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1. 发明授权

US08987361B2 Organosilane coupling agent 有权
标题翻译：有机硅烷偶联剂
公开(公告)号：US08987361B2
公开(公告)日：2015-03-24
申请号：US13321825
申请日：2010-05-20
申请人： Karine Longchambon , José Carlos Araujo Da Silva , Nicolas Seeboth , Sergey Ivanov
发明人： Karine Longchambon , José Carlos Araujo Da Silva , Nicolas Seeboth , Sergey Ivanov
IPC分类号： C08K5/24 , C07F7/08
CPC分类号： C07F7/0836
摘要： An organosilane of general formula I below: (HO)2R1Si—Z—Sm—R2 in which: R1, which are identical or different, each represent a monovalent hydrocarbon-based group chosen from alkyls, which are linear or branched, cycloalkyls or aryls, having from 1 to 18 carbon atoms; R2 represents a monovalent hydrocarbon-based group chosen from alkyls, which are linear or branched, cycloalkyls or aryls, having from 1 to 30 carbon atoms; Z represents a divalent bonding group comprising from 1 to 18 carbon atoms; and m is a number greater than or equal to 2.
摘要翻译：下述通式I的有机硅烷：（HO）2R1Si-Z-Sm-R2其中：相同或不同的R1各自表示选自烷基的一价烃基，其为直链或支链，环烷基或芳基具有1至18个碳原子; R2表示选自具有1至30个碳原子的直链或支链，环烷基或芳基的烷基的单价烃基; Z表示包含1至18个碳原子的二价键合基团; m是大于或等于2的数。

2. 发明授权

US08987353B2 Rubber composition including an organosilane coupling agent 有权
标题翻译：橡胶组合物，包括有机硅烷偶联剂
公开(公告)号：US08987353B2
公开(公告)日：2015-03-24
申请号：US13321824
申请日：2010-05-20
申请人： Karine Longchambon , José Carlos Araujo Da Silva , Nicolas Seeboth
发明人： Karine Longchambon , José Carlos Araujo Da Silva , Nicolas Seeboth
IPC分类号： C08J3/20 , C08K3/36 , B60C1/00 , C08K5/548 , C08L9/06 , C08L9/00 , C08L57/02
CPC分类号： C08K3/36 , B60C1/0016 , C08K5/548 , C08L9/00 , C08L9/06 , C08L57/02 , C08L21/00 , C08L2666/08
摘要： A rubber composition that can be used for the manufacture of tires, based on at least one diene elastomer; one sulphur-based crosslinking system; one inorganic filler as reinforcing filler; one coupling agent of general formula I below: (HO)3-nR1nSi—Z—Sm—R2 wherein in which: R1, which are identical or different, each represent a monovalent hydrocarbon-based group chosen from alkyls, which are linear or branched, cycloalkyls or aryls, having from 1 to 18 carbon atoms; R2 represents a monovalent hydrocarbon-based group chosen from alkyls, which are linear or branched, cycloalkyls or aryls, having from 1 to 30 carbon atoms; Z represents a divalent bonding group comprising from 1 to 18 carbon atoms; n is an integer equal to 0, 1 or 2; and m is a number greater than or equal to 2.
摘要翻译：一种可用于制造基于至少一种二烯弹性体的轮胎的橡胶组合物; 一种硫基交联体系; 一种无机填料作为增强填料; 一种下式I的偶联剂：（HO）3-nR1nSi-Z-Sm-R2其中：R1相同或不同，各自表示选自烷基的一价烃基，其为直链或支链具有1至18个碳原子的环烷基或芳基; R2表示选自具有1至30个碳原子的直链或支链，环烷基或芳基的烷基的单价烃基; Z表示包含1至18个碳原子的二价键合基团; n是等于0,1或2的整数; m是大于或等于2的数。

