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1. 发明申请

US20070088139A1 PROCESS FOR PRODUCING COPOLYMER 审中-公开
标题翻译：制备共聚物的方法
公开(公告)号：US20070088139A1
公开(公告)日：2007-04-19
申请号：US11562812
申请日：2006-11-22
申请人： Jun KAWASHIMA , Katsunari Inagaki , Tatsuo Sassa
发明人： Jun KAWASHIMA , Katsunari Inagaki , Tatsuo Sassa
IPC分类号： C08F4/68
CPC分类号： C08F210/18 , C08F4/68 , C08F4/631 , C08F210/06 , C08F236/20 , C08F2500/25 , C08F2500/03
摘要： There are provided (I) a process for producing a copolymer of ethylene, an α-olefin having from 3 to 20 carbon atoms and optionally a polyene, which comprises the step of copolymerizing those monomers in a polymerization reactor by feeding the following components (A), (B), (C1) and (D) to the polymerization reactor: (A) a transition metal complex, (B) an organic aluminum compound, (C1) a halogen-containing compound, and (D) a Lewis base, wherein those components are fed to the polymerization reactor without a preliminary contact of (1) the component (A) with the component (B), (2) the component (A) with the component (C1), (3) the component (B) with the component (C1), and (4) the component (B) with the component (D); and (II) a process for producing said copolymer, which comprises the step of copolymerizing those monomers in a polymerization reactor (i) by feeding to the polymerization reactor the components (A), (B), (D), (C2) a halogen-containing compound, which is a derivative of an aryl group-containing carboxylic acid, and (C3) a halogen-containing compound, which is not a derivative of a carboxylic acid, or (ii) by feeding thereto the components (A), (B), (D), (C3), and (C4) a halogen-containing compound, which is a derivative of a carboxylic acid containing an unsaturated bond-carrying linear organic group.
摘要翻译：提供（I）制备乙烯，具有3至20个碳原子的α-烯烃和任选的多烯的共聚物的方法，该方法包括通过将以下组分（A ），（B），（C1）和（D））：（A）过渡金属络合物，（B）有机铝化合物，（C1）含卤素化合物和（D）（A）与组分（B），（2）组分（A）与组分（C1），（3）的组分进行预先接触，将组分进料到聚合反应器中，（B）和（4）成分（B）与成分（D）的组成（B）。（II）生产所述共聚物的方法，其包括通过将聚合反应器中的组分（A），（B），（D），（C2）a 含有芳基的羧酸的衍生物的含卤素化合物和（C3）不是羧酸衍生物的含卤素化合物，或（ii）向其中加入组分（A），（B），（D），（C3）和（C4）含卤素化合物，其是含有不饱和键的线性有机基团的羧酸的衍生物。

2. 发明授权

US07262258B2 Process for producing copolymer 失效
标题翻译：制备共聚物的方法
公开(公告)号：US07262258B2
公开(公告)日：2007-08-28
申请号：US10885760
申请日：2004-07-08
申请人： Jun Kawashima , Katsunari Inagaki , Tatsuo Sassa
发明人： Jun Kawashima , Katsunari Inagaki , Tatsuo Sassa
IPC分类号： C08F4/622 , C08F6/29 , C08F6/68
CPC分类号： C08F210/18 , C08F4/68 , C08F4/631 , C08F210/06 , C08F236/20 , C08F2500/25 , C08F2500/03
摘要： There are provided (I) a process for producing a copolymer of ethylene, an α-olefin having from 3 to 20 carbon atoms and optionally a polyene, which comprises the step of copolymerizing those monomers in a polymerization reactor by feeding the following components (A), (B), (C1) and (D) to the polymerization reactor: (A) a transition metal complex, (B) an organic aluminum compound, (C1) a halogen-containing compound, and (D) a Lewis base, wherein those components are fed to the polymerization reactor without a preliminary contact of (1) the component (A) with the component (B), (2) the component (A) with the component (C1), (3) the component (B) with the component (C1), and (4) the component (B) with the component (D); and (II) a process for producing said copolymer, which comprises the step of copolymerizing those monomers in a polymerization reactor (i) by feeding to the polymerization reactor the components (A), (B), (D), (C2) a halogen-containing compound, which is a derivative of an aryl group-containing carboxylic acid, and (C3) a halogen-containing compound, which is not a derivative of a carboxylic acid, or (ii) by feeding thereto the components (A), (B), (D), (C3), and (C4) a halogen-containing compound, which is a derivative of a carboxylic acid containing an unsaturated bond-carrying linear organic group.
摘要翻译：提供（I）制备乙烯，具有3至20个碳原子的α-烯烃和任选的多烯的共聚物的方法，该方法包括通过将以下组分（A ），（B），（C1）和（D））：（A）过渡金属络合物，（B）有机铝化合物，（C1）含卤素化合物和（D）（A）与组分（B），（2）组分（A）与组分（C1），（3）的组分进行预先接触，将组分进料到聚合反应器中，（B）和（4）成分（B）与成分（D）的组成（B）。（II）生产所述共聚物的方法，其包括通过将聚合反应器中的组分（A），（B），（D），（C2）a 含有芳基的羧酸的衍生物的含卤素化合物和（C3）不是羧酸衍生物的含卤素化合物，或（ii）向其中加入组分（A），（B），（D），（C3）和（C4）含卤素化合物，其是含有不饱和键的线性有机基团的羧酸的衍生物。

