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1. 发明授权

US4764578A Compositions of polyaryloxypyridine oligomers with phthalonitrile end groups, their preparation and use for manufacturing polyaryloxypyridine co-phthalocyanine lattices 失效
标题翻译：具有邻苯二甲腈端基的聚芳氧基吡啶低聚物的组成及其制备和用于制备聚芳氧基吡啶共酞菁晶格
公开(公告)号：US4764578A
公开(公告)日：1988-08-16
申请号：US907905
申请日：1986-09-16
申请人： Jean Malinge , Guy Rabilloud , Bernard Sillion
发明人： Jean Malinge , Guy Rabilloud , Bernard Sillion
IPC分类号： C08G65/40 , C08G65/48 , C08G73/06 , C08G83/00 , C08G73/00
CPC分类号： C08G65/48 , C08G65/4006 , C08G73/0627 , C08G2650/64
摘要： The disclosed compositions of polyaryloxypyridine oligomers with phthalonile end groups are obtained by formation of a composition of polyaryloxypyridine oligomers with alkali phenolate end groups, followed with the reaction of said composition with 4-nitrophthalonitrile. Their average polycondensation degree may range from 1 to 50. They can be used in combination with a co-reactant derived from benzhydrol and containing one or two ortho-dinitrile functional groups, to constitute polyaryloxypyridine co-polyphthalocyanine lattices.
摘要翻译：所公开的具有邻苯二甲腈端基的聚芳氧基吡啶低聚物的组合物通过用碱性酚盐端基形成聚芳氧基吡啶低聚物的组合物，随后将所述组合物与4-硝基邻苯二腈反应而获得。它们的平均缩聚度可以在1至50之间。它们可以与衍生自二苯甲醛并含有一个或两个邻二甲苯基官能团的共反应物组合使用，以构成聚芳氧基吡啶共聚酞菁晶格。

2. 发明授权

US4987218A Polybenzhydrol compositions ending with ethylenic unsaturated groups, cross-linked polymides resulting from their thermal polyermization and the use of said compositions 失效
标题翻译：以乙烯基不饱和基团结束的聚二醇化合物组合物，由它们的热多化引起的交联聚酰亚胺和所述组合物的使用
公开(公告)号：US4987218A
公开(公告)日：1991-01-22
申请号：US55287
申请日：1987-05-29
申请人： Jean Malinge , Guy Rabilloud , Bernard Sillion
发明人： Jean Malinge , Guy Rabilloud , Bernard Sillion
IPC分类号： C08F299/02 , C08G73/10 , C08G73/12
CPC分类号： C08G73/1078 , C08G73/10 , C08G73/101
摘要： Polymer compositions comprising poly(benzhydrolimide) chains ending with ethylenic unsaturated groups complying with the general formula: ##STR1## wherein Ar is a divalent aromatic radical and R a hydrogen atom or a monovalent hydrocarbon radical. They can be prepared by reacting, under imidation condition, at least one primary diamine with at least one benzydrol 3,3', 4,4'-tetracarboxylic acid, a bis (ortho-acid-ester) or a tetraester of such acid and with an anhydride, an acid-ester or a diester of dicarboxylic cycloaliphatic acid with ethylenic unsaturation. These compositions may be converted to cross-linked polymides by thermal polyemrization. They can be used in particular for manufacturing composite materials, adhesives, molded articles and protective coatings withstanding high temperatures.
摘要翻译：聚合物组合物包含以乙烯不饱和基团结束的聚（苯甲酰亚胺）链，其符合以下通式：其中Ar为二价芳族基团，R为氢原子或一价烃基。它们可以通过在酰亚胺化条件下使至少一种伯二胺与至少一种苯并三氢呋喃3,3'，4,4'-四羧酸，这种酸的双（邻 - 酸酯）或四酯反应来制备，和与酸酐，酸酯或具有烯属不饱和度的二羧酸脂环族酸的二酯。这些组合物可以通过热聚合转化成交联聚酰亚胺。它们可以特别用于制造复合材料，粘合剂，模制品和耐高温保护涂层。

