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1. 发明申请

US20100116717A1 METHOD FOR THE DESULFURIZATION OF FUELS AND HIGHLY ACTIVE NICKEL CARRIER CATALYST BASED ON ALUMINUM OXIDE SUITABLE FOR SAID METHOD 有权
标题翻译：基于氧化铝的燃料和高活性镍催化剂的脱硫方法，适用于合适的方法
公开(公告)号：US20100116717A1
公开(公告)日：2010-05-13
申请号：US12531540
申请日：2008-03-13
申请人： Jurgen Ladebeck , Tiberius Regula , Klaus Wanninger , Wolfgang Gabriel , Frank Grossmann , Jürgen Koy
发明人： Jurgen Ladebeck , Tiberius Regula , Klaus Wanninger , Wolfgang Gabriel , Frank Grossmann , Jürgen Koy
IPC分类号： C10G45/06 , B01J23/755 , B01J21/04 , C10G29/16
CPC分类号： C10G25/003 , B01J20/08 , B01J20/28007 , B01J20/28014 , B01J20/2803 , B01J20/28057 , B01J20/28069 , B01J20/28078 , B01J23/755 , B01J23/78 , B01J23/892 , B01J35/0053 , B01J35/006 , B01J35/10 , B01J35/1019 , B01J35/1038 , B01J35/108 , B01J37/0009 , B01J37/03 , B82Y30/00 , C10G45/06 , C10G45/48 , C10G45/52 , C10G2300/202 , C10G2300/701 , C10G2400/02
摘要： A highly active nickel carrier catalyst based on aluminium oxide has a nickel content of approximately 20 to 70 wt.-% (as Ni) and optionally comprises a bonding agent and optionally a promoter, selected from the compounds of Mg, Ti, Pb, Pt, Ba, Ca and/or Cu, wherein the size of the Ni crystallites in the reduced state is in the range of approximately 3.5 to 4.5 nm and the distortion factor of the Ni crystallites is approximately 2 to 5%. In a method for the reduction of the content of sulphur compounds in hydrocarbon-based fuels by selective adsorption of the sulphur compounds on a nickel catalyst, a nickel catalyst based on aluminium oxide is used, particularly the nickel catalyst described above. A nickel catalyst based on aluminium oxide may be used for reducing the sulphur compound content in hydrocarbon-based fuels by selective adsorption of the sulphur compounds on said catalyst and/or for the hydrogenation of aromatic compounds.
摘要翻译：基于氧化铝的高活性镍载体催化剂的镍含量为约20至70重量％（如Ni），并且任选地包含粘合剂和任选的助催化剂，其选自Mg，Ti，Pb，Pt ，Ba，Ca和/或Cu，其中处于还原态的Ni微晶的尺寸在约3.5至4.5nm的范围内，并且Ni微晶的变形系数约为2％至5％。在通过硫化合物选择性吸附在镍催化剂上来降低烃基燃料中硫化合物含量的方法中，使用基于氧化铝的镍催化剂，特别是上述镍催化剂。基于氧化铝的镍催化剂可用于通过选择性吸附所述催化剂上的硫化合物和/或芳族化合物的氢化来还原烃基燃料中的硫化合物含量。

