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1. 发明授权

US6046128A Method of manufacturing catalyst for purifying exhaust gas 失效
标题翻译：制造废气净化催化剂的方法
公开(公告)号：US6046128A
公开(公告)日：2000-04-04
申请号：US117047
申请日：1998-07-27
申请人： Tadashi Kisen , Yoshimi Kawashima
发明人： Tadashi Kisen , Yoshimi Kawashima
IPC分类号： B01D53/86 , B01D53/94 , B01J29/40 , B01J29/46 , B01J29/82 , B01J27/14 , B01J8/00 , B01J21/00 , B01J29/18
CPC分类号： B01J29/46 , B01J29/40 , B01D2255/20738 , B01D2255/20746 , B01D2255/20761 , B01D53/8628 , B01D53/9418 , B01J2229/20 , B01J2229/40 , B01J29/82 , Y10S423/22 , Y10S423/23 , Y10S423/29 , Y10S423/34
摘要： A method of manufacturing a catalyst for purifying exhaust gas, the catalyst including a pentasil-type crystalline aluminosilicate catalyst carrier carrying thereon a copper component and a phosphorus component. The method is characterized by adding the catalyst carrier into a solution containing a copper component and a phosphorus component, or a buffer and having a predetermined pH adjusted with ammonia, and subsequently adding an acid to the solution so as to adjust the pH of the solution to 7.0 or less, to thereby incorporate the copper component and the phosphorus component into the catalyst carrier. According to the present invention, a catalyst for removing exhaust gases which is durable and which has a high NO.sub.X removal factor can be prepared in a stable manner.
摘要翻译： PCT No.PCT / JP96 / 03471 Sec。 371日期：1998年7月27日 102（e）1998年7月27日PCT PCT 1996年11月27日PCT公布。第WO98 / 23373号公报日期1998年6月4日制造用于净化废气的催化剂的方法，所述催化剂包括载有铜组分和磷组分的pentasil型结晶硅铝酸盐催化剂载体。该方法的特征在于将催化剂载体加入到含有铜成分和磷成分或缓冲液的溶液中，并用氨调节预定的pH，然后向溶液中加入酸以调节溶液的pH 至7.0以下，从而将铜成分和磷成分并入催化剂载体。根据本发明，可以以稳定的方式制备耐久且具有高NOX去除因子的废气去除催化剂。

2. 发明授权

US07670987B2 Reforming catalyst for hydrocarbon, method for producing hydrogen using such reforming catalyst, and fuel cell system 失效
标题翻译：烃的重整催化剂，使用这种重整催化剂生产氢的方法和燃料电池系统
公开(公告)号：US07670987B2
公开(公告)日：2010-03-02
申请号：US10589987
申请日：2005-02-17
申请人： Yoshimi Kawashima , Hiroshi Ohashi
发明人： Yoshimi Kawashima , Hiroshi Ohashi
IPC分类号： B01J23/00 , B01J23/10 , B01J23/32 , B01J23/56 , B01J23/44 , B01J23/42 , C01B3/26 , C01B3/12 , H01M8/04 , H01M8/18
CPC分类号： H01M8/0612 , B01J23/6562 , B01J37/0205 , C01B3/40 , C01B2203/0233 , C01B2203/0238 , C01B2203/0244 , C01B2203/0261 , C01B2203/0844 , C01B2203/1064 , C01B2203/1082 , C01B2203/142 , C01B2203/82 , Y02P20/52
摘要： A hydrocarbon reforming catalyst which maintains carrier strength even after a long-term thermal history and which exhibits high catalytic activity is prepared by causing at least one noble metal component selected from among a ruthenium component, a platinum component, a rhodium component, a palladium component, and an iridium component to be supported on a carrier containing manganese oxide, alumina, and at least one compound selected from among lanthanum oxide, cerium oxide, and zirconium oxide, or a carrier containing silicon oxide, manganese oxide, and alumina. By use of the reforming catalyst, hydrogen is produced through steam reforming (1), autothermal reforming (2), partial-oxidation reforming (3), or carbon dioxide reforming (4). A fuel cell system is constituted from a reformer employing the reforming catalyst, and a fuel cell employing, as a fuel, hydrogen produced by the reformer.
摘要翻译：通过使选自钌组分，铂组分，铑组分，钯组分中的至少一种贵金属组分，制备即使在长期热历史之后仍具有高催化活性的载体强度的烃重整催化剂以及负载在含有氧化锰，氧化铝和至少一种选自氧化镧，氧化铈和氧化锆中的化合物的载体上的铱组分，或含有氧化硅，氧化锰和氧化铝的载体。通过使用重整催化剂，通过蒸汽重整（1），自热重整（2），部分氧化重整（3）或二氧化碳重整（4）产生氢。燃料电池系统由使用重整催化剂的重整器和使用由重整器生产的氢气作为燃料的燃料电池构成。

