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1. 发明授权

US07544433B2 Electrode structure for polymer electrolyte fuel cells, and polymer electrolyte fuel cell using the same 有权
标题翻译：用于聚合物电解质燃料电池的电极结构和使用其的聚合物电解质燃料电池
公开(公告)号：US07544433B2
公开(公告)日：2009-06-09
申请号：US10714394
申请日：2003-11-17
申请人： Hiroshi Sohma , Masaru Iguchi , Nagayuki Kanaoka , Hayato Kaji , Hiroshi Morikawa , Naoki Mitsuta
发明人： Hiroshi Sohma , Masaru Iguchi , Nagayuki Kanaoka , Hayato Kaji , Hiroshi Morikawa , Naoki Mitsuta
IPC分类号： H01M8/10
CPC分类号： H01M8/1039 , C08G65/4025 , C08G65/4056 , C08G2650/64 , C08L65/00 , C08L71/00 , H01M4/8605 , H01M4/926 , H01M8/1004 , H01M8/1025 , H01M2008/1095 , H01M2300/0082 , C08L2666/22
摘要： The present invention provides an electrode structure for polymer electrolyte fuel cells, inexpensive, and exhibiting excellent power production capacity and durability even under high temperature/low humidity conditions, and also provides a polymer electrolyte fuel cell which incorporates the same electrode structure. The present invention also provides an electrical device and transportation device, each incorporating the same polymer electrolyte fuel cell. The electrode structure comprises a pair of electrode catalyst layers 1,1, each containing a catalyst supported by carbon particles, and polymer electrolyte membrane 2 placed between these electrode catalyst layers 1,1. The polymer electrolyte membrane 2 is of a sulfonated polyarylene composed of 0.5 to 100% by mol of the first repeating unit represented by the general formula (1) and 0 to 99.5% by mol of the second repeating unit represented by the general formula (2): (wherein, A is a divalent organic group; and a benzene ring includes its derivative), (wherein, —W— is a divalent electron attracting group; -T- is a divalent organic group; and R1 to R8 are a hydrogen atom or fluorine atom, an alkyl group, fluorine-substituted alkyl group, allyl group, aryl group or cyano group, and may be the same or different).
摘要翻译：本发明提供一种便宜的高分子电解质燃料电池用电极结构体，即使在高温/低湿度条件下也具有优异的动力产生能力和耐久性，并且还提供具有相同的电极结构的固体高分子型燃料电池。本发明还提供了一种电气装置和运输装置，每个装置和运输装置包括相同的聚合物电解质燃料电池。电极结构包括一对电极催化剂层1,1，每个电极催化剂层1,1都含有由碳颗粒负载的催化剂，以及聚合物电解质膜2，放置在这些电极催化剂层1,1之间。高分子电解质膜2是由通式（1）表示的第一重复单元的0.5〜100摩尔％和通式（2）表示的第二重复单元为0〜99.5摩尔％的磺化聚亚芳基）（式中，A为二价有机基团，苯环包含其衍生物）（式中，-W-为二价吸电子基团; -T-为二价有机基团，R1〜R8为氢原子原子或氟原子，烷基，氟取代的烷基，烯丙基，芳基或氰基，可以相同或不同）。