3. 发明申请

US20050014914A1 Process for producing copolymer 失效
标题翻译：制备共聚物的方法
公开(公告)号：US20050014914A1
公开(公告)日：2005-01-20
申请号：US10885760
申请日：2004-07-08
申请人： Jun Kawashima , Katsunari Inagaki , Tatsuo Sassa
发明人： Jun Kawashima , Katsunari Inagaki , Tatsuo Sassa
IPC分类号： C08F2/06 , C08F4/60 , C08F4/68 , C08F210/00 , C08F210/18 , C08F4/44
CPC分类号： C08F210/18 , C08F4/68 , C08F4/631 , C08F210/06 , C08F236/20 , C08F2500/25 , C08F2500/03
摘要： There are provided (I) a process for producing a copolymer of ethylene, an α-olefin having from 3 to 20 carbon atoms and optionally a polyene, which comprises the step of copolymerizing those monomers in a polymerization reactor by feeding the following components (A), (B), (C1) and (D) to the polymerization reactor: (A) a transition metal complex, (B) an organic aluminum compound, (C1) a halogen-containing compound, and (D) a Lewis base, wherein those components are fed to the polymerization reactor without a preliminary contact of (1) the component (A) with the component (B), (2) the component (A) with the component (C1), (3) the component (B) with the component (C1), and (4) the component (B) with the component (D); and (II) a process for producing said copolymer, which comprises the step of copolymerizing those monomers in a polymerization reactor (i) by feeding to the polymerization reactor the components (A), (B), (D), (C2) a halogen-containing compound, which is a derivative of an aryl group-containing carboxylic acid, and (C3) a halogen-containing compound, which is not a derivative of a carboxylic acid, or (ii) by feeding thereto the components (A), (B), (D), (C3), and (C4) a halogen-containing compound, which is a derivative of a carboxylic acid containing an unsaturated bond-carrying linear organic group.
摘要翻译：提供（I）制备乙烯，具有3至20个碳原子的α-烯烃和任选的多烯的共聚物的方法，该方法包括通过进料以下组分（A（A））将这些单体在聚合反应器中共聚的步骤），（B），（C1）和（D））：（A）过渡金属络合物，（B）有机铝化合物，（C1）含卤素化合物和（D）（A）与组分（B），（2）组分（A）与组分（C1），（3）的组分进行预先接触，将组分进料到聚合反应器中，（B）和（4）成分（B）与成分（D）的组成（B）。（II）生产所述共聚物的方法，其包括通过将聚合反应器中的组分（A），（B），（D），（C2）a 含有芳基的羧酸的衍生物的含卤素化合物和（C3）不是羧酸衍生物的含卤素化合物，或（ii）向其中加入组分（A），（B），（D），（C3）和（C4）含卤素化合物，其是含有不饱和键的线性有机基团的羧酸的衍生物。

