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1. 发明授权

US06455597B2 Catalytic partial oxidation — particulate catalysts 失效
标题翻译：催化部分氧化 - 颗粒催化剂
公开(公告)号：US06455597B2
公开(公告)日：2002-09-24
申请号：US09791985
申请日：2001-02-23
申请人： Keith L. Hohn , Lanny D. Schmidt , Sebastian C. Reyes , Jennifer S. Feeley
发明人： Keith L. Hohn , Lanny D. Schmidt , Sebastian C. Reyes , Jennifer S. Feeley
IPC分类号： C07C2700
CPC分类号： C01B3/386 , C01B3/40 , C01B2203/0261 , C01B2203/062 , C01B2203/1017 , C01B2203/1023 , C01B2203/1047 , C01B2203/1052 , C01B2203/1064 , C01B2203/1082 , C01B2203/1241 , Y02P20/52
摘要： Catalytic partial oxidation is effected in the presence of a supported, Group VIII metal catalyst by reacting a light hydrocarbon with an oxygen containing gas, the catalyst support being in a preferred size range.
摘要翻译：在负载的VIII族金属催化剂的存在下，通过使轻质烃与含氧气体反应，催化剂载体处于优选的尺寸范围内进行催化部分氧化。

2. 发明授权

US06726850B1 Catalytic partial oxidation using staged oxygen addition 失效
标题翻译：使用分期加氧的催化部分氧化
公开(公告)号：US06726850B1
公开(公告)日：2004-04-27
申请号：US09484378
申请日：2000-01-14
申请人： Sebastian C. Reyes , Jennifer S. Feeley , Frank Hershkowitz , Harry W. Deckman , Ioannis P. Androulakis
发明人： Sebastian C. Reyes , Jennifer S. Feeley , Frank Hershkowitz , Harry W. Deckman , Ioannis P. Androulakis
IPC分类号： C01B326
CPC分类号： C01B3/386 , C01B2203/0261 , C01B2203/061 , C01B2203/062 , C01B2203/065 , C01B2203/1011 , C01B2203/1029 , C01B2203/1052 , C01B2203/1064 , C01B2203/1082 , C01B2203/1241 , C01B2203/1276
摘要： A multistage catalytic partial oxidation (CPO) process for oxidizing a hydrocarbon feedstream comprising C1-C4 hydrocarbons, with an oxygen-containing feedstream to produce a product comprising CO and H2, also known as synthesis gas or syngas. The process employs a CPO catalyst, and controlled process features, including: (A) the total oxygen requirement for the process is introduced incrementally, in more than one reaction stage, using an oxygen-containing feedstream at more than one feed point in the process, each stage including a catalyst; (B) the oxygen-containing feedstream, hydrocarbon feedstream and, in reaction stages after the first of said multiple stages, the intermediate product produced in the prior stage, are mixed for a period of time, after they are brought into contact with one another, of less than about 1 millisecond to form a substantially uniform mixture, wherein the mixture is then contacted with the catalyst; (C) the oxygen-containing feedstream and the hydrocarbon feedstream are preheated prior to entry into the first stage, to a temperature of from about 450° C. to less than about 1,000° C.; and (D) the mixture temperature of the product in each stage following the first stage is from greater than about 600° C. to less than about 1,000° C. Preferably, the process comprises less than or equal to about five stages, the first stage preheat temperature recited in step (C) is greater than about 550° C. and the mixture temperature of the product in each stage following the first stage is at least 700° C.
摘要翻译：用于将包含C1-C4烃的烃进料流与含氧进料流氧化以产生包含CO和H 2的产物（也称为合成气或合成气）的多级催化部分氧化（CPO）方法。该方法采用CPO催化剂和受控工艺特征，包括：（A）在多于一个反应阶段中，使用含氧进料流在多于一个进料点的过程中逐步引入该方法的总氧需求量，每个阶段包括催化剂; （B）含氧进料流，烃类原料流，在上述多阶段第一阶段后的反应阶段中，将前一阶段生产的中间产物在彼此接触后混合一段时间，小于约1毫秒以形成基本均匀的混合物，其中混合物然后与催化剂接触; （C）在进入第一阶段之前将含氧进料流和烃进料流预热至约450℃至小于约1,000℃的温度; 和（D）在第一阶段之后的每个阶段中的产物的混合物温度为大于约600℃至小于约1000℃。优选地，该方法包括小于或等于约五个阶段，第一阶段步骤（C）中所述的阶段预热温度大于约550℃，并且在第一阶段之后的每个阶段中的产品的混合物温度为至少700℃