2. 发明申请

US20120178004A1 FUEL CELL 有权
标题翻译：燃料电池
公开(公告)号：US20120178004A1
公开(公告)日：2012-07-12
申请号：US13347595
申请日：2012-01-10
申请人： Kentaro Ishida , Akihiro Matsui , Narutoshi Sugita , Hayato Kaji
发明人： Kentaro Ishida , Akihiro Matsui , Narutoshi Sugita , Hayato Kaji
IPC分类号： H01M8/06 , H01M8/10
CPC分类号： H01M8/04156 , H01M8/0271 , H01M2008/1095 , Y02E60/50
摘要： A fuel cell includes a membrane-electrode assembly and a separator. The membrane-electrode assembly has an electrolyte and a pair of electrodes that are disposed on respective sides of the electrolyte. The membrane-electrode assembly and the separator are stacked in a stacking direction. A reaction surface of the membrane-electrode assembly is in a vertical direction along a direction of gravity and has a shape having a longer dimension in a horizontal direction. The fuel cell is provided with a reactant gas passage to allow a reactant gas to flow along a longitudinal direction of the reaction surface. The reactant gas is an oxidant gas or a fuel gas. A drain channel to allow product water from the reactant gas passage to be drained away is disposed between the membrane-electrode assembly and the separator and under the reaction surface in the direction of gravity.
摘要翻译：燃料电池包括膜 - 电极组件和隔膜。膜 - 电极组件具有电解质和设置在电解质的相应侧上的一对电极。膜 - 电极组件和隔板在堆叠方向上堆叠。膜 - 电极组件的反应表面沿着重力方向在垂直方向上，并且具有在水平方向上具有较长尺寸的形状。燃料电池设置有反应气体通道，以使反应气体沿着反应表面的纵向方向流动。反应气体是氧化剂气体或燃料气体。允许从反应物气体通道产生的产物水被排出的排水通道设置在膜 - 电极组件和分离器之间并且在重力方向的反作用表面下方。

3. 发明申请

US20060068269A1 Electrode structure for solid polymer type fuel cell 审中-公开
标题翻译：固体聚合物型燃料电池的电极结构
公开(公告)号：US20060068269A1
公开(公告)日：2006-03-30
申请号：US10532963
申请日：2003-10-21
申请人： Kaoru Fukuda , Masaki Tani , Hayato Kaji , Shigeru Inai , Takeshi Muro , Shinya Watanabe
发明人： Kaoru Fukuda , Masaki Tani , Hayato Kaji , Shigeru Inai , Takeshi Muro , Shinya Watanabe
IPC分类号： H01M4/94 , H01M4/96 , H01M8/10 , H01M8/04
CPC分类号： H01M8/1004 , H01M4/8605 , H01M4/8657 , H01M4/926
摘要： A water holding layer having a carbon-based material and a water holding material is arranged on an anode diffusion layer. The water holding material is contained at 5 to 20 wt % of total weight of the water holding material and an electron conductive material. Alternatively, carbon particles having water absorption amount at saturated water vapor pressure at 60° C. is not less than 150 cc/g are contained in the anode diffusion layer. Water absorption ratio of the anode diffusion layer at 60° C. is in a range of 40 to 85%, a differential pressure is in a range of 60 to 120 mmaq, and a ratio of quantity of electric charge of catalytic material of the cathode catalytic layer existing in proton conductive passage from the polymer electrolyte membrane is not less than 15% of the quantity of electric charge of all the catalytic material existing in the cathode catalytic layer. Furthermore, a layer including carbon particles having water absorption amount at saturated water vapor pressure at 60° C. of not less than 150 cc/g and fluorine resin, is arranged on a carbon-based material having a contact angle with water of not more than 90° by performing a hydrophilic treatment. The water absorption ratio at 60° C. is in a range of 40 to 85 wt %, and the penetration resistance is not more than 5 mΩ.
摘要翻译：具有碳基材料和保水材料的保水层设置在阳极扩散层上。保水材料的含水量为水保持材料的总重量的5〜20重量％和电子传导性材料。或者，阳极扩散层中含有在60℃的饱和水蒸气压下的吸水量为150cc / g以上的碳粒子。阳极扩散层在60℃下的吸水率在40〜85％的范围内，差压在60〜120mm范围内，阴极的催化剂材料的电荷比例存在于高分子电解质膜的质子传导路径中的催化剂层不低于存在于阴极催化剂层中的所有催化材料的电荷量的15％。此外，将具有不低于150cc / g的饱和水蒸汽压在60℃以下的吸水量为150cc / g以上的碳粒子和氟树脂的层设置在与水不接触的接触角的碳系材料上超过90°。 60℃下的吸水率为40〜85重量％，耐渗透性为5mOmega以下。