3. 发明授权

US08343456B2 Reforming catalyst for hydrocarbon, method for producing hydrogen using such reforming catalyst, and fuel cell system 有权
标题翻译：烃的重整催化剂，使用这种重整催化剂生产氢的方法和燃料电池系统
公开(公告)号：US08343456B2
公开(公告)日：2013-01-01
申请号：US12647645
申请日：2009-12-28
申请人： Yoshimi Kawashima , Hiroshi Ohashi
发明人： Yoshimi Kawashima , Hiroshi Ohashi
IPC分类号： C01B3/26 , H01M8/06
CPC分类号： H01M8/0612 , B01J23/6562 , B01J37/0205 , C01B3/40 , C01B2203/0233 , C01B2203/0238 , C01B2203/0244 , C01B2203/0261 , C01B2203/0844 , C01B2203/1064 , C01B2203/1082 , C01B2203/142 , C01B2203/82 , Y02P20/52
摘要： A hydrocarbon reforming catalyst which maintains carrier strength even after a long-term thermal history and which exhibits high catalytic activity is prepared by causing at least one noble metal component selected from among a ruthenium component, a platinum component, a rhodium component, a palladium component, and an iridium component to be supported on a carrier containing manganese oxide, alumina, and at least one compound selected from among lanthanum oxide, cerium oxide, and zirconium oxide, or a carrier containing silicon oxide, manganese oxide, and alumina. By use of the reforming catalyst, hydrogen is produced through steam reforming (1), autothermal reforming (2), partial-oxidation reforming (3), or carbon dioxide reforming (4). A fuel cell system is constituted from a reformer employing the reforming catalyst, and a fuel cell employing, as a fuel, hydrogen produced by the reformer.
摘要翻译：通过使选自钌组分，铂组分，铑组分，钯组分中的至少一种贵金属组分，制备即使在长期热历史之后仍具有高催化活性的载体强度的烃重整催化剂以及负载在含有氧化锰，氧化铝和至少一种选自氧化镧，氧化铈和氧化锆中的化合物的载体上的铱组分，或含有氧化硅，氧化锰和氧化铝的载体。通过使用重整催化剂，通过蒸汽重整（1），自热重整（2），部分氧化重整（3）或二氧化碳重整（4）产生氢。燃料电池系统由使用重整催化剂的重整器和使用由重整器生产的氢气作为燃料的燃料电池构成。

