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1. 发明授权

US4702977A Secondary battery using non-aqueous solvent 失效
标题翻译：二次电池使用非水溶剂
公开(公告)号：US4702977A
公开(公告)日：1987-10-27
申请号：US855826
申请日：1986-04-24
申请人： Kazuya Hiratsuka , Yuichi Sato , Yoshiyasu Aoki , Hiroshi Yui , Mitsutaka Miyabayashi , Akira Itsubo
发明人： Kazuya Hiratsuka , Yuichi Sato , Yoshiyasu Aoki , Hiroshi Yui , Mitsutaka Miyabayashi , Akira Itsubo
IPC分类号： H01M4/36 , H01M4/58 , H01M4/583 , H01M4/587 , H01M4/96 , H01M10/0525 , H01M10/36 , H01M4/38 , H01M10/40
CPC分类号： H01M4/583 , H01M10/0525 , H01M4/36 , H01M4/587
摘要： There is disclosed a secondary battery using a non-aqueous solvent which comprises using a carbonaceous material obtained by carbonating an organic compound and having a pseudographite structure of a hydrogen/carbon ratio being 0.15 or less, a d.sub.002 being 3.37 .ANG. or more and a Lc being 150 .ANG. or less as a negative electrode.The battery has a large electric density, less in self-discharging and excellent in preservability.
摘要翻译：公开了使用非水溶剂的二次电池，其包括使用通过碳酸化有机化合物获得的碳质材料，并且具有0.15或更小的氢/碳比的假型晶格结构，d002为3.37Ag或更大，Lc 作为负极为150A·cm以下。电池电量密度大，自放电少，保存性好。

2. 发明授权

US4725422A Electrode material 失效
标题翻译：电极材料
公开(公告)号：US4725422A
公开(公告)日：1988-02-16
申请号：US36176
申请日：1987-04-08
申请人： Mitsutaka Miyabayashi , Akira Itsubo , Yoshitomo Nakano , Masami Takahashi , Mituru Ueda
发明人： Mitsutaka Miyabayashi , Akira Itsubo , Yoshitomo Nakano , Masami Takahashi , Mituru Ueda
IPC分类号： C04B35/524 , H01M4/58 , H01M4/587 , H01M4/96 , H01M10/052 , H01M10/36 , C10B31/00 , C10B31/04
CPC分类号： H01M4/587 , C04B35/524 , H01M10/052 , H01M4/583 , H01M4/96
摘要： An electrode material made of a carbonaceous material that is obtained by the pyrolysis of an organic compound capable of forming the graphite structure is disclosed. This carbonaceous material is such that the spacing of (002) planes, d002, is at least 3.37 .ANG. and thecrystallite size in the direction of c axis, Lc, is not more than 220 .ANG., as determined by X-ray wide-angle diffractiometry, and the line width .DELTA.Hpp between peaks in the first differential of the absorption spectrum of electron spin resonance is at least 10 gauss. The electrode material made of such carbonaceous material is capable of providing a stable secondary battery that produces high electromotive force and which has high energy density.
摘要翻译：公开了一种由能够形成石墨结构的有机化合物的热解而获得的由碳质材料制成的电极材料。这种碳质材料使得（002）面的间距d002至少为3.37，并且在c轴方向上的微晶尺寸Lc不超过220，如通过X射线广角衍射法测定的，电子自旋共振吸收光谱的第一微分峰之间的线宽DELTA Hpp为至少10高斯。由这种碳质材料制成的电极材料能够提供产生高电动势并且具有高能量密度的稳定的二次电池。