4. 发明授权

US09160016B2 Fuel cell 有权
标题翻译：燃料电池
公开(公告)号：US09160016B2
公开(公告)日：2015-10-13
申请号：US13347595
申请日：2012-01-10
申请人： Kentaro Ishida , Akihiro Matsui , Narutoshi Sugita , Hayato Kaji
发明人： Kentaro Ishida , Akihiro Matsui , Narutoshi Sugita , Hayato Kaji
IPC分类号： H01M8/06 , H01M8/10 , H01M8/04 , H01M8/02
CPC分类号： H01M8/04156 , H01M8/0271 , H01M2008/1095 , Y02E60/50
摘要： A fuel cell includes a membrane-electrode assembly and a separator. The membrane-electrode assembly has an electrolyte and a pair of electrodes that are disposed on respective sides of the electrolyte. The membrane-electrode assembly and the separator are stacked in a stacking direction. A reaction surface of the membrane-electrode assembly is in a vertical direction along a direction of gravity and has a shape having a longer dimension in a horizontal direction. The fuel cell is provided with a reactant gas passage to allow a reactant gas to flow along a longitudinal direction of the reaction surface. The reactant gas is an oxidant gas or a fuel gas. A drain channel to allow product water from the reactant gas passage to be drained away is disposed between the membrane-electrode assembly and the separator and under the reaction surface in the direction of gravity.
摘要翻译：燃料电池包括膜 - 电极组件和隔膜。膜 - 电极组件具有电解质和设置在电解质的相应侧上的一对电极。膜 - 电极组件和隔板在堆叠方向上堆叠。膜 - 电极组件的反应表面沿着重力方向在垂直方向上，并且具有在水平方向上具有较长尺寸的形状。燃料电池设置有反应气体通道，以使反应气体沿着反应表面的纵向方向流动。反应气体是氧化剂气体或燃料气体。允许从反应物气体通道产生的产物水被排出的排水通道设置在膜 - 电极组件和分离器之间并且在重力方向的反作用表面下方。

5. 发明授权

US07722977B2 Fuel cell stack comprising current collector provided at least at one fluid passage 有权
标题翻译：包括至少设置在一个流体通道处的集流器的燃料电池堆
公开(公告)号：US07722977B2
公开(公告)日：2010-05-25
申请号：US11198779
申请日：2005-08-05
申请人： Masahiko Sato , Takahiro Takai , Makoto Tsuji , Masao Utsunomiya , Hayato Kaji , Shuhei Goto , Satoru Terada
发明人： Masahiko Sato , Takahiro Takai , Makoto Tsuji , Masao Utsunomiya , Hayato Kaji , Shuhei Goto , Satoru Terada
IPC分类号： H01M2/00 , H01M2/02 , H01M8/12
CPC分类号： H01M8/0206 , H01M8/0247 , H01M8/0258 , H01M8/0267 , H01M8/0271 , H01M8/0297 , H01M8/04029 , H01M8/241 , H01M8/242 , H01M8/2483 , H01M8/2484
摘要： A terminal plate, an insulating plate, and an end plate are stacked on a stack body. The terminal plate has current collectors at least at lower portions of an oxygen-containing gas supply passage, a coolant supply passage, a fuel gas discharge passage, a fuel gas supply passage, a coolant discharge passage, and an oxygen-containing gas discharge passage. The current collectors contact the water generated in the reaction or a coolant for collecting electricity.
摘要翻译：端子板，绝缘板和端板堆叠在堆叠体上。端子板至少在含氧气体供给通道，冷却剂供给通道，燃料气体排出通道，燃料气体供应通道，冷却剂排出通道和含氧气体排出通道的至少下部具有集流器。电流收集器接触反应中产生的水或用于收集电力的冷却剂。