3. 发明授权

US4645821A Precursor of copolyphthalocyanine-imide lattice, preparation, and the resultant lattice 失效
标题翻译：共聚酞菁 - 酰亚胺晶格的前体，制备和所得的晶格
公开(公告)号：US4645821A
公开(公告)日：1987-02-24
申请号：US758949
申请日：1985-07-25
申请人： Jean Malinge , Guy Rabilloud , Bernard Sillion
发明人： Jean Malinge , Guy Rabilloud , Bernard Sillion
IPC分类号： C08G73/00 , C07D209/48 , C08G73/10 , C08G73/06
CPC分类号： C07D209/48 , C08G73/10 , C08G73/1035
摘要： Aromatic polyimide compositions, precursors of copolyphthalocyanine-imides,heir manufacturing process and the resultant copolyphthalocyanine-imides, are described.These compositions may result for the reaction of 80.degree.-300.degree. C. of an aromatic tetra acid, diester-diacid, tetraester or dianhydride compound of formula: ##STR1## with an aromatic amino-dinitrile ##STR2## and optionally an aromatic diamine NH.sub.2 --Ar--NH.sub.2. A subsequent heating at 200.degree.-300.degree. C. provides, by cross-linking, copolyphthalocyanine-imides, which are hardened resins, stable at 250.degree.-300.degree. C. in continuous use.
摘要翻译：描述了芳族聚酰亚胺组合物，共聚酞菁 - 酰亚胺的前体，它们的制备方法和所得的共聚酞菁 - 酰亚胺。这些组合物可能导致80-300℃的芳香族四酸，二酯 - 二酸，四酯或二酐化合物与芳香族氨基二腈和任选的芳族二胺NH 2 -Ar-NH2。随后在200-300℃下加热，通过交联，共聚酞菁 - 酰亚胺，它们是硬化树脂，在250-300℃下连续使用时稳定。

4. 发明授权

US4310699A Process for synthesizing bis (phenylglyoxyloyl)benzenes usable for manufacturing polyphenylquinoxaline resins 失效
标题翻译：合成可用于制备聚苯基喹喔啉树脂的双（苯基乙氧基羰基）苯的方法
公开(公告)号：US4310699A
公开(公告)日：1982-01-12
申请号：US152895
申请日：1980-05-23
申请人： Guy Rabilloud , Bernard Sillion
发明人： Guy Rabilloud , Bernard Sillion
IPC分类号： C07C49/83 , C07C45/00 , C07C45/29 , C07C49/784 , C07C67/00 , C08G6/00 , C08G73/06 , C07C45/45
CPC分类号： C08G73/0694 , C07C45/00 , C07C45/29 , C07C45/292 , C07C45/296 , C07C45/298 , C07C49/784 , C08G6/00
摘要： Bis (phenylglyoxyloyl) benzenes are manufactured by a method comprising the reaction of terephthalic or isophthalic aldehyde first with a low proportion of an alkali metal cyanide in a solvent, and then with benzaldehyde; the resultant product is oxidized to the desired bis (phenylglyoxyloyl) benzene.
摘要翻译：双（苯基乙氧基）苯是通过包括在溶剂中首先与低比例的碱金属氰化物反应的对苯二甲酸或间苯二醛，然后与苯甲醛反应的方法制备的; 将所得产物氧化成所需的双（苯基乙氧基羰基）苯。

5. 发明授权

US3968085A Polyamine compositions useful as hardening agents for epoxy resins 失效
标题翻译：可用作环氧树脂硬化剂的多胺组合物
公开(公告)号：US3968085A
公开(公告)日：1976-07-06
申请号：US501696
申请日：1974-08-29
申请人： Guy Rabilloud , Bernard Sillion
发明人： Guy Rabilloud , Bernard Sillion
IPC分类号： C08G63/685 , C08L63/00 , C08G17/14
CPC分类号： C08G63/6856 , C08L63/00 , Y10T428/31525
摘要： The invention concerns new aromatic polyamine compositions useful as hardening agents containing a major proportion of polyamines of the formula: ##EQU1## IN WHICH Ar and Ar' are divalent aromatic radicals having from 1 to 6 rings, R.sub.1 is a divalent hydrocarbon radical or a radical (R.sub.4 -O).sub.m R.sub.4, R.sub.4 being an alkylene and m an integer from 1 to 100.
摘要翻译：本发明涉及可用作含有主要比例的下式的多胺的硬化剂的新型芳族多胺组合物：O OOO并行平行并行平行NH2-Ar-CO-R1-OC-Ar'-CO-R1-OC-Ar-NH2n 其中Ar和Ar'是具有1至6个环的二价芳族基团，R 1是二价烃基或基团（R 4 -O）m R 4，R 4是亚烷基，m是1至100的整数。