3. 发明授权

US5176969A Electrode for secondary battery 失效
标题翻译：二次电池用电极
公开(公告)号：US5176969A
公开(公告)日：1993-01-05
申请号：US689523
申请日：1991-04-23
申请人： Mitsutaka Miyabayashi , Manabu Hayashi , Eiki Yasukawa , Kikuko Miyata , Mitsumasa Kaitoh , Hiroshi Yui
发明人： Mitsutaka Miyabayashi , Manabu Hayashi , Eiki Yasukawa , Kikuko Miyata , Mitsumasa Kaitoh , Hiroshi Yui
IPC分类号： G02F1/136 , G02F1/1368 , H01L21/336 , H01L21/822 , H01L27/04 , H01L29/78 , H01L29/786 , H01M4/133 , H01M4/137 , H01M4/36 , H01M4/40 , H01M4/60 , H01M4/62 , H01M4/66 , H01M4/74 , H01M6/10 , H01M10/05
CPC分类号： H01M10/05 , H01M10/0525 , H01M4/0459 , H01M4/0461 , H01M4/131 , H01M4/36 , H01M4/364 , H01M4/587 , H01M4/60 , H01M4/602 , H01M4/622 , H01M4/623 , H01M10/0587 , H01M2300/0025 , H01M2300/0082 , H01M4/0404 , H01M4/405 , H01M4/74 , H01M6/10
摘要： Disclosed is an electrode for secondary battery, which comprises lithium or an alkali metal composed mainly of lithium doped as the active substance in a carrier composed of a mixture of a carbonaceous material satisfying the following conditions (A) and an organic polymer having ion conductivity of lithium.(A) a carbonaceous material with a hydrogen/carbon (H/C) atomic ratio of less than 0.15, a spacing (d.sub.002) of the (002) plane according to the X-ray wide angle diffraction method of 3.37 to 3.75 .ANG. and a crystallite size in the c-axis direction (Lc) of 5 .ANG. or more.
摘要翻译：公开了一种二次电池用电极，其包含锂或由主要由掺杂锂作为活性物质的碱金属构成的载体中，所述载体由满足以下条件（A）的碳质材料和具有以下条件（A）的含碳物质的混合物构成，锂。（A）氢/碳（H / C）原子比小于0.15的碳质材料，根据X射线广角衍射法的（002）面的间距（d002）为3.37〜3.75安 c轴方向（Lc）的微晶尺寸为5 ANGSTROM以上。

4. 发明授权

US5162170A Electrode for secondary battery 失效
标题翻译：二次电池电极
公开(公告)号：US5162170A
公开(公告)日：1992-11-10
申请号：US554137
申请日：1990-07-16
申请人： Mitsutaka Miyabayashi , Hiroshi Yui
发明人： Mitsutaka Miyabayashi , Hiroshi Yui
IPC分类号： H01M4/02 , H01M4/04 , H01M4/134 , H01M4/36 , H01M4/38 , H01M4/40 , H01M4/58 , H01M4/587 , H01M4/62 , H01M4/66 , H01M4/74 , H01M6/10 , H01M10/052 , H01M10/36
CPC分类号： H01M4/134 , H01M10/052 , H01M4/0459 , H01M4/0461 , H01M4/36 , H01M4/364 , H01M4/38 , H01M4/381 , H01M4/587 , H01M4/621 , H01M2004/027 , H01M2300/0025 , H01M2300/0065 , H01M4/0433 , H01M4/0492 , H01M4/405 , H01M4/625 , H01M4/661 , H01M4/74 , H01M6/10
摘要： An electrode for a secondary battery, comprising a net or sheet made of a metal having laminated thereon a mixture comprising 85 to 99.9% by weight of a carbonaceous material and 0.1 to 15% by weight of an elastomer. The carbonaceous material has a hydrogen/carbon (H/C) atomic ratio of less than 0.15, a spacing (d.sub.002) of the (002) plane according to an X-ray wide angle diffraction method of 3.37 .ANG. to 3.75 .ANG., a volume average particle size of 0.5 .mu.m and a total fine pore volume of 1.5.times.10.sup.-3 ml/g or more. Lithium or a material substantially comprising lithium is carried on the carbonaceous material. The electrode has a thickness of 5 to 500 .mu.m. The resultant electrode has an high energy density, and has the requisite flexibility to obtain a coil-shaped electrode.

