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1. 发明授权

US6147126A Gas conversion using hydrogen from syngas gas and hydroconversion tail gas 失效
标题翻译：使用合成气气体和加氢转化尾气的氢气进行气体转化
公开(公告)号：US6147126A
公开(公告)日：2000-11-14
申请号：US21476
申请日：1998-02-10
申请人： Charles W. DeGeorge , Robert J. Wittenbrink , Thomas M. Stark
发明人： Charles W. DeGeorge , Robert J. Wittenbrink , Thomas M. Stark
IPC分类号： C07C1/04 , C10G2/00 , C07C27/00
CPC分类号： C01B3/38 , C01B3/44 , C01B3/48 , C07C1/0485 , C07C1/049 , C10G2/00 , C10G2/332 , C01B2203/0233 , C01B2203/0244 , C01B2203/0261 , C01B2203/0415 , C01B2203/043 , C01B2203/0475 , C01B2203/0495 , C01B2203/062 , C01B2203/1241 , C01B2203/1258 , C01B2203/147
摘要： A gas conversion process including catalytic hydrocarbon synthesis from a synthesis gas comprising a mixture of H.sub.2 and CO, produces hydrogen from the synthesis gas and upgrades synthesized hydrocarbons by one or more hydroconversion operations which utilize this hydrogen. The hydroconversion also produces a hydrogen rich tail gas which is used in the process for at least one of (i) hydrocarbon synthesis catalyst rejuvenation, (ii) the hydrocarbon synthesis, and (iii) hydrogen production. In one embodiment the tail gas is used to hydrodesulfurize sulfur-containing hydrocarbon liquids recovered from the natural gas used to form the synthesis gas. The hydrogen production is accomplished by physical separation, such as PSA, with or without chemical means such as a water gas shift reaction.
摘要翻译：一种气体转化方法，包括从包含H 2和CO的混合物的合成气中进行的催化烃合成，从合成气产生氢气，并通过利用该氢气的一个或多个加氢转化操作来升级合成的烃。加氢转化还产生富氢尾气，其在该方法中用于（i）烃合成催化剂再生，（ii）烃合成和（iii）氢生产中的至少一种。在一个实施方案中，尾气用于加氢脱硫从用于形成合成气的天然气回收的含硫烃液体。氢气的产生是通过物理分离来实现的，如PSA，有或没有化学手段，如水煤气变换反应。

2. 发明授权

US6103773A Gas conversion using hydrogen produced from syngas for removing sulfur from gas well hydrocarbon liquids 失效
标题翻译：使用由合成气产生的氢气从气井烃液体中除去硫气的气体转化
公开(公告)号：US6103773A
公开(公告)日：2000-08-15
申请号：US14175
申请日：1998-02-27
申请人： Robert J. Wittenbrink , Charles W. DeGeorge
发明人： Robert J. Wittenbrink , Charles W. DeGeorge
IPC分类号： C10L3/10 , C01B3/48 , C01B3/56 , C10G45/02 , C10G49/00 , C10L3/06 , C07C1/04
CPC分类号： C10G49/007 , C01B3/48 , C01B3/56 , C10G45/02 , C10L3/06 , C01B2203/0283 , C01B2203/0415 , C01B2203/043 , C01B2203/0445 , C01B2203/0495 , C01B2203/062 , C01B2203/065 , C01B2203/0883 , C01B2203/1047 , C01B2203/1094 , C01B2203/1241 , C01B2203/1264 , C01B2203/127 , C01B2203/147 , C01B2203/148 , Y10S208/95
摘要： A gas conversion process comprising synthesis gas production, hydrocarbon synthesis and hydrogen production from the synthesis gas, also includes hydrodesulfurizing sulfur-containing hydrocarbon liquids separated from a mixture of natural gas and the liquids produced from a gas well. Hydrogen produced from the synthesis gas is used for the hydrodesulfurization, to remove at least a portion of the sulfur as H.sub.2 S and form desulfurized hydrocarbon liquid. The hydrogen is produced from the synthesis gas by one or more of (i) physical separation means such as pressure swing adsorption and (ii) chemical means such as a water gas shift reactor. The synthesized hydrocarbons are upgraded by hydroconversion. A portion of the hydrogen produced from the synthesis gas may also be used for at least one of (i) hydrocarbon synthesis catalyst rejuvenation and the hydroconversion.
摘要翻译：包括合成气生产，烃合成和来自合成气的氢气生产的气体转化方法还包括从天然气和由气井产生的液体的混合物中分离的含硫烃液体的加氢脱硫。由合成气产生的氢气用于加氢脱硫，将至少一部分硫作为H 2 S除去并形成脱硫烃液体。通过以下一种或多种（i）物理分离装置如变压吸附和（ii）化学方法如水煤气变换反应器，由合成气产生氢。合成的烃通过加氢转化来升级。从合成气产生的氢气的一部分也可以用于（i）烃合成催化剂再生和加氢转化中的至少一种。