4. 发明授权

US08088708B2 Catalyst precursor substance, and catalyst using the same 有权
标题翻译：催化剂前体物质和使用其的催化剂
公开(公告)号：US08088708B2
公开(公告)日：2012-01-03
申请号：US12594983
申请日：2008-04-02
申请人： Kozo Takatsu , Yoshimi Kawashima , Satoshi Nakai
发明人： Kozo Takatsu , Yoshimi Kawashima , Satoshi Nakai
IPC分类号： B01J23/00 , B01J23/60 , B01J23/72 , B01J23/02 , B01J23/06 , B01J23/70 , H01M8/22 , H01M8/06 , C01B31/20 , C01B3/16 , C01B3/18 , C10G25/00 , C10G45/04 , C10G45/60 , C10G29/00
CPC分类号： B01J35/006 , B01J23/80 , B01J35/002 , B01J35/1019 , B01J37/0009 , B01J37/03 , C01B3/16 , C01B3/326 , C01B2203/0233 , C01B2203/0283 , C01B2203/066 , C01B2203/1076 , C01B2203/1223 , C01B2203/1288 , H01M8/0618 , H01M8/0668 , Y02P20/52
摘要： The present invention provides a catalyst precursor substance containing copper, zinc, and aluminum and exhibiting an X-ray diffraction pattern having a broad peak at a specific interplanar spacing d (Å). The present invention also provides a method for producing the catalyst precursor substance by mixing a solution containing a copper salt, a zinc salt, and an aluminum salt with a solution containing an alkali metal hydroxide or an alkaline earth metal hydroxide, thereby forming a precipitate. In the present invention, a catalyst is prepared through calcining of the catalyst precursor; the catalyst is employed for water gas shift reaction; and carbon monoxide conversion is carried out by use of the catalyst. Thus, the present invention also provides a catalyst useful for water gas shift reaction, which exhibits high activity and durability and which, even when applied to a fuel cell, can be used for a long period of time with reduction in activity being suppressed; a carbon monoxide conversion method employing the catalyst; and a fuel cell system employing hydrogen produced through the carbon monoxide conversion method.
摘要翻译：本发明提供了含有铜，锌和铝的催化剂前体物质，并且具有在特定的晶面间距d（）下具有宽峰的X射线衍射图。本发明还提供了通过将含有铜盐，锌盐和铝盐的溶液与含有碱金属氢氧化物或碱土金属氢氧化物的溶液混合从而形成沉淀物来制备催化剂前体物质的方法。在本发明中，通过煅烧催化剂前体制备催化剂; 催化剂用于水煤气变换反应; 并且通过使用催化剂进行一氧化碳转化。因此，本发明还提供了可用于水煤气变换反应的催化剂，其具有高活性和耐久性，并且甚至当应用于燃料电池时可以长时间使用，同时抑制活性的降低; 使用该催化剂的一氧化碳转化方法; 以及使用通过一氧化碳转化法生产的氢的燃料电池系统。

5. 发明授权

US07776785B2 Catalyst for carbon monoxide conversion and method of carbon monoxide modification with the same 有权
标题翻译：一氧化碳转化催化剂和一氧化碳改性方法
公开(公告)号：US07776785B2
公开(公告)日：2010-08-17
申请号：US12445389
申请日：2007-10-10
申请人： Kozo Takatsu , Yoshimi Kawashima , Satoshi Nakai , Takashi Umeki
发明人： Kozo Takatsu , Yoshimi Kawashima , Satoshi Nakai , Takashi Umeki
IPC分类号： B01J23/06
CPC分类号： B01J23/80 , B01J23/002 , B01J35/002 , B01J35/006 , B01J35/1019 , B01J37/0009 , B01J37/03 , B01J2523/17 , B01J2523/27 , B01J2523/31 , C01B3/16 , C01B3/38 , C01B3/48 , C01B2203/0233 , C01B2203/0244 , C01B2203/0261 , C01B2203/0283 , C01B2203/066 , C01B2203/1058 , C01B2203/1064 , C01B2203/1241 , C01B2203/1247 , C01B2203/1258 , H01M8/0618 , Y02P20/52 , Y02P70/56
摘要： The invention provides a catalyst for carbon monoxide conversion, comprising from 10 to 90% by mass of a copper oxide ingredient, from 5 to 50% by mass of a zinc oxide ingredient and from 10 to 50% by mass of an aluminum oxide ingredient, and having a specific surface area of from 100 to 300 m2/g, a carbon monoxide adsorption of from 20 to 80 μmol/g, and a copper oxide crystallite diameter of at most 200 angstroms, as a catalyst suitable for carbon monoxide conversion for fully reducing carbon monoxide in the hydrogen gas obtained through reforming of a starting hydrocarbon material, for the purpose of enabling stable long-term operation of a fuel cell which uses hydrogen gas as a fuel and which is frequently and repeatedly started and stopped.
摘要翻译：本发明提供一氧化碳转化用催化剂，其含有10〜90质量％的氧化铜成分，5〜50质量％的氧化锌成分和10〜50质量％的氧化铝成分，比表面积为100〜300m2 / g，一氧化碳吸附量为20〜80μmol/ g，氧化铜微晶直径为200以下，作为适用于全部一氧化碳转化的催化剂为了能够使使用氢气作为燃料的燃料电池能够稳定地长期运行并且频繁且反复地开始和停止的目的，减少通过原料烃材料的重整获得的氢气中的一氧化碳。