5. 发明授权

US4945014A Secondary battery 失效
标题翻译：二次电池
公开(公告)号：US4945014A
公开(公告)日：1990-07-31
申请号：US305795
申请日：1989-02-02
申请人： Mitsutaka Miyabayashi , Toshifumi Nishii , Hiroshi Yui , Kuniaki Inada , Katsuji Ikeda , Hiroyoshi Nose , Kenji Tsuchiya
发明人： Mitsutaka Miyabayashi , Toshifumi Nishii , Hiroshi Yui , Kuniaki Inada , Katsuji Ikeda , Hiroyoshi Nose , Kenji Tsuchiya
IPC分类号： H01M4/02 , H01M4/04 , H01M4/134 , H01M4/36 , H01M4/40 , H01M4/58 , H01M4/587 , H01M4/62 , H01M10/052 , H01M10/36
CPC分类号： H01M4/134 , H01M10/052 , H01M4/0459 , H01M4/364 , H01M4/38 , H01M4/587 , H01M2004/027 , H01M2300/0025 , H01M2300/0068 , H01M2300/0082 , H01M4/0433 , H01M4/405 , H01M4/621 , H01M4/625
摘要： There is disclosed a secondary battery having a negative electrode composed of an active substance and a carrier carrying the active substance, which comprises(1) the active substance is lithium or an alkali metal mainly composed of lithium,(2) the carrier is a mixture composed of(a) a carbonaceous material having(i) an atomic ratio of hydrogen/carbon of less than 0.15 and(ii) a spacing of (002) planes (d.sub.002) as determined by X-ray wide angle diffraction of 3.37 .ANG. or more and a crystallite size in the direction of c axis of 150 .ANG. or less, and(b) a metal capable of forming an alloy with the active substance and/or an alloy with the active substance.

6. 发明授权

US4786709A Organic high molecular liquid crystals 失效
标题翻译：有机高分子液晶
公开(公告)号：US4786709A
公开(公告)日：1988-11-22
申请号：US44209
申请日：1987-04-30
申请人： Kazuyoshi Iimura , Naoyuki Koide , Mitsutaka Miyabayashi
发明人： Kazuyoshi Iimura , Naoyuki Koide , Mitsutaka Miyabayashi
IPC分类号： C08G63/52 , C08G63/54 , C09K19/16 , C09K19/32 , C09K19/38 , G11B7/25 , C09K19/52 , C08G63/02
CPC分类号： G11B7/25 , C08G63/54 , C09K19/16 , C09K19/32
摘要： An organic high molecular liquid crystal containing the moiety shown by the following structural formula (1) as the recurring unit and having a number average molecular weight of from 1,000 to 100,000: ##STR1## wherein m represents an integer of from 2 to 10; n represents an integer of from 1 to 12; and --A--represents an aromatic group.The high molecular liquid crystal of this invention can be used for performing optical recording by utilizing the thermooptical effect thereof and also can be used as a fluorescence scattering liquid crystal element since the liquid crystal has a property of emitting fluorescence.
摘要翻译：含有下述结构式（1）所示的部分作为重复单元且数均分子量为1,000〜100,000的有机高分子液晶：（1）其中m表示2〜 10; n表示1〜12的整数，并且-A代表芳族基团。本发明的高分子液晶可用于通过利用其光学效应进行光学记录，并且由于液晶具有发射荧光的性质，因此也可用作荧光散射液晶元件。

7. 发明授权

US4481336A Olefinic block copolymers of ethylene propylene and 1-butene 失效
标题翻译：乙烯丙烯和1-丁烯的烯烃嵌段共聚物
公开(公告)号：US4481336A
公开(公告)日：1984-11-06
申请号：US476838
申请日：1983-03-18
申请人： Masaki Fujii , Mitsutaka Miyabayashi
发明人： Masaki Fujii , Mitsutaka Miyabayashi
IPC分类号： C08F297/00 , C08F297/08 , C08L23/14
CPC分类号： C08F297/086 , C08F297/08 , C08L23/14 , C08L2205/02
摘要： A block copolymer comprising 60 to 95 parts by weight of a binary or tertiary random copolymer block A comprising propylene, ethylene and/or butene-1 and 5 to 40 parts by weight of a binary or tertiary random copolymer block B comprising butene-1, propylene and, optionally, ethylene. This block copolymer can be shaped into a film having excellent heat sealability, transparency and blocking resistance.
摘要翻译：包含60至95重量份的包含丙烯，乙烯和/或丁烯-1的二元或叔无规共聚物嵌段A和5至40重量份的包含丁烯-1的二元或叔无规共聚物嵌段B的嵌段共聚物，丙烯和任选的乙烯。该嵌段共聚物可以成形为具有优异的热封性，透明性和抗粘连性的膜。