2. 发明授权

US08992768B2 Method for the desulfurization of fuels and highly active nickel carrier catalyst based on aluminum oxide suitable for said method 有权
标题翻译：基于适用于所述方法的氧化铝的燃料脱硫和高活性镍载体催化剂的方法
公开(公告)号：US08992768B2
公开(公告)日：2015-03-31
申请号：US12531540
申请日：2008-03-13
申请人： Jürgen Ladebeck , Tiberius Regula , Klaus Wanninger , Wolfgang Gabriel , Frank Grossmann , Jürgen Koy
发明人： Jürgen Ladebeck , Tiberius Regula , Klaus Wanninger , Wolfgang Gabriel , Frank Grossmann , Jürgen Koy
IPC分类号： C10G25/00 , C10G45/06 , B01J20/08 , B01J20/28 , B01J23/755 , B01J23/78 , B01J23/89 , B01J35/10 , B01J37/03 , B82Y30/00 , C10G45/48 , C10G45/52 , B01J35/00 , B01J37/00
CPC分类号： C10G25/003 , B01J20/08 , B01J20/28007 , B01J20/28014 , B01J20/2803 , B01J20/28057 , B01J20/28069 , B01J20/28078 , B01J23/755 , B01J23/78 , B01J23/892 , B01J35/0053 , B01J35/006 , B01J35/10 , B01J35/1019 , B01J35/1038 , B01J35/108 , B01J37/0009 , B01J37/03 , B82Y30/00 , C10G45/06 , C10G45/48 , C10G45/52 , C10G2300/202 , C10G2300/701 , C10G2400/02
摘要： A highly active nickel carrier catalyst based on aluminium oxide has a nickel content of approximately 20 to 70 wt.-% (as Ni) and optionally comprises a bonding agent and optionally a promoter, selected from the compounds of Mg, Ti, Pb, Pt, Ba, Ca and/or Cu, wherein the size of the Ni crystallites in the reduced state is in the range of approximately 3.5 to 4.5 nm and the distortion factor of the Ni crystallites is approximately 2 to 5%. In a method for the reduction of the content of sulphur compounds in hydrocarbon-based fuels by selective adsorption of the sulphur compounds on a nickel catalyst, a nickel catalyst based on aluminium oxide is used, particularly the nickel catalyst described above. A nickel catalyst based on aluminium oxide may be used for reducing the sulphur compound content in hydrocarbon-based fuels by selective adsorption of the sulphur compounds on said catalyst and/or for the hydrogenation of aromatic compounds.
摘要翻译：基于氧化铝的高活性镍载体催化剂的镍含量为约20至70重量％（如Ni），并且任选地包含粘合剂和任选的助催化剂，其选自Mg，Ti，Pb，Pt ，Ba，Ca和/或Cu，其中处于还原态的Ni微晶的尺寸在约3.5至4.5nm的范围内，并且Ni微晶的变形系数约为2％至5％。在通过硫化合物选择性吸附在镍催化剂上来降低烃基燃料中硫化合物含量的方法中，使用基于氧化铝的镍催化剂，特别是上述镍催化剂。基于氧化铝的镍催化剂可用于通过选择性吸附所述催化剂上的硫化合物和/或芳族化合物的氢化来还原烃基燃料中的硫化合物含量。

3. 发明申请

US20130102819A1 CATALYST COMPOSITION FOR SELECTIVE HYDROGENATION WITH IMPROVED CHARACTERISTICS 审中-公开
标题翻译：具有改进特性的选择性氢化催化剂组合物
公开(公告)号：US20130102819A1
公开(公告)日：2013-04-25
申请号：US13276403
申请日：2011-10-19
申请人： Normen Szesni , Alfred Hagemeyer , Frank Grossmann , Richard Fischer , Michael Urbancic , Claus Lugmair , Mingyong Sun , Hongyi C. Hou , David Michael Lowe
发明人： Normen Szesni , Alfred Hagemeyer , Frank Grossmann , Richard Fischer , Michael Urbancic , Claus Lugmair , Mingyong Sun , Hongyi C. Hou , David Michael Lowe
IPC分类号： C07C5/09 , B01J23/50 , B01J23/52 , B01J31/02 , B01J23/62 , B01J23/89 , B01J23/644 , B01J23/58 , B01J23/44 , B01J23/60
CPC分类号： B01J23/44 , B01J21/04 , B01J23/50 , B01J23/52 , B01J23/58 , B01J23/60 , B01J23/62 , B01J23/626 , B01J23/628 , B01J23/6447 , B01J23/8926 , B01J31/0277 , B01J31/0279 , B01J31/0284 , B01J35/008 , B01J35/1009 , B01J35/1038 , B01J37/0201 , B01J37/024 , B01J37/16 , B01J2231/645 , B01J2531/824 , C07C7/167 , C10G45/40 , C10G2400/20 , Y02P20/52 , C07C11/04 , C07C11/06
摘要： This invention relates to heterogeneous catalysts useful for selective hydrogenation of unsaturated hydrocarbons, comprising palladium and optionally a promoter, supported on a substrate, having an uncoated BET surface area of ≦9 m2/g, the surface being coated with an ionic liquid. Also described are methods of making the catalysts and methods of selective hydrogenation of acetylene and/or dienes in front-end mixed olefin feed streams.
摘要翻译：本发明涉及可用于不饱和烃的选择性氢化的非均相催化剂，其包含负载在基材上的钯和任选的助催化剂，其具有未涂覆的BET表面积为9m 2 / g，该表面用离子液体涂覆。还描述了制备催化剂的方法和在前端混合烯烃进料流中乙炔和/或二烯烃的选择性氢化的方法。