3. 发明授权

US08957155B2 Blocked mercaptosilane coupling agent 有权
标题翻译：封闭的巯基硅烷偶联剂
公开(公告)号：US08957155B2
公开(公告)日：2015-02-17
申请号：US13141511
申请日：2009-12-18
申请人： Nicolas Seeboth , Karine Longchambon , Laure Belin , José Carlos Araujo Da Silva
发明人： Nicolas Seeboth , Karine Longchambon , Laure Belin , José Carlos Araujo Da Silva
IPC分类号： C08F8/42 , C07F7/18
CPC分类号： C07F7/1804
摘要： The invention relates to a blocked mercaptosilane of general formula I below: (HO)2R1—Si—Z—S—C(═O)-A in which: R1 represents a monovalent hydrocarbon-based group chosen from alkyls, which are linear or branched, cycloalkyls or aryls, having from 1 to 18 carbon atoms; A represents hydrogen or a monovalent hydrocarbon-based group chosen from alkyls, which are linear or branched, cycloalkyls or aryls, having from 1 to 18 carbon atoms; Z represents a divalent bonding group comprising from 1 to 18 carbon atoms.
摘要翻译：本发明涉及以下通式I的封端巯基硅烷：（HO）2R1-Si-Z-S-C（= O）-A，其中：R1表示选自烷基的一价烃基，其为直链或具有1至18个碳原子的支链，环烷基或芳基; A表示氢或选自具有1至18个碳原子的直链或支链，环烷基或芳基的烷基的一价烃基; Z表示包含1至18个碳原子的二价键合基团。

4. 发明申请

US20120157571A1 Rubber Composition Including an Organosilane Coupling Agent 有权
标题翻译：含有机硅烷偶联剂的橡胶组合物
公开(公告)号：US20120157571A1
公开(公告)日：2012-06-21
申请号：US13321824
申请日：2010-05-20
申请人： Karine Longchambon , José Carlos Araujo Da Silva , Nocolas Seeboth
发明人： Karine Longchambon , José Carlos Araujo Da Silva , Nocolas Seeboth
IPC分类号： C08L9/02 , C08J3/22 , C08K3/10
CPC分类号： C08K3/36 , B60C1/0016 , C08K5/548 , C08L9/00 , C08L9/06 , C08L57/02 , C08L21/00 , C08L2666/08
摘要： A rubber composition that can be used for the manufacture of tires, based on at least one diene elastomer; one sulphur-based crosslinking system; one inorganic filler as reinforcing filler; one coupling agent of general formula I below: (HO)3-nR1nSi—Z—Sm—R2 wherein in which: R1, which are identical or different, each represent a monovalent hydrocarbon-based group chosen from alkyls, which are linear or branched, cycloalkyls or aryls, having from 1 to 18 carbon atoms; R2 represents a monovalent hydrocarbon-based group chosen from alkyls, which are linear or branched, cycloalkyls or aryls, having from 1 to 30 carbon atoms; Z represents a divalent bonding group comprising from 1 to 18 carbon atoms; n is an integer equal to 0, 1 or 2; and m is a number greater than or equal to 2.
摘要翻译：一种可用于制造基于至少一种二烯弹性体的轮胎的橡胶组合物; 一种硫基交联体系; 一种无机填料作为增强填料; 一种下式I的偶联剂：（HO）3-nR1nSi-Z-Sm-R2其中：R1相同或不同，各自表示选自烷基的一价烃基，其为直链或支链具有1至18个碳原子的环烷基或芳基; R2表示选自具有1至30个碳原子的直链或支链，环烷基或芳基的烷基的单价烃基; Z表示包含1至18个碳原子的二价键合基团; n是等于0,1或2的整数; m是大于或等于2的数。

