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1. 发明授权

US4620868A N-[(4,6-dimethoxypyrimidin-2-yl)aminocarbonyl]-3[halo-substituted ethenyl (or propenyl)]-2-thiophenesulfonamides useful as herbicides 失效
标题翻译： N - [（4,6-二甲氧基嘧啶-2-基）氨基羰基] -3 [卤代取代的乙烯基（或丙烯基）] - 2-噻吩磺酰胺可用作除草剂
公开(公告)号：US4620868A
公开(公告)日：1986-11-04
申请号：US683219
申请日：1984-12-18
申请人： Fumio Kimura , Takahiro Haga , Kazuyuki Maeda , Kouji Hayashi , Toshio Seki , Tsunezo Yoshida
发明人： Fumio Kimura , Takahiro Haga , Kazuyuki Maeda , Kouji Hayashi , Toshio Seki , Tsunezo Yoshida
IPC分类号： A01N47/36 , C07D521/00 , A01N43/02 , C07D239/02
CPC分类号： C07D521/00 , A01N47/36
摘要： Novel substituted thiophenesulfonamide compounds useful as herbicides which are represented by the following formula, and salts thereof: ##STR1## wherein either one of X and Y is an ethenyl or propenyl group having all hydrogen atoms replaced by chlorine atoms and/or fluorine atoms, and the other is the group ##STR2## (wherein R.sub.1 and R.sub.2 are each a methyl or methoxy group, and A is .dbd.N-- or .dbd.CH--).
摘要翻译：用作下式表示的除草剂的新型取代的噻吩磺酰胺化合物及其盐：其中X和Y中的任一个是具有被氯原子和/或氟原子取代的全部氢原子的乙烯基或丙烯基，另一组是（其中R1和R2各自为甲基或甲氧基，A为= N-或= CH-）。

2. 发明授权

US4744814A N-[(4,6-dimetho xypyrimidin-2-yl)aminocarbonyl]-3-trifluoromethylpyridine-2-sulfonamide or salts thereof, herbicidal composition containing the same 失效
标题翻译： N - [（4,6-二甲氧基嘧啶-2-基）氨基羰基] -3-三氟甲基吡啶-2-磺酰胺或其盐，含有它们的除草组合物
公开(公告)号：US4744814A
公开(公告)日：1988-05-17
申请号：US802279
申请日：1985-11-27
申请人： Fumio Kimura , Takahiro Haga , Nobuyuki Sakashita , Chimoto Honda , Kouji Hayashi , Toshio Seki , Kouji Minamida
发明人： Fumio Kimura , Takahiro Haga , Nobuyuki Sakashita , Chimoto Honda , Kouji Hayashi , Toshio Seki , Kouji Minamida
IPC分类号： C07D401/12 , A01N43/54 , A01N47/36 , C07D213/71 , C07D521/00
CPC分类号： C07D521/00 , A01N47/36 , C07D213/71
摘要： N-[(4,6-Dimethoxypyrimidin-2-yl)aminocarbonyl]-3-trifluoromethylpyridine-2-sulfonamide or a salt thereof is disclosed. The compound of the invention is useful as a herbicide which has an extremely high herbicidal effect against a wide variety of weeds including strongly noxious weeds but which shows a high safety against tomato and turfs. A process for the production of N-[(4,6-dimethoxypyrimidin-2-yl)aminocarbonyl]-3-trifluoromethylpyridine-2-sulfonamide is also disclosed.
摘要翻译：公开了N - [（4,6-二甲氧基嘧啶-2-基）氨基羰基] -3-三氟甲基吡啶-2-磺酰胺或其盐。本发明的化合物可用作除草剂，其对多种杂草具有极高的除草效果，包括强烈的有害杂草，但对番茄和草皮显示出高的安全性。还公开了制备N - [（4,6-二甲氧基嘧啶-2-基）氨基羰基] -3-三氟甲基吡啶-2-磺酰胺的方法。

