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1. 发明授权

US07306876B2 Method for producing membrane-electrode structure and polymer electrolyte fuel cell 有权
标题翻译：膜 - 电极结构和聚合物电解质燃料电池的制造方法
公开(公告)号：US07306876B2
公开(公告)日：2007-12-11
申请号：US10721505
申请日：2003-11-26
申请人： Masaki Tani , Hiroshi Shinkai , Katsuhiko Kohyama , Ichiro Tanaka , Yuichiro Hama , Junichi Yano
发明人： Masaki Tani , Hiroshi Shinkai , Katsuhiko Kohyama , Ichiro Tanaka , Yuichiro Hama , Junichi Yano
IPC分类号： H01M4/00 , H01M4/88 , B05D5/12
CPC分类号： H01M4/926 , H01M4/8605 , H01M4/8814 , H01M4/8882 , H01M4/8896 , H01M4/921 , H01M8/0234 , H01M8/1004 , Y02P70/56
摘要： A membrane-electrode structure having an electrode catalyst layer adhered to a diffusion electrode, wherein the structure is manufactured by applying a catalyst paste onto a sheet substrate, and then dried to form a plurality of electrode catalyst layers. The electrode catalyst layers are thermally transferred onto each side of a polymer electrolyte membrane to form a laminated body. A first slurry is applied on a carbon substrate layer, and dried to form a water-repellent layer, and then, a second slurry is applied on the water-repellent layer, and dried to form a hydrophilic layer to form a diffusion electrode. The diffusion electrode is then laminated on the electrode catalyst layer through the hydrophilic layer, and then pressed under heating to integrate the laminated body and the diffusion electrode.
摘要翻译：一种具有粘附到扩散电极的电极催化剂层的膜 - 电极结构，其中通过将催化剂浆料涂布在片状基材上，然后干燥以形成多个电极催化剂层来制造该结构。将电极催化剂层热转印到聚合物电解质膜的每一侧上以形成层压体。将第一浆料涂布在碳基材层上，干燥形成防水层，然后将第二浆料涂覆在防水层上，干燥形成亲水层，形成扩散电极。然后通过亲水层将扩散电极层叠在电极催化剂层上，然后在加热下加压以使层叠体和扩散电极结合。

2. 发明申请

US20050008920A1 Membrane electrode assembly for polymer electrolyte fuel cell 审中-公开
标题翻译：用于聚合物电解质燃料电池的膜电极组件
公开(公告)号：US20050008920A1
公开(公告)日：2005-01-13
申请号：US10844583
申请日：2004-05-13
申请人： Katsuhiko Kohyama , Hiroshi Shinkai , Masaki Tani
发明人： Katsuhiko Kohyama , Hiroshi Shinkai , Masaki Tani
IPC分类号： H01M8/02 , H01M2/00 , H01M2/02 , H01M4/86 , H01M8/04 , H01M8/10 , H01M8/12
CPC分类号： H01M4/8605 , H01M4/8657 , H01M8/1004
摘要： A membrane electrode assembly for a polymer electrolyte fuel cell has, as basic components, a polymer electrolyte membrane, a pair of electrode layers which sandwich the polymer electrolyte membrane, and a pair of gas-diffusion layers disposed outside the respective electrode layers. Electric medium layers are respectively provided between the electrode layer and the gas-diffusion layer at one side and between the electric layer and the gas-diffusion layer at the other side. Each of the electric medium layers is constituted of a plurality of carbon whiskers, a plurality of carbon particles and a binder including an electrolyte material. A content GW of the carbon whiskers in each of the electric medium layers is set at 10 wt %≦GW≦25 wt %. Thus, the membrane electrode assembly for the polymer electrolyte fuel cell can keep a high power generating performance by reducing the contact resistance between the gas-diffusion layers and the electrode layers.
摘要翻译：固体高分子型燃料电池用的膜电极组件作为基本成分，具有高分子电解质膜，夹着聚合物电解质膜的一对电极层和配置在各电极层的外侧的一对气体扩散层。电介质层分别设置在电极层和气体扩散层之间的一侧以及电层和另一侧的气体扩散层之间。每个电介质层由多个碳晶须，多个碳颗粒和包含电解质材料的粘合剂构成。每个电介质层中的碳晶须的含量GW被设定为10重量％<= GW <= 25重量％。因此，通过降低气体扩散层和电极层之间的接触电阻，用于聚合物电解质燃料电池的膜电极组件可以保持高发电性能。