3. 发明授权

US07759533B2 Lightly branched higher olefin oligomerization with surface modified zeolite catalyst 有权
标题翻译：用表面改性沸石催化剂轻支化高级烯烃低聚
公开(公告)号：US07759533B2
公开(公告)日：2010-07-20
申请号：US11973101
申请日：2007-10-05
申请人： Jane C. Cheng , Sal Miseo , Stuart L. Soled , John S. Buchanan , Jennifer S. Feeley
发明人： Jane C. Cheng , Sal Miseo , Stuart L. Soled , John S. Buchanan , Jennifer S. Feeley
IPC分类号： C07C2/12
CPC分类号： C07C2/12 , B01J29/7076 , B01J29/7092 , B01J29/7096 , B01J2229/123 , B01J2229/18 , B01J2229/20 , B01J2229/42
摘要： A substantially surface-deactivated catalyst composition that is stable at least to 300° C. The catalyst includes a zeolite catalyst (e.g., ZSM-22, ZSM-23, or ZSM-57) having active internal Brönsted acid sites and a surface-deactivating amount of a rare earth or yttrium oxide (e.g., chosen from lanthanum oxide or lanthanides oxide). This catalyst is preferably used in a process for producing a higher olefin by oligomerizing a light olefin, wherein the process includes contacting a light olefin under oligomerization conditions with the substantially surface-deactivated catalyst composition.
摘要翻译：基本上表面失活的催化剂组合物，其稳定至少为300℃。催化剂包括具有活性内部布朗斯台德酸位点和表面失活的沸石催化剂（例如，ZSM-22，ZSM-23或ZSM-57）稀土或氧化钇的量（例如，选自氧化镧或氧化镧）。该催化剂优选用于通过低聚烯烃生产高级烯烃的方法，其中该方法包括在低聚条件下使轻质烯烃与基本上表面失活的催化剂组合物接触。

4. 发明申请

US20080175765A1 High throughput, microwave energy heated continuous hydrothermal synthesis apparatus 审中-公开
标题翻译：高通量，微波能量加热连续水热合成装置
公开(公告)号：US20080175765A1
公开(公告)日：2008-07-24
申请号：US12001907
申请日：2007-12-13
申请人： Guang Cao , Sabato Miseo , Stu L. Soled , Jennifer S. Feeley
发明人： Guang Cao , Sabato Miseo , Stu L. Soled , Jennifer S. Feeley
IPC分类号： B01J19/12
CPC分类号： B01J37/10 , B01J23/8885 , B01J37/0036
摘要： The present invention is a high throughput apparatus. The apparatus is an automated multi-channel preparation module that prepares a synthesis mixture, microwave heating zone, product collection vessels, and a means for continuously transferring the synthesis mixture through the apparatus.
摘要翻译：本发明是高产量装置。该装置是一种自动多通道制备模块，其制备合成混合物，微波加热区，产物收集容器以及用于将合成混合物连续转移通过该装置的装置。