6. 发明授权

US5036111A Expanded materials with nadimide resin base 失效
标题翻译：膨胀材料与纳迪尔树脂基体
公开(公告)号：US5036111A
公开(公告)日：1991-07-30
申请号：US597666
申请日：1990-10-17
申请人： Michel Senneron , Gilbert Parrain , Guy Rabilloud , Bernard Sillion
发明人： Michel Senneron , Gilbert Parrain , Guy Rabilloud , Bernard Sillion
IPC分类号： C08G65/48 , C08G73/10 , C08J9/02 , C08L67/00 , C08L67/02 , C08L71/12 , C08L77/00 , C08L79/08 , C08L81/00 , C08L81/06
CPC分类号： C08J9/02 , C08G73/101 , C08L79/085 , C08J2379/08
摘要： Expanded material obtained by heating a composition comprising at least onehermosetting nadimide resin, said heating being performed at a temperature and during a period which are sufficient to cause the expansion of said composition by release of cyclopentadiene. A nadimide resin of the polyimide type and having a number average molecular weight of 600 to 10,000 is preferably used. The composition further comprises preferably 1% to 50% by weight of a linear, preferably thermostable polymer.
摘要翻译：通过加热包含至少一种热固性nadimide树脂的组合物获得的膨胀材料，所述加热在足以通过释放环戊二烯而使所述组合物膨胀的温度和时间内进行。优选使用数均分子量为600〜10000的聚酰亚胺型纳米二酰亚胺树脂。组合物还优选包含1重量％至50重量％的线性，优选热稳定性聚合物。

7. 发明授权

US4736015A Aromatic polyimide compositions of high solubility and their uses 失效
标题翻译：高溶解度的芳族聚酰亚胺组合物及其用途
公开(公告)号：US4736015A
公开(公告)日：1988-04-05
申请号：US435153
申请日：1982-10-19
申请人： Guy Rabilloud , Michel Senneron , Choua Cohen , Paul Mariaggi , Bernard Sillion
发明人： Guy Rabilloud , Michel Senneron , Choua Cohen , Paul Mariaggi , Bernard Sillion
IPC分类号： C08L79/08 , C08G73/00 , C08G73/10 , C08G69/26
CPC分类号： C08G73/10
摘要： Aromatic polyimide compositions, useful in particular for manufacturing adhesive materials, varnishes and films withstanding high temperatures, having a high solubility in organic solvents, particularly polar solvents and which are manufactured by reacting, in such a solvent, a tetraester or diacid-diester of benzhydrol 3,3', 4, 4' tetracarboxylic acid with an aromatic diamine for a sufficient time to obtain a polycondensation reaction product having an inherent viscosity at 30.degree. C., at a concentration of 5 g/liter in N-methyl pyrrolidone, ranging from 0.1 to 2 dl/g.
摘要翻译：芳族聚酰亚胺组合物，特别用于制造粘合剂材料，耐高温清漆和薄膜，在有机溶剂特别是极性溶剂中具有高溶解度，并且通过在这种溶剂中使二苯甲酮的四酯或二酸二酯 3,3'，4,4'-四羧酸与芳族二胺反应足够的时间，得到在30℃下的特性粘度，在N-甲基吡咯烷酮中浓度为5g /升的缩聚反应产物，其范围为0.1〜2d / g。

8. 发明授权

US4143077A Diaryloxy-meta-terphenyl derivatives, their manufacture and uses 失效
标题翻译：二异戊二烯衍生物及其制备和用途
公开(公告)号：US4143077A
公开(公告)日：1979-03-06
申请号：US831447
申请日：1977-09-08
申请人： Bernard Masson , Guy Rabilloud , Bernard Sillion
发明人： Bernard Masson , Guy Rabilloud , Bernard Sillion
IPC分类号： C07C17/12 , C07C41/00 , C07C43/263 , C07C67/00 , C10L1/02 , C10M105/18 , C10N40/08 , C07C43/20 , C10M1/20 , C10M3/14
CPC分类号： C10M105/18 , C07C17/12 , C10M2207/04 , C10N2240/08
摘要： New aromatic compounds with ether functions particularly useful as power transmission fluids and as lubricants withstanding high temperatures, containing at least a major proportion of a compound of the formula: ##STR1## WHEREIN EACH Ar is selected from phenyl and metaphenoxy phenyl and optionally a minor proportion of at least one compound selected from those complying with the general formulas: ##STR2## WHEREIN Ar is defined as above.