6. 发明授权

US07232627B2 Electrode for solid polymer fuel cell 有权
标题翻译：固体聚合物燃料电池用电极
公开(公告)号：US07232627B2
公开(公告)日：2007-06-19
申请号：US10703072
申请日：2003-11-07
申请人： Kaoru Fukuda , Masaki Tani , Shigeru Inai , Hayato Kaji , Chikara Iwasawa , Shinya Watanabe , Katsuhiko Kohyama , Hiroshi Shinkai , Takeshi Muro
发明人： Kaoru Fukuda , Masaki Tani , Shigeru Inai , Hayato Kaji , Chikara Iwasawa , Shinya Watanabe , Katsuhiko Kohyama , Hiroshi Shinkai , Takeshi Muro
IPC分类号： H01M4/00
CPC分类号： H01M4/8821 , H01M4/8605 , H01M4/8636 , H01M4/921 , H01M4/926 , H01M8/0234 , H01M8/04097 , H01M8/04104 , H01M8/04291 , H01M8/1007
摘要： An electrode for a solid polymer fuel cell includes a gas diffusion layer, an electrode catalyst layer disposed between a solid polymer membrane of the fuel cell and the gas diffusion layer, and a water-holding layer disposed between the gas diffusion layer and the electrode catalyst layer. Under high-relative humidity conditions of reaction gases, flooding can be prevented because the electrode catalyst layer is made porous, while under low-relative humidity conditions of reaction gases, sufficient water contents can be stably provided thanks to the water-holding layer so that proton conductivity of the solid polymer membrane can be maintained appropriately. Consequently, high-performance and high-durability electrode and membrane electrode assembly for a solid polymer fuel cell can be provided such that the performance and the durability thereof are not affected by change in relative humidity in reactant gases supplied to the solid polymer fuel cell.
摘要翻译：固体高分子型燃料电池用电极包括气体扩散层，设置在燃料电池的固体聚合物膜与气体扩散层之间的电极催化剂层和配置在气体扩散层与电极催化剂之间的保水层层。在反应气体的高相对湿度条件下，由于电极催化剂层为多孔，可以防止溢流，而在反应气体的低相对湿度条件下，由于保水层能够稳定地提供足够的水含量，可以适当地维持固体聚合物膜的质子传导性。因此，可以提供用于固体聚合物燃料电池的高性能和高耐久性的电极和膜电极组件，使得其性能和耐久性不受供应到固体聚合物燃料电池的反应气体中相对湿度的变化的影响。

7. 发明申请

US20060040159A1 Fuel cell stack 有权
标题翻译：燃料电池堆
公开(公告)号：US20060040159A1
公开(公告)日：2006-02-23
申请号：US11198779
申请日：2005-08-05
申请人： Masahiko Sato , Takahiro Takai , Makoto Tsuji , Masao Utsunomiya , Hayato Kaji , Shuhei Goto , Satoru Terada
发明人： Masahiko Sato , Takahiro Takai , Makoto Tsuji , Masao Utsunomiya , Hayato Kaji , Shuhei Goto , Satoru Terada
IPC分类号： H01M2/02
CPC分类号： H01M8/0206 , H01M8/0247 , H01M8/0258 , H01M8/0267 , H01M8/0271 , H01M8/0297 , H01M8/04029 , H01M8/241 , H01M8/242 , H01M8/2483 , H01M8/2484
摘要： A terminal plate, an insulating plate, and an end plate are stacked on a stack body. The terminal plate has current collectors at least at lower portions of an oxygen-containing gas supply passage, a coolant supply passage, a fuel gas discharge passage, a fuel gas supply passage, a coolant discharge passage, and an oxygen-containing gas discharge passage. The current collectors contact the water generated in the reaction or a coolant for collecting electricity.
摘要翻译：端子板，绝缘板和端板堆叠在堆叠体上。端子板至少在含氧气体供给通道，冷却剂供给通道，燃料气体排出通道，燃料气体供应通道，冷却剂排出通道和含氧气体排出通道的至少下部具有集流器。电流收集器接触反应中产生的水或用于收集电力的冷却剂。

