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1. 发明申请

US20120059209A1 PROCESS FOR THE CONTINUOUS HYDROGENATION OF TRIGLYCERIDE CONTAINING RAW MATERIALS USING A NICKEL AND MOLYBDENUM-BASED CATALYST 有权
标题翻译：使用镍和基于钼的催化剂连续加氢含有原料的TRIGLYCERIDE
公开(公告)号：US20120059209A1
公开(公告)日：2012-03-08
申请号：US13226524
申请日：2011-09-07
申请人： Thierry CHAPUS , Nathalie Dupassieux , Antoine Daudin
发明人： Thierry CHAPUS , Nathalie Dupassieux , Antoine Daudin
IPC分类号： C07C1/207
CPC分类号： C10G3/60 , C10G3/46 , C10G3/50 , C10G3/54 , C10G2300/1014 , C10G2300/4018 , C10G2300/802 , C10G2400/04 , C10G2400/08 , C10L1/08 , Y02E50/13 , Y02P30/20
摘要： Process for the continuous hydrogenation of triglyceride containing raw materials in a fixed bed reactor system having several catalyst beds arranged in series and comprising at least e hydrogenation catalyst comprising an active phase constituted by a nickel and molybdenum element. The raw material feed, hydrogen containing gas and diluting agent are passed together through the catalyst beds at hydrogenation conditions. The raw material feed stream as well as the stream of hydrogen containing gas are divided into an equal number of different partial streams. These are each passed to one catalyst bed in such a manner that the weight ratio of diluting agent to raw material feed is essentially the same at the entrance of all catalyst beds and does not exceed 4:1. The claimed process is preferably conducted at low temperatures and allows the utilization of existing units due to the low recycle ratio.
摘要翻译：在具有串联排列的几个催化剂床的至少包含由镍和钼元素构成的活性相的至少e氢化催化剂的固定床反应器系统中连续氢化含甘油三酯的原料的方法。原料进料，含氢气体和稀释剂在氢化条件下通过催化剂床一起通入。将原料进料流以及含氢气流分成相等数量的不同部分流。将它们分别传送到一个催化剂床，使得稀释剂与原料进料的重量比在所有催化剂床的入口处基本相同，不超过4:1。要求保护的方法优选在低温下进行，并且由于低回收比而允许使用现有的单元。

2. 发明申请

US20110094149A1 METHOD OF HYDROTREATING FEEDS FROM RENEWABLE SOURCES WITH INDIRECT HEATING USING A CATALYST BASED ON MOLYBDENUM 审中-公开
标题翻译：使用基于钼的催化剂对具有间接加热的可再生来源的进料进行加氢的方法
公开(公告)号：US20110094149A1
公开(公告)日：2011-04-28
申请号：US12912025
申请日：2010-10-26
申请人： Wilfried Weiss , Laurent Bournay , Thierry Chapus , Antoine Daudin
发明人： Wilfried Weiss , Laurent Bournay , Thierry Chapus , Antoine Daudin
IPC分类号： C10L1/188
CPC分类号： C10G65/04 , C10G3/46 , C10G3/48 , C10G3/50 , C10G2300/1014 , C10G2300/1018 , C10G2300/4006 , C10G2300/4081 , Y02P30/20
摘要： The invention describes a method of treating feeds from renewable sources comprising a hydrotreatment stage comprising at least two catalytic zones in which the entry stream comprising said feed mixed with at least a part of a hydrotreated liquid effluent from stage b) is introduced into the first catalytic zone at a temperature comprised between 150 and 260° C., and the effluent from the first catalytic zone is then introduced, mixed with at least a part of a hydrotreated liquid effluent from stage b) and preheated, into the following catalytic zone or zones at a temperature comprised between 260 and 320° C., and a stage of separation of the effluent from the hydrotreatment stage permitting the separation of a gaseous effluent and a hydrotreated liquid effluent of which at least a part is recycled at the top of each catalytic zone, said method using, in at least the catalytic zone or zones following the first, a bulk or supported catalyst comprising an active phase constituted by a sulphidized group VIB element, the group VIB element being molybdenum.
摘要翻译：本发明描述了一种处理来自可再生来源的饲料的方法，该方法包括加氢处理阶段，该加氢处理阶段包括至少两个催化区，其中将包含所述进料的进料与至少一部分来自步骤b）的加氢处理液体流出物混合进入第一催化剂区域，然后引入来自第一催化区域的流出物，与来自阶段b）的加氢处理的液体流出物的至少一部分混合并预热到以下催化区或区域在260至320℃之间的温度下，流出物与加氢处理阶段的分离阶段允许分离气态流出物和加氢处理的液体流出物，其中至少一部分在每个催化剂的顶部被再循环所述方法在至少在第一个催化区域之后使用主体或负载的催化剂，其包含由硫化VIB族元素，VIB族元素为钼。

