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1. 发明授权

US5916488A Polyimide resin compositions for optical filters 失效
标题翻译：用于光学滤光片的聚酰亚胺树脂组合物
公开(公告)号：US5916488A
公开(公告)日：1999-06-29
申请号：US66808
申请日：1998-04-28
申请人： Keisuke Takuma , Kazuhiro Seino , Tsutami Misawa , Shoji Tamai , Wataru Yamashita
发明人： Keisuke Takuma , Kazuhiro Seino , Tsutami Misawa , Shoji Tamai , Wataru Yamashita
IPC分类号： C08G73/10 , C08K5/00 , C09D11/10 , G02B5/20 , G02B5/22 , F21V9/04 , C09D11/00
CPC分类号： G02B5/223 , C08G73/1039 , C08K5/0041 , C09D11/102 , G02B5/201
摘要： A printing ink for an optical filter, comprising a polyimide resin containing at least one perfluoroalkyl group in each recurring structural unit, at least one dyestuff soluble in the resin, the dyestuff having absorption in the visible range and/or the near infrared range and a solvent.
摘要翻译：一种用于滤光器的印刷油墨，包括在每个重复结构单元中含有至少一个全氟烷基的聚酰亚胺树脂，至少一种可溶于树脂的染料，所述染料在可见光范围和/或近红外范围内具有吸收，溶剂。

2. 发明授权

US5868968A Polyimide resin compositions for optical filters 失效
标题翻译：用于光学滤光片的聚酰亚胺树脂组合物
公开(公告)号：US5868968A
公开(公告)日：1999-02-09
申请号：US965195
申请日：1997-11-06
申请人： Keisuke Takuma , Kazuhiro Seino , Tsutami Misawa , Shoji Tamai , Wataru Yamashita
发明人： Keisuke Takuma , Kazuhiro Seino , Tsutami Misawa , Shoji Tamai , Wataru Yamashita
IPC分类号： C08G73/10 , C08K5/00 , C09D11/10 , G02B5/20 , G02B5/22 , F21V9/04 , F21V9/00
CPC分类号： G02B5/223 , C08G73/1039 , C08K5/0041 , C09D11/102 , G02B5/201
摘要： A polyimide resin composition for an optical filter which includes a colorless transparent polyimide resin containing at least one perfluoroalkyl group in each recurring structural unit and having excellent solvent solubility, and at least one dyestuff soluble in said resin. The dyestuff has absorption in the visible range and/or the near infrared range. A printing ink for an optical filter is composed of the polyimide resin composition and a solvent while an optical filter formed from a transparent base material and the polyimide resin composition can also be provided.
摘要翻译：一种滤光器用聚酰亚胺树脂组合物，其包含在每个重复结构单元中含有至少一个全氟烷基并且溶剂溶解性优异的无色透明聚酰亚胺树脂和至少一种可溶于所述树脂的染料。染料在可见光范围和/或近红外范围内具有吸收。用于滤光器的印刷油墨由聚酰亚胺树脂组合物和溶剂构成，同时也可以提供由透明基材形成的滤光器和聚酰亚胺树脂组合物。

3. 发明授权

US5719256A Process for preparing polycondensation polymer compound 失效
标题翻译：制备缩聚高分子化合物的方法
公开(公告)号：US5719256A
公开(公告)日：1998-02-17
申请号：US730362
申请日：1996-10-15
申请人： Shoji Tamai , Yukiko Mori , Kenichi Goto , Katsuji Watanabe , Osamu Kohgo , Kotaro Shimizu , Toshiyuki Kataoka , Takashi Kuroki , Wataru Yamashita , Hideki Mizuta , Teruyuki Nagata
发明人： Shoji Tamai , Yukiko Mori , Kenichi Goto , Katsuji Watanabe , Osamu Kohgo , Kotaro Shimizu , Toshiyuki Kataoka , Takashi Kuroki , Wataru Yamashita , Hideki Mizuta , Teruyuki Nagata
IPC分类号： C08G63/82 , C08G63/87 , C08G69/04 , C08G69/28 , C08G73/10 , C08G75/26 , C08G63/06
CPC分类号： C08G73/1007 , C08G63/823 , C08G63/87 , C08G69/04 , C08G69/28 , C08G75/26
摘要： The invention provides a novel preparation process of a polycondensation type polymer, an excellent polymer which is represented by lactic acid and the preparation process of the polymer, a polycondensation agent used for the preparation process, and an intermediate. Specifically, the invention provides a preparation process of the polycondensation type polymer, for example, polyamide, polyimide, polythioester and polyester, comprising bonding a carboxyl group comprising compound with an active hydrogen group comprising compound in the presence of haloiminium salt. The invention provides excellent polylactic acid having a controlled D/L-isomer ratio in the repeating structural units and preparation process of polylactic acid, and further provides a haloiminium salt compound used for the preparation process and an intermediate compound of acid chloride.
摘要翻译：本发明提供了一种缩聚型聚合物的新型制备方法，由乳酸代表的优异聚合物和聚合物的制备方法，用于制备方法的缩聚剂和中间体。具体地说，本发明提供缩聚型聚合物，例如聚酰胺，聚酰亚胺，聚硫酯和聚酯的制备方法，包括在卤代鎓盐存在下将包含羧基的化合物与含活性氢基团的化合物结合。本发明提供了在重复结构单元和聚乳酸的制备方法中具有受控的D / L异构体比例的优异的聚乳酸，并且还提供了用于制备方法的卤代亚铵盐化合物和酰氯的中间体化合物。