6. 发明申请

US20100112397A1 CATALYST PRECURSOR SUBSTANCE, AND CATALYST USING THE SAME 有权
标题翻译：催化剂前体物质和使用该催化剂的催化剂
公开(公告)号：US20100112397A1
公开(公告)日：2010-05-06
申请号：US12594983
申请日：2008-04-02
申请人： Kozo Takatsu , Yoshimi Kawashima , Satoshi Nakai
发明人： Kozo Takatsu , Yoshimi Kawashima , Satoshi Nakai
IPC分类号： B01J23/06 , B01D53/62 , H01M8/06 , B01J23/72
CPC分类号： B01J35/006 , B01J23/80 , B01J35/002 , B01J35/1019 , B01J37/0009 , B01J37/03 , C01B3/16 , C01B3/326 , C01B2203/0233 , C01B2203/0283 , C01B2203/066 , C01B2203/1076 , C01B2203/1223 , C01B2203/1288 , H01M8/0618 , H01M8/0668 , Y02P20/52
摘要： The present invention provides a catalyst precursor substance containing copper, zinc, and aluminum and exhibiting an X-ray diffraction pattern having a broad peak at a specific interplanar spacing d (Å). The present invention also provides a method for producing the catalyst precursor substance by mixing a solution containing a copper salt, a zinc salt, and an aluminum salt with a solution containing an alkali metal hydroxide or an alkaline earth metal hydroxide, thereby forming a precipitate. In the present invention, a catalyst is prepared through calcining of the catalyst precursor; the catalyst is employed for water gas shift reaction; and carbon monoxide conversion is carried out by use of the catalyst. Thus, the present invention also provides a catalyst useful for water gas shift reaction, which exhibits high activity and durability and which, even when applied to a fuel cell, can be used for a long period of time with reduction in activity being suppressed; a carbon monoxide conversion method employing the catalyst; and a fuel cell system employing hydrogen produced through the carbon monoxide conversion method.
摘要翻译：本发明提供了含有铜，锌和铝的催化剂前体物质，并且具有在特定的晶面间距d（）下具有宽峰的X射线衍射图。本发明还提供了通过将含有铜盐，锌盐和铝盐的溶液与含有碱金属氢氧化物或碱土金属氢氧化物的溶液混合从而形成沉淀物来制备催化剂前体物质的方法。在本发明中，通过煅烧催化剂前体制备催化剂; 催化剂用于水煤气变换反应; 并且通过使用催化剂进行一氧化碳转化。因此，本发明还提供了可用于水煤气变换反应的催化剂，其具有高活性和耐久性，并且甚至当应用于燃料电池时可以长时间使用，同时抑制活性的降低; 使用该催化剂的一氧化碳转化方法; 以及使用通过一氧化碳转化法生产的氢的燃料电池系统。

7. 发明授权

US5422333A Exhaust gas purifying catalyst 失效
标题翻译：废气净化催化剂
公开(公告)号：US5422333A
公开(公告)日：1995-06-06
申请号：US110377
申请日：1993-08-23
申请人： Yasuhide Kano , Yoshimi Kawashima , Toshiaki Hayasaka , Hiroshi Akama
发明人： Yasuhide Kano , Yoshimi Kawashima , Toshiaki Hayasaka , Hiroshi Akama
IPC分类号： B01D53/86 , B01D53/94 , B01J29/46 , B01J29/04
CPC分类号： B01J29/46 , B01D53/9418 , B01D2255/20761 , B01D2255/50
摘要： An exhaust gas purification catalyst of high resistance which allows highly effective purification of nitric oxide into nontoxic gas, even for an exhaust gas containing oxygen at a high concentration. A carrier of the catalyst includes crystalline pentasil-type aluminosilicate and supports copper and phosphori, the amount of the phosphori being supported ranges from 0.01% to 6.0% by weight as a conversion to P.sub.2 O.sub.5, and ratio of the phosphorus to the copper, i.e., P/Cu (molar ratio) is in 0
摘要翻译：一种高电阻的排气净化催化剂，即使对于含有高浓度氧的废气也能高效地将一氧化氮纯化成无毒气体。催化剂的载体包括结晶pentasil型硅铝酸盐并且支持铜和磷，所支持的磷的量为作为P 2 O 5的转化率的0.01重量％至6.0重量％，以及磷与铜的比例，即， P / Cu（摩尔比）为0 <（P / Cu）≤0.7。在氧化气氛中，在200-800℃的反应温度下，在总体THC浓度/ NOx浓度为0.5-50的烃存在下，在排气中还原和除去氮氧化物的方法。