3. 发明授权

US08481981B2 Method of smoothing solid surface with gas cluster ion beam and solid surface smoothing apparatus 有权
标题翻译：用气体团簇离子束和固体表面平滑装置平滑固体表面的方法
公开(公告)号：US08481981B2
公开(公告)日：2013-07-09
申请号：US12312203
申请日：2007-10-30
申请人： Akiko Suzuki , Akinobu Sato , Emmanuel Bourelle , Jiro Matsuo , Toshio Seki
发明人： Akiko Suzuki , Akinobu Sato , Emmanuel Bourelle , Jiro Matsuo , Toshio Seki
IPC分类号： G21K5/04
CPC分类号： H01L21/3065 , H01J2237/0812 , H01J2237/202 , H01J2237/3151
摘要： Surface roughness having intervals of several tens of nanometers to about a hundred micrometers in a solid surface is reduced by directing a gas cluster ion beam to the surface. An angle formed between the normal to the solid surface and the gas cluster ion beam is referred to as an irradiation angle, and an irradiation angle at which the distance of interaction between the solid and the cluster colliding with the solid dramatically increases is referred to as a critical angle. A solid surface smoothing method includes an irradiation step of directing the gas cluster ion beam onto the solid surface at an irradiation angle not smaller than the critical angle. The critical angle is 70°.
摘要翻译：通过将气体团簇离子束引导到表面，在固体表面中具有数十纳米至约百微米间隔的表面粗糙度被减小。被称为固体表面和气体团簇离子束的法线之间的角度被称为照射角度，并且固体和团簇与固体之间的相互作用距离急剧增加的照射角度被称为一个临界角。固体表面平滑化方法包括将气体团簇离子束以不小于临界角的照射角度引导到固体表面的照射步骤。临界角为70°。

4. 发明申请

US20090305507A1 Method of processing solid surface with gas cluster ion beam 有权
标题翻译：用气体簇离子束处理固体表面的方法
公开(公告)号：US20090305507A1
公开(公告)日：2009-12-10
申请号：US12312266
申请日：2007-10-30
申请人： Akiko Suzuki , Akinobu Sato , Emmanuel Bourelle , Jiro Matsuo , Toshio Seki
发明人： Akiko Suzuki , Akinobu Sato , Emmanuel Bourelle , Jiro Matsuo , Toshio Seki
IPC分类号： H01L21/308 , H01L21/302
CPC分类号： H01L21/3083 , H01J2237/0812 , H01L21/3065
摘要： A solid surface is processed while corner portions of a relief structure are protected from deformation. A method of processing a solid surface with a gas cluster ion beam includes a cluster protection layer formation step of forming, on the solid surface, a relief structure having protrusions with a cluster protection layer formed to cover an upper part thereof and recesses without the cluster protection layer; an irradiation step of emitting a gas cluster ion beam onto the solid surface having the relief structure formed in the cluster protection layer formation step; and a removal step of removing the cluster protection layer. A thickness T of the cluster protection layer satisfies T > nY + ( b 2  Y 2  n - nY 2  ( b 4 - 16  a 2 ) 1 2 2 ) 1 2 , where n is a dose of the gas cluster ion beam, and Y is an etching efficiency of the cluster protection layer, expressed as an etching volume per cluster (a and b are constants).
摘要翻译：处理浮雕结构的角部以防止变形的实心表面。用气体簇离子束处理固体表面的方法包括：簇保护层形成步骤，在固体表面上形成具有突起的浮雕结构，所述突起具有形成为覆盖其上部的簇保护层和没有簇的凹部保护层; 在所述簇保护层形成工序中形成有具有所述浮雕结构的固体表面上的气体簇离子束的照射工序; 以及去除簇保护层的去除步骤。簇保护层的厚度T满足T> nY +（b 2 y 2 n n n 2（b 4 - 16 a a 2）1 2 2）1 2，其中n是气体簇的剂量离子束，Y是簇保护层的蚀刻效率，表示为每簇的蚀刻体积（a和b是常数）。

