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1. 发明授权

US06365764B1 Bridged bis-fluorenyl metallocenes process for the preparation thereof and use thereof in catalysts for the polymerization of olefins 失效
标题翻译：桥联双芴基金属茂方法及其在烯烃聚合催化剂中的应用
公开(公告)号：US06365764B1
公开(公告)日：2002-04-02
申请号：US09596502
申请日：2000-06-19
申请人： Luigi Resconi , Robert L. Jones
发明人： Luigi Resconi , Robert L. Jones
IPC分类号： C07F730
CPC分类号： C07F17/00 , C08F4/61912 , C08F4/61927 , C08F4/65912 , C08F10/00 , C08F110/06 , Y10S526/943 , C08F4/65927 , C08F2500/17
摘要： Metallocene compounds having two fluorenyl ligands bridged with a single silicon or germanium atom, said atom having two substituent groups containing a total of at least four carbon atoms, are useful as catalyst components for the polymerization of olefins. Particularly, it is possible to prepare high molecular weight atactic polypropylene with improved yields with respect to the known catalysts.
摘要翻译：具有两个与单个硅或锗原子桥接的芴基配体的金属茂化合物，所述原子具有两个含有至少四个碳原子的取代基，可用作烯烃聚合的催化剂组分。特别地，相对于已知的催化剂，可以制备具有提高的产率的高分子量无规立构聚丙烯。

2. 发明授权

US07094847B2 Metallocene compounds and use thereof in catalysts for the polymerization of olefins 失效
标题翻译：茂金属化合物及其在烯烃聚合催化剂中的应用
公开(公告)号：US07094847B2
公开(公告)日：2006-08-22
申请号：US09823393
申请日：2001-03-30
申请人： Clyde E. Bishop , Robert L. Jones, Jr. , Krishna Raman , Vu Anh Dang , Lin-Chen Yu , Luigi Resconi , Tiziano Dall'Occo , Maurizio Galimberti
发明人： Clyde E. Bishop , Robert L. Jones, Jr. , Krishna Raman , Vu Anh Dang , Lin-Chen Yu , Luigi Resconi , Tiziano Dall'Occo , Maurizio Galimberti
IPC分类号： C08F4/42
CPC分类号： C08F10/00 , C07C2/862 , C07C49/643 , C07C49/675 , C07F7/0805 , C07F17/00 , C08F4/65912 , C08F4/65922 , C08F4/65927 , C08F110/02 , C08F110/06 , C08F210/16 , Y10S526/943 , C08F2500/12 , C08F2500/17 , C08F2500/03 , C08F2500/20 , C08F210/08 , C08F210/06
摘要： A class of bridged or unbridged metallocene compounds is disclosed, wherein the cyclopentadienyl ligands have two or four adjacent substituents forming one or two alkylenic cycles of from 4 to 8 carbon atoms.These metallocenes are useful as catalyst components for the polymerization of olefins, particularly for the (co)polymerization of ethylene and for the polymerization of propylene.
摘要翻译：公开了一类桥连或未桥连的茂金属化合物，其中环戊二烯基配体具有形成1-4个碳原子的一个或两个亚烷基化循环的两个或四个相邻的取代基。这些金属茂可用作烯烃聚合的催化剂组分，特别是用于乙烯的（共）聚合和丙烯的聚合。

3. 发明授权

US06211108B1 Metallocene compounds and use thereof in catalysts for the polymerization of olefins 失效
公开(公告)号：US06211108B1
公开(公告)日：2001-04-03
申请号：US08417735
申请日：1995-04-05
申请人： Clyde E. Bishop , Robert L. Jones, Jr. , Krishna Raman , Vu Anh Dang , Lin-Chen Yu , Luigi Resconi , Tiziano Dall'Occo , Maurizio Galimberti
发明人： Clyde E. Bishop , Robert L. Jones, Jr. , Krishna Raman , Vu Anh Dang , Lin-Chen Yu , Luigi Resconi , Tiziano Dall'Occo , Maurizio Galimberti
IPC分类号： B01J3100
CPC分类号： C08F10/00 , C07C2/862 , C07C49/643 , C07C49/675 , C07F7/0805 , C07F17/00 , C08F4/65912 , C08F4/65922 , C08F4/65927 , C08F110/02 , C08F110/06 , C08F210/16 , Y10S526/943 , C08F2500/12 , C08F2500/17 , C08F2500/03 , C08F2500/20 , C08F210/08 , C08F210/06
摘要： A class of bridged or unbridged metallocene compounds is disclosed, wherein the cyclopentadienyl ligands have two or four adjacent substituents forming one or two alkylenic cycles of from 4 to 8 carbon atoms. These metallocenes are useful as catalyst components for the polymerization of olefins, particularly for the (co)polymerization of ethylene and for the polymerization of propylene.