4. 发明授权

US5480965A Readily soluble, amorphous polyimide, and preparation process of same 失效
标题翻译：易溶，无定形聚酰亚胺及其制备方法相同
公开(公告)号：US5480965A
公开(公告)日：1996-01-02
申请号：US280551
申请日：1994-07-26
申请人： Wataru Yamashita , Yuichi Okawa , Hideaki Oikawa , Tadashi Asanuma , Yuko Ishihara , Mitsunori Matsuo , Keizaburo Yamaguchi , Akihiro Yamaguchi , Shoji Tamai
发明人： Wataru Yamashita , Yuichi Okawa , Hideaki Oikawa , Tadashi Asanuma , Yuko Ishihara , Mitsunori Matsuo , Keizaburo Yamaguchi , Akihiro Yamaguchi , Shoji Tamai
IPC分类号： C07C201/12 , C07C205/45 , C07C221/00 , C07C225/22 , C08G73/10 , C08G73/12 , C08J5/18 , C08L79/08 , C08G69/26 , C08L77/00
CPC分类号： C08G73/10 , C08G73/1007 , C08G73/1014 , C08G73/1017 , C08G73/1067 , Y10T428/31504 , Y10T428/31721
摘要： This invention relates to a novel thermoplastic and amorphous polyimide which is readily soluble in organic solvent, a novel aromatic diamino compound used for the polyimide, a preparation process thereof, a polyimide-based resin composition comprising the thermoplastic polyimide and a fibrous reinforcement, a process for preparing the resin composition, an injection molded article of the resin composition, a polyimide-based composite obtained by molding the above soluble and thermoplastic polyimide in combination with a fibrous reinforcement, and a fibrous reinforcement having a surface modified with the above polyimide.The polyimide comprise a requisite structural unit having one or more recurring structural units of the formula: ##STR1## wherein m and n are individually an integer of 0 or 1, and R is ##STR2## The polyimide of the invention is essentially amorphous, excellent in melt flow stability in the decreased temperature as compared with conventionally known polyimide and has greatly improved processability.The polyimide of the invention obtained by using a novel aromatic diamino compound as a monomer can control various properties such as melt flow ability and solubility in solvents by side chains and not by principal chain of polyimide. Thus, excellent melt flow property and solubility in solvents can be obtained while maintaining high heat resistance and adhesive property which are derived from benzophenone structure of the diamino compound of the the invention.
摘要翻译：本发明涉及易溶于有机溶剂的新型热塑性和无定形聚酰亚胺，用于聚酰亚胺的新型芳族二氨基化合物及其制备方法，包含热塑性聚酰亚胺和纤维增强剂的聚酰亚胺基树脂组合物，用于制备树脂组合物的树脂组合物的注塑制品，通过将上述可溶性和热塑性聚酰亚胺与纤维增强剂组合成型而获得的聚酰亚胺类复合材料和具有用上述聚酰亚胺改性的表面的纤维增强剂。聚酰亚胺包含必需的结构单元，其具有一个或多个下式的重复结构单元：其中m和n分别为0或1的整数，R为本发明的聚酰亚胺基本上为与常规已知的聚酰亚胺相比，在降低的温度下的熔体流动稳定性优异并且具有极大的改进的加工性。通过使用新颖的芳族二氨基化合物作为单体获得的本发明的聚酰亚胺可以通过侧链而不是聚酰亚胺的主链来控制各种性能如熔体流动性和在溶剂中的溶解度。因此，在保持由本发明的二氨基化合物的二苯甲酮结构得到的高耐热性和粘合性的同时，可以获得优异的熔体流动性和溶剂中的溶解性。

