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1. 发明授权

US4879076A Process for the production of polyethylene materials 失效
标题翻译：聚乙烯材料生产工艺
公开(公告)号：US4879076A
公开(公告)日：1989-11-07
申请号：US061226
申请日：1987-06-12
申请人： Akira Sano , Seizo Kobayashi , Kazuo Matsuura , Shigeki Yokoyama , Takeshi Kamiya
发明人： Akira Sano , Seizo Kobayashi , Kazuo Matsuura , Shigeki Yokoyama , Takeshi Kamiya
IPC分类号： B29C55/30 , C08F110/02 , C08F297/08 , C08J5/18 , C08L23/06 , D01F6/04
CPC分类号： C08J5/18 , B29C55/30 , C08F110/02 , C08F297/083 , C08L23/06 , D01F6/04 , B29K2023/06 , C08J2323/06
摘要： A process for producing polyethylene materials is disclosed in which particulate polyethylene is drawn at lower temperatures than its melting point, the polymer having an intrinsic viscosity of 5-50 dl/g at 135.degree. C. in decalin and resulting from the polymerization of ethylene at temperatures below the above melting point and with use of a selected catalyst. The polyethylene materials excel in mechanical strength and elastic modulus.
摘要翻译：公开了一种生产聚乙烯材料的方法，其中颗粒聚乙烯在比其熔点低的温度下被拉伸，该聚合物在135℃下在十氢化萘中的特性粘度为5-50dl / g，并且由乙烯在温度低于上述熔点，并使用选定的催化剂。聚乙烯材料的机械强度和弹性模量优异。

2. 发明授权

US5026511A Process for the production of polyethylene materials 失效
标题翻译：聚乙烯材料生产工艺
公开(公告)号：US5026511A
公开(公告)日：1991-06-25
申请号：US485248
申请日：1990-02-26
申请人： Akira Sano , Hirofumi Kamiishi , Seizo Kobayashi , Kazuo Matsuura , Shigeki Yokoyama
发明人： Akira Sano , Hirofumi Kamiishi , Seizo Kobayashi , Kazuo Matsuura , Shigeki Yokoyama
IPC分类号： C08F4/64 , B29C55/00 , B29C55/18 , C08F4/60 , C08F4/685 , C08F110/00 , C08F110/02 , C08J5/18 , C08L23/06 , D01F6/04
CPC分类号： C08J5/18 , B29C55/005 , B29C55/18 , C08L23/06 , D01F6/04 , B29K2023/06 , C08J2323/06
摘要： A process for producing a polyethylene material for use in products requiring high mechanical strength and high elastic modulus is disclosed. The process involves the use of a specific class of particulate polyethylenes having an intrinsic viscosity of 5-50 dl/g in decalin at 135.degree. C. and the steps of compression molding, solvent immersing, solid-phase extruding or rolling and finally drawing the material in that order.

3. 发明授权

US5445883A Laminate 失效
标题翻译：层压板
公开(公告)号：US5445883A
公开(公告)日：1995-08-29
申请号：US272629
申请日：1994-07-11
申请人： Seizo Kobayashi , Takashi Mizoe , Yoshimu Iwanami , Shigeki Yokoyama , Keizi Jimbo
发明人： Seizo Kobayashi , Takashi Mizoe , Yoshimu Iwanami , Shigeki Yokoyama , Keizi Jimbo
IPC分类号： B32B27/32 , C09J7/02
CPC分类号： B32B27/32 , Y10S428/91 , Y10T428/2878 , Y10T428/31913 , Y10T428/31928
摘要： An anisotropy-free laminate having much higher strength and stiffness as compared with conventional articles is here disclosed which can be prepared by laminating an orientated ultra-high-molecular-weight polyethylene onto an adhesive layer obtained by modifying an olefin polymer with an unsaturated carboxylic acid and/or its derivative at a temperature lower than the melting point of the orientated ultra-high-molecular-weight polyethylene. The anisotropy-free material having high strength and high stiffness of the present invention can be substituted for various materials such as metals, lumber and FRP, and is also lightweight and excellent in water resistance.
摘要翻译：这里公开了与常规制品相比具有高得多的强度和刚度的无向异性层压材料，其可以通过将取向的超高分子量聚乙烯层压到通过用不饱和羧酸改性烯烃聚合物获得的粘合剂层上来制备和/或其衍生物在低于取向的超高分子量聚乙烯的熔点的温度下进行。本发明的具有高强度和高硬度的各向异性材料可以代替金属，木材和FRP等各种材料，并且重量轻且耐水性优异。