3. 发明授权

US06855246B2 Process and apparatus employing a plurality of catalytic beds in series for the production of low sulphur gas oil 失效
标题翻译：使用多个催化床串联制备低硫瓦斯油的方法和装置
公开(公告)号：US06855246B2
公开(公告)日：2005-02-15
申请号：US09780418
申请日：2001-02-12
申请人： Thierry Chapus , Frédéric Morel
发明人： Thierry Chapus , Frédéric Morel
IPC分类号： C10G45/08 , C10G65/04 , C10G67/02 , C10G45/04
CPC分类号： C10G65/04
摘要： A process for hydrotreating gas oil comprises: a first gas oil desulfurization step carried out in a first catalytic zone comprising a desulfurization catalyst; at least partial elimination of the hydrogen sulphide formed at the end of the first gas oil desulfurization step; one or more additional desulfurization steps carried out in one or more catalytic zones comprising a desulfurization catalyst. The distribution of the catalyst in the different zones can be selected so as to maximise the catalytic activity, and thus minimize the volume of catalyst required for a unit of a given capacity operating at fixed operating temperature and pressure, so as to obtain an intensely desulfurized gas oil.
摘要翻译：一种加氢处理瓦斯油的方法包括：在包含脱硫催化剂的第一催化区中进行的第一瓦斯油脱硫步骤; 至少部分消除在第一瓦斯油脱硫步骤结束时形成的硫化氢; 在包含脱硫催化剂的一个或多个催化区中进行一个或多个另外的脱硫步骤。可以选择催化剂在不同区域中的分布，以使催化活性最大化，从而最小化在固定操作温度和压力下操作的给定容量单位所需的催化剂体积，从而获得强烈脱硫瓦斯油。

4. 发明授权

US6007704A Process for the production of catalytic cracking gasoline with a low sulphur content 失效
标题翻译：用于生产硫含量低的催化裂化汽油的方法
公开(公告)号：US6007704A
公开(公告)日：1999-12-28
申请号：US936101
申请日：1997-09-23
申请人： Thierry Chapus , Blaise Didillon , Christian Marcilly , Charles Cameron
发明人： Thierry Chapus , Blaise Didillon , Christian Marcilly , Charles Cameron
IPC分类号： B01J23/42 , B01J23/85 , B01J31/12 , C10G27/00 , C10G29/06 , C10G45/06 , C10G45/10 , C10G45/40 , C10G65/00 , C10G65/06 , C10G67/00 , C10G67/04 , C10G67/12 , C10G67/16
CPC分类号： C10G65/00 , C10G2400/02
摘要： Catalytic cracking gaseolines are treated by: (a) fractionating the raw gasoline cut into two cuts; (b) optional selective diene hydrodenation of the light cut, then mild hydrotreatment and stripping; (c) sweetening the light cut which is conducted before the mild hydrotreatment step by contact with a supported catalyst containing 0.1-1% by weight of palladium, or after the mild hydrotreatment step and which is then an extractive sweetening step, or with a catalyst having an alkaline base optionally incorporated and also an oxidizing agent. The heavy gaseoline fraction is optionally desilphurized in a hydrotreatment unit. The desulpurized and sweetened light gaesoline can be added to the gasoline pool either directly or mixed with the desulphurized heavy gaseoline cut.
摘要翻译：催化裂化球菌是通过以下方式处理的：（a）将原油汽油分馏成两个馏分; （b）轻馏分选择性二烯烃加氢反应，然后轻度加氢处理和汽提; （c）通过与含有0.1-1重量％钯的负载催化剂接触，或在轻度加氢处理步骤之后，然后进行萃取甜化步骤，或用催化剂，使在温和加氢处理步骤之前进行的轻馏分变甜具有任选地并入的碱性碱，还有氧化剂。任选地在加氢处理装置中将沉淀的gaseoline馏分去溶解。脱硫和甜化的光泽石可以直接添加到汽油池中或与脱硫的重质gaseoline切割混合。