5. 发明授权

US5470943A Polyimide 失效
标题翻译：聚酰亚胺
公开(公告)号：US5470943A
公开(公告)日：1995-11-28
申请号：US360584
申请日：1994-12-21
申请人： Yoshihiro Sakata , Wataru Yamashita , Yuichi Okawa , Shoji Tamai , Tsutomu Ishida , Mitsunori Matsuo , Keizaburo Yamaguchi , Akihiro Yamaguchi
发明人： Yoshihiro Sakata , Wataru Yamashita , Yuichi Okawa , Shoji Tamai , Tsutomu Ishida , Mitsunori Matsuo , Keizaburo Yamaguchi , Akihiro Yamaguchi
IPC分类号： C08G73/10 , C08G77/10 , C07D213/69 , C08G69/26
CPC分类号： C08G73/1039 , C08G73/1085
摘要： This invention relates to a novel fluorine-containing polyimide or polyimide copolymer being colorless and having transparency and very low dielectric characteristics, and has a novel aromatic diamino compound used for the polyimide, a preparation process thereof, a polyimide-based resin composition comprising the polyimide or polyimide copolymer and a fibrous reinforcement, a process for preparing the resin composition, an injection molded article of the resin composition.The polyimide comprise a requisite structural unit having one or more recurring structural units of the formula: ##STR1## wherein Ar is a tetravalent radical having 6 to 27 carbon atoms and being selected from the group consisting of a monoaromatic radical, condensed polyaromatic radical and noncondensed polyaromatic radical having aromatic radicals connected to each other with a direct bond or a bridge member, a trifluoromethyl radical is situated at the 3- or the 4-position on a pyridine nucleus, and an imide nitrogen atom is connected at the 3- or the 4-position to an ether bond.The polyimide or polyimide copolymer has excellent heat resistance, outstanding melt-flow stability and greatly improved processability, and also is colorless and has high transparency and very low dielectric coefficient, and can be expected to be used as raw materials for electric.cndot.electronic appliances and optical instruments due to the above characteristics.
摘要翻译：本发明涉及一种新颖的含氟聚酰亚胺或聚酰亚胺共聚物，其具有透明性和非常低的介电特性，并且具有用于聚酰亚胺的新型芳族二氨基化合物及其制备方法，该聚酰亚胺系树脂组合物含有聚酰亚胺或聚酰亚胺共聚物和纤维增强剂，树脂组合物的制备方法，树脂组合物的注塑制品。聚酰亚胺包含具有一个或多个下式的重复结构单元的必需结构单元：其中Ar是具有6至27个碳原子的四价基团，并且选自单芳族基团，缩合多芳族基团具有芳族基团的自由基和非缩合多芳族基团彼此直接键合或桥接成员，三氟甲基位于吡啶核上的3-或4-位，酰亚胺氮原子连接在3 - 或4-位到醚键。聚酰亚胺或聚酰亚胺共聚物具有优异的耐热性，优异的熔体流动稳定性和极好的加工性，并且是无色的，具有高透明度和非常低的介电系数，并且可以预期用作电气电子设备的原料光学仪器由于上述特点。

6. 发明授权

US5763537A Polyimide based resin composition 失效
标题翻译：聚酰亚胺基树脂组合物
公开(公告)号：US5763537A
公开(公告)日：1998-06-09
申请号：US577517
申请日：1995-12-22
申请人： Tomomi Yoshimura , Wataru Yamashita , Shoji Tamai , Akihiro Yamaguchi
发明人： Tomomi Yoshimura , Wataru Yamashita , Shoji Tamai , Akihiro Yamaguchi
IPC分类号： C08K5/3417 , C08L67/00 , C08L79/08
CPC分类号： C08K5/3417
摘要： A is a polyimide based resin molding composition comprising 100 parts by weight of crystalline polyimide having recurring structural units of the formula (1): ##STR1## and 1.about.50 parts by weight of crystallization accelerators selected from bisimide compounds of specific structure, a mixture of bisimide compounds, and imide based oligomer. The composition remarkably accelerates the crystallization velocity of polyimide of the formula (1), crystallization can be completed within a greatly reduced cooling time after melt processing, and the crystallized polyimide resin has excellent properties.
摘要翻译： A是一种聚酰亚胺基树脂模制组合物，其包含100重量份具有式（1）的重复结构单元的结晶聚酰亚胺：1分钟和50分钟的选自特定结构的双酰亚胺化合物的结晶促进剂，双酰亚胺化合物和基于酰亚胺的低聚物的混合物。该组合物显着加速式（1）的聚酰亚胺的结晶速度，在熔融加工后的冷却时间内可以结晶化，结晶化聚酰亚胺树脂具有优异的性能。

