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1. 发明授权

US06218334B1 Catalysts which can be used in conversion reactions of hydrocarbons and containing silicon 失效
标题翻译：可用于烃和含硅转化反应的催化剂
公开(公告)号：US06218334B1
公开(公告)日：2001-04-17
申请号：US08973407
申请日：1997-12-15
申请人： Fabio Alario , Jean-Marie Deves , Patrick Euzen
发明人： Fabio Alario , Jean-Marie Deves , Patrick Euzen
IPC分类号： B01J2713
CPC分类号： C10G35/09 , B01J23/56 , B01J23/58 , B01J23/63 , B01J23/8933 , B01J27/13
摘要： The invention relates to a catalyst comprising: a matrix consisting of 0 and 100% by weight of &lgr; transition alumina, the complement up to 100% by weight of the matrix being in &ggr; transition alumina, and relative to the total weight of the catalyst, from 0.001 to 2% by weight of silicon, from 0.1 to 15% by weight of at least one halogen chosen from the group formed by fluorine, chlorine, bromine and iodine, from 0.01 to 2% by weight of at least one noble metal from the platinum group, from 0.005 to 10% by weight of at least one promoter metal chosen from the group formed by tin, germanium, indium, gallium, thallium, antimony, lead, rhenium, manganese, chromium, molybdenum and tungsten, and if required from 0.001 to 10% by weight of a doping metal.
摘要翻译：本发明涉及一种催化剂，其包括：由0和100重量％的羔羊酸过渡氧化铝组成的基体，所述基体的重量比率高达100重量％，并且相对于催化剂的总重量， 0.001至2重量％的硅，0.1至15重量％的至少一种选自氟，氯，溴和碘的卤素，0.01至2重量％的至少一种贵金属，选自0.005至10重量％的至少一种选自由锡，锗，铟，镓，铊，锑，铅，铼，锰，铬，钼和钨形成的助催化剂金属， 0.001〜10重量％的掺杂金属。

2. 发明授权

US6045689A Process for catalytic conversion of hydrocarbons into aromatic compounds with a catalyst containing silicon 失效
标题翻译：用含有催化剂的烃催化转化成芳族化合物的方法
公开(公告)号：US6045689A
公开(公告)日：2000-04-04
申请号：US973402
申请日：1997-12-15
申请人： Fabio Alario , Jean-Marie Deves , Patrick Euzen
发明人： Fabio Alario , Jean-Marie Deves , Patrick Euzen
IPC分类号： B01J23/56 , B01J23/63 , B01J23/64 , B01J27/13 , B01J27/135 , C10G35/09 , C10G35/06 , C10G35/085
CPC分类号： C10G35/09 , B01J23/56 , B01J23/63 , B01J27/13
摘要： A process for converting hydrocarbons into aromatic compounds, which entails contacting a composition containing hydrocarbons with a catalyst under temperature and pressure conditions to produce the aromatic compounds, the catalyst containing a matrix of .eta. transition alumina and/or .gamma. transition alumina. The catalyst contains 0.001 to 2 wt % of silicon, 0.1 to 15 wt % of at least one platinum group metal, and 0.005 to 10 wt % of at least one promoter metal. The promoter metals may be tin, germanium, indium, gallium, thallium, antimony, lead, rhenium, manganese, chromium, molybdenium or tungsten. The catalyst may also contain a doping metal.
摘要翻译： PCT No.PCT / FR96 / 00919 Sec。 371 1997年12月15日第 102（e）日期1997年12月15日PCT Filted 1996年6月14日PCT公布。出版物WO97 / 00306 日期1997年1月3日一种将烃转化为芳族化合物的方法，其需要在温度和压力条件下使含烃的组合物与催化剂接触以产生芳族化合物，所述催化剂含有等离子体氧化铝和/或γ过渡氧化铝。催化剂含有0.001〜2重量％的硅，0.1〜15重量％的至少一种铂族金属和0.005〜10重量％的至少一种助催化剂金属。助催化剂金属可以是锡，锗，铟，镓，铊，锑，铅，铼，锰，铬，钼或钨。催化剂也可以含有掺杂金属。

