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1. 发明申请

US20110237817A1 PROCESS FOR THE PREPARATION OF ACYLATED SECONDARY ALCOHOL ALKOXYLATES AND SECONDARY ALCOHOL ALKOXYLATES 失效
标题翻译：酰化次级醇酸烷基酯和次级醇酸烷基酯的制备方法
公开(公告)号：US20110237817A1
公开(公告)日：2011-09-29
申请号：US13126200
申请日：2009-10-28
申请人： Harry Van Der Heijden , Renata Helena Van Der Made , Jan Hermen Hendrik Meurs , Quoc An On , Arie Van Zon
发明人： Harry Van Der Heijden , Renata Helena Van Der Made , Jan Hermen Hendrik Meurs , Quoc An On , Arie Van Zon
IPC分类号： C07C303/24 , C07C67/29
CPC分类号： C07C67/04 , C07C41/26 , C07C67/26 , C07C303/24 , C08G65/2615 , C08G65/2648 , C08G65/2675 , C08G65/2678 , C08G65/269 , C07C305/10 , C07C69/14 , C07C43/11
摘要： A process for the preparation of acylated secondary alcohol alkoxylates anda process for making secondary alcohol alkoxy sulfates comprising the steps of:preparing secondary alcohol alkoxylates by the afore-mentioned process; andsulfating the secondary alcohol alkoxylates is described.
摘要翻译：一种制备酰化仲醇烷氧基化物的方法和制备仲醇烷氧基硫酸盐的方法，包括以下步骤：通过上述方法制备仲醇烷氧基化物; 并描述了仲醇烷氧基化物的硫酸化。

2. 发明授权

US06984755B2 Processes for the preparation of a carboxylic anhydride and use of the carboxylic anhydride as an acylation agent 失效
标题翻译：用于制备羧酸酐的方法和使用羧酸酐作为酰化剂
公开(公告)号：US06984755B2
公开(公告)日：2006-01-10
申请号：US10504913
申请日：2003-02-18
申请人： Eit Drent , Renata Helena Van Der Made , Robert Ian Pugh
发明人： Eit Drent , Renata Helena Van Der Made , Robert Ian Pugh
IPC分类号： C07C51/56
CPC分类号： C07C67/08 , C07C51/56 , C07C67/38 , C07C53/122 , C07C69/017 , C07C69/24
摘要： A process for the preparation of an carboxylic anhydride by reaction of an ethylenically unsaturated compound with carbon monoxide and an carboxylic acid in the presence of a catalyst involving: a) a source of a group VIII metal; b) a bidentate diphosphine of formula I, wherein R1 represents a bivalent radical that together with the phosphorus atom to which it is attached is an optionally substituted 2-phospha-tricyclo[3.3.1.1 {3,7}]-decyl group or a derivative thereof in which one or more of the carbon atoms are replaced by heteroatoms (“2-PA” group); wherein R2 and R3 independently represent univalent radicals of up to 20 atoms or jointly form a bivalent radical of up to 20 atoms; and wherein R represents a bivalent organic bridging group; and, c) a complexing anion; wherein the complexing anion is the anion of the carboxylic acid. A process wherein the carboxylic acid is prepared in-situ and use of the carboxylic anhydride as an acylation agent.
摘要翻译：一种通过烯属不饱和化合物与一氧化碳和羧酸在催化剂存在下反应来制备羧酸酐的方法，所述催化剂包括：a）VIII族金属源; b）式I的二齿二膦，其中R 1表示与连接的磷原子一起为任选取代的2-磷杂三环[3.3.1.1 {3， 7}] - 癸基或其衍生物，其中一个或多个碳原子被杂原子（“2-PA”基团）代替）; 其中R 2和R 3独立地表示至多20个原子的一价基团或共同形成至多20个原子的二价基团; 并且其中R表示二价有机桥基; 和c）络合阴离子; 其中络合阴离子是羧酸的阴离子。其中羧酸原位制备并使用羧酸酐作为酰化剂的方法。