3. 发明授权

US07119155B2 Polymerized catalyst composition II 失效
标题翻译：聚合催化剂组合物II
公开(公告)号：US07119155B2
公开(公告)日：2006-10-10
申请号：US10692902
申请日：2003-10-24
申请人： Stanley Wai-Yan Chow , Guo-Xin Jin , Zerong Lin , Robert J. Wittenbrink , Dao Zhang
发明人： Stanley Wai-Yan Chow , Guo-Xin Jin , Zerong Lin , Robert J. Wittenbrink , Dao Zhang
IPC分类号： C08F4/80
CPC分类号： B01J31/1658 , B01J31/143 , B01J31/223 , B01J31/2243 , B01J31/24 , B01J2231/122 , B01J2231/20 , B01J2531/847 , C07F15/04 , C07F15/045 , C07F15/06 , C07F15/065 , C08F10/00 , C08F10/02 , C08F110/02 , C08F212/08 , C08F2500/03 , C08F4/7022 , C08F4/80
摘要： Copolymerization of Ni(II) phenol imine complexes containing olefinic substituents on aryl groups with styrene in the presence of a radical initiator results in polymerized late transition metal catalysts which can be used for olefin polymerization or oligomerization. These catalysts have high catalyst activity for olefin polymerization or oligomerization.
摘要翻译：在自由基引发剂的存在下，在芳基上含有烯属取代基的Ni（II）苯酚亚胺络合物与苯乙烯的共聚合导致可用于烯烃聚合或低聚的聚合后期过渡金属催化剂。这些催化剂对于烯烃聚合或低聚反应具有高催化剂活性。

4. 发明授权

US06284806B1 Water emulsions of Fischer-Tropsch waxes 失效
标题翻译：费托蜡的水乳液
公开(公告)号：US06284806B1
公开(公告)日：2001-09-04
申请号：US08928237
申请日：1997-09-12
申请人： Tapan Chakrabarty , Robert J. Wittenbrink , Paul J. Berlowitz , Loren L. Ansell
发明人： Tapan Chakrabarty , Robert J. Wittenbrink , Paul J. Berlowitz , Loren L. Ansell
IPC分类号： B01F312
CPC分类号： C10L1/32 , Y10S516/924 , Y10S516/928 , Y10T137/0391
摘要： Hydrocarbon in water emulsions comprising Fischer-Tropsch process water, at least 20 to about 90 weight percent of a Fischer-Tropsch wax, a first nonionic surfactant having an HLB of at least 11 and a second nonionic surfactant having an HLB less than 11. Said emulsions are liquid at room temperature and pour by ordinary gravity. Also disclosed are methods of making said hydrocarbon in water emulsions.
摘要翻译：包含费 - 托工艺水，至少20至约90重量％的费 - 托蜡，HLB为至少11的第一非离子表面活性剂和HLB小于11的第二非离子表面活性剂的水包油乳液。乳液在室温下为液体，通过普通重力倾倒。还公开了制备所述烃水溶液乳液的方法。