3. 发明授权

US06007700A Process for the catalyst conversion of hydrocarbons into aromatics using a catalyst containing at least one doping metal chosen from the group consisting of titanium, zirconium, hafnium, cobalt, nickel, zinc, and/or the lanthanides 失效
标题翻译：使用含有选自钛，锆，铪，钴，镍，锌和/或镧系元素中的至少一种掺杂金属的催化剂将烃转化成芳族化合物的方法
公开(公告)号：US06007700A
公开(公告)日：1999-12-28
申请号：US973404
申请日：1997-12-15
申请人： Fabio Alario , Jean-Marie Deves , Patrick Euzen
发明人： Fabio Alario , Jean-Marie Deves , Patrick Euzen
IPC分类号： B01J21/04 , B01J21/06 , B01J23/56 , B01J23/63 , B01J23/656 , B01J27/13 , B01J37/02 , B01J37/24 , C10G35/06 , C10G35/09 , C10G35/095 , C10G45/68 , C10G35/085
CPC分类号： C10G45/68 , B01J21/04 , B01J23/56 , B01J23/63 , B01J23/6567 , B01J27/13 , C10G35/06 , C10G35/065 , C10G35/09 , C10G35/095 , B01J21/06 , B01J21/063 , B01J21/066 , B01J37/0209 , B01J37/24
摘要： Gasolines are reformed and parafin and naphthene hydrocarbons are converted to aromatic compounds by contacting the hydrocarbons with a catalyst comprising a matrix of .eta. transition alumina and .gamma. transition alumina. The catalyst contains at least one doping metal, at least one halogen, at least one noble metal and at least one promoter metal. The doping metals are selected from titanium, zirconium, hafnium, cobalt, nickel, zinc, and the lanthanides and the promoter metals are selected from tin, germanium, indium, gallium, thallium, antimony, lead, rhenium, manganese, chromium, molybdenum and tungsten.
摘要翻译： PCT No.PCT / FR96 / 00917 Sec。 371 1997年12月15日第 102（e）日期1997年12月15日PCT Filted 1996年6月14日PCT公布。公开号WO97 / 00305 PCT 日期1997年1月3日通过使烃与包含等离子体氧化铝和γ过渡氧化铝的基质的催化剂接触来改变石脑油并将石蜡和环烷烃转化为芳族化合物。催化剂含有至少一种掺杂金属，至少一种卤素，至少一种贵金属和至少一种助催化剂金属。掺杂金属选自钛，锆，铪，钴，镍，锌和镧系元素，助催化剂金属选自锡，锗，铟，镓，铊，锑，铅，铼，锰，铬，钼和钨。