5. 发明申请

US20110306700A1 RUBBER COMPOSITION COMPRISING A BLOCKED MERCAPTOSILANE COUPLING AGENT 有权
标题翻译：包含堵塞的联合硅烷偶联剂的橡胶组合物
公开(公告)号：US20110306700A1
公开(公告)日：2011-12-15
申请号：US13141206
申请日：2009-12-18
申请人： Laure Belin , Karine Longchambon , José Carlos Araujo Da Silva
发明人： Laure Belin , Karine Longchambon , José Carlos Araujo Da Silva
IPC分类号： C08L9/00 , C08K3/36 , C08J3/22 , C08J5/14 , C08L7/00 , C08K3/10
CPC分类号： C08K3/0033 , B60C1/0016 , C08K3/013 , C08K5/548 , Y10T152/10819 , C08L21/00
摘要： The invention relates to a rubber composition that is free of zinc or that contains less than 0.5 phr of zinc, which can be used for the manufacture of tyres, based on at least: one diene elastomer; one sulphur-based crosslinking system; one inorganic filler as reinforcing filler; one blocked mercaptosilane of general formula I below: (R3O)R2R1—Si—Z—S—C(═O)-A in which: R1 and R2, which are identical or different, represent a monovalent hydrocarbon-based group chosen from alkyls, which are linear or branched, cycloalkyls or aryls, having from 1 to 18 carbon atoms; R3 represents a monovalent hydrocarbon-based group chosen from linear or branched alkyls having from 1 to 4 carbon atoms; A represents hydrogen or a monovalent hydrocarbon-based group chosen from alkyls, which are linear or branched, cycloalkyls or aryls, having from 1 to 18 carbon atoms; Z represents a divalent bonding group comprising from 1 to 18 carbon atoms.
摘要翻译：本发明涉及一种橡胶组合物，其不含锌或含有少于0.5phr的锌，其可用于制造轮胎，至少基于一种二烯弹性体; 一种硫基交联体系; 一种无机填料作为增强填料; 一种下面通式I的巯基硅烷：（R3O）R2R1-Si-Z-S-C（= O）-A，其中：R1和R2相同或不同，表示选自烷基的一价烃基其为具有1至18个碳原子的直链或支链的环烷基或芳基; R3表示选自具有1至4个碳原子的直链或支链烷基的单价烃基; A表示氢或选自具有1至18个碳原子的直链或支链，环烷基或芳基的烷基的一价烃基; Z表示包含1至18个碳原子的二价键合基团。

6. 发明授权

US09624358B2 Rubber tire composition comprising an azo-silane coupling agent 有权
公开(公告)号：US09624358B2
公开(公告)日：2017-04-18
申请号：US14008620
申请日：2012-03-28
申请人： Christelle Darnaud , José Carlos Araujo Da Silva , Karine Longchambon , Anne Veyland
发明人： Christelle Darnaud , José Carlos Araujo Da Silva , Karine Longchambon , Anne Veyland
IPC分类号： C08K3/36 , C08K5/5455 , C08L7/00 , C08L21/00 , C08F136/08
CPC分类号： C08K5/5455 , C08F136/08 , C08K3/36 , C08L7/00 , C08L21/00
摘要： The invention relates to a tire rubber composition based on at least one diene elastomer, an inorganic filler as reinforcing filler, a coupling agent providing the bonding between the inorganic filler and the diene elastomer, characterized in that the coupling agent is an azosilane compound of following formula (I): (G1)3-a(G2)aSi—Z—NH—C(O)—N═N—C(O)—NH—Z—Si(G1)3-a(G2)a (I) in which: G1, identical to or different from one another, each represent a monovalent hydrocarbon-based group chosen from branched or unbranched, substituted or unsubstituted alkyls, having from 1 to 18 carbon atoms, substituted or unsubstituted cycloalkyls or aryls, having from 5 to 18 carbon atoms, G2, identical to or different from one another, each represent a hydroxyl group or a monovalent group in the form (G3)n-OG1 in which G3 is a divalent linking group having from 1 to 18 carbon atoms and comprising one or more heteroatoms chosen from O, S, Si and N, n being a number equal to or higher than 0 and less than or equal to 18, Z represents a divalent linking group having from 1 to 18 carbon atoms, a is equal to 1, 2 or 3.

7. 发明授权

US09000092B2 Rubber composition comprising a blocked mercaptosilane coupling agent 有权
标题翻译：橡胶组合物，其包含封端的巯基硅烷偶联剂
公开(公告)号：US09000092B2
公开(公告)日：2015-04-07
申请号：US13141206
申请日：2009-12-18
申请人： Laure Belin , Karine Longchambon , José Carlos Araujo Da Silva
发明人： Laure Belin , Karine Longchambon , José Carlos Araujo Da Silva
IPC分类号： C08F8/42 , B60C15/06 , C08K3/00 , B60C1/00 , C08K5/548
CPC分类号： C08K3/0033 , B60C1/0016 , C08K3/013 , C08K5/548 , Y10T152/10819 , C08L21/00
摘要： The invention relates to a rubber composition that is free of zinc or that contains less than 0.5 phr of zinc, which can be used for the manufacture of tires, based on at least: one diene elastomer; one sulphur-based crosslinking system; one inorganic filler as reinforcing filler; one blocked mercaptosilane of general formula I below: (R3O)R2R1—Si—Z—S—C(═O)-A in which: R1 and R2, which are identical or different, represent a monovalent hydrocarbon-based group chosen from alkyls, which are linear or branched, cycloalkyls or aryls, having from 1 to 18 carbon atoms; R3 represents a monovalent hydrocarbon-based group chosen from linear or branched alkyls having from 1 to 4 carbon atoms; A represents hydrogen or a monovalent hydrocarbon-based group chosen from alkyls, which are linear or branched, cycloalkyls or aryls, having from 1 to 18 carbon atoms; Z represents a divalent bonding group comprising from 1 to 18 carbon atoms.
摘要翻译：本发明涉及一种橡胶组合物，其不含锌或含有少于0.5phr的锌，其可用于制造轮胎，至少基于一种二烯弹性体; 一种硫基交联体系; 一种无机填料作为增强填料; 一种下面通式I的巯基硅烷：（R3O）R2R1-Si-Z-S-C（= O）-A，其中：R1和R2相同或不同，表示选自烷基的一价烃基其为具有1至18个碳原子的直链或支链的环烷基或芳基; R3表示选自具有1至4个碳原子的直链或支链烷基的单价烃基; A表示氢或选自具有1至18个碳原子的直链或支链，环烷基或芳基的烷基的一价烃基; Z表示包含1至18个碳原子的二价键合基团。