5. 发明申请

US20100096263A1 Solid surface smoothing apparatus 审中-公开
标题翻译：固体表面平滑装置
公开(公告)号：US20100096263A1
公开(公告)日：2010-04-22
申请号：US12642633
申请日：2009-12-18
申请人： Akinobu Sato , Akiko Suzuki , Emmanuel Bourelle , Jiro Matsuo , Toshio Seki , Takaaki Aoki
发明人： Akinobu Sato , Akiko Suzuki , Emmanuel Bourelle , Jiro Matsuo , Toshio Seki , Takaaki Aoki
IPC分类号： C23C14/34
CPC分类号： H01J37/08 , C23F4/00 , H01J2237/0812 , H01J2237/3151 , H01L21/302 , H01L21/3105 , H01L21/321
摘要： In a method of irradiating a gas cluster ion beam on a solid surface and smoothing the solid surface, the angle formed between the solid surface and the gas cluster ion beam is chosen to be between 1° and an angle less than 30°. In case the solid surface is relatively rough, the processing efficiency is raised by first irradiating a beam at an irradiation angle θ chosen to be something like 90° as a first step, and subsequently at an irradiation angle θ chosen to be 1° to less than 30° as a second step. Alternatively, the set of the aforementioned first step and second step is repeated several times.
摘要翻译：在固体表面上照射气体团簇离子束并平滑固体表面的方法中，将固体表面和气体团簇离子束之间形成的角度选择在1°和小于30°的角度之间。在固体表面比较粗糙的情况下，通过首先以照射角照射光束来提高加工效率; 选择作为第一步的90°，随后在照射角度＆amp; 选择为1°至小于30°作为第二步。或者，将上述第一步骤和第二步骤的组合重复多次。

6. 发明授权

US07405394B2 Gas cluster-ion irradiation apparatus 失效
标题翻译：气体簇离子照射装置
公开(公告)号：US07405394B2
公开(公告)日：2008-07-29
申请号：US11173023
申请日：2005-07-05
申请人： Shigeru Ono , Shinji Sasaki , Kenji Furusawa , Jiro Matsuo , Toshio Seki
发明人： Shigeru Ono , Shinji Sasaki , Kenji Furusawa , Jiro Matsuo , Toshio Seki
IPC分类号： B01D59/44
CPC分类号： H01J37/3053 , H01J2237/04756 , H01J2237/0812 , H01J2237/304
摘要： In a cluster ion beam irradiation apparatus including an apparatus for measuring size and energy distribution of gas cluster ions by using the time of flight (TOF) mass spectrometry, a unit for applying a retarding voltage is disposed in a stage preceding a TOF measuring instrument including a drift tube and a current measuring instrument. By measuring the size and energy distribution of the gas cluster ions and adjusting ionization conditions, cluster ions having predetermined energy and size are supplied to a work surface. In addition, a product of a pressure in an ion transportation device and an ion transportation length is controlled so as to satisfy the relation P×L≦30/N2/3/E1/2 Pa·m, where N is the size of gas cluster ions used for irradiation, and E is kinetic energy (eV) of the gas cluster ions.
摘要翻译：在包括用于通过使用飞行时间（TOF）质谱法测量气体簇离子的尺寸和能量分布的装置的集束离子束照射装置中，在TOF测量仪器之前的阶段中设置用于施加延迟电压的单元，包括漂移管和电流测量仪器。通过测量气体团簇离子的尺寸和能量分布并调节电离条件，将具有预定能量和尺寸的簇离子供应到工作表面。此外，控制离子输送装置中的压力和离子输送长度的乘积，以满足关系式PxL <= 30 / N 2/3 / E 1/2 Pa.m，其中N是用于照射的气体簇离子的大小，E是气体簇离子的动能（eV）。

7. 发明授权

US4997834A Trans-4-amino(alkyl)-1-pyridylcarbamoylcyclohexane compounds and pharmaceutical use thereof 失效
标题翻译：反式-4-氨基（烷基）-1-吡啶基氨基甲酰基环己烷化合物及其药物用途
公开(公告)号：US4997834A
公开(公告)日：1991-03-05
申请号：US440374
申请日：1989-11-22
申请人： Tomio Muro , Toshio Seki , Masao Abe , Jun Inui , Hiroyuki Sato
发明人： Tomio Muro , Toshio Seki , Masao Abe , Jun Inui , Hiroyuki Sato
IPC分类号： C07D213/75 , C07D213/82 , C07D213/89 , C07D401/12
CPC分类号： C07D213/75 , C07D213/82 , C07D213/89 , C07D401/12
摘要： A trans-4-amino(alkyl)-1-pyridylcarbamoylcyclohexane compound of the formula: ##STR1## wherein R.sup.1 and R.sup.2 are the same or different, and respectively represent hydrogen, C.sub.1-10 alkyl, C.sub.2-5 alkanoyl, formyl, C.sub.1-4 alkoxy-carbonyl, amidino, C.sub.3-7 cycloalkyl, C.sub.3-7 cycloalkylcarbonyl, phenyl, phenylalkyl, benzoyl, naphthoyl, phenylalkoxycarbonyl, benzylidene, pyridylcarbonyl, piperidyl, pyrrolidylidene or piperidylidene which may be optionally substituted on the ring or R.sup.1 and R.sup.2 together with the adjacent nitrogen atom form 5 to 6-membered cycle which may have oxygen atom, sulfur atom or optionally substituted nitrogen atom in the cycle, or together with the adjacent nitrogen atom form phthalimido, R.sup.3 represents hydrogen or C.sub.1-4 alkyl, R.sup.4 represents hydrogen or C.sub.1-4 alkyl, R.sup.5 represents hydrogen, hydroxy, C.sub.1-4 alkyl or phenylalkoxy. R.sup.6 represents hydrogen or C.sub.1-4 alkyl, A represents single bond, C.sub.1-5 straight chain alkylene, or alkylene which is substituted by C.sub.1-4 alkyl, n represents 0 to 1, an optical isomer thereof and a pharmaceutically acceptable acid addition salt thereof.These compounds possess antihypertensive activity, and coronary, cerebral and kidney circulation-improving activities and are useful as antihypertensive agents and agents for prevention and treatment of circulatory diseases.

