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1. 发明授权

US4698324A Method for manufacture of catalyst composite having gold or mixture of gold with catalytic metal oxide deposited on carrier 失效
标题翻译：制备具有金或催化金属氧化物的金的混合物沉积在载体上的催化剂复合物的方法
公开(公告)号：US4698324A
公开(公告)日：1987-10-06
申请号：US898945
申请日：1986-08-21
申请人： Masatake Haruta , Hiroshi Sano , Tetsuhiko Kobayashi
发明人： Masatake Haruta , Hiroshi Sano , Tetsuhiko Kobayashi
IPC分类号： B01D53/86 , B01J23/52 , B01J23/68 , B01J23/89 , F23D14/18 , B01J23/72 , B01J23/74
CPC分类号： B01J23/52 , B01J23/685 , B01J23/688 , B01J23/89
摘要： A catalyst composite having gold or a mixture of gold with a catalytic metal oxide deposited on a carrier is produced by immersing a carrier in an aqueous solution containing a water-soluble salt of gold or water-soluble salts respectively of gold and other catalytic metal and urea and/or acetamide thereby allowing a precipitate to be deposited on the carrier and then firing the carrier holding the deposited precipitate thereon.
摘要翻译：通过将载体浸入含有金或其它催化金属的金或水溶性盐的水溶性盐的水溶液中制备具有金或金与沉积在载体上的催化金属氧化物的混合物的催化剂复合物，以及脲和/或乙酰胺，从而使沉淀物沉积在载体上，然后在其上烧结保持沉积的沉淀物的载体。

2. 发明授权

US4839327A Method for the production of ultra-fine gold particles immobilized on a metal oxide 失效
标题翻译：用于生产固定在金属氧化物上的超细金颗粒的方法
公开(公告)号：US4839327A
公开(公告)日：1989-06-13
申请号：US171810
申请日：1988-03-22
申请人： Masatake Haruta , Tetsuhiko Kobayashi
发明人： Masatake Haruta , Tetsuhiko Kobayashi
IPC分类号： G01N27/12 , B01D53/94 , B01J23/52 , B01J23/68 , B01J23/89 , B22F1/02 , C01B13/14 , C01G3/02 , C01G45/02 , C01G49/02 , C01G51/04 , C01G53/04 , C04B41/45 , C04B41/81 , H01M4/86 , H01M4/90
CPC分类号： C04B41/009 , B01J23/52 , B01J23/68 , B01J23/89 , C04B41/4584 , C04B41/81 , H01M4/90 , H01M2004/8684
摘要： A composite having ultra-fine gold particles uniformly and strongly immobilized in a deposited state on a metal oxide is obtained by preparing a solution containing the metal oxide as a carrier and a gold compound, adjusting the pH value of the solution to a specific level thereby inducing precipitation and deposition of gold hydroxide or gold on the carrier and, when the precipitate is in the form of gold hydroxide, further, firing the precipitate. The ultra-fine gold particles immobilized on metal oxides are useful as a catalyst for reduction and oxidation, in sensor elements for flammable gases, and as an electrode catalyst.
摘要翻译：通过制备包含金属氧化物作为载体的溶液和金化合物，将溶液的pH值调节到特定的水平，得到在金属氧化物上以沉积状态均匀且牢固固定的超细金粒子的复合体，在载体上引起金氢氧化物或金沉淀和沉积，并且当沉淀物为氢氧化金的形式时，进一步烧制沉淀物。固定在金属氧化物上的超细金颗粒可用作还原和氧化的催化剂，可燃气体的传感器元件和电极催化剂。

3. 发明授权

US5051394A Method for production of ultra-fine gold particle-immobilized oxides 失效
标题翻译：用于生产超细金颗粒固定氧化物的方法
公开(公告)号：US5051394A
公开(公告)日：1991-09-24
申请号：US484238
申请日：1990-02-26
申请人： Masatake Haruta , Tetsuhiko Kobayashi , Susumu Tsubota , Yoshiko Nakahara
发明人： Masatake Haruta , Tetsuhiko Kobayashi , Susumu Tsubota , Yoshiko Nakahara
IPC分类号： C01B13/36 , B01J23/66 , C01F7/34 , C01G7/00 , C01G9/02 , C01G19/02 , C01G23/053 , C07C55/06 , C07C55/08 , C07C55/10 , C07C55/12 , C07C57/145 , C07C59/06 , C07C59/08 , C07C59/245 , C07C59/255 , C07C59/265
CPC分类号： C07C59/245 , B01J23/66 , C07C55/06 , C07C55/08 , C07C55/10 , C07C55/12 , C07C57/145 , C07C59/06 , C07C59/08 , C07C59/255 , C07C59/265
摘要： An ultra-fine gold particle-immobilized oxide is produced by a method which comprises adding an alkali compound to an aqueous solution containing a gold compound and a water-soluble metal salt thereby giving rise to a coprecipitate in the aqueous solution, separating the coprecipitate from the aqueous solution, and calcining the separated coprecipitate. This method is characterized by allowing the presence of a carboxylic acid or a carboxylate in the aqueous solution from the beginning or after the occurrence of the coprecipitate.
摘要翻译：通过包括向含有金化合物和水溶性金属盐的水溶液中加入碱性化合物，从而在水溶液中引起共沉淀物的方法制备超细金颗粒固定氧化物，将共沉淀物从水溶液，并煅烧分离的共沉淀物。该方法的特征在于从共沉淀物的开始或发生之后，在水溶液中存在羧酸或羧酸盐。