9. 发明授权

US4045414A New di-substituted meta-terphenyl compounds and resulting polymers 失效
标题翻译：新的二取代的次三联苯化合物和得到的聚合物
公开(公告)号：US4045414A
公开(公告)日：1977-08-30
申请号：US643837
申请日：1975-12-23
申请人： Guy Rabilloud , Bernard Sillion
发明人： Guy Rabilloud , Bernard Sillion
IPC分类号： C07C45/43 , C08G73/06
CPC分类号： C07C45/43 , C07C45/28 , C07C45/46 , C08G73/0694
摘要： New tetracarbonyl compounds of the formulae: ##STR1## where R is a hydrogen atom, an alkyl radical or an aryl radical. The invention also contemplates the thermostable polymers obtained by reacting an aromatic tetra-amine with at least one of the above tetracarbonyl compounds.
摘要翻译：新的具有下式的四羰基化合物：其中R是氢原子，烷基或芳基。本发明还考虑通过使芳族四胺与至少一种上述四羰基化合物反应而获得的热稳定性聚合物。

10. 发明授权

US5104968A Polyimide precursor composition and application therefrom 失效
标题翻译：聚酰亚胺前体组合物及其应用
公开(公告)号：US5104968A
公开(公告)日：1992-04-14
申请号：US564236
申请日：1990-08-08
申请人： Serge Gonzalez , Paul Mariaggi , Guy Rabilloud , Bernard Sillion
发明人： Serge Gonzalez , Paul Mariaggi , Guy Rabilloud , Bernard Sillion
IPC分类号： C08G73/10 , C09D5/25 , H01B3/30
CPC分类号： C08G73/1003 , C08G73/1007 , C08G73/1042 , H01B3/306 , Y10T428/31504
摘要： Polyimide precursor compositions incorporating at least one compound of fula (1), at least one compound of formula (2), at least one compound of formula (3) and at least one compound of formula (4) ##STR1## in which one of the groups R.sup.3 and R.sup.4 represents a hydrogen atom and the other, in the same way as the groups R.sup.1 and R.sup.2, which can be the same or different, in each case represent a hydrocarbon group having 1 to 16 carbon atoms, m is a number between 5 and 20, n is an integer between 1 and 5 and R.sup.5 represents a hydrogen atom, a halogen atom, a hydrocarbon group with 1 to 16 carbon atoms, or a group of formula R.sup.6 --O-- in which R.sup.6 represents a hydrocarbon group having 1 to 16 carbon atoms. The preferred composition contains 30 to 70% by weight of dry matter of compounds of formulas (1), (2) and (3), in which the groups R.sup.1, R.sup.2 and one of the groups R.sup.3 and R.sup.4 is a methyl or ethyl group and the compound of formula (4) is benzyl alcohol. These compositions are usable as smoothing and/or protective coatings for metals, metal alloys or other substrates and in particular in the electrical and electronic industries, e.g. for the formation of dielectric films.
摘要翻译：引入至少一种式（1）化合物，至少一种式（2）化合物，至少一种式（3）化合物和至少一种式（4）化合物的聚酰亚胺前体组合物图像（2）（3）（4）其中R3和R4中的一个代表氢原子，另一个与R1和R2基团相同，可以相同或者不同，在每种情况下都表示具有1至16个碳原子的烃基，m是5至20之间的数，n是1和5之间的整数，R 5表示氢原子，卤素原子，具有1个至16个碳原子的基团，或其中R 6表示具有1至16个碳原子的烃基的式R6-O-基团。优选的组合物包含30至70重量％的式（1），（2）和（3）化合物的干物质，其中基团R 1，R 2和基团R 3和R 4中的一个是甲基或乙基并且式（4）的化合物是苄醇。这些组合物可用作金属，金属合金或其它基材的平滑和/或保护涂层，特别是在电气和电子工业中。用于形成介电膜。

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