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1. 发明授权

US06277445B1 Organopolysiloxane compound and composition containing the same 失效
标题翻译：有机聚硅氧烷化合物及其组合物
公开(公告)号：US06277445B1
公开(公告)日：2001-08-21
申请号：US09415222
申请日：1999-10-12
申请人： Kouhei Hasegawa , Motohiko Hirai , Satoshi Kuwata
发明人： Kouhei Hasegawa , Motohiko Hirai , Satoshi Kuwata
IPC分类号： B05D302
CPC分类号： D21H19/32 , C09D183/08 , D21H21/16 , D21H25/06
摘要： Disclosed is a novel modified organopolysiloxane compound characteristically having carboxylalk(en)ylcarbonyl groups substituting for the hydrogen atoms on the N atoms in an aminoalkyl group-containing organopolysiloxane as introduced by the reaction of a dicarboxylic acid anhydride such as maleic anhydride and succinic anhydride with an aminoalkyl group-containing organopolysiloxane. This modified organopolysiloxane compound serves as a principal ingredient in an aqueous emulsion composition for a finishing treatment of various fabric material to impart excellent touch feeling of softness to the fabric material with little problem of yellowing of the fabric material unavoidable with conventional aminoalkyl group-containing organopolysiloxane compounds. The inventive modified organopolysiloxane compound in the form of an aqueous emulsion is also useful for a waterproofing treatment of paperboards for plasterboards to serve as a covering sheet on the core board of hydrated gypsum.
摘要翻译：公开了一种新型改性的有机聚硅氧烷化合物，其特征在于具有取代含氨基烷基的有机聚硅氧烷中的N原子上的氢原子的羧基（烯）基羰基，通过二羧酸酐如马来酸酐和琥珀酸酐与含氨基烷基的有机聚硅氧烷。该改性的有机基聚硅氧烷化合物在水性乳液组合物中作为主要成分，用于各种织物材料的整理处理，以赋予织物材料柔软性优良的接触感，而不需要常规含氨基烷基的有机基聚硅氧烷化合物。本发明的水性乳液形式的改性有机聚硅氧烷化合物也可用于石膏板纸板的防水处理，以用作水合石膏芯板上的覆盖片。

2. 发明授权

US6117420A Hair-care treatment toiletry composition 失效
标题翻译：头发护理化妆水组成
公开(公告)号：US6117420A
公开(公告)日：2000-09-12
申请号：US188098
申请日：1998-11-09
申请人： Satoshi Kuwata , Motohiko Hirai
发明人： Satoshi Kuwata , Motohiko Hirai
IPC分类号： A61K8/72 , A61K8/00 , A61K8/89 , A61K8/893 , A61K8/898 , A61Q5/00 , A61Q5/02 , A61Q5/12 , C08G77/26 , C08G77/388 , C08L83/08 , A61K7/06
CPC分类号： A61Q5/12 , A61K8/898 , A61Q5/02
摘要： Disclosed is a hair-care treatment toiletry composition, such as hair shampoo and hair rinse compositions, capable of imparting excellent smoothness and pliability as well as an adequate moisturized touch feeling to the hair treated therewith. The hair-care treatment toiletry composition contains, as the characteristic ingredient in addition to the usual ingredients acceptable as constituents of a hair-care treatment toiletry composition, a specified amount of a specific morpholino-modified diorganopolysiloxane, e.g., a dimethylpolysiloxane substituted by 3-morpholinopropyl groups for a part of the methyl groups as bonded to the silicon atoms in the organopolysiloxane molecules.
摘要翻译：公开了一种能够赋予对其进行处理的毛发具有优异的平滑性和柔韧性以及足够的保湿触摸感的护发剂洗发剂组合物，例如洗发剂和洗发剂组合物。护发剂洗发剂组合物除了作为头发护理化妆品组合物的成分可接受的通常成分外还含有特定量的特定的吗啉代改性的二有机基聚硅氧烷，例如由3- 一部分甲基的吗啉代丙基与有机聚硅氧烷分子中的硅原子键合。