4. 发明授权

US5578373A Split polyethylene stretched material and process for producing the same 失效
标题翻译：分离聚乙烯拉伸材料及其制备方法
公开(公告)号：US5578373A
公开(公告)日：1996-11-26
申请号：US357089
申请日：1994-12-15
申请人： Seizo Kobayashi , Takashi Mizoe , Yoshimu Iwanami , Osamu Otsu , Shigeki Yokoyama , Kazuhiko Kurihara , Hiroshi Yazawa
发明人： Seizo Kobayashi , Takashi Mizoe , Yoshimu Iwanami , Osamu Otsu , Shigeki Yokoyama , Kazuhiko Kurihara , Hiroshi Yazawa
IPC分类号： B29C43/22 , B29C55/18 , B29D28/00 , D02G1/02 , D02G3/00 , B29K43/48
CPC分类号： B30B5/067 , B29C43/228 , B29C43/48 , B29C55/18 , B29D28/00 , B29C2043/483 , B29K2023/0683 , B29L2028/00 , Y10S264/47 , Y10S428/901 , Y10T428/2913 , Y10T428/2925
摘要： The present invention provides a split polyethylene stretched material having a tensile strength of at least 0.7 GPa when twisted in the range of 50-500 times/m, which material is produced by subjecting a polyethylene having an intrinsic viscosity of 5-50 dl/g as measured at 135.degree. C. in decalin, i.e. an ultra-high-molecular-weight polyethylene to stretching and then subjecting the stretched polyethylene to splitting, as well as a process for producing said material. The split polyethylene stretched material according to the present invention has a large surface area and accordingly can be easily laminated to other materials, and has a high strength and flexibility.
摘要翻译：本发明提供了一种裂解聚乙烯拉伸材料，其在50-500次/ m的范围内扭曲时的拉伸强度至少为0.7GPa，该材料通过使特性粘度为5-50dl / g的聚乙烯如在135℃下在十氢化萘中测量的，即超高分子量聚乙烯，以拉伸然后使拉伸的聚乙烯分裂，以及制备所述材料的方法。根据本发明的分裂聚乙烯拉伸材料具有大的表面积，因此可以容易地层压到其它材料上，并且具有高强度和柔韧性。

5. 发明授权

US5106555A Process for the continuous production of high-strength and high-modulus polyethylene material 失效
标题翻译：连续生产高强度和高模量聚乙烯材料的工艺
公开(公告)号：US5106555A
公开(公告)日：1992-04-21
申请号：US557654
申请日：1990-07-25
申请人： Seizo Kobayashi , Takashi Mizoe , Yoshimu Iwanami , Shigeki Yokoyama , Kazuhiko Kurihara , Hiroshi Yazawa , Mihoko Okada
发明人： Seizo Kobayashi , Takashi Mizoe , Yoshimu Iwanami , Shigeki Yokoyama , Kazuhiko Kurihara , Hiroshi Yazawa , Mihoko Okada
IPC分类号： B29C43/22 , B29C43/48 , B29C55/02 , B29C55/18 , B29K23/00
CPC分类号： B29C55/18 , B29C43/228 , B29C2043/483 , B29K2023/06
摘要： A process is provided for the continuous production of a high-strength and high-modulus polyethylene material having excellent properties. According to the process, powder composed of ultra-high-molecular-weight polyethylene powder as a principal component is subjected to compression molding, rolling and stretching. The polyethylene powder has an intrinsic viscosity of 5-50 dl/g as measured at 135.degree. C. in decalin. The compression molding is carried out by feeding the polyethylene powder between endless belts arranged in an opposing up-and-down relation, and conveying the polyethylene powder while holding the same between the endless belts and at the same time, continuously compression molding the polyethylene powder at a temperature lower than its melting point by a compressing means provided inside of the endless belts. In at least one of the compression molding step and rolling step, an olefin polymer having a molecular weight lower than the polyolefin polymer is concurrently processed.