8. 发明授权

US5851694A Redox flow type battery 失效
标题翻译：氧化还原流式电池
公开(公告)号：US5851694A
公开(公告)日：1998-12-22
申请号：US873453
申请日：1997-06-12
申请人： Mitsutaka Miyabayashi , Kanji Sato , Toshiyuki Tayama , Yoshiteru Kageyama , Haruo Oyama
发明人： Mitsutaka Miyabayashi , Kanji Sato , Toshiyuki Tayama , Yoshiteru Kageyama , Haruo Oyama
IPC分类号： H01M4/86 , H01M8/02 , H01M8/04 , H01M8/18 , H01M8/24 , H01M8/20
CPC分类号： B60L11/1868 , B60L11/1879 , H01M8/0273 , H01M8/188 , H01M8/246 , H01M8/0289 , Y02E60/528 , Y02T10/7005 , Y02T10/7066
摘要： The present invention relates to a liquid-circulating type redox flow battery which comprises (a) said battery being defined by a ratio (H/L) where (H) is the average height of each of said porous electrodes in a flow direction of each of said electrolytic solutions, and (L) is the length of each of said porous electrodes in a direction perpendicular to the flow direction of each of said electrolytic solutions, the ratio (H/L) being in the range of 0.18 to 1.95; and (b) said battery being defined by ratios (.SIGMA.s.sub.ai /S.sub.a) and (.SIGMA.s.sub.ci /S.sub.c) where (.SIGMA.s.sub.ai) is the sum of the cross-sectional area of an inlet for introducing said positive electrolytic solution into said positive cell, (.SIGMA.s.sub.ci) is the sum of the cross-sectional area of an inlet for introducing said negative electrolytic solution into said negative cell, (S.sub.a) is the average of the cross-sectional area of said porous electrode in a direction perpendicular to the flow direction of said positive electrolytic solution, and (S.sub.c) is the average of the cross-sectional area of said porous electrode in a direction perpendicular to the flow direction of said negative electrolytic solution, each of the ratios (.SIGMA.s.sub.ai /S.sub.a) and (.SIGMA.s.sub.ci /S.sub.c) being in the range of 0.001 to 0.04, and said battery being further defined by ratios (.SIGMA.s.sub.ao /S.sub.a) and (.SIGMA.s.sub.co /S.sub.c) where (.SIGMA.s.sub.ao) is the sum of the cross-sectional area of an outlet for discharging said positive electrolytic solution out of said positive cell, (.SIGMA.s.sub.co) is the sum of the cross-sectional area of an outlet for discharging said negative electrolytic solution out of said negative cell, and (S.sub.a) and (S.sub.c) are as denoted above, each of the ratios (.SIGMA.s.sub.ao /S.sub.a) and (.SIGMA.s.sub.co /S.sub.c) being in the range of 0.001 to 0.04.
摘要翻译：液体循环型氧化还原液流电池本发明涉及一种液体循环型氧化还原液流电池，其包括（a）所述电池以（H / L）的比例（H / L）定义，其中（H）是每个所述多孔电极在每个所述多孔电极的流动方向上的平均高度的所述电解液，（L）是所述多孔电极在与所述电解液各流动方向垂直的方向上的长度，所述比例（H / L）在0.18〜1.95的范围内; 和（b）所述电池由比率（SIGMA sai / Sa）和（SIGMA sci / Sc）定义，其中（SIGMA sai）是用于将所述正电解液引入所述阳性电池的入口的横截面面积的总和，（SIGMA sci）是用于将所述负电解质溶液引入所述负电池的入口的横截面面积的总和，（Sa）是所述多孔电极在垂直于所述负电池的方向上的横截面积的平均值所述正电解液的流动方向和（Sc）是所述多孔电极在与所述负电解质溶液的流动方向垂直的方向上的横截面积的平均值，每个比率（SIGMA sai / Sa）和（SIGMA sci / Sc）在0.001至0.04的范围内，并且所述电池进一步由比率（SIGMA sao / Sa）和（SIGMA sco / Sc）限定，其中（SIGMA sao）是横截面积用于排出所述正电解液的出口在所述阳性细胞中，（SIGMA sco）是用于从所述负电池中排出所述负电解质溶液的出口的横截面面积的总和，并且（Sa）和（Sc）如上所述，比例（SIGMA sao / Sa）和（SIGMA sco / Sc）在0.001至0.04的范围内。

