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1. 发明授权

US5989704A Integrally molded automotive waterproof connector comprising thermoplastic resin and oil-bleeding silicone rubber 失效
标题翻译：整体模制汽车防水连接器，包括热塑性树脂和出油硅橡胶
公开(公告)号：US5989704A
公开(公告)日：1999-11-23
申请号：US766963
申请日：1996-12-16
申请人： Hiroshi Hashimoto , Masahiro Kanda , Shigeru Muramatsu , Naoto Obayashi , Hironao Fujiki , Shigeki Shudo , Manabu Narumi
发明人： Hiroshi Hashimoto , Masahiro Kanda , Shigeru Muramatsu , Naoto Obayashi , Hironao Fujiki , Shigeki Shudo , Manabu Narumi
IPC分类号： F16L21/02 , B32B25/20 , C08K3/36 , C08K5/54 , C08K5/5419 , C08L67/06 , C08L69/00 , C08L83/05 , C08L83/07 , H01R13/52 , H01R43/18 , B32B5/16 , B32B27/36
CPC分类号： H01R43/18 , C08L67/06 , C08L69/00 , H01R13/5216 , Y10T428/259 , Y10T428/31507 , Y10T428/31667
摘要： An integrally molded automotive waterproof connector is disclosed which comprises a thermoplastic resin and integrated therewith an oil-bleeding silicone rubber, the thermoplastic resin containing a thermoplastic resin oligomer containing at least one aliphatic unsaturated group. In the connector, the adhesion between the thermoplastic resin and the silicone rubber is satisfactory regardless of the length of storage period as compared with connectors comprising a thermoplastic resin and a silicone rubber integrated therewith after priming. Further, the connector of the present invention is excellent in production efficiency and workability, is reduced in connector housing fitting force, and can retain satisfactory waterproofness.
摘要翻译：公开了一种整体模制的汽车防水连接器，其包括热塑性树脂并与其一体的止油硅橡胶，该热塑性树脂含有含有至少一个脂族不饱和基团的热塑性树脂低聚物。在连接器中，热封树脂和硅橡胶之间的粘附性与包含热塑性树脂的连接器和在起动之后与其一体化的硅橡胶相比，与储存周期长度无关，是令人满意的。此外，本发明的连接器的生产效率和加工性优异，连接器壳体配合力降低，能够保持良好的防水性。

2. 发明授权

US5879809A Thermoplastic resin/oil-bleeding silicone rubber integrally molded articles 失效
标题翻译：热塑性树脂/止油硅胶一体成型制品
公开(公告)号：US5879809A
公开(公告)日：1999-03-09
申请号：US760337
申请日：1996-12-04
申请人： Shigeru Muramatsu , Naoto Obayashi , Hironao Fujiki , Shigeki Shudo
发明人： Shigeru Muramatsu , Naoto Obayashi , Hironao Fujiki , Shigeki Shudo
IPC分类号： C08K3/36 , B29C45/16 , B32B25/08 , B32B25/20 , C08K5/5419 , C08L67/00 , C08L69/00 , C08L83/05 , C08L83/07 , C08L101/00 , B32B27/28
CPC分类号： B32B25/20 , B32B25/08 , B29C45/1676 , B29K2083/005 , Y10T428/31507 , Y10T428/31663 , Y10T428/31681 , Y10T428/31692 , Y10T428/31739
摘要： A thermoplastic resin, especially a thermoplastic resin having blended therein a thermoplastic resin oligomer containing an aliphatic unsaturated group is integrally molded with an oil-bleeding silicone rubber, yielding a molded article wherein the resin and the rubber are firmly integrated.
摘要翻译：一种热塑性树脂，特别是其中掺有含有脂肪族不饱和基团的热塑性树脂低聚物的热塑性树脂与排油性硅橡胶一体成型，得到其中树脂和橡胶牢固地结合的成型制品。