4. 发明授权

US5968345A Process for the catalytic conversion of hydrocarbons into aromatic compounds using a catalyst containing alkali of alkaline-earth metals 失效
标题翻译：使用含有碱土金属碱的催化剂将烃催化转化成芳族化合物的方法
公开(公告)号：US5968345A
公开(公告)日：1999-10-19
申请号：US973406
申请日：1997-12-15
申请人： Fabio Alario , Jean-Marie Deves , Patrick Euzen
发明人： Fabio Alario , Jean-Marie Deves , Patrick Euzen
IPC分类号： B01J23/62 , B01J21/04 , B01J23/56 , B01J23/58 , B01J23/64 , B01J23/644 , B01J23/652 , B01J23/656 , B01J27/08 , B01J27/13 , C10G35/085 , C10G35/09
CPC分类号： B01J21/04 , B01J23/56 , B01J23/58 , B01J23/6567 , C10G35/085 , B01J23/62 , B01J23/6445 , B01J23/652 , B01J23/656 , B01J27/13
摘要： A process for the conversion of a hydrocarbon load containing paraffin, naphthene and aromatic hydrocarbons having 5 to 12 carbon atoms into aromatic compounds, which entails contacting the load with a catalyst under temperature and pressure conditions to produce the aromatic compounds, the catalyst containing:a matrix consisting of 0 to 100% by weight of .eta. transition alumina, the remaining weight percentage of the matrix, up to 100%, consisting of .gamma. transition alumina, andat least one doping metal selected from the group consisting of alkali metals and alkaline-earth metals,at least one halogen selected from the group consisting of fluorine, chlorine, bromine and iodine,at least one noble metal selected from the platinum group, andat least one promoter metal selected from the group consisting of tin, germanium, indium, gallium, thallium, antimony, lead, rhenium, manganese chromium, molybdenum and tungsten,the catalyst having previously been hydrothermally treated at a temperature of 300 to 1,000.degree. C. in a gaseous atmosphere containing steam, the atmosphere also containing chlorine in a molar content of greater than 0 but no more than 20%.
摘要翻译： PCT No.PCT / FR96 / 00915 Sec。 371 1997年12月15日第 102（e）日期1997年12月15日PCT Filted 1996年6月14日PCT公布。公开号WO97 / 00303 日本1997年1月3日将含有碳原子数为5〜12的烷烃，环烷烃和芳烃的烃负荷转化成芳香族化合物的方法，其需要使负载与催化剂在温度和压力条件下接触以产生芳族化合物，所述催化剂包含：由0-100重量％的η转变氧化铝组成的基体，所述基体的剩余重量百分比，至多100％，由γ转变氧化铝组成，以及至少一种掺杂金属，其选自碱金属和碱土金属，选自氟，氯，溴和碘的至少一种卤素，选自铂族的至少一种贵金属和选自锡的至少一种助催化剂金属，锗，铟，镓，铊，锑，铅，铼，锰铬，钼和钨，催化剂先前已被水热在含有蒸汽的气体气氛中，在300〜1000℃的温度下处理，气氛中还含有摩尔含量大于0但不大于20％的氯。

5. 发明授权

US5922639A Catalysts for use in hydrocarbon conversion reactions and containing one doping metal chosen from the group consisting of titanium, zirconium, hafnium, cobalt, nickel, zinc, the lanthanides and alkali and alkaline-earth metals 失效
标题翻译：用于烃转化反应并含有选自钛，锆，铪，钴，镍，锌，镧系元素和碱金属和碱土金属的一种掺杂金属的催化剂
公开(公告)号：US5922639A
公开(公告)日：1999-07-13
申请号：US973403
申请日：1997-12-15
申请人： Fabio Alario , Jean-Marie Deves , Patrick Euzen
发明人： Fabio Alario , Jean-Marie Deves , Patrick Euzen
IPC分类号： B01J23/56 , B01J23/58 , B01J23/63 , B01J27/13 , B01J27/138 , B01J37/02 , C10G35/09 , B01J27/06 , B01J27/125 , B01J27/135
CPC分类号： C10G35/09 , B01J23/56 , B01J23/58 , B01J23/63 , B01J27/13
摘要： The present invention relates to a catalyst comprising :a matrix consisting of a mixture of .eta. transition alumina, .gamma. transition alumina, andat least one doping metal chosen from the group made up of titanium, zirconium, hafnium, cobalt, nickel, zinc, the lanthanides, the alkali metals and alkaline-earth metals,at least one halogen chosen from the group made up of fluorine, chlorine, bromine and iodine,at least one noble metal from the platinum group, andat least one promoter metal chosen from the group made up of tin, germanium, indium, gallium, thallium, antimony, lead, rhenium, manganese, chromium, molybdenum and tungsten.
摘要翻译： PCT No.PCT / FR96 / 00916 Sec。 371 1997年12月15日第 102（e）日期1997年12月15日PCT Filted 1996年6月14日PCT公布。公开号WO97 / 00304 日本1997年1月3日本发明涉及一种催化剂，其包含：由等离子体氧化铝，γ过渡氧化铝和至少一种掺杂金属的混合物组成的基体，所述掺杂金属选自钛，锆，铪，钴，镍，锌，镧系元素，碱金属和碱土金属，选自氟，氯，溴和碘的至少一种卤素，至少一种来自铂族的贵金属，以及至少一种助催化剂选自由锡，锗，铟，镓，铊，锑，铅，铼，锰，铬，钼和钨组成的组中的金属。