3. 发明授权

US07232627B2 Electrode for solid polymer fuel cell 有权
标题翻译：固体聚合物燃料电池用电极
公开(公告)号：US07232627B2
公开(公告)日：2007-06-19
申请号：US10703072
申请日：2003-11-07
申请人： Kaoru Fukuda , Masaki Tani , Shigeru Inai , Hayato Kaji , Chikara Iwasawa , Shinya Watanabe , Katsuhiko Kohyama , Hiroshi Shinkai , Takeshi Muro
发明人： Kaoru Fukuda , Masaki Tani , Shigeru Inai , Hayato Kaji , Chikara Iwasawa , Shinya Watanabe , Katsuhiko Kohyama , Hiroshi Shinkai , Takeshi Muro
IPC分类号： H01M4/00
CPC分类号： H01M4/8821 , H01M4/8605 , H01M4/8636 , H01M4/921 , H01M4/926 , H01M8/0234 , H01M8/04097 , H01M8/04104 , H01M8/04291 , H01M8/1007
摘要： An electrode for a solid polymer fuel cell includes a gas diffusion layer, an electrode catalyst layer disposed between a solid polymer membrane of the fuel cell and the gas diffusion layer, and a water-holding layer disposed between the gas diffusion layer and the electrode catalyst layer. Under high-relative humidity conditions of reaction gases, flooding can be prevented because the electrode catalyst layer is made porous, while under low-relative humidity conditions of reaction gases, sufficient water contents can be stably provided thanks to the water-holding layer so that proton conductivity of the solid polymer membrane can be maintained appropriately. Consequently, high-performance and high-durability electrode and membrane electrode assembly for a solid polymer fuel cell can be provided such that the performance and the durability thereof are not affected by change in relative humidity in reactant gases supplied to the solid polymer fuel cell.
摘要翻译：固体高分子型燃料电池用电极包括气体扩散层，设置在燃料电池的固体聚合物膜与气体扩散层之间的电极催化剂层和配置在气体扩散层与电极催化剂之间的保水层层。在反应气体的高相对湿度条件下，由于电极催化剂层为多孔，可以防止溢流，而在反应气体的低相对湿度条件下，由于保水层能够稳定地提供足够的水含量，可以适当地维持固体聚合物膜的质子传导性。因此，可以提供用于固体聚合物燃料电池的高性能和高耐久性的电极和膜电极组件，使得其性能和耐久性不受供应到固体聚合物燃料电池的反应气体中相对湿度的变化的影响。

4. 发明申请

US20070020504A1 Fuel cell 有权
标题翻译：燃料电池
公开(公告)号：US20070020504A1
公开(公告)日：2007-01-25
申请号：US10558229
申请日：2004-05-21
申请人： Narutoshi Sugita , Katsuhiko Kohyama , Shuhei Goto , Hiroshi Shinkai , Hiroyuki Tanaka , Takaki Nagawa
发明人： Narutoshi Sugita , Katsuhiko Kohyama , Shuhei Goto , Hiroshi Shinkai , Hiroyuki Tanaka , Takaki Nagawa
IPC分类号： H01M8/24 , H01M4/94
CPC分类号： H01M8/0271 , H01M8/0247 , H01M8/0258 , H01M8/0263 , H01M8/241 , H01M8/2483 , H01M2008/1095 , Y02E60/50
摘要： An assembling operation of a fuel cell is effectively simplified. With the simple and economical structure, the desired sealing function is achieved. The fuel cell includes a membrane electrode assembly and first and second metal separators sandwiching the membrane electrode assembly. Connection channels are provided on the first metal separator. The connection channels connect the oxygen-containing gas supply passage and the oxygen-containing gas discharge passage to the oxygen-containing gas flow field. The membrane electrode assembly has first overlapping portions overlapped on the connection channels for sealing the connection channels. The first overlapping portions comprise, in effect, a gas diffusion layer.
摘要翻译：有效地简化燃料电池的组装操作。通过简单经济的结构，实现了所需的密封功能。燃料电池包括膜电极组件和夹住膜电极组件的第一和第二金属分离器。连接通道设置在第一金属分离器上。连接通道将含氧气体供给通道和含氧气体排出通道连接到含氧气体流场。膜电极组件具有在连接通道上重叠的第一重叠部分，用于密封连接通道。实际上，第一重叠部分包括气体扩散层。