4. 发明申请

US20090234084A1 Metallocene Compounds 审中-公开
标题翻译：茂金属化合物
公开(公告)号：US20090234084A1
公开(公告)日：2009-09-17
申请号：US11922668
申请日：2006-06-27
申请人： Michael J. Elder , Robert L. Jones , Luigi Resconi
发明人： Michael J. Elder , Robert L. Jones , Luigi Resconi
IPC分类号： C07D333/78 , B01J31/14 , C08F4/52
CPC分类号： C07F17/00 , C08F4/65912 , C08F110/08 , C08F2420/06 , C08F2500/17 , C08F4/65927
摘要： A metallocene compound of formula (I) wherein M is zirconium titanium or hafnium; X is hydrogen, halogen or an hydrocarbon group; R4, R5, R6, R7, R8, R9, R10, and R11, R12 and R13 are hydrogen atoms, or C1-C40 hydrocarbon radicals optionally containing heteroatoms belonging to groups 13-17 of the Periodic Table of the Elements; R1 and R2, equal to or different from each other, are linear or branched, C1-C20-alkyl radicals, and R3 is a C1-C40 hydrocarbon radical optionally containing heteroatoms belonging to groups 13-17 of the Periodic Table of the Elements;
摘要翻译：式（I）的茂金属化合物，其中M是锆钛或铪; X是氢，卤素或烃基; R 4，R 5，R 6，R 7，R 8，R 9，R 10和R 11，R 12和R 13是氢原子，或任选地含有元素周期表第13-17族杂原子的C 1 -C 40烃基; R1和R2彼此相同或不同，为直链或支链的C1-C20烷基，R3为任选含有元素周期表第13-17族杂原子的C1-C40烃基;

5. 发明授权

US06180733B2 Bridged bis-fluorenyl metallocenes, process for the preparation thereof and use thereof in catalysts for the polymerization of olefins 失效
标题翻译：桥联双芴基金属茂，其制备方法及其在烯烃聚合催化剂中的应用
公开(公告)号：US06180733B2
公开(公告)日：2001-01-30
申请号：US09086807
申请日：1998-05-29
申请人： Luigi Resconi , Robert L. Jones
发明人： Luigi Resconi , Robert L. Jones
IPC分类号： C08F444
CPC分类号： C07F17/00 , C08F4/61912 , C08F4/61927 , C08F4/65912 , C08F10/00 , C08F110/06 , Y10S526/943 , C08F4/65927 , C08F2500/17
摘要： Metallocene compounds having two fluorenyl ligands bridged with a single silicon or germanium atom, said atom having two substituent groups containing a total of at least four carbon atoms, are useful as catalyst components for the polymerization of olefins. Particularly, it is possible to prepare high molecular weight atactic polypropylene with improved yields with respect to the known catalysts.
摘要翻译：具有两个与单个硅或锗原子桥接的芴基配体的金属茂化合物，所述原子具有两个含有至少四个碳原子的取代基，可用作烯烃聚合的催化剂组分。特别地，相对于已知的催化剂，可以制备具有提高的产率的高分子量无规立构聚丙烯。