3. 发明授权

US5792812A Thermoplastic resin compoistions for use in integral molding with silicone rubber and integrally molded parts 失效
标题翻译：用于与硅橡胶和整体模制零件一体成型的热塑性树脂组合物
公开(公告)号：US5792812A
公开(公告)日：1998-08-11
申请号：US579627
申请日：1995-12-26
申请人： Hironao Fujiki , Shigeki Shudo
发明人： Hironao Fujiki , Shigeki Shudo
IPC分类号： B29C45/16 , C08J5/12 , C08L69/00 , C08L83/04 , C08L83/07 , C08L101/00 , C08L23/16 , C08L25/10 , C08L55/02
CPC分类号： C08L69/00 , B29C45/1676 , C08J5/12 , C08L101/00 , B29K2083/005 , B29K2283/00 , C08L83/04 , Y10T428/31507 , Y10T428/31663 , Y10T428/31667
摘要： A thermoplastic resin composition comprising 100 parts by weight of a thermoplastic resin and 2 to 12 parts by weight of a thermoplastic resin oligomer containing 0.1 to 35% by weight of an aliphatic unsaturated group is molded with silicone rubber to form an integrally molded part. The thermoplastic resin composition maintains the inherent properties of the thermoplastic resin and firmly bonds with silicone rubber.
摘要翻译：将含有100重量份热塑性树脂和2〜12重量份含有0.1〜35重量％脂肪族不饱和基团的热塑性树脂低聚物的热塑性树脂组合物用硅橡胶成型，形成整体成型体。热塑性树脂组合物保持热塑性树脂的固有性质并与硅橡胶牢固结合。

4. 发明授权

US5616632A Silicone compositions 失效
标题翻译：有机硅组合物
公开(公告)号：US5616632A
公开(公告)日：1997-04-01
申请号：US560586
申请日：1995-11-20
申请人： Hironao Fujiki , Shigeki Shudo , Takashi Kondou
发明人： Hironao Fujiki , Shigeki Shudo , Takashi Kondou
IPC分类号： C08K9/10 , C08L83/04
CPC分类号： C08K9/10 , C08L83/04 , C08G77/12 , C08G77/20 , C08G77/24 , C08G77/70
摘要： In a silicone composition comprising an aliphatic unsaturated group-containing diorganopolysiloxane and an organohydrogenpolysiloxane, there is blended a hydrosilylation catalyst. The catalyst is obtained by stabilizing a platinum group compound with an organopolysiloxane of formula (3):R.sup.4.sub.f R.sup.5.sub.g (CH.sub.3).sub.h SiO.sub.(4-f-g-h)/2 (3)wherein R.sup.4 is a C.sub.2-8 aliphatic unsaturated group, R.sup.5 is a monovalent hydrocarbon group excluding an aliphatic unsaturated group and methyl group, letters f, g, and h are (f+g)/(f+g+h).gtoreq.0.10, 0.0001
摘要翻译：在包含含脂族不饱和基团的二有机聚硅氧烷和有机氢聚硅氧烷的硅氧烷组合物中，混合氢化硅烷化催化剂。通过用式（3）的有机聚硅氧烷稳定铂族化合物得到催化剂：R4fR5g（CH3）hSiO（4-fgh）/ 2（3）其中R4是C2-8脂族不饱和基团，R5是一价烃不包括脂族不饱和基团和甲基的基团，字母f，g和h分别为（f + g）/（f + g + h）> / = 0.10,0.0001