5. 发明授权

US5509798A Stabilized catalyst carrier and improved carrier configuration for catalytic combustion system 失效
公开(公告)号：US5509798A
公开(公告)日：1996-04-23
申请号：US318020
申请日：1994-10-04
申请人： Jennifer S. Feeley , Dianne O. Simone , Leonard M. Quick , Martha M. Hamil
发明人： Jennifer S. Feeley , Dianne O. Simone , Leonard M. Quick , Martha M. Hamil
IPC分类号： F23C99/00 , B01J21/14 , B01J23/44 , B01J35/00 , B01J37/02 , B01J37/10 , C10L3/00 , F23C13/00 , F23D3/40
CPC分类号： F23C13/08 , B01J35/0006 , B01J37/0217 , B01J37/10
摘要： A catalyst member for use in processes for the catalytic combustion of gaseous carbonaceous fuels is made from a stabilized carrier having a plurality of gas flow passages extending therethrough defined by channel walls and a catalyst material disposed on the channel walls, wherein the carrier is stabilized against interaction with the catalyst material. The stabilized carrier may be prepared from a monolith comprising silica, magnesia and alumina that has a coating of alumina on the channel walls and by subjecting the coated monolith to stabilizing conditions. The stabilizing conditions may include exposure to high temperature steam.

6. 发明授权

US5968861A Trimetallic zeolite catalyst and method of NO.sub.x abatement using the same 失效
标题翻译：三金属沸石催化剂及其减排方法
公开(公告)号：US5968861A
公开(公告)日：1999-10-19
申请号：US22724
申请日：1998-02-12
申请人： Jennifer S. Feeley , Michel Deeba , Robert J. Farrauto , Dinh Dang
发明人： Jennifer S. Feeley , Michel Deeba , Robert J. Farrauto , Dinh Dang
IPC分类号： B01D53/02 , B01D53/86 , B01D53/94 , B01J29/072 , B01J29/46
CPC分类号： B01J29/46 , B01D53/9418 , B01J29/072 , B01D2251/208 , B01D2255/20738 , B01D2255/20746 , B01D2255/20761 , B01D2255/504
摘要： A catalytic material useful for the abatement of NO.sub.x in a lean environment containing a zeolite material having incorporated therein copper, cobalt and iron as catalytically active species. The catalytically active metals are preferably incorporated into the zeolite by ion exchange and precipitation. The catalytic material may typically contain from about 2.0 to about 8.0 percent copper, from about 1.0 to about 4.0 percent iron and from about 0.25 to about 4.0 percent cobalt by weight of the catalytic material, i.e., by weight of the zeolite material plus the catalytic metals incorporated therein. Optionally, the catalytic material may be admixed with a binder and applied as an adherent coating onto a carrier to be placed in a gas stream containing the nitrogen oxides.
摘要翻译：一种催化材料，用于在含有其中掺入有铜，钴和铁作为催化活性物质的沸石材料的稀薄环境中减少NOx。催化活性金属优选通过离子交换和沉淀引入到沸石中。催化材料通常可以含有按重量计的催化材料的约2.0至约8.0％的铜，约1.0至约4.0％的铁和约0.25至约4.0％的钴，即以沸石材料的重量加催化剂并入其中的金属。任选地，催化材料可以与粘合剂混合并作为粘附涂层施加到载体上以放置在含有氮氧化物的气流中。