4. 发明授权

US06717155B1 Electron impact ion source 有权
标题翻译：电子冲击离子源
公开(公告)号：US06717155B1
公开(公告)日：2004-04-06
申请号：US10110261
申请日：2002-06-05
申请人： Guenter Zschornack , Vladimir Petrovich Ovsyannikov , Frank Grossmann , Oleg Konstantinovich Koulthachev
发明人： Guenter Zschornack , Vladimir Petrovich Ovsyannikov , Frank Grossmann , Oleg Konstantinovich Koulthachev
IPC分类号： G01K108
CPC分类号： H01J27/18
摘要： The invention provides an electron impact ion source for the generation of multiply- or super-highly-chared ions including an electron gun with cathode and anode for the creation and acceleration of electrons, a device for the axial-symmetric focussing of the electron beam, a device for introducing ionisable substances into an ion trap, which may be opened and closed, in the region of the axial-symmetric focussed electron beam, a device for destroying the electrons after they have passed the ion trap, and a device for creating a vacuum around the axial-symmetrically focussed electron beam and the ion trap within said beam. The device for the axial-symmetric focussing of the electron beam comprises at least two ring structures radially magnetized in opposing directions and each of these ring structures enclosed the electron beam. The two ring structures radially magnetized in opposing directions are connected by magnetic conductors to form a unified magnet system, whereby the closing magnetic field passes the ion residence zone in the ion trap. The cathode has a very high emissivity of ≧25 A/cm2 with a small cathode diameter. A vacuum of from 10−7 to 10−11 Torr in the ion residence zone can be set while operating the electron impact ion source.
摘要翻译：本发明提供了用于产生多次或超高度冷却离子的电子冲击离子源，包括具有用于产生和加速电子的阴极和阳极的电子枪，用于电子束的轴对称聚焦的装置，用于将可离子化物质引入可以在轴对称聚焦电子束的区域中开启和关闭的离子阱的装置，用于在它们通过离子阱之后破坏电子的装置，以及用于产生围绕轴对称聚焦电子束的真空和所述光束内的离子阱。用于电子束的轴对称聚焦的装置包括沿相反方向径向磁化的至少两个环结构，并且这些环结构中的每一个都包围电子束。在相反方向上径向磁化的两个环形结构通过磁性导体连接形成一个统一的磁体系统，由此闭合磁场通过离子阱中的离子驻留区。阴极具有非常高的发射率> = 25A / cm 2，阴极直径小。在操作电子碰撞离子源的同时，可以在离子驻留区中设置10 -7至10 -7乇的真空度。

5. 发明申请

US20110166395A1 METHOD FOR THE PRODUCTION OF NANOCRYSTALLINE NICKEL OXIDES 审中-公开
标题翻译：制备纳米镍镍氧化物的方法
公开(公告)号：US20110166395A1
公开(公告)日：2011-07-07
申请号：US12995272
申请日：2009-05-29
申请人： Hans-Jörg Wölk , Alfred Hagemeyer , Frank Grossmann , Silvia Neumann , Gerhard Mestl
发明人： Hans-Jörg Wölk , Alfred Hagemeyer , Frank Grossmann , Silvia Neumann , Gerhard Mestl
IPC分类号： C01G53/04 , C07C29/141 , C07C1/20
CPC分类号： C01G53/04 , B01J21/04 , B01J23/755 , B01J35/1019 , B01J37/0045 , C01P2002/72 , C01P2004/61 , C01P2004/62 , C01P2006/12 , C01P2006/14 , C01P2006/16 , C01P2006/17 , C01P2006/80
摘要： The present invention relates to a method for the production of nanocrystalline nickel oxides as well as the nickel oxides produced by the method according to the invention and the use thereof as catalyst following reduction to nickel metal, in particular for hydrogenation reactions.
摘要翻译：本发明涉及一种制备纳米晶体氧化镍的方法以及通过本发明的方法生产的氧化镍及其在镍金属还原之后作为催化剂的用途，特别是用于氢化反应。