3. 发明授权

US07202193B2 Process for the carbonylation of an ethylenically unsaturated compound and catalyst therefore 有权
标题翻译：因此烯属不饱和化合物和催化剂的羰基化方法
公开(公告)号：US07202193B2
公开(公告)日：2007-04-10
申请号：US10505019
申请日：2003-02-18
申请人： Eit Drent , Renata Helena Van Der Made , Robert Ian Pugh , Paul Gerard Pringle
发明人： Eit Drent , Renata Helena Van Der Made , Robert Ian Pugh , Paul Gerard Pringle
IPC分类号： B01J27/185 , C07C51/14
CPC分类号： B01J31/2485 , B01J31/28 , B01J2231/321 , B01J2531/80 , B01J2531/822 , B01J2531/824 , B01J2531/828 , B01J2531/847 , C07C51/14 , C07F9/65683 , C07C53/122
摘要： A process for the carbonylation of an ethylenically unsaturated compound with carbon monoxide and a co-reactant. The carbonylation reaction is carried out in the presence of a novel catalyst involving: a) a source of a group VIII metal; b)a bidentate diphosphine of formula I, wherein R1 represents a bivalent radical that together with the phosphorus atom to which it is attached is an optionally substituted 2-phospha-tricyclo[3.3.1.1{3,7}]- decyl group or a derivative thereof in which one or more of the carbon atoms are replaced by heteroatoms (“2-PA” group); wherein R2 and R3 independently represent univalent radicals of up to 20 atoms or jointly form a bivalent radical of up to 20 atoms; and wherein A1 and A2 independently represent optionally substituted alkylene groups and R represents an optionally substituted aromatic group; and, c) a source of anions.
摘要翻译：用一氧化碳和共反应物羰基化烯属不饱和化合物的方法。羰基化反应在新催化剂存在下进行

4. 发明授权

US07057082B2 Process for the telomerization of a conjugated diene, catalyst and bidentate ligand useful therein 失效
标题翻译：用于其中的共轭二烯，催化剂和二齿配体的调聚方法
公开(公告)号：US07057082B2
公开(公告)日：2006-06-06
申请号：US10882932
申请日：2004-07-01
申请人： Eit Drent , Michael Rolf Eberhard , Paul Gerald Pringle , Renata Helena van der Made
发明人： Eit Drent , Michael Rolf Eberhard , Paul Gerald Pringle , Renata Helena van der Made
IPC分类号： C07C2/36
CPC分类号： B01J31/248 , B01J23/44 , B01J31/1895 , B01J31/24 , B01J2231/20 , B01J2531/80 , B01J2531/824 , C07C2/36 , C07C2/406 , C07C41/06 , C07C253/30 , C07C2531/24 , C07C2531/28 , C07D201/08 , C07F9/5027 , C07F9/65683 , C07C255/19 , C07C11/12 , C07C43/15
摘要： Process for the telomerization of a conjugated diene,wherein the conjugated diene is reacted with a compound containing an active hydrogen atom and having a formula R′—H in the presence of a telomerization catalyst based on: (a) a source of group VIII metal, (b) a bidentate ligand wherein the bidentate ligand has the general formula I R1R2M1—R—M2R3R4 (I) wherein M1 and M2 are independently P, As or Sb; R1, R2, R3 and R4 independently represent a monovalent aliphatic group; or R1, R2 and M1 together and/or R3, R4 and M2 together independently represent an optionally substituted aliphatic cyclic group with at least 5 ring atoms, of which one is the M1 or M2 atom, respectively; R represents a bivalent organic bridging group; and novel bidentate diphosphines which can be used in this process.
摘要翻译：共轭二烯的调聚方法，其中在调聚催化剂的存在下，共轭二烯与含有活性氢原子的化合物反应并具有式R'-H，其基于：（a）VIII族金属源，（b）二齿配位体，其中二齿配位体具有通式I <βin-line-formula description =“In-line Formulas”end =“lead”？> R＆lt; （1）＆lt; 2＆gt; 1＆gt; -RM＆lt; 2＆gt; line-formula description =“In-line Formulas”end =“tail”？>其中M 1和M 2独立地是P，As或Sb; R 1，R 2，R 3和R 4独立地表示一价脂族基团; 或R 1，R 2和M 1一起和/或R 3，R 4， / SUP＆amp;和M＆gt; 2共同独立地表示具有至少5个环原子的任选取代的脂族环基，其中一个是M 1或M 2， / SUP>原子; R表示二价有机桥基; 和可用于该方法的新型二齿二膦。