3. 发明授权

US4990552A Flame retardant silicone oil composition 失效
标题翻译：阻燃硅油组合物
公开(公告)号：US4990552A
公开(公告)日：1991-02-05
申请号：US301084
申请日：1989-01-25
申请人： Shigeru Mori , Satoshi Kuwata , Motohiko Hirai
发明人： Shigeru Mori , Satoshi Kuwata , Motohiko Hirai
IPC分类号： C08K5/00 , C08K5/01 , C08K5/05 , C08K5/5415 , C08K5/5425 , C08L83/04 , C08L83/07 , H01B3/46
CPC分类号： C08K5/01 , C08K5/5415
摘要： A silicone oil used, for example, as an electric insulation oil can be imparted with greatly increased flame retardancy when it is compounded with a soluble platinum compound, e.g., chloroplatinic acid, and an alkynyloxy, e.g., ethynyloxy, containing compound or, in particular, an ethynyloxy-containing organosilicon compound. The heat resistance of the silicone oil composition can be further improved by admixing the composition with an organosilicon compound having at least one imino-containing aromatic group such as a 4-anilinophenoxy group bonded to the silicon atom.
摘要翻译：当与可溶性铂化合物（例如氯铂酸）和炔氧基（例如含乙炔氧基）的化合物复合时，例如作为电绝缘油使用的硅油可以赋予极大增加的阻燃性，含乙炔氧基的有机硅化合物。通过将组合物与具有至少一个含亚氨基的芳族基团的有机硅化合物（例如与硅原子键合的4-苯胺基苯氧基）混合，可以进一步提高硅油组合物的耐热性。

4. 发明申请

US20050053570A1 Hair care products 审中-公开
标题翻译：护发产品
公开(公告)号：US20050053570A1
公开(公告)日：2005-03-10
申请号：US10497140
申请日：2002-11-28
申请人： Motohiko Hirai , Mituhiro Takarada , Naoki Omura , Kiyomi Tachibana
发明人： Motohiko Hirai , Mituhiro Takarada , Naoki Omura , Kiyomi Tachibana
IPC分类号： A61K8/894 , A61K8/895 , A61K8/898 , A61Q5/00 , A61Q5/06 , A61Q5/12 , A61K7/06 , A61K7/11
CPC分类号： A61K8/894 , A61K8/898 , A61K2800/594 , A61Q5/00 , A61Q5/06 , A61Q5/12
摘要： It is a hair-care toiletry composition containing 0.01-20% by weight of a composition (A) consisting of a single kind or two kinds or more of the organopolysiloxanes having an amino group and a polyoxyalkylene group as represented by the general formulas (1), (2), (3) and (4) given below. R1R2R3Si—[O—Si(R1)2]n—OSiR1R2R3; (1) R3R22Si—[O—Si(R1)2]n—OSiR3R22; (2) R3R2R1Si—[O—Si(R1)2]n—OSiR13; and (3) R3R22Si—[O—Si(R1)2]n—OSiR13. (4)Besides, the hair-care toiletry composition of the present invention is a combination of the organopolysiloxane as the composition (A) with (B) a cationic surface active agent or a combination of (A) with (C) an anionic surface active agent and/or an amphoteric surface active agent.
摘要翻译：包含0.01〜20重量％的由通式（1）表示的具有氨基和聚氧化烯基的单种或两种以上的有机聚硅氧烷组成的组合物（A）为0.01〜20重量％），（2），（3）和（4）。 R 1 R 2 R 3 Si- [O-Si（R 1）2] n-OSiR 1 R 2 R 3; （1）R 3 R 2 2Si- [O-Si（R 1）2] n-OSiR 3 R 2; （2）R 3 R 2 R 1 Si- [O-Si（R 1）2] n-OSiR 1 3; 和（3）R 3 R 2 2Si- [O-Si（R 1）2] n-OSiR 1 3。（4）此外，本发明的护发梳妆用组合物是作为组合物（A）的有机聚硅氧烷与（B）阳离子表面活性剂或（A）与（C）阴离子表面的组合的组合活性剂和/或两性表面活性剂。