6. 发明申请

US20080227631A1 Method for Producing a Catalyst for the Desulfurization of Hydrocarbon Flows 审中-公开
标题翻译：生产烃流脱硫催化剂的方法
公开(公告)号：US20080227631A1
公开(公告)日：2008-09-18
申请号：US11814388
申请日：2006-01-31
申请人： Friedrich Schmidt , Frank Grossmann , Richard Fischer , Michael Rau
发明人： Friedrich Schmidt , Frank Grossmann , Richard Fischer , Michael Rau
IPC分类号： B01J23/28 , B01J23/72 , B01J23/06
CPC分类号： C10G45/04 , B01D53/8603 , B01J23/8873 , B01J35/002 , B01J35/1014 , B01J35/1038 , B01J35/108 , B01J37/03 , C10L3/10
摘要： The invention relates to a process for preparing a catalyst for the desulfurization of hydrocarbon streams, which comprises the steps: (a) preparation of an aqueous suspension comprising: a thermally decomposable copper source, a thermally decomposable molybdenum source, and a solid zinc source; (b) heating of the suspension to a temperature at which the thermally decomposable copper source and the thermally decomposable molybdenum source decompose so that a suspension of a precipitate comprising zinc compounds, copper compounds and molybdenum compounds is obtained; (c) cooling of the suspension obtained in step (b); (d) separation of the precipitate from the suspension; (e) drying of the precipitate. The invention further relates to a catalyst which can be obtained by the process of the invention and also to its use for the desulfurization of hydrocarbon streams.
摘要翻译：本发明涉及一种制备用于烃流脱硫的催化剂的方法，其包括以下步骤：（a）制备含水悬浮液，其包括：可热分解的铜源，可热分解的钼源和固体锌源; （b）将悬浮液加热到可热分解的铜源和可热分解的钼源分解的温度，从而获得包含锌化合物，铜化合物和钼化合物的沉淀物的悬浮液; （c）冷却步骤（b）中获得的悬浮液; （d）沉淀物与悬浮液的分离; （e）沉淀物的干燥。本发明还涉及可通过本发明的方法获得的催化剂，以及其用于烃流脱硫的用途。

7. 发明授权

US10315188B2 Catalyst molded body containing graphite 有权
公开(公告)号：US10315188B2
公开(公告)日：2019-06-11
申请号：US14431054
申请日：2013-06-18
申请人： Martin Paulus , Frank Grossmann , Karl-Heinz Stadler
发明人： Martin Paulus , Frank Grossmann , Karl-Heinz Stadler
IPC分类号： B01J23/889 , B01J37/08 , B01J21/18 , B01J23/72 , B01J37/00 , B01J37/16 , B01J37/18 , B01J35/00 , B01J35/10 , C10G2/00 , B01J35/02 , B01J37/04 , B01J23/34 , B01J37/03 , B01J23/02 , B01J23/06 , B01J23/28 , B01J23/74 , B01J33/00
摘要： The invention relates to a catalyst molded body, which is produced by deforming a mixture of a metal oxide and a special graphite. The invention further relates to a method for producing the corresponding catalyst molded bodies and to the use of the catalyst molded bodies for catalytic reactions in which hydrogen acts as a reaction reactant or reaction product, in particular hydrogenation, hydrogenolysis, and dehydrogenation reactions. The catalysts are characterized by an improvement in the activity and selectivity in particular in hydrogenation, hydrogenolysis, and dehydrogenation reactions, said improvement being achieved by adding special graphites.

