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1. 发明授权

US07399393B2 Oxide ion conductive ceramic membrane structures for high-pressure oxygen production 有权
标题翻译：氧化物离子导电陶瓷膜结构用于高压氧气生产
公开(公告)号：US07399393B2
公开(公告)日：2008-07-15
申请号：US10470169
申请日：2001-12-18
申请人： Christophe Chaput , Thierry Terracol , Gisèle Bach , Guylaine Gouriou , Pascal Del Gallo
发明人： Christophe Chaput , Thierry Terracol , Gisèle Bach , Guylaine Gouriou , Pascal Del Gallo
IPC分类号： C25B13/04
CPC分类号： B01D69/12 , B01D53/228 , B01D53/326 , B01D69/02 , B01D71/024 , C01B13/0255 , C01B2210/0046 , H01M4/9033 , H01M8/0206 , H01M8/0226 , H01M8/1213 , H01M8/1246 , Y02E60/525 , Y02P70/56
摘要： The invention concerns an oxide ion conductive ceramic membrane, characterized in that it comprises a non-null finite volume with non-null total thickness E, comprising, a dense layer (CD) of a solid electrolyte, a so-called bonding layer (CA), of mixed conductive porous cathode (EP) and porous anode (EP′), a cathode current collector (CC) and an anode current collector (CC′), a coating porous layer (ER), and a coating porous layer (ER′), and characterized in that the volume E of said membrane, is equal to the sum of the thickness of said elements. The membrane is used for separating oxygen from air or from a gas mixture containing same and in particular for producing ultra-pure oxygen under high pressure in a closed chamber.
摘要翻译：本发明涉及一种氧化物离子传导陶瓷膜，其特征在于其包括具有非零总厚度E的非零有限体积，包括固体电解质的致密层（CD），所谓的粘结层（CA ），多孔阳极（EP'），阴极集电体（CC）和阳极集电体（CC'），涂层多孔层（ER）和涂层多孔层 '），其特征在于所述膜的体积E等于所述元件的厚度之和。膜用于从空气或含有其的气体混合物中分离氧气，特别是用于在密闭室中在高压下生产超纯氧。

2. 发明授权

US07300561B2 Oxide ion conductive ceramic membrane stacked microstructures; use for separating oxygen from air 有权
标题翻译：氧化物离子导电陶瓷膜堆叠微结构; 用于从空气中分离氧气
公开(公告)号：US07300561B2
公开(公告)日：2007-11-27
申请号：US10470172
申请日：2001-12-18
申请人： Christophe Chaput , Thierry Terracol , Gisèle Bach , Guylaine Gouriou , Pascal Del Gallo
发明人： Christophe Chaput , Thierry Terracol , Gisèle Bach , Guylaine Gouriou , Pascal Del Gallo
IPC分类号： C25B13/04
CPC分类号： B01D69/12 , B01D53/228 , B01D53/326 , B01D69/02 , B01D71/024 , C01B13/0255 , C01B2210/0046
摘要： The invention concerns an oxide ion conductive ceramic membrane, characterized in that it comprises a non-null finite volume with non-null total thickness E, comprising a dense layer (CD) of a solid electrolyte, a so-called bonding layer (CA), of two porous electrodes (EP) and (EP′), two porous current collectors (CC) and (CC′), and at least at least a coating porous layer (ER), characterized in that the thickness E of the volume of said membrane, is equal to the sum of the thickness of each of said elements. The membrane is used for separating oxygen from air or from a gas mixture containing same.
摘要翻译：本发明涉及一种氧化物离子传导性陶瓷膜，其特征在于，其包括具有非零无效总厚度E的非零有限体积，包括固体电解质的致密层（CD），即所谓的结合层（CA）的两个多孔电极（EP）和（EP'），两个多孔集电器（CC）和（CC'），以及至少一个涂覆多孔层（ER），其特征在于，所述膜等于每个所述元件的厚度之和。膜用于从空气或含有它们的气体混合物中分离氧气。