5. 发明授权

US5536803A Adhesive silicone compositions 失效
标题翻译：粘合硅胶组合物
公开(公告)号：US5536803A
公开(公告)日：1996-07-16
申请号：US461012
申请日：1995-06-05
申请人： Hironao Fujiki , Shigeki Shudo , Toshiaki Takahashi , Hiroyasu Hara , Takeshi Miyao
发明人： Hironao Fujiki , Shigeki Shudo , Toshiaki Takahashi , Hiroyasu Hara , Takeshi Miyao
IPC分类号： C08L83/07 , C09J183/04 , C09J183/07 , C08G77/08
CPC分类号： C09J183/04
摘要： An adhesive silicone composition comprising a diorganopolysiloxane, an organohydrogenpolysiloxane, and a platinum catalyst is blended with an organohydrogenpolysiloxane having at least two hydrogen atoms each bonded to a silicon atom in a molecule and containing an aromatic ring-bearing hydrocarbon radical in an amount of at least 12 mol % of the entire monovalent organic radicals bonded to silicon atoms, or a compound containing at least one hydrogen atom bonded to a silicon atom in a molecule and having a radical of two benzene rings separated by --R.sup.13 R.sup.14 Si--, --R.sup.13 R.sup.14 SiO--, --OR.sup.13 R.sup.14 SiO-- or --R.sup.13 R.sup.14 SiOR.sup.13 R.sup.14 Si-- wherein R.sup.13 and R.sup.14 are a monovalent hydrocarbon radical. The composition firmly adheres to organic resins, but is readily releasable from metal molds.
摘要翻译：将包含二有机聚硅氧烷，有机氢聚硅氧烷和铂催化剂的粘合性有机硅组合物与具有至少两个氢原子的有机氢聚硅氧烷共混，每个氢原子分子键合至硅原子并且含有至少含有芳环的烃基与硅原子键合的全部一价有机基团的12摩尔％，或分子中含有与硅原子键合的至少一个氢原子的化合物，其具有由-R 13 R 14 -Si，-R 13 R 14 SiO， - OR13R14SiO-或-R13R14SiOR13R14Si-，其中R13和R14是一价烃基。组合物牢固地粘附到有机树脂上，但是容易从金属模具中剥离。

6. 发明授权

US5418065A Integrally molded article of silicone rubber and modified polypropylene resin 失效
标题翻译：硅橡胶和改性聚丙烯树脂的整体成型制品
公开(公告)号：US5418065A
公开(公告)日：1995-05-23
申请号：US163553
申请日：1993-12-09
申请人： Hironao Fujiki , Shigeki Shudo , Akira Matsuda , Yasushi Yamamoto , Noboru Shimamoto , Eiji Kuchiki , Yuji Fujita
发明人： Hironao Fujiki , Shigeki Shudo , Akira Matsuda , Yasushi Yamamoto , Noboru Shimamoto , Eiji Kuchiki , Yuji Fujita
IPC分类号： B29C45/16 , B32B37/00 , C08J5/12 , B32B7/04 , B32B25/20 , B32B27/32
CPC分类号： C08J5/12 , B29C45/1676 , B29K2023/12 , B29K2083/00 , B29K2083/005 , B29K2283/00 , B29L2009/00 , Y10T428/31663 , Y10T428/31667
摘要： In a polypropylene resin/silicone rubber integrally molded article, a polypropylene resin having an aliphatic unsaturated bond is integrally joined to an addition type silicone rubber at high bond strength. It is prepared by injection molding a modified polypropylene resin into a preform, injection molding a silicone rubber composition over the preform, and curing the composition at a temperature below the softening point of the polypropylene resin. Stronger bond is established when the silicone rubber contains a tackifier in the form of a compound containing in a molecule at least one hydrogen atom directly attached to a silicon atom and an alkoxysilyl, glycidyl or acid anhydride group or a --(CH.sub.2).sub.n -- linkage.
摘要翻译：在聚丙烯树脂/硅橡胶一体成型体中，具有脂肪族不饱和键的聚丙烯树脂以高粘合强度与加成型硅橡胶一体地接合。通过将改性聚丙烯树脂注塑成预成型体，在预成型体上注射成型硅橡胶组合物，并在低于聚丙烯树脂的软化点的温度下固化该组合物来制备。当硅橡胶含有在分子中含有至少一个直接连接到硅原子上的氢原子和烷氧基甲硅烷基，缩水甘油基或酸酐基团或 - （CH2）n-键的化合物形式的增粘剂时，形成更强的键。