4. 发明授权

US4937219A Ultra-fine gold particle-immobilized alkaline earth metal compounds and methods for production thereof 失效
标题翻译：超细金颗粒固定碱土金属化合物及其制备方法
公开(公告)号：US4937219A
公开(公告)日：1990-06-26
申请号：US247651
申请日：1988-09-22
申请人： Masatake Haruta , Susumu Tsubota , Tetsuhiko Kobayashi , Yoshiko Nakahara
发明人： Masatake Haruta , Susumu Tsubota , Tetsuhiko Kobayashi , Yoshiko Nakahara
IPC分类号： B01D53/86 , B01J23/66 , B01J27/232 , B01J35/02 , B01J37/03 , C01F5/02 , C01F5/24 , C01F11/02 , C01G23/00 , G01N27/16
CPC分类号： B01J37/031 , B01D53/8628 , B01D53/864 , B01J23/66 , B01J27/232 , G01N27/16
摘要： An ultra-fine gold particle-immobilized alkaline earth metal compound having ultra-fine gold particles immobilized on an alkaline earth metal compound is useful as a catalyst or as an inflammable gas sensor. This compound is produced by (1) adding an aqueous solution of a gold compound dropwise to an aqueous solution containing an alkaline earth metal compound and having a pH value kept in the range of 7 to 11 thereby inducing immobilization of gold hydroxide on the compound, separating from the solution the gold hydroxide-immobilized compound, and calcining the separated compound at a temperature in the range of 80.degree. to 800.degree. C., (2) by adding a reducing agent to an aqueous solution of an alkaline earth metal having a gold compound dissolved therein, (3) by adding carbon dioxide gas or an acidic aqueous solution to an aqueous solution containing a gold compound and an alkaline earth metal compound thereby inducing immobilization of gold hydroxide on the alkaline earth metal compound, separating from the solution the gold hydroxide-immobilized compound, and calcining the separated compound at a temperature in the range of 100.degree. to 800.degree. C., or (4) by coprecipitating a gold compound and an alkaline earth metal and calcining the coprecipitate at a temperature in the range of 80.degree. to 800.degree. C.
摘要翻译：具有固定在碱土金属化合物上的超细金粒子的超细金粒子固定碱土金属化合物可用作催化剂或可燃性气体传感器。该化合物通过（1）将金化合物的水溶液滴加到含有碱土金属化合物的水溶液中并且将pH值保持在7〜11的范围内，从而引发金氢氧化物固定在化合物上，从金属氢氧化物固定化合物溶液中分离，并在80〜800℃的温度范围内煅烧分离出的化合物，（2）通过向碱土金属的水溶液中加入还原剂金化合物溶解在其中，（3）通过将二氧化碳气体或酸性水溶液加入到含有金化合物和碱土金属化合物的水溶液中，从而导致氢氧化物固定在碱土金属化合物上，与溶液分离金氢氧化物固定化合物，并在100-800℃的温度下煅烧分离的化合物，或（4）通过共沉淀金化合物和碱土金属，并在80至800℃的温度下煅烧共沉淀物。

5. 发明授权

US5879943A Humidity detection method 失效
标题翻译：湿度检测方法
公开(公告)号：US5879943A
公开(公告)日：1999-03-09
申请号：US872940
申请日：1997-06-11
申请人： Masanori Ando , Tetsuhiko Kobayashi , Masatake Haruta
发明人： Masanori Ando , Tetsuhiko Kobayashi , Masatake Haruta
IPC分类号： G01N21/59 , G01N21/81 , G01N33/18
CPC分类号： G01N21/81
摘要： A humidity detection material includes oxide of at least one metal selected from the group consisting of Mg, Ca, Mn, Fe, Co, Ni, and Cu. The metal oxide is preferably in the form of a porous material. The metal oxide is formed preferably in the form of a thin film on a transparent substrate. The humidity detection material is contacted with water vapor in the presence of a gas such as air, and the optical absorbance of the humidity detection material is measured to detect the humidity. The humidity can be detected by an optical method.
摘要翻译：湿度检测材料包括选自Mg，Ca，Mn，Fe，Co，Ni和Cu中的至少一种金属的氧化物。金属氧化物优选为多孔材料的形式。金属氧化物优选在透明基板上以薄膜的形式形成。湿度检测材料在空气等气体的存在下与水蒸汽接触，测定湿度检测材料的吸光度，以检测湿度。可以通过光学方法检测湿度。

