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1. 发明授权

US4666945A Catalyst composition suitable for synthesis of methanol 失效
标题翻译：适用于合成甲醇的催化剂组合物
公开(公告)号：US4666945A
公开(公告)日：1987-05-19
申请号：US775114
申请日：1985-09-11
申请人： Minoru Osugi , Makoto Takagawa , Tadasi Nakamura , Takashi Kojima , Kinya Tsuji
发明人： Minoru Osugi , Makoto Takagawa , Tadasi Nakamura , Takashi Kojima , Kinya Tsuji
IPC分类号： C07C29/15 , B01J23/00 , B01J23/80 , B01J23/847 , B01J23/86 , B01J27/18 , C07B61/00 , C07C27/00 , C07C29/154 , C07C31/04 , C07C67/00 , C07C27/06 , C07C27/08
CPC分类号： B01J23/80 , C07C29/154 , Y02P20/52
摘要： A catalyst composition comprising copper oxide, zinc oxide and zirconium oxide, the content of zirconium oxide being 30 to 70% by weight. This catalyst composition is useful for synthesis of methanol from carbon monoxide and/or carbon dioxide and hydrogen by a gas-liquid-solid phase fluidized bed method or a gas-solid phase fluidized bed method.
摘要翻译：包含氧化铜，氧化锌和氧化锆的催化剂组合物，氧化锆的含量为30〜70重量％。该催化剂组合物可用于通过气 - 液 - 固相流化床法或气 - 固相流化床法从一氧化碳和/或二氧化碳和氢气合成甲醇。

2. 发明授权

US4386017A Preparation of improved catalyst composition 失效
标题翻译：改进的催化剂组合物的制备
公开(公告)号：US4386017A
公开(公告)日：1983-05-31
申请号：US205594
申请日：1980-11-10
申请人： Tadasi Nakamura , Minoru Osugi , Yoriko Obata , Shuji Ebata
发明人： Tadasi Nakamura , Minoru Osugi , Yoriko Obata , Shuji Ebata
IPC分类号： C07C29/15 , B01J23/80 , C07B61/00 , C07C27/00 , C07C29/154 , C07C31/04 , C07C67/00 , B01J23/08 , B01J21/02 , B01J27/24
CPC分类号： B01J23/80 , C07C29/154 , Y02P20/52
摘要： A process for preparing a catalyst composition comprising copper oxide, zinc oxide and aluminum oxide as essential ingredients and optionally containing boron oxide, which comprises(a) a step of precipitating from an aqueous solution of a water-soluble copper salt optionally containing a water-soluble boron compound the copper component, together with the boron component if it is present, using an alkaline substance selected from alkali carbonates and alkali bicarbonates as a precipitant;(b) a step of blowing carbon dioxide gas into an aqueous dispersion of a zinc compound selected from zinc oxide and zinc hydroxide optionally containing a water-soluble boron compound to convert the zinc compound to basic zinc carbonate and simultaneously precipitate the boron component if it is present; and(c) a step of calcining a mixture of the solid products obtained in steps (a) and (b) in the presence of an alumina precursor compound.The resulting catalyst is useful for synthesizing methanol from a gaseous mixture of carbon monoxide and/or carbon dioxide and hydrogen.
摘要翻译：一种制备包含氧化铜，氧化锌和氧化铝作为必要成分并任选地含有氧化硼的催化剂组合物的方法，其包括（a）从任选含有水溶性铜盐的水溶性铜盐的水溶液中沉淀出的步骤，使用选自碱金属碳酸盐和碱金属碳酸氢盐的碱性物质作为沉淀剂，将铜组分与硼组分一起存在; （b）将任选含有水溶性硼化合物的锌化合物的锌化合物的水分散体吹入二氧化碳气体的步骤，将锌化合物转化为碱式碳酸锌，同时使硼成分沉淀存在; 和（c）在氧化铝前体化合物的存在下煅烧步骤（a）和（b）中获得的固体产物的混合物的步骤。所得催化剂可用于从一氧化碳和/或二氧化碳和氢气的气体混合物合成甲醇。