5. 发明授权

US08865366B2 Fuel cell with protruded gas diffusion layer 有权
标题翻译：具有突出气体扩散层的燃料电池
公开(公告)号：US08865366B2
公开(公告)日：2014-10-21
申请号：US13434100
申请日：2012-03-29
申请人： Narutoshi Sugita , Katsuhiko Kohyama , Shuhei Goto , Hiroshi Shinkai , Hiroyuki Tanaka , Takaki Nakagawa
发明人： Narutoshi Sugita , Katsuhiko Kohyama , Shuhei Goto , Hiroshi Shinkai , Hiroyuki Tanaka , Takaki Nakagawa
IPC分类号： H01M8/10 , H01M8/02 , H01M8/24
CPC分类号： H01M8/0271 , H01M8/0247 , H01M8/0258 , H01M8/0263 , H01M8/241 , H01M8/2483 , H01M2008/1095 , Y02E60/50
摘要： An assembling operation of a fuel cell is effectively simplified. With the simple and economical structure, the desired sealing function is achieved. The fuel cell (10) includes a membrane electrode assembly (14) and first and second metal separators (16, 18) sandwiching the membrane electrode assembly (14). Connection channels (28a, 28b) are provided on the first metal separator (16). The connection channels (28a, 28b) connect the oxygen-containing gas supply passage (20a) and the oxygen-containing gas discharge passage (20b) to the oxygen-containing gas flow field (26). The membrane electrode assembly (14) has first overlapping portions (66a, 66b) overlapped on the connection channels (28a, 28b) for sealing the connection channels (28a, 28b). The first overlapping portions (66a, 66b) comprise, in effect, a gas diffusion layer.
摘要翻译：有效地简化燃料电池的组装操作。通过简单经济的结构，实现了所需的密封功能。燃料电池（10）包括膜电极组件（14）和夹着膜电极组件（14）的第一和第二金属隔板（16,18）。连接通道（28a，28b）设置在第一金属分离器（16）上。连接通道（28a，28b）将含氧气体供给通路（20a）和含氧气体排出通路（20b）连接到含氧气体流场（26）。膜电极组件（14）具有重叠在连接通道（28a，28b）上的第一重叠部分（66a，66b），用于密封连接通道（28a，28b）。实际上，第一重叠部分（66a，66b）包括气体扩散层。

6. 发明申请

US20070042261A1 Solid polymer electrolyte fuel cell and electrode structure for the fuel cell 有权
标题翻译：固体聚合物电解质燃料电池和燃料电池的电极结构
公开(公告)号：US20070042261A1
公开(公告)日：2007-02-22
申请号：US10551349
申请日：2004-03-26
申请人： Katsuhiko Kohyama , Hiroshi Shinkai , Hiroyuki Tanaka
发明人： Katsuhiko Kohyama , Hiroshi Shinkai , Hiroyuki Tanaka
IPC分类号： H01M8/10 , H01M8/02 , H01M4/94 , H01M2/08
CPC分类号： H01M8/0247 , H01M8/0258 , H01M8/0263 , H01M8/0271 , H01M8/1004 , H01M8/241 , H01M8/2457 , H01M8/2483
摘要： A solid polymer electrolyte fuel cell (2) is formed from an electrode structure (7) and first and second separators (8, 9). The electrode structure (7) has a solid polymer electrolyte membrane (10), first and second electrode layers (11, 12), and first and second diffusion layers (13, 14). The first separator (8) forms a first gas passage (PH) through which a fuel gas (H) flows, and the second separator (9) forms a second gas passage (PA) through which an oxidizing gas (A) flows. A first jutting-out portion (15) of the solid polymer electrolyte membrane (10) and a second jutting-out portion (16) of the second diffusion layer (14) are joined together over the entire peripheries thereof via a cured adhesive layer (17), and the second jutting-out portion (16) is in a state in which it is impregnated by cured adhesive. A seal (27) of the first separator (8) is in intimate contact with the surface of the first jutting-out portion (15), and a seal (21) of the second separator (9) is in intimate contact with the surface of the second jutting-out portion (16). It is therefore possible to eliminate the problem of leaked fuel gas and oxidizing gas reacting with each other around the electrode structure.
摘要翻译：固体聚合物电解质燃料电池（2）由电极结构（7）和第一和第二隔板（8,9）形成。电极结构（7）具有固体聚合物电解质膜（10），第一和第二电极层（11,12）以及第一和第二扩散层（13,14）。第一分离器（8）形成燃料气体（H）流过的第一气体通道（P H H H），第二分离器（9）形成第二气体通路（P＆lt; A＆gt; （A）流过氧化气体。固体高分子电解质膜（10）的第一突出部分（15）和第二扩散层（14）的第二突出部分（16）通过固化的粘合剂层（在其整个周边）连接在一起 17），第二突出部（16）处于被固化的粘合剂浸渍的状态。第一分离器（8）的密封件（27）与第一突出部分（15）的表面紧密接触，并且第二分离器（9）的密封件（21）与表面紧密接触的第二突出部分（16）。因此可以消除泄漏的燃料气体和氧化气体在电极结构周围彼此反应的问题。