8. 发明申请

US20100172826A1 REFORMING CATALYST FOR HYDROCARBON, METHOD FOR PRODUCING HYDROGEN USING SUCH REFORMING CATALYST, AND FUEL CELL SYSTEM 有权
标题翻译：烃改性催化剂，使用这种改性催化剂生产氢的方法和燃料电池系统
公开(公告)号：US20100172826A1
公开(公告)日：2010-07-08
申请号：US12647645
申请日：2009-12-28
申请人： Yoshimi KAWASHIMA , Hiroshi OHASHI
发明人： Yoshimi KAWASHIMA , Hiroshi OHASHI
IPC分类号： C01B3/02
CPC分类号： H01M8/0612 , B01J23/6562 , B01J37/0205 , C01B3/40 , C01B2203/0233 , C01B2203/0238 , C01B2203/0244 , C01B2203/0261 , C01B2203/0844 , C01B2203/1064 , C01B2203/1082 , C01B2203/142 , C01B2203/82 , Y02P20/52
摘要： A hydrocarbon reforming catalyst which maintains carrier strength even after a long-term thermal history and which exhibits high catalytic activity is prepared by causing at least one noble metal component selected from among a ruthenium component, a platinum component, a rhodium component, a palladium component, and an iridium component to be supported on a carrier containing manganese oxide, alumina, and at least one compound selected from among lanthanum oxide, cerium oxide, and zirconium oxide, or a carrier containing silicon oxide, manganese oxide, and alumina. By use of the reforming catalyst, hydrogen is produced through steam reforming (1), autothermal reforming (2), partial-oxidation reforming (3), or carbon dioxide reforming (4). A fuel cell system is constituted from a reformer employing the reforming catalyst, and a fuel cell employing, as a fuel, hydrogen produced by the reformer.
摘要翻译：通过使选自钌组分，铂组分，铑组分，钯组分中的至少一种贵金属组分，制备即使在长期热历史之后仍具有高催化活性的载体强度的烃重整催化剂以及负载在含有氧化锰，氧化铝和至少一种选自氧化镧，氧化铈和氧化锆中的化合物的载体上的铱组分，或含有氧化硅，氧化锰和氧化铝的载体。通过使用重整催化剂，通过蒸汽重整（1），自热重整（2），部分氧化重整（3）或二氧化碳重整（4）产生氢。燃料电池系统由使用重整催化剂的重整器和使用由重整器生产的氢气作为燃料的燃料电池构成。