8. 发明申请

US20100207041A1 Method of Smoothing Solid Surface with Gas Cluster Ion Beam and Solid Surface Smoothing Apparatus 审中-公开
标题翻译：用气体簇离子束和固体表面平滑装置平滑固体表面的方法
公开(公告)号：US20100207041A1
公开(公告)日：2010-08-19
申请号：US12312265
申请日：2007-10-30
申请人： Akinobu Sato , Akiko Suzuki , Emmanuel Bourelle , Jiro Matsuo , Toshio Seki
发明人： Akinobu Sato , Akiko Suzuki , Emmanuel Bourelle , Jiro Matsuo , Toshio Seki
IPC分类号： H01J37/30
CPC分类号： C23F4/00 , H01J27/026 , H01J37/20 , H01J37/3053 , H01J37/317 , H01J2237/20207 , H01J2237/20214 , H01L21/3065
摘要： Scratches or similar surface roughness in a solid surface is reduced by gas cluster ion beam irradiation. A method of smoothing a solid surface with a gas cluster ion beam includes an irradiation step in which the solid surface is irradiated with a gas cluster ion beam, and the irradiation step includes a process of causing clusters from a plurality of directions to collide with at least an area (spot) irradiated with the gas cluster ion beam on the solid surface. Collision of the clusters from a plurality of directions with the spot is brought about by an irradiation of the gas cluster ion beam in which flight directions of the clusters diverge with respect to a center of the beam, for example.
摘要翻译：通过气体簇离子束照射减少了固体表面中的划痕或类似的表面粗糙度。利用气体簇离子束平滑固体表面的方法包括其中固体表面被气体团簇离子束照射的照射步骤，并且照射步骤包括使来自多个方向的团簇与至少在固体表面上用气体团簇离子束照射的面积（斑点）。例如，聚簇从多个方向与斑点的碰撞是通过其中簇的飞行方向相对于束的中心发散的气体团簇离子束的照射引起的。

9. 发明申请

US20060278611A1 Method and device for flattening surface of solid 有权
标题翻译：固体表面平整的方法和装置
公开(公告)号：US20060278611A1
公开(公告)日：2006-12-14
申请号：US10573942
申请日：2004-09-29
申请人： Akinobu Sato , Akiko Suzuki , Emmanuel Bourelle , Jiro Matsuo , Toshio Seki , Takaaki Aoki
发明人： Akinobu Sato , Akiko Suzuki , Emmanuel Bourelle , Jiro Matsuo , Toshio Seki , Takaaki Aoki
IPC分类号： C23F1/00 , C03C15/00
CPC分类号： H01J37/3244 , C23F4/00 , H01J37/08 , H01J37/3053 , H01J2237/0812 , H01J2237/3151
摘要： In a method of irradiating a gas cluster ion beam on a solid surface and smoothing the solid surface, the angle formed between the solid surface and the gas cluster ion beam is chosen to be between 1° and an angle less than 30°. In case the solid surface is relatively rough, the processing efficiency is raised by first irradiating a beam at an irradiation angle θ chosen to be something like 90° as a first step, and subsequently at an irradiation angle θ chosen to be 1° to less than 30° as a second step. Alternatively, the set of the aforementioned first step and second step is repeated several times.
摘要翻译：在固体表面上照射气体团簇离子束并平滑固体表面的方法中，将固体表面和气体团簇离子束之间形成的角度选择在1°和小于30°的角度之间。在固体表面相对粗糙的情况下，通过首先以选择为90°的照射角度θ照射光束来提高加工效率，作为第一步骤，然后以选择为1°以下的照射角度θ 超过30°作为第二步。或者，将上述第一步骤和第二步骤的组合重复多次。