3. 发明授权

US4547482A Catalyst composition suited for synthesis of methanol 失效
标题翻译：适用于合成甲醇的催化剂组合物
公开(公告)号：US4547482A
公开(公告)日：1985-10-15
申请号：US515933
申请日：1983-07-20
申请人： Minoru Osugi , Tadasi Nakamura , Shuji Ebata
发明人： Minoru Osugi , Tadasi Nakamura , Shuji Ebata
IPC分类号： C07C29/15 , B01J27/16 , B01J27/18 , C07B61/00 , C07C27/00 , C07C29/153 , C07C29/154 , C07C31/04 , C07C67/00 , B01J23/80
CPC分类号： B01J27/1817 , C07C29/153 , Y02P20/52
摘要： A catalyst composition comprising copper oxide, zinc oxide and an oxyacid of phosphorus or its salt; and a method for producing methanol by reacting carbon monoxide and/or carbon dioxide with hydrogen in the vapor phase in the presence of a catalyst, wherein the catalyst is the aforesaid catalyst composition which has been activated by reduction with a hydrogen-containing gas.
摘要翻译：包含氧化铜，氧化锌和磷或其盐的含氧酸的催化剂组合物; 以及在催化剂存在下，使气相中的一氧化碳和/或二氧化碳与氢气反应生成甲醇的方法，其中催化剂是通过用含氢气体还原而活化的上述催化剂组合物。

4. 发明授权

US4806516A Process for producing fluidized catalyst for synthesis of methanol 失效
标题翻译：制备甲醇合成流化催化剂的方法
公开(公告)号：US4806516A
公开(公告)日：1989-02-21
申请号：US77641
申请日：1987-07-24
申请人： Minoru Osugi , Tadasi Nakamura , Yoriko Obata
发明人： Minoru Osugi , Tadasi Nakamura , Yoriko Obata
IPC分类号： B01J23/80 , B01J37/00 , C07B61/00 , C07C27/00 , C07C29/154 , C07C29/16 , C07C31/04 , C07C67/00 , B01J21/02 , B01J21/06 , B01J23/06 , B01J23/72
CPC分类号： C07C29/154 , B01J23/80 , B01J37/0045 , Y02P20/52
摘要： A process for producing a fluidized catalyst for synthesis of methanol, which comprises molding a composition comprising(A) 10 to 55% by weight of a mixture composed of water-insoluble copper, zinc and zirconium compounds convertible respectively to copper, zinc and zirconium oxides under calcination conditions, said mixture optionally containing a boron compound,(B) 45 to 90% by weight of water, and(C) 0.01 to 1% by weight of ammonia into fine particles, and calcining the fine particles.

5. 发明授权

US4014939A Process for producing formaldehyde 失效
标题翻译：生产甲醛的方法
公开(公告)号：US4014939A
公开(公告)日：1977-03-29
申请号：US584366
申请日：1975-06-05
申请人： Minoru Osugi , Takako Endo
发明人： Minoru Osugi , Takako Endo
IPC分类号： B01J23/80 , B01J37/20 , C07C45/00 , C07C45/86 , C07C45/16 , C07C47/04
CPC分类号： C07C45/002 , B01J23/80 , B01J37/20 , C07C45/86
摘要： Methanol is dehydrogenated at 500-750.degree. C. using a catalyst whose active components are copper, zinc and sulfur to form a stable product containing 30 to 85% by weight of formaldehyde, 0 to 2% by weight of water, the balance being methanol.
摘要翻译：使用活性成分为铜，锌和硫的催化剂，在500-750℃下脱甲醇，形成含有30〜85重量％甲醛，0〜2重量％水的稳定产物，余量为甲醇。

6. 发明授权

US4149009A Process for producing methyl formate 失效
标题翻译：甲酸甲酯生产方法
公开(公告)号：US4149009A
公开(公告)日：1979-04-10
申请号：US853234
申请日：1977-11-21
申请人： Mikio Yoneoka , Minoru Osugi
发明人： Mikio Yoneoka , Minoru Osugi
IPC分类号： B01J23/00 , C07B61/00 , C07C67/00 , C07C67/40 , C07C69/06
CPC分类号： C07C67/00 , C07C67/40
摘要： A process for producing methyl formate which comprises dehydrogenating methanol in vapor phase in the presence as a catalyst of copper, zirconium and zinc and optionally aluminum is disclosed.
摘要翻译：公开了一种生产甲酸甲酯的方法，其包括在作为铜，锆和锌以及任选的铝的催化剂存在下气相中的甲醇脱氢。

7. 发明授权

US06716403B2 Method of recovering a cleaning agent 失效
公开(公告)号：US06716403B2
公开(公告)日：2004-04-06
申请号：US09986606
申请日：2001-11-09
申请人： Kenji Otsuka , Takashi Shimada , Minoru Osugi , Kei Kawaguchi
发明人： Kenji Otsuka , Takashi Shimada , Minoru Osugi , Kei Kawaguchi
IPC分类号： C01G300
CPC分类号： C22B3/44 , B01J23/92 , B01J23/94 , B01J38/60 , B01J38/68 , C22B7/009 , C22B15/00 , Y02P10/214 , Y02P10/234
摘要： The invention provides a method of recovering a copper component or a manganese component from a cleaning agent containing copper oxide, a cleaning agent containing basic copper carbonate, a cleaning agent containing copper hydroxide, or a cleaning agent containing copper oxide and manganese oxide, the cleaning agents having been used for removing, through contact with a harmful gas, a phosphine contained as a harmful component in the harmful gas. Also, the invention provides a method of recovering a copper component or a manganese component from a cleaning agent containing basic copper carbonate, a cleaning agent containing copper hydroxide, or a cleaning agent containing copper oxide and manganese oxide, the cleaning agents having been used for removing, through contact with a harmful gas, a phosphine contained as a harmful component in the harmful gas. According to the present invention, the copper component and/or the manganese component can be effectively recovered from the cleaning agents in a recyclable form.