6. 发明授权

US5506273A Catalyst for hydrogenation and method for hydrogenation therewith 失效
标题翻译：氢化催化剂及其氢化方法
公开(公告)号：US5506273A
公开(公告)日：1996-04-09
申请号：US263234
申请日：1994-06-21
申请人： Masatake Haruta , Hiroaki Sakurai , Tetsuhiko Kobayashi , Susumu Tsubota , Atsushi Ueda , Masanori Ando
发明人： Masatake Haruta , Hiroaki Sakurai , Tetsuhiko Kobayashi , Susumu Tsubota , Atsushi Ueda , Masanori Ando
IPC分类号： B01J23/52 , B01J23/54 , B01J23/89 , C07C29/154 , C07C29/156 , C07C27/06
CPC分类号： C07C29/154 , B01J23/52 , B01J23/54 , B01J23/89 , C07C29/156 , Y02P20/52
摘要： A catalyst for the hydrogenation of CO and CO.sub.2 consists essentially of a metal oxide and gold. Synthesis of methanol and hydrocarbons by hydrogenation of CO and CO.sub.2 comprises establishing contact between a gaseous mass consisting of CO, CO.sub.2, and hydrogen and a catalyst consisting essentially of a metal oxide and gold.
摘要翻译： CO和CO 2的氢化催化剂主要由金属氧化物和金组成。通过CO和CO 2的氢化合成甲醇和烃包括建立由CO，CO 2和氢组成的气体物质和基本上由金属氧化物和金组成的催化剂之间的接触。

7. 发明授权

US5789337A Material having ultrafine gold particles immobilized thereon and method for production thereof 失效
标题翻译：固定有超细金粒子的材料及其制造方法
公开(公告)号：US5789337A
公开(公告)日：1998-08-04
申请号：US744249
申请日：1996-11-05
申请人： Masatake Haruta , Mitsutaka Okumura , Koji Tanaka , Atsushi Ueda , Susumu Tsubota , Tetsuhiko Kobayashi
发明人： Masatake Haruta , Mitsutaka Okumura , Koji Tanaka , Atsushi Ueda , Susumu Tsubota , Tetsuhiko Kobayashi
IPC分类号： G01N27/12 , B01D53/86 , B01J19/00 , B01J23/38 , B01J23/52 , B01J23/54 , B01J23/68 , B01J23/89 , B01J35/00 , B01J37/02 , B01J37/08 , C01B32/50 , C07F1/12 , G01N27/16 , B01J27/04
CPC分类号： B01J37/0203 , B01D53/8628 , B01D53/864 , B01J23/52 , B01J35/0013 , B01J37/086 , B01D2255/106 , B01J35/006
摘要： A material having ultrafine gold particles immobilized thereon consists essentially of at least one support selected from the group consisting of metal oxides, metal sulfides, and carbonaceous substances and ultrafine gold particles having a maximum particle diameter of 250 angstroms and deposited on the support with strong interaction. The material exhibits high activity as a catalyst for the oxidation of carbon monoxide to carbon dioxide. It is produced by causing a vaporized organic gold complex to contact at least one support selected from the group consisting of metal oxides, metal sulfides, and carbonaceous substances in an atmosphere of reduced pressure thereby inducing adsorption of the vapor of organic gold complex on the support and then heating the product of the adsorption to a temperature in the range of 100.degree.-700.degree. C.
摘要翻译：固定有超细金粒子的材料基本上由选自金属氧化物，金属硫化物和含碳物质的至少一种载体和最大粒径为250埃的超细金颗粒组成，并以强相互作用沉积在载体上。该材料作为用于将一氧化碳氧化成二氧化碳的催化剂具有高活性。通过使蒸发的有机金络合物在减压气氛中与选自金属氧化物，金属硫化物和碳质物质的至少一种载体接触而产生，从而诱导有机金络合物的蒸气吸附在载体上然后将吸附产物加热至100〜700℃的温度。