7. 发明授权

US07094492B2 Electrode for polymer electrolyte fuel cell 有权
标题翻译：聚合物电解质燃料电池用电极
公开(公告)号：US07094492B2
公开(公告)日：2006-08-22
申请号：US10268104
申请日：2002-10-10
申请人： Takeshi Matsubara , Katsuhiko Kohyama , Hiroshi Shinkai
发明人： Takeshi Matsubara , Katsuhiko Kohyama , Hiroshi Shinkai
IPC分类号： H01M4/86 , H01M4/96 , C25B11/04
CPC分类号： H01M4/8828 , H01M4/8605 , H01M4/8896 , H01M4/92 , H01M4/96 , H01M8/1004
摘要： A polymer electrolyte fuel cell has a catalytic layer comprising a material and a polymer electrolyte, and the catalytic layer contains a fibrous material such as carbon whiskers or hydrophilic fibers. The polymer electrolyte fuel cell in the present invention having a catalytic layer comprising a catalytic material, an ion conducting material, an electron conducting material, and a void forming agent, and voids having diameters of from 60 to 1000 nm in the catalytic layer has a void volume of from 0.15 to 0.25 cm3/g.
摘要翻译：聚合物电解质燃料电池具有由材料和聚合物电解质构成的催化剂层，催化剂层含有碳晶须或亲水性纤维等纤维材料。在催化剂层中具有催化剂层，离子传导材料，电子传导性材料，空隙形成剂的催化剂层和具有60〜1000nm直径的空隙的本发明的固体高分子型燃料电池具有空隙体积为0.15至0.25cm 3 / g。

8. 发明授权

US08153333B2 Fuel cell with protruded gas diffusion layer 有权
标题翻译：具有突出气体扩散层的燃料电池
公开(公告)号：US08153333B2
公开(公告)日：2012-04-10
申请号：US10558229
申请日：2004-05-21
申请人： Narutoshi Sugita , Katsuhiko Kohyama , Shuhei Goto , Hiroshi Shinkai , Hiroyuki Tanaka , Takaki Nakagawa
发明人： Narutoshi Sugita , Katsuhiko Kohyama , Shuhei Goto , Hiroshi Shinkai , Hiroyuki Tanaka , Takaki Nakagawa
IPC分类号： H01M4/02 , H01M4/36 , H01M8/10
CPC分类号： H01M8/0271 , H01M8/0247 , H01M8/0258 , H01M8/0263 , H01M8/241 , H01M8/2483 , H01M2008/1095 , Y02E60/50
摘要： An assembling operation of a fuel cell is effectively simplified. With the simple and economical structure, the desired sealing function is achieved. The fuel cell includes a membrane electrode assembly and first and second metal separators sandwiching the membrane electrode assembly. Connection channels are provided on the first metal separator. The connection channels connect the oxygen-containing gas supply passage and the oxygen-containing gas discharge passage to the oxygen-containing gas flow field. The membrane electrode assembly has first overlapping portions overlapped on the connection channels for sealing the connection channels. The first overlapping portions comprise, in effect, a gas diffusion layer.
摘要翻译：有效地简化燃料电池的组装操作。通过简单经济的结构，实现了所需的密封功能。燃料电池包括膜电极组件和夹住膜电极组件的第一和第二金属分离器。连接通道设置在第一金属分离器上。连接通道将含氧气体供给通道和含氧气体排出通道连接到含氧气体流场。膜电极组件具有在连接通道上重叠的第一重叠部分，用于密封连接通道。实际上，第一重叠部分包括气体扩散层。