4. 发明授权

US08278404B2 Process for producing copolymer 失效
标题翻译：制备共聚物的方法
公开(公告)号：US08278404B2
公开(公告)日：2012-10-02
申请号：US13114577
申请日：2011-05-24
申请人： Jun Kawashima , Katsunari Inagaki , Tatsuo Sassa
发明人： Jun Kawashima , Katsunari Inagaki , Tatsuo Sassa
IPC分类号： C08F4/622 , C08F4/68
CPC分类号： C08F210/18 , C08F4/68 , C08F4/631 , C08F210/06 , C08F236/20 , C08F2500/25 , C08F2500/03
摘要： There are provided (I) a process for producing a copolymer of ethylene, an α-olefin having from 3 to 20 carbon atoms and optionally a polyene, which comprises the step of copolymerizing those monomers in a polymerization reactor by feeding the following components (A), (B), (C1) and (D) to the polymerization reactor: (A) a transition metal complex, (B) an organic aluminum compound, (C1) a halogen-containing compound, and (D) a Lewis base, wherein those components are fed to the polymerization reactor without a preliminary contact of (1) the component (A) with the component (B), (2) the component (A) with the component (C1), (3) the component (B) with the component (C1), and (4) the component (B) with the component (D); and (II) a process for producing said copolymer, which comprises the step of copolymerizing those monomers in a polymerization reactor (i) by feeding to the polymerization reactor the components (A), (B), (D), (C2) a halogen-containing compound, which is a derivative of an aryl group-containing carboxylic acid, and (C3) a halogen-containing compound, which is not a derivative of a carboxylic acid, or (ii) by feeding thereto the components (A), (B), (D), (C3), and (C4) a halogen-containing compound, which is a derivative of a carboxylic acid containing an unsaturated bond-carrying linear organic group.
摘要翻译：提供（I）制备乙烯，具有3至20个碳原子的α-烯烃和任选的多烯的共聚物的方法，该方法包括通过进料以下组分（A（A））将这些单体在聚合反应器中共聚的步骤），（B），（C1）和（D））：（A）过渡金属络合物，（B）有机铝化合物，（C1）含卤素化合物和（D）（A）与组分（B），（2）组分（A）与组分（C1），（3）的组分进行预先接触，将组分进料到聚合反应器中，（B）和（4）成分（B）与成分（D）的组成（B）。（II）生产所述共聚物的方法，其包括通过将聚合反应器中的组分（A），（B），（D），（C2）a 含有芳基的羧酸的衍生物的含卤素化合物和（C3）不是羧酸衍生物的含卤素化合物，或（ii）向其中加入组分（A），（B），（D），（C3）和（C4）含卤素化合物，其是含有不饱和键的线性有机基团的羧酸的衍生物。

5. 发明授权

US08367765B2 Conjugated diene-based polymer, conjugated diene-based polymer composition, and process for producing conjugated diene-based polymer 有权
标题翻译：共轭二烯系聚合物，共轭二烯类聚合物组合物，以及共轭二烯类聚合物的制造方法
公开(公告)号：US08367765B2
公开(公告)日：2013-02-05
申请号：US13206167
申请日：2011-08-09
申请人： Mana Ito , Katsunari Inagaki , Mayumi Oshima
发明人： Mana Ito , Katsunari Inagaki , Mayumi Oshima
IPC分类号： C08L43/04 , C08F230/08 , C08F36/04
CPC分类号： C08F236/10 , C08K3/36 , C08F4/48 , C08L9/06
摘要： Disclosed are a conjugated diene-based polymer from which a polymer composition excellent in fuel cost-saving properties and elongation at break can be obtained, a polymer composition containing the conjugated diene-based polymer and a reinforcing agent, and a process for producing the conjugated diene-based polymer. There is provided a conjugated diene-based polymer having a conjugated diene unit, a monomer unit based on a compound represented by the following formula (1) and a monomer unit based on a compound represented by the following formula (2). wherein R11 represents a hydrogen atom or a hydrocarbyl group, m is 0 or 1, R12 represents a hydrocarbylene group, and X1, X2 and X3 each independently represent a substituted amino group, or a hydrocarbyl group optionally having a substituent, provided that at least one of X1, X2 and X3 is a substituted amino group. wherein R21 represents a hydrogen atom or a hydrocarbyl group, n is 0 or 1, R22 represents a hydrocarbylene group, and A represents a substituted amino group, or a nitrogen-containing heterocyclic group.
摘要翻译：公开了一种共轭二烯类聚合物，其中可以获得具有优异的燃料成本节约性能和断裂伸长率的聚合物组合物，含有共轭二烯系聚合物和增强剂的聚合物组合物，以及制备共轭二烯系聚合物的方法二烯基聚合物。提供具有共轭二烯单元的共轭二烯系聚合物，基于下述式（1）所示的化合物的单体单元和基于下述式（2）表示的化合物的单体单元。其中R11表示氢原子或烃基，m为0或1，R12表示亚烃基，X1，X2和X3各自独立地表示取代的氨基或任选具有取代基的烃基，条件是至少 X 1，X 2和X 3中的一个是取代的氨基。其中R21表示氢原子或烃基，n为0或1，R22表示亚烃基，A表示取代氨基或含氮杂环基。