7. 发明授权

US5776423A Trimetallic zeolite catalyst and method of NO.sub.x abatement using the same 失效
标题翻译：三金属沸石催化剂及其减排方法
公开(公告)号：US5776423A
公开(公告)日：1998-07-07
申请号：US699676
申请日：1996-08-15
申请人： Jennifer S. Feeley , Michel Deeba , Robert J. Farrauto , Dinh Dang
发明人： Jennifer S. Feeley , Michel Deeba , Robert J. Farrauto , Dinh Dang
IPC分类号： B01D53/02 , B01D53/86 , B01D53/94 , B01J29/072 , B01J29/46 , B01J8/00
CPC分类号： B01J29/46 , B01D53/9418 , B01J29/072 , B01D2251/208 , B01D2255/20738 , B01D2255/20746 , B01D2255/20761 , B01D2255/504
摘要： A catalytic material useful for the abatement of NO.sub.X in a lean environment containing a zeolite material having incorporated therein copper, cobalt and iron as catalytically active species. The catalytically active metals are preferably incorporated into the zeolite by ion exchange and precipitation. The catalytic material may typically contain from about 2.0 to about 8.0 percent copper, from about 1.0 to about 4.0 percent iron and from about 0.25 to about 4.0 percent cobalt by weight of the catalytic material, i.e., by weight of the zeolite material plus the catalytic metals incorporated therein. Optionally, the catalytic material may be admixed with a binder and applied as an adherent coating onto a carrier to be placed in a gas stream containing the nitrogen oxides.
摘要翻译：一种催化材料，其用于在含有其中掺入有铜，钴和铁作为催化活性物质的沸石材料的稀薄环境中减少NOX。催化活性金属优选通过离子交换和沉淀引入到沸石中。催化材料通常可以含有按重量计的催化材料的约2.0-约8.0％的铜，约1.0-约4.0％的铁和约0.25-约4.0％的钴，即按沸石材料的重量加催化剂并入其中的金属。任选地，催化材料可以与粘合剂混合并作为粘附涂层施加到载体上以放置在含有氮氧化物的气流中。

8. 发明授权

US6080377A Method of abating NO.sub.x and a catalytic material therefor 失效
标题翻译：减轻NOx及其催化材料的方法
公开(公告)号：US6080377A
公开(公告)日：2000-06-27
申请号：US430065
申请日：1995-04-27
申请人： Michel Deeba , Jennifer S. Feeley , Robert J. Farrauto
发明人： Michel Deeba , Jennifer S. Feeley , Robert J. Farrauto
IPC分类号： B01D53/86 , B01D53/94 , B01J29/40 , B01J29/44 , B01J29/70 , B01J8/00
CPC分类号： B01J29/44 , B01D53/9418 , B01D2251/208 , B01D2255/1021 , B01D2255/1026 , B01D2255/502 , B01D2255/504 , B01D2255/912 , Y02C20/10
摘要： A method for reducing gaseous nitrogen oxides present in a gas stream by reaction with a reductant species is practiced by flowing the gas stream under lean NO.sub.X -reducing conditions in contact with a catalytic material containing a catalytically effective amount of a catalytic species, e.g., a platinum group metal, and a reductant storage material, e.g., a zeolite, effective for storing reductant species for reaction with NO.sub.X, and providing an intermittent supply of the reductant to the gas stream. The catalytic material may be prepared in any manner, but one method is to incorporate a catalytically effective amount of the platinum into a template-bearing molecular sieve material, preferably ZSM-5 zeolite, to hinder the platinum from being incorporated into the pores of the molecular sieve material, and then calcining the molecular sieve material, whereby the template is removed from the molecular sieve material after the platinum is incorporated therein. Another method is to add a blocking agent to the molecular sieve material, then incorporate the platinum therein, and then calcine the material to remove the blocking agent. The catalytic material may contain less than about two percent by weight of zeolite plus platinum, e.g., less than about 0.5%, or from about 0.025% to 0.1% or 0.2% platinum.
摘要翻译：通过与还原剂物质反应来还原存在于气流中的气态氮氧化物的方法是通过在贫NOX还原条件下与含有催化有效量的催化物质（例如，铂族金属和还原剂储存材料，例如有效地存储用于与NOX反应的还原剂物质的沸石，以及向气流中间歇地供应还原剂。催化材料可以以任何方式制备，但是一种方法是将催化有效量的铂掺入含模板的分子筛材料，优选ZSM-5沸石中，以阻止铂被引入到分子筛材料，然后煅烧分子筛材料，由此在引入铂后，从分子筛材料中除去模板。另一种方法是向分子筛材料中加入封闭剂，然后在其中加入铂，然后煅烧该材料以除去封闭剂。催化材料可以含有小于约2重量％的沸石加铂，例如小于约0.5％，或约0.025％至0.1％或0.2％的铂。