5. 发明授权

US08692040B2 Production of vapour-cracking loads with a high yield of the resulting ethylene, propylene and polymers by hydroprocessing of vegetable oils 有权
标题翻译：通过植物油的加氢处理，生成乙烯，丙烯和聚合物的高产率的蒸汽裂解负荷
公开(公告)号：US08692040B2
公开(公告)日：2014-04-08
申请号：US12664132
申请日：2008-06-03
申请人： Quentin Debuisschert , Jean Cosyns , Thierry Chapus , Damien Hudebine
发明人： Quentin Debuisschert , Jean Cosyns , Thierry Chapus , Damien Hudebine
IPC分类号： C07C1/00
CPC分类号： C10G9/36 , C10G3/46 , C10G3/50 , C10G3/54 , C10G45/08 , C10G47/04 , C10G47/06 , C10G69/06 , C10G2300/1003 , C10G2300/1014 , C10G2300/1018 , C10G2300/1044 , C10G2300/1055 , C10G2300/4006 , C10G2300/4012 , C10G2300/4018 , C10G2400/20 , C11C3/123 , C11C3/126 , Y02P30/20 , Y02P30/42
摘要： The invention describes a process for treatment of a feedstock that is obtained from a renewable source that comprises a hydrotreatment stage in the presence of at least one fixed-bed catalyst, whereby said catalyst comprises a hydro-dehydrogenating function and an amorphous substrate, at a temperature of between 50 and 450° C., at a pressure of between 1 MPa and 10 MPa, at an hourly volumetric flow rate of between 0.1 h−1 and 10 h−1, and in the presence of a total quantity of hydrogen that is mixed with the feedstock such that the hydrogen/feedstock ratio is between 50 and 1000 Nm3 of hydrogen/m3 of feedstock, followed by a separation from the hydrotreated effluent that is obtained from stage a) of hydrogen, gases, and at least one liquid hydrocarbon effluent that consists of at least 50% linear n-paraffins, and a steam-cracking of at least one portion of the liquid hydrocarbon effluent that is obtained from stage b).
摘要翻译：本发明描述了一种处理从可再生来源获得的原料的方法，该方法包括在至少一种固定床催化剂存在下的加氢处理阶段，由此所述催化剂包含加氢脱氢功能和非晶基质，温度为50-450℃，压力为1MPa至10MPa，小时体积流速为0.1h-1至10h-1，在总氢存在下，与原料混合使得氢/原料比为50至1000Nm 3的氢/ m3原料，然后与从氢气，气体和至少一种液体的a）段获得的加氢处理流出物分离由至少50％线性正链烷烃组成的碳氢化合物流出物，以及从阶段b）获得的液体烃流出物的至少一部分的蒸汽裂解。

6. 发明授权

US08282815B2 Method of converting feedstocks from renewable sources to good-quality diesel fuel bases using a zeolite catalyst without intermediate gas-liquid separation 有权
标题翻译：使用无中间气液分离的沸石催化剂将来自可再生资源的原料转化为优质柴油燃料基料的方法
公开(公告)号：US08282815B2
公开(公告)日：2012-10-09
申请号：US12490647
申请日：2009-06-24
申请人： Christophe Bouchy , Antoíne Daudin , Emmanuelle Guillon , Nathalie Dupassieux , Thierry Chapus
发明人： Christophe Bouchy , Antoíne Daudin , Emmanuelle Guillon , Nathalie Dupassieux , Thierry Chapus
IPC分类号： C10G35/09 , C10G35/095
CPC分类号： C10G65/043 , C10G3/46 , C10G3/50 , C10G3/54 , C10G45/02 , C10G45/08 , C10G45/64 , C10G2300/1014 , C10G2300/1018 , C10G2300/202 , C10G2300/4006 , C10G2300/4012 , C10G2300/4018 , Y02P30/20
摘要： The invention relates to a method of treating feedstocks from renewable sources without intermediate gas-liquid separation in order to produce diesel fuel bases of excellent quality. The feedstocks used can be raw vegetable oils or such oils that have been previously subjected to a prerefining stage, animal fats, or mixtures of such feedstocks. The invention relates to a method allowing high diesel fuel base yields to be obtained from such feedstocks.
摘要翻译：本发明涉及一种从可再生能源处理原料而不进行中间气液分离的方法，以生产质量优良的柴油燃料基料。所使用的原料可以是先前经受预精制阶段，动物脂肪或这些原料的混合物的生植物油或这种油。本发明涉及允许从这些原料获得高柴油燃料碱产率的方法。