5. 发明授权

US06794553B2 Process for the telomerization of a conjugated diene, catalyst and bidentate ligand useful therein 失效
标题翻译：用于其中的共轭二烯，催化剂和二齿配体的调聚方法
公开(公告)号：US06794553B2
公开(公告)日：2004-09-21
申请号：US10287731
申请日：2002-11-04
申请人： Eit Drent , Michael Rolf Eberhard , Paul Gerald Pringle , Renata Helena van der Made
发明人： Eit Drent , Michael Rolf Eberhard , Paul Gerald Pringle , Renata Helena van der Made
IPC分类号： C07C132
CPC分类号： B01J31/248 , B01J23/44 , B01J31/1895 , B01J31/24 , B01J2231/20 , B01J2531/80 , B01J2531/824 , C07C2/36 , C07C2/406 , C07C41/06 , C07C253/30 , C07C2531/24 , C07C2531/28 , C07D201/08 , C07F9/5027 , C07F9/65683 , C07C255/19 , C07C11/12 , C07C43/15
摘要： Process for the telomerization of a conjugated diene, wherein the conjugated diene is reacted with a compound containing an active hydrogen atom and having a formula R′—H in the presence of a telomerization catalyst based on: (a) a source of group VIII metal, (b) a bidentate ligand wherein the bidentate ligand has the general formula I R1R2M1—R—M2R3R4 (I) wherein M1 and M2 are independently P, As or Sb; R1, R2, R3 and R4 independently represent a monovalent aliphatic group; or R1, R2 and M1 together and/or R3, R4 and M2 together independently represent an optionally substituted aliphatic cyclic group with at least 5 ring atoms, of which one is the M1 or M2 atom, respectively; R represents a bivalent organic bridging group; and novel bidentate diphosphines which can be used in this process.
摘要翻译：共轭二烯的调聚方法，其中在调聚催化剂的存在下，共轭二烯与含有活性氢原子的化合物反应并具有式R'-H，其基于：（a）VIII族金属源，（b）二齿配位体中的二齿配位体具有通式I，其中M 1和M 2独立地为P，As或Sb; R 1，R 2，R 3和R 4 >独立地表示一价脂族基团;或R 1，R 2和M 1一起和/或R 3，R 4和M 2一起独立地表示任选取代的脂族环基具有至少5个环原子，其中一个是M 1或M 2原子; R代表二价有机桥基; 和可用于该方法的新型二齿二膦。

6. 发明授权

US08664423B2 Process for the preparation of acylated secondary alcohol alkoxylates and secondary alcohol alkoxylates 失效
标题翻译：酰化仲醇烷氧基化物和仲醇烷氧基化物的制备方法
公开(公告)号：US08664423B2
公开(公告)日：2014-03-04
申请号：US13126200
申请日：2009-10-28
申请人： Harry Van Der Heijden , Renata Helena Van Der Made , Jan Hermen Hendrik Meurs , Quoc An On , Arie Van Zon
发明人： Harry Van Der Heijden , Renata Helena Van Der Made , Jan Hermen Hendrik Meurs , Quoc An On , Arie Van Zon
IPC分类号： C07C41/26 , C07C67/04 , C07C67/26 , C07C303/24 , C07C69/003 , C07C305/10 , C07C69/14 , C07C69/16 , C07C67/29
CPC分类号： C07C67/04 , C07C41/26 , C07C67/26 , C07C303/24 , C08G65/2615 , C08G65/2648 , C08G65/2675 , C08G65/2678 , C08G65/269 , C07C305/10 , C07C69/14 , C07C43/11
摘要： A process for the preparation of acylated secondary alcohol alkoxylates and a process for making secondary alcohol alkoxy sulfates comprising the steps of:— preparing secondary alcohol alkoxylates by the afore-mentioned process; and sulfating the secondary alcohol alkoxylates is described.
摘要翻译：一种制备酰化仲醇烷氧基化物的方法和制备仲醇烷氧基硫酸盐的方法，包括以下步骤： - 通过上述方法制备仲醇烷氧基化物; 并描述了仲醇烷氧基化物的硫酸化。