8. 发明申请

US20110201847A1 METHOD FOR THE PRODUCTION OF NANOCRYSTALLINE NICKEL OXIDES 有权
标题翻译：制备纳米镍镍氧化物的方法
公开(公告)号：US20110201847A1
公开(公告)日：2011-08-18
申请号：US12994963
申请日：2009-05-29
申请人： Hans-Jörg Wölk , Alfred Hagemeyer , Frank Grossmann , Silvia Neumann
发明人： Hans-Jörg Wölk , Alfred Hagemeyer , Frank Grossmann , Silvia Neumann
IPC分类号： B01J23/755 , C01G53/04 , B01J21/18 , C07C33/32 , C07C5/10 , C07C33/30 , C22C19/03
CPC分类号： C01G53/04 , B01J21/04 , B01J23/755 , B01J35/023 , B01J35/1019 , C01B2203/0445 , C01G53/00 , C01P2004/45 , C01P2004/61 , C01P2004/62 , C01P2006/12 , C01P2006/14 , C01P2006/16 , C01P2006/17 , C01P2006/60 , C01P2006/80
摘要： A method for the production of nanocrystalline nickel oxides as well as the nickel oxides produced by the method according to the invention and the use thereof as catalyst following reduction to nickel metal, in particular for hydrogenation reactions.
摘要翻译：一种生产纳米晶体氧化镍的方法以及通过本发明的方法生产的氧化镍及其在镍金属还原之后作为催化剂的用途，特别是用于氢化反应。

9. 发明申请

US20110160485A1 METHOD FOR THE PRODUCTION OF MIXED OXIDES CONTAINING COPPER AND CHROMIUM 审中-公开
标题翻译：用于生产含铜和铬的混合氧化物的方法
公开(公告)号：US20110160485A1
公开(公告)日：2011-06-30
申请号：US12994909
申请日：2009-05-29
申请人： Hans-Jörg Wölk , Alfred Hagemeyer , Frank Grossmann
发明人： Hans-Jörg Wölk , Alfred Hagemeyer , Frank Grossmann
IPC分类号： B01J23/86 , C01G37/02 , C07C47/00 , C07C209/32 , C07C29/149 , B82Y30/00
CPC分类号： C01G37/14 , B01J23/002 , B01J23/868 , B01J37/03 , B01J37/08 , B01J2523/00 , C01G37/006 , C01P2002/32 , C01P2002/60 , C01P2006/12 , Y10T428/2982 , B01J2523/17 , B01J2523/25 , B01J2523/67
摘要： The present invention relates to a method for producing a nanocrystalline mixed oxide material containing copper and chromium as well as the mixed oxide material containing copper and chromium produced by the method according to the invention and its use as catalyst, in particular for dehydrogenating alcohols, for hydrogenation reactions, for reducing nitrocompounds, for hydrogenating carboxylic acids and for hydrogenating free fatty acids to fatty alcohols.
摘要翻译：本发明涉及一种含有铜和铬的纳米晶混合氧化物材料的制造方法以及通过本发明的方法生产的含有铜和铬的混合氧化物材料及其作为催化剂的用途，特别是用于脱氢醇的方法用于还原硝基化合物的氢化反应，用于氢化羧酸和将游离脂肪酸氢化成脂肪醇。

10. 发明授权

US10035137B2 Hydrogenation catalyst and process for production thereof by the use of uncalcined starting material 有权
公开(公告)号：US10035137B2
公开(公告)日：2018-07-31
申请号：US14432004
申请日：2013-09-25
申请人： Martin Paulus , Frank Grossmann , Karl-Heinz Stadler
发明人： Martin Paulus , Frank Grossmann , Karl-Heinz Stadler
IPC分类号： B01J33/00 , B01J23/889 , B01J37/18 , B01J37/03 , B01J37/04 , B01J37/08 , B01J23/72 , B01J35/00 , B01J35/10 , B01J37/00 , C07C29/149 , B01J37/06
CPC分类号： B01J23/8892 , B01J23/72 , B01J33/00 , B01J35/002 , B01J35/1038 , B01J35/1042 , B01J35/109 , B01J37/0009 , B01J37/0063 , B01J37/031 , B01J37/04 , B01J37/06 , B01J37/08 , B01J37/18 , C07C29/149 , C07C31/125
摘要： The invention relates to a process for preparing a shaped Cu—Al catalyst body for the hydrogenation of organic compounds containing a carbonyl function. More particularly, the shaped catalyst body is suitable for the hydrogenation of aldehydes, ketones and of carboxylic acids or esters thereof, specifically of fatty acids or esters thereof, such as fatty acid methyl esters, to the corresponding alcohols such as butanediol. The present invention further relates to Cu—Al catalysts obtainable by the preparation process.

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