9. 发明授权

US5551239A Catalytic combustion system including a separator body 失效
标题翻译：催化燃烧系统包括分离器体
公开(公告)号：US5551239A
公开(公告)日：1996-09-03
申请号：US271244
申请日：1994-07-07
申请人： Jennifer S. Feeley , James C. Fu , Matthew P. Larkin , Dianne O. Simone
发明人： Jennifer S. Feeley , James C. Fu , Matthew P. Larkin , Dianne O. Simone
IPC分类号： B01J23/44 , B01J23/63 , F23C13/00 , F23C99/00 , F23R3/40 , F02C3/00
CPC分类号： F23C13/00 , F23R3/40 , F23C2900/13002
摘要： A combustor for supporting the catalytic combustion of gaseous carbonaceous fuel contains a catalyst zone in which is disposed a catalyst body comprising at least one catalyst member, a separator zone comprising a separator body and a downstream zone where homogeneous combustion occurs. The catalyst member contains a carrier and a catalyst material deposited thereon. The catalyst body may, optionally, contain additional catalyst members downstream of the at least one catalyst member. The separator body contains a carrier-type monolith containing ceramic fibers in a matrix. One of the optional additional catalyst members may also contain such a monolith on which the catalyst composition is disposed.
摘要翻译：用于支撑气态含碳燃料的催化燃烧的燃烧器包含催化剂区域，其中设置有包括至少一个催化剂构件的催化剂体，包括分离器体的分离区和发生均匀燃烧的下游区。催化剂构件包含沉积在其上的载体和催化剂材料。催化剂体可以任选地在至少一个催化剂构件的下游含有另外的催化剂组分。分离器主体包含载体型整料，其包含基体中的陶瓷纤维。任选的另外的催化剂构件之一也可以含有这样的整料，其上设置催化剂组合物。

10. 发明授权

US5474441A Catalyst configuration for catalytic combustion systems 失效
标题翻译：用于催化燃烧系统的催化剂配置
公开(公告)号：US5474441A
公开(公告)日：1995-12-12
申请号：US22248
申请日：1993-02-25
申请人： Robert J. Farrauto , Jennifer S. Feeley , Dianne O. Simone , Yiu K. Lui , Teresa Kennelly
发明人： Robert J. Farrauto , Jennifer S. Feeley , Dianne O. Simone , Yiu K. Lui , Teresa Kennelly
IPC分类号： B01J23/10 , F23C13/00 , F23R3/40 , F23D3/40
CPC分类号： F23C13/00 , F23C13/08 , F23R3/40
摘要： A catalyst bed (30) for a combustor (18) for supporting the catalytic combustion of a gaseous air/fuel (e.g., methane or natural gas) combustion mixture contains an igniter catalyst member (1) upstream of a promoter catalyst member (2). The catalyst members each comprise carrier monoliths, the igniter catalyst member (1) having an igniter catalyst material deposited thereon and the promoter catalyst member (2) having a promoter catalyst material deposited thereon. The igniter catalyst material is distinguished from the promoter catalyst material in one or more of the following ways: the igniter catalyst material may have (a) a higher catalytic activity for combustion of the air/fuel mixture, (b) a lower catalyst deactivation temperature than the promoter catalyst material, and/or (c) the promoter catalyst regeneration temperature range brackets the upper limit of the regeneration temperature range of the igniter catalyst.
摘要翻译：用于支撑气态空气/燃料（例如，甲烷或天然气）燃烧混合物的催化燃烧的燃烧器（18）的催化剂床（30）在促进剂催化剂构件（2）的上游含有点火器催化剂构件（1）。催化剂构件各自包括载体整料，其上沉积有点火器催化剂材料的点火器催化剂构件（1）和其上沉积有助催化剂材料的助催化剂构件（2）。点火器催化剂材料以一种或多种以下方式与助催化剂材料不同：点火器催化剂材料可具有（a）对于空气/燃料混合物燃烧的较高催化活性，（b）较低的催化剂失活温度和/或（c）助催化剂催化剂再生温度范围包括点火器催化剂的再生温度范围的上限。

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