamakawa , Nagayuki Kanaoka , Kaoru Fukuda , Ryoichiro Takahashi , Hiroshi Shinkai
发明人： Makoto Higami , Igor Rozhanskii , Yoshitaka Yamakawa , Nagayuki Kanaoka , Kaoru Fukuda , Ryoichiro Takahashi , Hiroshi Shinkai
IPC分类号： H01M8/10
CPC分类号： C08G61/02 , C08G73/028 , C08J5/2256 , C08J2371/12 , H01M4/8652 , H01M4/8807 , H01M4/92 , H01M4/926 , H01M8/0239 , H01M8/1023 , H01M8/1025 , H01M8/1027 , H01M8/103 , H01M8/1032 , H01M8/1048 , H01M8/106
摘要： This invention provides an electrode electrolyte for a solid polymer-type fuel cell, in which a cost problem and a problem related to recovery of catalyst metals are solved, having excellent proton conductivity, dimensional stability and heat resistance.An electrode electrolyte for a solid polymer electrolyte-type fuel cell contains a polymer, which has a polyphenylene structure as a main chain and both a sulfonic acid group and a nitrogen-containing heterocyclic group as a side chain. A side chain having the nitrogen-containing heterocyclic group has a structure represented by the following general formula (D). (In formula, Z represents at least one kind of structures selected from a group consisting of a direct bond, —O— and —S—, Y represents at least one kind of structures selected from a group consisting of —CO—, —SO2—, —SO—, —CONH—, —COO—, —(CF2)1— (1 is an integer of 1 to 10) and —C(CF3)2— and R20 represents a nitrogen-containing heterocyclic group. q represents an integer of 1 to 5 and p represents an integer of 0 to 4.)The above nitrogen-containing heterocyclic group is at least one kind of group derived from a compound selected from the group consisting of nitrogen-containing heterocyclic compounds including pyrrole, thiazole, isothiazole, oxazole, isoxazole, pyridine, imidazole, imidazoline, pyrazole, 1,3,5-triazine, pyrimidine, pyridazine, pyrazine, indole, quinoline, isoquinoline, purine, benzimidazole, benzoxazole, benzothiazole, tetrazole, tetrazine, triazole, carbazole, acridine, quinoxaline and quinazoline and derivatives thereof.
摘要翻译：本发明提供一种固体聚合物型燃料电池用电极电解质，其中解决了成本问题和与催化剂金属的回收相关的问题，具有优异的质子传导性，尺寸稳定性和耐热性。固体高分子电解质型燃料电池用电极电解质含有作为主链的聚亚苯基结构和磺酸基和含氮杂环基作为侧链的聚合物。具有含氮杂环基的侧链具有由以下通式（D）表示的结构。（式中，Z表示选自由直链，-O-和-S-组成的组中的至少一种结构，Y表示选自-CO - ， - SO 2的至少一种结构 - ， - SO - ， - CONH - ， - COO - ， - （CF 2）1 - （1为1〜10的整数）和-C（CF 3）2 - ，R 20为含氮杂环基 1〜5的整数，p表示0〜4的整数。）上述含氮杂环基是选自包含吡咯，噻唑等含氮杂环化合物的化合物中的至少一种异噻唑，恶唑，异恶唑，吡啶，咪唑，咪唑啉，吡唑，1,3,5-三嗪，嘧啶，哒嗪，吡嗪，吲哚，喹啉，异喹啉，嘌呤，苯并咪唑，苯并恶唑，苯并噻唑四唑，四嗪，三唑，，吖啶，喹喔啉和喹唑啉及其衍生物。

10. 发明申请

US20070020504A1 Fuel cell 有权
标题翻译：燃料电池
公开(公告)号：US20070020504A1
公开(公告)日：2007-01-25
申请号：US10558229
申请日：2004-05-21
申请人： Narutoshi Sugita , Katsuhiko Kohyama , Shuhei Goto , Hiroshi Shinkai , Hiroyuki Tanaka , Takaki Nagawa
发明人： Narutoshi Sugita , Katsuhiko Kohyama , Shuhei Goto , Hiroshi Shinkai , Hiroyuki Tanaka , Takaki Nagawa
IPC分类号： H01M8/24 , H01M4/94
CPC分类号： H01M8/0271 , H01M8/0247 , H01M8/0258 , H01M8/0263 , H01M8/241 , H01M8/2483 , H01M2008/1095 , Y02E60/50
摘要： An assembling operation of a fuel cell is effectively simplified. With the simple and economical structure, the desired sealing function is achieved. The fuel cell includes a membrane electrode assembly and first and second metal separators sandwiching the membrane electrode assembly. Connection channels are provided on the first metal separator. The connection channels connect the oxygen-containing gas supply passage and the oxygen-containing gas discharge passage to the oxygen-containing gas flow field. The membrane electrode assembly has first overlapping portions overlapped on the connection channels for sealing the connection channels. The first overlapping portions comprise, in effect, a gas diffusion layer.
摘要翻译：有效地简化燃料电池的组装操作。通过简单经济的结构，实现了所需的密封功能。燃料电池包括膜电极组件和夹住膜电极组件的第一和第二金属分离器。连接通道设置在第一金属分离器上。连接通道将含氧气体供给通道和含氧气体排出通道连接到含氧气体流场。膜电极组件具有在连接通道上重叠的第一重叠部分，用于密封连接通道。实际上，第一重叠部分包括气体扩散层。

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