7. 发明授权

US5508377A Polyimide 失效
标题翻译：聚酰亚胺
公开(公告)号：US5508377A
公开(公告)日：1996-04-16
申请号：US357193
申请日：1994-12-13
申请人： Wataru Yamashita , Yuichi Okawa , Shoji Tamai , Akihiro Yamaguchi
发明人： Wataru Yamashita , Yuichi Okawa , Shoji Tamai , Akihiro Yamaguchi
IPC分类号： C08G73/10 , C08L79/08 , C08G69/26
CPC分类号： C08G73/1085 , C08G73/10 , C08G73/1039 , C08G73/105 , C08G73/1053 , C08G73/1071 , C08L79/08
摘要： This invention relates to a novel polyimide or polyimide copolymer having excellent heat resistance and greatly improved processability, and has a novel aromatic diamino compound used for the polyimide, a preparation process thereof, a polyimide-based resin composition comprising the polyimide or polyimide copolymer and a fibrous reinforcement, a process for preparing the resin composition, an injection molded article of the resin composition.The polyimide comprise a requisite structural unit having one or more recurring structural units of the formula: ##STR1## wherein L is an oxygen atom, carbonyl, isopropylidene or hexafluoroisopropylidene, and X is ##STR2## and Ar is a tetravalent radical having 6 to 27 carbon atoms and being selected from the group consisting of a monoaromatic radical, condensed polyaromatic radical and noncondensed polyaromatic radical having aromatic radicals connected to each other with a direct bond or a bridge member.The polyimide or polyimide copolymer is outstanding in melt-flow stability, and has greatly improved processability and excellent heat resistance. Consequently, the polyimide or polyimide copolymer can be applied to structural materials, and electic.cndot.electronic appliances.
摘要翻译：本发明涉及耐热性优异且加工性极佳的新型聚酰亚胺或聚酰亚胺共聚物，具有用于聚酰亚胺的新型芳族二氨基化合物及其制备方法，包含聚酰亚胺或聚酰亚胺共聚物的聚酰亚胺系树脂组合物和纤维增强材料，树脂组合物的制备方法，树脂组合物的注塑制品。聚酰亚胺包括具有一个或多个下式的重复结构单元的必需结构单元：其中L是氧原子，羰基，异亚丙基或六氟异亚丙基，X是（5）和Ar 是具有6至27个碳原子的四价基团，并且选自具有芳族基团的单芳族基团，缩合多芳族基团和具有直接键合或桥连构件彼此连接的非缩合多芳族基团。聚酰亚胺或聚酰亚胺共聚物在熔体流动稳定性方面是突出的，并且具有极大的改进的加工性和优异的耐热性。因此，聚酰亚胺或聚酰亚胺共聚物可以应用于结构材料和电子电器。

8. 发明授权

US5484880A Polyimide 失效
标题翻译：聚酰亚胺
公开(公告)号：US5484880A
公开(公告)日：1996-01-16
申请号：US354806
申请日：1994-12-13
申请人： Wataru Yamashita , Yuichi Okawa , Shoji Tamai , Mitsunori Matsuo , Tsutomu Ishida , Keizaburo Yamaguchi , Akihiro Yamaguchi
发明人： Wataru Yamashita , Yuichi Okawa , Shoji Tamai , Mitsunori Matsuo , Tsutomu Ishida , Keizaburo Yamaguchi , Akihiro Yamaguchi
IPC分类号： C07C225/22 , C07B61/00 , C07C221/00 , C08G73/10 , C08L79/08 , C08G77/10 , C08G69/26
CPC分类号： C08G73/1071 , C08G73/1014 , C08G73/105 , C08G73/1064 , C08L79/08
摘要： The present invention relates to an amorphous polyimide or a polyimide copolymer having a requisite structural unit consisting of one or more recurring structural units represented by the formula (1): ##STR1## wherein X is a direct bond, oxygen atom or sulfur atom, and R.sub.1, R.sub.2, R.sub.3 and R.sub.4 are individually a hydrogen atom or methyl, and Ar is a tetravalent radical having 6 to 27 carbon atoms and being selected from the group consisting of a monoaromatic radical, condensed polyaromatic radical and noncondensed polyaromatic radical having aromatic radicals connected to each other with a direct bond or a bridge member.Polyimide and the polyimide copolymer of the invention has excellent heat resistance, is outstanding in melt-flow stability, has greatly improved processability, and can be applied to structural materials, and electric- electronic appliances.
摘要翻译：本发明涉及具有必要结构单元的无定形聚酰亚胺或聚酰亚胺共聚物，所述结构单元由一个或多个由式（1）表示的重复结构单元：原子或硫原子组成，并且R 1，R 2，R 3和R 4分别为氢原子或甲基，Ar是具有6至27个碳原子的四价基团，并且选自具有芳族基团的单芳族基团，缩合多芳族基团和具有直接键或桥键的彼此连接的非缩合多芳族基团会员。本发明的聚酰亚胺和聚酰亚胺共聚物具有优异的耐热性，熔体流动稳定性优异，加工性能大大提高，可应用于结构材料和电子电器。