8. 发明授权

US4302360A Catalyst for catalytic combustion of hydrogen 失效
标题翻译：用于催化燃烧氢的催化剂
公开(公告)号：US4302360A
公开(公告)日：1981-11-24
申请号：US111253
申请日：1980-01-11
申请人： Masatake Haruta , Hirosi Sano , Tomizo Nakamura
发明人： Masatake Haruta , Hirosi Sano , Tomizo Nakamura
IPC分类号： B01J23/68 , B01J23/89 , B01J23/34 , B01J23/50 , B01J23/74
CPC分类号： B01J23/68 , B01J23/8913 , B01J23/8986
摘要： A catalyst for the catalytic combustion of hydrogen, comprising a composite oxide of silver and cobalt and/or manganese. The catalyst permits hydrogen to be burnt safely at low temperatures.
摘要翻译：用于催化燃烧氢的催化剂，其包含银和钴和/或锰的复合氧化物。催化剂允许氢气在低温下安全燃烧。

9. 发明授权

US5688442A Nonlinear optical materials and process for producing the same 失效
标题翻译：非线性光学材料及其制造方法
公开(公告)号：US5688442A
公开(公告)日：1997-11-18
申请号：US640714
申请日：1996-05-01
申请人： Masanori Ando , Kohei Kadono , Masatake Haruta , Toru Sakaguchi , Masaru Miya
发明人： Masanori Ando , Kohei Kadono , Masatake Haruta , Toru Sakaguchi , Masaru Miya
IPC分类号： G02F1/355 , F21V9/00 , G02F1/35
CPC分类号： G02F1/3551 , Y10T428/256
摘要： There are provided a third-order nonlinear optical material comprising a film formed on the surface of a transparent substrate and consisting essentially of an oxide of a metal selected from the group consisting of V, Cr, Mn, Fe, Co, Ni and Cu; and a third-order nonlinear optical material of the type as described above wherein the film additionally contains a metal selected from the group consisting of Au, Ag and Cu in the form of particles dispersed therein and having a particle size of at most 500 nm.
摘要翻译：提供一种三阶非线性光学材料，其包括在透明基板的表面上形成的膜，其基本上由选自V，Cr，Mn，Fe，Co，Ni和Cu的金属的氧化物组成; 以及如上所述类型的三阶非线性光学材料，其中所述膜另外包含选自Au，Ag和Cu中的金属，其分散在其中的颗粒形式，并且具有至多500nm的粒度。

10. 发明申请

US20080008639A1 Catalyst for Carbon Monoxide Removal and Method of Removing Carbon Monoxide With the Catalyst 审中-公开
标题翻译：用于一氧化碳去除的催化剂和用催化剂除去一氧化碳的方法
公开(公告)号：US20080008639A1
公开(公告)日：2008-01-10
申请号：US11628799
申请日：2005-05-17
申请人： Hiroaki Sakurai , Susumu Tsubota , Masatake Haruta , Masato Kiuchi
发明人： Hiroaki Sakurai , Susumu Tsubota , Masatake Haruta , Masato Kiuchi
IPC分类号： B01D53/86 , B01J23/52 , B01J29/12
CPC分类号： B01D53/864 , B01D2255/106 , B01D2257/502 , B01J21/06 , B01J21/063 , B01J23/52 , B01J35/0013 , B01J37/03 , Y10T428/24 , Y10T428/24149
摘要： The present invention provides a method for effectively suppressing the deactivation of a gold nanoparticle catalyst by removing both carbon dioxide and water from a gas to be treated, thereby effectively removing carbon monoxide over a long period of time. The present invention relates to a catalyst for removing carbon monoxide having a carbon dioxide and water remover and a gold nanoparticle catalyst in which gold particles with an average particle diameter of 25 nm or less are supported on a metal oxide; and a method for removing carbon monoxide from a gas containing carbon monoxide, having a step of treating a gas containing carbon monoxide with the carbon dioxide and water remover and the gold nanoparticle catalyst in which gold particles with an average particle diameter of 25 nm or less are supported on a metal oxide.
摘要翻译：本发明提供了一种通过从被处理气体中除去二氧化碳和水来有效地抑制金纳米颗粒催化剂失活的方法，从而有效地长时间地除去一氧化碳。本发明涉及一种除去二氧化碳和除水剂的一氧化碳的催化剂和金纳米颗粒催化剂，其中平均粒径为25nm以下的金颗粒负载在金属氧化物上; 以及从含有一氧化碳的气体中除去一氧化碳的方法，其具有通过二氧化碳和除水剂处理含有一氧化碳的气体的步骤和金纳米颗粒催化剂，其中平均粒径为25nm以下的金颗粒负载在金属氧化物上。

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