3. 发明授权

US06475657B1 Ceramic membrane which is in an oxide ion conductor based on yttrium-stabilized zirconia 失效
标题翻译：基于钇稳定氧化锆的氧化物离子导体中的陶瓷膜
公开(公告)号：US06475657B1
公开(公告)日：2002-11-05
申请号：US09617501
申请日：2000-07-17
申请人： Pascal Del Gallo , Guylaine Gouriou
发明人： Pascal Del Gallo , Guylaine Gouriou
IPC分类号： H01M810
CPC分类号： B01D67/0041 , B01D53/228 , B01D53/326 , B01D71/024 , B01D2325/26 , C01B13/0255 , C01B2210/0046
摘要： A ceramic membrane having a non-zero volume and including: a) a dense layer, having opposed faces of areas S and S′ and having a non-zero thickness e, of a solid electrolyte; b) two porous electrodes, which are hybrid conductors and have non-zero thicknesses e1 and e′1, which are identical or different, coated on non-zero areas s1 and s′1, which are identical or different, of the two opposed faces of areas S and S′ of the solid electrolyte; c) two porous current collectors, of non-zero thicknesses, e2 and e′2, which are identical or different, coated on non-zero areas s2 and S′2, which are identical or different, of the two porous electrodes; and d) at least one porous covering layer, of non-zero thickness e3, coated on a non-zero area s3, of at least one of the collectors, a thickness E of the membrane is equal to the sum of the thickness of each of the elements a)-d).
摘要翻译：一种具有非零体积的陶瓷膜，包括：a）致密层，其具有固体电解质的非零厚度e的区域S和S'的相对面; b）两个多孔电极，其是混合的导体，并且具有相同或不同的非零厚度e1和e'1，其涂覆在相同或不同的区域S和S'的两个相对面的非零区域s1和s'1上固体电解质; c）两个相同或不同的非零厚度e2和e'2的两个多孔集电器涂覆在两个多孔的非零区域s2和S'2上，它们是相同或不同的电极和）至少一个涂覆在至少一个收集器的非零区域s3上的非零厚度e3的多孔覆盖层，膜的厚度E等于每个的厚度的总和元素a）-d）。

4. 发明授权

US08241715B2 Gas vessel packing structure having a crystalline phase 有权
标题翻译：具有结晶相的气体容器包装结构
公开(公告)号：US08241715B2
公开(公告)日：2012-08-14
申请号：US12877855
申请日：2010-09-08
申请人： Gilles Cannet , Pascal Del Gallo , Thierry Chartier , Emmanuel Baune , Jérome Cantonnet , Jean-François Imbault
发明人： Gilles Cannet , Pascal Del Gallo , Thierry Chartier , Emmanuel Baune , Jérome Cantonnet , Jean-François Imbault
IPC分类号： A47G19/22 , B28B11/00 , B28B21/00 , B28B21/72 , B28B23/08 , B29D22/00 , B29D23/00
CPC分类号： C04B28/18 , B01D5/0015 , B01D5/009 , C04B2/10 , C04B35/22 , C04B35/62655 , C04B2111/00948 , C04B2235/3206 , C04B2235/3208 , C04B2235/3217 , C04B2235/3272 , C04B2235/3418 , C04B2235/3454 , C04B2235/5427 , C04B2235/80 , C04B2235/96 , F17C11/00 , F17C11/002 , Y02E60/321 , Y02P40/615 , Y02W30/97 , Y10T428/13 , Y10T428/131 , Y10T428/249932 , C04B14/043 , C04B14/06 , C04B14/42 , C04B18/24 , C04B40/024 , C04B14/28 , C04B14/386
摘要： The present invention relates to a container packing structure, characterized in that it comprises a crystalline phase containing 55 to 97% by weight of xonotlite crystallites and 3 to 45% by weight of tobermorite crystallites. It also relates to a method for fabricating such a packing structure, and the container containing same, and its use for storing fluids such as gases.
摘要翻译：本发明涉及一种容器包装结构，其特征在于，其包含含有55-97重量％的硬硅钙石微晶和3〜45重量％的雪硅钙石微晶的结晶相。它还涉及一种用于制造这种包装结构的方法，以及包含其的容器及其用于储存诸如气体的流体的用途。