9. 发明授权

US5371168A Amorphous polyimide powder, preparation process of the powder, and heat-resistant adhesive and bonding method by use of the powder 失效
标题翻译：无定形聚酰亚胺粉末，粉末的制备工艺，耐热粘合剂和使用粉末的粘合方法
公开(公告)号：US5371168A
公开(公告)日：1994-12-06
申请号：US894422
申请日：1992-06-05
申请人： Wataru Yamashita , Shoji Tamai , Akihiro Yamaguchi
发明人： Wataru Yamashita , Shoji Tamai , Akihiro Yamaguchi
IPC分类号： C08G73/10 , C09J179/08 , C08G8/02 , C08G69/26
CPC分类号： C08G73/1067 , C08G73/1014 , C09J179/08 , Y10S526/935
摘要： Amorphous polyimide powder which has recurring structural units of the formula (I): ##STR1## as a fundamental skeleton, is blocked at the polymer chain end with dicarboxylic anhydride represented by the formula (II) ##STR2## wherein Z is a divalent radical having from 6 to 27 carbon atoms and selected from the group consisting of a monoaromatic radical, condensed polyaromatic radical and noncondensed aromatic radical connected to each other with a direct bond or a bridge member, and essentially has no reactive radical at the polymer chain end, preparation process of the amorphous polyimide powder, heat-resistant adhesive comprising the polyimide, and bonding method using the adhesive.
摘要翻译：具有式（I）的重复结构单元：作为基本骨架的重复结构单元的无定形聚酰亚胺粉末在聚合物链端用由式（II）表示的二羧酸酐封闭，其中 Z是具有6至27个碳原子并且选自由直接键或桥连接在一起的单芳族基团，缩合多芳族基团和非缩合芳族基团的二价基团，并且基本上没有反应性基团聚合物链端，非晶聚酰亚胺粉末的制备方法，包含聚酰亚胺的耐热粘合剂和使用该粘合剂的粘合方法。

10. 发明授权

US5260388A Polyimide and process for the preparation thereof 失效
标题翻译：聚酰亚胺及其制备方法
公开(公告)号：US5260388A
公开(公告)日：1993-11-09
申请号：US894940
申请日：1992-06-08
申请人： Shoji Tamai , Wataru Yamashita , Yuichi Okawa , Yuko Ishihara , Keizaburo Yamaguchi , Akihiro Yamaguchi
发明人： Shoji Tamai , Wataru Yamashita , Yuichi Okawa , Yuko Ishihara , Keizaburo Yamaguchi , Akihiro Yamaguchi
IPC分类号： C07C225/22 , C08G73/10 , C08G73/14 , C08G8/02 , C08G69/26
CPC分类号： C07C225/22 , C08G73/1014 , C08G73/1017 , C08G73/1039 , C08G73/1067 , C08G73/14
摘要： A heat-resistant and thermoplastic polyimide which has low dielectric characteristics and recurring structural units of the following formula ##STR1## wherein R is a tetravalent radical having from 2 to 27 carbon atoms and selected from the group consisting of an aliphatic radical, alicyclic radical, monoaromatic radical, condensed polyaromatic radical and noncondensed aromatic radical connected each other with a direct bond or a bridge member; aromatic diamines which are useful for the raw material monomers of the polyimide and have following formulas: ##STR2## and ##STR3## and a process for preparing the polyimide of the above formula by reacting these aromatic diamines with a tetracarboxylic dianhydride in the presence of an aromatic dicarboxylic anhydride or aromatic monoamine, and successively thermally or chemically imidizing the resultant polyamic acid.

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