10. 发明授权

US5318969A Benzopyran compound and its pharmaceutical use 失效
标题翻译：苯并吡喃化合物及其药物用途
公开(公告)号：US5318969A
公开(公告)日：1994-06-07
申请号：US897253
申请日：1992-06-11
申请人： Tsutomu Yamanaka , Toshio Seki , Tohru Nakajima , Osamu Yaoka
发明人： Tsutomu Yamanaka , Toshio Seki , Tohru Nakajima , Osamu Yaoka
IPC分类号： C07D311/68 , A61K31/35 , A61K31/352 , A61K31/443 , A61K31/4433 , A61K31/455 , A61K31/50 , A61K31/535 , A61P9/08 , A61P9/10 , A61P9/12 , A61P25/02 , C07D311/70 , C07D311/96 , C07D405/04 , C07D405/12 , C07D407/12 , C07D409/12
CPC分类号： C07D405/12 , C07D311/68 , C07D407/12
摘要： A benzopyran compound of the general formula (I) ##STR1## wherein A represents --OR.sup.1 or --NH--COR.sup.2 ; R.sup.3 represents hydrogen, a lower alkyl, a lower alkoxy, amino, a mono- or di-lower alkylamino, an amino-lower alkyl, a hydroxy-lower alkyl, a halo-lower alkyl, a lower alkoxy-lower alkyl, an acyloxy-lower alkyl, a lower alkoxycarbonyl-lower alkyl, an aryl or a heteroaryl, or R.sup.2 and R.sup.3 combinedly together form an alkylene having 1 to 2 carbon atoms; R.sup.4 and R.sup.5 are the same or different, and respectively represent hydrogen or a lower alkyl, or combinedly together form an alkylene having 2 to 5 carbon atoms; R.sup.6 represents hydroxyl group, formyloxy, an alkanoyloxy, a haloalkanoyloxy, a lower alkoxycarbonyloxy, an aroyloxy, a heteroaroyloxy, carbamoyloxy, a mono- or di-lower alkylcarbamoyloxy and R.sup.7 represents hydrogen, or R.sup.6 and R.sup.7 combinedly together form a bond and X and Y are the same or different, and respectively represent hydrogen, halogen, nitro, cyano, a lower alkyl, a lower alkoxy, a halo-lower alkyl, carboxyl, formyl, an alkanoyl, an aroyl, a halo-alkanoyl, carbamoyl, a lower alkylsulfinyl, an arylsulfinyl, a lower alkylsulfonyl, an arylsulfonyl, sulfonamido or a mono- or di-lower alkylsulfonamido, or their pharmaceutically acceptable salts and its pharmaceutical use.
摘要翻译：通式（I）的苯并吡喃化合物其中A表示-OR1或-NH-COR2; R 3表示氢，低级烷基，低级烷氧基，氨基，一或二低级烷基氨基，氨基 - 低级烷基，羟基 - 低级烷基，卤代低级烷基，低级烷氧基 - 低级烷基，酰氧基低级烷基，低级烷氧基羰基 - 低级烷基，芳基或杂芳基，或R2和R3组合在一起形成具有1至2个碳原子的亚烷基; R4和R5相同或不同，分别表示氢或低级烷基，或者组合在一起形成具有2-5个碳原子的亚烷基; R6表示羟基，甲酰氧基，烷酰氧基，卤代烷酰氧基，低级烷氧基羰氧基，芳酰氧基，杂芳氧基，氨基甲酰氧基，一或二低级烷基氨基甲酰氧基，R7表示氢，或R6和R7组合在一起形成键，X和 Y分别相同或不同，分别表示氢，卤素，硝基，氰基，低级烷基，低级烷氧基，卤代低级烷基，羧基，甲酰基，烷酰基，芳酰基，卤代烷酰基，氨基甲酰基，低级烷基亚磺酰基，芳基亚磺酰基，低级烷基磺酰基，芳基磺酰基，亚磺酰氨基或单 - 或二 - 低级烷基亚磺酰氨基，或其药学上可接受的盐及其药物用途。

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