5. 发明申请

US20110118112A1 Supported Catalyst For Producing H2 And/Or CO From Low Molecular Weight Hydrocarbons 有权
标题翻译：用于从低分子量烃生产H2和/或CO的负载型催化剂
公开(公告)号：US20110118112A1
公开(公告)日：2011-05-19
申请号：US12949289
申请日：2010-11-18
申请人： Francesco Basile , Pascal Del Gallo , Giuseppe Fornasari , Daniel Gary , Valentina Rosetti , Angelo Vaccari
发明人： Francesco Basile , Pascal Del Gallo , Giuseppe Fornasari , Daniel Gary , Valentina Rosetti , Angelo Vaccari
IPC分类号： B01J21/10
CPC分类号： C01B3/40 , B01J23/002 , B01J23/005 , B01J23/892 , B01J37/08 , B01J2523/00 , C01B3/386 , C01B2203/0233 , C01B2203/0238 , C01B2203/0261 , C01B2203/1011 , C01B2203/1023 , C01B2203/1052 , C01B2203/1064 , C01P2002/72 , Y02P20/52 , B01J2523/22 , B01J2523/31 , B01J2523/822 , B01J2523/847
摘要： Chemical combination (C) between an active solid phase which is covalently bound to the surface of an inert solid phase, characterized in that said solid active phase essentially consists in a solid solution of a mixture of at least a magnesium oxide type phase compound and at least a magnesium silicate type phase compound in which Al, and Rh and/or Ni cations are soluted and characterized in that said inert solid phase is either a compound represented by the general formula (I): AlaNibRhcMgdSieOf (I) wherein a, b, c, d, and e are integers which are greater than or equal to 0, f is an integer greater than 0, the sum a+b+c+d≠0, and wherein (3a+2b+3c+2d+4e)/2=f, or a mixture of compounds represented by the said general formula (I), provided that at least one of the Si, Al, Mg, Rh or Ni elements, which is present in the solid active phase, is also present in the solid inert phase. Use of a catalyst in chemical reactions involving the conversion of hydrocarbonaceous feedstocks.
摘要翻译：在与惰性固相表面共价结合的活性固相之间的化学组合（C），其特征在于所述固体活性相基本上由至少一种氧化镁型相化合物的混合物和至少一种其中Al和Rh和/或Ni阳离子被溶解并表征的硅酸镁型相化合物，其特征在于所述惰性固相是由通式（I）表示的化合物：AlaNibRhcMgdSieOf（I）其中a，b， c，d和e是大于或等于0的整数，f是大于0的整数，和a + b + c + d≠0，其中（3a + 2b + 3c + 2d + 4e） / 2 = f或由所述通式（I）表示的化合物的混合物，条件是存在于固体活性相中的Si，Al，Mg，Rh或Ni元素中的至少一种也存在在固体惰性相中。在涉及烃类原料转化的化学反应中使用催化剂。