5. 发明授权

US08329816B2 Silicone microemulsion composition 有权
标题翻译：硅胶微乳液组合物
公开(公告)号：US08329816B2
公开(公告)日：2012-12-11
申请号：US13448651
申请日：2012-04-17
申请人： Yuji Ando , Motohiko Hirai
发明人： Yuji Ando , Motohiko Hirai
IPC分类号： C08K3/00
CPC分类号： A61K8/068 , A61K8/89 , A61Q19/00 , C08G77/14 , C08G77/46 , C08L83/12 , C08L83/00
摘要： A silicone microemulsion composition obtained by microemulsifying a carboxy-modified organopolysiloxane, and having a lower surface tension than conventional microemulsions. The composition includes 100 parts by mass of a specific carboxy-modified organopolysiloxane (A), 25 to 75 parts by mass of a specific polyether-modified organopolysiloxane (B), 0.1 to 10 parts by mass of an anionic surfactant, and 20 to 6,000 parts by mass of water, wherein the average particle size of the emulsion particles is not more than 100 nm.
摘要翻译：通过微乳化羧基改性的有机聚硅氧烷并且具有比常规微乳液更低的表面张力获得的硅氧烷微乳液组合物。该组合物包含100质量份特定的羧基改性的有机聚硅氧烷（A），25〜75质量份的特定的聚醚改性的有机聚硅氧烷（B），0.1〜10质量份的阴离子表面活性剂和20〜6,000 质量份的水，乳液颗粒的平均粒径不大于100nm。

6. 发明申请

US20120270985A1 SILICONE MICROEMULSION COMPOSITION 有权
标题翻译：硅胶微乳液组合物
公开(公告)号：US20120270985A1
公开(公告)日：2012-10-25
申请号：US13448651
申请日：2012-04-17
申请人： Yuji ANDO , Motohiko Hirai
发明人： Yuji ANDO , Motohiko Hirai
IPC分类号： C08K5/053 , C08L83/06 , B82Y30/00
CPC分类号： A61K8/068 , A61K8/89 , A61Q19/00 , C08G77/14 , C08G77/46 , C08L83/12 , C08L83/00
摘要： A silicone microemulsion composition obtained by microemulsifying a carboxy-modified organopolysiloxane, and having a lower surface tension than conventional microemulsions. The composition includes 100 parts by mass of a specific carboxy-modified organopolysiloxane (A), 25 to 75 parts by mass of a specific polyether-modified organopolysiloxane (B), 0.1 to 10 parts by mass of an anionic surfactant, and 20 to 6,000 parts by mass of water, wherein the average particle size of the emulsion particles is not more than 100 nm.
摘要翻译：通过微乳化羧基改性的有机聚硅氧烷并且具有比常规微乳液更低的表面张力获得的硅氧烷微乳液组合物。该组合物包含100质量份特定的羧基改性的有机聚硅氧烷（A），25〜75质量份的特定的聚醚改性的有机聚硅氧烷（B），0.1〜10质量份的阴离子表面活性剂和20〜6,000 质量份的水，乳液颗粒的平均粒径不大于100nm。

7. 发明授权

US4775493A Flame-retardant silicone fluid composition 失效
标题翻译：阻燃硅油组合物
公开(公告)号：US4775493A
公开(公告)日：1988-10-04
申请号：US132931
申请日：1987-12-15
申请人： Shigeru Mori , Motohiko Hirai
发明人： Shigeru Mori , Motohiko Hirai
IPC分类号： H01B3/46 , C08K3/16 , C08K3/24 , C08K5/02 , C08L83/04 , C08L83/07
CPC分类号： C08K3/16 , C08L83/04 , C08G77/20 , C08G77/24 , C08G77/26 , C08G77/70
摘要： Silicone fluid-based electric insulation oils can be imparted with greatly enhanced flame retardancy when the base organopolysiloxane contains 0.1 to 30% by moles of vinyl groups relative to the monovalent hydrocarbon groups bonded to the silicone atoms and is admixed with a platinum compound soluble therein, such as chloroplatinic acid, dissolved thereiin in a specified amount. The flame retardancy of the organopolysiloxane/platinum compound composition can be further improved by the addition of a low-viscosity fluorinated hydrocarbon oil such as an oligomeric polymer of chlorotrifluoroethylene.