6. 发明授权

US4071591A Method of manufacturing foamed thermoplastic resin profiles 失效
标题翻译：发泡热塑性树脂型材的制造方法
公开(公告)号：US4071591A
公开(公告)日：1978-01-31
申请号：US603766
申请日：1975-08-11
申请人： Seizo Kobayashi , Toshiharu Hirayama , Takeshi Kamiya , Seiju Kezuka , Hidesuke Takeuchi
发明人： Seizo Kobayashi , Toshiharu Hirayama , Takeshi Kamiya , Seiju Kezuka , Hidesuke Takeuchi
IPC分类号： B29C44/50 , B29D27/00
CPC分类号： B29C47/0042 , B29C44/50 , B29K2023/00 , B29K2025/00 , B29K2105/12 , B29K2105/24 , B29K2309/08 , Y10S264/14 , Y10S264/18
摘要： A method for producing foamed thermoplastic resin profiles with an outer skin layer of increased hardness and an inner foam structure which may be used in place of wooden articles. The outer skin has a smooth surface and a good appearance, and the inner portion enclosed by the skin has a uniform foam structure. Also, with this method an improved foaming efficiency can be obtained. The method comprises a step of melting and kneading a mixture consisting of a thermoplastic resin and a foaming agent without causing the gasification of the foaming agent, a step of heating the melted and kneaded mixture obtained in the previous step to cause the gasification of the foaming agent without agitating the mixture and under a pressure sufficient to supress the substantial foaming of the mixture, thereby forming an expandable melted resin mixture containing microbubbles which are prevented from gathering and uniting, and a third step of causing the melted resin obtained in the previous step to expand while cooling the resin by leading the resin to a foaming die under low temperature and low pressure conditions.
摘要翻译：一种生产发泡热塑性树脂轮廓的方法，其具有增加硬度的外层和可用于代替木制品的内泡沫结构。外皮具有光滑的表面和良好的外观，并且由皮肤包围的内部部分具有均匀的泡沫结构。此外，通过该方法，可以获得改善的发泡效率。该方法包括将由热塑性树脂和发泡剂组成的混合物熔融和捏合而不引起发泡剂气化的步骤，加热在前一步骤中获得的熔融和捏合的混合物以使发泡气化在不搅拌混合物的条件下，在足以抑制混合物的大量发泡的压力下，形成包含防止聚集和结合的微泡的可膨胀熔融树脂混合物，以及第三步骤，使上一步骤中获得的熔融树脂通过在低温低压条件下将树脂引入发泡模具来冷却树脂。

7. 发明授权

US4822855A Thermoplastic elastomer compositions 失效
标题翻译：热塑性弹性体组合物
公开(公告)号：US4822855A
公开(公告)日：1989-04-18
申请号：US81464
申请日：1987-08-04
申请人： Seizo Kobayashi , Katumi Usui , Takashi Mizoe , Noboru Yamaoka , Kazuo Matsuura
发明人： Seizo Kobayashi , Katumi Usui , Takashi Mizoe , Noboru Yamaoka , Kazuo Matsuura
IPC分类号： C08L23/00 , C08L23/08 , C08L23/10 , C08L23/12 , C08L23/14 , C08L23/16 , C08L53/00 , C08L23/28 , C08L23/18
CPC分类号： C08L23/10 , C08L23/12 , C08L23/16 , C08L2205/03 , C08L23/0815 , C08L23/142 , C08L2312/00 , C08L53/00
摘要： A thermoplastic elastomer composition prepared by partially crosslinking a composition comprising the following components (A), (B) and (C):(A) 30-70 parts by weight of an ethylene/.alpha.-olefin copolymer prepared by copolymerizing ethylene and an .alpha.-olefin having 3 to 12 carbon atoms in the presence of a catalyst comprising a solid component and an organoaluminum compound which solid component contains at least magnesium and titanium, said ethylene/.alpha.-olefin copolymer having the following properties (I) to (IV):______________________________________ (I) Melt index 0.01-100 g/10 min (II) Density 0.860-0.910 g/cm.sup.3 (III) Maximum peak not lower than 100.degree. C. temperature as measured according to a differential scanning calorimetry (DSC) (IV) Insolubles in boiling not less than 10 wt. % n-hexane ______________________________________ (B) 70-30 parts by weight of a propylene polymer; and(C) 70-200 parts by weight, based on 100 parts by weight of the components (A) and (B), of an ethylene/.alpha.-olefin copolymer rubber.
摘要翻译：通过部分交联包含以下组分（A），（B）和（C）的组合物制备的热塑性弹性体组合物：（A）30-70重量份通过乙烯共聚合制备的乙烯/α-烯烃共聚物所述乙烯/α-烯烃共聚物具有以下特性（I）至（IV），所述催化剂包含固体组分和有机铝化合物，所述有机铝化合物至少含有镁和钛，： - （I）熔体指数0.01-100g / 10min - （II）密度0.860-0.910g / cm3 - （III）最高峰不低于100℃ - 测量温度 - 根据差示扫描 - 量热法（DSC） - （Ⅳ）不溶物不溶于10重量％％ - 正己烷 - （B）70-30重量份丙烯聚合物; 和（C）基于100重量份的组分（A）和（B））为70-200重量份的乙烯/α-烯烃共聚物橡胶。