8. 发明授权

US4232171A Process for producing methyl formate 失效
标题翻译：甲酸甲酯生产方法
公开(公告)号：US4232171A
公开(公告)日：1980-11-04
申请号：US28681
申请日：1979-04-10
申请人： Mikio Yoneoka , Minoru Osugi , Takeo Ikarashi
发明人： Mikio Yoneoka , Minoru Osugi , Takeo Ikarashi
IPC分类号： C07C69/06 , B01J23/00 , B01J23/72 , C07C20060101 , C07C67/00 , C07C67/40
CPC分类号： C07C67/40
摘要： A process for producing methyl formate which comprises dehydrogenating methanol in the vapor phase in the presence of a catalyst containing copper and a cement is disclosed.
摘要翻译：公开了一种生产甲酸甲酯的方法，该方法包括在含有铜和水泥的催化剂存在下，使气相中的甲醇脱氢。

9. 发明授权

US4054609A Process for the preparation for formaldehyde 失效
标题翻译：甲醛制备方法
公开(公告)号：US4054609A
公开(公告)日：1977-10-18
申请号：US697255
申请日：1976-06-17
申请人： Minoru Osugi , Takako Uchiyama
发明人： Minoru Osugi , Takako Uchiyama
IPC分类号： C07C47/055 , B01J23/00 , B01J27/057 , C07B61/00 , C07C45/00 , C07C47/052 , C07C67/00 , C07C47/04
CPC分类号： B01J27/0573 , C07C45/002
摘要： A process for the preparation of formaldehyde by subjecting methanol to dehydrogenation in the presence of a catalyst consisting of copper, zinc and selenium as metallic components.
摘要翻译：在由铜，锌和硒作为金属组分的催化剂存在下使甲醇脱氢而制备甲醛的方法。

10. 发明授权

US07297315B2 Method of recovering a cleaning agent 失效
标题翻译：回收清洗剂的方法
公开(公告)号：US07297315B2
公开(公告)日：2007-11-20
申请号：US10768671
申请日：2004-02-02
申请人： Kenji Otsuka , Takashi Shimada , Minoru Osugi , Kei Kawaguchi
发明人： Kenji Otsuka , Takashi Shimada , Minoru Osugi , Kei Kawaguchi
IPC分类号： C01G3/00
CPC分类号： C22B3/44 , B01J23/92 , B01J23/94 , B01J38/60 , B01J38/68 , C22B7/009 , C22B15/00 , Y02P10/214 , Y02P10/234
摘要： The invention provides a method of recovering a copper component or a manganese component from a cleaning agent containing copper oxide, a cleaning agent containing basic copper carbonate, a cleaning agent containing copper hydroxide, or a cleaning agent containing copper oxide and manganese oxide, the cleaning agents having been used for removing, through contact with a harmful gas, a phosphine contained as a harmful component in the harmful gas. Also, the invention provides a method of recovering a copper component or a manganese component from a cleaning agent containing basic copper carbonate, a cleaning agent containing copper hydroxide, or a cleaning agent containing copper oxide and manganese oxide, the cleaning agents having been used for removing, through contact with a harmful gas, a phosphine contained as a harmful component in the harmful gas. According to the present invention, the copper component and/or the manganese component can be effectively recovered from the cleaning agents in a recyclable form.
摘要翻译：本发明提供一种从含有氧化铜的清洗剂，含碱性碳酸铜的清洗剂，含有氢氧化铜的清洗剂或含有氧化铜和氧化锰的清洗剂中回收铜成分或锰成分的方法，已经用于通过与有害气体接触除去在有害气体中作为有害成分含有的磷化氢的试剂。另外，本发明提供了从含有碱性碳酸铜的清洗剂，含有氢氧化铜的清洗剂或含有氧化铜和氧化锰的清洗剂中回收铜成分或锰成分的方法，所述清洗剂已被用于通过与有害气体的接触除去在有害气体中作为有害成分含有的磷化氢。根据本发明，可以以可回收的形式从清洗剂中有效地回收铜成分和/或锰成分。

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