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1. 发明申请

US20060134527A1 Long life lithium batteries with stabilized electrodes 有权
公开(公告)号：US20060134527A1
公开(公告)日：2006-06-22
申请号：US11297120
申请日：2005-12-08
申请人： Khalil Amine , Jun Liu , Donald Vissers , Wenquan Lu
发明人： Khalil Amine , Jun Liu , Donald Vissers , Wenquan Lu
IPC分类号： H01M10/40
CPC分类号： H01M10/0567 , H01M4/13 , H01M4/366 , H01M4/505 , H01M4/5825 , H01M10/052 , H01M10/0525 , H01M10/0568 , H01M10/0569
摘要： The present invention relates to non-aqueous electrolytes having electrode stabilizing additives, stabilized electrodes, and electrochemical devices containing the same. Thus the present invention provides electrolytes containing an alkali metal salt, a polar aprotic solvent, and an electrode stabilizing additive. In some embodiments the additives include a substituted or unsubstituted cyclic or spirocyclic hydrocarbon containing at least one oxygen atom and at least one alkenyl or alkynyl group. When used in electrochemical devices with, e.g., lithium manganese oxide spinel electrodes or olivine or carbon-coated olivine electrodes, the new electrolytes provide batteries with improved calendar and cycle life.

2. 发明授权

US09012096B2 Long life lithium batteries with stabilized electrodes 有权
标题翻译：长寿命的锂电池具有稳定的电极
公开(公告)号：US09012096B2
公开(公告)日：2015-04-21
申请号：US11338902
申请日：2006-01-24
申请人： Khalil Amine , Jun Liu , Donald R. Vissers , Wenquan Lu
发明人： Khalil Amine , Jun Liu , Donald R. Vissers , Wenquan Lu
IPC分类号： H01M10/0567 , H01M10/0568 , H01M10/0569
CPC分类号： H01M10/0567 , H01M10/0568 , H01M10/0569
摘要： The present invention relates to non-aqueous electrolytes having electrode stabilizing additives, stabilized electrodes, and electrochemical devices containing the same. Thus the present invention provides electrolytes containing an alkali metal salt, a polar aprotic solvent, and an electrode stabilizing additive. In certain electrolytes, the alkali metal salt is a bis(chelato)borate and the additives include substituted or unsubstituted linear, branched or cyclic hydrocarbons comprising at least one oxygen atom and at least one aryl, alkenyl or alkynyl group. In other electrolytes, the additives include a substituted aryl compound or a substituted or unsubstituted heteroaryl compound wherein the additive comprises at least one oxygen atom. There are also provided methods of making the electrolytes and batteries employing the electrolytes. The invention also provides for electrode materials. Cathodes of the present invention may be further stabilized by surface coating the particles of the spinel or olivine with a material that can neutralize acid or otherwise lessen or prevent leaching of the manganese or iron ions. In some embodiments the coating is polymeric and in other embodiments the coating is a metal oxide such as ZrO2, TiO2, ZnO, WO3, Al2O3, MgO, SiO2, SnO2 AlPO4, Al(OH)3, a mixture of any two or more thereof.
摘要翻译：本发明涉及具有电极稳定添加剂，稳定电极和含有这些电极的电化学装置的非水电解质。因此，本发明提供了含有碱金属盐，极性非质子溶剂和电极稳定添加剂的电解质。在某些电解质中，碱金属盐是双（螯合）硼酸盐，并且添加剂包括取代或未取代的包含至少一个氧原子和至少一个芳基，烯基或炔基的直链，支链或环状烃。在其他电解质中，添加剂包括取代的芳基化合物或取代或未取代的杂芳基化合物，其中添加剂包含至少一个氧原子。还提供了使用电解质的电解质和电池的制造方法。本发明还提供电极材料。通过用可以中和酸或以其它方式减少或防止锰或铁离子浸出的材料表面涂覆尖晶石或橄榄石的颗粒，可以进一步稳定本发明的阴极。在一些实施方案中，涂层是聚合物，并且在其它实施方案中，涂层是诸如ZrO 2，TiO 2，ZnO，WO 3，Al 2 O 3，MgO，SiO 2，SnO 2，AlPO 4，Al（OH）3的金属氧化物，其任何两种或更多种的混合物。

3. 发明申请

US20110104551A1 NANOTUBE COMPOSITE ANODE MATERIALS SUITABLE FOR LITHIUM ION BATTERY APPLICATIONS 审中-公开
标题翻译：用于锂离子电池应用的纳米复合阳极材料
公开(公告)号：US20110104551A1
公开(公告)日：2011-05-05
申请号：US12938638
申请日：2010-11-03
申请人： Junbing YANG , Wenquan LU
发明人： Junbing YANG , Wenquan LU
IPC分类号： H01M4/485 , H01M10/26 , H01M4/58 , H01M4/56 , H01M4/60 , H01M4/525 , H01M4/54 , H01M4/583 , H01M6/42 , B82Y30/00
CPC分类号： H01M10/052 , B82Y30/00 , H01M4/133 , H01M4/134 , H01M4/137 , H01M4/38 , H01M4/40 , H01M4/44 , H01M4/46 , H01M4/583 , H01M4/587 , H01M4/60
摘要： The present invention provides a composite material suitable for use in an anode for a lithium ion battery, the composite material comprising a layer of a lithium-alloying material on the walls of an aligned nanotubular base material. Preferably, the lithium-alloying material comprises a material selected from the group consisting of Si, Sn, Pb, Al, Au, Pt, Zn, Cd, Ag, Mg, and a combination of two or more of the foregoing.
摘要翻译：本发明提供一种适合用于锂离子电池的阳极的复合材料，该复合材料包括在合适的纳米管基材的壁上的锂合金材料层。优选地，锂合金材料包括选自由Si，Sn，Pb，Al，Au，Pt，Zn，Cd，Ag，Mg组成的组的材料，以及上述两种或更多种的组合。