8. 发明授权

US4775722A Thermoplastic elastomer compositions 失效
标题翻译：热塑性弹性体组合物
公开(公告)号：US4775722A
公开(公告)日：1988-10-04
申请号：US91831
申请日：1987-09-01
申请人： Seizo Kobayashi , Katumi Usui , Takashi Mizoe , Noboru Yamaoka , Kazuo Matsuura
发明人： Seizo Kobayashi , Katumi Usui , Takashi Mizoe , Noboru Yamaoka , Kazuo Matsuura
IPC分类号： C08K5/14 , C08L23/00 , C08L23/08 , C08L23/10 , C08L23/12 , C08L23/14 , C08L23/16 , C08L53/00 , C08L23/26 , C08L23/04
CPC分类号： C08L23/0815 , C08L23/0869 , C08L23/10 , C08L23/12 , C08L23/142 , C08L23/16 , C08L2205/035 , C08L2207/04 , C08L2312/00 , C08L53/00
摘要： A thermoplastic elastomer composition prepared by partially crosslinking a composition comprising the following components (A), (B), (C) and (D):(A) 10-40% by weight of an ethylene/.alpha.-olefin copolymer prepared by copolymerizing ethylene and an .alpha.-olefin having 3 to 12 carbon atoms in the presence of a catalyst comprising a solid component and an organoaluminum compound which solid component contains at least magnesium and titanium, said ethylene/.alpha.-olefin copolymer having the following properties (I) to (IV):(I) Melt index: 0.01-50 g/10 min(II) Density: 0.860-0.910 g/cm.sup.3(III) Maximum peak temperature as measured according to a differential scanning calorimetry (DSC): not lower than 100.degree. C.(IV) Insolubles in boiling n-hexane: not less than 10 wt. %(B) 15-35% by weight of a propylene polymer;(C) 10-40% by weight of an ethylene/.alpha.-olefin copolymer rubber; and(D) 10-40% by weight of an ethylene/unsaturated monocarboxylic acid ester copolymer in which the carboxylate unit content is 2-10 mol %.
摘要翻译：通过将包含以下组分（A），（B），（C）和（D））的组合物部分交联制备的热塑性弹性体组合物：（A）10-40重量％的通过共聚制备的乙烯/α-烯烃共聚物乙烯和具有3至12个碳原子的α-烯烃，在包含固体组分和固体组分至少含有镁和钛的有机铝化合物的催化剂存在下，所述乙烯/α-烯烃共聚物具有以下性质（I）至（IV）：（I）熔融指数：0.01-50g / 10分钟（II）密度：0.860-0.910g / cm3（III）根据差示扫描量热法（DSC）测量的最大峰值温度：不低于 100℃（Ⅳ）沸腾正己烷不溶物不少于10wt。％（B）15-35重量％的丙烯聚合物; （C）10-40重量％的乙烯/α-烯烃共聚物橡胶; 和（D）10-40重量％的羧酸酯单元含量为2-10摩尔％的乙烯/不饱和一元羧酸酯共聚物。