6. 发明授权

US06054404A Bridged bis-fluorenyl metallocenes, process for the preparation thereof and use thereof in catalysts for the polymerization of olefins 失效
标题翻译：桥联双芴基金属茂，其制备方法及其在烯烃聚合催化剂中的应用
公开(公告)号：US06054404A
公开(公告)日：2000-04-25
申请号：US123385
申请日：1998-07-27
申请人： Luigi Resconi , Robert L. Jones
发明人： Luigi Resconi , Robert L. Jones
IPC分类号： B01J31/00 , C07F7/08 , C07F7/30 , C07F17/00 , C08F4/44 , C08F4/60 , C08F4/602 , C08F4/619 , C08F4/6192 , C08F4/642 , C08F4/659 , C08F4/6592 , C08F10/00 , C08F110/06
CPC分类号： C07F17/00 , C08F10/00 , C08F110/06 , C08F4/61912 , C08F4/61927 , C08F4/65912 , Y10S526/943
摘要： Metallocene compounds having two fluorenyl ligands bridged with a single silicon or germanium atom, said atom having two substituent groups containing a total of at least four carbon atoms, are useful as catalyst components for the polymerization of olefins. Particularly, it is possible to prepare high molecular weight atactic polypropylene with improved yields with respect to the known catalysts.
摘要翻译：具有两个与单个硅或锗原子桥接的芴基配体的金属茂化合物，所述原子具有两个含有至少四个碳原子的取代基，可用作烯烃聚合的催化剂组分。特别地，相对于已知的催化剂，可以制备具有提高的产率的高分子量无规立构聚丙烯。

7. 发明授权

US5786495A Bridged bis-fluorenyl metallocenes, process for the preparation thereof and use thereof in catalysts for the polymerization of olefins 失效
标题翻译：桥联双芴基金属茂，其制备方法及其在烯烃聚合催化剂中的应用
公开(公告)号：US5786495A
公开(公告)日：1998-07-28
申请号：US609721
申请日：1996-03-01
申请人： Luigi Resconi , Robert L. Jones
发明人： Luigi Resconi , Robert L. Jones
IPC分类号： B01J31/00 , C07F7/08 , C07F7/30 , C07F17/00 , C08F4/44 , C08F4/60 , C08F4/602 , C08F4/619 , C08F4/6192 , C08F4/642 , C08F4/659 , C08F4/6592 , C08F10/00 , C08F110/06 , C07F9/00 , C07F7/00 , C07F7/28
CPC分类号： C07F17/00 , C08F10/00 , C08F110/06 , C08F4/61912 , C08F4/61927 , C08F4/65912 , Y10S526/943
摘要： Metallocene compounds of a Group 4 or 5 metal having two fluorenyl ligands bridged with a single silicon or germanium atom, said atom having two substituent groups containing a total of at least four carbon atoms, are useful as catalyst components for the polymerization of olefins. Particularly, it is possible to prepare high molecular weight atactic polypropylene with improved yields with respect to the known catalysts.
摘要翻译：具有两个与单个硅或锗原子桥接的芴基配体的第4或5族金属的金属茂化合物，所述原子具有两个含有至少四个碳原子的取代基，可用作烯烃聚合的催化剂组分。特别地，相对于已知的催化剂，可以制备具有提高的产率的高分子量无规立构聚丙烯。