9. 发明授权

US07776464B2 Solid polymer electrolyte fuel cell and electrode structure for the fuel cell 有权
标题翻译：燃料电池固体聚合物电解质燃料电池和电极结构
公开(公告)号：US07776464B2
公开(公告)日：2010-08-17
申请号：US10551349
申请日：2004-03-26
申请人： Katsuhiko Kohyama , Hiroshi Shinkai , Hiroyuki Tanaka
发明人： Katsuhiko Kohyama , Hiroshi Shinkai , Hiroyuki Tanaka
IPC分类号： H01M2/00 , H01M2/02 , H01M2/08
CPC分类号： H01M8/0247 , H01M8/0258 , H01M8/0263 , H01M8/0271 , H01M8/1004 , H01M8/241 , H01M8/2457 , H01M8/2483
摘要： A solid polymer electrolyte fuel cell (2) is formed from an electrode structure (7) and first and second separators (8, 9). The electrode structure (7) has a solid polymer electrolyte membrane (10), first and second electrode layers (11, 12), and first and second diffusion layers (13, 14). The first separator (8) forms a first gas passage (PH) through which a fuel gas (H) flows, and the second separator (9) forms a second gas passage (PA) through which an oxidizing gas (A) flows. A first jutting-out portion (15) of the solid polymer electrolyte membrane (10) and a second jutting-out portion (16) of the second diffusion layer (14) are joined together over the entire peripheries thereof via a cured adhesive layer (17), and the second jutting-out portion (16) is in a state in which it is impregnated by cured adhesive. A seal (27) of the first separator (8) is in intimate contact with the surface of the first jutting-out portion (15), and a seal (21) of the second separator (9) is in intimate contact with the surface of the second jutting-out portion (16). It is therefore possible to eliminate the problem of leaked fuel gas and oxidizing gas reacting with each other around the electrode structure.
摘要翻译：固体聚合物电解质燃料电池（2）由电极结构（7）和第一和第二隔板（8,9）形成。电极结构（7）具有固体聚合物电解质膜（10），第一和第二电极层（11,12）以及第一和第二扩散层（13,14）。第一分离器（8）形成燃料气体（H）流过的第一气体通道（PH），第二分离器（9）形成氧化气体（A）流过的第二气体通道（PA）。固体高分子电解质膜（10）的第一突出部分（15）和第二扩散层（14）的第二突出部分（16）通过固化的粘合剂层（在其整个周边）连接在一起 17），第二突出部（16）处于被固化的粘合剂浸渍的状态。第一分离器（8）的密封件（27）与第一突出部分（15）的表面紧密接触，并且第二分离器（9）的密封件（21）与表面紧密接触的第二突出部分（16）。因此可以消除泄漏的燃料气体和氧化气体在电极结构周围彼此反应的问题。

10. 发明授权

US4829082A Pharmaceutical compositions for the treatment of skin diseases 失效
标题翻译：用于治疗皮肤疾病的药物组合物
公开(公告)号：US4829082A
公开(公告)日：1989-05-09
申请号：US902299
申请日：1986-08-29
申请人： Hiroshi Shinkai , Takao Kishiye
发明人： Hiroshi Shinkai , Takao Kishiye
IPC分类号： C07D311/72 , A61K31/352 , A61K31/355 , A61P17/00
CPC分类号： A61K31/355 , Y10S514/928
摘要： This invention relates to pharmaceutical compositions for the treatment of skin diseases which comprises as an active ingredient vitamin A esters of .alpha.-tocopherol.

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