8. 发明授权

US08101533B2 Fabric treating composition, detergent and softener, and fabric article treated therewith 有权
标题翻译：织物处理组合物，洗涤剂和柔软剂以及用其处理的织物制品
公开(公告)号：US08101533B2
公开(公告)日：2012-01-24
申请号：US12468427
申请日：2009-05-19
申请人： Motohiko Hirai
发明人： Motohiko Hirai
IPC分类号： B32B5/02 , B32B27/04 , B32B27/12 , C08G77/04
CPC分类号： C11D3/3742 , Y10T442/20 , Y10T442/2311 , Y10T442/2328 , Y10T442/2352 , Y10T442/2393
摘要： A fabric treating composition comprising primarily an organopolysiloxane of formula (1) having a viscosity of 100 to 1,000,000 mPa-s at 25° C. is provided. R1 is a monovalent hydrocarbon group, R2 is a monovalent organic group of formula: —R4(NR5CH2CH2)aNR6R7 wherein R4 is a divalent hydrocarbon group, R5 to R7 are hydrogen, monovalent hydrocarbon groups, or R8, R8 is a group of formula: —(CO—C5H10O)b—R9 (R9 is hydrogen or a monovalent hydrocarbon group, b is 1 to 50), a is 0 to 4, with the proviso that at least one of R5, R6 and R7 present in the organopolysiloxane is R8, R3 is hydroxyl, —OR10, R1, or R2, R10 being a monovalent hydrocarbon group, m is 10 to 1,500, and n is 0 to 100, with the proviso that when n=0, at least one R3 is R2.
摘要翻译：提供主要包含在25℃下粘度为100至1,000,000mPa·s的式（1）的有机聚硅氧烷的织物处理组合物。 R1是一价烃基，R2是下式的-R4（NR5CH2CH2）aNR6R7的一价有机基团，其中R4是二价烃基，R5至R7是氢，一价烃基或R8，R8是下式的基团： - （CO-C5H10O）b-R9（R9为氢或一价烃基，b为1至50），a为0至4，条件是存在于有机聚硅氧烷中的R5，R6和R7中的至少一个为 R8，R3为羟基，-OR10，R1或R2，R10为一价烃基，m为10〜1500，n为0〜100，条件是当n = 0时，至少一个R 3为R 2。

9. 发明授权

US5356549A Silicone grease 失效
标题翻译：硅油脂
公开(公告)号：US5356549A
公开(公告)日：1994-10-18
申请号：US6286
申请日：1993-01-19
申请人： Takayuki Takahashi , Motohiko Hirai
发明人： Takayuki Takahashi , Motohiko Hirai
IPC分类号： C10M105/76 , C10M169/00 , C10M169/02 , C10N20/00 , C10N20/02 , C10N30/08 , C10N50/10 , C10N60/00
CPC分类号： C10M169/00 , C10M169/02 , C10M2201/041 , C10M2201/0416 , C10M2201/042 , C10M2201/0426 , C10M2201/0606 , C10M2201/0616 , C10M2201/062 , C10M2201/0626 , C10M2201/0656 , C10M2201/0666 , C10M2201/0806 , C10M2201/0856 , C10M2201/0866 , C10M2201/0876 , C10M2201/1013 , C10M2201/1026 , C10M2201/103 , C10M2201/1036 , C10M2201/105 , C10M2201/12 , C10M2201/126 , C10M2207/024 , C10M2207/1225 , C10M2207/1245 , C10M2207/125 , C10M2207/1265 , C10M2207/1285 , C10M2207/129 , C10M2207/166 , C10M2207/186 , C10M2207/206 , C10M2207/246 , C10M2207/281 , C10M2207/282 , C10M2207/283 , C10M2207/284 , C10M2207/286 , C10M2211/006 , C10M2211/022 , C10M2211/04 , C10M2211/06 , C10M2211/066 , C10M2211/086 , C10M2213/02 , C10M2213/062 , C10M2215/006 , C10M2215/026 , C10M2215/062 , C10M2215/064 , C10M2215/0813 , C10M2215/1013 , C10M2215/102 , C10M2215/1026 , C10M2215/121 , C10M2215/22 , C10M2215/2206 , C10M2215/221 , C10M2215/223 , C10M2215/225 , C10M2215/226 , C10M2215/227 , C10M2215/2275 , C10M2215/30 , C10M2223/04 , C10M2223/041 , C10M2229/025 , C10M2229/0405 , C10M2229/0415 , C10M2229/0425 , C10M2229/0435 , C10M2229/0445 , C10M2229/0455 , C10M2229/0465 , C10M2229/0475 , C10M2229/0485 , C10M2229/0505 , C10M2229/0515 , C10M2229/052 , C10M2229/0525 , C10M2229/0535 , C10M2229/0545 , C10N2210/00 , C10N2210/01 , C10N2210/02 , C10N2210/03 , C10N2210/04 , C10N2220/02
摘要： Silicone grease comprising (A) an amino-modified silicone fluid having an amine equivalent of 10,000 to 200,000 g/mol and a viscosity of 10 to 100,000 cs at 25.degree. C., and (B) a thickener exhibits improved heat resistance and low-temperature resistance.
摘要翻译：硅氧烷润滑脂包含（A）氨基改性的硅氧烷流体，其胺当量为10,000至200,000g / mol，在25℃下的粘度为10至100,000cs，和（B）增稠剂具有改善的耐热性，耐温性。