7. 发明授权

US08110091B2 Process for the conversion of feedstocks resulting from renewable sources for producing gas oil fuel bases with a low sulphur content and with an improved cetane number 有权
标题翻译：用于生产低硫含量和十六烷值较高的瓦斯油燃料基的可再生能源转化原料的方法
公开(公告)号：US08110091B2
公开(公告)日：2012-02-07
申请号：US11963231
申请日：2007-12-21
申请人： Thierry Chapus , Karin Marchand
发明人： Thierry Chapus , Karin Marchand
IPC分类号： C10G65/12
CPC分类号： C10G65/12 , C10G3/46 , C10G3/48 , C10G3/50 , C10G3/54 , C10G45/02 , C10G45/08 , C10G2300/1003 , C10G2300/1014 , C10G2300/1018 , C10G2300/1074 , C10G2300/202 , C10G2300/207 , C10G2300/301 , C10G2300/4006 , C10G2300/4012 , C10G2300/4018 , C10G2400/04 , Y02P30/20
摘要： The invention relates to a process for the treatment of heavy petroleum feedstocks in order to produce a gas oil fraction having a sulphur content of less than 50 ppm and generally 10 ppm which comprises the following stages: e) mild hydrocracking in a catalyst fixed bed, f) separation of the hydrogen sulphide, of a distillate cut including a gas oil fraction and of a fraction which is heavier than the gas oil, g) hydrotreating, by contact with at least one catalyst, of at least a portion of the distillate cut obtained in stage b) including the gas oil fraction, as a mixture with a feedstock resulting from a crude or refined renewable source, h) separation of a gas oil cut comprising less than 50 ppm of sulphur. Advantageously, the heavy fraction is sent for catalytic cracking. Preferably, the process is carried out with makeup hydrogen introduced in stage c) and very advantageously all the makeup hydrogen for the process is introduced in stage c). The invention also relates to a plant which can be used for implementing this process.
摘要翻译：本发明涉及一种用于处理重质石油原料的方法，以生产硫含量小于50ppm，通常为10ppm的瓦斯油馏分，其包括以下阶段：e）催化剂固定床中的轻度加氢裂化， f）硫化氢分离，包括粗柴油馏分和比瓦斯油重的馏分馏出物，g）通过与至少一种催化剂接触至少部分馏出物馏分进行加氢处理在步骤b）中获得的，包括粗柴油馏分作为与原油或精制可再生来源产生的原料的混合物，h）分离包含少于50ppm硫的瓦斯油馏分。有利地，将重馏分送入催化裂化。优选地，通过在阶段c）中引入的补充氢来进行该方法，并且非常有利地，用于该方法的所有补充氢在阶段c）中引入。本发明还涉及可用于实施该方法的设备。

8. 发明申请

US20100292518A1 TWO-STEP HYDROTREATMENT OF A FEED DERIVED FROM A RENEWABLE SOURCE USING A FIRST, METALLIC, CATALYST AND A SECOND, SULPHURIZED, CATALYST 失效
标题翻译：使用第一，金属，催化剂和第二种硫化催化剂从可再生来源获得的进料的两步骤加氢
公开(公告)号：US20100292518A1
公开(公告)日：2010-11-18
申请号：US12664136
申请日：2008-06-03
申请人： Quentin Debuisschert , Jean Cosyns , Thierry Chapus , Damien Hudebine
发明人： Quentin Debuisschert , Jean Cosyns , Thierry Chapus , Damien Hudebine
IPC分类号： C07C5/373
CPC分类号： C10G3/42 , C07C1/2078 , C10G3/46 , C10G3/47 , C10G3/48 , C10G3/50 , C10G45/08 , C10G51/02 , C10G2300/1014 , C10G2300/1018 , C10G2300/4018 , C11C3/123 , Y02P30/20
摘要： The invention describes a two-step process for hydrotreatment of a feed derived from a renewable source, comprising: a) a first step, termed a mild pre-hydrogenation step, operating in the presence of a first, metallic, catalyst comprising an active hydrodehydrogenating phase constituted by at least one metal from group VIII and/or at least one metal from group VIB and an amorphous mineral support; and b) a second step, termed the second treatment step, operating in the presence of a second, sulphurized, catalyst comprising an active hydrodehydrogenating phase constituted by at least one non-noble metal from group VIII and/or at least one metal from group VIB and an amorphous mineral support.
摘要翻译：本发明描述了用于加氢处理源自可再生源的进料的两步法，该方法包括：a）第一步骤，称为温和预氢化步骤，在第一金属催化剂存在下操作，其包含活性氢化氢由至少一种来自第VIII族的金属和/或至少一种来自VIB族的金属和无定形矿物载体构成; 和b）称为第二处理步骤的第二步骤，在第二种硫化催化剂存在下操作，该催化剂包含由至少一种来自第VIII族的非贵金属和/或至少一种来自基团的金属构成的活性氢化氢化相 VIB和无定形矿物支持。