8. 发明申请

US20140228479A1 RUBBER TIRE COMPOSITION COMPRISING AN AZO-SILANE COUPLING AGENT 有权
标题翻译：包含AZO-硅烷偶联剂的橡胶轮胎组合物
公开(公告)号：US20140228479A1
公开(公告)日：2014-08-14
申请号：US14008620
申请日：2012-03-28
申请人： Christelle Darnaud , José Carlos Araujo Da Silva , Karine Longchambon , Anne Veyland
发明人： Christelle Darnaud , José Carlos Araujo Da Silva , Karine Longchambon , Anne Veyland
IPC分类号： C08K5/5455 , C08F136/08 , C08K3/36
CPC分类号： C08K5/5455 , C08F136/08 , C08K3/36 , C08L7/00 , C08L21/00
摘要： The invention relates to a tire rubber composition based on at least one diene elastomer, an inorganic filler as reinforcing filler, a coupling agent providing the bonding between the inorganic filler and the diene elastomer, characterized in that the coupling agent is an azosilane compound of following formula (I): (G1)3-a(G2)aSi—Z—NH—C(O)—N═N—C(O)—NH—Z—Si(G1)3-a(G2)a (I) in which: G1, identical to or different from one another, each represent a monovalent hydrocarbon-based group chosen from branched or unbranched, substituted or unsubstituted alkyls, having from 1 to 18 carbon atoms, substituted or unsubstituted cycloalkyls or aryls, having from 5 to 18 carbon atoms, G2, identical to or different from one another, each represent a hydroxyl group or a monovalent group in the form (G3)n-OG1 in which G3 is a divalent linking group having from 1 to 18 carbon atoms and comprising one or more heteroatoms chosen from O, S, Si and N, n being a number equal to or higher than 0 and less than or equal to 18, Z represents a divalent linking group having from 1 to 18 carbon atoms, a is equal to 1, 2 or 3.
摘要翻译：本发明涉及一种基于至少一种二烯弹性体，无机填料作为增强填料的轮胎橡胶组合物，提供无机填料和二烯弹性体之间的结合的偶联剂，其特征在于偶联剂是下列的偶氮硅烷化合物式（I）：（G1）3-a（G2）aSi-Z-NH-C（O）-N = N-C（O）-NH-Z-Si I），其中：G1彼此相同或不同，各自表示选自具有1至18个碳原子的支链或非支链，取代或未取代的烷基，取代或未取代的环烷基或芳基的单价烃基，其具有 5〜18个碳原子，相互相同或不同的G2分别表示（G3）n-OG1中的羟基或一价基团，其中G3为碳原子数为1〜18的二价连接基团并且包含一个或多个选自O，S，Si和N的杂原子，n等于或高于 r大于0且小于或等于18，Z表示具有1至18个碳原子的二价连接基团，a等于1,2或3。