6. 发明授权

US06548305B1 Automatic multi-reactor catalyst evaluation method an device with in-line analysis without liquid-gas separation 有权
标题翻译：自动多反应器催化剂评价方法一种无液气分离的在线分析装置
公开(公告)号：US06548305B1
公开(公告)日：2003-04-15
申请号：US09604736
申请日：2000-06-28
申请人： Jean-Marie Deves , Jean-Yves Bernhard , Bernard Chatelain , Pierre Toutant , José Brandely , Corinne Guitton
发明人： Jean-Marie Deves , Jean-Yves Bernhard , Bernard Chatelain , Pierre Toutant , José Brandely , Corinne Guitton
IPC分类号： G01N3110
CPC分类号： G01N31/10 , Y10T436/24
摘要： A method and an equipment carry out measurements on an effluent resulting from a chemical reaction taking place in a reactor containing a catalyst. The method includes, in combination, injecting at least one feedstock into at least two reactors, sending the effluent coming from one of the reactors for analysis and measuring controlling the pressure and the temperature of the effluent in the circuit contained between downstream from the reactors and upstream from the analysis device, and allowing automatic monitoring and control of the chemical reaction in the reactors and of the analysis and measurement cycle performed on the effluent produced by the reaction.
摘要翻译：一种方法和设备对在含有催化剂的反应器中发生的化学反应产生的流出物进行测量。该方法包括组合地将至少一种原料注入至少两个反应器中，送出来自反应器之一的流出物进行分析和测量，以控制在反应器下游包含的回路中的流出物的压力和温度，以及并且允许对反应器中的化学反应的自动监测和控制以及对由反应产生的流出物进行的分析和测量循环进行。

7. 发明授权

US06387246B1 Catalyst that comprises a partially amorphous Y zeolite and its use in hydroconversion of hydrocarbon petroleum feedstocks 有权
标题翻译：包含部分无定形Y沸石的催化剂及其在烃类石油原料加氢转化中的用途
公开(公告)号：US06387246B1
公开(公告)日：2002-05-14
申请号：US09572970
申请日：2000-05-18
申请人： Eric Benazzi , Jean-Marie Deves , Bernadette Rebours , Frédéric Chaigne , Tivadar Cseri , Slavik Kasztelan
发明人： Eric Benazzi , Jean-Marie Deves , Bernadette Rebours , Frédéric Chaigne , Tivadar Cseri , Slavik Kasztelan
IPC分类号： C01G4718
CPC分类号： B01J29/084 , B01J29/166 , B01J2229/20 , B01J2229/22 , B01J2229/36 , B01J2229/37 , B01J2229/42 , C10G45/12 , C10G47/16
摘要： The invention relates to a catalyst that contains at least one matrix, a partially amorphous Y zeolite, optionally at least one metal that is selected from the group that is formed by the metals of group VIB and group VIII of the periodic table, optionally at least one element that is selected from the group that is formed by phosphorus, boron and silicon, optionally at least one element of group VIIA, and optionally at least one element of group VIIB. The partially amorphous Y zeolite has a peak rate that is less than 0.4, and a crystalline fraction that is expressed relative to a reference zeolite in sodium form and that is less than 60%. The invention also relates to the use of this catalyst in hydroconversion, in particular hydrocracking and hydrorefining of hydrocarbon feedstocks.
摘要翻译：本发明涉及一种催化剂，其含有至少一种基质，部分无定形Y沸石，任选至少一种金属，其选自由元素周期表第ⅥB族和Ⅷ族金属形成的基团，任选至少选自由磷，硼和硅形成的基团，任选的ⅦA族的至少一种元素和任选的至少一种ⅦB族元素的一种元素。部分无定形的Y沸石具有小于0.4的峰值速率和相对于钠形式的参考沸石表达并且小于60％的结晶部分。本发明还涉及该催化剂在加氢转化中的用途，特别是烃原料的加氢裂化和加氢精制。