6. 发明授权

US06207038B1 Process for preparing a composite electrolyte based on BIMEVOX and the use of said compound in separating oxygen from a gas mixture 失效
标题翻译：基于BIMEVOX制备复合电解质的方法以及所述化合物在从气体混合物中分离氧气中的用途
公开(公告)号：US06207038B1
公开(公告)日：2001-03-27
申请号：US09346308
申请日：1999-07-02
申请人： César Marlu Steil , Jacques Fouletier , Michel Kleitz , Gilles Lagrange , Pascal Del Gallo , Gaëtan Mairesse , Jean-Claude Boivin
发明人： César Marlu Steil , Jacques Fouletier , Michel Kleitz , Gilles Lagrange , Pascal Del Gallo , Gaëtan Mairesse , Jean-Claude Boivin
IPC分类号： C25C110
CPC分类号： C01G31/006 , B01D53/326 , B01D2257/104 , C01B13/0233 , C01B2210/0046 , C01P2002/54 , C01P2004/03 , C01P2006/40 , G01N27/4073
摘要： A process for preparing a solid composite electrolyte comprising at least one compound of the BIMEVOX family is provided. The process comprises at least one step of preparing a mixture of one or more compounds of the BIMEVOX family with one or more chemically inert compounds, at least one step of compacting the mixture obtained, and at least one sintering step during which the temperature reached, over a nonzero time interval, has a value greater than the optimum sintering temperature for the compound of the BIMEVOX family.
摘要翻译：提供了一种制备包含至少一种BIMEVOX族化合物的固体复合电解质的方法。该方法包括至少一个步骤：制备一种或多种BIMEVOX族化合物与一种或多种化学惰性化合物的混合物，至少一个压实所获得混合物的步骤和至少一个烧结步骤，在非零时间间隔内，具有大于BIMEVOX系列化合物的最佳烧结温度的值。

7. 发明授权

US08105973B2 Supported catalyst for producing H2 and/or CO from low molecular weight hydrocarbons 有权
标题翻译：用于从低分子量烃生产H2和/或CO的负载型催化剂
公开(公告)号：US08105973B2
公开(公告)日：2012-01-31
申请号：US12949289
申请日：2010-11-18
申请人： Francesco Basile , Pascal Del Gallo , Giuseppe Fornasari , Daniel Gary , Valentina Rosetti , Angelo Vaccari
发明人： Francesco Basile , Pascal Del Gallo , Giuseppe Fornasari , Daniel Gary , Valentina Rosetti , Angelo Vaccari
IPC分类号： B01J21/06 , C01B3/26
CPC分类号： C01B3/40 , B01J23/002 , B01J23/005 , B01J23/892 , B01J37/08 , B01J2523/00 , C01B3/386 , C01B2203/0233 , C01B2203/0238 , C01B2203/0261 , C01B2203/1011 , C01B2203/1023 , C01B2203/1052 , C01B2203/1064 , C01P2002/72 , Y02P20/52 , B01J2523/22 , B01J2523/31 , B01J2523/822 , B01J2523/847
摘要： Chemical combination (C) between an active solid phase which is covalently bound to the surface of an inert solid phase, characterized in that said solid active phase essentially consists in a solid solution of a mixture of at least a magnesium oxide type phase compound and at least a magnesium silicate type phase compound in which Al, and Rh and/or Ni cations are soluted and characterized in that said inert solid phase is either a compound represented by the general formula (I): AlaNibRhcMgdSieOf (I) wherein a, b, c, d, and e are integers which are greater than or equal to 0, f is an integer greater than 0, the sum a+b+c+d≠0, and wherein (3a+2b+3c+2d+4e)/2=f, or a mixture of compounds represented by the said general formula (I), provided that at least one of the Si, Al, Mg, Rh or Ni elements, which is present in the solid active phase, is also present in the solid inert phase.Use of a catalyst in chemical reactions involving the conversion of hydrocarbonaceous feedstocks.
摘要翻译：在与惰性固相表面共价结合的活性固相之间的化学组合（C），其特征在于所述固体活性相基本上由至少一种氧化镁型相化合物的混合物和至少一种其中Al和Rh和/或Ni阳离子被溶解并表征的硅酸镁型相化合物，其特征在于所述惰性固相是由通式（I）表示的化合物：AlaNibRhcMgdSieOf（I）其中a，b， c，d和e是大于或等于0的整数，f是大于0的整数，和a + b + c + d≠0，其中（3a + 2b + 3c + 2d + 4e） / 2 = f或由所述通式（I）表示的化合物的混合物，条件是存在于固体活性相中的Si，Al，Mg，Rh或Ni元素中的至少一种也存在在固体惰性相中。在涉及烃类原料转化的化学反应中使用催化剂。