9. 发明申请

US20070172416A1 Reforming catalyst for hydrocarbon, method for producing hydrogen using such reforming catalyst, and fuel cell system 失效
标题翻译：烃的重整催化剂，使用这种重整催化剂生产氢的方法和燃料电池系统
公开(公告)号：US20070172416A1
公开(公告)日：2007-07-26
申请号：US10589987
申请日：2005-02-17
申请人： Yoshimi Kawashima , Hiroshi Ohashi
发明人： Yoshimi Kawashima , Hiroshi Ohashi
IPC分类号： C01B3/02 , C01B3/26 , B01J21/00 , B01J23/00 , B01J23/10 , H01M8/06
CPC分类号： H01M8/0612 , B01J23/6562 , B01J37/0205 , C01B3/40 , C01B2203/0233 , C01B2203/0238 , C01B2203/0244 , C01B2203/0261 , C01B2203/0844 , C01B2203/1064 , C01B2203/1082 , C01B2203/142 , C01B2203/82 , Y02P20/52
摘要： A hydrocarbon reforming catalyst which maintains carrier strength even after a long-term thermal history and which exhibits high catalytic activity is prepared by causing at least one noble metal component selected from among a ruthenium component, a platinum component, a rhodium component, a palladium component, and an iridium component to be supported on a carrier containing manganese oxide, alumina, and at least one compound selected from among lanthanum oxide, cerium oxide, and zirconium oxide, or a carrier containing silicon oxide, manganese oxide, and alumina. By use of the reforming catalyst, hydrogen is produced through steam reforming (1), autothermal reforming (2), partial-oxidation reforming (3), or carbon dioxide reforming (4). A fuel cell system is constituted from a reformer employing the reforming catalyst, and a fuel cell employing, as a fuel, hydrogen produced by the reformer.
摘要翻译：通过使选自钌组分，铂组分，铑组分，钯组分中的至少一种贵金属组分，制备即使在长期热历史之后仍具有高催化活性的载体强度的烃重整催化剂以及负载在含有氧化锰，氧化铝和至少一种选自氧化镧，氧化铈和氧化锆中的化合物的载体上的铱组分，或含有氧化硅，氧化锰和氧化铝的载体。通过使用重整催化剂，通过蒸汽重整（1），自热重整（2），部分氧化重整（3）或二氧化碳重整（4）产生氢。燃料电池系统由使用重整催化剂的重整器和使用由重整器生产的氢气作为燃料的燃料电池构成。

10. 发明申请

US20100015023A1 CATALYST FOR CARBON MONOXIDE CONVERSION AND METHOD OF CARBON MONOXIDE MODIFICATION WITH THE SAME 有权
标题翻译：一氧化碳转化催化剂及其一氧化碳修饰方法
公开(公告)号：US20100015023A1
公开(公告)日：2010-01-21
申请号：US12445389
申请日：2007-10-10
申请人： Kozo Takatsu , Yoshimi Kawashima , Satoshi Nakai , Takashi Umeki
发明人： Kozo Takatsu , Yoshimi Kawashima , Satoshi Nakai , Takashi Umeki
IPC分类号： B01D53/62 , B01J23/80
CPC分类号： B01J23/80 , B01J23/002 , B01J35/002 , B01J35/006 , B01J35/1019 , B01J37/0009 , B01J37/03 , B01J2523/17 , B01J2523/27 , B01J2523/31 , C01B3/16 , C01B3/38 , C01B3/48 , C01B2203/0233 , C01B2203/0244 , C01B2203/0261 , C01B2203/0283 , C01B2203/066 , C01B2203/1058 , C01B2203/1064 , C01B2203/1241 , C01B2203/1247 , C01B2203/1258 , H01M8/0618 , Y02P20/52 , Y02P70/56
摘要： The invention provides a catalyst for carbon monoxide conversion, comprising from 10 to 90% by mass of a copper oxide ingredient, from 5 to 50% by mass of a zinc oxide ingredient and from 10 to 50% by mass of an aluminum oxide ingredient, and having a specific surface area of from 100 to 300 m2/g, a carbon monoxide adsorption of from 20 to 80 μmol/g, and a copper oxide crystallite diameter of at most 200 angstroms, as a catalyst suitable for carbon monoxide conversion for fully reducing carbon monoxide in the hydrogen gas obtained through reforming of a starting hydrocarbon material, for the purpose of enabling stable long-term operation of a fuel cell which uses hydrogen gas as a fuel and which is frequently and repeatedly started and stopped.
摘要翻译：本发明提供一氧化碳转化用催化剂，其含有10〜90质量％的氧化铜成分，5〜50质量％的氧化锌成分和10〜50质量％的氧化铝成分，比表面积为100〜300m2 / g，一氧化碳吸附量为20〜80mumol / g，氧化铜微晶直径为200以下，作为适用于全部一氧化碳转化的催化剂为了能够使使用氢气作为燃料的燃料电池能够稳定地长期运行并且频繁且反复地开始和停止的目的，减少通过原料烃材料的重整获得的氢气中的一氧化碳。

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