5. 发明授权

US6103099A Production of synthetic lubricant and lubricant base stock without dewaxing 失效
标题翻译：合成润滑剂和润滑油基础油的生产，无需脱蜡
公开(公告)号：US6103099A
公开(公告)日：2000-08-15
申请号：US148282
申请日：1998-09-04
申请人： Robert J. Wittenbrink , Daniel F. Ryan , Douglas R. Boate
发明人： Robert J. Wittenbrink , Daniel F. Ryan , Douglas R. Boate
IPC分类号： C10G2/00 , C10G45/58 , C10G45/60 , C10M105/04 , C10N20/00 , C10N30/02 , C10N40/00 , C10N40/04 , C10N40/08 , C10N40/12 , C10N40/25 , C10N70/00 , C10G25/00
CPC分类号： B01J35/023 , C10G2300/1022 , C10G2300/202 , C10G2300/301 , C10G2300/80 , C10G2400/10 , Y10S208/95
摘要： A lubricating base stock useful for forming lubricants such as a multigrade automotive oils, automatic transmission oils, greases and the like is prepared by hydroisomerizing a waxy hydrocarbon feed fraction having an initial boiling point in the 650-750.degree. F. range and an end point of at least 1050.degree. F., synthesized by a slurry Fischer-Tropsch hydrocarbon synthesis process. The hydroisomerization forms a hydroisomerate containing the desired base stock which is recovered, without dewaxing the hydroisomerate. The hydroisomerization is conducted at conditions effective to convert at least 67 wt. % of the 650-750.degree. F.+ waxy feed hydrocarbons to lower boiling hydrocarbons. When combined with a standard lubricant additive package, these base stocks have been formed into multigrade automotive crankcase oils, transmission oils and hydraulic oils meeting the specifications for these oils.
摘要翻译：通过将初始沸点在650-750°F范围内的蜡质烃进料馏分加氢异构化，并且终点为止，制备用于形成诸如多级汽车油，自动变速器油，润滑脂等润滑剂的润滑基础油料至少1050°F，通过浆料费 - 托烃合成方法合成。加氢异构化形成含有所需原料的加氢异构体，其被回收，而不脱蜡加氢异构体。加氢异构化在有效转化至少67wt。％的650-750°F +蜡质原料烃转化为低沸点烃。当与标准润滑剂添加剂组合使用时，这些基础油已经形成符合这些油的规格的多级汽车曲轴箱油，变速箱油和液压油。

6. 发明授权

US6080301A Premium synthetic lubricant base stock having at least 95% non-cyclic isoparaffins 有权
标题翻译：具有至少95％非环状异链烷烃的优质合成润滑剂基础油料
公开(公告)号：US6080301A
公开(公告)日：2000-06-27
申请号：US148280
申请日：1998-09-04
申请人： Paul J. Berlowitz , Jacob J. Habeeb , Robert J. Wittenbrink
发明人： Paul J. Berlowitz , Jacob J. Habeeb , Robert J. Wittenbrink
IPC分类号： C10G67/04 , C10G2/00 , C10G45/58 , C10G45/60 , C10G45/62 , C10G45/64 , C10G65/04 , C10G67/00 , C10G73/06 , C10M105/04 , C10M111/00 , C10N20/00 , C10N70/00 , C10G71/00 , C07C7/20
CPC分类号： C10G2/00 , C10G2/30 , C10G2/32 , C10G2/332 , C10G45/60 , C10G45/64 , C10G65/04 , C10G67/04 , C10G2300/1022 , C10G2300/202 , C10G2300/301 , C10G2300/304 , C10G2400/10
摘要： A premium synthetic lubricating oil base stock having a high VI and low pour point is made by hydroisomerizing a Fischer-Tropsch synthesized waxy, paraffinic feed wax and then dewaxing the hydroisomerate to form a 650-750.degree. F.+ dewaxate. The waxy feed has an initial boiling point in the range of about 650-750.degree. F., from which it continuously boils up to at least 1050.degree. F. and has a T.sub.90 -T.sub.10 temperature difference of at least 350.degree. F. The feed is preferably hydroisomerized without any pretreatment, other than optional fractionation. The 650-750.degree. F.+ dewaxate is fractionated into two or more base stocks of different viscosity.
摘要翻译：具有高VI和低倾点的优质合成润滑油基础油料通过将费 - 托合成的蜡状，链烷烃进料蜡加氢异构化，然后脱蜡加氢异构体来形成650-750°F +脱蜡。蜡状原料的初始沸点在约650-750°F范围内，从而连续沸腾至至少1050°F，并具有至少350°F的T90-T10温度差。进料优选加氢异构化而不进行任何预处理，而不是任选分馏。将650-750°F +脱蜡剂分馏成两种或更多种不同粘度的基础油料。