8. 发明授权

US07955526B2 Addition of (a) blocking agent(s) in a ceramic membrane for clocking crystalline growth of grains during atmospheric sintering 有权
标题翻译：（a）在陶瓷膜中加入封闭剂，用于在大气烧结过程中晶粒生长
公开(公告)号：US07955526B2
公开(公告)日：2011-06-07
申请号：US10577867
申请日：2004-11-05
申请人： Pascal Del Gallo , Thierry Chartier , Gregory Etchegoyen
发明人： Pascal Del Gallo , Thierry Chartier , Gregory Etchegoyen
IPC分类号： H01B1/00
CPC分类号： B01D71/024 , B01D67/0041 , B01D71/02 , B01D71/022 , B01D2323/08 , B01D2323/18 , B01J8/009 , B01J19/2475 , B01J23/002 , B01J23/02 , B01J23/10 , B01J23/78 , B01J23/83 , B01J35/0006 , B01J35/065 , B01J2523/00 , C01B3/386 , C01B13/0255 , C01B2203/0261 , C01B2203/1241 , C01B2203/1258 , C01B2210/0046 , C01G49/009 , C01P2004/80 , C04B35/2641 , C04B35/62685 , C04B2235/3206 , C04B2235/3213 , C04B2235/3227 , C04B2235/3232 , C04B2235/3236 , C04B2235/3274 , C04B2235/3286 , C04B2235/768 , C04B2235/786 , C04B2235/80 , Y02P20/52 , B01J2523/24 , B01J2523/3706 , B01J2523/842 , B01J2523/22 , B01J2523/47 , B01J2523/31 , B01J2523/32
摘要： A composite material (M) comprising: at least 75% by volume of a mixed electronic conductor compound oxygen anions O (C1) selected from doped ceramic compounds which, at the temperature of use, are present in the form of a crystalline network having ion oxide lattice vacancies and, more particularly, in the form of a cubic phase, a fluorite phase, a perovskite phase, of the aurivillius variety, a Brown-Millerite phase or a pyrochlore phase; and 0.01%-25% by volume of a compound (C2) which is different from compound (C1), selected from oxide-type ceramic materials, non-oxide type ceramic materials, metals, metal alloys or mixtures of said different types of material; and 0%-2.5% by volume of a compound (C3) produced from at least one chemical reaction represented by the equation: xFC1+yFC2 - - - >zFC3, wherein FC1, FC2 and FC3 represent the raw formulae of compounds (C1), (C2) and (C3) and x, y and z represent rational numbers above or equal to 0. The invention also relates to a method for the preparation and use thereof as mixed conductor material for a membrane catalytic reactor used to synthesize synthetic gas by catalytic oxidation of methane or natural gas and/or as mixed conductor material for a ceramic membrane.
摘要翻译：一种复合材料（M），其包含：至少75体积％的混合电子导体化合物氧阴离子O 2（C1），其选自掺杂的陶瓷化合物，其在使用温度下以具有离子氧化物晶格空位的晶体网络，更具体地，呈立方相，萤石相，钙钛矿相，褐铁矿相或烧绿石相的形式; 和0.01％-25％体积的选自氧化物型陶瓷材料，非氧化物型陶瓷材料，金属，金属合金或所述不同类型材料的混合物的不同于化合物（C1）的化合物（C2） ; 和由下式表示的至少一种化学反应产生的化合物（C3）的0％-2.5％（体积）：其中FC1，FC2和FC3代表化合物（C1）的原始化学式，，（C2）和（C3），x，y和z表示高于或等于0的有理数。本发明还涉及一种制备和使用它作为用于合成合成气体的膜催化反应器的混合导体材料的方法通过甲烷或天然气的催化氧化和/或用作陶瓷膜的混合导体材料。