7. 发明授权

US5366806A Integrated thermoplastic resin/silicone rubber articles and method for making 失效
标题翻译：综合热塑性树脂/硅橡胶制品及其制造方法
公开(公告)号：US5366806A
公开(公告)日：1994-11-22
申请号：US965303
申请日：1992-10-23
申请人： Hironao Fujiki , Shigeki Shudo
发明人： Hironao Fujiki , Shigeki Shudo
IPC分类号： B32B25/08 , B29C43/00 , B32B25/20 , B32B37/00 , B32B37/06 , C08F291/00 , C08J5/12 , B29C43/20 , B29K19/00
CPC分类号： C08J5/12 , C08F291/00 , B29C43/00 , B29K2023/00 , B29K2027/12 , B29K2069/00 , B29K2077/00 , B29K2083/00 , B29K2096/02 , Y10T428/31507 , Y10T428/3154 , Y10T428/31598 , Y10T428/31663 , Y10T428/31667
摘要： An integrated thermoplastic resin/silicone rubber article is prepared by modifying a thermoplastic resin with a silicon-containing compound in monomer or polymer form, molding the thermoplastic resin into a shape, contacting an uncured silicone rubber with the molded thermoplastic resin, and curing the silicone rubber at a temperature below the softening point of the thermoplastic resin. The article in which the thermoplastic resin is firmly united with the silicone rubber is useful in electric, electronic and automotive applications while taking advantage of the inherent reliability in heat resistance, weather resistance and electrical properties of the silicone rubber.
摘要翻译：通过用单体或聚合物形式的含硅化合物改性热塑性树脂来制备整体热塑性树脂/硅橡胶制品，将热塑性树脂模塑成形状，使未固化的硅橡胶与模制的热塑性树脂接触，并固化硅树脂橡胶的温度低于热塑性树脂的软化点。其中热塑性树脂与硅橡胶牢固结合的制品可用于电气，电子和汽车应用中，同时利用硅橡胶的耐热性，耐候性和电性能的固有可靠性。

8. 发明授权

US5366805A Polycarbonate resin/silicone rubber integrally molded article and method for making 失效
标题翻译：聚碳酸酯树脂/硅橡胶一体成形品及其制造方法
公开(公告)号：US5366805A
公开(公告)日：1994-11-22
申请号：US163543
申请日：1993-12-09
申请人： Hironao Fujiki , Shigeki Shudo , Akira Matsuda , Noriyoshi Ogawa , Toshiaki Takata
发明人： Hironao Fujiki , Shigeki Shudo , Akira Matsuda , Noriyoshi Ogawa , Toshiaki Takata
IPC分类号： B29C45/14 , B29C45/16 , B29K83/00 , B32B25/20 , B32B27/36 , B32B37/00 , C08J5/12 , C08L83/04 , C09J183/00 , C09J183/07 , B32B27/28 , B29K69/00
CPC分类号： C08J5/12 , B29C45/1676 , C08L83/04 , B29K2069/00 , B29K2083/00 , B29K2083/005 , B29K2283/00 , B29L2009/00 , C08G77/12 , C08G77/20 , C08G77/70 , Y10T428/31507
摘要： In a polycarbonate resin/silicone rubber integrally molded article, a polycarbonate resin having an aliphatic unsaturated group, typically an isopropenyl group is integrally joined to an addition type silicone rubber containing a tackifier component at high bond strength. It is prepared by injection molding a modified polycarbonate resin into a preform, injection molding a silicone rubber composition over the preform, and curing the composition at a temperature below the softening point of the polycarbonate resin.
摘要翻译：在聚碳酸酯树脂/硅橡胶一体成型体中，具有脂肪族不饱和基团（通常为异丙烯基）的聚碳酸酯树脂与含有高粘合强度的增粘剂成分的添加型硅橡胶一体地接合。通过将改性聚碳酸酯树脂注塑成预成型体，在预成型体上注射成型硅橡胶组合物，并在低于聚碳酸酯树脂的软化点的温度下固化该组合物来制备。