9. 发明授权

US07718050B2 Process of mild hydrocracking including a dilution of the feedstock 有权
标题翻译：轻度加氢裂化的方法，包括原料稀释
公开(公告)号：US07718050B2
公开(公告)日：2010-05-18
申请号：US11449867
申请日：2006-06-09
申请人： Christophe Gueret , Thierry Chapus , Damien Hudebine
发明人： Christophe Gueret , Thierry Chapus , Damien Hudebine
IPC分类号： C10G57/00 , B01J8/18
CPC分类号： C10G69/04 , C10G11/18 , C10G47/00
摘要： The invention relates to a process for FCC pretreatment by mild hydrocracking of a hydrocarbon feedstock that comprises a vacuum distillate fraction or a deasphalted oil or else a mixture of these two fractions, said primary feedstock, to produce gas oil and an effluent having an initial boiling point of more than 320° C., said effluent (FCC feedstock) then being subjected to a catalytic cracking, process in which at least 85% by weight of said primary feedstock ends above 375° C. and at least 95% by weight of said primary feedstock ends below 650° C., whereby the mild hydrocracking is performed under an absolute pressure of 2 to 12 MPa and at a temperature of between 300 and 500° C., characterized in that the hydrocarbon feedstock also comprises a lighter hydrocarbon fraction, a so-called secondary feedstock, of which at least 50% by weight ends below 375° C. and at least 80% ends above 200° C.
摘要翻译：本发明涉及通过烃原料的轻度加氢裂化来进行FCC预处理的方法，所述烃原料包括真空蒸馏馏分或脱沥青油，或者所述主要原料的这两个馏分的混合物，以产生瓦斯油和具有初始沸点的流出物所述流出物（FCC原料）然后进行催化裂化，其中至少85重量％的所述主要原料在375℃以上终止，并且至少95重量％所述主要原料终止于650℃以下，由此在2至12MPa的绝对压力和300至500℃的温度下进行轻度加氢裂化，其特征在于，烃原料还包含较轻的烃馏分，所谓的二次原料，其中至少50重量％终止于375℃以下且至少80％在200℃以上结束。

10. 发明申请

US20090326290A1 METHOD OF CONVERTING FEEDSTOCKS FROM RENEWABLE SOURCES TO GOOD-QUALITY DIESEL FUEL BASES USING A ZEOLITE CATALYST WITHOUT INTERMEDIATE GAS-LIQUID SEPARATION 有权
标题翻译：使用不具有中间气液分离的沸石催化剂将可再生来源的原料转化为优质柴油燃料的方法
公开(公告)号：US20090326290A1
公开(公告)日：2009-12-31
申请号：US12490647
申请日：2009-06-24
申请人： Christophe Bouchy , Antoine Daudin , Emmanuelle Guillon , Nathalie Dupassieux , Thierry Chapus
发明人： Christophe Bouchy , Antoine Daudin , Emmanuelle Guillon , Nathalie Dupassieux , Thierry Chapus
IPC分类号： C07C5/13
CPC分类号： C10G65/043 , C10G3/46 , C10G3/50 , C10G3/54 , C10G45/02 , C10G45/08 , C10G45/64 , C10G2300/1014 , C10G2300/1018 , C10G2300/202 , C10G2300/4006 , C10G2300/4012 , C10G2300/4018 , Y02P30/20
摘要： The invention relates to a method of treating feedstocks from renewable sources without intermediate gas-liquid separation in order to produce diesel fuel bases of excellent quality. The feedstocks used can be raw vegetable oils or such oils that have been previously subjected to a prerefining stage, animal fats, or mixtures of such feedstocks. The invention relates to a method allowing high diesel fuel base yields to be obtained from such feedstocks.
摘要翻译：本发明涉及一种从可再生能源处理原料而不进行中间气液分离的方法，以生产质量优良的柴油燃料基料。所使用的原料可以是先前经受预精制阶段，动物脂肪或这些原料的混合物的生植物油或这种油。本发明涉及允许从这些原料获得高柴油燃料碱产率的方法。

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