7. 发明授权

US5756420A Supported hydroconversion catalyst and process of preparation thereof 失效
标题翻译：负载型加氢转化催化剂及其制备方法
公开(公告)号：US5756420A
公开(公告)日：1998-05-26
申请号：US740971
申请日：1996-11-05
申请人： Robert J. Wittenbrink , Daniel F. Ryan , William C. Baird, Jr. , Kenneth L. Riley , Jack W. Johnson
发明人： Robert J. Wittenbrink , Daniel F. Ryan , William C. Baird, Jr. , Kenneth L. Riley , Jack W. Johnson
IPC分类号： B01J23/85 , B01J23/885 , C10G45/60 , B01J23/70 , B01J23/72 , B01J23/74 , B01J23/75
CPC分类号： B01J23/85 , B01J23/885 , C10G45/60
摘要： Hydroconversion of paraffin containing hydrocarbon feeds is effected over a supported Group VIII and Group VI metal containing catalyst also containing a hydrocracking suppressant such as a Group IB metal, wherein the catalyst is preferably prepared by fixing the Group IB metal on to the support prior to incorporating the Group VI metal on to the support.
摘要翻译：含有烃的烃进料的加氢转化在含有还含有加氢裂化抑制剂如IB族金属的负载的第VIII族和第VI族金属催化剂上进行，其中催化剂优选通过将IB族金属固定在载体上而制备，第六组金属对支持。

8. 发明授权

US07319083B2 Polymerized catalyst composition 失效
标题翻译：聚合催化剂组合物
公开(公告)号：US07319083B2
公开(公告)日：2008-01-15
申请号：US10692900
申请日：2003-10-24
申请人： Guo-Xin Jin , Zerong Lin , Robert J. Wittenbrink , Chang-Kun Liu
发明人： Guo-Xin Jin , Zerong Lin , Robert J. Wittenbrink , Chang-Kun Liu
IPC分类号： C08F4/06 , B01J31/00
CPC分类号： B01J31/1815 , B01J2231/10 , B01J2531/0241 , B01J2531/842 , B01J2531/845 , C08F10/00 , C08F110/02 , C08F4/04 , C08F4/34 , C08F2/00 , C08F4/7042
摘要： A composition is provided that includes a product of combining, in the presence of a free radical initiator a catalyst precursor and at least one monomer wherein the monomer and the catalyst precursor are poiymerizable by free-radical polymerization and wherein the catalyst precursor compound is represented by the formula: wherein each X is an abstractable ligand; each R, R′, R″, R′″, Rp1 and Rp2 is independently hydrogen or a hydrocarbyl group provided at least one of Rp1, Rp2, and R′″ can be polymerized by a free radical initiator; and M is a Group-4-11 metal.
摘要翻译：提供了一种组合物，其包括在自由基引发剂存在下将催化剂前体与至少一种单体组合的产物，其中单体和催化剂前体可通过自由基聚合而聚合，并且其中催化剂前体化合物由其中每个X是可抽出的配体; 每个R，R'，R“，R”'，R“p1和R”p2“独立地是氢或提供至少一个R” p1，R p2，和R“'可以通过自由基引发剂聚合; M是4-11族金属。