9. 发明授权

US07329691B2 Perovskite catalyst for the partial oxidation of natural gas 有权
标题翻译：用于部分氧化天然气的钙钛矿催化剂
公开(公告)号：US07329691B2
公开(公告)日：2008-02-12
申请号：US10712691
申请日：2003-11-13
申请人： Francesco Basile , Giuseppe Fornasari , Angelo Vaccari , Pascal Del Gallo , Daniel Gary
发明人： Francesco Basile , Giuseppe Fornasari , Angelo Vaccari , Pascal Del Gallo , Daniel Gary
IPC分类号： C07C27/06 , C07C27/00 , B01J23/00 , B01J23/40 , B01J23/42
CPC分类号： C01B3/40 , B01J23/002 , B01J23/63 , B01J23/83 , B01J23/894 , B01J23/8946 , B01J2523/00 , C01B2203/0233 , C01B2203/0238 , C01B2203/0261 , C01B2203/044 , C01B2203/1052 , C01B2203/1064 , Y02P20/142 , Y02P20/52 , B01J2523/3706 , B01J2523/3712 , B01J2523/822 , B01J2523/842 , B01J2523/847
摘要： A composition and method for a Catalytic Partial Oxidation (CPO) of methane to synthesis gas. The catalyst allows the process to proceed at low residence time providing a long time thermal stability. The perovskite structure [AzA′1-z][B1-x-yNix Rhy] O3-δ of the catalyst is obtained using mainly La, Sr, as A and A′ cation sites (A, A′: actinide and/or lanthanide, elements and/or elements from Group I and II) and mainly Fe, Ni, as B cation sites (B: transition metal element and/or element from Group III to V).
摘要翻译：甲烷对合成气的催化部分氧化（CPO）的组成和方法。催化剂允许该方法在低停留时间下进行，提供长时间的热稳定性。钙钛矿结构[A 1 Z 1 -Z 1] - [B 1-xy N 2 N z N 2 使用主要为La，Sr作为A和A'阳离子位点（A，A'：锕系元素和/或镧系元素，元素和/或镧系元素）获得催化剂的O 3-δ /或来自组I和II的元素）和主要是Fe，Ni，作为B阳离子位点（B：过渡金属元素和/或从III至V族的元素）。

10. 发明授权

US06230614B1 Device for reducing the oxidation of food products 失效
标题翻译：减少食品氧化的装置
公开(公告)号：US06230614B1
公开(公告)日：2001-05-15
申请号：US09692220
申请日：2000-10-20
申请人： Pascal Del Gallo , Gilles Lagrange , Lucie Prost
发明人： Pascal Del Gallo , Gilles Lagrange , Lucie Prost
IPC分类号： A23L334
CPC分类号： B01D53/326 , A23L3/3418 , A23L3/3436 , B01D71/024
摘要： Provided is a device for treating a food product in order to reduce or eliminate the detrimental effects of the presence of oxygen which is in contact with the external surface of the product. The device includes a vat provided with a hood, containing a food product whose free surface is in contact with the atmospheric air, a solid electrolyte membrane, each face of the membrane being connected to an electrode, each electrode being connected to a current generator, a heater for making the electrolyte operate at the desired working temperature, a pump for discharging oxygen extracted, by the solid electrolyte, from the atmospheric air present above the food product, in a pipe, a pump for circulating the atmosphere to be treated, an oxygen analyzer for measuring the oxygen level in the gas atmosphere above the food product, a control unit for modifying the operation of the solid electrolyte as a function of the oxygen level and the gas atmosphere to be treated and the recirculation rate of the atmosphere and, optionally, a cooling unit.
摘要翻译：提供了一种用于处理食品的装置，以便减少或消除与产品的外表面接触的氧的存在的有害影响。该装置包括具有罩的容器，其容纳食品，其自由表面与大气接触;固体电解质膜，膜的每个面与电极连接，每个电极连接到电流发生器，用于使电解液在期望的工作温度下工作的加热器，用于排出由固体电解质从存在于食品上方的大气中排出的氧的泵，管道，用于循环待处理气氛的泵，用于测量食品上方的气体气氛中的氧气含量的氧分析器，用于改变固体电解质作为氧水平和待处理气体气氛以及大气再循环的函数的操作的控制单元，可选地，冷却单元。

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