8. 发明申请

US20120251900A1 FUEL CELL SYSTEM 审中-公开
标题翻译：燃油电池系统
公开(公告)号：US20120251900A1
公开(公告)日：2012-10-04
申请号：US13433600
申请日：2012-03-29
申请人： Tatsuya SUGAWARA , Tomoki KOBAYASHI , Motohiro SUZUKI , Takuma KANAZAWA , Takuya WAKABAYASHI , Hayato KAJI
发明人： Tatsuya SUGAWARA , Tomoki KOBAYASHI , Motohiro SUZUKI , Takuma KANAZAWA , Takuya WAKABAYASHI , Hayato KAJI
IPC分类号： H01M8/06
CPC分类号： H01M8/04089 , H01M8/04201 , H01M8/0441 , H01M8/04559 , H01M8/04589 , H01M2008/1095 , H01M2250/407 , Y02E60/563
摘要： A fuel cell system is equipped with an expander which is driven by an off-gas exhausted from an oxidant eject path, and which transmits motive power to a compressor, a bypass route in the oxidant eject path which bypasses a humidifier, a flow control valve which changes an opening degree of the bypass route, a voltage sensor which detects an output voltage of the fuel cell stack, a current sensor which detects an output current of the fuel cell stack, and a bypass controlling member which changes a bypass ratio which is a ratio of a magnitude of a flow rate of the off-gas circulating the bypass route with respect to an overall flow rate of the off-gas ejected from the fuel cell stack to the oxidant eject path by the flow control valve according to the output power of the fuel cell stack.
摘要翻译：燃料电池系统配备有膨胀器，其由从氧化剂排放路径排出的废气驱动，并且将动力传递到压缩机，绕过加湿器的氧化剂排放路径中的旁路路线，流量控制阀其改变旁路路径的开度，检测燃料电池堆的输出电压的电压传感器，检测燃料电池堆的输出电流的电流传感器，以及改变旁路比的旁路控制构件，循环旁路通路的废气的流量的大小相对于从燃料电池堆喷射到氧化剂喷出路径的废气的总流量的比率，通过流量控制阀根据输出燃料电池堆的功率。

9. 发明授权

US06847518B2 Membrane electrode assembly for polymer electrolyte fuel cell 有权
标题翻译：用于聚合物电解质燃料电池的膜电极组件
公开(公告)号：US06847518B2
公开(公告)日：2005-01-25
申请号：US10725331
申请日：2003-12-02
申请人： Kaoru Fukuda , Masaki Tani , Hayato Kaji , Shigeru Inai , Takeshi Muro , Shinya Watanabe , Tomoyuki Tada , Masahiko Inoue
发明人： Kaoru Fukuda , Masaki Tani , Hayato Kaji , Shigeru Inai , Takeshi Muro , Shinya Watanabe , Tomoyuki Tada , Masahiko Inoue
IPC分类号： H01M4/90 , H01G9/02 , H01G9/04 , H01M4/86 , H01M4/88 , H01M4/92 , H01M4/96 , H01M8/10
CPC分类号： H01M4/926 , H01M4/8605 , H01M4/921 , H01M8/1004
摘要： A membrane electrode assembly for a polymer electrolyte fuel cell has a polymer electrolyte membrane, an anode, and a cathode having a catalytic layer and a diffusion layer. The alloy catalyst contains ruthenium in the anode diffusion layer. The assembly has less loss of efficiency, particularly when operated at high potentials.
摘要翻译：用于聚合物电解质燃料电池的膜电极组件具有聚合物电解质膜，阳极和具有催化层和扩散层的阴极。合金催化剂在阳极扩散层中含有钌。该组件的效率损失较小，特别是在高电位下运行时。

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