7. 发明授权

US07135542B2 Bidentate ligands for the carbonylation of unsaturated compounds 失效
标题翻译：用于不饱和化合物羰基化的二齿配位体
公开(公告)号：US07135542B2
公开(公告)日：2006-11-14
申请号：US10494901
申请日：2002-11-05
申请人： Eit Drent , Roelof Van Ginkel , Renata Helena Van Der Made
发明人： Eit Drent , Roelof Van Ginkel , Renata Helena Van Der Made
IPC分类号： C08G69/08
CPC分类号： B01J31/1895 , B01J23/44 , B01J31/24 , B01J31/2414 , B01J2231/321 , B01J2531/80 , B01J2531/824 , C07C2/406 , C07C67/38 , C07C253/30 , C07C2531/24 , C07C2531/28 , C07D201/08 , C07F9/5027 , C07C255/19 , C07C69/24
摘要： Bidentate ligand of formula (I), R1R2M1-R-M2R3R4 wherein M1 and M2 each indenpendently represent P, As or Sb; R1, R2, R3 and R4 each independently represent the same or a different optionally substituted organic group and at least one of R1, R2, R3 and R4 contains a tertiary carbon atom through which the group is linked to M1 or M2; and R represents a bridging group based on a trimethylene group connecting M1 and M2 of which the middle carbon atom is double bonded to a non-metal element chosen from group 14, 15 or 16 of the periodic table of elements. Catalyst comprising this bidentate ligand and carbonylation process n which this catalyst is used.
摘要翻译：式（I）的二齿配体，R 1，R 2，R 2，...，R 2，R 3，其中M 1和M 2各自独立地表示P，As或Sb; R 1，R 2，R 3和R 4各自独立地表示相同或不同的任选取代的有机物并且R 1，R 2，R 3和R 4中的至少一个含有叔碳原子该基团通过其与M 1或M 2连接; 并且R表示基于连接M 1和M 2的三亚甲基的桥连基团，其中中碳原子与选自第14族的非金属元素双键结合，元素周期表中的15或16个。包含该二齿配体和使用该催化剂的羰基化方法n的催化剂。