9. 发明授权

US5612125A Process for producing prepreg 失效
标题翻译：生产预浸料的方法
公开(公告)号：US5612125A
公开(公告)日：1997-03-18
申请号：US354268
申请日：1994-12-12
申请人： Seizo Kobayashi , Kazutosi Nomiyama , Yoshimu Iwanami , Sumio Yoshida , Kazuhiko Kurihara , Hiroshi Yazawa
发明人： Seizo Kobayashi , Kazutosi Nomiyama , Yoshimu Iwanami , Sumio Yoshida , Kazuhiko Kurihara , Hiroshi Yazawa
IPC分类号： B29B11/16 , B29B15/08 , B29B15/12 , B29C55/02 , B29C55/18 , B29C70/50 , B29K105/06 , B29L7/00 , C08J5/04 , C08J5/24 , B29C70/10
CPC分类号： C08J5/04 , B29B15/122 , B29C43/228 , B29C43/48 , B29C55/18 , B29C70/504 , C08J5/24 , B29C2043/483 , B29K2023/0683 , Y10S264/47 , Y10S428/902 , Y10T442/291
摘要： The present invention provides a prepreg obtained by stretching a material including, as a main component, an ultra-high-molecular-weight polyethylene having an intrinsic viscosity of 5-50 dl/g as measured at 135.degree. C. in decalin, to a total draw ratio of at least 20, subjecting the resulting stretched polyethylene material to a splitting treatment, and impregnating the resulting material with a thermosetting resin, and a process for producing said prepreg. The split stretched polyethylene material has improved adhesion to the impregnant resin and can be used as a good base material for prepreg.
摘要翻译：本发明提供一种预浸料，其通过将包含作为主要成分的特性粘度为5-50dl / g的超高分子量聚乙烯在135℃下在十氢化萘中拉伸而获得，总拉伸比为至少20，对所得拉伸聚乙烯材料进行裂化处理，并用热固性树脂浸渍所得材料，以及制备所述预浸料的方法。分裂拉伸聚乙烯材料具有改善的对浸渍树脂的粘附性，并且可以用作预浸料的良好基材。

10. 发明授权

US5723388A Prepreg of ultra-high-molecular-weight polyethylene 失效
标题翻译：超高分子量聚乙烯预浸料
公开(公告)号：US5723388A
公开(公告)日：1998-03-03
申请号：US779841
申请日：1997-01-07
申请人： Seizo Kobayashi , Kazutosi Nomiyama , Yoshimu Iwanami , Sumio Yoshida , Kazuhiko Kurihara , Hiroshi Yazawa
发明人： Seizo Kobayashi , Kazutosi Nomiyama , Yoshimu Iwanami , Sumio Yoshida , Kazuhiko Kurihara , Hiroshi Yazawa
IPC分类号： B29B11/16 , B29B15/08 , B29B15/12 , B29C55/02 , B29C55/18 , B29C70/50 , B29K105/06 , B29L7/00 , C08J5/04 , C08J5/24 , B29C70/10
CPC分类号： C08J5/04 , B29B15/122 , B29C43/228 , B29C43/48 , B29C55/18 , B29C70/504 , C08J5/24 , B29C2043/483 , B29K2023/0683 , Y10S264/47 , Y10S428/902 , Y10T442/291
摘要： The present invention provides a prepreg obtained by stretching a material including, as a main component, an ultra-high-molecular-weight polyethylene having an intrinsic viscosity of 5-50 dl/g as measured at 135.degree. C. in decalin, to a total draw ratio of at least 20, subjecting the resulting stretched polyethylene material to a splitting treatment, and impregnating the resulting material with a thermosetting resin. The split stretched polyethylene material has improved adhesion to the impregnant resin and can be used as a good base material for prepreg.
摘要翻译：本发明提供一种预浸料，其通过将包含作为主要成分的特性粘度为5-50dl / g的超高分子量聚乙烯在135℃下在十氢化萘中拉伸而获得，总拉伸比至少为20，对所得拉伸聚乙烯材料进行裂化处理，并用热固性树脂浸渍所得材料。分裂拉伸聚乙烯材料具有改善的对浸渍树脂的粘附性，并且可以用作预浸料的良好基材。

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