8. 发明授权

US6103652A Staged combustion process and apparatus for regenerating a reforming or aromatic compound production catalyst in a moving bed 失效
标题翻译：用于在移动床中再生重整或芳族化合物生产催化剂的分段燃烧方法和装置
公开(公告)号：US6103652A
公开(公告)日：2000-08-15
申请号：US59292
申请日：1998-04-14
申请人： Fran.cedilla.ois-Xavier Brunet , Emmanuelle Bromet , Jean-Marie Deves
发明人： Fran.cedilla.ois-Xavier Brunet , Emmanuelle Bromet , Jean-Marie Deves
IPC分类号： B01J27/32 , B01J23/96 , B01J38/14 , B01J38/20 , B01J38/24 , B01J38/34 , B01J38/44 , C07B61/00 , C10G35/12 , B01J20/34 , B01J38/12 , B01J38/22
CPC分类号： B01J8/12 , B01J23/96 , B01J38/20 , B01J38/24 , B01J38/44 , C10G35/12
摘要： The invention concerns a process for moving bed regeneration of a reforming or aromatic hydrocarbon production catalyst. The catalyst includes a support, at least one noble metal and at least one halogen. The process includes a combustion step in which the catalyst is treated in at least two successive combustion zones. Also, the process includes each combustion zone separated from adjacent combustion zones allowing catalyst to pass and preventing passage of gas, at least one oxygen-containing gas introduced into each zone and produced gases extracted from each zone, and the severity of the operating conditions in each zone increasing in the direction of catalyst flow. Advantageously, the combustion step ends in a zone for monitoring and controlling combustion completion characterized by a low or zero oxygen consumption.
摘要翻译：本发明涉及一种用于移动重整或芳族烃生产催化剂的床再生的方法。催化剂包括载体，至少一种贵金属和至少一种卤素。该方法包括燃烧步骤，其中在至少两个连续的燃烧区域中处理催化剂。此外，该方法还包括从相邻燃烧区分离的每个燃烧区，使得催化剂通过并防止气体的通过，至少一个引入每个区域的含氧气体和从每个区域提取的产生的气体，以及操作条件的严重性每个区域在催化剂流动方向上增加。有利地，燃烧步骤终止于用于监测和控制燃烧完成的区域，其特征在于低或零氧气消耗。