8. 发明申请

US20140220326A1 MULTI-LAYER BIAXIALLY ORIENTED POLYMER FILM 审中-公开
标题翻译：多层双面聚合物薄膜
公开(公告)号：US20140220326A1
公开(公告)日：2014-08-07
申请号：US14128059
申请日：2012-06-19
申请人： Luigi Resconi , Nina Ackermans , Joachim Fiebig , Kristin Reichelt
发明人： Luigi Resconi , Nina Ackermans , Joachim Fiebig , Kristin Reichelt
IPC分类号： B32B27/08 , B32B7/02 , B32B27/32
CPC分类号： B32B27/08 , B32B7/02 , B32B27/304 , B32B27/308 , B32B27/32 , B32B27/34 , B32B27/36 , B32B2250/03 , B32B2250/24 , B32B2250/40 , B32B2439/70 , C08L23/14 , C08L23/142 , C08L2203/16 , C08L2205/025 , Y10T428/24975 , Y10T428/263 , Y10T428/265 , Y10T428/2826 , C08F210/06 , C08F4/65925 , C08F210/16 , C08F210/14 , C08F2500/03 , C08F2500/12 , C08F2500/15 , C08F2500/26
摘要： A multi-layer biaxially oriented polymer film comprising a core layer (CL) and at least one sealing layer (SL), said sealing layer(s) (SL) comprise(s) a propylene copolymer composition (P) having a comonomer content in the range of 3.0 to 8.0 wt.-%, the comonomers are C5 to C12 α-olefins, said propylene copolymer composition (P) comprises a polypropylene (A) and a polypropylene (B) in the weight ratio [(A)/(B)] of 20/80 to 80/20, wherein said polypropylene (A) has a comonomer content of equal or below 4.0 wt.-%, the comonomers are C5 to C12 α-olefins, and said propylene copolymer (B) has a comonomer content of 4.0 to 20.0 wt.-%, the comonomers are C5 to C12 α-olefins.
摘要翻译：一种包含芯层（CL）和至少一个密封层（SL）的多层双轴取向聚合物膜，所述密封层（SL）包含具有共聚单体含量的丙烯共聚物组合物（P） 3.0〜8.0重量％的范围，共聚单体为C 5〜C 12α-烯烃，所述丙烯共聚物组合物（P）包含聚丙烯（A）和聚丙烯（B），重量比[（A）/（ B）]为20/80至80/20，其中所述聚丙烯（A）的共聚单体含量等于或低于4.0重量％，共聚单体为C 5至C 12α-烯烃，并且所述丙烯共聚物（B）具有共聚单体含量为4.0〜20.0重量％，共聚单体为C 5〜C 12α-烯烃。

9. 发明申请

US20140206819A1 HETEROPHASIC COPOLYMERS 有权
标题翻译：异构共聚物
公开(公告)号：US20140206819A1
公开(公告)日：2014-07-24
申请号：US14131549
申请日：2012-07-06
申请人： Norbert Hafner , Luigi Resconi , Markus Gahleitner , Jimgbo Wang , Pascal Castro , Pavel Sergeevich Kulyabin , Vyatcheslav Izmer , Alexander Virkkunen , Dmitry Kononovich , Ville Virkkunen
发明人： Norbert Hafner , Luigi Resconi , Markus Gahleitner , Jimgbo Wang , Pascal Castro , Pavel Sergeevich Kulyabin , Vyatcheslav Izmer , Alexander Virkkunen , Dmitry Kononovich , Ville Virkkunen
IPC分类号： C08L23/12
CPC分类号： C07F7/081 , C07C13/36 , C07C13/38 , C07C13/465 , C07C41/01 , C07F17/00 , C08F4/65912 , C08F4/65916 , C08F4/65927 , C08F10/06 , C08F110/06 , C08F210/06 , C08L23/12 , C08L2207/02 , C08L2314/06 , C08L23/16 , C08F2500/03 , C08F2500/12 , C08F210/16
摘要： A heterophasic polypropylene resin comprising a polypropylene homopolymer matrix phase (A) and an ethylene-propylene copolymer phase (B) dispersed within the matrix, wherein the xylene soluble fraction of the heterophasic polypropylene resin is in the range 20 to less than 50 wt %; the heterophasic polypropylene resin has an MFR2 of 0.01 to 50 g/10 min; the ethylene content of the xylene soluble fraction of the heterophasic polypropylene resin is in the range of at least 20 wt % to less than 50 wt %; the heterophasic polypropylene resin has a notched charpy impact strength at −20 C of at least 25 kJ/m2, preferably at least 50 kJ/m2; and wherein the MFR2 (Matrix)/MFR2(XS)≧5, preferably ≧10.
摘要翻译：包含分散在基质内的聚丙烯均聚物基质相（A）和乙烯 - 丙烯共聚物相（B）的多相聚丙烯树脂，其中所述多相聚丙烯树脂的二甲苯可溶部分在20至小于50重量％的范围内; 多相聚丙烯树脂的MFR 2为0.01〜50g / 10分钟; 多相聚丙烯树脂的二甲苯可溶级分的乙烯含量在至少20重量％至小于50重量％的范围内; 多相聚丙烯树脂在-20℃下具有至少25kJ / m 2，优选至少50kJ / m 2的缺口夏比冲击强度; 并且其中MFR 2（Matrix）/ MFR 2（XS）≥5，优选≥10。