6. 发明授权

US08436097B2 Process for producing modified polymer rubber 有权
公开(公告)号：US08436097B2
公开(公告)日：2013-05-07
申请号：US12608550
申请日：2009-10-29
申请人： Katsunari Inagaki , Seiichi Mabe , Mayumi Oshima
发明人： Katsunari Inagaki , Seiichi Mabe , Mayumi Oshima
IPC分类号： C08F8/00 , C08F8/42
CPC分类号： C08C19/44 , C08K3/013 , C08L25/18 , C08L15/00
摘要： A process for producing a modified polymer rubber comprising the steps of: (1) polymerizing a conjugated diene monomer or a combination thereof with an aromatic vinyl monomer in a hydrocarbon solvent, in the presence of an alkali metal catalyst or a specified alkali metal compound, to form an alkali metal end-carrying active polymer, and (2) reacting the alkali metal end-carrying active polymer with a specified isocyanurate compound or a combination thereof with a specified coupling agent in a hydrocarbon solvent.

7. 发明授权

US08304488B2 Conjugated diene polymer, conjugated diene polymer composition, and method for producing conjugated diene polymer 有权
标题翻译：共轭二烯聚合物，共轭二烯聚合物组合物和共轭二烯聚合物的制造方法
公开(公告)号：US08304488B2
公开(公告)日：2012-11-06
申请号：US13053938
申请日：2011-03-22
申请人： Toru Fujii , Katsunari Inagaki
发明人： Toru Fujii , Katsunari Inagaki
IPC分类号： C08L43/04 , C08F230/08 , C08F293/00
CPC分类号： C08F236/10 , C08K3/36 , C08F4/48 , C08L19/006
摘要： Conjugated diene polymer is provided that comprises a constitutional unit based on a conjugated diene and a constitutional unit based on a compound represented by Formula (1) below: R1Si(—R2-A)mR33-m (1) wherein m represents an integer of 1 to 3; R1 represents a hydrocarbyl group having a polymerizable carbon-carbon double bond; R2 represents a hydrocarbylene group, and, when there are plural R2s, R2s each may be the same or different; A represents a substituted amino group, and, when there are plural A's, A's each may be the same or different; R3 represents a hydrocarbyl group, a substituted hydrocarbyl group or a substituted amino group, and, when there are plural R3s, R3s each may be the same or different.
摘要翻译：提供了包含基于共轭二烯的结构单元和基于由下式（1）表示的化合物的结构单元的共轭二烯聚合物：R1Si（-R2-A）mR33-m（1）其中m表示 1〜3; R1表示具有可聚合碳 - 碳双键的烃基; R2表示亚烃基，当有多个R2时，各自可以相同或不同， A表示取代的氨基，当存在多个A时，A各自可以相同或不同; R 3表示烃基，取代烃基或取代氨基，当有多个R 3时，R 3可以相同也可以不同。

8. 发明申请

US20120190771A1 PROCESS FOR PRODUCING CONJUGATED DIENE-BASED POLYMER, CONJUGATED DIENE-BASED POLYMER, AND CONJUGATED DIENE-BASED POLYMER COMPOSITION 有权
标题翻译：生产基于二烯的聚合物，共混二烯基聚合物和共混的基于二烯的聚合物组合物的方法
公开(公告)号：US20120190771A1
公开(公告)日：2012-07-26
申请号：US13357371
申请日：2012-01-24
申请人： Mana Ito , Katsunari Inagaki , Mayumi Oshima
发明人： Mana Ito , Katsunari Inagaki , Mayumi Oshima
IPC分类号： C08J5/14 , C08F4/48
CPC分类号： C08F236/06 , C08K3/013 , C08F212/08 , C08F4/48 , C08L21/00 , C08L15/00
摘要： The present invention provides a process for producing a conjugated diene-based polymer, comprising polymerizing a monomer component containing a conjugated diene compound and a silicon-containing vinyl compound using a polymerization initiator represented by the following formula (1) wherein, R11 represents a hydrocarbylene group having 6 to 100 carbon atoms, R12 and R13 represent a hydrocarbyl group optionally having a substituent, or a trihydrocarbylsilyl group, or R12 and R13 are bonded to represent a hydrocarbylene group optionally having, as a hetero atom, at least one kind atom selected from the atomic group consisting of a silicon atom, a nitrogen atom and an oxygen atom.
摘要翻译：本发明提供一种共轭二烯系聚合物的制造方法，其特征在于，使用由下式（1）表示的聚合引发剂使含有共轭二烯化合物的单体成分和含硅乙烯基化合物聚合，其中，R 11表示亚烃基具有6至100个碳原子的基团，R 12和R 13表示任选具有取代基的烃基或三烃基甲硅烷基，或R 12和R 13键合以表示任选具有作为杂原子的至少一种选自来自由硅原子，氮原子和氧原子组成的原子团。