9. 发明授权

US08728404B1 Vessel for regeneration of a catalyst including monitoring and monitoring and control of combustion completion 有权
标题翻译：用于再生催化剂的容器，包括监测和监测和控制燃烧完成
公开(公告)号：US08728404B1
公开(公告)日：2014-05-20
申请号：US09551831
申请日：2000-04-18
申请人： François-Xavier Brunet , Emmanuelle Bromet , Jean-Marie Deves , Dominique Humeau , Eric Sanchez
发明人： François-Xavier Brunet , Emmanuelle Bromet , Jean-Marie Deves , Dominique Humeau , Eric Sanchez
IPC分类号： B01J38/14 , B01J38/20 , B01J38/22
CPC分类号： B01J8/12 , B01J38/12 , B01J38/14 , B01J38/20 , B01J38/24 , C10G35/12
摘要： A vessel for regenerating used catalyst comprising at least one combustion zone provided with at least two walls (5a, 5b) between which the catalyst circulates as a moving bed, and provided with at least one conduit (4) for introducing at least one oxygen-containing gas entering the moving bed via one of the walls and leaving via another wall, characterized in that it also comprises a zone (FC) for monitoring and controlling the end of combustion located after the end of the flame front of the last combustion zone (Z2), provided with a conduit (11) for introducing an oxygen-containing monitoring and control gas and at least one means for measuring the temperature and/or the oxygen content in the gas and/or the catalyst leaving the monitoring and control zone.A separator (29) is located between the monitoring and control zone and the last combustion zone for preventing the passage of gas while allowing for the passage of the catalyst.
摘要翻译：一种用于再生所用催化剂的容器，包括至少一个燃烧区，该燃烧区设置有至少两个壁（5a，5b），催化剂在其之间作为移动床循环，并且设置有至少一个导管（4），用于引入至少一个氧 - 包含气体通过一个壁进入移动床并通过另一个壁离开，其特征在于，其还包括用于监测和控制位于最后燃烧区域的火焰前端的末端之后的燃烧端的区域（FC） Z2），其具有用于引入含氧监测和控制气体的导管（11）和用于测量离开监测和控制区的气体和/或催化剂中的温度和/或氧含量的至少一种装置。分离器（29）位于监测和控制区域与最后一个燃烧区之间，用于防止气体通过，同时允许催化剂通过。

10. 发明申请

US20050214176A1 Process and device for the production of aromatic compounds including a reduction of the catalyst 审中-公开
标题翻译：用于生产芳族化合物的方法和装置，包括催化剂的还原
公开(公告)号：US20050214176A1
公开(公告)日：2005-09-29
申请号：US10703546
申请日：2003-11-10
申请人： Francois-Xavier Brunet , Olivier Clause , Jean-Marie Deves , Eric Sanchez , Frederic Hoffmann
发明人： Francois-Xavier Brunet , Olivier Clause , Jean-Marie Deves , Eric Sanchez , Frederic Hoffmann
IPC分类号： B01J38/04 , C07B61/00 , C07C5/42 , C07C15/04 , C07C15/06 , C07C15/08 , C10G35/09 , C10G35/12 , C10G35/22 , B01J8/18
CPC分类号： B01J8/12 , C10G35/12
摘要： The invention relates to a process for the production of aromatic compounds from a hydrocarbon fraction with a catalyst that preferably circulates in a moving bed, a process that comprises at least the following successive stages that take place in at least one zone: treatment of the fraction in the presence of hydrogen and implementing at least one reaction for dehydrogenation of naphthenes; separation of the gas effluent that contains hydrogen, the liquid product and the catalyst; regeneration of the catalyst; reduction of the catalyst; and reintroduction of the catalyst for the treatment stage; recycling in the treatment stage of at least a portion of the gas effluent that contains the hydrogen that is called recycling gas; process in which the reduction stage is carried out in the presence of recycling gas that is introduced in an amount such that the amount of pure hydrogen that is provided is between 1-10 kg/kg of catalyst, whereby the effluent that is obtained from the reduction is then separated from the catalytic bed. The invention also pertains to the related device.
摘要翻译：本发明涉及一种由具有优选在移动床中循环的催化剂的烃馏分生产芳族化合物的方法，该方法至少包括在至少一个区域中发生的以下连续阶段：处理馏分在氢的存在下，并且实施至少一个用于环烷酸脱氢的反应; 分离含有氢气，液体产物和催化剂的气体流出物; 催化剂再生; 还原催化剂; 并重新引入用于治疗阶段的催化剂; 在处理阶段回收至少一部分含有称为再循环气体的氢气的气体流出物; 在再循环气体的存在下进行还原阶段的方法，该再循环气体的导入量使得提供的纯氢的量在1-10kg / kg的催化剂之间，由此得到的流出物然后将还原与催化床分离。本发明也涉及相关设备。

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