9. 发明授权

US5187035A Electrode for secondary battery 失效
标题翻译：二次电池电极
公开(公告)号：US5187035A
公开(公告)日：1993-02-16
申请号：US709973
申请日：1991-06-04
申请人： Mitsutaka Miyabayashi , Manabu Hayashi
发明人： Mitsutaka Miyabayashi , Manabu Hayashi
IPC分类号： H01M4/02 , H01M4/04 , H01M4/13 , H01M4/36 , H01M4/40 , H01M4/58 , H01M4/587 , H01M4/62 , H01M4/66 , H01M4/74 , H01M6/10 , H01M8/04
CPC分类号： H01M4/13 , H01M4/045 , H01M4/0459 , H01M4/0461 , H01M4/0469 , H01M4/364 , H01M4/38 , H01M4/587 , H01M4/622 , H01M2004/027 , H01M2300/0025 , H01M2300/0065 , H01M4/0404 , H01M4/0433 , H01M4/405 , H01M4/661 , H01M4/74 , H01M6/10 , H01M8/04186
摘要： Disclosed is an electrode for secondary battery, which comprises an alkali metal as the active substance carried on a carrier composed of(1) 100 parts by weight of a carbonaceous material satisfying the following conditions:(A) a hydrogen/carbon atomic ratio of less than 0.15 and(B) a spacing (d.sub.002) of the (002) plane according to the X-ray wide angle diffraction method of 3.37 .ANG. or more and a crystallite size in the c-axis direction of (Lc) of 5 .ANG. or more, and0 to 70 parts by weight of a metal capable of forming an alloy with the active substance or an alloy of said metal and(2) 0.1 to 40 parts by weight of a fibrous organic polymer as the binder, which can give a negative electrode having excellent charging and discharging cycle characteristics and good flexibility to obtain secondary battery having large charging capacity.
摘要翻译：公开了一种二次电池用电极，其包含作为活性物质的碱金属，载体在载体上，所述载体由（1）100重量份满足以下条件的碳质材料构成：（A）氢/碳原子比小于根据X射线广角衍射方法，根据X射线广角衍射法，（002）面的间距（d002）为（3.00），（C）的5轴方向的c轴方向的微小尺寸，更多和0至70重量份的能够与活性物质或所述金属的合金形成合金的金属和（2）0.1至40重量份的纤维状有机聚合物作为粘合剂，其可以产生负极具有优异的充放电循环特性和良好的柔性，以获得具有大的充电容量的二次电池。

10. 发明授权

US4454306A Olefinic block copolymer and crosslinked product thereof 失效
标题翻译：烯属嵌段共聚物及其交联产物
公开(公告)号：US4454306A
公开(公告)日：1984-06-12
申请号：US409834
申请日：1982-08-20
申请人： Masaki Fujii , Mitsutaka Miyabayashi
发明人： Masaki Fujii , Mitsutaka Miyabayashi
IPC分类号： C08F4/16 , C08F297/08 , C08F293/00 , C08L53/00
CPC分类号： C08F297/08
摘要： A crosslinked product is derived from an olefinic block copolymer comprising 5 to 70 parts by weight of at least one block (A), which is selected from homopolymer blocks of propylene and random copolymer blocks of propylene and ethylene or a C.sub.4-12 .alpha.-olefin and has a propylene content of 60 to 100% by weight, and 30 to 95 parts by weight of at least one block (B), which is a random copolymer of ethylene and at least one C.sub.3-12 .alpha.-olefin and has an ethylene content of 10 to 85% by weight. This crosslinked product is characterized in that:(1) the content therein of hot xylene insoluble components is from 5 to 75% by weight; and(2) the fluidity thereof, i.e., the quantity thereof flowing per second (cc/sec..times.10.sup.-3) out through the orifice of Koka flow tester, is 3 to 500 cc/sec..times.10.sup.-3 when measured by this flow tester having a cylinder diameter of 10 mm, an orifice diameter of 1 mm, and an orifice height of 2 mm and operated with a load of 30 Kg and a temperature of the crosslinked product of 200.degree. C.
摘要翻译：交联产物衍生自烯烃嵌段共聚物，其包含5-70重量份的至少一个嵌段（A），其选自丙烯和丙烯和乙烯或C 4-12α-烯烃的无规共聚物嵌段的均聚物嵌段丙烯含量为60〜100重量％，以及30〜95重量份的至少一个嵌段（B），其是乙烯和至少一种C 3-12α-烯烃的无规共聚物，并具有乙烯含量为10〜85重量％。该交联物的特征在于：（1）热二甲苯不溶成分的含量为5〜75重量％和（2）其流动性，即其通过Koka流量计的孔流出的每秒流出量（cc / sec.x10-3）为3至500cc / sec×10-3，当通过该流量圆筒直径为10mm，孔直径为1mm，孔高为2mm，负荷为30Kg，交联物温度为200℃的试验机。

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