9. 发明申请

US20090005515A1 METHOD FOR PRODUCING CONJUGATED DIENE POLYMER, CONJUGATED DIENE POLYMER, AND CONJUGATED DIENE POLYMER COMPOSITION 审中-公开
标题翻译：生产聚合二烯聚合物，共轭二烯聚合物和共轭二烯聚合物组合物的方法
公开(公告)号：US20090005515A1
公开(公告)日：2009-01-01
申请号：US12140312
申请日：2008-06-17
申请人： Naoaki MAEDA , Mayumi Oshima , Katsunari Inagaki
发明人： Naoaki MAEDA , Mayumi Oshima , Katsunari Inagaki
IPC分类号： C08L9/00 , C08F136/04 , C08F2/06
CPC分类号： C08C19/44 , C08K3/013 , C08K3/04 , C08K5/56 , C08L15/00 , C08L21/00 , C08L2666/08 , C08L9/06
摘要： A method for producing a conjugated diene polymer is provided that includes a step A of polymerizing a conjugated diene-containing monomer in a hydrocarbon solvent in the presence of an alkali metal catalyst, thus giving a polymer having a catalyst-derived alkali metal at one terminus of a polymer chain comprising a conjugated diene-based monomer unit, and a step B of reacting the polymer obtained in step A with a compound represented by the formula below. (In the formula, M denotes an oxygen atom or a sulfur atom, R1, R2, and R3 independently denote an alkyl group having 1 to 4 carbon atoms, m denotes an integer of 1 to 5, and n denotes an integer of 0 to 5.)
摘要翻译：提供了一种共轭二烯聚合物的制造方法，其包括在碱金属催化剂的存在下，在烃溶剂中使含共轭二烯的单体聚合的步骤A，从而得到在一个末端具有催化剂衍生的碱金属的聚合物的包含共轭二烯基单体单元的聚合物链，以及使步骤A中获得的聚合物与下式表示的化合物反应的步骤B. （式中，M表示氧原子或硫原子，R1，R2，R3分别表示碳原子数1〜4的烷基，m表示1〜5的整数，n表示0〜 5.）

10. 发明授权

US06541592B1 Thermoplastic elastomer composition and ethylene-&agr;-olefin copolymer 失效
标题翻译：热塑性弹性体组合物和乙烯-α-烯烃共聚物
公开(公告)号：US06541592B1
公开(公告)日：2003-04-01
申请号：US09636651
申请日：2000-08-09
申请人： Katsunari Inagaki , Tadaaki Nishiyama
发明人： Katsunari Inagaki , Tadaaki Nishiyama
IPC分类号： C08F1014
CPC分类号： C09K3/10 , C08L23/02 , C08L23/04 , C08L23/08 , C08L23/0815 , C08L23/0853 , C08L23/0869 , C09K2200/0617 , C09K2200/062 , C09K2200/0622 , C09K2200/0625 , C08L2666/04
摘要： A thermoplastic elastomer composition comprising 5 to 95 wt % of the following (A) and 5 to 95 wt % of the following (B), wherein the flowability index I according to a test for flow properties with a capillary rheometer is 1.35 or more: (A) an ethylene-&agr;-olefin copolymer having a tensile stress M100 measured according to JIS-K-6251 of 2.5 MPa or less, (B) a polyolefin-based resin having a tensile stress M100 measured according to JIS-K-6251 of 2.5 MPa or more.
摘要翻译：一种热塑性弹性体组合物，其包含5至95重量％的以下（A）和5至95重量％的以下（B），其中根据毛细管流变仪的流动性试验的流动指数I为1.35以上：（A）根据JIS-K-6251测定的拉伸应力M100为2.5MPa以下的乙烯-α-烯烃共聚物，（B）根据JIS-K-6251测定的拉伸应力M100的聚烯烃系树脂为2.5MPa以上。

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