4. 发明授权

US07507503B2 Long life lithium batteries with stabilized electrodes 有权
标题翻译：长寿命的锂电池具有稳定的电极
公开(公告)号：US07507503B2
公开(公告)日：2009-03-24
申请号：US11297120
申请日：2005-12-08
申请人： Khalil Amine , Jun Liu , Donald R. Vissers , Wenquan Lu
发明人： Khalil Amine , Jun Liu , Donald R. Vissers , Wenquan Lu
IPC分类号： H01M6/16
CPC分类号： H01M10/0567 , H01M4/13 , H01M4/366 , H01M4/505 , H01M4/5825 , H01M10/052 , H01M10/0525 , H01M10/0568 , H01M10/0569
摘要： The present invention relates to non-aqueous electrolytes having electrode stabilizing additives, stabilized electrodes, and electrochemical devices containing the same. Thus the present invention provides electrolytes containing an alkali metal salt, a polar aprotic solvent, and an electrode stabilizing additive. In some embodiments the additives include a substituted or unsubstituted cyclic or spirocyclic hydrocarbon containing at least one oxygen atom and at least one alkenyl or alkynyl group. When used in electrochemical devices with, e.g., lithium manganese oxide spinel electrodes or olivine or carbon-coated olivine electrodes, the new electrolytes provide batteries with improved calendar and cycle life.
摘要翻译：本发明涉及具有电极稳定添加剂，稳定电极和含有这些电极的电化学装置的非水电解质。因此，本发明提供了含有碱金属盐，极性非质子溶剂和电极稳定添加剂的电解质。在一些实施方案中，添加剂包括含有至少一个氧原子和至少一个烯基或炔基的取代或未取代的环状或螺环烃。当用于具有例如锂锰氧化物尖晶石电极或橄榄石或碳涂覆的橄榄石电极的电化学装置中时，新的电解质提供具有改善的日历和循环寿命的电池。

5. 发明申请

US20060147809A1 Long life lithium batteries with stabilized electrodes 有权
标题翻译：长寿命的锂电池具有稳定的电极
公开(公告)号：US20060147809A1
公开(公告)日：2006-07-06
申请号：US11338902
申请日：2006-01-24
申请人： Khalil Amine , Jun Liu , Donald Vissers , Wenquan Lu
发明人： Khalil Amine , Jun Liu , Donald Vissers , Wenquan Lu
IPC分类号： H01M10/40
CPC分类号： H01M10/0567 , H01M10/0568 , H01M10/0569
摘要： The present invention relates to non-aqueous electrolytes having electrode stabilizing additives, stabilized electrodes, and electrochemical devices containing the same. Thus the present invention provides electrolytes containing an alkali metal salt, a polar aprotic solvent, and an electrode stabilizing additive. In certain electrolytes, the alkali metal salt is a bis(chelato)borate and the additives include substituted or unsubstituted linear, branched or cyclic hydrocarbons comprising at least one oxygen atom and at least one aryl, alkenyl or alkynyl group. In other electrolytes, the additives include a substituted aryl compound or a substituted or unsubstituted heteroaryl compound wherein the additive comprises at least one oxygen atom. There are also provided methods of making the electrolytes and batteries employing the electrolytes. The invention also provides for electrode materials. Cathodes of the present invention may be further stabilized by surface coating the particles of the spinel or olivine with a material that can neutralize acid or otherwise lessen or prevent leaching of the manganese or iron ions. In some embodiments the coating is polymeric and in other embodiments the coating is a metal oxide such as ZrO2, TiO2, ZnO, WO3, Al2O3, MgO, SiO2, SnO2 AlPO4, Al(OH)3, a mixture of any two or more thereof.
摘要翻译：本发明涉及具有电极稳定添加剂，稳定电极和含有这些电极的电化学装置的非水电解质。因此，本发明提供了含有碱金属盐，极性非质子溶剂和电极稳定添加剂的电解质。在某些电解质中，碱金属盐是双（螯合）硼酸盐，并且添加剂包括取代或未取代的包含至少一个氧原子和至少一个芳基，烯基或炔基的直链，支链或环状烃。在其他电解质中，添加剂包括取代的芳基化合物或取代或未取代的杂芳基化合物，其中添加剂包含至少一个氧原子。还提供了使用电解质的电解质和电池的制造方法。本发明还提供电极材料。通过用可以中和酸或以其它方式减少或防止锰或铁离子浸出的材料表面涂覆尖晶石或橄榄石的颗粒，可以进一步稳定本发明的阴极。在一些实施方案中，涂层是聚合物，在其它实施方案中，涂层是金属氧化物，例如ZrO 2，TiO 2，ZnO，WO 3，，Al 2 O 3，MgO，SiO 2，SnO 2，AlPO 4，N 2 O 3，，Al（OH）3 N 3，其中任何两种或更多种的混合物。

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