9. 发明申请

US20140371345A1 RUBBER TIRE COMPOSITION COMPRISING AN AZO-SILANE COUPLING AGENT 审中-公开
标题翻译：包含AZO-硅烷偶联剂的橡胶轮胎组合物
公开(公告)号：US20140371345A1
公开(公告)日：2014-12-18
申请号：US14008832
申请日：2012-03-28
申请人： Christelle Darnaud , José Carlos Araujo Da Silva , Karine Longchambon , Anne Veyland
发明人： Christelle Darnaud , José Carlos Araujo Da Silva , Karine Longchambon , Anne Veyland
IPC分类号： C08K5/5455 , C08K13/02 , C08K3/36 , C08L7/00 , C08K3/04
CPC分类号： C08K5/5455 , C08K3/04 , C08K3/36 , C08K13/02 , C08L7/00 , C08L21/00
摘要： A tire rubber composition based on at least one diene elastomer, an inorganic filler as reinforcing filler, a coupling agent providing the bonding between the inorganic filler and the diene elastomer, wherein the coupling agent is an azosilane compound of formula (I): (G1)3-a(G2)aSi—Z—NH—C(O)—N═N—C(O)—NH—Z—Si(G1)3-a(G2)a (I) wherein: G1, identical to or different, each represent a monovalent hydrocarbon group chosen from branched or unbranched, substituted or unsubstituted alkyls having from 1 to 18 carbon atoms, substituted or unsubstituted cycloalkyls or aryls having from 5 to 18 carbon atoms, G2, identical to or different, each represent a hydroxyl group or a monovalent group chosen from branched or unbranched, substituted or unsubstituted alkoxyls having from 1 to 18 carbon atoms, substituted or unsubstituted cycloalkoxyls having from 5 to 18 carbon atoms, Z represents a divalent linking group having from 1 to 18 carbon atoms, a is equal to 1, 2 or 3.
摘要翻译：一种基于至少一种二烯弹性体，无机填料作为增强填料的轮胎橡胶组合物，提供无机填料和二烯弹性体之间的结合的偶联剂，其中偶联剂是式（I）的偶氮硅烷化合物：（G1 ）3-a（G2）aSi-Z-NH-C（O）-N = N-C（O）-NH-Z-Si（G1）3-a（G2）a（I）其中：G1，各自表示选自具有1至18个碳原子的支链或非支链，取代或未取代的烷基，取代或未取代的环烷基或具有5至18个碳原子的芳基，G 2，各自相同或不同的一价烃基表示选自具有1至18个碳原子的支链或非支链，取代或未取代烷氧基的羟基或一价基团，具有5至18个碳原子的取代或未取代的环烷氧基，Z表示具有1至18个碳原子的二价连接基团原子a等于1,2或3。

10. 发明授权

US08492475B2 Rubber composition for tire comprising an organosiloxane coupling agent 有权
标题翻译：包含有机硅氧烷偶联剂的轮胎用橡胶组合物
公开(公告)号：US08492475B2
公开(公告)日：2013-07-23
申请号：US13038887
申请日：2011-03-02
申请人： José Carlos Araujo Da Silva , Karine Longchambon , Sebastien Sterin
发明人： José Carlos Araujo Da Silva , Karine Longchambon , Sebastien Sterin
IPC分类号： B60C1/00 , C08G77/26
CPC分类号： C08K5/5419 , B60C1/00 , B60C1/0016 , B60C1/0025 , B60C2015/0614 , C08K5/5465 , Y10T428/2995 , C08L21/00
摘要： A subject-matter of the present invention is a rubber composition intended for the manufacture of tires or of tire semi-finished products, based on at least one isoprene elastomer, an inorganic filler as reinforcing filler and a polyfunctional organosiloxane coupling agent capable of providing the bonding between the reinforcing inorganic filler and the isoprene elastomer, comprising per molecule, grafted to its silicon atoms, on the one hand at least one hydroxyl or hydrolysable functional group allowing it to be grafted to the reinforcing inorganic filler and, on the other hand, at least one group bearing at least one azodicarbonyl functional group —CO—N═N—CO— allowing it to be grafted to the isoprene elastomer.
摘要翻译：本发明的主题是用于制造轮胎或轮胎半成品的橡胶组合物，其基于至少一种异戊二烯弹性体，作为增强填料的无机填料和能够提供该功能的多官能有机硅氧烷偶联剂增强无机填料和异戊二烯弹性体之间的键合，一方面包含每分子接枝到其硅原子上的至少一个羟基或可水解官能团，使其能够接枝到增强无机填料上，另一方面，至少一个带有至少一个偶氮二羰基官能团-CO-N = N-CO-的基团，使其能够接枝到异戊二烯弹性体上。

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