9. 发明授权

US5405896A Adhesive silicone rubber compositions 失效
标题翻译：粘合硅橡胶组合物
公开(公告)号：US5405896A
公开(公告)日：1995-04-11
申请号：US163556
申请日：1993-12-09
申请人： Hironao Fujiki , Shigeki Shudo , Akira Matsuda
发明人： Hironao Fujiki , Shigeki Shudo , Akira Matsuda
IPC分类号： C07F7/08 , C07F7/21 , C08K5/5419 , C08L83/04 , C08L83/07 , C09J183/00 , C09J183/04 , C09J183/07 , C08K5/24 , C08F8/00 , C08G77/06 , C08L83/00
CPC分类号： C08L83/04 , C07F7/0896 , C07F7/21 , C08K5/5419 , C08G77/12 , C08G77/20 , C08G77/70
摘要： An adhesive silicone rubber composition of addition reaction curing type comprising (a) an organopolysiloxane containing an alkenyl group; (b) an organohydrogenpolysiloxane having at least one hydrogen atom directly attached to a silicon atom in a molecule; (c) an addition reaction catalyst; and (d) an adhesive agent selected from compounds of the following formulae (I), (II) and (III):A-(D-B).sub.x -D-A (I)C-(B-D).sub.x -B-C (II)A-E (III)wherein each of A and B is a silane or siloxane group, each group having at least one hydrogen atom directly attached to a silicon atom and an optional substituent which is a substituted or unsubstituted monovalent hydrocarbon group having 1 to 8 carbon atoms attached to the same or different silicon atom, A being monovalent and B being divalent,each of C and D is a group having contained therein at least one member selected from the group consisting of a substituted or unsubstituted aryl group, a substituted or unsubstituted arylene group, ##STR1## and an optional substituent which is selected from alkyl or alkylene groups, C being monovalent and D being divalent,E is a monovalent group as defined for C, with the proviso that the total number of atoms in E other than hydrogen and halogen atoms is at least 8, andletter x is 0 or a positive number,said adhesive silicone rubber composition giving a cured product that does not adhere to metal.
摘要翻译：一种加成反应固化型粘合性硅橡胶组合物，其包含（a）含有烯基的有机聚硅氧烷; （b）具有至少一个氢原子的有机氢聚硅氧烷，其直接连接到分子中的硅原子上; （c）加成反应催化剂; 和（d）选自下式（I），（II）和（III）的化合物的粘合剂：A-（DB）xDA（I）C-（BD）xBC（II）AE（III）的A和B是硅烷或硅氧烷基团，每个基团具有至少一个与硅原子直接相连的氢原子和任选的取代基，其是具有1-8个碳原子的取代或未取代的一价烃基彼此相连或不同硅原子，A为一价，B为二价，C和D各自为含有至少一个选自取代或未取代的芳基，取代或未取代的亚芳基，取代或未取代的亚芳基，和选自烷基或亚烷基的任选的取代基，C为一价，D为二价，E为C定义的一价基团，条件是除氢和卤素原子以外的E中的原子总数至少为 8，字母x为0或正数，所述粘合性硅橡胶组合物产生不粘附到金属上的固化产物。

10. 发明授权

US08158738B2 Adhesive silicone rubber composition and separator seal material for fuel cells 有权
标题翻译：用于燃料电池的胶粘硅橡胶组合物和隔板密封材料
公开(公告)号：US08158738B2
公开(公告)日：2012-04-17
申请号：US12599421
申请日：2008-06-20
申请人： Chisato Kato , Kazutaka Iizuka , Osamu Hayashida , Takashi Aketa , Shigeki Shudo
发明人： Chisato Kato , Kazutaka Iizuka , Osamu Hayashida , Takashi Aketa , Shigeki Shudo
IPC分类号： C08G77/08
CPC分类号： H01M8/0284 , C08G77/12 , C08G77/20 , C08K3/10 , C08K5/5435 , C08L83/00 , C09J183/04 , H01M8/0271 , H01M8/0297 , H01M2008/1095
摘要： An adhesive silicone rubber composition comprising (A) 100 pbw of an organopolysiloxane containing at least two silicon-bonded alkenyl radicals, (B) 0.5-20 pbw of an organohydrogenpolysiloxane containing at least two Si—H radicals, (C) a hydrosilylation catalyst, and (D) 0.1-50 pbw of an organosilicon compound having at least one phenyl structure, at least one alicyclic epoxy radical, and at least one Si—H radical is applicable to an electrolyte membrane and a separator in a polymer electrolyte fuel cell to form a firm integrally molded part.
摘要翻译：一种粘合性硅橡胶组合物，其包含（A）100pbw的含有至少两个与硅键合的烯基的有机聚硅氧烷，（B）0.5-20pbw的含有至少两个Si-H基团的有机氢聚硅氧烷，（C）氢化硅烷化催化剂，和（D）0.1-50pbw的具有至少一个苯基结构的有机硅化合物，至少一个脂环族环氧基和至少一个Si-H基团可应用于聚合物电解质燃料电池中的电解质膜和隔膜，形成牢固的整体模制件。

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