10. 发明授权

US6001422A Method for finishing treatment of a fabric material 失效
标题翻译：织物材料整理处理方法
公开(公告)号：US6001422A
公开(公告)日：1999-12-14
申请号：US58162
申请日：1998-04-10
申请人： Motohiko Hirai , Fujio Yagihashi
发明人： Motohiko Hirai , Fujio Yagihashi
IPC分类号： C07F7/08 , C07F7/18 , C08L83/08 , D06M15/643 , D06M101/00 , D06M101/02 , D06M101/06 , D06M101/08 , B05D3/02
CPC分类号： D06M15/6436 , D06M2101/06 , D06M2101/08 , D06M2101/12 , D06M2101/26 , D06M2101/32 , D06M2101/34 , D06M2101/38 , D06M2200/25 , D06M2200/50
摘要： Proposed is a method for the finishing treatment of various kinds of fabric materials with an aminoalkyl-modified dimethylpolysiloxane to impart the fabric material with excellent softness and smoothness with less disadvantages of yellowing of the treated fabric material than in the prior art using similar aminoalkyl-modified dimethylpolysiloxanes. In the inventive method, the aminoalkyl-modified dimethylpolysiloxane is represented by the general formulaA--SiR.sub.2 --O--(--SiR.sub.2 --O--).sub.p --(--SiRQ--O--).sub.q --SiR.sub.2 --A,in which R is a monovalent hydrocarbon group having 1 to 20 carbon atoms, Q is an aminoalkyl group expressed by the general formula--R.sup.1 --(--NH--CH.sub.2 --CH.sub.2 --).sub.n --NH.sub.2,R.sup.1 being a divalent hydrocarbon group having 1 to 8 carbon atoms and the subscript n being 2 or 3, A is a hydroxyl group, R, OR or Q, the subscript p is an average number in the range from 5 to 2000 and the subscript q is 0 or an average number not exceeding 100 with the proviso that q is not 0 when the groups denoted by A in a molecule are each a hydroxyl group, R or OR, and having an amine equivalent in the range from 5000 to 100,000 g/mole.
摘要翻译：提出了使用氨基烷基改性的二甲基聚硅氧烷对各种织物进行精加工处理的方法，以使得织物材料具有优异的柔软性和光滑度，而与已有技术相似的氨基烷基改性的处理过的织物材料变黄的缺点较少二甲基聚硅氧烷。在本发明的方法中，氨基烷基改性的二甲基聚硅氧烷由通式A-SiR2-O-（-SiR2-O-）p - （ - SiRQ-O-）q-SiR2-A表示，其中R是一价 Q为由通式-R1 - （ - NH-CH2-CH2-）n-NH2表示的氨基烷基，R1为碳原子数为1〜8的二价烃基，下标为 n为2或3，A为羟基，R，OR或Q，下标p为5至2000的平均数，下标q为0或平均数不超过100，条件是q 分子中由A表示的基团各自为羟基，R或OR，胺当量为5000〜100,000g / mol时，不为0。

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