9. 发明授权

US06776898B1 Process for softening fischer-tropsch wax with mild hydrotreating 有权
标题翻译：用轻度加氢处理软化费 - 托蜡的方法
公开(公告)号：US06776898B1
公开(公告)日：2004-08-17
申请号：US09542894
申请日：2000-04-04
申请人： Robert J. Wittenbrink , Daniel Francis Ryan
发明人： Robert J. Wittenbrink , Daniel Francis Ryan
IPC分类号： C10G4500
CPC分类号： C10G73/44
摘要： A novel process for forming hydrocarbon waxes from synthesis gas is disclosed. This invention teaches a process whereby a Fischer-Tropsch wax can be formulated such that the wax softness as defined by ASTM Standard Test Method for Needle Penetration of waxes (ASTM D-1321) can be adjusted to within a region most preferred for end use applications while simultaneously removing undesirable impurities, such as oxygenates (e.g., primary alcohols), olefins, and trace levels of aromatics. In a Fischer-Tropsch reactor, Fischer-Tropsch wax is formed from synthesis gas in a catalyzed reaction. The Fischer Tropsch wax is then subjected to a relatively mild hydroprocessing over a hydroisomerization catalyst under conditions such that essentially no boiling point conversion is obtained, but yet chemical conversions (e.g., hydrogenation and mild isomerization) occur yielding a high purity, hydrocarbon wax product of reduced hardness.
摘要翻译：公开了一种从合成气中形成烃蜡的新方法。本发明教导了一种方法，其中可以配制费 - 托蜡，使得ASTM标准测试方法针对蜡的渗透（ASTM D-1321）所定义的蜡柔软度可以调整到最适用于最终用途应用的区域内同时除去不需要的杂质，例如含氧化合物（例如伯醇），烯烃和痕量芳族化合物。在费 - 托反应器中，费 - 托蜡在催化反应中由合成气形成。然后在基本上不获得沸点转化率的条件下，在加氢异构化催化剂上进行相对温和的加氢处理，但是仍然发生化学转化（例如氢化和轻度异构化），产生高纯度烃蜡产物降低硬度。

10. 发明授权

US06245709B1 Supported Ni-Cu hydroconversion catalyst 失效
标题翻译：负载Ni-Cu加氢转化催化剂
公开(公告)号：US06245709B1
公开(公告)日：2001-06-12
申请号：US08918531
申请日：1997-08-22
申请人： Janet R. Clark , Robert J. Wittenbrink , Stephen M. Davis , Kenneth L. Riley
发明人： Janet R. Clark , Robert J. Wittenbrink , Stephen M. Davis , Kenneth L. Riley
IPC分类号： B01J2340
CPC分类号： C10G73/44 , B01J21/12 , B01J23/755 , B01J35/0026 , B01J35/1019 , B01J35/1038 , C10G1/002 , C10G45/60 , C10G47/12 , C10G65/00
摘要： Nickel-copper catalysts supported on an amorphous silica-alumina acidic carrier, preferably containing a binder, and having an iso-electric point of ≧6.5 are used to hydroisomerize paraffins, particularly Fischer-Tropsch paraffins, boiling at 350° F.+ into lighter, more valuable products.
摘要翻译：负载在无定形二氧化硅 - 氧化铝酸性载体上的镍铜催化剂，优选含有粘合剂，并且具有> = 6.5的等电点，用于将在350°F +沸腾的石蜡，特别是费 - 托石蜡加氢异构化更轻，更有价值的产品。

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