10. 发明申请

US20140018506A1 BRIDGED METALLOCENE CATALYSTS 有权
标题翻译： BRIDGED METALLOCENE催化剂
公开(公告)号：US20140018506A1
公开(公告)日：2014-01-16
申请号：US13996831
申请日：2011-12-20
申请人： Luigi Resconi , Pascal Castro , Alexander Z. Voskoboynikov , Vyatcheslav V. Izmer , Dmitry S. Kononovich
发明人： Luigi Resconi , Pascal Castro , Alexander Z. Voskoboynikov , Vyatcheslav V. Izmer , Dmitry S. Kononovich
IPC分类号： C08F4/76 , C08F4/52
CPC分类号： C08F4/76 , B01J31/2295 , B01J2231/122 , B01J2531/48 , B01J2531/49 , C07F17/00 , C08F4/52 , C08F4/65908 , C08F4/65927 , C08F10/00 , C08F110/06 , C08F210/06 , C08F4/65912 , C08F2500/03 , C08F2500/12 , C08F210/16
摘要： A solid, particulate catalyst comprising: (i) a complex of formula (I) wherein M is zirconium or hafnium; each X is a sigma ligand; L is a divalent bridge selected from —R′2C—, —R′2C—CR′2—, —R′2Si—, —R′2Si—SiR′2—, —R′2Ge—, wherein each R′ is independently a hydrogen atom, C1-C20-hydrocarbyl, tri(C1-C20-alkyl)silyl, C6-C20-aryl, C7-C20-arylalkyl or C7-C20-alkylaryl; each R1 is a C4-C20 hydrocarbyl radical branched at the β-atom to the cyclopentadienyl ring, optionally containing one or more heteroatoms belonging to groups 14-16, or is a C3-C20 hydrocarbyl radical branched at the β-atom to the cyclopentadienyl ring where the β-atom is an Si-atom; each R18 is a C1-C20 hydrocarbyl radical optionally containing one or more heteroatoms belonging to groups 14-16; each R4 is a hydrogen atom or a C1-6-hydrocarbyl radical; each W is a 5 or 6 membered aryl or heteroaryl ring wherein each atom of said ring is optionally substituted with at least one R5 group; each R5 is the same or different and is a C1-C20 hydrocarbyl radical optionally containing one or more heteroatoms belonging to groups 14-16; and optionally two adjacent R5 groups taken together can form a further mono or multicyclic ring condensed to W optionally substituted by one or two groups R5; and each R7 is a C1-C20 hydrocarbyl radical; and (ii) a cocatalyst, preferably comprising an organometallic compound of a Group 13 metal.
摘要翻译：一种固体颗粒催化剂，其包含：（i）式（I）的络合物，其中M为锆或铪; 每个X是σ配体; L是选自-R'2C-，-R'2C-CR'2-，-R'2Si-，-R'2Si-SiR'2-，-R'2Ge-的二价桥，其中每个R' 独立地为氢原子，C 1 -C 20烃基，三（C 1 -C 20烷基）甲硅烷基，C 6 -C 20 - 芳基，C 7 -C 20 - 芳基烷基或C 7 -C 20 - 烷基芳基; 每个R 1是在β-原子处与环戊二烯基环分支的C 4 -C 20烃基，任选地含有一个或多个属于第14-16族的杂原子，或者是在β-原子处分支到环戊二烯基的C 3 -C 20烃基 β原子是Si原子的环; 每个R18是任选地含有一个或多个属于第14-16族的杂原子的C1-C20烃基; 每个R 4是氢原子或C 1-6烃基; 每个W是5或6元芳基或杂芳基环，其中所述环的每个原子任选被至少一个R 5基团取代; 每个R 5相同或不同，并且是任选地含有一个或多个属于第14-16族的杂原子的C 1 -C 20烃基; 并且任选地两个相邻的R5基团可以形成另外的一个或多个环，其被稠合至可任选地被一个或两个基团R 5取代的W; 并且每个R 7是C 1 -C 20烃基; 和（ii）助催化剂，优选包含第13族金属的有机金属化合物。

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