8. 发明授权

US07491859B2 Process for the telomerization of a conjugated diene, catalyst and bidentate ligand useful therein 失效
标题翻译：用于其中的共轭二烯，催化剂和二齿配体的调聚方法
公开(公告)号：US07491859B2
公开(公告)日：2009-02-17
申请号：US11299101
申请日：2005-12-09
申请人： Eit Drent , Michael Rolf Eberhard , Paul Gerald Pringle , Renata Helena van der Made
发明人： Eit Drent , Michael Rolf Eberhard , Paul Gerald Pringle , Renata Helena van der Made
IPC分类号： B01J31/18 , B01J31/22 , C07C2/32 , C07C2/36
CPC分类号： B01J31/248 , B01J23/44 , B01J31/1895 , B01J31/24 , B01J2231/20 , B01J2531/80 , B01J2531/824 , C07C2/36 , C07C2/406 , C07C41/06 , C07C253/30 , C07C2531/24 , C07C2531/28 , C07D201/08 , C07F9/5027 , C07F9/65683 , C07C255/19 , C07C11/12 , C07C43/15
摘要： Process for the telomerization of a conjugated diene,wherein the conjugated diene is reacted with a compound containing an active hydrogen atom and having a formula R′—H in the presence of a telomerization catalyst based on:(a) a source of group VIII metal,(b) a bidentate ligandwherein the bidentate ligand has the general formula I R1R2M1-R-M2R3R4 (I) wherein M1 and M2 are independently P, As or Sb; R1, R2, R3 and R4 independently represent a monovalent aliphatic group; or R1, R2 and M1 together and/or R3, R4 and M2 together independently represent an optionally substituted aliphatic cyclic group with at least 5 ring atoms, of which one is the M1 or M2 atom, respectively; R represents a bivalent organic bridging group; and novel bidentate diphosphines which can be used in this process.
摘要翻译：共轭二烯的调聚方法，其中在调聚催化剂的存在下，共轭二烯与含有活性氢原子的化合物反应并具有式R'-H，其基于：（a）VIII族金属源，（b）双齿配体，其中二齿配体具有通式I <βin-line-formula description =“In-line Formulas”end =“lead”→> R1R2M1-R-M2R3R4（I） line-formula description =“In-line Formulas”end =“tail”？>其中M1和M2独立地为P，As或Sb; R1，R2，R3和R4独立地表示一价脂族基团; 或R 1，R 2和M 1一起和/或R 3，R 4和M 2一起独立地表示任选取代的具有至少5个环原子的脂族环基，其中一个是分别为M1或M2原子; R表示二价有机桥基; 和可用于该方法的新型二齿二膦。

9. 发明授权

US07098369B2 Process for the production of primary alcohols 失效
标题翻译：制备伯醇的方法
公开(公告)号：US07098369B2
公开(公告)日：2006-08-29
申请号：US10669916
申请日：2003-09-24
申请人： Eit Drent , Renata Helena Van Der Made
发明人： Eit Drent , Renata Helena Van Der Made
IPC分类号： C07C29/145 , C07C29/16
CPC分类号： C07C29/16 , B01J31/0215 , B01J31/24 , C07C31/125
摘要： A process for producing primary alcohols from secondary alcohols and/or tertiary alcohols and/or ketones, wherein the process comprises reacting a compound selected from a secondary alcohol, a tertiary alcohol, a ketone, or mixtures thereof, with carbon monoxide and hydrogen in the presence of a catalyst based on: (i) a source of Group VIII metal, (ii) a bidentate ligand having the general formula (I): R1R2M1-R-M2R3R4 (I) wherein M1 and M2 are independently P, As or Sb; R1 and R2 together represent a bivalent substituted or unsubstituted cyclic aliphatic group whereby the two free valencies are linked to M1; R3 and R4 independently represent a substituted or unsubstituted hydrocarbyl group, or together represent a bivalent or non-substituted cyclic group whereby the two free valencies are linked to M2; and R represents a bivalent aliphatic bridging group; and (iii) an acid having a pKa of 3 or less which is in excess over the Group VIII metal.
摘要翻译：由仲醇和/或叔醇和/或酮生产伯醇的方法，其中该方法包括使选自仲醇，叔醇，酮或其混合物的化合物与一氧化碳和氢气在基于以下的催化剂的存在：（i）第VIII族金属源，（ii）具有通式（I）的二齿配体：<？在线公式描述=“在线式”末端=“铅 “”> R“1”2“2”“”“”“”“”“”“”“”“”“”“”“”“”“”“”“”“”“”“”“”“”“ （I）<？in-line-formula description =“In-line Formulas”end =“tail”？>其中M 1和M 2 < / SUP>独立为P，As或Sb; R 1和R 2一起代表二价取代或未取代的环状脂族基，其中两个自由价与M 1连接; R 3和R 4独立地表示取代或未取代的烃基，或一起表示二价或未取代的环状基团，由此两个自由价与M ^{2 ; R表示二价脂肪族桥基; 和（iii）具有超过第Ⅷ族金属的pK _{a <3的3或更小的酸。}}

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